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All sourcesNASA NTRSDOE OSTI
NASA NTRS1980

Plasma chemistry for inorganic materials

Practical application of plasma chemistry to the development of inorganic materials using both low temperature and warm plasmas are summarized. Topics cover: the surface nitrification and oxidation of metals; chemical vapor deposition; formation of minute oxide particles; the composition of oxides from chloride vapor; the composition of carbides and nitrides; freezing high temperature phases by plasma arc welding and plasma jet; use of plasma in the development of a substitute for petroleum; the production of silicon for use in solar cell batteries; and insulating the inner surface of nuclear fusion reactor walls.

Matsumoto, O.↗
NASA NTRS1980

Plasma double-layers produced by ponderomotive force

Non-linear rectification of the RF electric fields excited in a convectively amplifying electron beam-plasma interaction results in a dc electric field, and a corresponding ponderomotive force acting on the charged particles to produce a space-charge separation, i.e. a type of plasma double-layer. This paper analyses the effect, taking into account plasma electron temperature and electron-neutral collisions. To measure such double-layers, an electron beam probe constitutes a convenient non-perturbing diagnostic technique, but great care is required in its calibration. An analysis is presented taking into account significant non-linear effects which had been neglected in previous work. The paper concludes with some preliminary experimental results illustrating the use of the technique in a beam-plasma interaction for which a weak double-layer electric field is predicted.

Levine, J. S.↗
NASA NTRS1986

Condensation modes in sheared magnetic fields

The present study of the condensation modes in coronal cylindrical plasmas, with attention to magnetic shear effects on stability, notes that such shear is insignificant in the initiation of condensation in the case of low beta coronal plasmas. The effects of magnetic field shear, twist, and strength on condensation modes differ, depending on the wave vector. The stability of condensation modes strongly depends on the choice of equilibrium temperature and density profiles. If plasma temperature increases with twist but density does not, condensation modes are unstable for low field twist; by contrast, if plasma density increases with twist but temperature does not, condensation modes are unstable for high twist.

An, C.-H.↗
NASA NTRS1999

Subresolution Fibrillation in X-Ray Microflares Observed by Yohkoh SXT

We analyze the cooling of the X-ray plasma in microflares observed in active regions by the Yohkoh Soft X-ray Telescope (SXT). A typical microflare appears to be a transient brightening of an entire small magnetic loop, often having a diameter near the limit of resolution (approx. 2 x 10(exp 8) cm). The plasma heated to X-ray temperatures in the body of the loop cools by emission of XUV radiation and by heat conduction to the cooler plasma at the feet of the loop. The cooling rate is determined by the plasma temperature and density and the loop length. The plasma density is determined from the observed X-ray brightness of the loop in combination with the temperature, the loop diameter, and the filling factor. The filling factor is the volume fraction of the loop occupied by the subset of magnetic tubes that is fluid by the X-ray plasma and that contains practically all of the X-ray plasma present in the microflare loop. Taking typical values from the hundreds of microflares measured by Shimizu (X-ray brightness through the thin aluminum filter - 4 x 10(exp 3) DN/s/pixeL lifetime approx. 5 min, temperature approx. 6 x 10(exp 6) K, loop length approx. 10(exp 9) cm, loop diameter approx. 3 x 10(exp 8) cm), we find that for filling factors greater than approx. 1%: (1) the cooling time is much shorter than the duration of the microflare, and (2) conductive cooling strongly dominates over radiative cooling. Because the cooling time is so short and because the conductive heat flux goes mainly into increasing the plasma density via chromospheric evaporation, we are compelled to conclude that: (1) heating to X-ray temperatures continues through nearly the entire lifetime of the microflare, (2) die heating keeps changing to different field lines, so that any one magnetic tube in the sequence of heated tubes emits X-rays only briefly in the life of the microflare, and (3) at any instant during the microflare the tubes filled with X-ray plasma occupy only a small fraction (approx. 10%) of the microflare loop. Hence, we expect that coronal X-ray images with spatial resolution 2-3 times better than from the Yohkoh SXT will show plenty of rapidly changing filamentary substructure in microflares. Our results also suggest that the heating in microflares may result from progressive reconnection similar to that inferred in many larger flares.

Moore, Ron↗
DOE OSTI2020

Effective viscosities in a hydrodynamically expanding boost-invariant QCD plasma

Background: The near-equilibrium properties of a QCD plasma can be encoded into transport coefficients such as bulk and shear viscosity. In QCD, the ratio of these transport coefficients to entropy density, ζ/$\textit{s}$ and η/$\textit{s}$, depends nontrivially on the plasma's temperature. This is unlike in conformal systems where they take constant values such as η/$\textit{s}$ = 1/(4π). Purpose: In this work, we show that in a (0 + 1)D boost-invariant fluid with no transverse expansion, a temperature-dependent ζ/$\textit{s(T)}$ or η/$\textit{s(T)}$ can be described by an equivalent effective viscosity $\langleζ/s\rangle_{\text{eff}}$ or $\langleη/s\rangle_{\text{eff}}$. This effective viscosity combines the actual temperature-dependent ζ/$\textit{s(T)}$ or η/$\textit{s(T)}$ with the temperature profile of the fluid. Further, we extend the concept of effective viscosity in systems with transverse expansion and discuss how effective viscosities can be used to identify families of ζ/$\textit{s(T)}$ and η /$\textit{s(T)}$ that lead to similar hydrodynamic evolution. Methods: The Navier-Stokes relativistic hydrodynamic equations are used to provide a first definition of effective viscosity, in (0 + 1)D and (1 + 1)D. In the (0 + 1)D case, the analysis is extended to Israel-Stewart-type second-order hydrodynamics to clarify the effect of higher-order hydrodynamics corrections on the effective viscosity. Results: In a boost-invariant fluid with no transverse expansion [(0 + 1)D], the effective viscosity is expressed as a simple integral of ζ/$\textit{s(T)}$ or η/$\textit{s(T)}$ over temperature, with a weight determined by the speed of sound of the fluid. The result is general for any equation of state with a moderate temperature dependence of the speed of sound, including the QCD equation of state. This definition of effective viscosity can be used to identify infinite families of ζ/$\textit{s(T)}$ or η/$\textit{s(T)}$ that produce essentially indistinguishable temperature profiles. In a boost-invariant cylindrical system [(1 + 1)D], a similar definition of effective viscosity is obtained in terms of characteristic trajectories in time and transverse direction. This leads to an infinite number of constraints on an infinite functional space for ζ/$\textit{s(T)}$ and η/$\textit{s(T)}$. Realistic examples are presented by using a finite number of constraints on a finite functional space. Conclusions: The definition of effective viscosity in a (0 + 1)D system clarifies how infinite families of ζ/$\textit{s(T)}$ and η/$\textit{s(T)}$ can result in nearly identical hydrodynamic temperature profiles. By extending the study to a boost-invariant cylindrical [(1 + 1)D] fluid, we identify an approximate but more general definition of effective viscosity that highlights the potential and limits of the concept of effective viscosity in fluids with limited symmetries.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
NASA NTRS1975

Behavior of some singly ionized, heavy-ion impurities during compression in a theta-pinch plasma

The introduction of a small percentage of an impurity gas containing a desired element into a theta-pinch plasma is a standard procedure used to investigate the spectra and atomic processes of the element. This procedure assumes that the mixing ratio of impurity-to-fill gases remains constant during the collapse and heating phase. Spectroscopic investigations of the constant-mixing-ratio assumption for a 2% neon and argon impurity verifies the assumption only for the neon impurity. However, for the 2% argon impurity, only 20 to 25% of the argon is in the high-temperature compressed plasma. It is concluded that the constant-mixing-ratio assumption is not applicable to the argon impurity.

Jalufka, N. W.↗
DOE OSTI2024

Formation of a spherical plasma liner for plasma-jet-driven magneto-inertial fusion

Plasma-jet-driven magneto-inertial fusion is an alternative approach to controlled nuclear fusion, which aims to utilize a line-replaceable dense plasma liner as a repetitive spherical compression driver. In this experiment, first measurements of the formation of a spherical argon plasma liner formed from 36 discrete pulsed plasma jets are obtained on the Plasma Liner Experiment. Properties including liner uniformity and morphology, plasma density, temperature, and ram pressure are assessed as a function of time throughout the implosion process and indicate an apparent transition from initial kinetic inter-jet interpenetration to collisional regime near stagnation times, in accordance with theoretical expectation. A lack of primary shock structures between adjacent jets during flight implies that arbitrarily smooth liners may be formed by way of corresponding improvements in jet parameters and control. The measurements facilitate the benchmarking of computational models and understanding the scaling of plasma liners toward fusion-relevant energy density.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
NASA NTRS2008

Flare Plasma Iron Abundance

The equivalent width of the iron-line complex at 6.7 keV seen in flare X-ray spectra suggests that the iron abundance of the hottest plasma at temperatures >approx.10 MK may sometimes be significantly lower than the nominal coronal abundance of four times the photospheric value that is commonly assumed. This conclusion is based on X-ray spectral observations of several flares seen in common with the Ramaty High Energy Solar Spectroscopic Imager (RHESSI) and the Solar X-ray Spectrometer (SOXS) on the second Indian geostationary satellite, GSAT-2. The implications of this will be discussed as it relates to the origin of the hot flare plasma - either plasma already in the corona that is directly heated during the flare energy release process or chromospheric plasma that is heated by flare-accelerated particles and driven up into the corona. Other possible explanations of lower-than-expected equivalent widths of the iron-line complex will also be discussed.

Dennis, Brian R.↗
NASA NTRS1990

Hot plasma parameters in Neptune's magnetosphere

This paper presents values of particle spectral parameters and estimates of plasma densities, temperatures, and beta parameters, obtained with the Low Energy Charged Particle instrument during the Voyager 2 encounter with Neptune on August 24-25, 1989. In addition, trapped electron intensities are compared with the whistler mode stably trapped limits. The results revealed a very good inbound-outbound symmetry for both the proton and the electron profiles, suggesting that there was little dynamical activity in Neptune's magnetosphere during the Voyager encounter. The similarities and differences observed between Neptune and Uranus in the values of plasma density, pressure, and beta are discussed.

Krimigis, S. M.↗
NASA NTRS1994

The magnetosheath of Neptune: Models and observations

This paper gives a complete overview of the plasma and magnetic field in the magnetosheath of Neptune. A more sophisticated method is used to reanalyze the plasma data. This method provides better values of plasma density, velocity, and temperature in the magnetosheath both inbound and outbound from the planet than published previously. The data are compared to results obtained from a gasdynamic model of low around a planetary magnetosphere. Agreement of theory and data is good for some parameters and poor for others. We show that some discrepancies between the model predictions and observations may be due to changes in the solar wind parameters. The model results and data are used to check the hypothesis that Voyager encountered the high-latitude plasma mantle downstream from Neptune. The deviations of the data from the model results in this region are consistent with those expected for a mantle crossing, with the exception of the plasma temperature which decreases in one crossing and increases in the other. This may indicate that our knowledge of the nature of the mantle-magnetosheath boundary is not complete.

Richardson, John D.↗
NASA NTRS1985

Electromagnetic electron beam instabilities - Hot, isotropic beams

This paper considers the linear theory of electromagnetic instabilities driven by an electron beam in a homogeneous, nonrelativistic, Vlasov plasma. The beam is relatively hot, isotropic in its own frame, and streams parallel or antiparallel to a magnetic field B. Numerical solutions of the full dispersion equation for propagation parallel or antiparallel to B are presented, and the linear properties of the whistler heat flux and electron beam firehose instabilities are exhibited and compared. Under a broad range of parmameters the former mode has the lower beam speed threshold, and the larger maximum growth rate. In addition, it is demonstrated that, for a sufficiently large relative beam density, relative beam temperature, and plasma beta the whistler heat flux instability has a much lower beam speed threshold than the electrostatic electron beam instability. The application of these instabilities to first-order Fermi acceleration of electrons at space plasma shocks is discussed.

Gary, S. P.↗
NASA NTRS2010

Early Chromospheric Response During a Solar Microflare Observed with SOHO's CDS and RHESSI

We observed a solar microflare with RHESSI and SOHO's Coronal Diagnostic Spectrometer (CDS) on 2009 July 5. With CDS we obtained rapid cadence (7 s) stare spectra within a narrow field of view toward the center of AR 11024. The spectra contain emission lines from ions that cover a wide range of temperature, including He I (< 0.025 MK), O V (0.25 MK), Si XII (2 MK), and Fe XIX (8 MK). The start of a precursor burst of He I and O V line emission preceded the steady increase of Fe XIX line emission by about 1 minute, and the emergence of 3-12 keV X-ray emission by about 4 minutes. Thus the onset of the microflare was observed in upper chromospheric (He I) and transition region (O V) line emission before it was detected in high temperature flare plasma emission. Redshifted O V emission during the precursor suggests explosive chromospheric evaporation, but no corresponding blueshifts were found with either Fe XIX (which was very weak) or Si XII. Similarly, in subsequent microflare brightenings the O V and He I intensities increased (between 49 s and almost 2 minutes) before emissions from the hot flare plasma. Although these time differences likely indicate heating by a nonthermal particle beam, the RHESSI spectra provide no additional evidence for such a beam. In intervals lasting up to about 3 minutes during several bursts, the He I and O V emission line profiles showed secondary, highly blueshifted ( approximately 200 km/s) components; during intervals lasting nearly 1 minute the velocities of the primary and secondary components were oppositely directed. Combined with no corresponding blueshifts in either Fe XIX or Si XII, this indicates that explosive chromospheric evaporation occurred predominantly at either comparatively cool temperatures (< 2 MK) or within a hot temperature range to which our observations were not sensitive (e.g., between 2 and 8 MK).

Brosius, Jeffrey W.↗
DOE OSTI2022

Reduction in RF sheath rectification with insulating antenna enclosure walls

Abstract Radiofrequency (RF) sheath rectification is one of the most prominent deleterious effects associated with ion cyclotron range of frequencies (ICRF) heating in fusion plasmas. RF sheaths and associated effects, such as impurity generation and convective cell generation, need to be mitigated to ensure that ICRF is a viable option for heating in future fusion devices. Experiments were performed on the Large Plasma Device (LAPD) at UCLA to explore the effects of using electrically-insulating antenna enclosures on RF rectified sheaths. Three different enclosure side-wall materials were used, including copper, MACOR (electrically insulating), and MACOR over copper. In the case of the MACOR–copper side walls, the non-conductive MACOR material was exposed to the bulk plasma but a layer of copper was added below to allow for image currents to flow. All three of the experiments had similar plasma density, temperature, and background magnetic field. In the case of the copper enclosure, RF rectified potentials, many times the local electron temperature, and associated formation of convective cells were observed and reported Martin M. et al (2017 Phys. Rev. Lett. 119 205002). In the experiments with MACOR and MACOR–copper enclosures, RF rectification was significantly reduced. Additionally, these latter two experiments showed no evidence of convective cell formation. Although the results from the MACOR experiment are reminiscent of the results obtained in ASDEX-U with a three-strap antenna optimized to reduce image currents on the antenna limiters Bobkov V. et al (2016 Nucl. Fusion 56 084001), the MACOR–copper experiment seems to suggest that insulating plasma facing materials have at least an equally strong impact on reducing potential rectification.

Physics↗
NASA NTRS1971

Measurements of plasma parameters in a simulated thermionic converter

Cesium-filled thermionic energy converters are examined as candidate electrical energy sources in spacecraft requiring tens to hundreds of kilowatts of electric power. The high operating temperatures necessary for a large specific power and high efficiency inevitably impose stringent constraints on the converter fabrication to achieve the desired reliability of the power system. The converter physics for reducing operating temperatures and cesium plasma losses are studied to achieve high reliability without sacrificing the power performance of the converters. Various cesium parameters which affect the converter performance are: (1) electron temperatures, (2) plasma ion densities, and (3) electric potential profiles. These were investigated using a Langmuir probe in a simulated converter. The parameters were measured in different cesium discharge modes.

Shimada, K.↗
DOE OSTI2022

Ultrafast Laser Material Damage Simulation—A New Look at an Old Problem

The chirped pulse amplification technique has enabled the generation of pulses of a few femtosecond duration with peak powers multi-Tera and Peta–Watt in the near infrared. Its implementation to realize even shorter pulse duration, higher energy, and higher repetition rate laser systems relies on overcoming the limitations imposed by laser damage of critical components. In particular, the laser damage of coatings in the amplifiers and in post-compression optics have become a bottleneck. The robustness of optical coatings is typically evaluated numerically through steady-state simulations of electric field enhancement in multilayer stacks. However, this approach cannot capture crucial characteristics of femtosecond laser induced damage (LID), as it only considers the geometry of the multilayer stack and the optical properties of the materials composing the stack. This approach neglects that in the interaction of an ultrashort pulse and the materials there is plasma generation and associated material modifications. Here, we present a numerical approach to estimate the LID threshold of dielectric multilayer coatings based on strong field electronic dynamics. In this dynamic scheme, the electric field propagation, photoionization, impact ionization, and electron heating are incorporated through a finite-difference time-domain algorithm. We applied our method to simulate the LID threshold of bulk fused silica, and of multilayer dielectric mirrors and gratings. The results are then compared with experimental measurements. The salient aspects of our model, such as the implementation of the Keldysh photoionization model, the impact ionization model, the electron collision model for ‘low’-temperature, dense plasma, and the LID threshold criterion for few-cycle pulses are discussed.

36 MATERIALS SCIENCE↗
DOE OSTI2024

In Situ Monitoring of Non-Thermal Plasma Cleaning of Surfactant Encapsulated Nanoparticles

Surfactants are widely used in the synthesis of nanoparticles, as they have a remarkable ability to direct their growth to obtain well-defined shapes and sizes. However, their post-synthesis removal is a challenge, and the methods used often result in morphological changes that defeat the purpose of the initial controlled growth. Moreover, after the removal of surfactants, the highly active surfaces of nanomaterials may undergo structural reconstruction by exposure to a different environment. Thus, ex situ characterization after air exposure may not reflect the effect of the cleaning methods. Here, combining X-ray photoelectron spectroscopy, in situ infrared reflection absorption spectroscopy, and environmental transmission electron microscopy measurements with CO probe experiments, we investigated different surfactant-removal methods to produce clean metallic Pt nanoparticles from surfactant-encapsulated ones. It was demonstrated that both ultraviolet-ozone (UV-ozone) treatment and room temperature O2 plasma treatment led to the formation of Pt oxides on the surface after the removal of the surfactant. On the other hand, when H2 was used for plasma treatment, both the Pt0 oxidation state and nanoparticle size distribution were preserved. In addition, H2 plasma treatment can reduce Pt oxides after O2-based treatments, resulting in metallic nanoparticles with clean surfaces. These findings provide a better understanding of the various options for surfactant removal from metal nanoparticles and point toward non-thermal plasmas as the best route if the integrity of the nanoparticle needs to be preserved.

36 MATERIALS SCIENCE↗