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All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Gamma-Ray Emitting Radionuclides Concentrations and Decontamination Factors of ATR Loop Liquid Samples Cycle 171B

This report contains the gamma-ray emitting radionuclides concentration and decontamination factor results from gamma-ray spectrometry measurements of ATR loop liquid samples by the Radiation Measurements Laboratory (RML) for ATR Cycle 171B Jun. 20, 2023, to Sep. 27, 2023. This report consists of five subsections, one for each loop. Each subsection contains the results for each sampling of the loop along with the date and time of sampling, spectral data identifications, sample type, and reactor power (MW). The results are reported in units of disintegrations per minute per milliliter of sample. The results are obtained with the gamma-ray spectral data analysis routines of the RML computer. Some of this report is also generated by RML data storage and handling routines.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2024

Gamma-Ray Emitting Radionuclides Concentrations and Decontamination Factors of ATR Loop Liquid Samples: Cycle 172A

This report contains the gamma-ray emitting radionuclides concentration and decontamination factor results from gamma-ray spectrometry measurements of ATR loop liquid samples by the Radiation Measurements Laboratory (RML) for ATR Cycle 172A running March 2, 2024, to March 16, 2024. This report consists of five subsections, one for each loop. Each subsection contains the results for each sampling of the loop along with the date and time of sampling, spectral data identifications, sample type, and reactor power (MW). The results are reported in units of disintegrations per minute per milliliter of sample. The results are obtained with the gamma-ray spectral data analysis routines of the RML computer. Some of this report is also generated by RML data storage and handling routines.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2024

Phase II Final Technical Report: Dynamic Gamma-ray Imaging for In Vivo Tracking of Microelement Transport Across Plant-Microbial Systems

The Department of Energy Office of Biological and Environmental Research (DOE BER) Mesoscale to Molecules Bioimaging Technology Program aims to develop new imaging and measurement technology to enable in situ and dynamic imaging across a range of spatial and temporal scales. Various imaging modalities are required to span the complete spatiotemporal landscape for bioenergy and environmental bioimaging needs. The high-resolution gamma-ray spectroscopy, imaging, and sensitivity of new high-purity germanium (HPGe) instruments provide a unique opportunity to complement and enhance these research goals. The HPGe-based Gamma-ray Imager for Plant Research (GIPR) developed here provides non-invasive, in vivo measurements to dynamically track the uptake and distribution of multiple gamma-emitting radioactive elements simultaneously as they move from the soil microbiome into living plants. The hand portable GIPR utilizes commercially available radioisotopes to provide spatial and temporal imaging of plant microelement exchange for the broader scientific community.

Kiser, Matthew↗
DOE OSTI2024

Gamma-Ray Emitting Radionuclides Concentrations and Decontamination Factors of ATR Loop Liquid Samples Cycle 173A Revision 0

This report contains the gamma-ray emitting radionuclides concentration and decontamination factor results from gamma-ray spectrometry measurements of ATR loop liquid samples by the Radiation Measurements Laboratory (RML) for ATR Cycle 173A running May 3, 2024, to July 6, 2024. This report consists of five subsections, one for each loop. Each subsection contains the results for each sampling of the loop along with the date and time of sampling, spectral data identifications, sample type, and reactor power (MW). The results are reported in units of disintegrations per minute per milliliter of sample. The results are obtained with the gamma-ray spectral data analysis routines of the RML computer. Some of this report is also generated by RML data storage and handling routines.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2024

Scoping Study: Highly Enriched Uranium Isotopic Assessments Using Gamma Spectroscopy Relative Efficiency Analysis When No Uranium-232 Is Present

This report documents results for a scoping study evaluating the viability of using the higher energy, low yield U-235 gamma emission at 345.9 keV to link low energy U-235 emissions to high energy U-238 emissions (rather than U-232 decay products gamma emissions) for highly enriched uranium isotopic gamma spectroscopy relative efficiency assessments when no or little U-232 is present and the U-235 signal is strong.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2024

Radioisotope Identification with List-Mode Gamma Ray Data: A rigorous assessment on the value of temporal information applied to radioisotope identification.

This work explores the potential of utilizing temporal data from gamma-ray detectors, known as list-mode data, to enhance radioisotope identification. Traditional identification methods, which rely on full gamma-ray spectrum analysis, often require long dwell times and struggle with “confuser” sources, or spectra with similarly spaced spectral peaks. We hypothesize that by leveraging the probabilistic nature of nuclear decay and the time-encoded information from decay sequences and interactions with surrounding materials, we can improve classification accuracy over static spectral analysis. This research rigorously examines the temporal content of list-mode data through exploratory data analysis via correlation discovery and information theory. We further propose a basic classification model that can utilize spectral or temporal data (or both) to determine if the incorporation of temporal information can improve radioisotope identification. The findings suggest that the temporal information present in list-mode gamma-ray data has merit and should be further investigated.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2025

Ratio of 1,275 and 186 keV Gamma Ray Count Rates for Age Determination of Material in UF 6 Cylinders

In this work, a method for using ratios of passive gamma ray measurements to determine the time since the filling of UF 6 cylinders was explored. This method uses the 186 keV gamma ray emitted by 235 U and the 1,275 keV gamma ray that results from interactions of alpha particles in fluorine. Studies were made using MCNP models of both 30B cylinders and smaller 5A cylinders. Results indicate that for enrichments at or above that of natural uranium, this approach may provide a method for determining age up to 10 years or identifying whether the age is greater than 10 years, even if the uranium enrichment is unknown. The calculated results show the same behavior as the results of a recent measurement campaign, indicating the possibility of using this method for real-world cylinders.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2025

Testing, Calibration, and UxS Integration of the Kromek GR1 Plus CZT Gamma Spectrometer

Collecting radiation measurements can be a hazardous task, especially in the presence of highly active sources. Various scenarios necessitate source search, classification, and quantification, often with limited or no a priori information. Activities such as disaster mitigation, emergency response, environmental monitoring, and site remediation may involve dangerous radioactive sources. In these situations, there is a pressing need for remote monitoring capabilities that protect human operators from potential harm and enhance adherence to the principle of “As Low as Reasonably Achievable” (ALARA) for radiation doses. The first step toward achieving remote radiation measurement capabilities is the remote operation of a radiation sensor. Once this milestone is reached, the next challenge is to integrate this remote sensing capability into suitable actuation agents, collectively referred to as uncrewed systems (UxS). These systems include familiar platforms such as robotic quadrupeds, aerial multirotor vehicles, and ground vehicles, any of which may be teleoperated, act autonomously, or utilize a combination of both. A critical factor in achieving remote radiation sensing is the availability of data from the appropriate sensor. Many commercially available radiation sensors have closed-source documentation for their communication protocols. Typical end-user products are often self-contained, handheld devices designed for manual measurement scenarios. While there are commercial off-the-shelf (COTS) integrations of radiation sensors with UxS available for purchase, these solutions are typically tailored for specific use cases and may not meet the requirements of different applications. This paper discusses efforts to remotely acquire radiation measurements from a small form-factor CZT gamma spectrometer. Sandia National Laboratories has successfully demonstrated the initial capability to integrate low size, weight, and power (SWaP) gamma spectroscopy into various UxS, alongside co-located GPS data logging and sensor calibration and qualification. With remote gamma spectroscopy achieved, the stage is set for UxS integration of this capability.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2023

Cosmic Supernova Neutrino and Gamma-Ray Backgrounds in the MeV Regime

Cosmic multimessenger backgrounds include relic diffuse components created in the early universe and contributions from individual sources. Here, we study both type Ia supernovae (SNe Ia) and core-collapse supernovae (CCSNe) contributions to the diffuse neutrino and gamma-ray backgrounds in the MeV regime referred to as DSNB and DSGB respectively. We show that the diffuse SN Ia background is 10 6 times lower (for $\overline{v}_e$) than the CCSN background making it negligible. Our predicted DSNB $\overline{v}_e$ flux at earth in the 19.3–32 MeV regime is 0.36 ν cm -2 s -1 . We also find that the DSNB flux in the energy range from 11.3 to 32 MeV varies by +29% with a change in the SFRD model from Madau & Fragos which yielded a minimum predicted flux, to the extragalactic background light reconstruction model (maximum predicted flux). The diffuse SN Ia gamma-ray background and its dependence on the progenitor supernova delay time distribution are also evaluated. Furthermore, we address the origin of the CGB (Cosmic Gamma-ray Background) in the 0.1–7 MeV regime by adding contributions from sources such as SNe Ia, CCSNe, radio-quiet Active Galactic Nuclei, Flat spectrum radio quasars (FSRQs) and Neutron star—neutron star mergers. We find that our modeled background (including uncertainties) matches the observed CGB above 1.0 MeV, but is a factor ≈2 lower than the observed flux in the 0.1–1.0 MeV range, highlighting the need for future MeV missions to establish the CGB spectrum more reliably, and to possibly identify additional sources or even source classes in the underexplored MeV band.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2023

A Multiwavelength Investigation of PSR J2229+6114 and its Pulsar Wind Nebula in the Radio, X-Ray, and Gamma-Ray Bands

Abstract G106.3+2.7, commonly considered to be a composite supernova remnant (SNR), is characterized by a boomerang-shaped pulsar wind nebula (PWN) and two distinct (“head” and “tail”) regions in the radio band. A discovery of very-high-energy gamma-ray emission (E γ > 100 GeV) followed by the recent detection of ultrahigh-energy gamma-ray emission (E γ > 100 TeV) from the tail region suggests that G106.3+2.7 is a PeVatron candidate. We present a comprehensive multiwavelength study of the Boomerang PWN (100″ around PSR J2229+6114) using archival radio and Chandra data obtained two decades ago, a new NuSTAR X-ray observation from 2020, and upper limits on gamma-ray fluxes obtained by Fermi-LAT and VERITAS observatories. The NuSTAR observation allowed us to detect a 51.67 ms spin period from the pulsar PSR J2229+6114 and the PWN emission characterized by a power-law model with Γ = 1.52 ± 0.06 up to 20 keV. Contrary to the previous radio study by Kothes et al., we prefer a much lower PWNB-field (B∼ 3μG) and larger distance (d∼ 8 kpc) based on (1) the nonvarying X-ray flux over the last two decades, (2) the energy-dependent X-ray size of the PWN resulting from synchrotron burn-off, and (3) the multiwavelength spectral energy distribution (SED) data. Our SED model suggests that the PWN is currently re-expanding after being compressed by the SNR reverse shock ∼1000 yr ago. In this case, the head region should be formed by GeV–TeV electrons injected earlier by the pulsar propagating into the low-density environment.

Astronomy & Astrophysics↗
DOE OSTI2025

Wino and Real Minimal Dark Matter Excluded by Fermi Gamma-Ray Observations

We show that minimal, fermionic dark matter (DM) models in the $n$-dimensional representation of the weak force with zero hypercharge that make up 100% of the DM under the standard cosmological history are strongly excluded for $n < 9$. This includes the thermal wino, which we show is ruled out even allowing for DM core sizes up to $\sim$6.7 kpc with the preferred local DM density or $\sim$3.7 kpc in addition to the local DM density being half the preferred value, at less than $0.2$ GeV/cm$^3$. We reach these conclusions through dedicated searches with 14 years of Fermi gamma-ray data in the inner Galaxy between 30 GeV and 2 TeV for the continuum gamma-rays produced in the decays of unstable particles produced in DM annihilation and bound-state formation processes. We consider a variety of Milky Way DM profiles in our analyses, including those motivated by modern hydrodynamic cosmological simulations, and show that all the $n < 9$ minimal DM models are disfavored even under the most conservative assumptions for these density profiles. While wino, quintuplet ($n=5$), and $n = 7$ DM models are strongly disfavored by our analyses under the standard cosmology, we discuss how non-standard cosmological histories or DM sub-fractions could still allow for these particles to be realized in nature, with discovery opportunities at next-generation particle colliders and gamma-ray telescopes.

Cosmology and Nongalactic Astrophysics (astro-ph.C↗
NASA NTRS1972

Effect of continuous gamma-ray exposure on performance of learned tasks and effect of subsequent fractionated exposures on blood-forming tissue

Sixteen monkeys trained to perform continuous and discrete-avoidance and fixed-ratio tasks with visual and auditory cues were performance-tested before, during, and after 10-day gamma-ray exposures totaling 0, 500, 750, and 1000 rads. Approximately 14 months after the performance-test exposures, surviving animals were exposed to 100-rad gamma-ray fractions at 56-day intervals to observe injury and recovery patterns of blood-forming tissues. The fixed-ratio, food-reward task performance showed a transient decline in all dose groups within 24 hours of the start of gamma-ray exposure, followed by recovery to normal food-consumption levels within 48 to 72 hours. Avoidance tasks were performed successfully by all groups during the 10-day exposure, but reaction times of the two higher dose-rate groups in which animals received 3 and 4 rads per hour or total doses of 750 and 1000 rads, respectively, were somewhat slower.

Spalding, J. F.↗
NASA NTRS1972

The design of a source to simulate the gamma-ray spectrum emitted by a radioisotope thermoelectric generator

A simulated source was designed to duplicate the gamma spectrum of a uniform cylindrical 2200-watt Pu02 radioisotope thermoelectric generator containing 81% Pu-238 and 1.2 ppm Pu-236. Gamma rays from the decay of Pu-238, Am-241, Pu-239, and the 0-18(alpha,n)Ne-21 reaction were catalogued in broad energy groups. Two 46- and one 22-mc Th-228 sources provided simulation at various times in the life of the fuel capsule up to 18 years, which covers the time span of an outer planet mission. Emission from Th-228 represents the overwhelming contribution of the gamma spectrum after the first few years. The sources, in the form of 13-inch rods, were placed in a concentric hole in a cylinder of depleted uranium, which provided shielding equivalent to the self-shielding of the fuel capsule. The thickness of the U-238 cylinder (0.55cm) was determined by Monte Carlo calculations to insure that the spectrum emerging from the simulated source matched that of the fuel capsule.

Reier, M.↗
NASA NTRS1972

Some neutron and gamma radiation characteristics of plutonium cermet fuel for isotopic power sources

Gamma and neutron measurements on various types of plutonium sources are presented in order to show the effects of O-17, O-18 F-19, Pu-236, age of the fuel, and size of the source on the gamma and neutron spectra. Analysis of the radiation measurements shows that fluorine is the main contributor to the neutron yields from present plutonium-molybdenum cermet fuel, while both fluorine and Pu-236 daughters contribute significantly to the gamma ray intensities.

Neff, R. A.↗
NASA NTRS1972

The response of a 0.03-cm silicon detector to a mixed neutron and gamma field as a function of shield material and thickness

The neutron and gamma radiation from a MHW-RTG was used to evaluate the total response of a shielded 0.3-mm silicon detector. The generator employs a 2200 W(th) PuO2 heat source concept known as the HELIPAK. The total integrated neutron and gamma ray fluxes at 100 cm away from the source along the radial direction were 1.67 x 1,000 n/sq cm/s and 1.49 x 10,000 gamma sq cm/s, respectively. Experimental values of the response function of the shielded silicon detector were used to determine the total counting rates due to photons at bias energies ranging from 50 to 200 keV. For neutrons, analytically computed response functions were used to determine the total counting rates at the same bias energies. It was found that for an aluminum shield the neutrons are not significant, regardless of the thickness of the shield. However, the magnitude of the total counting rate due to neutrons increases with increased atomic number of the shield and becomes comparable to the counting rate due to photons for a platinum shield thickness of 5 cm.

Taherzadeh, M.↗
NASA NTRS1972

Gamma-ray observations of the galactic center and some possible point sources.

A 0.5 x 0.5-m digitized spark-chamber gamma-ray telescope was flown on three balloon flights to look at the galactic center region, Virgo, and the Crab Nebula. An excess flux above atmospheric background of over 4 standard deviations was found for gamma-rays exceeding 100 MeV coming from the galactic center region, but there was no statistically significant excess in the 50-100 MeV interval. As a result, there is only a 6% chance that Compton or synchrotron radiation from electrons with a power-law spectrum having an exponent of 2.6 could make as much as a 50% contribution to the gamma-radiation in this energy range.

Fitchtel, C. E.↗
NASA NTRS1972

A gamma ray monitor for the OSO-7 spacecraft.

A NaI(T2) gamma ray spectrometer with a CsI(Na) charged particle and anti-Compton shield has been developed for the spacecraft. The spacecraft telemetry system employs a 800 Hz clock and reads data out on a basic 32-word (byte) Main Frame cycle. The data from the instrument include spectral data, X-ray data, and housekeeping data. The gamma ray pulses from the anode of the central detector flow through the front end electronics, where they are amplified by a charge sensitive preamplifier. The admission of the desired gamma ray into the data stream is controlled by a linear gate.

Higbie, P. R.↗
NASA NTRS1972

Gamma-neutrino angular correlations in muon capture.

Using a high-resolution Ge(Li) spectrometer, it proved possible to observe several Doppler-broadened gamma-ray transitions in Al-28 excited by muon capture in Si-28. Several of these transitions are shown to be suitable for analysis in terms of angular correlations between the neutrino and a deexcitation nuclear gamma-ray. The observed transitions are interpreted in terms of gamma-neutrino correlation coefficients which are functions of the weak-interaction coupling constants.

Miller, G. H.↗