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DOE OSTI2024

FIU Project 2: Environmental Remediation Science & Technology [Slides]

FIU’s research under this project involves conducting basic and applied science to fill knowledge gaps and validate potential remediation technologies for contaminated soil and groundwater and the assessment of the fate and transport of contaminants in the environment. The aim of FIU’s research is to reduce the potential for contaminant mobility or toxicity in the surface and subsurface through the development and application of state-of-the-art scientific and environmental remediation technologies at the Hanford Site, Savannah River Site (SRS), and the Waste Isolation Pilot Plant (WIPP), which is the Nation’s only mined geologic repository for permanent disposal of transuranic waste. FIU collaborates with scientists from Pacific Northwest National Laboratory (PNNL), Savannah River National Laboratory (SRNL), Savannah River Ecology Laboratory (SREL), Los Alamos National Laboratory (LANL) and the DOE Carlsbad Field Office (CBFO) in order to plan and execute research that is synergistic with the work being conducted at the sites, and that supports the resolution of critical science and engineering needs which leads to a better understanding of the long-term behavior of subsurface contaminants. The knowledge gained through this research will be used to transform experimental and modeling innovations into practical applications deployed at the sites to support EM’s primary goal of expediting the closure of major contaminated soil and groundwater sites and waste units. Collaborative relationships between FIU and the national laboratories have provided large benefits over the years to FIU, the national laboratories, the DOE complex, and the DOE EM mission. By working closely with the national laboratories, FIU’s research is not only closely aligned with the cleanup mission priorities at the DOE sites, but complements and supports ongoing work at the national laboratories for screening of new remedial technologies. This coordination and leveraging of research efforts results in time- and cost-savings, and will accelerate progress of the DOE EM environmental restoration mission.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2020

Reflector coatings development (FY2020 End of Year Report)

X-ray detection instrumentation has been developed and manufactured at LANL for various DOE programs. One way to improve light collection efficiency, for a scintillator type detector, is to apply suitable reflectors. The coating capability and fabrication procedure for Al reflective coatings was established in FY19 at MST-7. Al reflective coatings with good stability, good adhesion to LSO, and reflectivity (R) up to 78% were fabricated. Materials with higher diffuse reflectivity (such as Teflon tape R=99%) are desirable. A literature search revealed a number of materials in the form of paint or free standing tape with diffuse R = 98- 99%. However, for the intended application such reflectors have to be applied in the form of a coating with strong adhesion to LSO crystals. The purpose of the FY20 project was to develop thin film coating techniques for PTFE (known as Teflon) reflectors and fabricate reflective coatings on provided LSO crystals.

36 MATERIALS SCIENCE↗

DOE OSTI2020

Safeguards by Design Projects (FY2020 Final Report)

This University Engagement project challenged engineering students at universities, that do not have Bachelor degrees in nuclear engineering but do have research reactors and some nuclear engineering coursework, to incorporate Safeguards by Design concepts into their Senior Capstone Design Project. This University Engagement project was part of the U. S. Department of Energy’s (DOE) National Nuclear Security Administration (NNSA), Office of Defense Nuclear Nonproliferation, Office of International Nuclear Safeguards, Next Generation Safeguards Initiative, Human Capital Development: University Engagement Program. This program exposed university students with Mechanical Engineering majors and Nuclear Engineering minors to the concepts of international nuclear safeguards. FY20, three teams at the University of Rhode Island and one team at the University of Texas - Austin participated in researching, designing, building, and testing projects to support international nuclear safeguards measurements or verification. The projects involved engaging in activities at the university’s research reactors. All the projects engaged students with prototyping a design and/or tool for application at the Universities’ reactor. At the end of the course, most of the students expressed the experience was a positive and they learned more about international nuclear safeguards and applying requirements than they had previously encountered. This school year the projects were further complicated by the COVID-19 pandemic. Both universities cancelled in class room classes, and limited direct student/professor interactions. Furthermore, Los Alamos National Laboratory (LANL) greatly restricted travel, therefore making it impossible to visit the students at the end of the semester for the review of their design projects. The final design and review meeting for the projects happened via the internet. Additionally, while the teams planned to build prototypes this did not happen since there was a social distancing ban on students meeting in person.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

DOE OSTI2020

Generating MCNP Input Files for Unstructured Mesh Geometries

Los Alamos National Laboratory's (LANL) Monte Carlo N-Particle (MCNP) transport code version 6 has the capability for tracking particles on unstructured mesh (UM) geometry models. The MCNP UM feature has been developed for performing calculations of complex geometry models. This capability tracks particles on hybrid geometries where finite element meshes are embedded into constructive solid geometry (CSG) cells. The MCNP UM feature was originally designed to read UM models created by Abaqus/CAE software suite. MCNP versions 6.2.0 and later can process UM models read from Abaqus input les or MCNPUM les converted from Abaqus input les. Sandia National Laboratory's Cubit Toolkit and other finite element analysis software packages may generate UM models and then convert these models into Abaqus input formats.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2020

Evaluation of the 2018 Version of the Integrated Surveillance Program Database Pressure Equation

The Integrated Surveillance Program (ISP) Database Pressure Equation was developed to determine with reasonable certainty the total maximum pressure of hydrogen and other gases in packaged 3013 containers stored at Savannah River Site (SRS) in support of the destructive evaluation (DE) process. The pressure equation in the Department of Energy (DOE) 3013 Standard, “Standard for Stabilization, Packaging and Storage of Plutonium- Bearing Materials” (DOE-STD-3013-2004) used a bounding assumption that all the water is decomposed to form hydrogen. However, the results of Los Alamos National Laboratory (LANL) shelf-life experiments showed that hydrogen is consumed, and that the maximum pressures would not approach the design pressure of the 3013 container. Therefore, the ISP Database Pressure Equation was revised in 2008 to include terms for the generation of helium and hydrogen as a function of time, as well as the consumption of water and destruction of hydrogen based on shelf-life results. The 2008 ISP Database Pressure Equation provided a more reasonable estimate of the total maximum pressure in packaged 3013 containers than the pressure equation in versions of the 3013 Standard issued prior to 2018.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

DOE OSTI2020

Using the CAP88 Plume Model & Dose Assessment Code for the FTWC Project

The Environmental Protection & Compliance Division (EPC) uses the Clean Air Act Assessment Package – 1988 (CAP88) plume model and dose assessment code to evaluate measured emissions or projected emissions of airborne radionuclides from Los Alamos National Laboratory (LANL) facilities. This software package will use facility data (e.g., stack height and exit velocity), emissions parameters (chemical form and quantity), and environmental data (wind speed and direction) to predict downwind concentrations of radioactive material and subsequent dose to a member of the public at that location. The United States Environmental Protection Agency (EPA) has approved CAP88 for use in demonstrating compliance with the Radionuclide NESHAP2, that portion of the Clean Air Act addressing emissions of airborne radioactive material from Department of Energy facilities. EPC Division has two procedures which discuss the use of CAP88.

61 RADIATION PROTECTION AND DOSIMETRY↗

DOE OSTI2020

Shocking Cerium into a New Phase

A material's equation of state (EOS) - which indicates its state under various conditions of pressure, temperature, volume, and energy, and relates them to various phases - is a vital part of understanding the material’s behavior and response in different environments and applications. However, determining the EOS and complete phase diagrams of some materials can pose daunting challenges. One of these materials is cerium, for which some regions of the phase diagram have proven elusive. Investigators from the U.S. Department of Energy’s (DOE’s) Los Alamos National Laboratory (LANL) employed the U.S. DOE’s Advanced Photon Source (APS) to probe the high-pressure solid phase of cerium through shock-wave experiments that provided a detailed look at the cerium's transition from the α-ϵ phases. Their work, which provides the first evidence that an α-ϵ phase transition can be shock-induced in cerium, was published in the Journal of Applied Physics.

36 MATERIALS SCIENCE↗

DOE OSTI2020

Neutron Imaging Using Grating Interferometry: Exploiting phase contrast and dark-field imaging for <1μm feature detection in bulk materials (Summary Report)

Radiography is an important non-destructive characterization tool for many LANL missions. Contrast in conventional radiography results from attenuation of the incoming x-ray or neutron beam by the object. Neutrons have a great benefit in detecting light elements (e.g. hydrogen) in the presence of heavier elements and penetrate deeper than X-rays into many materials, but neutron radiography resolution is typically limited to ~50 μm. Cracks, voids, pores and a variety of other features smaller than this resolution are therefore undetectable in attenuation based neutron imaging. However, novel neutron imaging modalities leveraging off of interferometric methods, so-called neutron grating interferometry (NGI), are able to spatially map sub-micron features and interfacial features while also exploiting the neutron’s sensitivity to light elements and isotope specific contrast to enable material characterization otherwise impossible.

36 MATERIALS SCIENCE↗

DOE OSTI2020

Documenting Development of Processing Parameters for Fabrication of Doped and Undoped Fuel Pellets (Summary Report)

Early FY20 restructuring of the TREAT work package FT-20LA02020608 Enriched Fuel Fabrication for Safety Testing, and associated deliverables necessitated the rescoping of existing LANL deliverables. This rescoped carryover report summarizes work to date on doped and undpoped fuel pellet fabrication development of proceeding parameters. This summary also includes a status update of intended research activities that fall under the activity associated with this work package.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

DOE OSTI2020

Hands-on Introduction to Shock Physics (2020 Report, RR2020-IPD-1)

Los Alamos National Laboratory (LANL) researchers have played key roles in the development of high-pressure science and shock physics since the 1950s. Central to the Laboratory’s experimental capability are multiple impact systems and explosive loading capabilities that span impact velocities in excess of 8 km/s. More recently, our efforts have taken us to 3rd and 4th generation light sources where these loading platforms are coupled to X-ray diagnostics that are now providing new insights into matter-at-extremes. As the availability of these new diagnostics and loading techniques increases, there is an increased need within the high pressure community for researchers with the knowledge base and expertise to use them. Few institutions offer any level of theoretical or experimental coursework designed to train students for work in the field of shock physics or dynamic compression science, and those that do cannot meet the current demand of the national laboratories.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2020

Global Disease Modeling & Forecasting Center [PowerPoint]

The Global Disease Modeling & Forecasting Center works in union with academia, industry, the US Government and global partners to develop, validate, and operationalize epidemiological models to combat infectious diseases. It's mission is to Apply multi-scale modeling and advanced data science to help the world detect, understand, forecast, prevent, and provide decision support in response to emerging and re-emerging disease outbreaks. The presentation explains LANL's role in more detail.

59 BASIC BIOLOGICAL SCIENCES↗

DOE OSTI2020

Monitoring urban hydrological environment monitoring using fiber optical sensing

The goal of this research is to develop an innovative approach to monitoring urban dynamic hydrological environment using optical-fiber-based distributed acoustic sensing (DAS). We propose to employ surface-wave dispersion inversion and coda-wave interferometry inversion based on natural and anthropogenic seismic ambient noises acquired using a DAS array to accurately invert for time-lapse changes of groundwater in urban areas. Through this work, we aim to provide the first cost-effective, city-scale, high-resolution approach to monitoring urban groundwater changes that is otherwise difficult or expensive to achieve using conventional techniques. This work will create LANL’s DAS-based near-surface and groundwater monitoring capability, which can also be leveraged in solving relevant applied energy and national security problems.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DOE OSTI2020

The ASD Scorpius Accelerator at the NNSS. Recruitment Slides for the University of Nevada, Reno [Slides]

The Scorpius Accelerator: Supports the maintenance of the US nuclear stockpile, helps the US not return to nuclear testing, is one of four diagnostics being installed 963 feet below ground, probes subcritical implosions of nuclear material, and supports the validation of LANL and LLNL computer codes. We are searching engineers and scientists with experienced in: Mechanical Engineering, Electrical Engineering, Pulsed Power, Plasma Physics, Controls, Diagnostics, and Fluids and pressure systems.

42 ENGINEERING↗

DOE OSTI2020

Filter Test System for Nuclear Container Filters

The purpose of this procedure is to measure the collection efficiency of the filters that are integrated into the lids of containers for nuclear material at Los Alamos National Laboratory (LANL). As an application of this procedure, a filter test report certificate can be created to document the measurement process. This procedure is intended to describe the TA-55, PF-4 (room 6A) operation of a Filter Test System (FTS) for Hagan and SAVY storage containers.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

DOE OSTI2020

Unattended Single Channel Analyzer (USCA) FY20 Summary Report

In FY20 LANL was funded to design, fabricate, test and document an instrument that can be used by the IAEA for gamma ray measurements in scintillator applications. This instrument, the Unattended Single Channel Analyzer (USCA), will be part of the family of IAEA unattended instruments and completes the suite of most used data acquisition needs provided by the previously designed UNAP instrument. The USCA is designed to meet all the same IAEA requirements designed into the UMSR and UDCM. The new instrument has the same look and feel making it simple for agency staff to move between instruments. This project taps into all the design functions developed during the UMSR and UDCM development. Along with the design and fabrication of a USCA, this project included production of a prototype for IAEA testing and a complete set of documentation.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DOE OSTI2020

Celebrating Native American Heritage Month: Area’s earliest inhabitants become valuable part of Lab workforce

By the time the then-secret laboratory was established in Los Alamos in 1943, the nearby pueblos we know today were well-established communities. To complete its wartime mission to build the world’s first nuclear weapons, the Laboratory needed many workers for all aspects of the project. As such, many Native Americans were hired to work at the Lab in various roles, such as technicians, researchers, machinists, and support staff. By the end of the Manhattan Project in 1945, shortly after the end of World War II, many friendships had been forged between employees from the pueblos and other workers at Los Alamos. This was evidenced by gatherings, such as a post-war celebration at the San Ildefonso Pueblo, as well as individual relationships between Lab staff and pueblo residents. Meanwhile, pueblo residents remained on as valuable members of the post-war Lab staff with additional workers hired as well. In honor of November’s Native American Heritage Month, staff at the National Security Research Center are taking a look back to LANL’s early workforce and the contributions -- both to our mission and our cultural enrichment -- made by Native Americans.

96 KNOWLEDGE MANAGEMENT AND PRESERVATION↗

DOE OSTI2020

National Geographic Interview -- Pit Manufacturing

Los Alamos has been contacted by a freelance reporter working on assignment for National Geographic, Sarah Scoles. Scoles is working on a story about plutonium pit production. She says the story will be an explainer -- detailing the pit production process from start to finish, in context with the planned increase in production. Scoles is seeking to interview a LANL expert or experts to help explain the process, the Lab's history in pit production, and future role.

36 MATERIALS SCIENCE↗

DOE OSTI2020

(U) Jezebel Densities and Uncertainties

The 239 Pu Jezebel benchmark is a keystone for plutonium nuclear data evaluation. At a recent presentation at a nuclear data workshop, Morgan White (LANL P-27) presented a slide about the Jezebel plutonium-alloy part densities and their uncertainties. There are two major errors and one opinion presented as fact.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗