A cloud optical and microphysical property product for the advanced geosynchronous radiation imager onboard China's Fengyun-4 satellites: The first version
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Chao Liu↗
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ELECTROPHYSICAL PROPERTIES OF PHOTOSENSORS BASED ON RADIATION-RESISTANT HG2MNINTE6 CRYSTALS
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JAMES, RALPH B.↗
Simulation of superposed coherent and chaotic radiation of arbitrary spectral shape.
A simulation technique is described and utilized to generate superposed coherent and chaotic (thermal) radiation of arbitrary spectral shape. The statistical properties of a simulated radiation field with a Lorentzian spectral density are investigated with a photoelectron counting experiment. The experimental photocount distribution and normalized mth-order factorial moments are compared to theory and verify that the simulated radiation field, an appropriately modulated laser beam, has the expected statistical properties. The concept described indicates that one may, in principle, generate a thermal source of comparable intensity to that of a laser, arbitrary spectral shape, and bandwidth.
Ruggieri, N. F.↗
Tethered balloon-borne profile measurements of atmospheric properties in the cloudy atmospheric boundary layer over the Arctic sea ice during MOSAiC: Overview and first results
The tethered balloon-borne measurement system BELUGA (Balloon-bornE moduLar Utility for profilinG the lower Atmosphere) was deployed over the Arctic sea ice for 4 weeks in summer 2020 as part of the Multidisciplinary drifting Observatory for the Study of Arctic Climate expedition. Using BELUGA, vertical profiles of dynamic, thermodynamic, aerosol particle, cloud, radiation, and turbulence properties were measured from the ground up to a height of 1,500 m. BELUGA was operated during an anomalously warm period with frequent liquid water clouds and variable sea ice conditions. Three case studies of liquid water phase, single-layer clouds observed on 3 days (July 13, 23, and 24, 2020) are discussed to show the potential of the collected data set to comprehensively investigate cloud properties determining cloud evolution in the inner Arctic over sea ice. Simulated back-trajectories show that the observed clouds have evolved within 3 different air masses (“aged Arctic,” “advected over sea ice,” and “advected over open ocean”), which left distinct fingerprints in the cloud properties. Strong cloud top radiative cooling rates agree with simulated results of previous studies. The weak warming at cloud base is mostly driven by the vertical temperature profile between the surface and cloud base. In-cloud turbulence induced by the cloud top cooling was similar in strength compared to former studies. From the extent of the mixing layer, it is speculated that the overall cloud cooling is stronger and thus faster in the warm oceanic air mass. Larger aerosol particle number concentrations and larger sizes were observed in the air mass advected over the sea ice and in the air mass advected over the open ocean.
Arctic↗
Recovery of electrical properties in 45 Mev electron-irradiated N-type Si from 80 deg K to 350 deg K
45 MeV electron radiation effect on electrical properties and isochronal annealing behavior of N-type silicon
ELECTRON RADIATION↗
Irradiation improves properties of an aromatic polyester
Aromatic polyester, PEN-2,6, is improved through cross-linking effected by radiation. Polymer retains properties of high tensile strength and toughness and stability at high temperatures.
Bell, V. L., Jr.↗
TPSAS-NF1676L-33601-DND
The Clouds and the Earth's Radiant Energy System (CERES) project now has over 18 years of an accurately observed top-of-the-atmosphere (TOA) flux record for climate monitoring and diagnostic studies. CERES provides the climate community the following parameters: coincident instantaneous 1? gridded CERES observed TOA fluxes, computed profile and surface fluxes, as well as MODIS cloud and aerosol retrievals. Clouds and radiation interaction one key factor that dominates climate feedbacks and is also the most difficult problem with large uncertainty. To further advance our understanding of the cloud-radiation interaction, the climate community need data with accurate fluxes and their associated cloud properties for both observational and modelling study. The new CERES FluxByCldTyp data product is produced for this purpose. The flux product combines for the first time CERES measured TOA fluxes along with the associated MODIS cloud properties, which links radiative flux directly to a specific cloud type. This was achieved by computing sub-footprint fluxes for the clear-sky and cloudy portions of the CERES footprint. The spatially distributed cloud properties within the CERES footprint were retrieved from 2-km MODIS pixels, that were stratified by cloud type. The sub-footprint fluxes were estimated from MODIS radiances based on empirically derived narrowband to broadband coefficients. The combined sub-footprint fluxes can then be validated with the observed footprint flux. This presentation will focus on the algorithm development of the flux-by-cloud-type product and its validation.
Moguo Sun↗
TPSAS-NF1676L-33753-DND
The Clouds and the Earth's Radiant Energy System (CERES) project now has over 18 years of an accurately observed top-of-the-atmosphere (TOA) flux record for climate monitoring and diagnostic studies. CERES provides the climate community the following parameters: coincident instantaneous 1 gridded CERES observed TOA fluxes, computed profile and surface fluxes, as well as MODIS cloud and aerosol retrievals. Clouds and radiation interaction one key factor that dominates climate feedbacks and is also the most difficult problem with large uncertainty. To further advance our understanding of the cloud-radiation interaction, the climate community need data with accurate fluxes and their associated cloud properties for both observational and modelling study. The new CERES FluxByCldTyp data product is produced for this purpose. The flux product combines for the first time CERES measured TOA fluxes along with the associated MODIS cloud properties, which links radiative flux directly to a specific cloud type. This was achieved by computing sub-footprint fluxes for the clear-sky and cloudy portions of the CERES footprint. The spatially distributed cloud properties within the CERES footprint were retrieved from 2-km MODIS pixels, that were stratified by cloud type. The sub-footprint fluxes were estimated from MODIS radiances based on empirically derived narrowband to broadband coefficients. The combined sub-footprint fluxes can then be validated with the observed footprint flux. This presentation will focus on the algorithm development of the flux-by-cloud-type product and its validation. The paper will also discuss CERES FlxbyCldTyp simulator and its application.
Moguo Sun↗
Reflective overcoats for radiation control surfaces
Theoretical models are developed to predict the surface properties of a coating layer composed of particles of a known size distribution, applied to an opaque substrate, such as a metal or reaction cured glass (RCG). The surface temperature attained at radiative equilibrium by an overcoated surface subject to a given heat flux is calculated. The incident radiation was assumed to exhibit the spectral distribution characteristic of a black body at different temperatures or equivalently, having different peak wavelengths, with the energy level scaled to give a range of desired surface radiative heat fluxes. This approach allows a straightforward comparison of the thernal response of a surface to incident radiation having the energy predominantly in a characteristic wavelength band and a well-defined spectral distribution. The ratio of the radiative heat flux to the total heat flux was varied, and the different geometric and material parameters of such overcoat layers were explored. The model was applied to representative surface heating rates to the Aeroasssisted Flight Experiment (AFE) and to Aeroassisted Space Transfer Vehicles (ASTVs). The predicted radiative energy flux to the surface of the AFE vehicle gives a single-point comparison of the surface temperatures attained with and without a selective-reflector overcoat on the vehicle surface. The specific objective of this work is to identify the most desirable radiative properties of an overcoat/substrate system for this environment.
White, Susan M.↗
Direct Aerosol Radiative Forcing: Calculations and Measurements from the Tropospheric
Radiative forcing is defined as the change in the net (downwelling minus upwelling) radiative flux at a given level in the atmosphere. This net flux is the radiative power density available to drive climatic processes in the earth-atmosphere system below that level. Recent research shows that radiative forcing by aerosol particles is a major source of uncertainty in climate predictions. To reduce those uncertainties, TARFOX was designed to determine direct (cloud-free) radiative forcing by the aerosols in one of the world's major industrial pollution plumes--that flowing from the east coast of the US over the Atlantic Ocean. TARFOX measured a variety of aerosol radiative effects (including direct forcing) while simultaneously measuring the chemical, physical, and optical properties of the aerosol particles causing those effects. The resulting data sets permit a wide variety of tests of the consistency, or closure, among the measurements and the models that link them. Because climate predictions use the same or similar model components, closure tests help to assess and reduce prediction uncertainties. In this work we use the TARFOX-determined aerosol, gas, and surface properties to compute radiative forcing for a variety of aerosol episodes, with inadvisable optical depths ranging from 0.07 to 0.6. We calculate forcing by several techniques with varying degrees of sophistication, in part to test the range of applicability of simplified techniques--which are often the only ones feasible in climate predictions by general circulation models (GCMs). We then compare computed forcing to that determined from: (1) Upwelling and downwelling fluxes (0.3-0.7 mm and 0.7-3.0 mm) measured by radiometers on the UK MRF C-130. and (2) Daily average cloud-free absorbed solar and emitted thermal radiative flux at the top of the atmosphere derived from the AVHRR radiometer on the NOAA- 14 satellite. The calculations and measurements all yield aerosol direct radiative forcing in the range -50 to -190 W sq m per unit inadvisable optical depth. The magnitudes are about 15 to 100 times larger than the global-average direct forcing expected for the global-average sulfate aerosol optical depth of 0.04. The reasons for the larger forcing in TARFOX include the relatively large optical depths and the focus on cloud-free, daytime conditions over the dark ocean surface. These are the conditions that produce the actual major radiative forcing events that contribute to any global-average climate effect. Detailed comparisons of calculated and measured forcings for specific events are used for more refined tests of closure.
Russell, P. B.↗
Stratospheric aerosols and climatic change
Stratospht1ic sulfuric acid particles scatter and absorb sunlight and they scatter, absorb and emit terrestrial thermal radiation. These interactions play a role in the earth's radiation balance and therefore affect climate. The stratospheric aerosols are perturbed by volcanic injection of SO2 and ash, by aircraft injection of SO2, by rocket exhaust of Al2O3 and by tropospheric mixing of particles and pollutant SO2 and COS. In order to assess the effects of these perturbations on climate, the effects of the aerosols on the radiation balance must be understood and in order to understand the radiation effects the properties of the aerosols must be known. The discussion covers the aerosols' effect on the radiation balance. It is shown that the aerosol size distribution controls whether the aerosols will tend to warm or cool the earth's surface. Calculations of aerosol properties, including size distribution, for various perturbation sources are carried out on the basis of an aerosol model. Calculations are also presented of the climatic impact of perturbed aerosols due to volcanic eruptions and Space Shuttle flights.
Toon, O. B.↗
Long-range transported North American wildfire aerosols observed in marine boundary layer of eastern North Atlantic
Wildfire is a major source of biomass burning aerosols, which greatly impact Earth climate. Tree species in North America (NA) boreal forests can support high-intensity crown fires, resulting in elevated injection height and longer lifetime (on the order of months) of the wildfire aerosols. Given the long lifetime, the properties of aged NA wildfire aerosols are required to understand and quantify their effects on radiation and climate. Here we present comprehensive characterization of climatically relevant properties, including optical properties and cloud condensation nuclei (CCN) activities of aged NA wildfire aerosols, emitted from the record-breaking Canadian wildfires in August 2017. Despite the extreme injection height of ~12 km, some of the wildfire plumes descended into the marine boundary layer in the eastern North Atlantic over a period of ~2 weeks, owing to the dry intrusions behind mid-latitude cyclones. The aged wildfire aerosols have high single scattering albedos at 529 nm (ω 529 ; 0.92–0.95) while low absorption Ångström exponents (Å abs ) at 464 nm/648 nm (0.7–0.9). In comparison, Å abs of fresh/slightly aged ones are typically 1.4–3.5. This low Å abs 529 and low Å abs ~110 nm diameter) with thick non-absorbing coatings. The accelerated descent of the wildfire plume also led to strong increase of CCN concentration at the supersaturation levels representative of marine low clouds. The hygroscopicity parameter, κ CCN , of the aged wildfire aerosols varies from 0.2 to 0.4, substantially lower than that of background marine boundary layer aerosols. However, the high fraction of particles with large diameter (i.e., within accumulation size ranges, ~100–250 nm) compensates for the low values of κ, and as a result, the aged NA wildfire aerosols contribute more efficiently to CCN population. These results provide direct evidence that the long-range transported NA wildfires can strongly influence CCN concentration in remote marine boundary layer, therefore the radiative properties of marine low clouds. Given the expected increases of NA wildfire intensity and frequency and regular occurrence of dry intrusion following mid-latitude cyclones, the influence of NA wildfire aerosols on CCN and clouds in remote marine environment need to be further examined.
54 ENVIRONMENTAL SCIENCES↗
Cyclotron maser radiation from a source structure localized perpendicular to the ambient magnetic field
Particle simulations were used to investigate the properties of electromagnetic radiation produced by the cyclotron maser instability in a source region which is localized in the direction perpendicular to the uniform magnetic field. In the procedure used, the simulation model of Pritchett and Strangeway (1985) for the generation of auroral kilometric radiation (AKR) along an auroral field line was modified to include inhomogeneities perpendicular to the magnetic field. The results are compared with the previous homogeneous simulations with regard to efficiency and saturation mechanism and with expectations based on the feedback model. The implications for the generation and propagation of AKR are discussed.
Pritchett, P. L.↗
Vulnerability of Passive Microwave Snowfall Retrievals to Physical Properties of Snowpack: A Perspective from Dense Media Radiative Transfer Theory
The uncertainty of passive microwave retrievals of snowfall is notoriously high where the high-frequency surface emissivity is significantly reduced and varies markedly in response to changes of snowpack physical properties. Using the dense media radiative transfer theory, this article studies the potential effects of terrestrial snow-cover depth, density, and6grain size on high-frequency channels 89 and 166 GHz of the radiometer onboard the Global Precipitation Measurement (GPM) core satellite, which are commonly used to capture the snowfall scattering signals. Integrating the inference across all feasible grain sizes, ranges of snowpack density and depth are identified over which the snowfall scattering signatures can be time varying and potentially obscured. Using 10 years of reanalysis data, the seasonal vulnerability of snowfall retrievals to changes of snowpack emissivity in the Northern Hemisphere is mapped in a probabilistic sense and connections are made with uncertainties of the GPM passive microwave snowfall retrievals. It is found that among different snow classes, relatively light Arctic tundra snow in fall, with a density below 260kg m−3, and shallow prairie snow during the winter, with a depth of less than 40cm, can reduce the surface emissivity and obscure the snowfall passive microwave signatures. It is demonstrated that, during the winter, the highly vulnerable areas are over Kazakhstan, and Mongolia with taiga and prairie snow. In the fall, these areas are largely over tundra and taiga snow in north of Russia and the Arctic Archipelagos as well as prairies in Canada and the Great Plains in the United States.
Reyhaneh Rahimi↗
Advancements in the Representation of Cloud-Aerosol Microphysics in the GEOS-5 AGCM
Despite numerous challenges, the physical parameterization of cloud-aerosol interactions in atmospheric GCMs has become a top priority for advancement because of our need to simulate and understand past, current, and future indirect effects of aerosols on clouds. The challenges stem from the involvement of wide range of cloud-scale dynamics and aerosol activation physical processes. Cloud dynamics modulate cloud areal extent and condensate, while aerosol activation depends on aerosol mass load, size distribution, internal mixing state, and nucleating properties, and ultimately determines cloud optical properties via particle sizes. Both macro- and micro-scale processes are obviously important for cloud-radiation interactions. We will present the main features of cloud microphysical properties in the GEOS- 5 Atmospheric GCM (AGCM) as simulated by the McRAS-AC (Microphysics of Clouds with Relaxed Arakawa-Schubert and Aerosol-Cloud interaction) scheme. McRAS-AC uses Fountoukis and Nenes (2005) aerosol activation for liquid clouds, and has an option for either Liu and Penner (2005) or Barahona and Nenes (2008, 2009) aerosol activation for ice clouds. Aerosol loading (on-line or climatological) comes from GOCART, with an assumed log-normal size distribution. Other features of McRAS-AC are level-by-level cloud-scale thermodynamics, and Seifert-Beheng (2001)-type precipitation microphysics, particularly from moist convection. Results from Single-Column Model simulations will be shown to demonstrate how cloud radiative properties, lifetimes, and precipitation are influenced by different parameterization assumptions. Corresponding fields from year-long simulations of the full AGCM will also be presented with geographical distributions of cloud effective particle sizes compared to satellite retrievals. While the primary emphasis will be on current climate, simulation results with perturbed aerosol loadings will also be shown to expose the radiative sensitivity of the microphysical parameterization.
Lee, D.↗
Shortwave Radiative Fluxes, Solar-Beam Transmissions, and Aerosol Properties: TARFOX and ACE-2 Find More Absorption from Flux Radiometry than from Other Measurements
The Tropospheric Aerosol Radiative Forcing Observational Experiment (TARFOX) and the Second Aerosol Characterization Experiment (ACE-2) made simultaneous measurements of shortwave radiative fluxes, solar-beam transmissions, and the aerosols affecting those fluxes and transmissions. Besides the measured fluxes and transmissions, other obtained properties include aerosol scattering and absorption measured in situ at the surface and aloft; aerosol single scattering albedo retrieved from skylight radiances; and aerosol complex refractive index derived by combining profiles of backscatter, extinction, and size distribution. These measurements of North Atlantic boundary layer aerosols impacted by anthropogenic pollution revealed the following characteristic results: (1) Better agreement among different types of remote measurements of aerosols (e.g., optical depth, extinction, and backscattering from sunphotometers, satellites, and lidars) than between remote and in situ measurements; 2) More extinction derived from transmission measurements than from in situ measurements; (3) Larger aerosol absorption inferred from flux radiometry than from other measurements. When the measured relationships between downwelling flux and optical depth (or beam transmission) are used to derive best-fit single scattering albedos for the polluted boundary layer aerosol, both TARFOX and ACE-2 yield midvisible values of 0.90 +/- 0.04. The other techniques give larger single scattering albedos (i.e. less absorption) for the polluted boundary layer, with a typical result of 0.95 +/- 0.04. Although the flux-based results have the virtue of describing the column aerosol unperturbed by sampling, they are subject to questions about representativeness and other uncertainties (e.g., unknown gas absorption). Current uncertainties in aerosol single scattering albedo are large in terms of climate effects. They also have an important influence on aerosol optical depths retrieved from satellite radiances. More tests are needed of the consistency among different methods and of the effects of changing humidity on aerosol.
Russell, Philip B.↗
Uncertainty of SW Cloud Radiative Effect in Atmospheric Models Due to the Parameterization of Liquid Cloud Optical Properties
Clouds are largely responsible for the spread of climate models predictions. Here we focus on the uncertainties in cloud shortwave radiative effect due to the parameterization of liquid cloud single scattering properties (SSPs) from liquid water content (LWC) and droplet number concentration (N), named parameterization of cloud optical properties. Uncertainties arise from not accounting for the droplet size distribution (DSD)—which affects the estimation of the effective radius (r eff ) and modulates the r eff -dependency of the SSPs—and from averaging SSPs over wide spectral bands. To assess these uncertainties a series of r eff -dependent SSPs parameterizations corresponding to various DSDs and spectral averaging methods are derived and implemented in a radiative code. Combined with the DSD-dependent estimation of r eff they are used to compute the bulk radiative properties (reflectance, transmittance, absorptance) of various clouds (defined in terms of LWC and N), including a homogeneous cloud, more realistic case studies, and outputs of a climate model. The results show that the cloud radiative forcing can vary up to 20% depending on the assumed DSD. Likewise, differences up to 20% are obtained for heating rates. The estimation of r eff is the main source of uncertainty, while the SSPs parameterization contributes to around 20% of the total uncertainty. Spectral averaging is less an issue, except for atmospheric absorption. Overall, global shortwave cloud radiative effect can vary by 6 W m –2 depending on the assumed DSD shape, which is about 13% of the best observational estimate.
54 ENVIRONMENTAL SCIENCES↗
Vibration Studies for the CLARA Interferometer
The purpose of the CLARA experiment is to study the nature of undulator radiation emitted by single electrons circulating in the IOTA storage ring. The classical and quantum properties of the radiation are investigated by measuring its coherence length, intensity fluctuations and time correlations. The experiment took data in IOTA Run 4 (2022-2023). The key component of the apparatus is a Mach-Zehnder interferometer (MZI), in which the optical length of one of the arms can be precisely controlled. For some measurements, the fine regulation of the arm length must be smaller than the radiation wavelength. For this reason, the apparatus is particularly sensitive to mechanical vibrations. In this note, we model and measure the effect of vibrations on the performance of the MZI under various conditions. Several improvements of the setup were implemented to minimize systematic distortions of the observed interference patterns. In this report, we present a mathematical model of the effect of mechanical vibrations on observed detector and coincidence rates. We also describe the measurements that were made to estimate the magnitude and spectra of rate fluctuations and their sources in the CLARA MZI under various conditions. Finally, we estimate the magnitude of arm length fluctuations and we deduce the sensitivity to coincidence-rate variations in our apparatus.
43 PARTICLE ACCELERATORS↗