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At least 1,027 records · Page 57
All sourcesNASA NTRSDOE OSTI
DOE OSTI2014

The role of orbital order in the stabilization of the (π, 0) ordered magnetic state in a minimal two-band model for iron pnictides

Spin wave excitations and stability of the (π, 0) ordered magnetic state are investigated in a minimal two-band itinerant-electron model for iron pnictides. Presence of hopping anisotropy generates a strong ferro-orbital order in the d{sub xz} and d{sub yz} Fe orbitals in the (π, 0) state. The orbital order sign is as observed in experiments. The induced ferro-orbital order strongly enhances the spin wave energy scale and stabilizes the magnetic state by optimizing the strength of the emergent antiferromagnetically and ferromagnetically spin couplings through optimal band fillings in the two orbitals. The calculated spin-wave dispersion is in quantitative agreement with neutron scattering measurements. Finite inter-orbital Hund's coupling is shown to further enhance the spin wave energies state by coupling the two magnetic sub-systems. A more realistic two-band model with less hopping anisotropy is also considered, which yields not only the circular hole pockets but also correct ferro-orbital order and emergent F spin coupling.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2021

Magnetization dynamics fingerprints of an excitonic condensate t 2 g 4 magnet

The competition between spin-orbit coupling (SOC) λ and electron-electron interaction U leads to a plethora of novel states of matter, extensively studied in the context of t 2 g 4 and t 2 g 5 materials, such as ruthenates and iridates. Excitonic magnets—the antiferromagnetic state of bounded electron-hole pairs-are prominent examples of phenomena driven by those competing energy scales. Interestingly, recent theoretical studies predicted that excitonic magnets can be found in the ground state of SOC t 2 g 4 Hubbard models. Here we present a detailed computational study of the magnetic excitations in that excitonic magnet, employing one-dimensional chains (via density matrix renormalization group) and small two-dimensional clusters (via Lanczos). Specifically, first we show that the low-energy spectrum is dominated by a dispersive (acoustic) magnonic mode, with extra features arising from the λ = 0 state in the phase diagram. Second, and more importantly, we found a novel magnetic excitation forming a high-energy optical mode with the highest intensity at wave-vector q → 0 . In the excitonic condensation regime at large U , we also have found a novel high-energy π mode composed solely of orbital excitations. Overall, these features do not appear all together in any of the neighboring states in the phase diagram and thus constitute unique fingerprints of the t 2 g 4 excitonic magnet, of importance in the analysis of neutron and resonant inelastic x-ray scattering experiments.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2013

Second harmonic effect on geodesic modes in tokamak plasmas

Results of a kinetic treatment of Geodesic Acoustic Modes (GAMs) that fully takes into account ion parallel dynamics, including the magnetic field component, are presented. The finite-orbit-width (FOW) parameter is considered in the calculation of the second harmonic effect on GAMs. For larger values of the FOW parameter, it is shown that dispersive effects related to the m = 2 harmonics is the cause of the mode frequency splitting and the modes appear due to the interaction with the ion sound mode. Furthermore, the modes may have enhanced damping rates due to second harmonic Landau damping.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2014

Analytic studies of dispersive properties of shear Alfvén and acoustic wave spectra in tokamaks

The properties of the low frequency shear Alfvén and acoustic wave spectra in toroidal geometry are examined analytically and numerically considering wave particle interactions with magnetically trapped and circulating particles, using the theoretical model described in [I. Chavdarovski and F. Zonca, Plasma Phys. Controlled Fusion 51, 115001 (2009)] and following the framework of the generalized fishbone-like dispersion relation. Effects of trapped particles as well as diamagnetic effects on the frequencies and damping rates of the beta-induced Alfvén eigenmodes, kinetic ballooning modes and beta-induced Alfvén-acoustic eigenmodes are discussed and shown to be crucial to give a proper assessment of mode structure and stability conditions. Present results also demonstrate the mutual coupling of these various branches and suggest that frequency as well as mode polarization are crucial for their identification on the basis of experimental evidence.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2026

Structural Origins of High MoO 3 Solubility in Peraluminous Borosilicate Glasses

Molybdenum (Mo) imposes strict loading limits in conventional borosilicate nuclear waste glasses due to the tendency of tetrahedral molybdate [MoO 4 ] 2− species to phase-separate and crystallize as alkali molybdates. Here, we demonstrate an unprecedented 13.96 wt % (7.51 mol %) MoO 3 solubility in peraluminous sodium aluminoborosilicate glasses a ∼15× increase over their peralkaline counterparts. Using Raman spectroscopy, multinuclear and dipolarcorrelation magic angle spinning nuclear magnetic resonance (MAS NMR), electron paramagnetic resonance (EPR), and scanning transmission electron microscopy (STEM)-energy dispersive spectroscopy (EDS), we reveal that Nadeficient, low optical basicity conditions stabilize octahedral MoO 6 units, which polymerize into molybdite-like Mo−O clusters dispersed within the glass matrix. These Mo-rich clusters suppress the formation of depolymerized [MoO 4 ] 2− environments typically responsible for Na 2 MoO 4 precipitation and instead promote the formation of Na 2 Mo 2 O 7 as the saturation phase. Concurrently, Mo solubility drives the conversion of AlO 4 − to higher-coordination AlO 5 species, liberating Na + that is subsequently sequestered in molybdate-rich domains. The combined evolution of Mo coordination, modifier redistribution, and network depolymerization provides a mechanistic basis for the markedly enhanced Mo solubility in peraluminous compositions. These findings establish new structural guidelines for designing aluminoborosilicate waste forms with substantially greater capacity to incorporate Mo-rich nuclear waste streams.

Amorphous materials↗
DOE OSTI2013

SELF-CONSISTENT ION CYCLOTRON ANISOTROPY-BETA RELATION FOR SOLAR WIND PROTONS

We derive a set of self-consistent marginally stable states for a system of ion-cyclotron waves propagating parallel to the large-scale magnetic field through a homogeneous proton-electron plasma. The proton distributions and the wave dispersions are related through the condition that no further ion-cyclotron resonant particle scattering or wave growth/damping may take place. The thermal anisotropy of the protons in these states therefore defines the threshold value for triggering the proton-cyclotron anisotropy instability. A number of recent papers have noted that the anisotropy of solar wind protons at 1 AU does not seem to be limited by the proton-cyclotron anisotropy threshold, even at low plasma beta. However, this puzzle seems to be due solely to the estimation of this anisotropy threshold under the assumption that the protons have a bi-Maxwellian distribution. We note that bi-Maxwellian distributions are never marginally stable to the resonant cyclotron interaction, so these estimates do not represent physically valid thresholds. The threshold anisotropies obtained from our marginally stable states are much larger, as a function of proton parallel beta, than the bi-Maxwellian estimates, and we show that the measured data remains below these more rigorous thresholds. Thus, the results of this paper resolve the apparent contradiction presented by the solar wind anisotropy observations at 1 AU: the bi-Maxwellian anisotropies are not rigorous thresholds, and so do not limit the proton distributions in the solar wind.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2015

STABILITY OF ROTATING MAGNETIZED JETS IN THE SOLAR ATMOSPHERE. I. KELVIN–HELMHOLTZ INSTABILITY

Observations show various jets in the solar atmosphere with significant rotational motions, which may undergo instabilities leading to heat ambient plasma. We study the Kelvin–Helmholtz instability (KHI) of twisted and rotating jets caused by the velocity jumps near the jet surface. We derive a dispersion equation with appropriate boundary conditions for total pressure (including centrifugal force of tube rotation), which governs the dynamics of incompressible jets. Then, we obtain analytical instability criteria of KHI in various cases, which were verified by numerical solutions to the dispersion equation. We find that twisted and rotating jets are unstable to KHI when the kinetic energy of rotation is more than the magnetic energy of the twist. Our analysis shows that the azimuthal magnetic field of 1–5 G can stabilize observed rotations in spicule/macrospicules and X-ray/extreme-ultraviolet (EUV) jets. On the other hand, nontwisted jets are always unstable to KHI. In this case, the instability growth time is several seconds for spicule/macrospicules and a few minutes (or less) for EUV/X-ray jets. We also find that standing kink and torsional Alfvén waves are always unstable near the antinodes, owing to the jump of azimuthal velocity at the surface, while the propagating waves are generally stable. Kelvin–Helmholtz (KH) vortices may lead to enhanced turbulence development and heating of surrounding plasma; therefore, rotating jets may provide energy for chromospheric and coronal heating.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2026

Discovery of van Hove singularities: electronic fingerprints of 3Q magnetic order in a van der Waals quantum magnet

Magnetically intercalated transition metal dichalcogenides are emerging as a rich platform for exploring exotic quantum states in van der Waals magnets. Among them, Co x TaS 2 has attracted intense interest following the recent discovery of a distinctive 3Q magnetic ground state and a pronounced topological Hall effect below a critical doping of x ≈ 1/3, both intimately tied to cobalt concentration. To date, direct signatures of this enigmatic 3Q magnetic order in the electronic structure remain elusive. Here we report a comprehensive doping dependent angle resolved photoemission spectroscopy study that unveils these long-sought fingerprints. Our data reveal an unexpected inverse-Mexican-hat dispersion along the K-M-K' direction, accompanied by two van Hove singularities. These features are consistent with theoretical predictions for a 3Q magnetic order near three-quarters band filling on a cobalt triangular lattice. These results provide evidence of 3Q magnetic order in the electronic structure, establishing TMD van der Waals magnets as tunable materials to explore the interplay between magnetism and topology.

Luo, Hai-Lan [University of California, Berkeley, ↗
DOE OSTI2013

Electron cyclotron maser emission in coronal arches and solar radio type V bursts

Solar radio type V bursts were classified as a special spectral class based on their moderately long duration, wide bandwidth, and sense of polarization opposite of associated type III bursts. However, type V bursts are also closely related to the preceding type III bursts. They have an approximately equal source height and the same dispersion of position with frequency. Electron cyclotron maser (ECM) instability driven by beam electrons has been used to explain type III bursts in recent years. We propose ECM emission as the physical process of type V solar radio bursts. According to the observed properties of type V and III bursts, we propose that energetic electrons in excited type V continuum are trapped in coronal loops, which are adjacent to the open field lines traced by type III electrons. With the proposed magnetic field configuration and the ECM emission mechanism, the observed properties of type V bursts, such as long duration, wide bandwidth, and opposite sense of polarization can be reasonably explained by our model.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2023

Observation of flat and weakly dispersing bands in the van der Waals semiconductor Nb 3 Br 8 with breathing kagome lattice

Niobium halides, Nb 3 ⁢X 8 (X=Cl,Br,I), which are predicted two-dimensional magnets, have recently gotten attention due to their breathing kagome geometry. Here we have studied the electronic structure of Nb 3⁢ Br 8 by using angle-resolved photoemission spectroscopy (ARPES) and first-principles calculations. ARPES results depict the presence of multiple flat and weakly dispersing bands. These bands are well explained by the theoretical calculations, which show they have Nbd character indicating their origination from the Nb atoms forming the breathing kagome plane. This van der Waals material can be easily thinned down via mechanical exfoliation to the ultrathin limit and such ultrathin samples are stable as depicted from the time-dependent Raman spectroscopy measurements at room temperature. Finally, these results demonstrate that Nb 3 ⁢Br 8 is an excellent material not only for studying breathing kagome induced flat band physics and its connection with magnetism but also for heterostructure fabrication and for practical application.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2012

Effect of neutral collision and radiative heat-loss function on self-gravitational instability of viscous thermally conducting partially-ionized plasma

The problem of thermal instability and gravitational instability is investigated for a partially ionized self-gravitating plasma which has connection in astrophysical condensations. We use normal mode analysis method in this problem. The general dispersion relation is derived using linearized perturbation equations of the problem. Effects of collisions with neutrals, radiative heat-loss function, viscosity, thermal conductivity and magnetic field strength, on the instability of the system are discussed. The conditions of instability are derived for a temperature-dependent and density-dependent heat-loss function with thermal conductivity. Numerical calculations have been performed to discuss the effect of various physical parameters on the growth rate of the gravitational instability. The temperature-dependent heat-loss function, thermal conductivity, viscosity, magnetic field and neutral collision have stabilizing effect, while density-dependent heat-loss function has a destabilizing effect on the growth rate of the gravitational instability. With the help of Routh-Hurwitz's criterion, the stability of the system is discussed.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2014

Dispersion relations for electromagnetic wave propagation in chiral plasmas

The dispersion relations for electromagnetic wave propagation in chiral plasmas are derived using a simplified method and investigated in detail. With the help of the dispersion relations for each eignwave, we explore how the chiral plasmas exhibit negative refraction and investigate the frequency region for negative refraction. The results show that chirality can induce negative refraction in plasmas. Moreover, both the degree of chirality and the external magnetic field have a significant effect on the critical frequency and the bandwidth of the frequency for negative refraction in chiral plasmas. The parameter dependence of the effects is calculated and discussed.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2017

Direct Laser Writing of Magneto-Photonic Sub-Microstructures for Prospective Applications in Biomedical Engineering

Here, we report on the fabrication of desired magneto-photonic devices by a low one-photon absorption (LOPA) direct laser writing (DLW) technique on a photocurable nanocomposite consisting of magnetite ( Fe 3 O 4 ) nanoparticles and a commercial SU-8 photoresist. The magnetic nanocomposite was synthesized by mixing Fe 3 O 4 nanoparticles with different kinds of SU-8 photoresists. We demonstrated that the degree of dispersion of Fe 3 O 4 nanoparticles in the nanocomposite depended on the concentration of Fe 3 O 4 nanoparticles, the viscosity of SU-8 resist, and the mixing time. By tuning these parameters, the most homogeneous magnetic nanocomposite was obtained with a concentration of about 2 wt % of Fe 3 O 4 nanoparticles in SU-8 2005 photoresist for the mixing time of 20 days. The LOPA-based DLW technique was employed to fabricate on demand various magneto-photonic submicrometer structures, which are similar to those obtained without Fe 3 O 4 nanoparticles. The magneto-photonic 2D and 3D structures with sizes as small as 150 nm were created. Finally, we demonstrated the strong magnetic field responses of the magneto-photonic nanostructures and their use as micro-actuators when immersed in a liquid solution. View Full-Text

36 MATERIALS SCIENCE↗
DOE OSTI2012

FORMATION OF TURBULENT AND MAGNETIZED MOLECULAR CLOUDS VIA ACCRETION FLOWS OF H I CLOUDS

Using three-dimensional magnetohydrodynamic simulations, including the effects of radiative cooling/heating, chemical reactions, and thermal conduction, we investigate the formation of molecular clouds in the multi-phase interstellar medium. As suggested by recent observations, we consider the formation of molecular clouds due to accretion of H I clouds. Our simulations show that the initial H I medium is piled up behind the shock waves induced by accretion flows. Since the initial medium is highly inhomogeneous as a consequence of thermal instability, a newly formed molecular cloud becomes very turbulent owing to the development of the Richtmyer-Meshkov instability. The kinetic energy of the turbulence dominates the thermal, magnetic, and gravitational energies throughout the entire 10 Myr evolution. However, the kinetic energy measured using CO-fraction-weighted densities is comparable to the other energies, once the CO molecules are sufficiently formed as a result of UV shielding. This suggests that the true kinetic energy of turbulence in molecular clouds as a whole can be much larger than the kinetic energy of turbulence estimated using line widths of molecular emission. We find that clumps in a molecular cloud show the following statistically homogeneous evolution: the typical plasma {beta} of the clumps is roughly constant ({beta}) {approx_equal} 0.4; the size-velocity dispersion relation is {Delta}v {approx_equal} 1.5 km s{sup -1} (l/1 pc){sup 0.5}, irrespective of the density; the clumps evolve toward magnetically supercritical, gravitationally unstable cores; and the clumps seem to evolve into cores that satisfy the condition for fragmentation into binaries. These statistical properties may represent the initial conditions of star formation.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2016

Robust upward dispersion of the neutron spin resonance in the heavy fermion superconductor Ce 1−x Yb x CoIn 5

The neutron spin resonance is a collective magnetic excitation that appears in the unconventional copper oxide, iron pnictide and heavy fermion superconductors. Although the resonance is commonly associated with a spin-exciton due to the d(s ± )-wave symmetry of the superconducting order parameter, it has also been proposed to be a magnon-like excitation appearing in the superconducting state. Here we use inelastic neutron scattering to demonstrate that the resonance in the heavy fermion superconductor Ce 1−x Yb x CoIn 5 with x=0, 0.05 and 0.3 has a ring-like upward dispersion that is robust against Yb-doping. By comparing our experimental data with a random phase approximation calculation using the electronic structure and the momentum dependence of the d x 2 -y 2 -wave superconducting gap determined from scanning tunnelling microscopy (STM) for CeCoIn 5 , we conclude that the robust upward-dispersing resonance mode in Ce 1−x Yb x CoIn 5 is inconsistent with the downward dispersion predicted within the spin-exciton scenario.

43 PARTICLE ACCELERATORS↗
DOE OSTI2013

Dielectric and magnetic properties of some gadolinium silica nanoceramics

Some nanostructure gadolinium silica glass-ceramics were obtained undergoing a sol gel method and a heat-treatment at 1000°C about two hours. The magnetic and dielectric properties of these samples were studied. The magnetic properties were evidenced performing susceptibility measurements in the 80-300K temperature range. A Curie-Weiss behavior has acquired. The values estimated for paramagnetic Curie temperature being small and positive suggest the presence of weak ferromagnetic interactions between Gd{sup 3+} ions. The dielectric properties were evaluated from dielectric permittivity (ε{sub r}) and dielectric loss (tanδ) measurements at the frequency 1 kHz, 10 kHz and 100 kHz, in the 25-225°C temperature range and dielectric dispersion at room temperature for 79.5 kHz - 1GHz frequency area. The dielectric properties suggest that the main polarization mechanism corresponds to interfacial polarization, characteristic for polycrystalline-structured dielectrics. The polycrystalline structure of the samples is due to the polymorphous transformations of the nanostructure silica crystallites in the presence of gadolinium oxide. They were highlighted by SEM micrographs.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Measurement of Compton Scattering at MAMI for the Extraction of the Electric and Magnetic Polarizabilities of the Proton

A precise measurement of the differential cross sections dσ/dΩ and the linearly polarized photon beam asymmetry Σ 3 for Compton scattering on the proton below pion threshold has been performed with a tagged photon beam and almost 4π detector at the Mainz Microtron. The incident photons were produced by the recently upgraded Glasgow-Mainz photon tagging facility and impinged on a cryogenic liquid hydrogen target, with the scattered photons detected in the Crystal Ball/TAPS setup. Using the highest statistics Compton scattering data ever measured on the proton along with two effective field theories (both covariant baryon and heavy-baryon) and one fixed-t dispersion relation model, constraining the fits with the Baldin sum rule, we have obtained the proton electric and magnetic polarizabilities with unprecedented precision: α E1 = 10.99 ± 0.16 ± 0.47 ± 0.17 ± 0.34, β M1 = 3.14 ± 0.21 ± 0.24 ± 0.20 ± 0.35; in units of 10 -4 fm 3 where the errors are statistical, systematic, spin polarizability dependent, and model dependent.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Dispersive nonreciprocity between a qubit and a cavity

The dispersive interaction between a qubit and a cavity is ubiquitous in circuit and cavity quantum electrodynamics. It describes the frequency shift of one quantum mode in response to excitations in the other and, in closed systems, is necessarily bidirectional, i.e., reciprocal. Here, we present an experimental study of a nonreciprocal dispersive-type interaction between a transmon qubit and a superconducting cavity, arising from a common coupling to dissipative intermediary modes with broken time reversal symmetry. We characterize the qubit-cavity dynamics, including asymmetric frequency pulls and photon shot noise dephasing, under varying degrees of nonreciprocity by tuning the magnetic field bias of a ferrite component in situ. We introduce a general master equation model for nonreciprocal interactions in the dispersive regime, providing a compact description of the observed qubit-cavity dynamics agnostic to the intermediary system. Our result provides an example of quantum nonreciprocal phenomena beyond the typical paradigms of non-Hermitian Hamiltonians and cascaded systems.

74 ATOMIC AND MOLECULAR PHYSICS↗