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DOE OSTI2024

Opportunities and new developments for the study of surfaces and interfaces in soft condensed matter at the SIRIUS beamline of Synchrotron SOLEIL

The SIRIUS beamline of Synchrotron SOLEIL is dedicated to X-ray scattering and spectroscopy of surfaces and interfaces, covering the tender to mid-hard X-ray range (1.1–13 keV). The beamline has hosted a wide range of experiments in the field of soft interfaces and beyond, providing various grazing-incidence techniques such as diffraction and wide-angle scattering (GIXD/GIWAXS), small-angle scattering (GISAXS) and X-ray fluorescence in total reflection (TXRF). SIRIUS also offers specific sample environments tailored for in situ complementary experiments on solid and liquid surfaces. Recently, the beamline has added compound refractive lenses associated with a transfocator, allowing for the X-ray beam to be focused down to 10 µm × 10 µm while maintaining a reasonable flux on the sample. This new feature opens up new possibilities for faster GIXD measurements at the liquid–air interface and for measurements on samples with narrow geometries.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

NASA NTRS1972

Resonance scattering of the first positive system of N2 in the dayglow.

Rocket measurements of the differential photoelectron flux and the volume emission rate of the N2(0, 0) second positive band are used to calculate the daytime concentration of metastable A(super 3)Sigma(sub u)+ molecules, and consequently the resonance scattering contribution to the N2 first positive emission in the dayglow. The dominant source of N2 first positive emission is found to be photoelectron impact, with resonance scattering contributing only 10-20 per cent the total emission.

Feldman, P. D.↗

NASA NTRS1978

Work on power-plant (air) plumes involving remote sensing of SO2

Acquisition of air quality and concurrent meteorological data was used for dispersion model development and plant siting needs of the Maryland power plants. One of the major instruments in these studies was the Barringer correlation spectrometer, a remote sensor, using atmospherically scattered sunlight that was used to measure the total amount of SO2 in a cross section of the plume. Correlation spectrometer and its role in this measurement program are described.

White, C. L., Jr.↗

NASA NTRS1978

Spectroscopic mapping of solar wind velocities

During the total solar eclipse of 1970, measurements of resonantly scattered Lyman-alpha radiation from the solar corona revealed a means to determine temperatures and densities in the solar corona beyond 1.5 R solar radii. A natural extension of this work is to use the Solar Probe to measure the spectral line profile of Lyman-alpha radiation backscattered toward the Sun from coronal regions between 4 R solar radii and 10 R solar radii. The backscattered profile would provide unique and quantitative determinations of the outlaw velocities of coronal material into the solar wind. Such information is of critical importance for understanding solar-wind formation and solar-terrestrial effects on the earth's climate. There is no known way to obtain this information without a Solar Probe-type mission.

Kohl, J. L.↗

NASA NTRS1981

Radio emission of sea surface at centimeter wavelengths and is fluctuations

The eigen thermal radio emission of the sea was examined as well as the agitated surface of the sea when the reflection (scattering) is similar in nature to diffused scattering. The contribution of this emission to the total emission of the sea is practically constant in time, and the time fluctuations of the radio emissions of the sea are basically determined only by a change in the eigen emission of the sea, connected with the agitation.

Tseytlin, N. M.↗

NASA NTRS1985

X-ray resonance scattering in a spherically symmetric coronal model

In the solar corona the opacities of some of the prominent X-ray emission lines are on the order of tau of about I over typical coronal path lengths. A particular solution of the radiative transfer problem involving an extended, spherically symmetric coronal shell radiating isotropic, homogeneous emission in which single-scattering also takes place is presented and discussed. Within the context of this simplified model, it is found that scattered radiation is an important contribution to the total emergent resonance line flux and that for the He-like family of resonance (r), intercombination (i), and forbidden (f) lines, the ratio G = (f + i)/r would decrease as a function of optical depth for disk-center emission in an extended spherically symmetric corona.

Haisch, B. M.↗

NASA NTRS1986

Measuring interstellar dust grains from the haloes of binary X-ray sources

A method for determining the location, size distribution, and composition of interstellar dust grains from the haloes of binary X-ray sources is described. The method is based on the time dependence of the halo X-ray emission during an eclipse of the point source. The distance of the dust cloud is inferred directly from observations of the growth of the dark circle around the eclipsed point source. Grain size distribution in the interstellar dust clouds is derived from the halo brightness profile at a given photon energy. The composition of the grains is obtained by observing the spectral features in the total optical depth due to X-ray scattering near the photoionization thresholds of the elements in the grains. The haloes become dim just below the ionization threshold, and sharply increase in function brightness as the photon energy increases beyond the absorption edge of the relevant atom. The method makes it possible to observe and analyze the halo emission during eclipse even without imaging the source. It is suggested that haloes probably account for the soft X-rays observed during eclipses and dips observed in sources including 4U1915-05 and X1755-338.

Xu, Y.↗

NASA NTRS1987

CO observations of nearby galaxies and the efficiency of star formation

The CO distributions and total molecular content of 160 galaxies were observed using the 14 meter millimeter telescope of the FCRAO. For the luminous, relatively face-on Sc galaxies, the azimuthally averaged CO distributions are centrally peaked, while for the Sb and Sa galaxies the Co distributions often exhibit central CO holes up to 5 kpc across. None of the Sc galaxies have CO distributions which resemble the Milky Way. A general correlation was found between total CO and IR luminosities in galaxies. The scatter in this relation is highly correlated with dust temperature. No strong correlation of IR luminosities was found with HI masses, and it was thereby concluded that the infrared emission is more directly tied to the molecular content of galaxies. It is suggested that galaxies which have high Star Formation Effiencies (SFEs) produce more stars per unit molecular mass, thereby increasing the average temperature of the dust in the star forming regions. Irregular galaxies and galaxies previously identified as mergers have the highest observed star formation efficiencies. For the mergers, evidence was found that the IR/CO luminosity ratio increases with the merger age estimated by Joseph and Wright (1985).

Young, Judith S.↗

NASA NTRS2004

Investigation of Acoustical Shielding by a Wedge-Shaped Airframe

Experiments on a scale model of an advanced unconventional subsonic transport concept, the Blended Wing Body (BWB), have demonstrated significant shielding of inlet-radiated noise. A computational model of the shielding mechanism has been developed using a combination of boundary integral equation method (BIEM) and equivalent source method (ESM). The computation models the incident sound from a point source in a nacelle and determines the scattered sound field. In this way the sound fields with and without the airfoil can be estimated for comparison to experiment. An experimental test bed using a simplified wedge-shape airfoil and a broadband point noise source in a simulated nacelle has been developed for the purposes of verifying the analytical model and also to study the effect of engine nacelle placement on shielding. The experimental study is conducted in the Anechoic Noise Research Facility at NASA Langley Research Center. The analytic and experimental results are compared at 6300 and 8000 Hz. These frequencies correspond to approximately 150 Hz on the full scale aircraft. Comparison between the experimental and analytic results is quite good, not only for the noise scattering by the airframe, but also for the total sound pressure in the far field. Many of the details of the sound field that the analytic model predicts are seen or indicated in the experiment, within the spatial resolution limitations of the experiment. Changing nacelle location produces comparable changes in noise shielding contours evaluated analytically and experimentally. Future work in the project will be enhancement of the analytic model to extend the analysis to higher frequencies corresponding to the blade passage frequency of the high bypass ratio ducted fan engines that are expected to power the BWB.

Gerhold, Carl H.↗

NASA NTRS2006

Investigation of Acoustical Shielding by a Wedge-Shaped Airframe

Gerhold, Carl H.↗

NASA NTRS2004

Estimation of Soil Moisture with L-band Multi-polarization Radar

Through analyses of the model simulated data-base, we developed a technique to estimate surface soil moisture under HYDROS radar sensor (L-band multi-polarizations and 40deg incidence) configuration. This technique includes two steps. First, it decomposes the total backscattering signals into two components - the surface scattering components (the bare surface backscattering signals attenuated by the overlaying vegetation layer) and the sum of the direct volume scattering components and surface-volume interaction components at different polarizations. From the model simulated data-base, our decomposition technique works quit well in estimation of the surface scattering components with RMSEs of 0.12,0.25, and 0.55 dB for VV, HH, and VH polarizations, respectively. Then, we use the decomposed surface backscattering signals to estimate the soil moisture and the combined surface roughness and vegetation attenuation correction factors with all three polarizations.

Shi, J.↗

NASA NTRS2017

A Spaceflight Experiment to Determine the Effect of Chamfered Sample Holders on Atomic Oxygen Erosion

The exteriors of low Earth orbit (LEO) spacecraft are subjected to many environmental threats that can cause the surface materials to degrade. One of these threats is atomic oxygen (AO), which is formed by photo dissociation of molecular oxygen by energetic UV radiation. Atomic oxygen exposure can result in oxidative erosion of polymers leading to structural or thermal failure of spacecraft components. The amount of AO erosion expected during a mission can be calculated by knowing the AO erosion yield (Ey, volume loss per incident atom) of the material and the AO fluence expected for the mission. The Ey can be determined through dehydrated mass loss measurements of test samples if one knows the AO fluence, density, and exposure area. Such measurements have been made as part of flight experiments, including the Materials International Space Station Experiment 2 (MISSE 2) Polymers Experiment. The MISSE 2 Polymers Experiment sample holders had chamfered circular apertures that controlled the exposure area, but also allowed some additional AO to scatter from the chamfered edges onto the samples thus causing some samples to erode thru and peel at their perimeter due to this scattering effect. By modeling the scattered AO flux one can predict the actual total AO fluence, and hence more accurate sample Ey. Sample holders with different chamfered-perimeter to exposed-area ratios have been designed for future spaceflight experiments that allow a more accurate determination of the Ey for large area polymers, representative of their use on spacecraft surfaces.

Earth Orbital Environments↗

DOE OSTI2020

Deep Exclusive p 0 Electroproduction Measured in Hall A at Jefferson Lab with the Upgraded CEBAF

Our understanding of the proton's structure in terms of its fundamental degrees of freedom, quarks and gluons, is incomplete. Generalized Parton Distributions (GPDs) can enhance our understanding of the partonic structure of the proton as it includes the correlation between the momentum and transverse position of partons. Exclusive electroproduction of the pion (ep→e'p'π 0 ) is one of the potential channels to access the GPDs. GPDs are defined at the Bjorken limit where the total amplitude can be factorized in a hard scattering of the photon off the quark and a soft part described by the GPDs. At sufficiently high Q 2 , a factorization scheme for exclusive meson production processes exists but only for longitudinally polarized virtual photons. As long as the longitudinally polarized virtual photons dominate the cross-section, we can have factorization and extract the GPDs. But the existing data for π 0 production at low Q 2 and low x B show the dominance of transverse part of the cross-section over the longitudinal one. Some transversity GPD models have found that an effective way to factorize the contribution from transversely polarized virtual photons to explain the dominance of σ T over σ L , shown by existing data. The experiment E12-06-114 ran in experimental Hall A during 2014-2016. The primary goal of this experiment was to measure the DVCS cross-section but the experimental configuration also allows the measurement of deep exclusive π 0 production. Taking advantage of the upgraded CEBAF at Jefferson Lab, we explored the high Bjorken-x (0.60) and high Q 2 regime for the first time. The extracted cross-section terms for π 0 production helps us to test the validity of QCD factorization in our kinematic regime. Our π 0 production results can be used to test and improve the existing models of proton structure. Cross-section results will be presented at two different Q 2 values for fixed x B of 0.60.

Karki, Bishnu↗

DOE OSTI2014

Measurement of Ratios of ν μ Charged-Current Cross Sections on C, Fe, and Pb to CH at Neutrino Energies 2–20 GeV

We present measurements of ν μ charged-current cross section ratios on carbon, iron, and lead relative to a scintillator (CH) using the fine-grained MINERvA detector exposed to the NuMI neutrino beam at Fermilab. The measurements utilize events of energies 2 < E ν < 20 GeV , with ( E ν ) = 8 GeV , which have a reconstructed μ - scattering angle less than 17° to extract ratios of inclusive total cross sections as a function of neutrino energy E ν and flux-integrated differential cross sections with respect to the Bjorken scaling variable x . These results provide the first high-statistics direct measurements of nuclear effects in neutrino scattering using different targets in the same neutrino beam. Measured cross section ratios exhibit a relative depletion at low x and enhancement at large x . Both become more pronounced as the nucleon number of the target nucleus increases. The data are not reproduced by GENIE , a conventional neutrino-nucleus scattering simulation, or by the alternative models for the nuclear dependence of inelastic scattering that are considered.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

NASA NTRS1991

Benchmark calculations of thermal reaction rates. I - Quantal scattering theory

The thermal rate coefficient for the prototype reaction H + H2 yields H2 + H with zero total angular momentum is calculated by summing, averaging, and numerically integrating state-to-state reaction probabilities calculated by time-independent quantum-mechanical scattering theory. The results are very carefully converged with respect to all numerical parameters in order to provide high-precision benchmark results for confirming the accuracy of new methods and testing their efficiency.

Chatfield, David C.↗

DOE OSTI2016

Bistatic and Monostatic Radar Cross Section of Radially Inhomogeneous Spheres

The exact radar cross section (RCS) of a sphere made of perfect electrical conductor (PEC) can be computed from the well - known Mie series, and this has made the metal sphere a very useful object for calibrating radar. However, the scattering behavior for homogeneous dielectric spheres, radially - inhomogeneous layered dielectric spheres, or PEC spheres surrounded by multiple homogeneous layers of dielectric material is much more interesting than that of the simple PEC sphere. For example, a homogeneous dielectric sphere can have an RCS that is considerably larger than that of an identically sized PEC sphere, or a PEC sphere with appropriate dielectric coatings can appear much smaller than the uncoated sphere. Possibly more surprising, a dielectric sphere made of the correct magic material can become totally invisible to a monostatic radar, while exhibiting significant scattering in directions away from the back - scatter direction. Exact formulations, based on expansions of the field using vector spherical harmonics, are derived for the bistatic and monostatic RCS of these more complex spheres.

47 OTHER INSTRUMENTATION↗

DOE OSTI2016

THE IMPACT OF ACCURATE EXTINCTION MEASUREMENTS FOR X-RAY SPECTRAL MODELS

Interstellar extinction includes both absorption and scattering of photons from interstellar gas and dust grains, and it has the effect of altering a source's spectrum and its total observed intensity. However, while multiple absorption models exist, there are no useful scattering models in standard X-ray spectrum fitting tools, such as XSPEC. Nonetheless, X-ray halos, created by scattering from dust grains, are detected around even moderately absorbed sources, and the impact on an observed source spectrum can be significant, if modest, compared to direct absorption. By convolving the scattering cross section with dust models, we have created a spectral model as a function of energy, type of dust, and extraction region that can be used with models of direct absorption. This will ensure that the extinction model is consistent and enable direct connections to be made between a source's X-ray spectral fits and its UV/optical extinction.

79 ASTRONOMY AND ASTROPHYSICS↗

NASA NTRS1989

Modeling and observation of the radar polarization signature of forested areas

To understand radar measurements of forested areas, the authors have developed a model of L-band (25-cm) microwave scattering from a forest. The forest floor is modeled as a rough dielectric surface above which is a layer of nearly vertical dielectric cylinders representing tree trunks. Above this layer is a second layer consisting of randomly oriented cylinders which represent branches. The authors identify several scattering mechanisms and calculate the corresponding Stokes matrices, which combine to give the total Stokes matrix and resulting polarization signature. It is found that this simple model permits accurate prediction of the polarization of the scattered waves and that additional mechanisms, including the effects of leaves and twigs, are not required for the 25-cm observation of the forests studied. The authors present measurements of the polarization signature acquired over a forested area and show comparisons with model calculations.

Durden, Stephen L.↗