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At least 1,045 records · Page 58
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Observed and Simulated Variability of Droplet Spectral Dispersion in Convective Clouds Over the Amazon

Abstract In this study, the variability of the spectral dispersion of droplet size distributions (DSDs) in convective clouds is investigated. Analyses are based on aircraft measurements of growing cumuli near the Amazon basin, and on numerical simulations of an idealized ice‐free cumulus. In cleaner clouds, the relative dispersion , defined as the ratio of the standard deviation to the mean value of the droplet diameter, is negatively correlated with the ratio of the cloud water content ( ) to the adiabatic liquid water content ( ), while no strong correlation between and is seen in polluted clouds. Bin microphysics numerical simulations suggest that these contrasting behaviors are associated with the effect of collision‐coalescence in cleaner clouds, and secondary droplet activation in polluted clouds, in addition to the turbulent mixing of parcels that experienced different paths within the cloud. Collision‐coalescence simultaneously broadens the DSDs and decreases , explaining the inverse relationship between and in cleaner clouds. Secondary droplet activation broadens the DSDs but has little direct impact on . The combination of a rather modest DSD broadening due to weak collision‐coalescence with enhanced droplet activation in both diluted and highly undiluted cloud regions may contribute to maintain a relatively uniform within polluted clouds. These findings can be useful for parameterizing the shape parameter ( ) of gamma DSDs in bulk microphysics cloud‐resolving models. It is shown that emulating the observed relationship improves the estimation of the collision‐coalescence rate in bulk microphysics simulations compared to the bin simulations.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2017

Methods for Estimating 2D Cloud Size Distributions from 1D Observations

Abstract The two-dimensional (2D) size distribution of clouds in the horizontal plane plays a central role in the calculation of cloud cover, cloud radiative forcing, convective entrainment rates, and the likelihood of precipitation. Here, a simple method is proposed for calculating the area-weighted mean cloud size and for approximating the 2D size distribution from the 1D cloud-chord lengths measured by aircraft and vertically pointing lidar and radar. This simple method (which is exact for square clouds) compares favorably against the inverse Abel transform (which is exact for circular clouds) in the context of theoretical size distributions. Both methods also perform well when used to predict the size distribution of real clouds from a Landsat scene. When applied to a large number of Landsat scenes, the simple method is able to accurately estimate the mean cloud size. As a demonstration, the methods are applied to aircraft measurements of shallow cumuli during the Routine ARM Aerial Facility (AAF) Clouds with Low Optical Water Depths (CLOWD) Optical Radiative Observations (RACORO) campaign, which then allow for an estimate of the true area-weighted mean cloud size.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2019

Understanding and Constraining the Midlatitude Cloud Optical Depth Feedback in Climate Models (Final Report)

The objectives of this investigation are to provide a deeper understanding of the brightening of middle and high latitude clouds that occurs in many climate models as the climate warms, and to better understand why models give varying estimates of the strength of this negative feedback. The investigation may also provide new information on why models are deficient in their simulation of the present day clouds in these regions. The analysis will reveal which models simulate current clouds most realistically in the regions of interest, and relate this to the strength of the cloud feedbacks in the models. This will improve the uncertainty quantification of climate simulations and will provide theoretical understanding potentially leading to increased reliability of climate change projections. This will enhance the predictive understanding of the Earth system by analyzing the natural and anthropogenic components of global climate change in models. The primary methods involve the study of the clouds in the suite of CMIP5 model climate simulations and comparison of clouds in climate simulations with data from satellite measurement systems, with a particular emphasis on mixed-phase cloud physics, for which ice and water are present simultaneously. State-of-the-art climate model feedback analysis will be combined with new and more comprehensive observations of clouds available from modern measurement systems. Novel use of model simulations in combination with observations enables a deeper understanding of the role of clouds in climate change. Metrics that facilitate model-to-model and model-to-observation comparisons related to mixed-phase cloud physics will be developed and used to highlight challenges and opportunities for improving the state-of-the-science models. This investigation is a collaboration between the University of Washington, where the data work is concentrated and LLNL where the model data and the tools and expertise to do cloud feedback analysis are located. The grant supported the work of 3 different graduate students at different times (McCoy, Wall and Berry) Post-doctoral researcher Blaž Gasparini was also partially supported on this grant and led our collaboration with PNNL scientists. PNNL scientists also collaborated in the work of graduate student Wall (Po-Lun Ma). The main results of our research efforts are reported in 6 papers and 1 book chapter that were supported by this grant.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

Cloud Processing of Aerosol during SAIL Field Campaign Report

Globally, on average, the release rate of aerosols from clouds is estimated to be about 6,000 Tg/yr and an aerosol particle is estimated to experience about three cloud cycles. Cloud processing of aerosol produces aerosols that have dramatically different physicochemical properties compared to their original form. Cloud processing may transform particles to efficient cloud condensation nuclei (CCN) or ice nucleating particles (INP) that can further participate in cloud formation. We investigated cloud processing of aerosol during the U.S. Department of Energy (DOE)’s Atmospheric Radiation Measurement (ARM) Surface Atmosphere Integrated Field Laboratory (SAIL) field campaign using multi-modal offline analysis techniques available at DOE’s Environmental Molecular Sciences Laboratory (EMSL). The main scientific aim of this project was to understand the processes that transform aerosols (chemically, and physically), and influence aerosol-cloud interactions. Aerosol particles undergo significant modifications due to warm (cloud droplets) and cold cloud (ice crystals) processing. Cloud processing of aerosol has important effects on the atmospheric aerosol number and mass concentration, size distribution, phase separation, and chemical composition.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

Measurements and Analyses to Enable Science for the Eastern Pacific Cloud Aerosol Precipitation Experiment (EPCAPE)

Coastal cities provide the opportunity to characterize the substantial effects of manmade particles on marine cloud properties and processes. La Jolla lies to the north of San Diego, California, but it is often about a day directly downwind of the major pollution sources located in the ports of Los Angeles and Long Beach. The large dynamic range of aerosol particle concentrations combined with the multi-hour to multi-day persistence of stratocumulus cloud layers makes the site ideal for investigating the seasonal changes in cloud and aerosol properties as well as the quantitative relationships between cloud and aerosol properties. The Eastern Pacific Cloud Aerosol Precipitation Experiment (EPCAPE) characterized the extent, radiative properties, aerosol interactions, and precipitation characteristics of stratocumulus clouds in the Eastern Pacific across all four seasons at two coastal sites in La Jolla. This project was designed to enhance and expand the scientific uses of the ARM AMF1 measurements from EPCAPE. The goal was to ensure meaningful observations were collected that would enable science. The project included the following objectives: (1) Reviewing the ARM AMF1 measurements [ARM, 2021a; b] and circulating a summary of the measurements each week, (2) Comparing AMF1 measurements to those provided by collaborators (including filter measurements at the pier), (3) Collecting and analyzing filter samples from Scripps Pier by Fourier Transform Infrared spectroscopy (FTIR) and X-ray Fluorescence (XRF), (4) Assisting in operations of instruments provided by Guest PIs when possible, and (5) Providing an initial compilation of EPCAPE aerosol and cloud seasonal differences. The expected outcomes of these objectives were enhanced proposals and publications using EPCAPE measurements by helping to identify instrument issues, expanded data access and awareness by distributing weekly plots and related summaries, improved source-related attribution of aerosols with elemental tracers, additional observations provided by Guest PIs, and accelerated ACI studies enabled by the compiled seasonal summaries of aerosol and cloud properties. Three examples of the science enabled by this project are findings that (i) aerosol and cloud aqueous production contributes more than half of sulfate particle mass concentration, (ii) upwind sources make chemical composition very similar at nearby sites despite local differences in meteorology, and (iii) most of the large mass concentration of semi-volatile organic components is co-emitted and co-evaporated with nitrate. Together these findings illustrate how ARM extended field campaigns in coastal regions can be used to constrain ACI processes with direct observations. By using the unique ARM suite of cloud radiative products in addition to the measured aerosol properties at a coastal location, we were able to address the more specific question of which aerosol particles cause how much of the effects on clouds. Identifying this signature in coastal areas provides an opportunity to test the representation of aerosol sources by global models in a range of clean and urban-influenced conditions.

Russell, Lynn [Univ. of California, San Diego, CA ↗
DOE OSTI2026

3D Cloud Aerosol Precipitation Experiment at kennaook Cape Grim (3D-CAPE-k) Field Campaign Report

The objective of this campaign was to complement the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) User Facility’s Cloud And Precipitation Experiment at kennaook (CAPE-k) in northwest Tasmania by deploying scanning, fixed pointing angle, and in situ aerosol, cloud, and precipitation remote-sensing instruments during the last six months of the experiment. These instruments provided a three-dimensional (3D) context to the second ARM Mobile Facility (AMF2) vertically pointing observations collected at the kennaook Cape Grim (KCG) site and captured a portion of the life cycle of the clouds before and after the passage over the AMF2 vertical column. These 3D cloud measurements will be used in the near future to 1) investigate how the vertical profiles of aerosol and cloud properties are representative of the broader area and how these properties evolve during the portion of the cloud life cycle captured by the scanning instruments, 2) quantify how accurate the cloud fraction derived with assumptions from vertically pointing observations are compared with direct 3D cloud fraction measurements, 3) evaluate cloud fraction and liquid water path in the Australian Community Climate and Earth-System Simulator–Convective-scale (ACCESS-C) forecast model, and 4) evaluate aerosol and cloud products from the European Space Agency/Japanese Aerospace Exploration Agency (ESA/JAXA) Earth Cloud Aerosol Radiation Explorer (EarthCARE) mission using the scanning measurements, offering more chances of exact collocation, thereby complementing the statistical approach we are planning to employ with AMF2 observations for that same purpose.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2019

H i Clouds in LITTLE THINGS Dwarf Irregular Galaxies

We identify 814 discrete H i clouds in 40 dwarf irregular galaxies from the LITTLE THINGS survey using an automated cloud-finding algorithm. The cloud masses range from ∼10{sup 3} to 10{sup 7} M {sub ⊙}, have a surface density averaged over all of the clouds of ∼9.65 M {sub ⊙} pc{sup −2}, and constitute 2%–53% of the total H i mass of the host galaxy. For individual clouds, the mass including He varies with cloud radius as log M{sub gas}=(2.11±0.04) × log R{sub cl} +(0.78±0.08) and the internal velocity dispersion varies as log V{sub disp}=0.5 × log R{sub cl}−0.57±0.21. The H i clouds tend to be in the outer regions of the galaxies, with 72% of the galaxies having more than 70% of their clouds outside one disk scale length and 32% of the galaxies having more than 50% of their clouds outside the radius encircling the H ii emission. Thirty-six percent of the clouds are essentially non-self-gravitating from H i alone, with a virial parameter that exceeds α {sub vir} ∼ 10, and 5% have α {sub vir} ≤ 2. We estimate the missing molecular mass, based on the total star formation rate and a typical molecular consumption time of 2 Gyr, as observed in CO-rich galaxies. The resulting molecular fraction has a value averaged over the galaxies of 0.23 and correlates with both the surface density of star formation and the fraction of H i clouds in the outer regions. We conclude that a significant fraction of the inner parts of these dwarf galaxy disks is in the form of dark molecular gas, and that this fraction could be high enough to make the inner disks mildly gravitationally unstable as a precursor to star formation.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2017

Cloud Structure of Three Galactic Infrared Dark Star-forming Regions from Combining Ground- and Space-based Bolometric Observations

We have modified the iterative procedure introduced by Lin et al., to systematically combine the submillimeter images taken from ground-based (e.g., CSO, JCMT, APEX) and space (e.g., Herschel, Planck) telescopes. We applied the updated procedure to observations of three well-studied Infrared Dark Clouds (IRDCs): G11.11−0.12, G14.225−0.506, and G28.34+0.06, and then performed single-component, modified blackbody fits to each pixel to derive ∼10″ resolution dust temperature and column density maps. The derived column density maps show that these three IRDCs exhibit complex filamentary structures embedded with rich clumps/cores. We compared the column density probability distribution functions (N-PDFs) and two-point correlation (2PT) functions of the column density field between these IRDCs with several OB-cluster-forming regions. Based on the observed correlation between the luminosity-to-mass ratio and the power-law index of the N-PDF, and complementary hydrodynamical simulations for a 10{sup 4} M{sub ⊙} molecular cloud, we hypothesize that cloud evolution can be better characterized by the evolution of the (column) density distribution function and the relative power of dense structures as a function of spatial scales, rather than merely based on the presence of star-forming activity. An important component of our approach is to provide a model-independent quantification of cloud evolution. Based on the small analyzed sample, we propose four evolutionary stages, namely, cloud integration, stellar assembly, cloud pre-dispersal, and dispersed cloud. The initial cloud integration stage and the final dispersed cloud stage may be distinguished from the two intermediate stages by a steeper than −4 power-law index of the N-PDF. The cloud integration stage and the subsequent stellar assembly stage are further distinguished from each other by the larger luminosity-to-mass ratio (>40 L{sub ⊙}/M{sub ⊙}) of the latter. A future large survey of molecular clouds with high angular resolution may establish more precise evolutionary tracks in the parameter space of N-PDF, 2PT function, and luminosity-to-mass ratio.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2018

The efficacy of aerosol–cloud radiative perturbations from near-surface emissions in deep open-cell stratocumuli

Aerosol–cloud radiative effects are determined and quantified in simulationsof deep open-cell stratocumuli observed during the VAMOS Ocean-Cloud-Atmosphere-LandStudy Regional Experiment (VOCALS-REx) campaign offthe west coast of Chile. The cloud deck forms in a boundarylayer 1.5 km deep, with cell sizes reaching 50 km in diameter. Global databases of shiptracks suggest that these linear structures are seldom found in boundarylayers this deep. Here, we quantify the changes in cloud radiative propertiesto a continuous aerosol point source moving along a fixed emission linereleasing 10 17 particles per second. We show that a spatially coherentcloud perturbation is not evident along the emission line. Yet our modelsimulates an increase in domain-mean all-sky albedo of 0.05, corresponding toa diurnally averaged cloud radiative effect of 20 W m -2 , given theannual mean solar insolation at the VOCALS-REx site. Therefore, markedchanges in cloud radiative properties in precipitating deep open cells may bedriven by anthropogenic near-surface aerosol perturbations, such as thosegenerated by ships.Furthermore, we demonstrate that these changes in cloud radiative propertiesare masked by the naturally occurring variability within the organised cloudfield. A clear detection and attribution of cloud radiative effects to aperturbation in aerosol concentrations becomes possible when sub-filtering ofthe cloud field is applied, using the spatio-temporal distribution of theaerosol perturbation. Therefore, this work has implications for the detectionand attribution of effective cloud radiative forcing in marine stratocumuli,which constitutes one of the major physical uncertainties within the climatesystem. Our results suggest that ships may sometimes have a substantialradiative effect on marine clouds and albedo, even when ship tracks are notreadily visible.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2019

Mixed-phase orographic cloud microphysics during StormVEx and IFRACS

Wintertime mixed-phase orographic cloud (MPC) measurements were conducted at the Storm Peak Laboratory (SPL) during the Storm Peak Lab Cloud Property Validation Experiment (StormVEx) and Isotopic Fractionation in Snow (IFRACS) programs in 2011 and 2014, respectively. The data include 92 h of simultaneous measurements of supercooled liquid cloud droplet and ice particle size distributions (PSDs). Average cloud droplet number concentration (CDNC), droplet size (NMD), and liquid water content (LWC) were similar in both years, while ice particle concentration (Ni) and ice water content (IWC) were higher during IFRACS. The consistency of the liquid cloud suggests that SPL is essentially a cloud chamber that produces a consistent cloud under moist, westerly flow during the winter. A variable cloud condensation nuclei (CCN)-related inverse relationship between CDNC and NMD strengthened when the data were stratified by LWC. Some of this variation is due to changes in cloud base height below SPL. While there was a weak inverse correlation between LWC and IWC in the data as a whole, a stronger relationship was demonstrated for a case study on 9 February 2014 during IFRACS. A minimum LWC of 0.05 g m–3 showed that the cloud was not completely glaciated on this day. Erosion of the droplet distribution at high IWC was attributed to the Wegener–Bergeron–Findeisen process as the high IWC was accompanied by a 10-fold increase in Ni. A relationship between large cloud droplet concentration (25–35 µm) and small ice particles (75–200 µm) under cold (<–8 °C) but not warm (>–8 °C) conditions during IFRACS suggests primary ice particle production by contact or immersion freezing. The effect of blowing snow was evaluated from the relationship between wind speed and Ni and by comparing the relative (percent) ice particle PSDs at high and low wind speeds. These were similar, contrary to expectation for blowing snow. However, the correlation between wind speed and ice crystal concentration may support this explanation for high crystal concentrations at the surface. Secondary processes could have contributed to high crystal concentrations but there was no direct evidence to support this. Further experimental work is needed to resolve these issues.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

Impacts of long-range transport of aerosols on marine-boundary-layer clouds in the eastern North Atlantic

Vertical profiles of aerosols are inadequately observed and poorly represented in climate models, contributing to the current large uncertainty associated with aerosol–cloud interactions. The US Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) Aerosol and Cloud Experiments in the Eastern North Atlantic (ACE-ENA) aircraft field campaign near the Azores islands provided ample observations of vertical distributions of aerosol and cloud properties. Here we utilize the in situ aircraft measurements from the ACE-ENA and ground-based remote-sensing data along with an aerosol-aware Weather Research and Forecast (WRF) model to characterize the aerosols due to long-range transport over a remote region and to assess their possible influence on marine-boundary-layer (MBL) clouds. The vertical profiles of aerosol and cloud properties measured via aircraft during the ACE-ENA campaign provide detailed information revealing the physical contact between transported aerosols and MBL clouds. The European Centre for Medium-Range Weather Forecasts Copernicus Atmosphere Monitoring Service (ECMWF-CAMS) aerosol reanalysis data can reproduce the key features of aerosol vertical profiles in the remote region. The cloud-resolving WRF sensitivity experiments with distinctive aerosol profiles suggest that the transported aerosols and MBL cloud interactions (ACIs) require not only aerosol plumes to get close to the marine-boundary-layer top but also large cloud top height variations. Based on those criteria, the observations show that the occurrence of ACIs involving the transport of aerosol over the eastern North Atlantic (ENA) is about 62 % in summer. For the case with noticeable long-range-transport aerosol effects on MBL clouds, the susceptibilities of droplet effective radius and liquid water content are -0.11 and +0.14, respectively. When varying by a similar magnitude, aerosols originating from the boundary layer exert larger microphysical influence on MBL clouds than those entrained from the free troposphere.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2018

Exploring aerosol cloud interaction using VOCALS-REx aircraft measurements

In situ aircraft measurements during the VAMOS Ocean–Cloud–Atmosphere–Land Study-Regional Experiment (VOCALS-REx) field campaign are employed to study the interaction between aerosol and stratocumulus over the southeast Pacific Ocean, as well as entrainment process near the top of stratocumulus and its possible impacts on aerosol–cloud interaction. Our analysis suggest that the increase of liquid water content (LWC) is mainly contributed by cloud droplet number concentration (Nd) instead of effective radius of cloud droplets in the polluted case, in which more droplets form with smaller size, while the opposite is true in the clean case. By looking into the influences of dynamical conditions and aerosol microphysical properties on the cloud droplet formation, it is confirmed that cloud droplets are more easily to form under the conditions with large vertical velocity and aerosol size. An increase in aerosol concentration tends to increase both Nd and relative dispersion (ϵ), while an increase in vertical velocity (w) often increases Nd but decreases ϵ. After constraining the differences of cloud dynamics, positive correlation between ϵ and Nd become stronger, implying that perturbations of w could weaken the influence of aerosol on ϵ, and hence may result in an underestimation of aerosol dispersion effect. The difference of cloud microphysical properties between entrainment and non-entrainment zones confirms that the entrainment-mixing mechanism is predominantly extreme inhomogeneous in the stratocumulus that capped by a sharp inversion, namely the entrainment reduces Nd and LWC by 28.9 % and 24.8 % on average, respectively, while the size of droplets is relatively unaffected. In entrainment zone, smaller aerosols and drier air entrained from the top induce less cloud droplet with respect to total in-cloud particles (0.56 ± 0.22) than the case in non-entrainment zone (0.73 ± .0.13) by inhibiting aerosol activation and promoting cloud droplets evaporation.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Sunlight-absorbing aerosol amplifies the seasonal cycle in low-cloud fraction over the southeast Atlantic

Abstract. The mean altitude of the smoke loading over the southeast Atlantic moves from the boundary layer in July to the free troposphere by October. This study details the month-by-month changes in cloud properties and the large-scale environment as a function of the biomass burning aerosol loading at Ascension Island (8∘ S, 14.5∘ W) from July to October, based on island measurements, satellite retrievals, and reanalysis. In July and August, the smoke loading predominantly varies within the boundary layer. During both months, the low-cloud fraction is less and is increasingly cumuliform when more smoke is present, with the exception of a late morning boundary layer deepening that encourages a short-lived cloud development. The meteorology varies little, suggesting aerosol–cloud interactions explain the cloudiness changes. September marks a transition month during which midlatitude disturbances can intrude into the Atlantic subtropics, constraining the free tropospheric aerosol closer to the African coast. Stronger boundary layer winds on cleaner days help deepen, dry, and cool much of the marine boundary layer compared to that on days with high smoke loadings, with stratocumulus reducing everywhere but at the northern deck edge. The September free troposphere is better mixed on smoky days compared to October. Longwave cooling rates, generated by a sharp water vapor gradient at the aerosol layer top, encourage a small-scale vertical mixing that could help maintain the well-mixed smoky September free troposphere. The October meteorology primarily varies as a function of the strength of the free tropospheric winds advecting aerosol offshore. The free tropospheric aerosol loading is less than in September, and the moisture variability is greater. Low-level clouds increase and are more stratiform in October when the smoke loadings are higher. The increased free tropospheric moisture can help sustain the clouds through a reduction in evaporative drying during cloud-top entrainment. Enhanced subsidence above the coastal upwelling region, increasing cloud droplet number concentrations, may further prolong cloud lifetime through microphysical interactions. Reduced subsidence underneath stronger free tropospheric winds at Ascension Island supports slightly higher cloud tops during smokier conditions. Overall, the monthly changes in the large-scale aerosol and moisture vertical structure act to amplify the seasonal cycle in low-cloud amount and morphology. This is climatically important, as cloudiness changes dominate changes in the top-of-atmosphere radiation budget.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Contrasting characteristics of open- and closed-cellular stratocumulus cloud in the eastern North Atlantic

Abstract. Extensive regions of marine boundary layer cloud impact the radiative balance through their significant shortwave albedo while having little impact on outgoing longwave radiation. Despite this importance, these cloud systems remain poorly represented in large-scale models due to difficulty in representing the processes that drive their life cycle and coverage. In particular, the mesoscale organization and cellular structure of marine boundary clouds have important implications for the subsequent cloud feedbacks. In this study, we use long-term (2013–2018) observations from the Atmospheric Radiation Measurement (ARM) Facility's Eastern North Atlantic (ENA) site on Graciosa Island, Azores, Portugal, to identify cloud cases with open- or closed-cellular organization. More than 500 h of each organization type are identified. The ARM observations are combined with reanalysis and satellite products to quantify the cloud, precipitation, aerosol, thermodynamic, and large-scale synoptic characteristics associated with these cloud types. Our analysis shows that both cloud organization populations occur during similar sea surface temperature conditions, but the open-cell cases are distinguished by stronger cold-air advection and large-scale subsidence compared to the closed-cell cases, consistent with their formation during cold-air outbreaks. We also find that the open-cell cases were associated with deeper boundary layers, stronger low-level winds, and higher rain rates compared to their closed-cell counterparts. Finally, raindrops with diameters larger than 1 mm were routinely recorded at the surface during both populations, with a higher number of large drops during the open-cellular cases. The similarities and differences noted herein provide important insights into the environmental and cloud characteristics during varying marine boundary layer cloud mesoscale organization and will be useful for the evaluation of model simulations for ENA marine clouds.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

Do Arctic mixed-phase clouds sometimes dissipate due to insufficient aerosol? Evidence from comparisons between observations and idealized simulations

Abstract. Mixed-phase clouds are ubiquitous in the Arctic. These clouds can persist for days and dissipate in a matter of hours. It is sometimes unknown what causes this sudden dissipation, but aerosol–cloud interactions may be involved. Arctic aerosol concentrations can be low enough to affect cloud formation and structure, and it has been hypothesized that, in some instances, concentrations can drop below some critical value needed to maintain a cloud. We use observations from a Department of Energy ARM site on the northern slope of Alaska at Oliktok Point (OLI), the Arctic Summer Cloud Ocean Study (ASCOS) field campaign in the high Arctic Ocean, and the Integrated Characterisation of Energy, Clouds, Atmospheric state, and Precipitation at Summit – Aerosol Cloud Experiment (ICECAPS-ACE) project at the NSF (National Science Foundation) Summit Station in Greenland (SMT) to identify one case per site where Arctic boundary layer clouds dissipated coincidentally with a decrease in surface aerosol concentrations. These cases are used to initialize idealized large eddy simulations (LESs) in which aerosol concentrations are held constant until, at a specified time, all aerosols are removed instantaneously – effectively creating an extreme case of aerosol-limited dissipation which represents the fastest a cloud could possibly dissipate via this process. These LESs are compared against the observed data to determine whether cases could, potentially, be dissipating due to insufficient aerosol. The OLI case's observed liquid water path (LWP) dissipated faster than its simulation, indicating that other processes are likely the primary drivers of the dissipation. The ASCOS and SMT observed LWP dissipated at similar rates to their respective simulations, suggesting that aerosol-limited dissipation may be occurring in these instances. We also find that the microphysical response to this extreme aerosol forcing depends greatly on the specific case being simulated. Cases with drizzling liquid layers are simulated to dissipate by accelerating precipitation when aerosol is removed while the case with a non-drizzling liquid layer dissipates quickly, possibly glaciating via the Wegener–Bergeron–Findeisen (WBF) process. The non-drizzling case is also more sensitive to ice-nucleating particle (INP) concentrations than the drizzling cases. Overall, the simulations suggest that aerosol-limited cloud dissipation in the Arctic is plausible and that there are at least two microphysical pathways by which aerosol-limited dissipation can occur.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Rapid saturation of cloud water adjustments to shipping emissions

Abstract. Human aerosol emissions change cloud properties by providing additional cloud condensation nuclei. This increases cloud droplet numbers, which in turn affects other cloud properties like liquid-water content and ultimately cloud albedo. These adjustments are poorly constrained, making aerosol effects the most uncertain part of anthropogenic climate forcing. Here we show that cloud droplet number and water content react differently to changing emission amounts in shipping exhausts. We use information about ship positions and modeled emission amounts together with reanalysis winds and satellite retrievals of cloud properties. The analysis reveals that cloud droplet numbers respond linearly to emission amount over a large range (1–10 kg h−1) before the response saturates. Liquid water increases in raining clouds, and the anomalies are constant over the emission ranges observed. There is evidence that this independence of emissions is due to compensating effects under drier and more humid conditions, consistent with suppression of rain by enhanced aerosol. This has implications for our understanding of cloud processes and may improve the way clouds are represented in climate models, in particular by changing parameterizations of liquid-water responses to aerosol.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

Understanding aerosol–cloud interactions using a single-column model for a cold-air outbreak case during the ACTIVATE campaign

Marine boundary layer clouds play a critical role in Earth's energy balance. Their microphysical and radiative properties are highly impacted by ambient aerosols and dynamic forcings. In this study, we evaluate the representation of these clouds and related aerosol–cloud interaction processes in the single-column version of the E3SM climate model (SCM) against field measurements collected during the NASA ACTIVATE campaign over the western North Atlantic, as well as intercompare results with high-resolution process level models. We show that E3SM SCM reproduces the macrophysical properties of post-frontal boundary layer clouds in a cold-air outbreak (CAO) case well. However, it generates fewer but larger cloud droplets compared to aircraft measurements. Further sensitivity tests show that the underestimation of both aerosol number concentration and vertical velocity variance contributes to this bias. Aerosol–cloud interactions are examined by perturbing prescribed aerosol properties in E3SM SCM with fixed dynamics. Higher aerosol number concentration or hygroscopicity leads to more numerous but smaller cloud droplets, resulting in a stronger cooling via shortwave cloud forcing. This apparent Twomey effect is consistent with prior climate model studies. The cloud liquid water path shows a weakly positive relation with cloud droplet number concentration due to precipitation suppression. This weak aerosol effect on cloud macrophysics may be attributed to the dominant impact of strong dynamical forcing associated with the CAO. Our findings indicate that the SCM framework is a key tool to bridge the gap between climate models, process level models, and field observations to facilitate process level understanding.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Version 4 CALIPSO Imaging Infrared Radiometer ice and liquid water cloud microphysical properties – Part I: The retrieval algorithms

Following the release of the version 4 Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) data products from the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) mission, a new version (version 4; V4) of the CALIPSO Imaging Infrared Radiometer (IIR) Level 2 data products has been developed. The IIR Level 2 data products include cloud effective emissivities and cloud microphysical properties such as effective diameter and ice or liquid water path estimates. Dedicated retrievals for water clouds were added in V4, taking advantage of the high sensitivity of the IIR retrieval technique to small particle sizes. This paper (Part I) describes the improvements in the V4 algorithms compared to those used in the version 3 (V3) release, while results will be presented in a companion (Part II) paper. The IIR Level 2 algorithm has been modified in the V4 data release to improve the accuracy of the retrievals in clouds of very small (close to 0) and very large (close to 1) effective emissivities. To reduce biases at very small emissivities that were made evident in V3, the radiative transfer model used to compute clear-sky brightness temperatures over oceans has been updated and tuned for the simulations using Modern-Era Retrospective analysis for Research and Applications version 2 (MERRA-2) data to match IIR observations in clear-sky conditions. Furthermore, the clear-sky mask has been refined compared to V3 by taking advantage of additional information now available in the V4 CALIOP 5 km layer products used as an input to the IIR algorithm. After sea surface emissivity adjustments, observed and computed brightness temperatures differ by less than ±0.2 K at night for the three IIR channels centered at 08.65, 10.6, and 12.05 µm, and inter-channel biases are reduced from several tens of Kelvin in V3 to less than 0.1 K in V4. We have also improved retrievals in ice clouds having large emissivity by refining the determination of the radiative temperature needed for emissivity computation. The initial V3 estimate, namely the cloud centroid temperature derived from CALIOP, is corrected using a parameterized function of temperature difference between cloud base and top altitudes, cloud absorption optical depth, and CALIOP multiple scattering correction factor. As shown in Part II, this improvement reduces the low biases at large optical depths that were seen in V3 and increases the number of retrievals. As in V3, the IIR microphysical retrievals use the concept of microphysical indices applied to the pairs of IIR channels at 12.05 and 10.6 µm and at 12.05 and 08.65 µm. The V4 algorithm uses ice look-up tables (LUTs) built using two ice habit models from the recent “TAMUice2016” database, namely the single-hexagonal-column model and the eight-element column aggregate model, from which bulk properties are synthesized using a gamma size distribution. Four sets of effective diameters derived from a second approach are also reported in V4. Here, the LUTs are analytical functions relating microphysical index applied to IIR channels 12.05 and 10.6 µm and effective diameter as derived from in situ measurements at tropical and midlatitudes during the Tropical Composition, Cloud, and Climate Coupling (TC4) and Small Particles in Cirrus Science and Operations Plan (SPARTICUS) field experiments.

54 ENVIRONMENTAL SCIENCES↗