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At least 1,045 records · Page 58

Direct observation of heat dissipation in individual suspended carbon nanotubes using a two-laser technique

A two-laser technique is used to investigate heat spreading along individual single walled carbon nanotube (SWCNT) bundles in vacuum and air environments. A 532 nm laser focused on the center of a suspended SWCNT bundle is used as a local heat source, and a 633 nm laser is used to measure the spatial temperature profile along the SWCNT bundle by monitoring the G band downshifts in the Raman spectra. A constant temperature gradient is observed when the SWCNT bundle is irradiated in vacuum, giving direct evidence of diffusive transport of the phonons probed by the Raman laser. In air, however, we observe an exponentially decaying temperature profile with a decay length of about 7 {mu}m, due to heat dissipation from the SWCNT bundle to the surrounding gas molecules. The thermal conductivity of the suspended carbon nanotube (CNT) is determined from its electrical heating temperature profile as measured in vacuum and the nanotube bundle diameter measured via transmission electron microscopy. Based on the exponential decay curves measured in three different CNTs in air, the heat transfer coefficient between the SWCNTs and the surrounding air molecules is found to range from 1.5 x 10{sup 3} to 7.9 x 10{sup 4} W/m{sup 2} K, which is smaller than the 1 x 10{sup 5} W/m{sup 2} K thermal boundary conductance value calculated using the kinetic theory of gases. This measurement is insensitive to the thermal contact resistance, as no temperature drops occur at the ends of the nanotube. It is also insensitive to errors in the calibration of the G band temperature coefficient. The optical absorption is also obtained from these results and is on the order of 10{sup -5}.

36 MATERIALS SCIENCE↗

On the ion front of a plasma expanding into a vacuum

Calculations are reported on the expansion of a plasma into a vacuum, using a model of cold ions and Boltzmann electrons. The initial distribution of the ions at the edge of the plasma greatly affects the subsequent expansion. An initial abrupt drop of ion density leads to an expansion in which the abrupt drop is maintained. A finite slope, however, leads to the formation of a peak of ion density at the ion front. The subsequent behaviour may lead to wave breaking and the formation of multi-valued ion velocity distributions.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Optimization of ion-atomic beam source for deposition of GaN ultrathin films

We describe the optimization and application of an ion-atomic beam source for ion-beam-assisted deposition of ultrathin films in ultrahigh vacuum. The device combines an effusion cell and electron-impact ion beam source to produce ultra-low energy (20–200 eV) ion beams and thermal atomic beams simultaneously. The source was equipped with a focusing system of electrostatic electrodes increasing the maximum nitrogen ion current density in the beam of a diameter of ≈15 mm by one order of magnitude (j ≈ 1000 nA/cm{sup 2}). Hence, a successful growth of GaN ultrathin films on Si(111) 7 × 7 substrate surfaces at reasonable times and temperatures significantly lower (RT, 300 °C) than in conventional metalorganic chemical vapor deposition technologies (≈1000 °C) was achieved. The chemical composition of these films was characterized in situ by X-ray Photoelectron Spectroscopy and morphology ex situ using Scanning Electron Microscopy. It has been shown that the morphology of GaN layers strongly depends on the relative Ga-N bond concentration in the layers.

36 MATERIALS SCIENCE↗

Random lasing of microporous surface of Cr{sup 2+}:ZnSe crystal induced by femtosecond laser

We demonstrate a random lasing emission based on microporous surface of Cr{sup 2+}:ZnSe crystal prepared by femtosecond pulsed laser ablation in high vacuum (below 5 × 10{sup −4} Pa). The scanning electron microscope results show that there are a mass of micropores with an average size of ∼13 μm and smaller ones with ∼1.2 μm on the surface of Cr{sup 2+}:ZnSe crystal. The adjacent micropore spacing of the smaller micropores ranges from 1 μm to 5 μm. Under 1750 nm excitation of Nd:YAG (355 nm) pumped optical parametric oscillator, a random lasing emission with center wavelength of 2350 nm and laser-like threshold of 0.3 mJ/pulse is observed. The emission lifetime of 2350 nm laser reduces from 800 ns to 30 ns as the pump energy increases above threshold. The emission spectra and decay time of smooth surface, groove and microporous surface of Cr{sup 2+}:ZnSe crystal are contrasted. The optional pump wavelength range is from 1500 nm to 1950 nm, which in accordance with the optical absorption property of Cr{sup 2+}:ZnSe crystal. The peak position of excitation spectra is almost identical to the strongest absorption wavelength.

36 MATERIALS SCIENCE↗

Impact of spatiotemporal smoothing on the two-plasmon–decay instability

Higher levels of hot electrons from the two-plasmon–decay instability are observed when smoothing by spectral dispersion (SSD) is turned off in directly driven inertial confinement fusion experiments at the Omega Laser Facility. This finding is explained using a hot-spot model based on speckle statistics and simulation results from the laser–plasma simulation environment. The model accurately reproduces the relative increase in hot-electron activity at two different drive intensities, although it slightly overestimates the absolute number of hot electrons in all cases. Extrapolating from the current ≈ 360-GHz system while adhering to the logic of the hot-spot model suggests that larger SSD bandwidth should significantly mitigate hot-electron generation, and legacy 1-THz OMEGA experiments appear to support this conclusion. These results demonstrate that it is essential to account for laser speckles and spatiotemporal smoothing to obtain quantitative agreement with experiments. A compilation of hot-electron data from the past two decades reveals several other important points: (1) many prior experiments are more easily understood using recent results from multibeam absolute instability theory; and (2) experiments with ignition-scale conditions produce less hot electrons compared to OMEGA spherical experiments for a given vacuum overlapped intensity, which is a promising result for validating performance predictions based on hydrodynamic scaling relations.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Components Qualification for a Possible use in the Mu2e Calorimeter Waveform Digitizer

The Mu2e experiment at Fermilab searches for the charged flavor violating conversion of a muon into an electron in the Coulomb field of a nucleus. The detector consists of a straw tube tracker and a CSI crystal electromagnetic calorimeter, both housed in a superconducting solenoid. Both the front-end and the digital electronics, located inside the cryostat, will be operated in vacuum under a 1 T magnetic field, having to sustain the high flux of neutrons and ionizing particles coming from the muons stopping target. These harsh experimental conditions make the design of the calorimeter waveform digitizer quite challenging. All the selected commercial devices must be tested individually and qualified for radiation hardness and operation in high magnetic field. At the moment the expected particles flux and spectra at the digitizers location are not completely simulated and we are using initial rough estimates to select the components for the first prototype. We are gaining experience in the qualification procedures using the selected components but the choice will be frozen only when dose and neutron flux simulations will be completed. The experimental results of the first qualification campaign are presented.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Innovative compact braze-free accelerating cavity

We report that high energy physics experiments using particle accelerators as well as industrial and medical applications are continuously seeking more compact, robust and cheaper accelerating structures. As of today, stable operating gradients, exceeding 100 MV/m, have been demonstrated by the SLAC group in the X-Band (11.424 GHz). These experiments show that hard structures, fabricated without high-temperature processes, achieve a better high gradient performance in terms of accelerating gradients. Therefore, we present an innovative and compact type of accelerating cavity that avoids any high-temperature processes like brazing or diffusion bonding. All cells are joined together by means of specifically designed and proprietary screws which ensure good vacuum and RF contacts. Two three-cell standing-wave accelerating structures, designed to operate in the pi-mode at 11.424 GHz, have been successfully built and cold tested. In order to guarantee a vacuum envelope and mechanically robust assembly, we used the Electron Beam Welding (EBW) and the Tungsten Inert Gas (TIG) processes. Lastly, this work has been carried out in the framework of a funded project by the Vth Committee of the INFN for the Laboratori Nazionali di Frascati (LNF), within a large international collaboration between LNF, SLAC and KEK for the development of X-Band accelerating cavities using "hard structure" technology.

43 PARTICLE ACCELERATORS↗

Extending light WIMP searches to single scintillation photons in LUX

© 2020 American Physical Society. We present a novel analysis technique for liquid xenon time projection chambers that allows for a lower threshold by relying on events with a prompt scintillation signal consisting of single detected photons. The energy threshold of the LUX dark matter experiment is primarily determined by the smallest scintillation response detectable, which previously required a twofold coincidence signal in its photomultiplier arrays, enforced in data analysis. The technique presented here exploits the double photoelectron emission effect observed in some photomultiplier models at vacuum ultraviolet wavelengths. We demonstrate this analysis using an electron recoil calibration dataset and place new constraints on the spin-independent scattering cross section of weakly interacting massive particles (WIMPs) down to 2.5 GeV/c2 WIMP mass using the 2013 LUX dataset. This new technique is promising to enhance light WIMP and astrophysical neutrino searches in next-generation liquid xenon experiments.

79 ASTRONOMY AND ASTROPHYSICS↗

Delta-doping of boron atoms by photoexcited chemical vapor deposition

Boron delta-doped structures in Si crystals were fabricated by means of photoexcited chemical vapor deposition (CVD). Core electronic excitation with high-energy photons ranging from vacuum ultraviolet to soft x rays decomposes B{sub 2}H{sub 6} molecules into fragments. Combined with in situ monitoring by spectroscopic ellipsometry, limited number of boron hydrides can be delivered onto a Si(100) surface by using the incubation period before the formation of a solid boron film. The boron-covered surface is subsequently embedded in a Si cap layer by Si{sub 2}H{sub 6} photo-excited CVD. The crystallinity of the Si cap layer depended on its thickness and the substrate temperature. The evaluation of the boron depth profile by secondary ion mass spectroscopy revealed that boron atoms were confined within the delta-doped layer at a concentration of 2.5 x 10{sup 20} cm{sup -3} with a full width at half maximum of less than 9 nm, while the epitaxial growth of a 130-nm-thick Si cap layer was sustained at 420 deg. C.

36 MATERIALS SCIENCE↗

Effect of the anode material on the X-ray spectrum of micropinch discharge plasma

The effect of the elemental composition of the anode material on the parameters and X-ray spectrum of micropinch discharge plasma have been studied using a low-inductance vacuum spark device. It is shown that the plasma electron temperature T{sub e} and intensity of hard X-ray emission increase with increasing nuclear charge number Z of the anode material of the discharge system.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

EB Vs PAM Vs VAR for Uranium Alloys

Questions were raised during the February ’97 PDP Meeting at LLNL as to the advisability of funding three separate melting development programs (Advanced Vacuum Arc Remelt (VAR), Plasma Arc Melting (PAM) and Electron Beam Melting (EB)) through PDP in this era of shrinking research funds. The main issues seemed to be: 1) Have we evaluated the potentials of the three processes sufficiently to eliminate any of them out of hand and 2) Have any of these processes to date produced results which show clear advantages over the other two. The feeling at the meeting toward the latter seemed to be that all three processes required further development before they would be accepted by the complex as the standard. As far as evaluating potential for process improvements, however, we at Livermore did go through somewhat of a trade study in 1993 when we proposed the EB route. It seemed to us that even with the elimination of the skull caster via a VIM/VAR/VAR route, the problem of recycle limitations in the VIM step due to excessive carbon pick-up limited the potential for a great improvement in material utilization using this method. A single-step, cold hearth route looked to be the preferable choice. Both EB and PAM are used commercially as cold hearth processes, and both have been used for the production of refractory and specialty metals; EB since the mid 1950’s and PAM since the mid 1980’s. Both seem to have found their individual niches with some applications being suited to EB and others to PAM. Both can be adapted to continuous casting techniques and both are capable of imparting the high heat fluxes necessary to melt refractory metals. The major differences appear to be that for most applications, the EB process is capable of producing a purer product, while PAM results in less loss of volatile components. There exists an abundance of information in the open literature on the results of processing via both routes on various materials. The attached 1984 paper gives a good explanation of electron beam melting and plasma melting, and, I believe, a fair assessment of the advantages and limitations of both processes.

36 MATERIALS SCIENCE↗

Silicon solar cells by high-speed low-temperature processing

A new method for silicon solar cell fabrication is being developed around ion implantation and pulsed electron beam techniques. Cells are fabricated totally in a vacuum environment at room temperature. Major reductions result in the time, energy consumption, and waste material generation associated with solar cell production. Cells to date have exhibited air mass zero efficiencies exceeding 10 percent.

Kirkpatrick, A. R.↗

Ion tracking in an electrostatic potential distribution

An ion tracking system utilizing a single detector was designed to resolve two dimensional potential distributions in a vacuum. The ion detector consisted of a continuous dynode electron multiplier tube mounted behind a series of aperture plates. The detector was located on a track below a wedge shaped structure used to produce the desired potential distribution. A 150 volt electron beam aimed at selected regions, ionized the residual gas in the chamber. The ions were ejected from their source points by electrostatic forces causing them to drift downward toward the detector. Measurements of particle energy, detector position, and entry angle of the incoming particle flux were used to initialize a computer trajectory-tracing program. The program assumes a known theoretically calculated potential distribution near the wedge for computation of particle trajectories, providing a basis for evaluating the data. Special attention was given to characterization of the ion detector.

Ross, D. P.↗

Stabilization of He2(A(sup 3)Sigma(sub u)(+)) molecules in liquid helium by optical pumping for vacuum UV laser

A technique is disclosed for achieving large populations of metastable spin-aligned He2(a 3 Sigma u +) molecules in superfluid helium to obtain lasing in the vacuum ultraviolet wavelength regime around 0.0800 micron m by electronically exciting liquid (superfluid) helium with a comparatively low-current electron beam and spin aligning the metastable molecules by means of optical pumping with a modestly-powered (100mW) circularly-polarized continuous wave laser operating at, for example, 0.9096 or 0.4650 micron m. Once a high concentration of spin-aligned He2 (a 3 Sigma u +) is achieved with lifetimes of a few milliseconds, a strong microwave signal destroys the spin alignment and induces a quick collisional transition of He2 (a 3 Sigma u +) molecules to the a 1 Sigma u + state and thereby a lasing transition to the X 1 Sigma g + state.

Zmuidzinas, J. S.↗