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At least 1,009 records · Page 56
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Process-based and observation-constrained SOA simulations in China: the role of semivolatile and intermediate-volatility organic compounds and OH levels

Organic aerosol (OA) is a major component of tropospheric submicron aerosol that contributes to air pollution and causes adverse effects on human health. Chemical transport models have difficulties in reproducing the variability in OA concentrations in polluted areas, hindering understanding of the OA budget and sources. Herein, we apply both process-based and observation-constrained schemes to simulate OA in GEOS-Chem. Comprehensive data sets of surface OA, OA components, secondary organic aerosol (SOA) precursors, and oxidants were used for model–observation comparisons. The base models generally underestimate the SOA concentrations in China. In the revised schemes, updates were made on the emissions, volatility distributions, and SOA yields of semivolatile and intermediate-volatility organic compounds (SVOCs and IVOCs) and additional nitrous acid sources. With all the model improvements, both the process-based and observation-constrained SOA schemes can reproduce the observed mass concentrations of SOA and show spatial and seasonal consistency with each other. Our best model simulations suggest that anthropogenic SVOCs and IVOCs are the dominant source of SOA, with a contribution of over 50% in most of China, which should be considered for pollution mitigation in the future. The residential sector may be the predominant source of SVOCs and IVOCs in winter, despite large uncertainty remaining in the emissions of IVOCs from the residential sector in northern China. The industry sector is also an important source of IVOCs, especially in summer. More SVOC and IVOC measurements are needed to constrain their emissions. Besides, the results highlight the sensitivity of SOA to hydroxyl radical (OH) levels in winter in polluted environments. The addition of nitrous acid sources can lead to over 30% greater SOA mass concentrations in winter in northern China. It is important to have good OH simulations in air quality models.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

Dust pollution in China affected by different spatial and temporal types of El Niño

Dust is an important aerosol affecting air quality in China in the winter and spring seasons. Dust in China is potentially influenced by the interannual climate variability associated with El Niño. Here, the impacts of El Niño with different temporal and spatial types on dust pollution in boreal winter and spring in China and the potential mechanisms are investigated using a state-of-the-art Earth system model (E3SMv1). We find that the eastern Pacific (EP) and central Pacific (CP) El Niño both increase wintertime dust concentrations by 5–50 µg m –3 over central-eastern China. Due to a stronger wind and lower relative humidity, which favor dust emissions near sources, and a strengthened northwesterly and reduced precipitation, which are conducive to dust transport, dust concentrations during the CP El Niño are 5–20 µg m –3 higher in northern China than during the EP El Niño, although the changes are mostly insignificant. El Niño with a short duration (SD) increases boreal winter dust concentrations by 20–100 µg m –3 over northern China relative to the climatological mean, while there is a decrease of 5–50 µg m –3 during the long-duration (LD) El Niño, which is also related to the El Niño-induced changes in atmospheric circulation, precipitation, and relative humidity. In the following spring season, all types of El Niño events enhance dust over northern China, but only the increase during the LD El Niño is statistically significant, suggesting that the weaker intensity but longer duration of the LD El Niño events can significantly affect spring dust in China. Our results contribute to the current knowledge of the influence of El Niño on dust pollution, which has profound implications for air pollution control and dust storm prediction.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2020

Using respiration quotients to track changing sources of soil respiration seasonally and with experimental warming

Developing a more mechanistic understanding of soil respiration is hampered by the difficulty in determining the contribution of different organic substrates to respiration and in disentangling autotrophic-versus-heterotrophic and aerobic-versus-anaerobic processes. Here, we use a relatively novel tool for better understanding soil respiration: the apparent respiration quotient (ARQ). The ARQ is the amount of CO 2 produced in the soil divided by the amount of O 2 consumed, and it changes according to which organic substrates are being consumed and whether oxygen is being used as an electron acceptor. We investigated how the ARQ of soil gas varied seasonally, by soil depth, and by in situ experimental warming ( +4 ° C) in a coniferous-forest whole-soil-profile warming experiment over 2 years. We then compared the patterns in ARQ to those of soil δ 13 CO 2 . Our measurements showed strong seasonal variations in ARQ, from ≈0.9 during the late spring and summer to ≈0.7 during the winter. This pattern likely reflected a shift from respiration being fueled by oxidized substrates like sugars and organic acids derived from root and root respiration during the growing season to more reduced substrates such as lipids and proteins derived from microbial necromass during the winter. This interpretation was supported by δ 13 CO 2 values, which were lower, like lipids, in the winter and higher, like sugars, in the summer. Furthermore, experimental warming significantly changed how both ARQ and δ 13 CO 2 responded to soil temperature. Wintertime ARQ and δ 13 CO 2 values were higher in heated than in control plots, probably due to the warming-driven increase in microbial activity that may have utilized oxidized carbon substrates, while growing-season values were lower in heated plots. Experimental warming and phenology change the sources of soil respiration throughout the soil profile. The sensitivity of ARQ to these changes demonstrates its potential as a tool for disentangling the biological sources contributing to soil respiration.

59 BASIC BIOLOGICAL SCIENCES↗
DOE OSTI2022

Climate projections over the Great Lakes Region: using two-way coupling of a regional climate model with a 3-D lake model

Abstract. Warming trends in the Laurentian Great Lakes and surrounding areas have been observed in recent decades, and concerns continue to rise about the pace and pattern of future climate change over the world's largest freshwater system. To date, most regional climate models used for Great Lakes projections either neglected the lake-atmosphere interactions or are only coupled with a 1-D column lake model to represent the lake hydrodynamics. This study presents a Great Lakes climate change projection that has employed the two-way coupling of a regional climate model with a 3-D lake model (GLARM) to resolve 3-D hydrodynamics essential for large lakes. Using the three carefully selected Coupled Model Intercomparison Project Phase 5 (CMIP5) general circulation models (GCMs), we show that the GLARM ensemble average substantially reduces surface air temperature and precipitation biases of the driving GCM ensemble average in present-day climate simulations. The improvements are not only displayed from an atmospheric perspective but are also evident in the accurate simulations of lake temperature and ice coverage. We further present the GLARM projected climate change for the mid-21st century (2030–2049) and the late 21st century (2080–2099) in the Representative Concentration Pathway (RCP) 4.5 and RCP 8.5 scenarios. Under RCP 8.5, the Great Lakes basin is projected to warm by 1.3–2.1 ∘C by the mid-21st century and 4.1–5.0 ∘C by the end of the century relative to the early century (2000–2019). Moderate mitigation (RCP 4.5) reduces the mid-century warming to 0.8–1.8 ∘C and late-century warming to 1.8–2.7 ∘C. Annual precipitation in GLARM is projected to increase for the entire basin, varying from 0 % to 13 % during the mid-century and from 9 % to 32 % during the late century in different scenarios and simulations. The most significant increases are projected in spring and fall when current precipitation is highest and a minimal increase in winter when it is lowest. Lake surface temperatures (LSTs) are also projected to increase across the five lakes in all of the simulations, but with strong seasonal and spatial variability. The most significant LST increases occur in Lakes Superior and Ontario. The strongest warming is projected in spring that persists into the summer, resulting from earlier and more intense stratification in the future. In addition, diminishing winter stratification in the future suggests the transition from dimictic lakes to monomictic lakes by the end of the century. In contrast, a relatively smaller increase in LSTs during fall and winter is projected with heat transfer to the deep water due to the strong mixing and energy required for ice melting. Correspondingly, the highest monthly mean ice cover is projected to reduce to 3 %–15 % and 10 %–40 % across the lakes by the end of the century in RCP 8.5 and RCP 4.5, respectively. In the coastal regions, ice duration is projected to decrease by up to 60 d.

Xue, Pengfei (ORCID:000000025702421X)↗
DOE OSTI2021

WRF-simulated low-level jets over Iowa: characterization and sensitivity studies

Abstract. Output from 6 months of high-resolution simulations with the Weather Research and Forecasting (WRF) model are analyzed to characterize local low-level jets (LLJs) over Iowa for winter and spring in the contemporary climate. Low-level jets affect rotor plane aerodynamic loading, turbine structural loading and turbine performance, and thus accurate characterization and identification are pertinent. Analyses using a detection algorithm wherein the wind speed above and below the jet maximum must be below 80 % of the jet wind speed within a vertical window of approximately 20–530 m a.g.l. (above ground level) indicate the presence of an LLJ in at least one of the 14 700 4 km×4 km grid cells over Iowa on 98 % of nights. Nocturnal LLJs are most frequently associated with stable stratification and low turbulent kinetic energy (TKE) and hence are more frequent during the winter months. The spatiotemporal mean LLJ maximum (jet core) wind speed is 9.55 m s−1, and the mean height is 182 m. Locations of high LLJ frequency and duration across the state are seasonally varying, with a mean duration of 3.5 h. The highest frequency occurs in the topographically complex northwest of the state in winter and in the flatter northeast of the state in spring. Sensitivity of LLJ characteristics to the (i) LLJ definition and (ii) vertical resolution at which the WRF output is sampled is examined. LLJ definitions commonly used in the literature are considered in the first sensitivity analysis. These sensitivity analyses indicate that LLJ characteristics are highly variable with definition. Use of different definitions identifies both different frequencies of LLJs and different LLJ events. Further, when the model output is down-sampled to lower vertical resolution, the mean jet core wind speed height decreases, but spatial distributions of regions of high frequency and duration are conserved. Implementation of a polynomial interpolation to extrapolate down-sampled output to full-resolution results in reduced sensitivity of LLJ characteristics to down-sampling.

17 WIND ENERGY↗
NASA NTRS1971

The spectrum of electron content fluctuations in the ionosphere.

Continuous records of the electron content of the ionosphere, from 1965 to 1970, are used to obtain power spectra covering periods from 30 sec to 2 yr at latitudes of 34 deg S and 42 deg S. At periods up to 5 min amplitudes were less than 0.2% of the total electron content. Variations produced by gravity waves were very common in the range from 20 to 80 min, with no preferred periods. The amplitude increased during the day, particularly in winter when periodic components predominated. The cutoff at about 17 min was sharply defined, giving a mean scale height for the neutral atmosphere of about 43 km in summer, 47 km on winter days, and 42 km on winter nights.

Titheridge, J. E.↗
NASA NTRS1972

A global empirical model of thermospheric composition based on OGO-6 mass spectrometer measurements.

A global empirical model for magnetically quiet conditions has been developed to describe longitudinally averaged OGO-6 N2, O, and He densities (in the altitude range 400 to 600 km) by means of an expansion into spherical harmonics. The annual asymmetric component in N2 density corresponds to an increase of about 400 K between winter and summer poles, which is about a factor of three greater than in the Jacchia model. However, the corresponding oxygen component at satellite altitudes reflects an increase between winter and summer comparable to that in the Jacchia model; this implies that at 120 km atomic oxygen increases by more than a factor of two between summer and winter poles. The amplitude of the symmetric semiannual component in N2 is larger at the poles than the equator. At the poles, the N2 variation corresponds to a temperature decrease of about 70 K from mid-April to mid-July. At low latitudes, the daily temperature maximum occurs close to 16 hours local time, nearly in agreement with radar backscatter observations.

Hedin, A. E.↗
NASA NTRS1972

Ionospheric scale height from the refraction of satellite signals.

Accurate observations of the elevation angle of arrival of 20 MHz signals from the polar orbiting satellite Beacon-B for a 20 month period have provided transmission ionograms which may be reduced to give Hp the scale height at the peak of the ionosphere. Noon seasonal averages of Hp are 1.35 (in winter) to 1.55 (in summer) times greater than the scale height obtained from bottom-side ionograms. A comparison of scale height at the peak with routine measurements of total content and peak electron density indicates that the O+/H+ transition level is above 1000 km during the day but comes down to about 630 km on winter nights. A predawn peak in the overall scale height is caused by a lowering of the layer to a region of increased recombination and is magnified in winter by low O+/H+ transition levels.

Heron, M. L.↗
NASA NTRS1973

Horizontal variations in thermospheric composition.

Constant boundary conditions at 120 km have been so widely and successfully used in atmospheric modeling and in fitting atmospheric density data obtained from satellite drag to models that attention has been diverted from the variations that occur at 120 km, especially in composition. Atomic oxygen concentrations vary by factors as large as 4, with highest concentrations occurring in the winter hemisphere but at midlatitudes rather than over the polar region. A substantial additional degree of variability occurs that is especially associated with geomagnetic activity. The helium concentration varies by about an order of magnitude between poles, with the maximum concentration occurring at high winter latitudes and a secondary minimum occurring over the winter pole.

Johnson, F. S.↗
NASA NTRS1974

Dynamics of suspended sediment plumes in Lake Ontario

The absence of turbidity plumes during the winter was well documented in an ususually successful sequence of images obtained February 10 - 12, 1974. Useful imagery of the south shore of Lake Ontario was obtained on 3 successive days at a time when sky cover over the area normally approaches complete coverage. Imagery of the Oswego, Genesee, and Niagara rivers failed to detect any plumes, however faint. Despite strong northwest winds on February 11 there was no indication of shoreline erosion generated by wave action. Frozen ground, snow cover, shoreline icing and minimal construction and farm activity without doubt reduces the probability of sediment movement in winter. Thunderstorm activity over the study area is very rare during the cold season so that the erosive energy of rainfall is greatly reduced. Moreover, a fairly high percentage of the winter precipitation is in the form of snow or sleet further reducing the impact of rainfall energy on sediment transport.

Pluhowski, E. J.↗
NASA NTRS1974

Operation of agricultural test fields for study of stressed crops by remote sensing

A test site for the study of winter wheat development and collection of ERTS data was established in September of 1973. The test site is a 10 mile square area located 12.5 miles west of Amarillo, Texas on Interstate Hwy. 40, in Randall and Potter counties. The center of the area is the Southwestern Great Plains Research Center at Bushland, Texas. Within the test area all wheat fields were identified by ground truth and designated irrigated or dryland. The fields in the test area other than wheat were identified as to pasture or the crop that was grown. A ground truth area of hard red winter wheat was established west of Hale Center, Texas. Maps showing the location of winter wheat fields in excess of 40 acres in size within a 10 mile radius were supplied NASA. Satellite data was collected for this test site (ERTS-1).

Toler, R. W.↗
NASA NTRS1976

Seasonal variation of neutral thermospheric constituents in the Northern Hemisphere

The Atmosphere Explorer-C satellite carries a large number of experiments including an open source neutral mass spectrometer. Among the measurements obtained with this instrument were ones of particle densities of N2, O, and He at northern latitudes in early February and late June 1974. The orbital geometry of the satellite was such that comparisons could be made between the winter and summer values at the same altitudes and latitudes and at similar local solar times. The helium density shows in midmorning a winter to summer enhancement of a factor of 29 at 400 km. The enhancement at other altitudes, both higher and lower, is less. At 250 km the winter/summer oxygen ratio is 1.7, whereas the winter/summer nitrogen ratio is 0.6. Both ratios decrease with increasing altitudes. The analysis identifies an oxygen enhancement at low altitudes in winter and at high altitudes in summer.

Mauersberger, K.↗
NASA NTRS1975

Seasonal variations of NO and O3 at altitudes of 18.3 and 21.3 km

Nitric oxide and ozone concentrations have been measured in situ from a high-altitude research aircraft. Data which show the variations of NO and O3 with the time of year are presented for altitudes of 18.3 and 21.3 km. The extreme values of the observed NO concentrations at 21.3 km are 1.2 billion per cu cm in summer and 0.2 billion per cu cm in winter. At 18.3 km the extreme values are 1.6 billion per cu cm in summer and 0.1 billion per cu cm in winter. The smoothed NO seasonal data show a variation of about a factor of 2.5 at 21.3 km and a factor of 4 at 18.3 km. The ozone data show the generally expected magnitude and seasonal variation. We have used a photochemical model employing the measured ozone concentrations, the mean solar zenith angle, and seasonal HNO3 data reported by others to predict the seasonal NO variation at 20 km. The result is a summer-to-winter NO ratio of 2.5 which is in fair agreement with the observed ratios.

Loewenstein, M.↗
NASA NTRS1975

CARETS: A prototype regional environmental information system. Volume 7: Land use information and air quality planning

The pilot national land use information system developed by the U.S. Geological Survey in the Central Atlantic Regional Ecological Test Site project has provided an improved technique for estimating emissions, diffusion, and impact patterns of sulfur dioxide (S0 2 ) and particulate matter. Implementation of plans to control air quality requires land use information, which, until this time, has been inadequate. The pilot system, however, provided data for updating information on the sources of point and area emissions of S0 2 and particulate matter affecting the Norfolk--Portsmouth area of Virginia for the 1971-72 winter (Dec.-Jan.-Feb.) and the annual 1972 period, and for a future annual period--1985. This emission information is used as input to the Air Quality Display Model of the Environmental Protection Agency to obtain diffusion and impact patterns for the three periods previously mentioned. The results are: (1) During the 1971-72 winter, estimated SO 2 amounts over an area with a SW-NE-axis in the central section of Norfolk exceeded both primary and secondary levels; (2) future annual levels of SO 2 , estimated by anticipated residential development and point-source changes, are not expected to cause serious deterioration of the region's present air quality; and (3) for the 1971-72 winter and annual 1972 period the diffusion results showed that both primary and secondary standards for particulate matter are regularly exceeded in central Norfolk and Portsmouth. In additions on the bas is of current control programs, the 1985 levels of particulate matter are expected to exceed the presently established secondary air quality standards throughout central Norfolk and Portsmouth and in certain areas of Virginia Beach. The land use information can be used to estimate emissions for inputs to diffusion models and to interpret the implications of diffusion patterns for: (1) Implementing various control strategies (2) selecting sites of air sampling stations, and (3) predicting the effects that proposed changes in land use might have on emission patterns and air quality.

Remote sensing↗
NASA NTRS1977

Retransmission of hydrometric data in Canada

The author has identified the following significant results. During the winter of 1974-75, the number of transmissions dropped with lower temperatures and ceased at -20 C. During the winter of 1975-76, the same pattern occurred except that the platform ceased at slightly lower temperatures, probably due to the addition of 3, 1.5 V primary cells to the power supply. The next winter (1976-77), the same pattern occurred.

Halliday, R. A.↗
NASA NTRS1978

Quantitative calculations of helium ion escape fluxes from the polar ionospheres

An attempt is made to reduce the discrepancy between the earlier theoretical model and the recent experimental observations of H(+) outward fluxes for winter and summer hemispheres by improving the theoretical model. The helium photoionization cross sections used are accurate to 10%, the latest solar EUV fluxes measured by the Atmosphere Explorer satellites are incorporated, and the most recent MSIS model of the neutral atmosphere is contained in the model. A range of conditions covering solar cycle, seasonal, and geomagnetic conditions are studied. The results show a maximum H(+) escape flux of 1.4 times 10 to the 7th per sq cm per sec for solar maximum, winter, low magnetic activity conditions, which is within the scatter of the measured fluxes. The computed summer H(+) escape flux is a factor of 20 lower than the winter value. Possible reasons for the slight discrepancy between theory and experiment in summer are discussed.

Raitt, W. J.↗
NASA NTRS1979

Interplanetary magnetic field polarity and the size of low-pressure troughs near 180 deg W longitude

The relationship between interplanetary magnetic field polarity and the area of low pressure (300 mbar) troughs near 180 deg W longitude is examined. For most of the winters from 1951 to 1973, the trough size, as indicated by the vorticity area index, is found to be significantly greater when the interplanetary magnetic field is directed away from the sun than when the field is directed towards the sun. This relationship is shown to hold for various combinations of winters and for most months within a winter, and be most pronounced at the time when polarity was determined. It is suggested that the phenomenon is caused by merging of interplanetary magnetic field lines, when polarity is directed away from the sun, with geomagnetic field lines in the Northern Hemisphere (where these measurements were made), allowing energetic particle fluxes to have access to the north polar region

Wilcox, J. M.↗
NASA NTRS1979

The seasonal variation of ozone density in the Martian atmosphere

A one-dimensional, time-dependent model has been developed to investigate seasonal variations in ozone density in the Martian atmosphere. The model utilizes data for atmospheric temperature, pressure, and water vapor abundance observed by Viking. The results indicate that a high ozone density is not produced near the winter solstice but is in rather late winter, when the amount of water vapor is still small and the solar radiation can penetrate more deeply. A similar condition met in early winter does not necessarily produce a high ozone density because of the predicted higher HO2 density. Seasonal variations in ozone abundance are discussed in terms of the abundances of H2O and H2 and the seasonal variations in their reaction products H2O2 and HOx. The roles of transport, the effects of ozone loss to the surface, and the differences between northern and southern hemisphere ozone distributions are also discussed.

Shimazaki, T.↗