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At least 1,063 records · Page 59

Core-collapse supernovae from 9 to 120 solar masses based on neutrino-powered explosions

Nucleosynthesis, light curves, explosion energies, and remnant masses are calculated for a grid of supernovae (SNe) resulting from massive stars with solar metallicity and masses from 9.0 to 120 M{sub ⊙}. The full evolution is followed using an adaptive reaction network of up to 2000 nuclei. A novel aspect of the survey is the use of a one-dimensional neutrino transport model for the explosion. This explosion model has been calibrated to give the observed energy for SN 1987A, using five standard progenitors, and for the Crab SN using a 9.6 M{sub ⊙} progenitor. As a result of using a calibrated central engine, the final kinetic energy of the SN is variable and sensitive to the structure of each pre-SN star. Many progenitors with extended core structures do not explode, but become black holes (BHs), and the masses of exploding stars do not form a simply connected set. The resulting nucleosynthesis agrees reasonably well with the Sun provided that a reasonable contribution from SNe Ia is also allowed, but with a deficiency of light s-process isotopes. The resulting neutron star initial mass function has a mean gravitational mass near 1.4 M{sub ⊙}. The average BH mass is about 9 M{sub ⊙} if only the helium core implodes, and 14 M{sub ⊙} if the entire pre-SN star collapses. Only ∼10% of SNe come from stars over 20 M{sub ⊙}, and some of these are Type Ib or Ic. Some useful systematics of Type IIp light curves are explored.

79 ASTRONOMY AND ASTROPHYSICS↗

Characterization of MODIS VIS/NIR Spectral Band Detector-to-Detector Difference

MODIS has 36 spectral bands with wavelengths in the visible (VIS), near-infrared (NIR), shortwave infrared (SWTR), mid-wave infrared (MWIR), and long-wave infrared (LWIR). It makes observations at three nadir spatial resolutions: 0,25km for bands 1-2 with 40 detectors per band, 0.5km for bands 3-7 with 20 detectors per band, and 1km for bands 8-36 with 10 detectors per band. The VIS, NIR, and S\VIR spectral bands are the reflective solar bands (RSB), which are calibrated on-orbit by a solar diffuser (SD). In addition, MODIS lunar observations are used to track the RSB calibration stability. In this study, we examine detector-to-detector calibration difference for the VIStNIR spectral bands using the SD and lunar observations. The results will be compared with an independent analysis with additional information, such as polarization correction, derived from standard ocean color data products. The current MODIS RSB calibration approach only carries a band-averaged RVS (response versus scan angle) correction. The results from this study suggest that a detector-based RVS correction should be used to improve the L1B data quality, especially for several VIS bands in Terra MODIS due to large changes of the scan mirror's optical properties in recent years.

Xiong, X.↗

Determination of plutonium in spent nuclear fuel using high resolution X-ray

Characterization of Pu is an essential aspect of safeguards operations at nuclear fuel reprocessing facilities. A novel analysis technique called hiRX (high resolution X-ray) has been developed for the direct measurement of Pu in spent nuclear fuel dissolver solutions. hiRX is based on monochromatic wavelength dispersive X-ray fluorescence (MWDXRF), which provides enhanced sensitivity and specificity compared with conventional XRF techniques. A breadboard setup of the hiRX instrument was calibrated using spiked surrogate spent fuel (SSF) standards prepared as dried residues. Samples of actual spent fuel were utilized to evaluate the performance of the hiRX. The direct detection of just 39 ng of Pu is demonstrated. Initial quantitative results, with error of 4–27% and precision of 2% relative standard deviation (RSD), were obtained for spent fuel samples. The limit of detection for Pu (100 s) within an excitation spot of 200 μm diameter was 375 pg. This study demonstrates the potential for the hiRX technique to be utilized for the rapid, accurate, and precise determination of Pu. Moreover, the results highlight the analytical capability of hiRX for other applications requiring sensitive and selective nondestructive analyses.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

High-Resolution Measurement of Soil Thermal Properties and Moisture Content Using a Novel Heated Fiber Optics Approach

Hydrological parameters are scale dependent. Efficient monitoring techniques capable of measuring hydrological parameters, such as soil moisture content (θ), over a wide range of spatial scales are essential for understanding the complexity of water and energy movement across the landscape. Techniques to measure θ over spatial scales in the range from centimeters to thousands of meters, however, are sorely lacking. Recent improvements in the distributed temperature sensing (DTS) technology supported the development of novel techniques to fill that gap. However, improvements in the accuracy and applicability of DTS techniques are still needed. This study investigates the possibility of improving the accuracy of the fiber optics dual-probe heat-pulse (FO-DPHP) DTS technique by using a new design to maintain the spacing between the FO-DPHP probes and by introducing a novel data interpretation approach. The accuracy of the novel FO-DPHP design was tested at different θ in a sand column experiment. The FO-DPHP measurements obtained using traditional and novel data interpretation approaches were compared against independent measurements from several calibrated soil water content (EC5) sensors. Monte-Carlo analyses were also performed to assess the impact of DTS measurement errors on the accuracy achieved using the data interpretation approaches. The novel design and data interpretation approach allowed for accurate measurements of soil thermal properties and θ without the need to perform a hard-to-achieve soil-specific calibration. Measured θ had mean errors and standard deviations <0.03 and <0.01 m 3 m -3 , respectively, for moisture conditions ranging from dry to near saturation. The standard deviation in the measured heat capacity was <0.01 MJ m -3 K -1 .

42 ENGINEERING↗

Extreme ultraviolet microscope characterization using photomask surface roughness

We demonstrate a method for characterizing the field-dependent aberrations of a full-field synchrotron-based extreme ultraviolet microscope. The statistical uniformity of the inherent, atomic-scale roughness of readily-available photomask blanks enables a self-calibrating computational procedure using images acquired under standard operation. We characterize the aberrations across a 30-um field-of-view, demonstrating a minimum aberration magnitude of smaller than λ/21 rms averaged over the center 5-um area, with a measurement accuracy better than λ/180 rms. The measured field variation of aberrations is consistent with system geometry and agrees with prior characterizations of the same system. In certain cases, it may be possible to additionally recover the illumination wavefront from the same images. Our method is general and is easily applied to coherent imaging systems with steerable illumination without requiring invasive hardware or custom test objects; hence, it provides substantial benefits when characterizing microscopes and high-resolution imaging systems in situ.

47 OTHER INSTRUMENTATION↗

235 U– 231 Pa age dating of uranium materials for nuclear forensic investigations

Here, age dating of nuclear material can provide insight into source and suspected use in nuclear forensic investigations. We report here a method for the determination of the date of most recent chemical purification for uranium materials using the 235 U- 231 Pa chronometer. Protactinium is separated from uranium and neptunium matrices using anion exchange resin, followed by sorption of Pa to an SiO 2 medium. The concentration of 231 Pa is measured by isotope dilution mass spectrometry using 233 Pa spikes prepared from an aliquot of 237 Np and calibrated in-house using the rock standard Table Mountain Latite and the uranium isotopic standard U100. Combined uncertainties of age dates using this method are 1.5 to 3.5 %, an improvement over alpha spectrometry measurement methods. Model ages of five uranium standard reference materials are presented; all standards have concordant 235 U- 231 Pa and 234 U- 230 Th model ages.

07 ISOTOPE AND RADIATION SOURCES↗

Adsorption calorimetry during metal vapor deposition on single crystal surfaces: Increased flux, reduced optical radiation, and real-time flux and reflectivity measurements

Thin films of metals and other materials are often grown by physical vapor deposition. To understand such processes, it is desirable to measure the adsorption energy of the deposited species as the film grows, especially when grown on single crystal substrates where the structure of the adsorbed species, evolving interface, and thin film are more homogeneous and well-defined in structure. Our group previously described in this journal an adsorption calorimeter capable of such measurements on single-crystal surfaces under the clean conditions of ultrahigh vacuum [J. T. Stuckless, N. A. Frei, and C. T. Campbell, Rev. Sci. Instrum. 69, 2427 (1998)]. Here we describe several improvements to that original design that allow for heat measurements with ∼18-fold smaller standard deviation, greater absolute accuracy in energy calibration, and, most importantly, measurements of the adsorption of lower vapor-pressure materials which would have previously been impossible. These improvements are accomplished by: (1) using an electron beam evaporator instead of a Knudsen cell to generate the metal vapor at the source of the pulsed atomic beam, (2) changing the atomic beam design to decrease the relative amount of optical radiation that accompanies evaporation, (3) adding an off-axis quartz crystal microbalance for real-time measurement of the flux of the atomic beam during calorimetry experiments, and (4) adding capabilities for in situ relative diffuse optical reflectivity determinations (necessary for heat signal calibration). These improvements are not limited to adsorption calorimetry during metal deposition, but also could be applied to better study film growth of other elements and even molecular adsorbates.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

PROBING THE OUTER GALACTIC HALO WITH RR LYRAE FROM THE CATALINA SURVEYS

We present analysis of 12,227 type-ab RR Lyraes (RRLs) found among the 200 million public light curves in Catalina Surveys Data Release 1. These stars span the largest volume of the Milky Way ever surveyed with RRLs, covering {approx}20,000 deg{sup 2} of the sky (0 Degree-Sign < {alpha} < 360 Degree-Sign , -22 Degree-Sign < {delta} < 65 Degree-Sign ) to heliocentric distances of up to 60 kpc. Each of the RRLs is observed between 60 and 419 times over a six-year period. Using period finding and Fourier fitting techniques we determine periods and apparent magnitudes for each source. We find that the periods are generally accurate to {sigma} = 0.002% in comparison to 2842 previously known RRLs and 100 RRLs observed in overlapping survey fields. We photometrically calibrate the light curves using 445 Landolt standard stars and show that the resulting magnitudes are accurate to {approx}0.05 mag using Sloan Digital Sky Survey (SDSS) data for {approx}1000 blue horizontal branch stars and 7788 RRLs. By combining Catalina photometry with SDSS spectroscopy, we analyze the radial velocity and metallicity distributions for >1500 of the RRLs. Using the accurate distances derived for the RRLs, we show the paths of the Sagittarius tidal streams crossing the sky at heliocentric distances from 20 to 60 kpc. By selecting samples of Galactic halo RRLs, we compare their velocity, metallicity, and distance with predictions from a recent detailed N-body model of the Sagittarius system. We find that there are some significant differences between the distances and structures predicted and our observations.

79 ASTRONOMY AND ASTROPHYSICS↗

VALIDATION OF THE EQUILIBRIUM MODEL FOR GALAXY EVOLUTION TO z ∼ 3 THROUGH MOLECULAR GAS AND DUST OBSERVATIONS OF LENSED STAR-FORMING GALAXIES

We combine IRAM Plateau de Bure Interferometer and Herschel PACS and SPIRE measurements to study the dust and gas contents of high-redshift star-forming galaxies. We present new observations for a sample of 17 lensed galaxies at z = 1.4-3.1, which allow us to directly probe the cold interstellar medium of normal star-forming galaxies with stellar masses of ∼10{sup 10} M{sub ☉}, a regime otherwise not (yet) accessible by individual detections in Herschel and molecular gas studies. The lensed galaxies are combined with reference samples of submillimeter and normal z ∼ 1-2 star-forming galaxies with similar far-infrared photometry to study the gas and dust properties of galaxies in the SFR-M{sub *}-redshift parameter space. The mean gas depletion timescale of main-sequence (MS) galaxies at z > 2 is measured to be only ∼450 Myr, a factor of ∼1.5 (∼5) shorter than at z = 1 (z = 0), in agreement with a (1 + z){sup –1} scaling. The mean gas mass fraction at z = 2.8 is 40% ± 15% (44% after incompleteness correction), suggesting a flattening or even a reversal of the trend of increasing gas fractions with redshift recently observed up to z ∼ 2. The depletion timescale and gas fractions of the z > 2 normal star-forming galaxies can be explained under the 'equilibrium model' for galaxy evolution, in which the gas reservoir of galaxies is the primary driver of the redshift evolution of specific star formation rates. Due to their high star formation efficiencies and low metallicities, the z > 2 lensed galaxies have warm dust despite being located on the star formation MS. At fixed metallicity, they also have a gas-to-dust ratio 1.7 times larger than observed locally when using the same standard techniques, suggesting that applying the local calibration of the δ{sub GDR}-metallicity relation to infer the molecular gas mass of high-redshift galaxies may lead to systematic differences with CO-based estimates.

79 ASTRONOMY AND ASTROPHYSICS↗

Where did the tumor start? An inverse solver with sparse localization for tumor growth models

In this work, we present a numerical scheme for solving an inverse problem for parameter estimation in tumor growth models for glioblastomas, a form of aggressive primary brain tumor. The growth model is a reaction–diffusion partial differential equation (PDE) for the tumor concentration. We use a PDE-constrained optimization formulation for the inverse problem. The unknown parameters are the reaction coefficient (proliferation), the diffusion coefficient (infiltration), and the initial condition field for the tumor PDE. Segmentation of magnetic resonance imaging (MRI) scans drive the inverse problem where segmented tumor regions serve as partial observations of the tumor concentration. Like most cases in clinical practice, we use data from a single time snapshot. Moreover, the precise time relative to the initiation of the tumor is unknown, which poses an additional difficulty for inversion. We perform a frozen-coefficient spectral analysis and show that the inverse problem is severely ill-posed. We introduce a biophysically motivated regularization on the structure and magnitude of the tumor initial condition. In particular, we assume that the tumor starts at a few locations (enforced with a sparsity constraint on the initial condition of the tumor) and that the initial condition magnitude in the maximum norm is equal to one. We solve the resulting optimization problem using an inexact quasi-Newton method combined with a compressive sampling algorithm for the sparsity constraint. Our implementation uses PETSc and AccFFT libraries. We conduct numerical experiments on synthetic and clinical images to highlight the improved performance of our solver over a previously existing solver that uses standard two-norm regularization for the calibration parameters. The existing solver is unable to localize the initial condition. Our new solver can localize the initial condition and recover infiltration and proliferation. In clinical datasets (for which the ground truth is unknown), our solver results in qualitatively different solutions compared to the two-norm regularized solver.

97 MATHEMATICS AND COMPUTING↗

Reduced-order atomistic cascade method for simulating radiation damage in metals

Atomistic modeling of radiation damage through displacement cascades is deceptively non-trivial. Because of the high energy and stochastic nature of atomic collisions, individual primary knock-on atom (PKA) cascade simulations are computationally expensive and ill-suited for length and dose upscaling. Here, we propose a reduced-order atomistic cascade model capable of predicting and replicating radiation events in metals across a wide range of recoil energies. Our methodology approximates cascade and displacement damage production by modeling the cascade as a core-shell atomic structure composed of two damage production estimators, namely an athermal recombination corrected displacements per atom (arc-dpa) in the shell and a replacements per atom (rpa) representing atomic mixing in the core. These estimators are calibrated from explicit PKA simulations and a standard displacement damage model that incorporates cascade defect production efficiency and mixing effects. We highlight the predictability and accuracy of our reduced-order atomistic cascade method for the cases of copper and niobium by comparing its results with those from full PKA simulations in terms of defect production as well as the resulting cascade evolution and structure. We offer examples for simulating high energy cascade fragmentation and large dose ion-bombardment to demonstrate its possible applicability. Finally, we discuss the various practical considerations and challenges associated with this methodology especially when simulating subcascade formation and dose effects.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Projected evolution of droughts and human exposure in the contiguous United States under SSP5-8.5: a regional downscaling perspective

The increasingly unpredictable and extreme weather patterns under a warming climate underscore the urgency of accurate regional assessments of future drought risk. This study evaluates the projected drought evolution in the contiguous United States under the high-emission shared socioeconomic pathway 5–8.5 climate scenario for the coming decades. Using a multi-model ensemble of six Coupled Model Intercomparison Project Phase 6 global climate models combined with dynamical downscaling techniques, we analyzed near-term (2020–2039) and mid-term (2040–2059) drought patterns using the self-calibrating palmer drought severity index (ScPDSI), the standardized precipitation index (SPI-12), and the Standardized Precipitation-Evapotranspiration Index (SPEI-12). Results reveal a widespread increase in abnormally dry (D0) and moderate drought (D1) conditions, particularly in urban areas, while severe (D2), extreme (D3), and exceptional (D4) droughts are expected to become less common in many regions. Meanwhile, persistent and intensifying droughts are projected in the western and southwestern U.S., driven by long-term soil moisture deficits. The ScPDSI projects that 1.1 million urban residents will be affected by D0 conditions in 2050, while SPI-12 suggests a decrease in the total affected populations after 2040. ScPDSI indicates prolonged droughts in the West, and SPI-12 captures transient variability. Although the total drought-exposed population is expected to decrease, urban areas will continue to bear a greater burden, particularly for mild droughts (D0, D1). These findings highlight a shift toward more frequent mild droughts, fewer severe droughts, and persistent drying in the Southwest, emphasizing the need for region-specific adaptation strategies.

CMIP6↗

The iron oxidation state of Ryugu samples

The Hayabusa2 mission sampled Ryugu, an asteroid that did not suffer extensive thermal metamorphism, and returned rocks to the Earth with no significant air exposure. It therefore offers a unique opportunity to study the redox state of carbonaceous Cb-type asteroids and evaluate the overall redox state of the most primitive rocks of the solar system. An analytical framework was developed to investigate the iron mineralogy and valence state in extraterrestrial material at the micron scale by combining x-ray diffraction, conventional Mössbauer (MS), and nuclear forward scattering (NFS) spectroscopies. An array of standard minerals was analyzed and cross-calibrated between MS and NFS. Then, MS and NFS spectra on three Ryugu grains were collected at the bulk and the micron scales. In Ryugu samples, iron is essentially accommodated in magnetite, clay minerals (serpentine–smectite), and sulfides. Only a single set of Mössbauer parameters was necessary to account for the entire variability observed in MS and NFS spectra, at all spatial scales investigated. These parameters therefore make up a fully consistent iron mineralogical model for the Ryugu samples. As far as MS and NFS spectroscopies are concerned, Ryugu grains are overall similar to each other and share most of their mineralogical features with CI-type chondrites. In detail however, no ferrihydrite is found in Ryugu particles even at the very sensitive scale of Mössbauer spectroscopy. The typical Fe 3+ /Fe tot of clay minerals is much lower than typical redox ratios measured in CI chondrites (Fe 3+ /Fe tot = 85%–90%). Furthermore, magnetite from Ryugu is stoichiometric with no significant maghemite component, whereas up to 12% of maghemite was previously identified in the Orgueil's so-called magnetite. These differences suggest that most CI meteorites suffered terrestrial alteration and that the preterrestrial composition of these carbon-rich samples was less oxidized than previously measured. However, it is not clear yet whether or not the parent bodies of CI chondrites were as reduced as Ryugu. Finally, the high spatial resolution of NFS allows to disentangle the redox state and the crystal chemistry of iron accommodated in serpentine and smectite. The most likely polytype of serpentine is lizardite, containing <35% of Fe 3+ , a fraction of which being tetrahedrally coordinated. Smectite is more oxidized (Fe 3+ /Fe tot > 65%) and mainly contains octahedral ferric iron. In conclusion, this finding implies that these clays formed from highly alkaline fluids and the spatial variability highlighted here may suggest a temporal evolution or a spatial variability of the nature of this fluid.

58 GEOSCIENCES↗

Fast Spatially Resolved Exhaust Gas Recirculation (EGR) Distribution Measurements in an Internal Combustion Engine Using Absorption Spectroscopy

One effective method of reducing NO x emissions while improving efficiency is exhaust gas recirculation (EGR) in internal combustion engines. But, insufficient mixing between fresh air and exhaust gas can lead to cycle-to-cycle and cylinder-to-cylinder nonuniform charge gas mixtures of a multi-cylinder engine, which can in turn reduce engine performance and efficiency. Furthermore, a sensor packaged into a compact probe was designed, built and applied to measure spatiotemporal EGR distributions in the intake manifold of an operating engine. The probe promotes the development of more efficient and higher-performance engines by resolving high-speed in situ CO 2 concentration at various locations in the intake manifold. Our study employed mid-infrared light sources tuned to an absorption band of CO 2 near 4.3 μm, an industry standard species for determining EGR fraction. The calibrated probe was used to map spatial EGR distributions in an intake manifold with high accuracy and monitor cycle-resolved cylinder-specific EGR fluctuations at a rate of up to 1 kHz.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗

In-Situ Silver Acetylide Silver Nitrate Explosive Deposition Measurements Using X-Ray Fluorescence.

The Light Initiated High Explosive facility utilized a spray deposited coating of silver acetylide - silver nitrate explosive to impart a mechanical shock into targets of interest. A diagnostic was required to measure the explosive deposition in - situ. An X - ray fluorescence spectrometer was deployed at the facility. A measurement methodology was developed to measure the explosive quantity with sufficient accuracy. Through the use of a tin reference material under the silver based explosive, a field calibration relationship has been developed with a standard deviation of 3.2 % . The effect of the inserted tin material into the experiment configuration has been explored.

Covert, Timothy Todd↗

NREL Pyrheliometer Comparisons: September 26-October 7, 2016 (NPC-2016)

Accurate measurements of direct normal (beam) solar irradiance from pyrheliometers are important for developing and deploying solar energy conversion systems, improving our understanding of the Earth's energy budget for climate change studies, and for other science and technology applications involving solar flux. Providing these measurements places many demands on the quality system used by the operator of commercially available radiometers. Maintaining accurate radiometer calibrations that are traceable to an international standard is the first step in producing research-quality solar irradiance measurements. National Renewable Energy Laboratory (NREL) pyrheliometer comparisons (NPCs) are held annually at the Solar Radiation Research Laboratory (SRRL) in Golden, Colorado. Open to all pyrheliometer owners and operators, each NPC provides an opportunity to determine the unique World Radiometric Reference transfer factor (WRR-TF) for each participating pyrheliometer. By adjusting all subsequent pyrheliometer measurements by the appropriate WRR-TF, the solar irradiance data are traceable to the WRR. NPC-2016 was September 26 through October 7, 2016. Participants operated 45 absolute cavity radiometers and 27 conventional thermopile-based pyrheliometers to simultaneously measure clear-sky, direct normal solar irradiance during this period.

14 SOLAR ENERGY↗

RCT: Module 2.08, Radiological Source Control, Course 8774

radioactive source is material used for its emitted radiation. Sources are sealed or unsealed and are classified as accountable or exempt. Radioactive sources are used for response checks, functional checks, and the calibration of instruments and monitors to traceable standards. To ensure the safety and welfare of all personnel, it is important to maintain control of radioactive sources to minimize the potential for the spread of contamination, unnecessary exposure to personnel, loss or theft, and improper disposal. This course will prepare the student with the skills necessary for RCT qualification by passing quizzes, tests, and the RCT Comprehensive Phase 1, Unit 2 Examination (TEST 27566) and will provide in-the-field skills.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗