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At least 1,063 records · Page 59

All sources NASA NTRS DOE OSTI

DOE OSTI2023

Analysis and mitigation of an oscillating background on hybrid complementary metal-oxide semiconductor (hCMOS) imaging sensors at the National Ignition Facility

Nanosecond-gated hybrid complementary metal-oxide semiconductor imaging sensors are a powerful tool for temporally gated and spatially resolved measurements in high energy density science, including inertial confinement fusion, and in laser diagnostics. However, a significant oscillating background excited by photocurrent has been observed in image sequences during testing and in experiments at the National Ignition Facility (NIF). Characterization measurements and simulation results are used to explain the oscillations as the convolution of the pixel-level sensor response with a sensor-wide RLC circuit ringing. Finally, data correction techniques are discussed for NIF diagnostics, and for diagnostics where these techniques cannot be used, a proof-of-principle image correction algorithm is presented.

42 ENGINEERING↗

DOE OSTI2025

Thermal energy transport in laser-driven high x-ray conversion efficiency metallic silver nanowire foams

Here, we report on record brightness from Ag x-ray emission obtained using a novel laser-produced plasma source. The reported K-shell conversion efficiency of nearly 1% with a radiant energy of ≈ 0.6 kJ/sr from Ag ions is the highest presently recorded and is about twofold greater than more conventional metal-lined cavity targets. He-like Ag ions are the dominant radiators at ≈ 22.7 keV, which contrast the x-ray sources from other pulse power facilities that produce K-shell x-rays from Auger processes in near-neutral ions driven by the nonthermal hot electrons produced in the Z-pinch implosion. The reported x-ray emission was produced from a 4-mm-diameter, 4-mm-long underdense silver nanowire target at 10⁢ mg/⁢cm 3 . The National Ignition Facility laser beams deposited ≈ 1000 kJ of 3ω light into the target with a ≈ 400 TW, 2.5 ns square pulse. Finally, we show via comparisons of data with radiation-hydrodynamics simulations that flux-limited classical thermal energy transport models are inadequate in correctly modeling the behavior of these non-local thermodynamic equilibrium plasmas.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2021

Measurement of chromatic aberrations using phase retrieval

We explore the feasibility of measuring chromatic aberrations using a technique based on phase retrieval, primarily for the purpose of diagnostics on the OMEGA EP laser. A computational model and optimization strategy is described, issues of numerical efficiency are addressed, and the potential limitations of the method are studied using mathematical analysis and Monte Carlo simulations. As a result, the algorithm performs well in simulation and yields encouraging results in a small-scale laboratory experiment.

97 MATHEMATICS AND COMPUTING↗

DOE OSTI2023

Parallel Simulation of Beam Dynamics in Particle Accelerators [Slides]

Particle accelerators are among the most versatile and important tools of scientific discovery. The Nation's accelerators are responsible for a wealth of advances in materials science, chemistry, the biosciences, particle physics, and nuclear physics. They also have important applications to national security, the environment, energy, medicine, and on the quality of people's lives. LANL has a long history of making pioneering contributions to Accelerator Science including key contributions to the field of Computational Accelerator Physics. These include the development of early beam dynamics codes with space charge (such as PARMILA and PARMELA), the development of rf cavity codes and magnet codes (including Poisson and Superfish), and the development and distribution of codes to the accelerator community through the Los Alamos Accelerator Code Group. LANL researchers also helped pioneer the development of massively parallel space-charge codes. In project t22_accelsim we have moved beyond electrostatic models of collective effects (i.e., solving the Poisson equation in the bunch frame) to fully electromagnetic models based on the Lienard-Wiechert formalism. This approach enables the large-scale simulation of radiation production and collective effects in high brightness electron beams. This is highly relevant to LANL given its future goal of developing an X-ray Free Electron Laser (XFEL). It also directly impacts a LANL LDRD project to develop an undulator-based non-invasive beam profile monitor for beams created in laser-plasma accelerator systems.

43 PARTICLE ACCELERATORS↗

DOE OSTI2020

Modeling Time-Dependent Surrogates of Additive-Manufactured Nuclear Fuels Processes

Additive manufacturing (AM) technology is being increasingly adopted in a wide variety of application areas for its ability to rapidly produce, prototype, and customize designs. Recently, a hybrid AM technique was successfully developed at Idaho National Laboratory (INL) to manufacture nuclear fuels [1]. Despite the advantages, this AM technique needs optimization due to defects from a highly complex melting and sintering process. The complex metallurgical phenomena during AM processes are strongly related to parameters such as applied laser power, traveling speed, and scan style, which could lead to differences in density, residual stress, crystallographic texture, and mechanical properties. In addition, stochastic variations in laser energy interaction and associated multiscale/multiphysics phenomena cause variations in microstructure evolution and mechanical properties. Currently, researchers at INL are focusing on developing a comprehensive modeling framework, leveraging INL’s simulation tools MOOSE/MARMOT/BISON/RAVEN [2-4] to describe all steps of this AM process across multiple length scales. Although this advanced framework plays a critical role in enabling enhancements to traditional trial and error approaches for design and optimization of nuclear fuel materials, it remains computationally intense, limiting its use in sensitivity and optimization analysis. In this case, an accurate and inexpensive surrogate becomes an effective tool for providing a tractable approximation of the underlying underline physics. Surrogate models generally not based on the physics of a system are purely mathematical models used to capture the relationships between specific system inputs and outputs. Popular approaches, including neural networks [5], response surfaces [6], and subspace-based reduced order models [7], have been applied to a wide range of disciplines, such as nuclear reactor design, aerospace design and automotive design. In this summary, we employ advanced time-dependent surrogate models such as high-dimensional model representation (HDMR) [8] and physics-informed deep neural network (PINNs) [9] to accelerate the design and optimization of AM process.

42 ENGINEERING↗

DOE OSTI2023

Optimal gas cooling with minimal aero-opticaldistortion for next generation high-average-power lasers (Progress report, Year 2)

Next-generation lasers that combine high-peak-power ultrashort pulses with high repetition rates have the potential to efficiently deliver the high-average-power outputs required for inertial fusion energy generation, laser-based particle acceleration, and to generate compact secondary x- and 𝛾-ray radiation sources, among others. The combination of long gain length with high surface-to-volume ratio to remove residual heat makes gas-cooled multi-slab amplifier heads an inherently aperture- and average power scalable technology that enables this new class of solid-state lasers, and their thermal management becomes the most pressing technical challenge. As the index-of refraction depends on the gas density, heat removal from the slab surfaces unavoidably entails scattering of propagated light from regions of high temperature fluctuations. The requirement to maximize convective heat extraction from the gain medium under the constraint of minimum optical aberration of the beam renders amplifier slab cooling a technological challenge at the intersection of aero-optics, fluid-mechanics and heat transfer. The goal of this research is to leverage computational fluid dynamics and aero optics simulations of different levels of fidelity to devise a numerical modeling and optimization framework for gas-cooled multi-slab amplifiers. The project will be conducted in close collaboration with the Advanced Photon Technologies Group at Lawrence Livermore National Laboratory, where a gas-cooled test stand for laser materials and thermal management structures will be developed and installed. The final goal of the collaborative effort is to manufacture and benchmark a physical prototype of an numerically optimized amplifier head design. Measurement data on solid-state and thermo-optical distortions will be used for the validation of the numerical models. The key technical challenge in this multi-objective design problem is that of balancing optimal heat removal with minimal optical distortion. To facilitate computationally efficient design optimization and, at the same time, deepen our basic understanding of the interaction of light with turbulence, a complementary study that combines high and low-fidelity flow simulations and aero-optical models is proposed. Along the lines of these two objectives and solution strategies, the project is organized into two thrusts.

42 ENGINEERING↗

DOE OSTI2020

A new field solver for modeling of relativistic particle-laser interactions using the particle-in-cell algorithm

A customized finite-difference field solver for the particle-in-cell (PIC) algorithm that provides higher fidelity for wave-particle interactions in intense electromagnetic waves is presented. In many problems of interest, particles with relativistic energies interact with intense electromagnetic fields that have phase velocities near the speed of light. Numerical errors can arise due to (1) dispersion errors in the phase velocity of the wave, (2) the staggering in time between the electric and magnetic fields and between particle velocity and position and (3) errors in the time derivative in the momentum advance. Errors of the first two kinds are analyzed in detail. It is shown that by using field solvers with different -space operators in Faraday’s and Ampere’s law, the dispersion errors and magnetic field time-staggering errors in the particle pusher can be simultaneously removed for electromagnetic waves moving primarily in a specific direction. Here, the new algorithm was implemented into Osiris by using customized higher-order finite-difference operators. Schemes using the proposed solver in combination with different particle pushers are compared through PIC simulation. It is shown that the use of the new algorithm, together with an analytic particle pusher (assuming constant fields over a time step), can lead to accurate modeling of the motion of a single electron in an intense laser field with normalized vector potentials, eA / mc 2 , exceeding for typical cell sizes and time steps.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2020

Origin and effect of film sub-stoichiometry on ultraviolet, ns-laser damage resistance of hafnia single layers

Understanding the origin of laser damage-prone precursors in high index materials such as hafnia holds the key to the development of laser damage-resistant multilayer dielectric coated optics for high power and energy laser systems. In this study, we investigate the source of sub-stoichiometry, a potent laser damage precursor, in hafnia films produced by an ion beam sputtering (IBS) deposition method and the effect of such defects on the film performance upon ns ultraviolet (UV) laser (8 ns, 355 nm) exposure. Chemical analysis of data obtained via Rutherford backscattering spectroscopy (RBS) suggests that hafnia films deposited at two different planetary locations from the same deposition run exhibit anisotropic and location-dependent stoichiometries. While the oxygen-to-hafnium ratio is at the stoichiometric value of 2 for the hafnia film at the edge location, the ratio is significantly deviated and is 1.7 for that deposited at the planetary center. The sub-stoichiometric hafnia films display a much lower 1-on-1 damage onset at 1.6 ± 0.2 J/cm 2 compared to 2.3 ± 0.2 J/cm 2 in a stoichiometric film. The low damage performance films also have an over three times higher damage density at fluences above initiation. Coupled with Monte Carlo simulations, we reveal that sub-stoichiometry is primarily attributed to preferential removal of oxygen during film deposition by the bombardment of energetic reflected argon neutrals. The resulting oxygen deficiencies create the sub-bandgap states which facilitate the strong laser energy coupling and reduce the resistance to laser-induced damage in the hafnia single layer films.

36 MATERIALS SCIENCE↗

DOE OSTI2022

Extreme variation in fatigue: Fatigue life prediction and dependence on build volume location in laser powder bed fusion of 17-4 stainless steel

Laser powder bed fusion (LPBF), a metal additive manufacturing technology, is well-suited for design optimization but fatigue life is limited by manufacturing defects. In this work, 17-4 stainless steel components were manufactured in densely populated build volumes, simulating at-scale LPBF production. Tests revealed extreme variability in fatigue life data, analyzed via rigorous statistical tools. The El-Haddad model, modified for finite-life, enabled defect-based life prediction. Specimen location within the build volume correlated to life, which was heteroscedastic. Investigating defect concentration over the build volume explained typical life and scatter. Finally, these findings argue for qualification approaches which acknowledge high material lot variability.

36 MATERIALS SCIENCE↗

DOE OSTI2023

Non-thermal electron acceleration from magnetically driven reconnection in a laboratory plasma

Magnetic reconnection rapidly converts magnetic energy into some combination of plasma flow energy, thermal energy and non-thermal energetic particles. Various reconnection acceleration mechanisms have been theoretically proposed and numerically studied in different collisionless and low-β environments, where β refers to the plasma-to-magnetic pressure ratio. These mechanisms include Fermi acceleration, betatron acceleration, parallel electric field acceleration along magnetic fields and direct acceleration by the reconnection electric field. However, none of them have been experimentally confirmed, as the direct observation of non-thermal particle acceleration in laboratory experiments has been difficult due to short Debye lengths for in situ measurements and short mean free paths for ex situ measurements. Here we report the direct measurement of accelerated non-thermal electrons from magnetically driven reconnection at low β in experiments using a laser-powered capacitor coil platform. We use kilojoule lasers to drive parallel currents to reconnect megagauss-level magnetic fields in a quasi-axisymmetric geometry. The angular dependence of the measured electron energy spectrum and the resulting accelerated energies, supported by particle-in-cell simulations, indicate that the mechanism of direct electric field acceleration by the out-of-plane reconnection electric field is at work. Scaled energies using this mechanism show direct relevance to astrophysical observations.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2026

Structure of Self-Generated Magnetic Fields in Laser-Solid Interaction from Proton Tomography

Self-generated magnetic fields in laser-solid interactions are experimentally characterized to reveal the 3D location and local field strength, rather than path-integrated quantities, using multi-view proton radiography and tomographic inversion. We infer magnetic fields that extend several millimeters off the target into the hot, rarefied corona, sufficient to strongly magnetize the plasma (Ω e τ e ≫ 1). The data are compared to MHD simulations incorporating recent improvements in modeling magnetic field generation and transport; the volume-averaged coronal field strength and magnetic flux agree to within 25% using a model with magnetic re-localization of transport, although the near-target morphology is not reproduced. This work demonstrates tomographic proton radiography as a valuable tool for investigating magnetic fields in laser-produced plasmas.

High-energy-density plasmas↗

DOE OSTI2024

Diamond under extremes

Diamond is, by virtue of the covalent bonding between atoms and the very strong carbon to carbon bonds, the hardest natural material. It has been a fascinating material since its discovery, first as a decorative gem and more recently, for its numerous industrial uses because of its extreme hardness, elastic modulus, and optical transparency. In recent years, it has become a preferred ablator for laser shock experiments, and this has led to its choice as the capsule material for fusion experiments at the National Ignition Facility. Further, this review covers both experimental and computational (including machine learning) advancements in research on diamond subjected extreme conditions of temperature and pressure. The synergy between shock and ramp loading experiments and atomic level simulations is proving to be powerful in advancing our understanding of diamond under extremes.

36 MATERIALS SCIENCE↗

DOE OSTI2021

Pulse width dependence of magnetic field generation using laser-powered capacitor coils

Megagauss magnetic fields were generated by a current flowing through a U-shaped coil connecting two parallel copper foils. Two kJ-class lasers at various pulse widths from 2 ns to 9.9 ns passed through holes in the front foil and were focused on the back foil with an intensity of ~1.7×10 16 W/cm 2 . The coil current and resulting magnetic fields were characterized using ultrafast proton radiography, timed at the end of the laser pulses. Additionally, the measurements show that magnetic field strength decays with increasing laser pulse width. A lumped-circuit model was developed and showed consistency with the experimental measurements, demonstrating an ion shorting effect: as the ion current neutralizes the electron current contribution to interplate voltage, the coil current peaks on a timescale close to the ion transit time t i = d/v ion . FLASH simulations of the coil current are performed, and the calculated resistance values are used to constrain ion speed as a function of hot electron temperature.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2022

Direct Measurement of the Return Current Instability in a Laser-Produced Plasma

Measurements were made of the return current instability growth rate, demonstrating its concurrence with nonlocal transport. Thomson scattering was used to measure a maximum growth rate of 5.1 × 10 9 Hz, which was 3 times less than classical Spitzer-Härm theory predicts. Here, the measured plasma conditions indicate the heat flux was nonlocal, and Vlasov–Fokker-Planck simulations that account for nonlocality reproduce the measured growth rates. Furthermore, the threshold for the return current instability was measured (δ T = 0.017 ± 0.002) to be in good agreement with previous theoretical models.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2023

Characterization of Fe-6Si Soft Magnetic Alloy Produced by Laser-Directed Energy Deposition Additive Manufacturing

Abstract Commercial electrical steels, Fe-Si alloys with < 4 wt.% Si, are inexpensive and efficient materials for electrical power conversion. Further efficiency improvements require increasing the silicon concentration to 6 wt.%, at which point the material becomes brittle and difficult to form by conventional rolling and sheet fabrication methods. Additive manufacturing stands to overcome challenges with commercial manufacturing techniques by leveraging near-net-shape fabrication. The wide array of process conditions provides additive manufacturing with increased flexibility, enabling control over the microstructure and mechanical properties. This work explores the microstructures and magnetic properties of ring-shaped Fe-Si alloys produced using concentric and cross-hatch tool paths on a laser-directed energy deposition additive manufacturing system. Concentric-built samples exhibit elongated grain structures while cross-hatch-built samples comprise lower aspect ratio grain structures. Thermal finite element analysis simulations model the stress conditions produced by the different scan path geometries. Microhardness measurements probe the mechanical properties as a function of anneal temperature, providing a qualitative understanding of the intergranular defect density. Soft magnetic properties measured under quasistatic and AC conditions show frequency- and microstructure-dependent coercivity and permeability. Finally, analysis of the core loss quantifies how the build strategies and thermal treatments influence efficiency in electrical power conversion applications. Understanding the influences of scan path geometry and thermal treatment provides a pathway towards application of additively manufactured soft magnetic materials.

Adamczyk, Jesse M.↗

DOE OSTI2023

Cobalt Oxide-Coated Single Crystalline Bismuth Vanadate Photoanodes for Efficient Photoelectrochemical Chlorine Generation

Bismuth vanadate (BiVO 4 ) is an outstanding photoanode material for photoelectrochemical water splitting. Here in this work, a series of single crystalline BiVO 4 photoanodes are synthesized by pulsed laser deposition (PLD). Once coated with a thin layer of cobalt oxide (CoO x ) cocatalyst, also by PLD, the photoanodes support efficient photoelectrochemical generation of chlorine (Cl 2 ) from brine under simulated solar light. The activity of the chlorine generation reaction (ClER) is optimized when the thickness of CoO x is about 3 nm, with the faradic efficiency of ClER exceeding 60%. Detailed studies show that the CoO x cocatalyst layer is amorphous, uniform in thickness, and chemically robust. As such, the cocatalyst also effectively protects the underlying BiVO 4 photoanodes against chlorine corrosion. This work provides insights into using artificial photosynthesis for byproducts that carry significant economic value while avoiding the energetically expensive oxygen evolution reactions.

36 MATERIALS SCIENCE↗

DOE OSTI2025

Coherent phonon flatband generated in GaAs/AlAs superlattices via layer-selective optical pumping

Flatbands, characterized by their dispersionless energy levels in electronic, magnetic, and phononic systems, hold substantial potential for advancements in electronics and quantum information processing. Most flatbands exist in thermal equilibrium and cannot be easily created or annihilated externally, limiting their flexibility as switchable knobs for use in microelectronics and quantum applications. In our work, we demonstrate the generation of a coherent phonon flatband in a GaAs/AlAs superlattice using 800 nm femtosecond laser pulses. This coherent phonon flatband does not correspond to a phonon eigenmode at equilibrium and exhibits strong coupling with two branches of coherently excited longitudinal phonon modes. With molecular dynamics simulations, we show more generally that the coherent phonon flatband can be induced by coherently and spatially modulated optical excitations of superlattice structures. Our results highlight a pathway for coherent phonon flatband creation in the time domain that can be generalized to various superlattice systems, potentially inspiring the realization of coherent flatband generation of other quasiparticles.

Condensed-matter physics↗

DOE OSTI2024

Characterization and controllability of radiated power via extrinsic impurity seeding in strongly negative triangularity plasmas in DIII-D

Experiments with extrinsic impurity seeding in strongly negative triangularity shapes in DIII-D achieved radiated power fractions (relative to input power) of up to ≈85% total radiation and ≈55% core radiation in steady-operating conditions. The relationship between core and total radiation was sensitive to impurity species and input power. Attempts to reach higher radiation levels via higher impurity flows resulted in radiative collapse disruptions. Nitrogen, neon, argon, and krypton were tested. Injection was by gas puffing, usually controlled by feeding back real-time estimates for core or total radiating fractions ($P_\textrm{rad} / P_\textrm{input}$). Argon and krypton were controlled by feeding back total radiating fraction, whereas neon was controlled by feeding back the core radiating fraction, due to the lower efficiency of neon as a divertor radiator. Nitrogen flows were pre-programmed. Reasonable total $P_\textrm{rad}$ control target following was achieved with argon or krypton. Control was more challenging with the neon/core radiation configuration, which was more prone to slow response and overshooting of the control target. Poor particle removal contributed to the control challenge: neon particle inventory within the last closed flux surface was roughly constant for up to 1 s (the longest duration tested) after neon injection was halted. However, separate experiments with laser-blow off of non-recycling impurities measured a short impurity confinement time, on the scale of the energy confinement time of ∼100 ms. Modeling with the Aurora impurity transport simulation matched experimental neon density profiles with full recycling (R = 1.0) and weak pumping but predicted rapid decreases in neon inventory if pumping were increased or recycling decreased. This indicates that changes outside the confined plasma (adding a well-placed pump) would improve controllability for all highly recycling species.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗