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At least 1,027 records · Page 57
All sourcesNASA NTRSDOE OSTI
DOE OSTI2017

Evaluation of The Thermophysical Properties and Microstructure of UPu{sub 24}Zr{sub 15} Metallic Fuel

Featuring high burn-up, high fissile and fertile isotopic density, inherent safety characteristics, and favorable thermal response, actinide transmutation metallic fuels are considered to be among the most promising fuel classes for next generation fast reactors. During reactor operation, it is anticipated that fluctuations in chemical potential along the temperature gradient will lead to migration and redistribution of constituents between radial zones of the cylindrical fuel pin, resulting in compositional inhomogeneity and hence unpredictable fuel performance. Limited experimental fuel performance data is available for fuel selection and certification, therefore different compositions of options uranium-plutonium-zirconium (UPu- Zr) alloys have been investigated. Several complementary techniques, including scanning and transmission electron microscopy (SEM and TEM, respectively), differential scanning calorimetry (DSC), and laser flash diffusivity (LFD) techniques were used to characterize the phase distribution, microstructure, and thermophysical properties of unirradiated U-Pu-Zr fuels in both the as-cast and annealed condition. This information is necessary to understand the irradiated microstructure, properties, and performance of U-Pu-Zr fuels.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2012

Solidification characterization of a new rapidly solidified Ni-Cr-Co based superalloy

The solidification characterization of a new rapidly solidified Ni-Cr-Co based superalloy prepared by plasma rotating electrode process was investigated by means of optical microscope, scanning electron microscope, and transmission electron microscope. The results show that the solidification microstructure changes from dendrites to cellular and microcrystal structures with decreasing powder size. The elements of Co, Cr, W and Ni are enriched in the dendrites, while Mo, Nb and Ti are higher in the interdendritic regions. The relationships between powder size with the average solid-liquid interface moving rate, the average interface temperature gradient and the average cooling rate are established. Microsegregation is increased with larger powder size. The geometric integrity of MC Prime type carbides in the powders changes from regular to diverse with decreasing powder size. The morphology and quantity of carbides depend on the thermal parameters and non-equilibrium solute partition coefficients during rapid solidification. - Highlights: Black-Right-Pointing-Pointer The relations of solidification thermal parameters with powder size are established. Black-Right-Pointing-Pointer The relation of non-equilibrium solute partition with powder size is investigated. Black-Right-Pointing-Pointer The solidification microstructure is related to thermal parameters. Black-Right-Pointing-Pointer The segregation behavior is linked to non-equilibrium partition coefficients. Black-Right-Pointing-Pointer The morphology and quantity of carbides depend on the above combined factors.

36 MATERIALS SCIENCE↗
DOE OSTI2012

High-output-power densities from molecular beam epitaxy grown n- and p-type PbTeSe-based thermoelectrics via improved contact metallization

Electrical power densities of up to 33 W/cm{sup 2} and up to 12 W/cm{sup 2} were obtained for n-type and p-type PbTeSe-based stand-alone thermoelectric devices, respectively, at modest temperature gradients of {approx}200 deg. C (T{sub cold}= 25 deg. C). These large power densities were enabled by greatly improving electrical contact resistivities in the thermoelectric devices. Electrical contacts with contact resistivities as low as 3.9 x 10{sup -6}{Omega} cm{sup 2} and 4.0 x 10{sup -6}{Omega} cm{sup 2} for n- and p-type telluride-based- materials, respectively, were developed by investigating several metallization schemes and contact layer doping/alloy combinations, in conjunction with a novel contact application process. This process exposes heated semiconductor surfaces to an atomic hydrogen flux under high vacuum for surface cleaning (oxide and carbon removal), followed immediately by an in-situ electron-beam evaporation of the metal layers.

36 MATERIALS SCIENCE↗
DOE OSTI2017

Hydride Microstructure at the Metal-Oxide Interface of a Zircaloy-4 Fuel Clad from the H.B. Robinson Nuclear Reactor

During nuclear reactor operation, some of the hydrogen that is produced by the water side corrosion is uptaken by cladding. When the uptaken hydrogen content exceeds its solubility limit in the cladding at a specific temperature, it precipitates as hydride particles in the cladding. This process occurs immediately at the metal-oxide interface forming a hydride rim because of the temperature gradient in the cladding. The presence of hydride rim and its microstructure severely reduces the cladding strength and can induce crack initiation and propagation during design basis accidents, transportation, and wet/dry storage. Because hydrides platelets are one of the potent crack initiation sites, microstructural characterization of hydride rim becomes essential to the safe operation of nuclear reactor and spent nuclear fuel retrievability. Therefore, we investigate the hydride rim microstructure at the metal oxide interface using scanning transmission electron microscopy (S/TEM) with Energy Dispersive X-ray Spectroscopy (EDS) that allows for the microstructural and local chemistry characterization of hydride precipitates to be determined, and enables a relationship to be derived on how the precipitate sites are affected by the oxide and their complex stacking behavior of the precipitates.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2018

Propagation of input parameter uncertainties in transport models

Here, the many sources of uncertainty in validation studies of plasma turbulence in magnetically confined fusion devices are well-known. In this paper, we investigate how to efficiently transform uncertainties in experimentally derived transport model inputs into model prediction uncertainties, using the quasilinear trapped-gyro-Landau-fluid (TGLF) turbulent transport model. We use the rapidly converging and computationally inexpensive non-intrusive probabilistic collocation method (PCM) to propagate input parameter uncertainty probability distribution functions (PDFs) through TGLF, yielding PDFs of predicted transport fluxes. We observe in many cases that the flux PDFs exhibit significant non-normal features such as strong skewness, even when the input distributions were normal. To illustrate the utility of the PCM approach, we apply this methodology to transport predictions for a DIII-D ITER baseline plasma in which the mix of neutral beam injection (NBI) and electron cyclotron heating (ECH) was varied. The model predictions show clear changes in the parametric dependencies and sensitivities of the turbulence between the two heating mixes. Specifically, when only NBI heating was used, the transport fluxes responded significantly only to the ion temperature gradient scale length. However, when both NBI and ECH were applied, the electron transport channels demonstrate a strong sensitivity to the electron temperature and density gradients not observed in the NBI-only case. Additional context for the PCM approach is provided by comparing its predictions with those obtained via a local flux-matching approach. A new set of validation metrics based on the Wasserstein distance is proposed for PDF-based comparisons.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2013

RELATIVE PHOTOMETRY OF HAT-P-1b OCCULTATIONS

We present Hubble Space Telescope (HST) Space Telescope Imaging Spectrograph observations of two occultations of the transiting exoplanet HAT-P-1b. By measuring the planet to star flux ratio near opposition, we constrain the geometric albedo of the planet, which is strongly linked to its atmospheric temperature gradient. An advantage of HAT-P-1 as a target is its binary companion ADS 16402 A, which provides an excellent photometric reference, simplifying the usual steps in removing instrumental artifacts from HST time-series photometry. We find that without this reference star, we would need to detrend the lightcurve with the time of the exposures as well as the first three powers of HST orbital phase, and this would introduce a strong bias in the results for the albedo. However, with this reference star, we only need to detrend the data with the time of the exposures to achieve the same per-point scatter, therefore we can avoid most of the bias associated with detrending. Our final result is a 2{sigma} upper limit of 0.64 for the geometric albedo of HAT-P-1b between 577 and 947 nm.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2019

Microstructure and Mechanical Properties of As-Cast γ-TiAl Alloys with Different Cooling Rates

γ-TiAl alloys composed of Ti-45Al-5Nb-1W-1B (at.%) solidified at three different cooling rates by vacuum electromagnetic induction melting under a controlled degree of vacuum of under 2 Pa. The influence of the cooling rate on the microstructure and mechanical properties of the γ-TiAl alloy samples was investigated. A relatively large temperature gradient at the beginning of solidification led to a thin fine-grained layer around the graphite mold, and undercooling had two main effects: (a) promoting nucleation in the grain-refining surface layer and (b) promoting the growth of columnar crystals beneath the surface. Moreover, all prepared ingots of this alloy could be clearly divided into Regions S, M and C from the surface to the core. The colony size of Region M was larger than those of the other two regions due to composition segregation and the growth of columnar grains. The existence of tungsten led to micro-inhomogeneity, and the mechanical properties of the alloy changed according to concentration fluctuations. The degrees of homogeneity were expressed as H{sub 0.1} and H{sub 0.2}. The alloy with the highest values, which possesses the best mechanical properties, solidified at a relatively low cooling rate. The deformation mechanism is also discussed.

36 MATERIALS SCIENCE↗
DOE OSTI2012

Effect of secondary convective cells on turbulence intensity profiles, flow generation, and transport

This paper reports the results of gyrokinetic simulation studies of ion temperature gradient driven turbulence which investigate the role of non-resonant modes in turbulence spreading, turbulence regulation, and self-generated plasma rotation. Non-resonant modes, which are those without a rational surface within the simulation domain, are identified as nonlinearly driven, radially extended convective cells. Even though the amplitudes of such convective cells are much smaller than that of the resonant, localized turbulence eddies, we find from bicoherence analysis that the mode-mode interactions in the presence of such convective cells increase the efficiency of turbulence spreading associated with nonlocality phenomena. Artificial suppression of the convective cells shows that turbulence spreading is reduced, and that the turbulence intensity profile is more localized. The more localized turbulence intensity profile produces stronger Reynolds stress and E Multiplication-Sign B shear flows, which in turn results in more effective turbulence self-regulation. This suggests that models without non-resonant modes may significantly underestimate turbulent fluctuation levels and transport.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2019

Laser 3D Printing of Fe-Based Bulk Metallic Glass: Microstructure Evolution and Crack Propagation

This work presents a comprehensive study of microstructure evolution, crack development and hardness performance of Fe-based bulk metallic glass parts processed by laser 3D printing. The combination of a low scan speed and high energy density generates a low temperature gradient, leading to supercooling and the formation of coarse dendrite and cellular crystal microstructure. Columnar dendrites grow in a single direction with large stress, and cracks are easily formed between the dendrites. The stress intensity factor (SIF) caused by the crack surface tension is small, the crack healing effect is weak, and it is difficult to prevent crack propagation. Cellular grain growth is uniform and more easily accommodates the strain, preventing crack initiation and propagation. In contrast, use of a high scan speed with low energy input produces a fine and uniform dendrite or even nanocrystalline, microstructure with microcracks. The SIF caused by the crack surface tension is large, and the crack healing effect is strong and prevents crack initiation and propagation. For low energy density, the hardness of the sample is similar to the hardness of the cast amorphous. This result indicates that the printing sample retained some amorphous characteristics.

36 MATERIALS SCIENCE↗
DOE OSTI2012

Ballooning theory of the second kind-two dimensional tokamak modes

The 2-D ballooning transform, devised to study local high toroidal number (n) fluctuations in axisymmetric toroidal system (like tokamaks), yields a well-defined partial differential equation for the linear eigenmodes. In this paper, such a ballooning equation of the second kind is set up for ion temperature gradient driven modes pertinent to a 2-D non-dissipative fluid plasma; the resulting partial differential equation is numerically solved, to calculate the global eigenvalues, and the 2-D mode structure is presented graphically along with analytical companions. The radial localization of the mode results from translational symmetry breaking for growing modes and is a vivid manifestation of spontaneous symmetry breaking in tokamak physics. The eigenmode, poloidally ballooned at {theta}={+-}{pi}/2, is radially shifted from associated rational surface. The global eigenvalue is found to be very close to the value obtained in 1-D parameterized ({lambda}={+-}{pi}/2) case. The 2-D eigenmode theory is applied to estimate the toroidal seed Reynolds stress [Y. Z. Zhang, Nucl. Fusion Plasma Phys. 30, 193 (2010)]. The solution obtained from the relatively simplified ballooning theory is compared to the solution of the basic equation in original coordinate system (evaluated via FFTs); the agreement is rather good.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2012

THERMAL AND CHEMICAL STRUCTURE VARIATIONS IN TITAN'S STRATOSPHERE DURING THE CASSINI MISSION

We have developed a line-by-line Atmospheric Radiative Transfer for Titan code that includes the most recent laboratory spectroscopic data and haze descriptions relative to Titan's stratosphere. We use this code to model Cassini Composite Infrared Spectrometer data taken during the numerous Titan flybys from 2006 to 2012 at surface-intercepting geometry in the 600-1500 cm{sup -1} range for latitudes from 50 Degree-Sign S to 50 Degree-Sign N. We report variations in temperature and chemical composition in the stratosphere during the Cassini mission, before and after the Northern Spring Equinox (NSE). We find indication for a weakening of the temperature gradient with warming of the stratosphere and cooling of the lower mesosphere. In addition, we infer precise concentrations for the trace gases and their main isotopologues and find that the chemical composition in Titan's stratosphere varies significantly with latitude during the 6 years investigated here, with increased mixing ratios toward the northern latitudes. In particular, we monitor and quantify the amplitude of a maximum enhancement of several gases observed at northern latitudes up to 50 Degree-Sign N around mid-2009, at the time of the NSE. We find that this rise is followed by a rapid decrease in chemical inventory in 2010 probably due to a weakening north polar vortex with reduced lateral mixing across the vortex boundary.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2016

ON THE NATURE OF X-RAY SURFACE BRIGHTNESS FLUCTUATIONS IN M87

X-ray images of galaxy clusters and gas-rich elliptical galaxies show a wealth of small-scale features that reflect fluctuations in density and/or temperature of the intracluster medium. In this paper we study these fluctuations in M87/Virgo to establish whether sound waves/shocks, bubbles, or uplifted cold gas dominate the structure. We exploit the strong dependence of the emissivity on density and temperature in different energy bands to distinguish between these processes. Using simulations we demonstrate that our analysis recovers the leading type of fluctuation even in the presence of projection effects and temperature gradients. We confirm the isobaric nature of cool filaments of gas entrained by buoyantly rising bubbles, extending to 7′ to the east and southwest, and the adiabatic nature of the weak shocks at 40″ and 3′ from the center. For features of ∼5–10 kpc, we show that the central 4′ × 4′ region is dominated by cool structures in pressure equilibrium with the ambient hotter gas while up to 30% of the variance in this region can be ascribed to adiabatic fluctuations. The remaining part of the central 14′ × 14′ region, excluding the arms and shocks described above, is dominated by apparently isothermal fluctuations (bubbles) with a possible admixture (at the level of ∼30%) of adiabatic (sound waves) and by isobaric structures. Larger features, of about 30 kpc, show a stronger contribution from isobaric fluctuations. The results broadly agree with a model based on feedback from an active galactic nucleus mediated by bubbles of relativistic plasma.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2016

Spin-current-driven thermoelectric generation based on interfacial spin-orbit coupling

The longitudinal spin Seebeck effect (SSE) in Bi{sub 2}O{sub 3}/Cu/yttrium-iron-garnet (YIG) devices has been investigated. When an out-of-plane temperature gradient is applied to the Bi{sub 2}O{sub 3}/Cu/YIG device, a spin current is generated across the Cu/YIG interface via the SSE and then converted into electric voltage due to the spin–orbit coupling at the Bi{sub 2}O{sub 3}/Cu interface. The sign of the SSE voltage in the Bi{sub 2}O{sub 3}/Cu/YIG devices is opposite to that induced by the conventional inverse spin Hall effect in Pt/YIG devices. The SSE voltage in the Bi{sub 2}O{sub 3}/Cu/YIG devices disappears in the absence of the Bi{sub 2}O{sub 3} layer and its thermoelectric conversion efficiency is independent of the Cu thickness, indicating the important role of the Bi{sub 2}O{sub 3}/Cu interface. This result demonstrates that not only the bulk inverse spin Hall effect but also the spin–orbit coupling near the interface can be used for SSE-based thermoelectric generation.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2013

The effect of magnetic flutter on residual flow

The hypothesis that stochastic magnetic fields disrupt zonal flows associated with ion temperature gradient turbulence saturation is investigated analytically with a residual flow calculation in the presence of magnetic flutter. The calculation starts from the time-asymptotic zero-beta residual flow of Rosenbluth and Hinton [Phys. Rev. Lett. 80, 724 (1998)] with the sudden application of an externally imposed, fixed magnetic field perturbation. The short-time electron response from radial charge loss due to magnetic flutter is calculated from the appropriate gyrokinetic equation. The potential evolution has quadratic behavior, with a zero crossing at finite time. The crossing time and its parametric dependencies are compared with numerical results from a gyrokinetic simulation of residual flow in the presence of magnetic flutter. The numerical and analytical results are in good agreement and support the hypothesis that the high-beta runaway of numerical simulations is a result of the disabling of zonal flows by finite-beta charge losses associated with magnetic flutter.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2017

Magneto-thermal reconnection processes, related mode momentum and formation of high energy particle populations

In the context of a two-fluid theory of magnetic reconnection, when the longitudinal electron thermal conductivity is relatively large, the perturbed electron temperature tends to become singular in the presence of a reconnected field component and an electron temperature gradient. A finite transverse thermal diffusivity removes this singularity while a finite ‘inductivity’ can remove the singularity of the relevant plasma displacement. Then (i) a new ‘magneto-thermal’ reconnection producing mode, is found with characteristic widths of the reconnection layer remaining significant even when the macroscopic distances involved are very large; (ii) the mode phase velocities can be both in the direction of the electron diamagnetic velocity as well in the opposite (ion) direction. A numerical solution of the complete set of equations has been carried out with a simplified analytical reformulation of the problem. A sequence of processes is analyzed to point out that high-energy particle populations can be produced as a result of reconnection events. These processes involve mode-particle resonances transferring energy of the reconnecting mode to a superthermal ion population and the excitation of lower hybrid waves that can lead to a significant superthermal electron population. The same modes excited in axisymmetric (e.g. toroidal) confinement configurations can extract angular momentum from the main body of the plasma column and thereby sustain a local ‘spontaneous rotation’ of it.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2016

Investigation of the effect of resistivity on scrape off layer filaments using three-dimensional simulations

The propagation of filaments in the Scrape Off Layer (SOL) of tokamaks largely determines the plasma profiles in the region. In a conduction limited SOL, parallel temperature gradients are expected, such that the resistance to parallel currents is greater at the target than further upstream. Since the perpendicular motion of an isolated filament is largely determined by balance of currents that flow through it, this may be expected to affect filament transport. 3D simulations have thus been used to study the influence of enhanced parallel resistivity on the dynamics of filaments. Filaments with the smallest perpendicular length scales, which were inertially limited at low resistivity (meaning that polarization rather than parallel currents determines their radial velocities), were unaffected by resistivity. For larger filaments, faster velocities were produced at higher resistivities due to two mechanisms. First parallel currents were reduced and polarization currents were enhanced, meaning that the inertial regime extended to larger filaments, and second, a potential difference formed along the parallel direction so that higher potentials were produced in the region of the filament for the same amount of current to flow into the sheath. These results indicate that broader SOL profiles could be produced at higher resistivities.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2013

TURBULENCE IN THE SUPERMODEL: MASS RECONSTRUCTION WITH NONTHERMAL PRESSURE FOR A1835

The total mass derived from X-ray emission is biased low in a large number of clusters when compared with the mass estimated via strong and weak lensing. Suzaku and Chandra observations out to the virial radius report in several relaxed clusters' steep temperature gradients that on assuming pure thermal hydrostatic equilibrium (HE) imply an unphysically decreasing mass profile. Moreover, the gas mass fraction appears to be inconsistent with the cosmic value measured from the cosmic microwave background. Such findings can be interpreted as evidence for an additional nonthermal pressure in the outskirts of these clusters. This nonthermal component may be due to turbulence stirred by residual bulk motions of extragalactic gas infalling into the cluster. Here, we present a SuperModel analysis of A1835 observed by Chandra out to the virial radius. The SuperModel formalism can include in the equilibrium a nonthermal component whose level and distribution are derived imposing that the gas mass fraction (f{sub gas}) equals the cosmic value at the virial radius. Including such a nonthermal component, we reconstruct from X-rays an increasing mass profile consistent with the HE also in the cluster outskirts and in agreement at the virial boundary with the weak-lensing value. The increasing f{sub gas} profile confirms that the baryons are not missing but located at the cluster outskirts.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

Mode-space energy distribution in instability-driven plasma turbulence

Energy transfer to damped modes in gyrokinetic ion temperature gradient driven turbulence is studied to understand the transfer dynamics and find scaling representations for the heavily populated mode space. Proper orthogonal and linear eigenmode decompositions are introduced and examined to assess whether modes are well-resolved and what scales they encompass. It is observed that damped modes across a range of inhomogeneous scales receive energy simultaneously and directly from the unstable mode, constituting a form of parallel transfer, distinct from the serial mode-to-mode transfer of the wavenumber cascade of hydrodynamic turbulence. Controlling for modes that are well resolved and labeling the modes of the linear decomposition in order of damping rate, energy transfer in the mode space satisfies an equipartition of the energy dissipation rate, leading to a simple rule for the distribution of energy in the space of damped modes. Energy dissipation rate equipartition is the form that the canonical nonlinear invariance of energy transfer assumes in a dissipation range with parallel rather than serial transfer.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗