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At least 1,027 records · Page 57

Study of Helium Irradiation Effect on Al6061 Alloy Fabricated by Additive Friction Stir Deposition

Additive friction stir deposition (AFS-D) is considered a productive method of additive manufacturing (AM) due to its ability to produce dense mechanical parts at a faster deposition rate compared to other AM methods. Al6061 alloy finds extensive application in aerospace and nuclear engineering; nevertheless, exposure to radiation or high-energy particles over time tends to deteriorate their mechanical performance. However, the effect of radiation on the components manufactured using the AFS-D method is still unexamined. In this work, samples from the as-fabricated Al6061 alloy, by AFS-D, and the Al6061 feedstock rod were irradiated with He+ ions to 10 dpa at ambient temperature. The microstructural and mechanical changes induced by irradiation of He+ were examined using a scanning electron microscope (SEM), energy-dispersive X-ray spectroscopy (EDS), transmission electron microscopy (TEM), and nanoindentation. This study demonstrates that, at 10 dpa of irradiation damage, the feedstock Al6061 produced a bigger size of He bubbles than the AFS-D Al6061. Nanoindentation analysis revealed that both the feedstock Al6061 and AFS-D Al6061 samples have experienced radiation-induced hardening. These studies provide a valuable understanding of the microstructural and mechanical performance of AFS-D materials in radiation environments, offering essential data for the selection of materials and processing methods for potential application in aerospace and nuclear engineering.

36 MATERIALS SCIENCE↗

Dose and dose rate effects of whole-body gamma-irradiation: II. Hematological variables and cytokines

The goal of part II of this study was to evaluate the effects of gamma-radiation on circulating blood cells, functional characteristics of splenocytes, and cytokine expression after whole-body irradiation at varying total doses and at low- and high-dose-rates (LDR, HDR). Young adult C57BL/6 mice (n = 75) were irradiated with either 1 cGy/min or 80 cGy/min photons from a 60Co source to cumulative doses of 0.5, 1.5, and 3.0 Gy. The animals were euthanized at 4 days post-exposure for in vitro assays. Significant dose- (but not dose-rate-) dependent decreases were observed in erythrocyte and blood leukocyte counts, hemoglobin, hematocrit, lipopolysaccharide (LPS)-induced 3H-thymidine incorporation, and interleukin-2 (IL-2) secretion by activated spleen cells when compared to sham-irradiated controls (p < 0.05). Basal proliferation of leukocytes in the blood and spleen increased significantly with increasing dose (p < 0.05). Significant dose rate effects were observed only in thrombocyte counts. Plasma levels of transforming growth factor-beta 1 (TGF-beta 1) and splenocyte secretion of tumor necrosis factor-alpha (TNF-alpha) were not affected by either the dose or dose rate of radiation. The data demonstrate that the responses of blood and spleen were largely dependent upon the total dose of radiation employed and that an 80-fold difference in the dose rate was not a significant factor in the great majority of measurements.

NASA Discipline Radiation Health↗

Immunohistochemical evidence of rapid extracellular matrix remodeling after iron-particle irradiation of mouse mammary gland

High-LET radiation has unique physical and biological properties compared to sparsely ionizing radiation. Recent studies demonstrate that sparsely ionizing radiation rapidly alters the pattern of extracellular matrix expression in several tissues, but little is known about the effect of heavy-ion radiation. This study investigates densely ionizing radiation-induced changes in extracellular matrix localization in the mammary glands of adult female BALB/c mice after whole-body irradiation with 0.8 Gy 600 MeV iron particles. The basement membrane and interstitial extracellular matrix proteins of the mammary gland stroma were mapped with respect to time postirradiation using immunofluorescence. Collagen III was induced in the adipose stroma within 1 day, continued to increase through day 9 and was resolved by day 14. Immunoreactive tenascin was induced in the epithelium by day 1, was evident at the epithelial-stromal interface by day 5-9 and persisted as a condensed layer beneath the basement membrane through day 14. These findings parallel similar changes induced by gamma irradiation but demonstrate different onset and chronicity. In contrast, the integrity of epithelial basement membrane, which was unaffected by sparsely ionizing radiation, was disrupted by iron-particle irradiation. Laminin immunoreactivity was mildly irregular at 1 h postirradiation and showed discontinuities and thickening from days 1 to 9. Continuity was restored by day 14. Thus high-LET radiation, like sparsely ionizing radiation, induces rapid-remodeling of the stromal extracellular matrix but also appears to alter the integrity of the epithelial basement membrane, which is an important regulator of epithelial cell proliferation and differentiation.

NASA Discipline Radiation Health↗

Space Weathering of Silicates Simulated by Successive Laser Irradiation: in Situ Reflectance Measurements of Fo90, Fo99+, and SiO2

Pulsed-laser irradiation causes the visible-near-infrared spectral slope of olivine (Fo90 and Fo99+) and SiO2 to increase (redden), while the olivine samples darken and the SiO2 samples brighten slightly. XPS analysis shows that irradiation of Fo90 produces metallic Fe. Analytical SEM and TEM measurements confirm that reddening in the Fo90 olivine samples correlates with the production of "nanophase" metallic Fe (npFe0) grains, 20-50 nm in size. The reddening observed in the SiO2 sample is consistent with the formation of SiO or other SiOx species that absorb in the visible. The weak spectral brightening induced by laser irradiation of SiO2 is consistent with a change in surface topography of the sample. The darkening observed in the olivine samples is likely caused by the formation of larger npFe0 particles, such as the 100-400 nm diameter npFe0 identified during our TEM analysis of Fo90 samples. The Fo90 reflectance spectra are qualitatively similar to those in previous experiments suggesting that in all cases formation of npFe0 is causing the spectral alteration. Finally, we find that the accumulation of successive laser pulses cause continued sample darkening in the Vis-NIR, which suggests that repeated surface impacts are an efficient way to darken airless body surfaces.

Airless planetary bodies↗

The Formation of Nucleobases from the Irradiation of Purine in Astophysical Ices and Comparisons with Meteorites.

N-heterocycles have been identified in meteorites and their extraterrestrial origins are suggested by isotopic ratio measurements. Although small N- heterocycles have not been detected in the interstellar medium (ISM), recent experiments in our lab have shown that the irradiation of the aromatic molecules like benzene (C6H6) and naphthalene (C10H8) in mixed molecular ices leads to the formation of O- and N-heterocyclic molecules. Among the class of N-heterocycles are the nucleobases, which are of astrobiological interest because they are the information bearing units of DNA and RNA. Nucleobases have been detected in meteorites [3-5], with isotopic signatures that are also consistent with an extraterrestrial origin. Three of the biologically relevant nucleobases (uracil, cytosine, and guanine) have a pyrimidine core structure while the remaining two (adenine and guanine) possess a purine core. Previous experiments in our lab have demonstrated that all of the bio-logical nucleobases (and numerous other molecules) with a pyrimidine core structure can be produced by irradiating pyrimidine in mixed molecular ices of several compositions [6-8]. In this work, we study the formation of purine-based molecules, including the nucleobases adenine, and guanine, from the ultraviolet (UV) irradiation of purine in ices consisting mixtures of H2O and NH3 at low temperature. The experiments are designed to simulate the astrophysical conditions under which these species may be formed in dense molecular clouds, protoplanetary disks, or on the surfaces of icy bodies in planetary systems.

Astrochemistry↗

Solar Spectral Irradiance Variability in Cycle 24: Model Predictions and OMI Observations

Utilizing the excellent stability of the Ozone Monitoring Instrument (OMI), we characterize both short-term (solar rotation) and long-term (solar cycle) changes of the solar spectral irradiance (SSI) between 265-500 nanometers during the ongoing Cycle 24. We supplement the OMI data with concurrent observations from the GOME-2 (Global Ozone Monitoring Experiment - 2) and SORCE (Solar Radiation and Climate Experiment) instruments and find fair-to-excellent agreement between the observations and predictions of the NRLSSI2 (Naval Research Laboratory Solar Spectral Irradiance - post SORCE) and SATIRE-S (the Naval Research Laboratory's Spectral And Total Irradiance REconstruction for the Satellite era) models.

Sun↗

Solar Temperature Variations Computed from SORCE SIM Irradiances Observed During 2003-2020

NASA’s Solar Radiation and Climate Experiment (SORCE) Spectral Irradiance Monitor (SIM) instrument produced about 17 years of daily average Spectral Solar Irradiance ( SSI ) data for wavelengths 240 nm – 2416 nm. We choose a day of minimal solar activity, 2008-08-24, during the 2008 − 2009 minimum between cycles 23 and 24, and compute the brightness temperature (𝑇 o ) from that day’s solar spectral irradiance (𝑆𝑆𝐼 o ). We consider small variations of T and SSI about these reference values, and derive linear and quadratic analytic approximations by Taylor expansion about the reference day values. To determine approximation accuracy, we compare to exact brightness temperatures T computed from the Planck spectrum, by solving analytically for T , or equivalent root-finding in Wolfram Mathematica. We find that the linear analytic approximation overestimates, while the quadratic underestimates the exact result. This motivates search for statistical “fit” models “in between” the two analytic models, with minimum root-mean-square-error RMSE. We make this search using open-source statistical R software, determine coefficients for linear and quadratic fit models, and compare statistical with analytic RMSE’s. When only linear analytic and fit models are compared, the fit model is superior at ultraviolet, visible, and near infrared wavelengths. This again holds true when comparing only quadratic models. Quadratic is superior to linear for both analytic and statistical models, and statistical fits give smallest RMSE’s. Lastly, we use linear analytic and fit models to find an interpolating function in wavelength, useful in case the SIM results need adjustment to another choices of wavelengths, to compare or extend to any other instrument.

SORCE↗

Solar Irradiance Variability Monitor for the Galileo Solar Space Telescope Mission: Concept and Challenges

Long and reliable total solar irradiance (TSI) time series is one of the essential parameters for understanding solar contributions to climate change. The minor fluctuations of TSI in long timescales could impact the energy balance. Despite the improvement of accurate measurements provided by the instruments, at the time, long-term TSI variability and its effects had not been established. The space-borne radiometer era provided observations in short timescales from minutes to years. Therefore, this study presents an overview of irradiance observations, highlighting the importance of following its variability in different time scales. In this context, the Galileo Solar Space Telescope that has been developed by the Institute for Space Research (INPE), Brazil, includes the Irradiance Monitor Module with a radiometer cavity like the classical design and a next-generation compact radiometer.

total solar irradiance (TSI)↗

Clear Sky Irradiance Year-to-Year Variations and Trends: Preprint

Solar radiation data for seven SURFRAD stations for the period 1996-2018 show an increase in irradiance under clear skies over time, with an interannual variability of the increase. A popular implementation of a clear sky model provided modeled irradiances for comparison with the SURFRAD data under conditions screened for clear skies. The use of the clear sky model, which did not consider year-to-year variances in atmospheric turbidity, was found problematic for resolving small changes in irradiance important for determining PV system degradation over three or five years, but less problematic for a period of ten years.

41 EE - Solar Energy Technologies Office (EE-4S)↗

AGR-5/6/7 Post-Irradiation Examination Plan

This plan describes the PIE activities to be carried out on AGR-5/6/7 fuel and the non-fuel components of the AGR-5/6/7 irradiation test train. PIE of AGR-5/6/7 fuel and test train components will provide data on fuel performance over a range of irradiation conditions (e.g., burnup, neutron fluence, and temperature), test fuel under postulated accident conditions, and support development of fuel performance and fission product transport models. Examination of the non-fuel test train components will give information on TRISO fuel and compact performance and information on releases of radioactive fission products from the fuel compacts. PIE of the fuel compacts is used for many purposes including, but not limited to: updating the irradiation thermal calculations, measuring burnup, determining retention/release of fission products from the compacts and the TRISO particles, determining TRISO layer failure rates, determining fuel performance at elevated accident temperatures, determining fuel performance under oxidizing atmospheres, determining the distribution of fission products within the compact and fuel particles, and observing compact and particle morphology to explain mechanisms of TRISO layer failure and/or fission product release/retention.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Using an Absolute Cavity Pyrgeometer to Validate the Calibration of a Transfer Standard Pyrgeometer Outdoors, Independent from the Reference Value of the Atmospheric Longwave Irradiance

A unique method of pyrgeometer calibration has been developed to improve the measurement uncertainty [1]. The results of this method yielded irradiance values within ±3 W/m2 of those traceable to the World InfraRed Standard Group (WISG). The ACPs and pyrgeometer model PIR were deployed outdoors, and the irradiance measured by the PIR was compared against the irradiance measured by ACP95F3. Based on the results it is possible to achieve an uncertainty of ± 3.51 W/m2. These results suggest that the PIR calibration method might be useful in addressing the international need for a secondary standard pyrgeometer traceable to SI.

absolute cavity pyrgeometer↗

Vendor Irradiation Capsule A quick summary and update

Vendor Irradiation Capsule (VIC) update and summary. Includes what the VIC is, why it is needed, options, how data will be used, and what is concluded from using VIC. Also discusses realistic irradiation timelines, available MTRs and realisitic irradiation positions, disassembly and PIE timelines, processes and conclusions.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

ART Advance Graphite Creep (AGC) Irradiation Experiment

ART Advance Graphite Creep (AGC) Irradiation Experiment topics of discussion include: Schedule, AGC Experiment Update, AGC-4 Status, Anticipated areas data will be used, and Vendor specific irradiation capsule. This includes NRC/Licensing questions on irradiation behavior, behavior model development, and other collaborations.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Safety Considerations for Advanced Material Irradiation at the Advanced Test Reactor

The Advanced Test Reactor (ATR) is a light water reactor with aluminum-clad driver fuel. A primary mission of the ATR is to support the next generation of nuclear reactors. This support necessarily requires irradiation of advanced materials such as sodium, fuel salts, and metal eutectics. Irradiation of advanced materials in the ATR environment presents a challenge when completing accident analyses and demonstrating compliance to the Safety Analysis Report (SAR). Many advanced materials have the possibility to react with the ATR protective barriers such as the cladding or primary coolant system (PCS) boundary during postulated accident scenarios. Further, molten fuel experiments fall outside of the standard regulatory framework for dose consequence analyses. ATR is currently developing new safety analysis methods to support irradiation of advanced materials. The primary considerations for this development are 1) experiment containment design requirements, 2) primary coolant system response to an experiment containment failure, and 3) dose analyses for molten fuels.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

DESIGN AND PROTOYPING OF A FISSILE-BEARING CHLORIDE SALT IRRADIATION EXPERIMENT

Limited data exists on the properties of irradiated fueled chloride-based salts for use in advanced nuclear reactors. The design and prototyping of a salt irradiation experiment is underway. Mechanical design will integrate the experiment into existing assemblies in TRIGA type cores. Neutronics modeling demonstrated how targeted power densities can be reached and provide insight on radionuclide source term generation within the experiment. Thermal-hydraulic and computational fluid dynamics (CFD) analysis indicated that temperature ranges in the salt can satisfy both safety and programmatic requirements. Initial prototyping tests provided confidence in the ability to extract the salt post-irradiation, and in the heater performance. Future planned prototyping will provide an integral assessment of the proposed design prior to insertion in the reactor.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Safety Considerations for Advanced Material Irradiation at the ATR

The Advanced Test Reactor (ATR) is a light water reactor with aluminum-clad driver fuel. A primary mission of the ATR is to support the next generation of nuclear reactors. This support necessarily requires irradiation of advanced materials such as sodium, fuel salts, and metal eutectics. Irradiation of advanced materials in the ATR environment presents a challenge when completing accident analyses and demonstrating compliance to the Safety Analysis Report (SAR). Many advanced materials have the possibility to react with the ATR protective barriers such as the cladding or primary coolant system (PCS) boundary during postulated accident scenarios. Further, molten fuel experiments fall outside of the standard regulatory framework for dose consequence analyses. ATR is currently developing new safety analysis methods to support irradiation of advanced materials. The primary considerations for this development are 1) experiment containment design requirements, 2) primary coolant system response to an experiment containment failure, and 3) dose analyses for molten fuels.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

CCTE Irradiation Plan - PBNC 2024

This paper outlines the irradiation plan for the CCTE-ANEEL-1A experiment in the ATR including irradiation locations, test train geometry, and a summary of the experiment design analysis. ATR irradiation is expected to begin in Spring 2024, with burnup targets of 20, 40, and 60 GWd/MTU.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗