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At least 1,027 records · Page 57

Two-phase models of quasar emission line regions

It is demonstrated that the emitting gas in clouds of quasar emission line regions must be confined by a hot intercloud medium, provided only that the heating mechanisms are strong enough to drive the low-density intercloud gas above a few tens of millions degrees K. The study of the thermal properties of the gas presented includes heating by photoionization, Compton scattering, suprathermal particles, absorption of radio frequency radiation, cloud friction, thermal conduction, and shocks. Cooling curves for photoionized gases are presented, and phase diagrams analogous to the pressure-temperature diagrams used in studying the interstellar medium are constructed for various conditions. It is shown that two-phase equilibria occur over a wide range of mean density, but over a much narrower range of pressure. The implications of these results for the emission line region are discussed, and it is shown that the emission clouds may be short-lived.

Krolik, J. H.↗

Spectrally-Invariant Approximation Within Atmospheric Radiative Transfer

Certain algebraic combinations of single scattering albedo and solar radiation reflected from, or transmitted through, vegetation canopies do not vary with wavelength. These "spectrally invariant relationships" are the consequence of wavelength independence of the extinction coefficient and scattering phase function in vegetation. In general, this wavelength independence does not hold in the atmosphere, but in cloud~dominated atmospheres the total extinction and total scattering phase function vary only weakly with wavelength. This paper identifies the atmospheric conditions under which the spectrally invariant approximation can accurately describe the extinction. and scattering properties of cloudy atmospheres. The validity of the assumptions and the accuracy of the approximation are tested with ID radiative transfer calculations using publicly available radiative transfer models: Discrete Ordinate Radiative Transfer (DISORT) and Santa Barbara DISORT Atmospheric Radiative Transfer (SBDART). It is shown for cloudy atmospheres with cloud optical depth above 3, and for spectral intervals that exclude strong water vapor absorption, that the spectrally invariant relationships found in vegetation canopy radiative transfer are valid to better than 5%. The physics behind this phenomenon, its mathematical basis, and possible applications to remote sensing and climate are discussed.

Marshak, A.↗

Venus' spectroscopic phase variation - Implications of the Mariner 10 photographs

The recent ultraviolet photographs of Venus by Mariner 10 have shown an irregular cloud structure. There is an apparent tendency for clearing along a wide equatorial band more or less centered on the subsolar point. This synoptic picture is in marked contrast to the uniform cloud cover conventionally used in model calculations of the variation with phase of CO2 absorption bands. To illustrate the consequences of subsolar weakening of CO2 absorption, a mathematically simple (but realistically naive) model is used. Two conclusions are reached: (1) efforts to distinguish between single- and double-layer models for the clouds from spectroscopic data alone are not merely ambiguous (as argued earlier by Chamberlain and Smith); with present data they are hopeless; (2) the decrease in the CO2 absorption close to full phase, as reported by Young et al., could result entirely from an equatorial darkening that is relatively inconsequential at the crescent phase and increasingly predominant for fuller phases.

Chamberlain, J. W.↗

High-resolution spectra of Io's sodium emission

The shape of Io's sodium D2 emission profile varies markedly with Io's orbital phase, and its width suggests that the sodium cloud may be expanding with velocities up to 18 km/sec. This offers an explanation for at least part of the orbital phase asymmetry observed for the D-line emission.

Trafton, L.↗

Circumpolar hoods and clouds and their relation to the Martian H2O cycle

Water exists in both vapor and solid phases in the Martian atmosphere. The polar hoods are shrouds of condensate clouds which obscure both polar regions at times during their respective fall and winter seasons. The hemispheric asymmetries in the polar hood clouds are reviewed and their significance to the seasonal water cycle is discussed. Comparisons of images acquired using short wavelength filters, which provide maximum cloud contrast, and long wavelength filters, which are sensitive to surface features including the surface cap, provide correlations between cloud formation and large scale planetary dynamics.

James, Philip B.↗

Field Validation of Cloud Properties Sensor (SAIL Field Campaign Report)

The purpose of the Field Validation of Cloud Properties Sensor – SAIL campaign was to deploy Aerodyne’s extended-wavelength TWST cloud optical properties sensor (TWST-CPS) in an operationally relevant environment with co-located, externally validated sensors. Colocation with The U.S. Department of Energy Atmospheric Radiation Measurement (ARM) user facility’s deployment of its second Mobile Facility (AMF2) on the Surface Atmosphere Integrated Field Laboratory (SAIL) campaign at Crested Butte, Colorado was ideal because of the variety of operational sensors that can measure some of the same cloud properties using different modalities. While cloud property sensors have long existed, they tend to be costly to produce and maintain. Our sensor measures absolute spectral radiance over 440-1700 nm and retrieves cloud optical depth (COD), droplet effective radius (Reff), and thermodynamic phase (Phase). Our prototype is built predominantly from off-the-shelf components and uses uncooled spectrometers. A low-cost, easy-to-use sensor such as this could allow deployment at many more sites for greater spatial coverage. Instrument deployment to test robust operations and a new stray-light baffle design, and the continued development of analysis and retrieval algorithms using the data from this deployment, are central technical objectives of Aerodyne Research’s U.S. Department of Energy Small Business Innovative Research Phase 2 contract (DE-SC0020473, Low-cost shortwave spectroradiometer for retrieval of cloud properties).

54 ENVIRONMENTAL SCIENCES↗

Field Validation of Cloud Properties Sensor – SAIL Field Campaign Report

The purpose of the Field Validation of Cloud Properties Sensor – SAIL campaign was to deploy Aerodyne’s extended-wavelength TWST cloud optical properties sensor (TWST-CPS) in an operationally relevant environment with co-located, externally validated sensors. Colocation with The U.S. Department of Energy Atmospheric Radiation Measurement (ARM) user facility’s deployment of its second Mobile Facility (AMF2) on the Surface Atmosphere Integrated Field Laboratory (SAIL) campaign at Crested Butte, Colorado was ideal because of the variety of operational sensors that can measure some of the same cloud properties using different modalities. While cloud property sensors have long existed, they tend to be costly to produce and maintain. Our sensor measures absolute spectral radiance over 440-1700 nm and retrieves cloud optical depth (COD), droplet effective radius (Reff), and thermodynamic phase (Phase). Our prototype is built predominantly from off-the-shelf components and uses uncooled spectrometers. A low-cost, easy-to-use sensor such as this could allow deployment at many more sites for greater spatial coverage. Instrument deployment to test robust operations and a new stray-light baffle design, and the continued development of analysis and retrieval algorithms using the data from this deployment, are central technical objectives of Aerodyne Research’s U.S. Department of Energy Small Business Innovative Research Phase 2 contract (DE-SC0020473, Low-cost shortwave spectroradiometer for retrieval of cloud properties).

54 ENVIRONMENTAL SCIENCES↗

Simulating the Transport and Rupture of Pollen in the Atmosphere

Pollen, one type of primary biological aerosol particle (PBAP), is emitted from the terrestrial biosphere and can undergo physical changes in the atmosphere via particle rupture. To examine the fate of pollen and its atmospheric processing, a pollen emission and transport scheme is coupled to the Weather Research and Forecasting Model with Chemistry (WRF-Chem). We simulate the emission of pollen and its impacts on the cloud properties and precipitation in the Southern Great Plains from 12 to 19 April 2013, a period with both high pollen emissions and convective activity. We conduct a suite of ensemble runs that simulate primary pollen and three different pollen rupture mechanisms that generate subpollen particles, including (a) high humidity-induced surface rupture, (b) high humidity-induced in-atmosphere plus surface rupture, and (c) lightning-induced rupture, where in-cloud and cloud-to-ground lightning strikes trigger pollen rupture events. When relative humidity is high (>80%), coarse primary pollen (~1 μg m –3 ) is converted into fine subpollen particles (~1.2e –4 μg m –3 ), which produces 80% more subpollen particles than lightning-induced rupture. The in-atmosphere humidity-driven rupture predominantly produces subpollen particles, which is further enhanced during a frontal thunderstorm. During strong convection, vertical updrafts lift primary pollen and subpollen particles (~0.5e –4 μg m –3 ) to the upper troposphere (~12 km) and laterally transports the ruptured pollen in the anvil top outflow. In regions of high pollen and strong convection, ruptured pollen can influence warm cloud formation by decreasing low cloud (<4 km) cloud water mixing ratios and increasing ice phase hydrometeors aloft (>10 km)

54 ENVIRONMENTAL SCIENCES↗

Scattering in the atmosphere of Venus. III - Line profiles and phase curves for Rayleigh scattering

Spectral line profiles, curves of growth, and curves for the equivalent width of a line as a function of Venus phase angle have been computed for a Rayleigh scattering cloud and compared with those for a cloud of isotropic scatterers. The results are very similar for the two kinds of scattering, with the exception of the curves of equivalent width as a function of Venus phase angle. These latter curves exhibit the 'inverse phase effect' and rule out a scale height of the clouds much less than half the scale height of the gas. The optical depth of the clouds is approximately 100.

Young, L. D. G.↗

A Fourier approach to cloud motion estimation

A Fourier technique is described for estimating cloud motion from pairs of pictures using the phase of the cross spectral density. The method allows motion estimates to be made for individual spatial frequencies, which are related to cloud pattern dimensions. Results obtained are presented and compared with the results of a Fourier domain cross correlation scheme. Using both artificial and real cloud data show that the technique is relatively sensitive to the presence of mixtures of motions, changes in cloud shape, and edge effects.

Arking, A.↗

Larger Cloud Liquid Water Enhances Both Aerosol Indirect Forcing and Cloud Radiative Feedback in Two Earth System Models

Previous studies have noticed that the Coupled Model Intercomparison Project Phase 6 (CMIP6) models with a stronger cooling from aerosol-cloud interactions (ACI) also have an enhanced warming from positive cloud feedback, and these two opposing effects are counter-balanced in simulations of the historical period. However, reasons for this anti-correlation are less explored. In this study, we perturb the cloud ice microphysical processes to obtain cloud liquid of varying amounts in two Earth System Models (ESMs). We find that the model simulations with a larger liquid water path (LWP) tend to have a stronger cooling from ACI and a stronger positive cloud feedback. More liquid clouds in the mean-state present more opportunities for anthropogenic aerosol perturbations and also weaken the negative cloud feedback at middle to high latitudes. This work, from a cloud state perspective, emphasizes the influence of the mean-state LWP on effective radiative forcing due to ACI (ERF ACI ).

54 ENVIRONMENTAL SCIENCES↗

Spectrally Invariant Approximation within Atmospheric Radiative Transfer

Certain algebraic combinations of single scattering albedo and solar radiation reflected from, or transmitted through, vegetation canopies do not vary with wavelength. These spectrally invariant relationships are the consequence of wavelength independence of the extinction coefficient and scattering phase function in vegetation. In general, this wavelength independence does not hold in the atmosphere, but in cloud-dominated atmospheres the total extinction and total scattering phase function vary only weakly with wavelength. This paper identifies the atmospheric conditions under which the spectrally invariant approximation can accurately describe the extinction and scattering properties of cloudy atmospheres. The validity of the assumptions and the accuracy of the approximation are tested with 1D radiative transfer calculations using publicly available radiative transfer models: Discrete Ordinate Radiative Transfer (DISORT) and Santa Barbara DISORT Atmospheric Radiative Transfer (SBDART). It is shown for cloudy atmospheres with cloud optical depth above 3, and for spectral intervals that exclude strong water vapor absorption, that the spectrally invariant relationships found in vegetation canopy radiative transfer are valid to better than 5%. The physics behind this phenomenon, its mathematical basis, and possible applications to remote sensing and climate are discussed.

Marshak, A.↗

Chemistry of a polluted cloudy boundary layer

A one-dimensional photochemical model for cloud-topped boundary layers has been developed to include descriptions of gas- and aqueous-phase chemistry and the radiation field in and below the cloud. The model is applied to the accumulation of pollutants during a wintertime episode with low stratus over Bakersfield, CA. The mechanisms of sulfate production and the balance between the concentrations of acids and bases are examined. It is shown that most of the sulfate production may be explained by the Fe(III)-catalyzed autoxidation of S(IV). Another source of sulfate is the oxidation of SO2 by OH in both the gas and the aqueous phase. It is shown that the sulfate production in the model is controlled by the availability of NH3. It is suggested that this explains the balance observed between total concentration of acids and bases.

Jacob, Daniel J.↗

Shielding of CO from dissociating radiation in interstellar clouds

The paper investigates the photodissociation of CO in interstellar clouds in the light of recent laboratory studies which suggest that line rather than continuum processes dominate its dissociation by ultraviolet radiation. Using a simple radiative transfer model, the shielding of representative dissociating bands is estimated, including self-shielding, mutual shielding between different isotopes, and near coincidences with strong lines of H2. Each of these processes materially affects the photodestruction rates of the various isotopic species in the transition regions of molecular clouds. These results are combined with an appropriate gas phase chemical model to determine how the abundances of the CO isotopes vary with depth into the cloud. It is found that self-shielding and mutual shielding cause significant variations in isotopic ratios. In addition, fractionation enhances species containing C-13. The relationship between the column densities of CO and H2 is found to vary for the different isotopes and to be sensitive to local conditions.

Glassgold, A. E.↗

Jumping the Queue: From NASA to the Commercial Cloud

NASA's High-End Computing Capability (HECC) Project has made it possible for its users to run on commercial cloud resources in a seamless way. In the first of three phases, we implemented a pilot project for a few users, enabling them to “jump the queue” and burst jobs from the HECC environment to Amazon Web Services (AWS). By using GPU-accelerated nodes at AWS, the users were able to make significant advances in their research. The second phase of the project made AWS access available to all HECC users and added accounting to make users responsible for cloud charges. We are also enabling export-controlled work through the use of AWS GovCloud. In the third phase, we will add web-based mechanisms to permit non-HECC users to access cloud resources for their HPC projects.

Hood, Robert↗

Consequences of hot gas in the broad line region of active galactic nuclei

Models for hot gas in the broad line region of active galactic nuclei are discussed. The results of the two phase equilibrium models for confinement of broad line clouds by Compton heated gas are used to show that high luminosity quasars are expected to show Fe XXVI L alpha line absorption which will be observed with spectrometers such as those planned for the future X-ray spectroscopy experiments. Two phase equilibrium models also predict that the gas in the broad line clouds and the confining medium may be Compton thick. It is shown that the combined effects of Comptonization and photoabsorption can suppress both the broad emission lines and X-rays in the Einstein and HEAO-1 energy bands. The observed properties of such Compton thick active galaxies are expected to be similar to those of Seyfert 2 nuclei. The implications for polarization and variability are also discussed.

Kallman, T.↗

Consequences of hot gas in the broad-line region of active galactic nuclei

Models for hot gas in the broad line region of active galactic nuclei are discussed. The results of the two phase equilibrium models for confinement of broad line clouds by Compton heated gas are used to show that high luminosity quasars are expected to show Fe XXVI L alpha line absorption which will be observed with spectrometers such as those planned for the future X-ray spectroscopy experiments. Two phase equilibrium models also predict that the gas in the broad line clouds and the confining medium may be Compton thick. It is shown that the combined effects of Comptonization and photoabsorption can suppress both the broad emission lines and X-rays in the Einstein and HEAO-1 energy bands. The observed properties of such Compton thick active galaxies are expected to be similar to those of Seyfert 2 nuclei. The implications for polarization and variability are also discussed.

Kallman, T.↗

Molecules in interstellar clouds

The physical conditions and chemical compositions of the gas in interstellar clouds are reviewed in light of the importance of interstellar clouds for star formation and the origin of life. The Orion A region is discussed as an example of a giant molecular cloud where massive stars are being formed, and it is pointed out that conditions in the core of the cloud, with a kinetic temperature of about 75 K and a density of 100,000-1,000,000 molecules/cu cm, may support gas phase ion-molecule chemistry. The Taurus Molecular Clouds are then considered as examples of cold, dark, relatively dense interstellar clouds which may be the birthplaces of solar-type stars and which have been found to contain the heaviest interstellar molecules yet discovered. The molecular species identified in each of these regions are tabulated, including such building blocks of biological monomers as H2O, NH3, H2CO, CO, H2S, CH3CN and H2, and more complex species such as HCOOCH3 and CH3CH2CN.

Irvine, W. M.↗