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At least 1,027 records · Page 57

Deployment of ARM Aerial Facility (AAF) Scanning Mobility Particle Sizer Field Campaign Report

Atmospheric aerosols influence global climate by scattering and absorbing sunlight (direct effects) and by changing the microphysical structure, lifetime, and coverage of clouds (indirect effects). While it is widely accepted that aerosol indirect effects act to cool the Earth-atmosphere system by increasing cloud reflectivity and coverage, the magnitudes of the indirect effects are poorly quantified. One key aerosol property for understanding aerosol indirect effects is the ability of aerosol particles to form cloud droplets at atmospheric relevant supersaturations—i.e., cloud condensation nuclei (CCN) activity. For particles consisting of typical atmospheric inorganic compounds, their CCN activity is well understood and can be effectively predicted using Köhler theory based on physicochemical properties of the solute, such as its mass, molar volume, and activity coefficient. However, atmospheric aerosols often consist of hundreds of organic species, which can contribute ~20-90% to the total fine aerosol mass. Depending on their properties, organic species can significantly influence the ability of aerosol particles to act as CCN and form cloud droplets. This project focuses on the CCN activity of secondary organic aerosol compounds formed from key biogenic volatile organic compounds (VOCs) under representative conditions, and the relationship between the hygroscopicity and composition of organic aerosols. The ARM Aerial Facility (AAF) scanning mobility particles sizer (SMPS) was deployed during a ~ 6 week intensive measurement campaign, taking place June 15-July 31 2015 at the Pacific Northwest National Laboratory (PNNL) Environmental Simulation Chamber. The SMPS was operated with a CCN counter. Aerosol particles were first classified by the differential mobility analyzer inside the SMPS; the classified aerosol will then be simultaneously characterized by a condensation particle counter (part of the SMPS) and the CCN counter.

54 ENVIRONMENTAL SCIENCES↗

Advancing Clouds Lifecycle Representation in Numerical Models Using Innovative Analysis Methods that Bridge ARM Observations and Models Over a Breadth of Scales

This the final report for the DE-SC0007096 - Advancing Clouds Lifecycle Representation in Numerical Models Using Innovative Analysis Methods that Bridge ARM Observations and Models Over a Breadth of Scales - PI: Pavlos Kollias. The final report outline the main findings of the research conducted using the aforementioned award in the area of cloud research from the cloud scale (10-100 m) to the mesoscale (20-50 km).

58 GEOSCIENCES↗

Collaborative Research: Reducing tropical precipitation biases in CESM — Tests of unified parameterizations with ARM observations

In state-of-the-art climate models, each cloud type is treated using its own separate cloud parameterization and its own separate microphysics parameterization. This use of separate schemes for separate cloud regimes is undesirable because it is theoretically unfounded, it hampers interpretation of results, and it leads to the temptation to overtune parameters. In this grant, we are creating a climate model that contains a unified cloud parameterization and a unified microphysics parameterization. This model will be used to address the problems of excessive frequency of drizzle in climate models and excessively early onset of deep convection in the Tropics over land. The resulting model will be compared with ARM observations.

54 ENVIRONMENTAL SCIENCES↗

Marine ARM GPCI Investigation of Clouds Psychrometer Field Campaign Report

One of the most critical measurements in the suite of meteorological measurements used for the calculation of evaporation and latent heat flux is the relative humidity (RH). In order to achieve an overall net flux uncertainty < 10 W/m 2 (Bradley and Fairall, 2006), the RH must be accurate to < 2 %RH. Anyone experienced in shipboard meteorological measurements will recognize that this is a tough specification. During the U.S. Department of Energy (DOE) Marine Atmospheric Radiation Measurement (ARM) Climate Research Facility Global Energy and Water Experiment (GEWEX) Cloud System Study (GCSS) Pacific Cross-Section Intercomparison (GPCI) Investigation of Clouds (MAGIC) experiment, the meteorological package used three different RH sensors. We found approximately 3-4 % differences between units. To arbitrate the differences and to track calibration drift over the months of exposure, we used a precision psychrometer. The Assmann Psychrometer, Model 430101 is a classic, mercury-in-glass instrument that gives a precise measure of the wet and dry bulb temperatures from which atmospheric humidity and RH are computed. On a regular basis, typically after each balloon launch, a technician took the psychrometer to an exposed location on the bridge roof. That was just below the instruments on the mast and high enough into the mixed layer that the difference is negligible.

54 ENVIRONMENTAL SCIENCES↗

Model simulations of aerosol effects on clouds and precipitation in comparison with ARM data

Observation-based studies have shown that the aerosol cloud lifetime effect or the increase of cloud liquid water path (LWP) with increased aerosol loading may have been overestimated in climate models. Here, we simulate shallow warm clouds on 05/27/2011 at the Southern Great Plains (SGP) measurement site established by Department of Energy's Atmospheric Radiation Measurement (ARM) Program using a single column version of a global climate model (Community Atmosphere Model or CAM) and a cloud resolving model (CRM). The LWP simulated by CAM increases substantially with aerosol loading while that in the CRM does not. The increase of LWP in CAM is caused by a large decrease of the autoconversion rate when cloud droplet number increases. In the CRM, the autoconversion rate is also reduced, but this is offset or even outweighed by the increased evaporation of cloud droplets near cloud top, resulting in an overall decrease in LWP. Our results suggest that climate models need to include the dependence of cloud top growth and the evaporation/condensation process on cloud droplet number concentrations.

54 ENVIRONMENTAL SCIENCES↗

Contextual Multi-armed Bandits under Feature Uncertainty

We study contextual multi-armed bandit problems under linear realizability on rewards and uncertainty (or noise) on features. For the case of identical noise on features across actions, we propose an algorithm, coined NLinRel, having O(T⁷/₈(log(dT)+K√d)) regret bound for T rounds, K actions, and d-dimensional feature vectors. Next, for the case of non-identical noise, we observe that popular linear hypotheses including NLinRel are impossible to achieve such sub-linear regret. Instead, under assumption of Gaussian feature vectors, we prove that a greedy algorithm has O(T²/₃√log d)regret bound with respect to the optimal linear hypothesis. Utilizing our theoretical understanding on the Gaussian case, we also design a practical variant of NLinRel, coined Universal-NLinRel, for arbitrary feature distributions. It first runs NLinRel for finding the ‘true’ coefficient vector using feature uncertainties and then adjust it to minimize its regret using the statistical feature information. We justify the performance of Universal-NLinRel on both synthetic and real-world datasets.

97 MATHEMATICS AND COMPUTING↗