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DOE OSTI2024

Characterization of Nitrate, Nitrite, Ammonia, and Tritium in D0220 Cores

This report describes characterization of nitrogen species (nitrate, nitrite, ammonia) in aqueous and solid phases in cores taken in borehole D0220 (well 299-E25-245) under crib 216-A-37-1 at the Hanford Site in 2022 to evaluate (a) the types of nitrogen species currently in the vadose zone and (b) the migration of nitrogen species in the vadose zone. Ammonia and tritium from PUREX decladding condensate were sporadically discharged to the crib from 1977 to 1989. During discharge operations, the estimated travel time through the vadose zone to groundwater was 2.5 to 9 months. By 2003, a characterization borehole (C4106) showed residual pore water with elevated tritium and nitrate in the first 100 ft of the vadose zone, which is likely from the crib. However, there was significantly more nitrate present at the shallowest depth (15 to 22 ft), which may indicate a different source for nitrate, such as adsorbed ammonia slowly being oxidized or nitrogen species precipitates slowly dissolving. In this study, more extensive nitrogen species characterization was done on D0220 cores (drilled in 2022) at 40- and 262-ft depths, which included (a) aqueous nitrate, nitrite, and tritium; (b) adsorbed ammonia; (c) nitrogen in carbonates (or other minerals dissolved in acidic acid); (d) nitrogen in iron oxides (or other minerals dissolved in oxalic acid); and (e) nitrogen in hard-to-extract minerals (minerals dissolved in nitric acid). High pore water nitrate (226 to 331 mg/L) at 40-ft depth measured in D0220 (2022) compared to 60 mg/L at 40-ft depth in C4106 (2003) may indicate nitrate is migrating deeper. Tritium concentrations (pore water 132,000 to 148,000 pCi/L) measured in D0220 at 40-ft depth in 2022 were considerably higher than in C4106 at 40-ft depth (160 pCi/L). Additional nitrogen species mass was present in adsorbed and precipitated phases in D0220 cores. Low adsorbed ammonia was measured at 40.1- and 261.7-ft depths. Low concentrations of carbonate associated nitrogen and iron oxide-associated nitrogen were present at 40.1 and 40.6 ft depths. Nitrogen species in solid phase extractions indicate nitrogen precipitates or aqueous nitrate or ammonia trapped in sediment microfractures that are coated by precipitates. Overall, the nitrogen species and tritium characterization at two depths in D0220 showed that additional nitrogen species were present in the vadose zone. In addition, elevated pore water nitrate in D0220 at 40 ft depth from 2022 may indicate vertical migration compared to C4106 nitrate profile from 2003. Analysis of additional depths in D0220 and spatial variability of the nitrate plume along the length of the crib (from surface electrical resistivity) would be extremely useful for this comparison.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

DOE OSTI2024

Development of the tangent linear and adjoint models of the global online chemical transport model MPAS-CO 2 v7.3

We describe the development of the tangent linear (TL) and adjoint models of the Model for Prediction Across Scales (MPAS)-CO 2 transport model, which is a global online chemical transport model developed upon the non-hydrostatic Model for Prediction Across Scales – Atmosphere (MPAS-A). The primary goal is to make the model system a valuable research tool for investigating atmospheric carbon transport and inverse modeling. First, we develop the TL code, encompassing all CO 2 transport processes within the MPAS-CO 2 forward model. Then, we construct the adjoint model using a combined strategy involving re-calculation and storage of the essential meteorological variables needed for CO 2 transport. This strategy allows the adjoint model to undertake a long-period integration with moderate memory demands. To ensure accuracy, the TL and adjoint models undergo vigorous verifications through a series of standard tests. The adjoint model, through backward-in-time integration, calculates the sensitivity of atmospheric CO 2 observations to surface CO 2 fluxes and the initial atmospheric CO 2 mixing ratio. To demonstrate the utility of the newly developed adjoint model, we conduct simulations for two types of atmospheric CO 2 observations, namely the tower-based in situ CO 2 mixing ratio and satellite-derived column-averaged CO 2 mixing ratio (X CO 2 ). A comparison between the sensitivity to surface flux calculated by the MPAS-CO 2 adjoint model with its counterpart from CarbonTracker–Lagrange (CT-L) reveals a spatial agreement but notable magnitude differences. These differences, particularly evident for X CO 2 , might be attributed to the two model systems' differences in the simulation configuration, spatial resolution, and treatment of vertical mixing processes. Moreover, this comparison highlights the substantial loss of information in the atmospheric CO 2 observations due to CT-L's spatial domain limitation. Furthermore, the adjoint sensitivity analysis demonstrates that the sensitivities to both surface flux and initial CO 2 conditions spread out throughout the entire Northern Hemisphere within a month. MPAS-CO 2 forward, TL, and adjoint models stand out for their calculation efficiency and variable-resolution capability, making them competitive in computational cost. In conclusion, the successful development of the MPAS-CO 2 TL and adjoint models, and their integration into the MPAS-CO 2 system, establish the possibility of using MPAS's unique features in atmospheric CO 2 transport sensitivity studies and in inverse modeling with advanced methods such as variational data assimilation.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1975

Developing processing techniques for Skylab data

The author has identified the following significant results. The effects of misregistration and the scan-line-straightening algorithm on multispectral data were found to be: (1) there is greatly increased misregistration in scan-line-straightening data over conic data; (2) scanner caused misregistration between any pairs of channels may not be corrected for in scan-line-straightened data; and (3) this data will have few pure field center pixels than will conic data. A program SIMSIG was developed implementing the signature simulation model. Data processing stages of the experiment were carried out, and an analysis was made of the effects of spatial misregistration on field center classification accuracy. Fifteen signatures originally used for classifying the data were analyzed, showing the following breakdown: corn (4 signatures), trees (2), brush (1), grasses, weeds, etc. (5), bare soil (1), soybeans (1), and alfalfa (1).

Nalepka, R. F.↗

NASA NTRS1975

Remote sensor digital image data analysis using the General Electric Image 100 analysis system (a study of analysis speed, cost, and performance)

The author has identified the following significant results. It was found that the high speed man machine interaction capability is a distinct advantage of the image 100; however, the small size of the digital computer in the system is a definite limitation. The system can be highly useful in an analysis mode in which it complements a large general purpose computer. The image 100 was found to be extremely valuable in the analysis of aircraft MSS data where the spatial resolution begins to approach photographic quality and the analyst can exercise interpretation judgements and readily interact with the machine.

Mcmurtry, G. J.↗

NASA NTRS1975

Snow cover monitoring by machine processing of multitemporal LANDSAT MSS data

LANDSAT frames were geometrically corrected and data sets from six different dates were overlaid to produce a 24 channel (six dates and four wavelength bands) data tape. Changes in the extent of the snowpack could be accurately and easily determined using a change detection technique on data which had previously been classified by the LARSYS software system. A second phase of the analysis involved determination of the relationship between spatial resolution or data sampling frequency and accuracy of measuring the area of the snowpack.

Luther, S. G.↗

NASA NTRS1979

Computational methods for analyzing the transmission characteristics of a beta particle magnetic analysis system

Computational methods were developed to study the trajectories of beta particles (positrons) through a magnetic analysis system as a function of the spatial distribution of the radionuclides in the beta source, size and shape of the source collimator, and the strength of the analyzer magnetic field. On the basis of these methods, the particle flux, their energy spectrum, and source-to-target transit times have been calculated for Na-22 positrons as a function of the analyzer magnetic field and the size and location of the target. These data are in studies requiring parallel beams of positrons of uniform energy such as measurement of the moisture distribution in composite materials. Computer programs for obtaining various trajectories are included.

Singh, J. J.↗

NASA NTRS1980

Stability analysis for laminar flow control, part 2

Topics covered include: (1) optimization of the numerics of the SALLY stability analysis code; (2) relation between temporal and spatial stability theory; (3) compressible flow stability calculations; (4) spectral methods for the boundary layer equations; and (5) numerical study of nonlinear, nonparallel stability of incompressible flows.

Orszag, S. A.↗

NASA NTRS1980

Orbital analysis for the upper atmosphere research satellite missions

An orbital analysis has been performed to define the spatial and temporal coverage capabilities of limb scanning experiments for meeting the science requirements for the upper atmosphere research satellite missions. Results indicate that a combination of solar occultation experiments and limb thermal emission experiments having azimuthal scan capability can provide good temporal and spatial coverage of the earth from a 600-km, 56-deg inclined orbit for the first satellite mission. Using a 70-deg inclined orbit for the second satellite mission will complement the first mission and provide complete global coverage with the two types of experiments.

Harrison, E. F.↗

NASA NTRS1983

Repeated-Measures Analysis of Image Data

It is suggested that using a modified analysis of variance procedure on data sampled systematically from a rectangular array of image data can provide a measure of homogeneity of means over that array in single directions and how variation in perpendicular directions interact. The modification of analysis of variance required to account for spatial correlation is described theoretically and numerically on simulated data.

Newton, H. J.↗

NASA NTRS1985

Scattering of acoustic waves into Tollmien-Schlichting waves by small streamwise variations in surface geometry

By using the triple-deck scaling of Stewartson (1969) and Messiter (1970) it is shown that small but relatively sudden surface geometry variations that produce only very weak static pressure variations can nevertheless produce strong, i.e. O(1), coupling between an externally imposed acoustic disturbance and a spatially growing Tollmien-Schlichting wave. The analysis provides a qualitative explanation of the Leehey and Shapiro (1979) boundary-layer receptivity measurements and is in good quantitative agreement with the Aizin and Poliakov (1979) experiment. It may also explain why small 'trip wires' can promote early transition.

Goldstein, M. E.↗

NASA NTRS1986

Turbulent motion in galactic H II regions

An investigation of radial velocities across the face of NGC 1499, NGC 7000, and S252 reveals that the fine-scale (turbulent) motions are well ordered from the limit of spatial resolution to the full size of the nebulae. As in higher spatial resolution studies of S142 and M17, analysis of the dispersion relation reveals that there is agreement with Kolmogorov theory (1941). However, study of the structure function reveals the same result as found by Roy and Joncas (1985), that the structure function increases with separation much more slowly than theoretically expected, calling into question the application of Kolmogorov theory. The Roy-Joncas result that the fine-scale motion seems to begin at about the sonic velocity are confirmed. It is shown that a condition exists of near equipartition of energies between fine-scale mass motion and thermal gas motion, which raises the question of a possible link.

Odell, C. R.↗

NASA NTRS1987

Computational and experimental investigation of cavity flowfields

This paper presents a computational and experimental investigation of supersonic flow past a cavity in a flat plate. The source of the particular interest in this problem is the ongoing study of the aerodynamic interference effects between a separating store and its bay in the parent body. An upwind relaxation scheme, utilizing flux vector splitting and line-Gauss-Seidel iterations, is used to solve Reynolds-averaged Navier-Stokes equations. Spatial discretizations of this two-dimensional analysis are based on implicit and finite-volume methods. Turbulence is modeled and shocks are captured. The flowfield of the symmetry plane at the half-width is computationally visualized and all flow properties are computed. Experimental tests are conducted in the Langley Unitary Plan Wind Tunnel to measure wall pressures and to capture schlieren photographs. Qualitative as well as quantitative data of computations and experiments agree very well. These two vehicles of investigation are merged to show open, closed and transitional cavity flow behaviors.

Baysal, O.↗

NASA NTRS1987

An evaluation of various forms of VAS retrievals in the analysis of a preconvective environment

VISSR Atmospheric Sounder (VAS) radiance data obtained over the continental United States on July 20, 1981 are used to evaluate a variety of VAS retrieval procedures and parameters in the qualitative analysis and forecasting of severe weather events. The particular case analyzed contains two significantly different mesoscale convective events in the central plains. Retrievals of temperature, dewpoint temperature, equivalent potential temperature, total column precipitable water, and lifted index are shown to be physically consistent in space and time and to compare well with available radiosonde data. The analysis of the VAS retrievals identified significant spatial gradients and temporal changes in the thermal and moisture fields, including times and locations between radiosonde observations.

Petersen, R. A.↗

NASA NTRS1988

Remote sensing information sciences research group

Research conducted under this grant was used to extend and expand existing remote sensing activities at the University of California, Santa Barbara in the areas of georeferenced information systems, matching assisted information extraction from image data and large spatial data bases, artificial intelligence, and vegetation analysis and modeling. The research thrusts during the past year are summarized. The projects are discussed in some detail.

Estes, John E.↗

NASA NTRS1990

Asymptotic modal analysis and statistical energy analysis

The sound field of a structural-acoustic enclosure was subject to experimental analysis and theoretical description in order to develop an efficient and accurate method for predicting sound pressure levels in enclosures such as aircraft fuselages. Asymptotic Modal Analysis (AMA) is the method under investigation. AMA is derived from classical modal analysis (CMA) by considering the asymptotic limit of the sound pressure level as the number of acoustic and/or structural modes approaches infinity. Using AMA, results identical to those of Statistical Energy Analysis (SEA) were obtained for the spatially-averaged sound pressure levels in the interior. AMA is systematically derived from CMA and therefore the degree of generality of the end result can be adjusted through the choice of appropriate simplifying assumptions. For example, AMA can be used to obtain local sound pressure levels at particular points inside the enclosure, or to include the effects of varying the size and/or location of the sound source. AMA theoretical results were compared with CMA theory and also with experiment for the case where the structural-acoustic enclosure is a rectangular cavity with part of one wall flexible and vibrating, while the rest of the cavity is rigid.

Dowell, Earl H.↗

NASA NTRS1990

Design and analysis of a Schwarzschild imaging multilayer X-ray microscope

Several Schwarzschild X-ray microscope optics were designed. Diffraction analysis indicates that better than 600 A spatial resolution in the object plane up to a 0.7 mm field of view can be achieved with 100 A radiation. Currently, a 20 x normal incidence multilayer X-ray microscope of 1.35 m overall length is being fabricated. Other microscope systems for use in conjunction with X-ray telescopes were also analyzed and designed. This paper reports on the results of these studies and the X-ray microscope fabrication effort.

Shealy, David L.↗

NASA NTRS1989

Development of a normal incidence multilayer, imaging X-ray microscope

This paper describes the design, analysis, and fabrication of a normal-incidence multilayer 20x Schwarzschild imaging X-ray microscope. The microscope is being fabricated using much of the technology implemented in the Multispectral Solar Telescope Array. Results of diffraction analysis show that better than 400 A spatial resolution in the object plane up to a 1-mm field of view can be achieved with 125 A radiation. Other microscope systems for use in conjunction with X-ray telescopes are analyzed and designed.

Shealy, David L.↗

NASA NTRS1990

Dynamics of quiescent prominences; Proceedings of the 117th Colloquium of IAU, Hvar, Yugoslavia, Sept. 25-29, 1989

Topics discussed include formation of a filament around a magnetic region, evolution of fine structures in a filament, the spatial distribution of prominence threads, high resolution analysis of quiescent prominences at NSO/Sacramento Peak Observatory, small-scale Doppler velocities in a quiescent prominence, Doppler velocity oscillations in quiescent prominences, oscillatory relaxation of an eruptive prominence, and matter flow velocities in an active region emission loop observed in H-alpha. Attention is also given to an automated procedure for measurement of prominence transverse velocities, the nonlinear evolution of magnetized filaments, thermal equilibrium of coronal loops and prominence formation, thermal instability in planar coronal strucutres, radiative transfer in cylindrical prominence threads, numerical simulation of a catastrophe model for prominence eruptions, and the law of evolution and destruction of solar prominences.

Ruzdjak, Vladimir↗