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At least 1,045 records · Page 58

Passive Measurement of Organic-Scintillator Neutron Signatures for Nuclear Safeguards Applications

At nuclear facilities, domestically and internationally, most measurement systems used for nuclear materials’ control and accountability rely on He-3 detectors. Due to resource shortages, alternatives to He-3 systems are needed. This paper presents preliminary simulation and experimental efforts to develop a fast-neutron-multiplicity counter based on liquid organic scintillators. This mission also provides the opportunity to broaden the capabilities of such safeguards measurement systems to improve current neutron-multiplicity techniques and expand the scope to encompass advanced nuclear fuels.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Thermal Variance Investigation and Scintillation Mechanisms of Cs 2 LiLaBr 6-x Cl x :Ce (CLLBC) and Cs 2 LiYBr 6 :Ce (CLYB)

We perform an investigation into the scintillation processes and performance of elpasolites Cs 2 LiLaBr 6-x Cl x :Ce (CLLBC) and Cs 2 LiYBr 6 :Ce (CLYB) using a thermal cycle over a range of -20 to +50º C. At 10º increments, we acquire data with both a waveform digitizer and charge-integrating electronics. We identify decay components and evaluate decay times, thermal neutron gamma-equivalent energy (GEE), and pulse shape discrimination (PSD) performance. Results are compared to common Cs 2 LiYCl 6 :Ce (CLYC).

36 MATERIALS SCIENCE↗

Evaluation, Refurbishment, and Characterization of Fast Neutron Scintillators for the TREAT Fuel Motion Monitoring System

This paper details work being performed at the Idaho National Laboratory (INL) to evaluate, refurbish, and characterize proton-recoil scintillation (PRS) detectors utilized in a 360 channel array for the measurement of fast neutrons in a standalone system historically called a hodoscope located in the Transient Reactor Test Facility (TREAT). The TREAT hodoscope serves as the primary Fuel Motion Monitoring System for documenting real time fuel displacement during transient experiments. The detectors in the hodoscope have stood dormant for over 20 years and significant degradation must be addressed before the system can be brought back to operational status. The refurbishment process begins by decoupling the PRS from their matched photo multiplier tubes (PMTs) and treating the PRS with ethanol. This process cleans the surfaces, removing paint and legacy labels/ markings. During this procedure many physical variations can be observed. After cleaning, the PRS are physically measured using a digital caliper and the dimensions documented. Following this, a well-controlled 280nm LED light source is used to stimulate the PRS to produce an emission spectrum inside an integration sphere. This emission spectrum is then measured using a UV enhanced optical spectrometer. Spectral measurements are recorded from 185 nm to 580 nm in 0.4 nm steps. The PRS are then lightly sanded on the non-PMT mating surfaces and painted with commercially available reflective paint. A final emission spectrum is recorded for each PRS after painting.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Scintillator Evaluations: Long-Range Blur

Presentation describes evaluations of LYSO and long range blur on a Platts flash source, including source simulation, scintillator simulation, long range blur in monolithic LYSO, and data comparison.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

A prototype scintillating-fibre tracker for the cosmic-ray muon tomography of legacy nuclear waste containers

A prototype scintillating-fibre detector system has been developed at the University of Glasgow in collaboration with the UK National Nuclear Laboratory (NNL) for the nondestructive assay of UK legacy nuclear waste containers. This system consists of two tracking modules above, and two below, the container under interrogation. Each module consists of two orthogonal planes of 2 mm-pitch fibres yielding one space point. Per plane, 128 fibres are read out by a single Hamamatsu H8500 64-channel MAPMT with two fibres multiplexed onto each pixel. A dedicated mapping scheme has been developed to avoid space point ambiguities and retain the high spatial resolution provided by the fibres. The configuration allows the reconstruction of the incoming and scattered muon trajectories, thus enabling the container content, with respect to atomic number Z, to be determined. Results are shown from experimental data collected for high-Z objects within an air matrix and, for the first time, within a shielded, concrete-filled container. These reconstructed images show clear discrimination between the low, medium and high-Z materials present, with dimensions and positions determined with sub-centimetre precision. (authors)

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Counting neutrons from the spontaneous fission of {sup 238}U using scintillation detectors and mixed field analysers

It is well documented that {sup 238}U decays by spontaneous fission, and that it is the main component of most nuclear fuels. As nuclear fuels are largely classed as Special Nuclear Material (SNM), they have to be fully accounted for by owners and processing facilities. One possible method for verifying declared amounts of SNM is to count the spontaneous neutrons produced from {sup 238}U. Using four EJ-309 liquid scintillation detectors and a mixed field analyser, spontaneous neutrons from 16.4 g of depleted uranium (0.3% enrichment) have been assayed. The assay method shows promising results and this proof of principle will be researched further in order for it to be applied in an industrial setting. (authors)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Nuisance Alarm Reductions In Organic Scintillation Detector-Based Radiation Portal Monitors

A worldwide system of radiation portal monitors (RPMs) detects and deters the smuggling of special nuclear material (SNM) and other radiological sources that could be used by terrorist organizations in an improvised nuclear device or a radiological dispersal device. Nuisance alarms from non-SNM sources of radiation, however, account for the vast majority of RPM radiation alarms. We present research on a liquid organic scintillation detector-based RPM that reduces the impact of nuisance alarms through on-the- fly radionuclide identification. (authors)

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Characterization and Evaluation of Scintillating Fiber System Components

Idaho National Laboratory is studying long scintillation fibers (SF) in a project called “TRIPWIRE” which aims to verify containment in inaccessible nuclear waste repositories. This system will continuously monitor ionizing radiation, electromagnetic fields, and seismic activity in the vicinity of nuclear waste. Previous experiments have determined a better alternative to long SF is to couple shorter SF to kilometer scale optical fiber (OF) to reach electronics far outside of the repository. Minor signal attenuation from coupling these fibers has been observed using optical spectrometry. This experiment characterized two photomultiplier tubes (PMT) to reduce this loss by matching their spectral response characteristics to the SF’s emission spectrum. The experiment created a comparison between the two PMTs showing results that suggest other characteristics are playing a major role in improving signal attenuation when the SF is coupled to OF.

98 - NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL↗

Joint measurement of the atmospheric muon flux through the Puy de Dome volcano with plastic scintillators and Resistive Plate Chambers detectors

The muographic imaging of volcanoes relies on the measured transmittance of the atmospheric muon flux through the target. An important bias affecting the result comes from background contamination mimicking a higher transmittance. The MU-RAY and TOMUVOL collaborations measured independently in 2013 the atmospheric muon flux transmitted through the Puy de Dôme volcano using their early prototype detectors, based on plastic scintillators and on Glass Resistive Plate Chambers, respectively. These detectors had three (MU-RAY) or four (TOMUVOL) detection layers of 1 m 2 each, tens (MU-RAY) or hundreds (TOMUVOL) of nanosecond time resolution, a few millimeter position resolution, an energy threshold of few hundreds MeV, and no particle identification capabilities. The prototypes were deployed about 1.3 km away from the summit, where they measured, behind rock depths larger than 1000 m, remnant fluxes of 1.83±0.50(syst)±0.07(stat) m –2 d –1 deg –2 (MU-RAY) and 1.95±0.16(syst)±0.05(stat) m –2 d –1 deg –2 (TOMUVOL), that roughly correspond to the expected flux of high-energy atmospheric muons crossing 600 meters water equivalent (mwe) at 18° elevation. This implies that imaging depths larger than 500 mwe from 1 km away using such prototype detectors suffer from an overwhelming background. These measurements confirm that a new generation of detectors with higher momentum threshold, time-of-flight measurement, and/or particle identification is needed. As a result, the MU-RAY and TOMUVOL collaborations expect shortly to operate improved detectors, suitable for a robust muographic imaging of kilometer-scale volcanoes.

79 ASTRONOMY AND ASTROPHYSICS↗

Liquid Scintillation Counting of Environmental Radioisotopes: A Review of the Impact of Background Reduction

Liquid scintillation counting (LSC) is a versatile and commonplace method for radiometric measurement of charged particle emitting radionuclides. The LSC method provides utility in a range of environmental science applications including hydrological studies of water transport, anthropogenic releases of radionuclides into the environment, and vertical mixing rates within oceans. Instrumental measurement background is one limiting factor of radiometric measurement sensitivity. As part of the development of a custom low background LSC system located in a shallow underground laboratory at Pacific Northwest National Laboratory, a number of measurement applications of LSC have been considered and are summarized here. The focus is on determining which aspects of such measurements would gain the greatest benefit from the reduction of LSC backgrounds by a factor of 10-100 relative to values reported in the literature. Examples of benefits include lowering the minimum detectable activity, reducing the sample size required, and shortening the elapsed timeline of the processing and analysis sequence. In particular tritium, strontium, and actinium isotopes are examined as these isotopes cover a range of requirements related to the LSC measurement method (e.g., 3H: low energy; Sr: spectral deconvolution; Ac: alpha/beta discrimination).

actinium↗

A radioxenon detection system using CdZnTe, an array of SiPMs, and a plastic scintillator

This paper presents the design and characterization of a prototype compact beta–gamma radioxenon detection system that utilizes a coplanar CdZnTe crystal, an array of SiPMs, and a plastic scintillator. The detector is directly mounted on a custom PCB. The system provides the advantage of room-temperature operation, while being compact, low noise, and with simple readout electronics. Preliminary measurements using 137 Cs, 135 Xe, and 133/133m Xe were conducted to optimize various system parameters to achieve optimal resolution of key photopeaks. The purpose of this research was to explore the potential of these radiation detection elements for use in beta–gamma coincidence applications.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

Gaussian beam scintillation index for slant path in weak turbulence: closed form expressions

The scintillation index (SI) is an important issue in studying the effect of the atmospheric turbulence in the light waves. With the Rytov weak fluctuation theory, the SI is commonly referred to the Rytov parameter. The previous studies dealt with the plane wave and spherical wave models. Each of these gives an idea of how an optical beam will react to turbulence but are not realistic. One is infinitely long, while the other is an infinitesimal point source. The Gaussian beam wave is the most realistic of the optical waves, but also the most complex to use for calculations. In this paper, a closed form expression for Gaussian beam SI propagation in slant path and through weak fluctuation is derived using the polynomial model of the refractive index structure parameter. The slant path SI model of the plane and spherical waves can be generated from the SI expression of Gaussian beam. The analytic expressions are obtained and are then used to analyze the effect of propagation distance, transmitter/receiver heights, and elevation angle on the SI. Signal to noise ratio and bit error rate are calculated for performance evaluation showing a significant enhancement at elevation angles greater than 45°.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Measurement of the scintillation time spectra and pulse-shape discrimination of low-energy β and nuclear recoils in liquid argon with DEAP-1

The DEAP-1 low-background liquid argon detector has been used to measure scintillation pulse shapes of beta decays and nuclear recoil events and to demonstrate the feasibility of pulse-shape discrimination down to an electron-equivalent energy of 20 keV ee . The relative intensities of singlet/triplet states in liquid argon have been measured as a function of energy between 15 and 500 keVee for both beta and nuclear recoils. Using a triple-coincidence tag we find the fraction of beta events that are misidentified as nuclear recoils to be less than 6 x 10 -8 between 43-86 keV ee and that the discrimination parameter agrees with a simple analytic model. The discrimination measurement is currently limited by nuclear recoils induced by cosmic-ray generated neutrons, and is expected to improve by operating the detector underground at SNOLAB. The analytic model predicts a beta misidentification fraction of 10 -10 for an electron-equivalent energy threshold of 20 keV ee . This reduction allows for a sensitive search for spin-independent scattering of WIMPs from 1000 kg of liquid argon with a WIMP-nucleon cross-section sensitivity of 10 -46 cm 2 .

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Development of a scintillator based fast-ion loss detector for the Wendelstein 7-X stellarator

A new scintillator based fast-ion loss detector (FILD) system has been designed for the Wendelstein 7-X (W7-X) stellarator. The mechanical design of the system is presented here along with engineering analyses of the system. This includes an assessment of the structural loads which also considers electromagnetic forces calculated for possible disruption scenarios as well as a mode frequency analysis of the system. Furthermore, an analysis of the thermal characteristics of the actively cooled probe head under prescribed steady state and transient heat loads is presented. Finally, the optical relay system is described and its properties used to forward model synthetic camera signals using the FILDSIM code and based on theoretical fast-ion losses incident on the probe head calculated using the ASCOT5 code.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Study of the loss of xenon scintillation in xenon-trimethylamine mixtures

This work investigates the capability of TMA ((CH 3 ) 3 N) molecules to shift the wavelength of Xe VUV emission (160-188 nm) to a longer, more manageable, wavelength (260-350 nm). Light emitted from a Xe lamp was passed through a gas chamber filled with Xe-TMA mixtures at 800 Torr and detected with a photomultiplier tube. Using bandpass filters in the proper transmission ranges, no reemitted light was observed experimentally. Considering the detection limit of the experimental system, if reemission by TMA molecules occurs, it is below 0.3% of the scintillation absorbed in the 160-188 nm range. An absorption coefficient value for xenon VUV light by TMA of 0.43 ± 0.03 cm -1 Torr -1 was also obtained. These results can be especially important for experiments considering TMA as a molecular additive to Xe in large volume optical time projection chambers.

36 MATERIALS SCIENCE↗

Scintillation Light DAQ and Trigger System for the ICARUS T600 Experiment at Fermilab

ICARUS T600 will operate at shallow depths as far detector for the Short Baseline Neutrino (SBN) program at FNAL taking data from the BNB and NuMI beams. The entire apparatus will be exposed to the huge cosmic background which can mimic genuine neutrino interactions. To distinguish the signals related to the neutrino beams from those induced by cosmic rays, the detector will be provided with a trigger system that will exploit the coincidence of the prompt signals from the liquid argon scintillation light, detected by 360 Photomultiplier Tubes (PMTs), with a beam gate window generated in correspondence to the expected arrival time of neutrinos in the T600.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗