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At least 1,063 records · Page 59

Ultrafast formation of topological defects in a two-dimensional charge density wave

Topological defects play a central role in dynamical systems undergoing a non-adiabatic transition. In solids, topological defects as a result of femtosecond laser excitation have attracted increasing interest not only because they are key to understanding phase transitions but also because they can generate a variety of hidden orders that are not accessible in thermal equilibrium. Despite the common occurrence of these defects in a non-equilibrium system, the fundamental limit on how fast they can emerge in solids and the generic pathway for defect creation at such fast timescales have remained open questions. Here we apply ultrafast electron diffraction to study the reciprocal-space signatures of transient defects in a two-dimensional charge density wave, where simultaneous measurements of both defect and phonon dynamics yield a microscopic view of defect formation in the femtosecond regime. We find that one-dimensional domain walls are generated well within 1 ps following photoexcitation, during which the defect growth is not dictated by the amplitude of the order parameter but is mediated by a non-thermal population of longitudinal optical phonons. In conclusion, our work provides a framework for the ultrafast engineering of topological defects that are coupled to specific collective modes, which will prove useful for the dynamical control of non-equilibrium phases in correlated materials.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Quantum spin helices more stable than the ground state: Onset of helical protection

Topological magnetic structures are promising candidates for resilient information storage. An elementary example is spin helices in one-dimensional easy-plane quantum magnets. To quantify their stability, we numerically implement the stochastic Schrödinger equation and time-dependent perturbation theory for spin chains with fluctuating local magnetic fields. Here, we find two classes of quantum spin helices that can reach and even exceed ground-state stability: spin-current-maximizing helices and, for fine-tuned boundary conditions, the recently discovered “phantom helices.” Beyond that, we show that the helicity itself (left or right rotating) is even more stable. We explain these findings by separated helical sectors and connect them to topological sectors in continuous spin systems. The resulting helical protection mechanism is a promising phenomenon for stabilizing helical quantum structures, e.g., in ultracold atoms and solid-state systems. We also identify a third type of phantom helix in the system.

1-dimensional spin chains↗

Short-Depth QAOA circuits and Quantum Annealing on Higher-Order Ising Models (Rev.2)

The Quantum Alternating Operator Ansatz (QAOA) and Quantum Annealing (QA) are quantum algorithms that are both based on the adiabatic theorem and both have the goal of sampling the optimal solution(s) of combinatorial optimization problems. Quantum annealing has been physically instantiated on D-Wave devices using superconducting flux qubits, and QAOA can be programmed on digital gate-model quantum computers such as the programmable superconducting transmon qubits devices of the IBMQ series, for instance ibm washington. QAOA and QA address the same types of problems, but it is unclear how they will scale to large problem sizes and to larger and higher-fidelity quantum computers. In this article, we present a direct comparison between QAOA, one and two rounds, run on all 127 qubits of ibm washington and QA run on D-Wave Advantage system4.1 and Advantage system6.1. The problems which allow for this comparison are random Ising model problems whose connectivity matches the heavy hexagonal lattice topology of ibm washington and the Pegasus graph connectivity of the two D-Wave devices. We create two classes of problem instances for this comparison: one with higher order terms (ZZZ variable interactions), linear terms, and quadratic terms, and a separate problem type with only linear and quadratic terms. Our QAOA circuits are novel and extremely short depth, with a CNOT depth of 6 per round, which allows whole chip usage of ibm washington’s heavy hexagonal lattice and can be applied to future heavy-hex chips. We also test the effectiveness of the error suppression technique digital dynamical decoupling on the QAOA circuits. The QAOA circuits compiled to ibm washington are composed of several thousand circuit instructions, approximately 3, 000 depending on the details of the circuit, making these some the largest quantum circuits ever executed on a digital quantum processor. QAOA and QA are compared against the classical heuristic algorithm of simulated annealing and all problem instances are exactly solved using CPLEX in order to evaluate which samplers, if any, correctly found the ground state solution(s) of the problem instances. We find that (i) QA outperforms QAOA on all problem instances, (ii) QAOA samples the problems better than random sampling, and (iii) QAOA angle computation exhibits clear parameter concentration across the ensemble of Ising models.

127 Qubits↗

Quantum-limit phenomena and band structure in the magnetic topological semimetal EuZn 2 As 2

The interplay between magnetism and electronic topology in the quantum limit is a forefront subject of condensed matter physics. Here, we show the electronic and magnetic properties of layered antiferromagnet EuZn 2 As 2 in pulsed magnetic fields up to 60 T and temperatures down to 0.6 K. By analyzing the quantum oscillations observed in the magnetoresistance (MR) and proximity detector oscillator (PDO) frequency, we find that (1) the oscillation frequency F = 46 ± 6 T for H // c and 42 ± 2 T for H // ab; (2) the corresponding Berry phase is close to π for H // c, implying a nontrivial topology; and (3) the large linear MR occurs beyond the first Landau level, without any sign of saturation. From these observations, we conclude that the linear MR can be understood by considering diffusing cyclotron centers due to compressed Landau wavefunction, an emergent behavior in the quantum limit.

36 MATERIALS SCIENCE↗

Topology, criticality, and dynamically generated qubits in a stochastic measurement-only Kitaev model

Here we consider a paradigmatic solvable model of topological order in two dimensions, Kitaev's honeycomb Hamiltonian, and turn it into a measurement-only dynamics consisting of stochastic measurements of two-qubit bond operators. We find an entanglement phase diagram that resembles that of the Hamiltonian problem in some ways, while being qualitatively different in others. When one type of bond is dominantly measured, we find area-law entangled phases that protect two topological qubits (on a torus) for a time exponential in system size. This generalizes the recently proposed idea of Floquet codes, where logical qubits are dynamically generated by a time-periodic measurement schedule, to a stochastic setting. When all types of bonds are measured with comparable frequency, we find a critical phase with a logarithmic violation of the area law, which sharply distinguishes it from its Hamiltonian counterpart. The critical phase has the same set of topological qubits, as diagnosed by the tripartite mutual information, but protects them only for a time polynomial in system size. Furthermore, we observe an unusual behavior for the dynamical purification of mixed states, characterized at late times by the dynamical exponent z = $\frac{1}{2}$ a superballistic dynamics made possible by measurements.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Landau level of fragile topology

Here, we study the Hofstadter butterfly and Landau levels of the twisted bilayer graphene (TBG). We show that the nontrivial fragile topology of the lowest two bands near the charge neutral point makes their Hofstadter butterfly generically connected with higher bands, closing the gap between the first and second conduction (valence) bands at a certain magnetic flux per unit cell. We also develop a momentum space method for calculating the TBG Hofstadter butterfly, from which we identify three phases where the Hofstadter butterflies of the lowest two bands and the higher bands are connected in different ways. We show this leads to a crossing between the $\textit{ν}$ = 4 Landau fan from the charge neutral point and the zero-field band gap at one flux per moiré unit cell, which corresponds to a magnetic field 25$θ^2$ T (twist angle $\textit{θ}$ in degrees). This provides an experimentally testable feature of the fragile topology. In general, we expect it to be a generic feature that the Hofstadter butterfly of the topological bands are connected with the Hofstadter spectra of other bands. We further show the TBG band theory with Zeeman splitting being the most sizable splitting could result in Landau fans at the charge neutral point and half fillings near the magic angle, and we predict their variations under an in-plane magnetic field.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Hall viscosity of the composite-fermion Fermi seas for fermions and bosons

The Hall viscosity has been proposed as a topological property of incompressible fractional quantum Hall states and can be evaluated as Berry curvature. This paper reports on the Hall viscosities of composite-fermion Fermi seas at ν = 1/m, where m is even for fermions and odd for bosons. A well-defined value for the Hall viscosity is not obtained by viewing the 1/m composite-fermion Fermi seas as the n → ∞ limit of the Jain ν = n/(nm ± 1) states, whose Hall viscosities (±n + m)ℏρ/4 (ρ is the two-dimensional density) approach ±∞ in the limit n → ∞. A direct calculation shows that the Hall viscosities of the composite-fermion Fermi sea states are finite and also relatively stable with system size variation, although they are not topologically quantized in the entire τ space. Here, I find that the ν = 1/2 composite-fermion Fermi sea wave function for a square torus yields a Hall viscosity that is expected from particle-hole symmetry and is also consistent with the orbital spin of 1/2 for Dirac composite fermions. I compare my numerical results with some theoretical conjectures.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Universal signatures of Dirac fermions in entanglement and charge fluctuations

We study the entanglement entropy (EE) and charge fluctuations in models where the low-energy physics is governed by massless Dirac fermions. We focus on the response to flux insertion which, for the EE, is widely assumed to be universal, i.e., independent of the microscopic details. We provide an analytical derivation of the EE and charge fluctuations for the seminal example of graphene, using the dimensional reduction of its tight-binding model to the one-dimensional Su-Schrieffer-Heeger model. Our asymptotic expression for the EE matches the conformal field theory prediction. We show that the charge variance has the same asymptotic behavior, up to a constant prefactor. To check the validity of universality arguments, we numerically consider several models, with different geometries and numbers of Dirac cones, and either for strictly two-dimensional models or for a gapless surface mode of three-dimensional topological insulators. We also show that the flux response does not depend on the entangling surface geometry as long as it encloses the flux. Finally we consider the universal corner contributions to the EE. We show that in the presence of corners, the Kitaev-Preskill subtraction scheme provides nonuniversal, geometry-dependent results.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Interfacial Magnetic Skyrmions and Proximity Effects

The goal of this project is to study the fundamental physics of the magnetic skyrmion, an emergent topological spin texture with whirlpool-like spin winding configuration. Distinguishing functionality of the skyrmion can be achieved only when its exotic topological properties are fully understood and control of skyrmions is mastered. In this project, special attention is paid to creation and manipulation of interfacial skyrmions, and skyrmions in confined or hybrid structures. Relevant topics on interfacial magnetism in general are also covered. This project also promotes the skyrmion physics in national laboratories through partnership with the Argonne National Laboratory (ANL).

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Fracton-elasticity duality in twisted moiré superlattices

We formulate a fracton-elasticity duality for twisted moiré superlattices, taking into account that they are incommensurate crystals with dissipative phason dynamics. From a dual tensor-gauge formulation, as compared to standard crystals, we identify twice the number of conserved charges that describe topological lattice defects, namely, disclinations and another type of defects that we dub discompressions. Furthermore, the key implication of these conservation laws is that both glide and climb motions of lattice dislocations are suppressed, indicating that dislocation networks may become exceptionally stable. We also generalize our results to other planar incommensurate crystals and quasicrystals.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

A room temperature polar magnetic metal

The emergence of long-range magnetic order in noncentrosymmetric compounds has stimulated interest in the possibility of exotic spin transport phenomena and topologically protected spin textures for applications in next-generation spintronics. Polar magnets, with broken symmetries of spatial inversion and time reversal, usually host chiral spin textures. This work reports on a wurtzite-structure polar magnetic metal, identified as AA'-stacked (Fe 0.5 Co 0.5 ) 5 GeTe 2 , which exhibits a Néel-type skyrmion lattice as well as a Rashba-Edelstein effect at room temperature. Atomic resolution imaging of the structure reveals a structural transition as a function of Co-substitution, leading to the emergence of the polar phase at 50% Co. We report this discovery reveals an unprecedented layered polar magnetic system for investigating intriguing spin topologies, and it ushers in a promising new framework for spintronics.

36 MATERIALS SCIENCE↗

The hybrid topological longitudinal transmon qubit

We introduce a new hybrid qubit consisting of a Majorana qubit interacting with a transmon longitudinally coupled to a resonator. To do so, we equip the longitudinal transmon qubit with topological quasiparticles, supported by an array of heterostructure nanowires, and derive charge- and phase-based interactions between the Majorana qubit and the resonator and transmon degrees of freedom. Inspecting the charge coupling, we demonstrate that the Majorana self-charging can be eliminated by a judicious choice of charge offset, thereby maintaining the Majorana degeneracy regardless of the quasiparticles spatial arrangement and parity configuration. We perform analytic and numerical calculations to derive the effective qubit-qubit interaction elements and discuss their potential utility for state readout and quantum error correction. Further, we find that select interactions depend strongly on the overall superconducting parity, which may provide a direct mechanism to characterize deleterious quasiparticle poisoning processes.

36 MATERIALS SCIENCE↗

Fractional magnetic charges and channeling of Faraday lines by disclinations in artificial spin ice

We have studied the magnetic moments of artificial spin ice arrays of nanomagnets in both undistorted square arrays and in arrays with a topological defect induced by a single disclination. We confirm that the disclination induces global, macroscopic changes in the low-energy collective states of the nanomagnet moment configuration. Specifically, the disclination leads to Faraday lines of effective magnetic flux that run from the center all the way to the edge of the arrays. Moreover, the geometric deformation, induced by the topological defect, curves the geometry such that these Faraday lines are channeled preferentially by the arrays’ curved geometry. Our results demonstrate how the intentional combination of topology and geometry can be designed to control magnetic charges and the flow of local magnetization and thus manipulate associated collective excitations.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Anomalous Shiba states in topological iron-based superconductors

We demonstrate the formation of robust zero energy modes close to magnetic impurities in the iron-based superconductor FeSe 1–x Te x . We find that the Zeeman field generated by the impurity favors a spin-triplet inter-orbital pairing as opposed to the spin-singlet intra-orbital pairing prevalent in the bulk. The preferred spin-triplet pairing preserves time-reversal symmetry and is topological, as robust, topologically-protected zero modes emerge at the boundary between regions with different pairing states. Moreover, the zero modes form Kramers doublets that are insensitive to the direction of the spin polarization or to the separation between impurities. Here, we argue that our theoretical results are consistent with recent experimental measurements on FeSe 1–x Te x .

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Unitary Subharmonic Response and Floquet Majorana Modes

Detection and manipulation of excitations with non-Abelian statistics, such as Majorana fermions, are essential for creating topological quantum computers. To this end, we show the connection between the existence of such localized particles and the phenomenon of unitary subharmonic response (SR) in periodically driven systems. In particular, starting from highly nonequilibrium initial states, the unpaired Majorana modes exhibit spin oscillations with twice the driving period, are localized, and can have exponentially long lifetimes in clean systems. While the lifetime of SR is limited in translationally invariant systems, we show in this work that disorder can be engineered to stabilize the subharmonic response of Majorana modes. A viable observation of this phenomenon can be achieved using modern multiqubit hardware, such as superconducting circuits and cold atomic systems.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Floquet engineering of tilted and gapped Dirac bandstructure in 1T$$^\prime$$-MoS$$_2$$

Abstract We have developed a rigorous theoretical formalism for Floquet engineering, investigating, and subsequently tailoring most crucial electronic properties of 1T $$^\prime$$ ′ -MoS $$_2$$ 2 by applying an external high-frequency dressing field within the off-resonance regime. It was recently demonstrated that monolayer semiconducting 1T $$^\prime$$ ′ -MoS $$_2$$ 2 exhibits tunable and gapped spin- and valley-polarized tilted Dirac bands. The electron-photon dressed states depend strongly on the polarization of the applied irradiation and reflect a full complexity of the low-energy Hamiltonian for non-irradiated material. We have calculated and analyzed the properties of the electron dressed states corresponding to linear and circular polarization of a dressing field by focusing on their symmetry, anisotropy, tilting, direct and indirect band gaps. Circularly polarized dressing field is known for transition into a new electronic state with broken time-reversal symmetry and a non-zero Chern number, and therefore, the combination of these topologically non-trivial phases and transitions between them could reveal some truly unique and previously unknown phenomena and applications. We have also computed and discussed the density of states for various types of 1T $$^\prime$$ ′ -MoS $$_2$$ 2 materials and its modification in the presence of a dressing field.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Structural Chirality of Polar Skyrmions Probed by Resonant Elastic X-Ray Scattering

An escalating challenge in condensed-matter research is the characterization of emergent orderparameter nanostructures such as ferroelectric and ferromagnetic skyrmions. Their small length scales coupled with complex, three-dimensional polarization or spin structures makes them demanding to trace out fully. Resonant elastic x-ray scattering (REXS) has emerged as a technique to study chirality in spin textures such as skyrmions and domain walls. It has, however, been used to a considerably lesser extent to study analogous features in ferroelectrics. Here, in this study, we present a framework for modeling REXS from an arbitrary arrangement of charge quadrupole moments, which can be applied to nanostructures in materials such as ferroelectrics. With this, we demonstrate how extended reciprocal space scans using REXS with circularly polarized x rays can probe the three-dimensional structure and chirality of polar skyrmions. Measurements, bolstered by quantitative scattering calculations, show that polar skyrmions of mixed chirality coexist, and that REXS allows valuation of relative fractions of right- and left-handed skyrmions. Our quantitative analysis of the structure and chirality of polar skyrmions highlights the capability of REXS for establishing complex topological structures toward future application exploits.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Coexistence of non-Abelian chiral spin liquid and magnetic order in a spin-1 antiferromagnet

We study the ground-state properties of a spin-1 Heisenberg model on a square lattice with the first- and second-nearest-neighbor antiferromagnetic couplings $J_1$ and $J_2$ and a three-spin scalar chirality term $J_\chi$. Using the density matrix renormalization group calculation, we map out a global phase diagram including various magnetic order phases and an emergent quantum spin liquid phase. The nature of the spin liquid is identified as a bosonic non-Abelian Moore-Read state from the fingerprint of the entanglement spectra and identification of a full set of topological sectors. We further unveil a stripe magnetic order coexisting with this spin liquid. Furthermore, our results not only establish a rare example of non-Abelian spin liquids in simple spin systems but also demonstrate the coexistence of fractionalized excitations and magnetic order beyond mean-field descriptions.

2-dimensional systems↗