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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,045 records · Page 58
All sourcesNASA NTRSDOE OSTI
DOE OSTI2019

Back-contacted bottom cells with three terminals: Maximizing power extraction from current-mismatched tandem cells

Multi-junction cells can significantly improve the energy yield of photovoltaic systems over a single-junction cell. The internal interconnection scheme of the subcells is an important aspect in determining the resulting levelized cost of electricity. For a dual-junction cell, two approaches are commonly discussed: series-connected tandem cells with two terminals or independently working subcells in a four-terminal (4T) tandem device. In this paper, we explore the working principle and the operation modes of a third, rarely discussed option: a three-terminal (3T) tandem cell using a back-contacted bottom cell with 3Ts. We use current-voltage measurements of illuminated 3T interdigitated back contact cells and confirm that the front and rear base contacts are at similar quasi-Fermi level positions, which enables the bottom cell to either efficiently collect surplus carriers, in the case of a current-limiting or carrier injecting top cell, or inject majority carriers, in the case of a current-limiting bottom cell. As a result, no current matching is needed. The power output of an idealized 3T bottom cell without resistive effects is independent of the current density applied from the top cell. These characteristics of the 3T bottom cells enable a 3T tandem to operate as efficiently as a 4T tandem, while being compatible with monolithic design and not requiring intermediate grids. We propose a simple equivalent circuit model including additional resistive effects, which describes a real 3T bottom cell and achieves excellent agreement to the experiment. We deduce design guidelines for a 3T bottom cell in different operation regimes.

14 SOLAR ENERGY↗
DOE OSTI2018

Fast Algorithm for Evaluating Critical Current of High-Temperature Superconducting Pancake Coil

Second-generation (2G) high-temperature superconducting (HTS) tapes are now capable of carrying very high transport current and promising for a wide range of applications. The critical current of HTS coils is important for applications, such as superconducting electric machines, superconducting magnetic energy storage, and superconducting magnets. Therefore, precisely and quickly calculating critical current of HTS coils is very important for designing HTS devices. This paper provides a fast algorithm for evaluating critical current of HTS pancake coil. The fast algorithm is realized through a stationary model, which is based on finite element method (FEM) software. The stationary model means that the model is solved by stationary study instead of time-dependent study. To validate this method, a pancake HTS coil was wound and its critical current was measured. Meanwhile, an axial symmetric stationary model was built according to the geometry of the measured HTS coil. By comparing measured and calculated results, the effectiveness of the stationary model was demonstrated. Moreover, the stationary model is compared with H formulation model. The calculated results by the two models are nearly the same. However, by using stationary calculation, the stationary model can remarkably speed up the computational process. Due to the advantage of calculating speed, the stationary model can be used to characterize and design large-scale HTS applications.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2019

Fabrication and Tests of a Resistive-Type Superconducting Fault Current Limiter Module Based on Coated Conductors

The resistivetype superconducting fault current limiter (R-SFCL) is simple in structure, near zero impedance at normal state and can be quickly triggered by the fault current. Thus, it is a possible solution to limit the fault current in the power grid. In this paper, we report the fabrication and test for an R-SFCL module The R-SFCL module consists of seven bifilar coils connected in parallel, which were wound with two parallel 2G tapes. A 5mm spacer was co-wound between adjacent turns to act as the highvoltage insulation. In the tests, we test the current distribution among the bifilar coils, and then simulated short-circuit tests were conducted on the module to obtain its performance under fault current surge.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2018

Surface Current Approximation in Certain Problems of the Classical Theory of Superconductivity

The problems of the behavior of superconducting infinite plane-parallel plate and cylinder in an external magnetic field are solved in the approximation of the model of surface currents. The latter, in contrast to the conventional notation, enter as the currents of superconducting electrons into the boundary conditions for the magnetic induction. Surface currents are understood as the volumetric current flowing in the thickness of the near-surface layer, which is associated with the thickness of the London penetration depth of the field and currents into the thickness of the superconductor. It is shown that in this case, a jump in the magnetic quantities occurs at this thickness. The calculated average magnetization of the magnet is reduced to the strength of the external field. The proportionality coefficient, which is reasonable to call the mean magnetic susceptibility, turns out to be not exactly equal to –1, but has a slightly less value, because the field does not weaken immediately. The possibilities of experimental verification of the obtained effect are discussed.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2019

Beam Current Effect on Microstructure and Properties of Electron-Beam-Melted Ti-6Al-4V Alloy

In this study, a noncommercial 3D printing machine was used to fabricate Ti-6Al-4V alloy by electron-beam melting (EBM). The influence of beam current on the microstructure, phase composition and mechanical properties of electron-beam-melted Ti-6Al-4V alloy was investigated. Numerical simulation is implemented to evaluate thermal fields during electron-beam melting of Ti-6Al-4V powder. The decrease in beam current from 3.5 to 2.5 mA leads to refinement of microstructure: The average width of α plates decreases from 10 down to 6 μm. The formation of finer microstructure is attributed to higher cooling rate at lower beam current confirmed by simulation. The phase composition of EBM Ti-6Al-4V indirectly depends on the beam current. High content of β phase (7%) was achieved at the beam current of 3 mA. The produced Ti-6Al-4V samples are characterized by high microhardness (470-520 HV).

36 MATERIALS SCIENCE↗
DOE OSTI2016

Characteristics of persistent spin current components in a quasi-periodic Fibonacci ring with spin–orbit interactions: Prediction of spin–orbit coupling and on-site energy

In the present work we investigate the behavior of all three components of persistent spin current in a quasi-periodic Fibonacci ring subjected to Rashba and Dresselhaus spin–orbit interactions. Analogous to persistent charge current in a conducting ring where electrons gain a Berry phase in presence of magnetic flux, spin Berry phase is associated during the motion of electrons in presence of a spin–orbit field which is responsible for the generation of spin current. The interplay between two spin–orbit fields along with quasi-periodic Fibonacci sequence on persistent spin current is described elaborately, and from our analysis, we can estimate the strength of any one of two spin–orbit couplings together with on-site energy, provided the other is known. - Highlights: • Determination of Rashba and Dresselhaus spin–orbit fields is discussed. • Characteristics of all three components of spin current are explored. • Possibility of estimating on-site energy is given. • Results can be generalized to any lattice models.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2021

High-Fidelity Simulations of Gravity Currents Using a High-Order Finite-Difference Spectral Vanishing Viscosity Approach

This numerical work investigates the potential of a high-order finite-difference spectral vanishing viscosity approach to simulate gravity currents at high Reynolds numbers. The method introduces targeted numerical dissipation at small scales through altering the discretisation of the second derivatives of the viscous terms in the incompressible Navier-Stokes equations to mimic the spectral vanishing viscosity (SVV) operator, originally designed for the regularisation of spectral element method (SEM) solutions of pure advection problems. Using a sixth-order accurate finite-difference scheme, the adoption of the SVV method is straightforward and comes with a negligible additional computational cost. In order to assess the ability of this high-order finite-difference spectral vanishing viscosity approach, we performed large-eddy simulations (LES) of a gravity current in a channelised lock-exchange set-up with our SVV model and with the well-known explicit static and dynamic Smagorinsky sub-grid scale (SGS) models. The obtained data are compared with a direct numerical simulation (DNS) based on more than 800 million mesh nodes, and with experimental measurements. A framework for the energy budget is introduced to investigate the behaviour of the gravity current. First, it is found that the DNS is in good agreement with the experimental data for the evolution of the front location and velocity field as well as for the stirring and mixing inside the gravity current. Secondly, the LES performed with less than 0.4% of the total number of mesh nodes compared to the DNS, can reproduce the main features of the gravity currents, with the SVV model yielding slightly more accurate results. It is also found that the dynamic Smagorinsky model performs better than its static version. For the present study, the static and dynamic Smagorinsky models are 1.8 and 2.5 times more expensive than the SVV model, because the latter does not require the calculation of explicit SGS terms in the Navier-Stokes equations nor spatial filtering operations.

direct numerical simulation↗
DOE OSTI2021

Investigations on the effect of current density on SiO/Si composite electrodes

An oxide layer on the surface of silicon particles is inevitable and is necessary for their application as anode materials for lithium ion batteries with high capacity and durability. However, a thick surficial oxide layer could significantly reduce the capacity of a Si anode. Here, Si nanoparticles with a thick surficial oxide layer of ~20 nm (Si@SiO x ) were fabricated through thermal oxidation and investigated electrochemically. The results revealed that very low current density is needed to activate Si@SiO x anodes during the first formation cycle. Once activated, the Si@SiO x anode can deliver reversible capacity as high as ~1000 mAh/g with low current density. Then, the Si@SiO x can be cycled at higher current densities of >700 mAh/g. Electrochemical impedance spectroscopy (EIS) shows that the lower current density results in lower charge-transfer resistance of the Si@SiO x anode, suggesting a higher degree of lithiation of the surficial oxide layer during low-current activation. EIS analysis also reveals that the lithiation of the surficial oxide is irreversible. We believe that the surface silicon oxide layer is lithiated and forms lithium silicate during the initial activation process. Lithium silicate has high conductivity and allows the lithiation/delithiation of Si core under the oxide layer during following charge and discharge.

25 ENERGY STORAGE↗
DOE OSTI2019

TRANSP-based closed-loop simulations of current profile optimal regulation in NSTX-Upgrade

Active control of the toroidal current density profile is critical for the upgraded National Spherical Torus eXperiment device (NSTX-U) to maintain operation at the desired high-performance, MHD-stable, plasma regime. Initial efforts towards current density profile control have led to the development of a control-oriented, physics-based, plasma-response model, which combines the magnetic diffusion equation with empirical correlations for the kinetic profiles and the non-inductive current sources. The developed control-oriented model has been successfully tailored to the NSTX-U geometry and actuators. Moreover, a series of efforts have been made towards the design of model-based controllers, including a linear-quadratic-integral optimal control strategy that can regulate the current density profile around a prescribed target profile while rejecting disturbances. In this work, the tracking performance of the proposed current-profile optimal controller is tested in numerical simulations based on the physics-oriented code TRANSP. Furthermore, these high-fidelity closed-loop simulations, which are a critical step before experimental implementation and testing, are enabled by a flexible framework recently developed to perform feedback control design and simulation in TRANSP.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2019

Integrated current profile, normalized beta and NTM control in DIII-D

There is an increasing need for integrating individual plasma-control algorithms with the ultimate goal of simultaneously regulating more than one plasma property. Some of these integrated-control solutions should have the capability of arbitrating the authority of the individual plasma-control algorithms over the available actuators within the tokamak. Such decision-making process must run in real time since its outcome depends on the plasma state. Therefore, control architectures including supervisory and/or exception-handling algorithms will play an essential role in future fusion reactors like ITER. However, most plasma-control experiments in present devices have focused so far on demonstrating control solutions for isolated objectives. In this work, initial experimental results are reported for simultaneous current-profile control, normalized-beta control, and Neoclassical Tearing Mode (NTM) suppression in DIII-D. Neutral beam injection (NBI), electron-cyclotron (EC) heating & current drive (H&CD), and plasma current modulation are the actuation methods. The NBI power and plasma current are always modulated by the Profile Control category within the DIII-D Plasma Control System (PCS) in order to control both the current profile and the normalized beta. EC H&CD is utilized by either the Profile Control or the Gyrotron categories within the DIII-D PCS as dictated by the Off-Normal and Fault Response (ONFR) system, which monitors the occurrence of an NTM and regulates the authority over the gyrotrons. The total EC power and poloidal mirror angles are the gyrotron-related actuation variables. When no NTM suppression is required, the gyrotrons are used by the Profile Control category, but when NTM suppression is required, the ONFR transfers the authority over the gyrotrons to the NTM stabilization algorithm located in the Gyrotron category. Initial experimental results show that simultaneous control of different aspects of the plasma dynamics may improve the overall control and plasma performances. Also, the potential of the ONFR system to successfully integrate competing control algorithms is demonstrated.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2018

Formation of TiO2 nanoribbons by anodization under high current density

Highlights: • TiO{sub 2} nanotubes were obtained under low current density. • TiO{sub 2} nanoribbons were obtained under high current density. • The pore walls of top TiO{sub 2} nanotubes are obviously thinner than other part. • Micro-liquid-flow causes the appearance of TiO{sub 2} nanoribbons. - Abstract: Highly ordered TiO{sub 2} nanoribbons are obtained by anodizations in NH{sub 4}F electrolyte under high current density. Although intact TiO{sub 2} nanoribbons appear, there are still nanotubes beneath nanoribbons. It is reasonable to speculate that TiO{sub 2} nanoribbons evolve from TiO{sub 2} nanotubes. While the applied current is high, the electronic current is also high, which gives rise to lots of oxygen bubbles. With the accumulation of oxygen bubbles, oxygen bubbles must expand upward and rupture finally. Therefore, gas flow from oxygen bubbles results in the generation of micro-liquid-flow. Because of micro-liquid-flow, the nanotube wall is corroded and scoured. The corrosion of upper pore wall is the most sever and thus the upper pore wall becomes the thinnest locality of nanotube wall. As a result, the nanotubes can collapse easily. Finally, one TiO{sub 2} nanotube is divided into several TiO{sub 2} nanoribbons while there is still intact tube beneath nanoribbons.

77 NANOSCIENCE AND NANOTECHNOLOGY↗
DOE OSTI2020

Moderate pH changes alter the fluxes, selectivities and limiting currents in ion transport through polyelectrolyte multilayers deposited on membranes

Layer-by-layer (LBL) polyelectrolyte coatings on membranes are attractive for their high selectivities between monovalent and divalent ions. However, deposition of poly(4-styrenesulfonate) (PSS)/protonated poly(allylamine) (PAH) films on ion-exchange membranes leads to low ion fluxes that restrict productivity or current efficiency. This study shows that increasing the solution pH from 6.5 to 8.3 enhances cation fluxes and limiting currents through (PAH/PSS) 5 PAH-coated cation-exchange membranes while still achieving order of magnitude selectivity increases compared to bare membranes. In Donnan dialysis through (PAH/PSS) 5 PAH-coated Nafion, at pH 8.3 the K + /Mg 2+ selectivity is 100, and the K + flux is 22 times that at pH 6.5. Moreover, at the higher pH the electrodialysis limiting current through these membranes increases ~5-fold. This enables electrodialysis separation of K + and Mg 2+ with a current efficiency around 0.75, a selectivity of 18, and 50% K + recovery from the source phase. Transmembrane potential measurements and increases in Cl - /SO 4 2- selectivities (from 9.5 at pH 6.5 to ~70 at pH 8.3) for porous alumina membranes coated with (PSS/PAH) 5 PSS films suggest that the coating becomes cation-permselective at higher pH. Increased cation transference numbers in polyelectrolyte coatings likely lead to the enhanced limiting currents for coated Nafion at higher pH. Lastly, (PAH/PSS) 5 PAH-coated Nafion shows a Li + /Mg 2+ Donnan dialysis selectivity >700 at neutral pH and a selectivity of 10 at pH 8.3. However, the Li + flux is 6 times greater at pH 8.3, which might make operation at the higher pH desirable.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2021

Prevention of lithium-ion battery thermal runaway using polymer-substrate current collectors

Isolating electronically conducting material from internal short circuits is a promising way to prevent the onset of thermal runaway within lithium-ion cells. Here, a metal-coated polymer current collector, which is designed to disconnect internal short circuits by withdrawing from the heating region, is tested in 18650 cells. In addition to having lower mass and manufacturing costs, cells with metal-coated polymer current collectors demonstrate a reduced risk of thermal runaway during nail penetration. High-speed synchrotron X-ray radiography of 18650 cells during nail-penetration testing, in tandem with pre- and post-mortem X-ray computed tomography, provides insights into the function of the current collectors. The results are compared with those of 18650 cells with standard commercial aluminum and copper current collectors. Cells with aluminum-coated polymer current collectors demonstrated 100% success in thermal runaway prevention during nail penetration, retaining a cell voltage >4.00 V, while standard cells consistently experienced thermal runaway.

25 ENERGY STORAGE↗
DOE OSTI2020

High Current Cycling in a Superconcentrated Ionic Liquid Electrolyte to Promote Uniform Li Morphology and a Uniform LiF-Rich Solid Electrolyte Interphase

High-energy-density systems with fast charging rates and suppressed dendrite growth are critical for the implementation of efficient and safe next-generation advanced battery technologies such as those based on Li metal. However, there are few studies that investigate reliable cycling of Li metal electrodes under high-rate conditions. in this work, by employing a superconcentrated ionic liquid (IL) electrolyte, we highlight the effect of Li salt concentration and applied current density on the resulting Li deposit morphology and solid electrolyte interphase (SEI) characteristics, demonstrating exceptional deposition/dissolution rates and efficiency in these systems. Operation at higher current densities enhanced the cycling efficiency, e.g., from 64 ± 3% at 1 mA cm –2 up to 96 ± 1% at 20 mA cm –2 (overpotential <±0.2 V), while resulting in lower electrode resistance and dendrite-free Li morphology. A maximum current density of 50 mA cm –2 resulted in 88 ± 3% cycling efficiency, displaying tolerance for high overpotentials at the Ni working electrode (0.5 V). X-ray photoelectron microscopy (XPS), time-of-flight secondary-ion mass spectroscopy (ToF-SIMS), and scanning electron microscopy (SEM) surface measurements revealed that the formation of a stable SEI, rich in LiF and deficient in organic carbon species, coupled with nondendritic and compact Li morphologies enabled enhanced cycling efficiency at higher currents. Reduced dendrite formation at high current is further highlighted by the use of a highly porous separator in coin cell cycling (1 mAh cm –2 at 50 °C), sustaining 500 cycles at 10 mA cm –2 .

25 ENERGY STORAGE↗
DOE OSTI2012

Superconducting quantum interference devices based set-up for probing current noise and correlations in three-terminal devices

We have implemented a new experimental set-up for precise measurements of current fluctuations in three-terminal devices. The system operates at very low temperatures (30 mK) and is equipped with three superconducting quantum interference devices (SQUIDs) as low noise current amplifiers. A SQUID input coil is connected to each terminal of a sample allowing the acquisition of time-dependent current everywhere in the circuit. From these traces, we can measure the current mean value, the noise, and cross-correlations between different branches of a device. In this paper, we present calibration results of noise and cross-correlations obtained using low impedance macroscopic resistors. From these results, we can extract the noise level of the set-up and show that there are no intrinsic correlations due to the measurement scheme. We also studied noise and correlations as a function of a dc current and estimated the electronic temperature of various macroscopic resistors.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2013

Kelvin-Helmholtz instability in a current-vortex sheet at a 3D magnetic null

We report here, for the first time, an observed instability of a Kelvin-Helmholtz nature occurring in a fully three-dimensional (3D) current-vortex sheet at the fan plane of a 3D magnetic null point. The current-vortex layer forms self-consistently in response to foot point driving around the spine lines of the null. The layer first becomes unstable at an intermediate distance from the null point, with the instability being characterized by a rippling of the fan surface and a filamentation of the current density and vorticity in the shear layer. Owing to the 3D geometry of the shear layer, a branching of the current filaments and vortices is observed. The instability results in a mixing of plasma between the two topologically distinct regions of magnetic flux on either side of the fan separatrix surface, as flux is reconnected across this surface. We make a preliminary investigation of the scaling of the system with the dissipation parameters. Our results indicate that the fan plane separatrix surface is an ideal candidate for the formation of current-vortex sheets in complex magnetic fields and, therefore, the enhanced heating and connectivity change associated with the instabilities of such layers.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2013

Application of dynamic displacement current for diagnostics of subnanosecond breakdowns in an inhomogeneous electric field

The breakdown of different air gaps at high overvoltages in an inhomogeneous electric field was investigated with a time resolution of up to 100 ps. Dynamic displacement current was used for diagnostics of ionization processes between the ionization wave front and a plane anode. It is demonstrated that during the generation of a supershort avalanche electron beam (SAEB) with amplitudes of {approx}10 A and more, conductivity in the air gaps at the breakdown stage is ensured by the ionization wave, whose front propagates from the electrode of small curvature radius, and by the dynamic displacement current between the ionization wave front and the plane electrode. The amplitude of the dynamic displacement current measured by a current shunt is 100 times greater than the SAEB. It is shown that with small gaps and with a large cathode diameter, the amplitude of the dynamic displacement current during a subnanosecond rise time of applied pulse voltage can be higher than 4 kA.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2013

Specific characteristics of negative corona currents generated in short point-plane gap

The Trichel pulse is a typical kind of negative corona current observed in electronegative gases with a highly regular form. The characteristics of the Trichel pulse, such as the repetition frequency, the amplitude of each pulse, and the mean current, are dependent on different discharge conditions. Quite many scholars have studied the mean current and the current-voltage characteristic of Trichel pulses, yet the specific characteristics of the pulses have barely been investigated. In this paper, a series of experiments were carried out in a short point-to-plane discharge gap to investigate the detailed characteristics of Trichel pulses. After numerical fitting of the experiment results was performed, a new set of empirical formulas were derived to predict the specific characteristics of the negative corona current under different conditions. Different from existing literature, this paper uses as variables the average electric field intensity and the corona inception field intensity which is independent of the gap spacing in the empirical formulas. In the experiments, an inverse correlation between amplitude and repetition frequency of the pulses was observed. Based on the investigation of the remaining space charge in the discharge gap, this correlation is theoretically proved to be caused by the influence of space charges.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗