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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,009 records · Page 56
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DOE OSTI2021

First direct measurement of 59 Cu(p,α) 56 Ni: A step towards constraining the Ni-Cu cycle in the cosmos

Reactions on proton-rich nuclides drive the nucleosynthesis in core collapse supernovae (CCSNe) and in x-ray bursts (XRBs). CCSNe eject the nucleosynthesis products to the interstellar medium and hence are a potential inventory of p nuclei, whereas in XRBs nucleosynthesis powers the light curves. In both astrophysical sites the Ni-Cu cycle, which features a competition between 59 Cu(p,α) 56 Ni and 59 Cu(p,γ) 60 Zn, could potentially halt the production of heavier elements. Here, we report the first direct measurement of 59 Cu(p,α) 56 Ni using a reaccelerated 59Cu beam and a cryogenic solid hydrogen target. Furthermore, our results show that the reaction proceeds predominantly to the ground state of 56 Ni, and the experimental rate has been found to be lower than Hauser-Feshbach based statistical model predictions. New results hints that the νp process could operate at higher temperatures than previously inferred and therefore remains a viable site for synthesizing the heavier elements

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

Measurement of the Ne 18 ( α , p ) Na 21 reaction with the ANASEN active-target detector system at E c . m . = 2.5 – 4 MeV

The 18 Ne(α,p) 21 Na reaction plays a significant role in Type-I X-ray bursts. It is a major path in the breakout from the hot-CNO cycles to the synthesis of heavier elements in the αp- and rp-processes. An experiment to determine the cross section of this reaction was performed with the ANASEN active-target detector system, determining the cross section at energies between 2.5 and 4 MeV in the center-of-mass frame. The measured cross sections for reactions populating the ground state in 21 Na are consistent with results obtained from the time-inverse reaction, but significantly lower than the previously published experimental data of direct measurements. The total cross sections are also compared with those derived from indirect methods and statistical-model calculations. Furthermore, this experiment establishes a new experimental data set on the excitation function of the 18 Ne(α,p) 21 Na reaction, revealing the significance of the excited states' contributions to the total reaction cross section and allowing us to separate the contribution of the (α,2p) reaction. The impact of the measured cross section on thermal reaction rates is discussed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Cross sections of the 83 Rb⁢(p,γ)⁢ 84 Sr and 84 Kr⁢(p,γ)⁢ 85 Rb reactions at energies characteristic of the astrophysical γ process

We have measured the cross section of the Rb 83 ( p , γ ) Sr 84 radiative capture reaction in inverse kinematics using a radioactive beam of Rb 83 at incident energies of 2.4 and 2.7 A MeV. Prior to the radioactive beam measurement, the Kr 84 ( p , γ ) Rb 85 radiative capture reaction was measured in inverse kinematics using a stable beam of Kr 84 at an incident energy of 2.7 A MeV. The effective relative kinetic energies of these measurements lie within the relevant energy window for the γ process in supernovae. The central values of the measured partial cross sections of both reactions were found to be 0.17 – 0.42 times the predictions of statistical model calculations. Assuming the predicted cross section at other energies is reduced by the same factor leads to a slightly higher calculated abundance of the p nucleus Sr 84 , caused by the reduced rate of the Sr 84 ( γ , p ) Rb 83 reaction derived from the present measurement.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2015

Isotopic molybdenum total neutron cross section in the unresolved resonance region

Accurate isotopic molybdenum nuclear data are important because molybdenum can exist in nuclear reactor components including fuel, cladding, or as a high yield fission product. High-resolution time-of-flight neutron transmission measurements on highly enriched isotopic metallic samples of 95 Mo, 96 Mo, 98 Mo, and 100 Mo were performed in the resonance energy range from 1 to 620 keV. The measurements were taken with the newly developed modular 6 Li-glass transmission detector positioned at the 100-m experimental flight station. For the unresolved energy region (URR), new comprehensive methods of analysis were developed and validated in order to obtain accurate neutron total cross-section data from the measurement by correcting for background and transmission enhancement effects. Average parameters and fits to the total cross section for 95 Mo were obtained using the Hauser-Feshbach statistical model code FITACS, which is currently incorporated into the SAMMY code. Moreover, fits to the experimental data deviate from the current evaluated nuclear data file/B-VII.1 isotopic Mo evaluations by several percent in the URR.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗
DOE OSTI2016

Experimental study of the astrophysically important Na 23 ( α , p ) Mg 26 and Na 23 ( α , n ) Al 26 reactions

The 23 Na(α,p) 26 Mg and 23 Na(α,n) 26 Al reactions are important for our understanding of the 26 Al abundance in massive stars. The aim of this work is to report on a direct and simultaneous measurement of these astrophysically important reactions using an active target system. The reactions were investigated in inverse kinematics using 4 He as the active target gas in the detector. We measured the excitation functions in the energy range of about 2 to 6 MeV in the center of mass. We have found that the cross sections of the 23 Na(α,p) 26 Mg and the 23 Na(α,n) 26 Al reactions are in good agreement with previous experiments and with statistical-model calculations. As a result, the astrophysical reaction rate of the 23 Na(α,n) 26 Al reaction has been reevaluated and it was found to be larger than the recommended rate.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2017

Indirect study of the stellar Ar 34 ( α , p ) K 37 reaction rate through Ca 40 ( p , t ) Ca 38 reaction measurements

The 34 Ar(α,p) 37 K reaction is believed to be one of the last in a sequence of (α,p) and (p,γ) reactions within the T z = -1 , sd-shell nuclei, known as the αp-process. This process is expected to influence the shape and rise times of luminosity curves coming from type I x-ray bursts (XRBs). With very little experimental information known on many of the reactions within the αp-process, stellar rates are calculated using a statistical model, such as Hauser-Feshbach. Questions on the applicability of a Hauser-Feshbach model for the 34 Ar (α,p) 37 K reaction arise due to level density considerations in the compound nucleus, 38 Ca . We have performed high energy-resolution forward-angle 40 Ca (p,t) 38 Ca measurements with the K = 600 spectrograph at iThemba LABS in order to identify levels above the α-threshold in 38 Ca . States identified in this work were then used to determine the 34 Ar (α,p) 37 K reaction rate based on a narrow-resonance formalism. Comparisons are made to two standard Hauser-Feshbach model predicted rates at XRB temperatures.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2017

Accurate U 238 ( n , 2 n ) U 237 reaction cross-section measurements from 6.5 to 14.8 MeV

In this study, the cross section for the 238 U(n,2n) 237 U reaction has been measured in the incident neutron energy range from 6.5 to 14.8 MeV in small energy steps using an activation technique. Monoenergetic neutron beams were produced via the 2 H( d,n ) 3 He and 3 H ( d,n ) 4 He reactions. 238 U targets were activated along with Au and Al monitor foils to determine the incident neutron flux. The activity of the reaction products was measured in TUNL's low-background counting facility using high-resolution γ-ray spectroscopy. The results are compared with previous measurements and latest data evaluations. Statistical-model calculations, based on the Hauser-Feshbach formalism, have been carried out using the CoH 3 code and are compared with the experimental results. Finally, the present self-consistent and high-quality data are important for stockpile stewardship and nuclear forensic purposes as well as for the design and operation of fast reactors.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2017

Experimental measurement of 12 C + 16 O fusion at stellar energies

The total cross section of the 12 C + 16 O fusion reaction has been measured at low energies to investigate the role of this reaction during late stellar evolution burning phases. A high-intensity oxygen beam, produced by the 5 MV pelletron accelerator at the University of Notre Dame, impinged on a thick, ultrapure graphite target. Protons and γ rays were simultaneously measured in the center-of-mass energy range from 3.64 to 5.01 MeV for singles and from 3.73 to 4.84 MeV for coincidence events, using silicon and Ge detectors. Statistical model calculations were employed to interpret the experimental results. The emergence of a new resonance-like broad structure and a decreasing trend in the S-factor data towards lower energies (opposite to previous data) are found for the 12 C + 16 O fusion reaction. Furthermore, based on these results the uncertainty range of the reaction rate within the temperature range of late stellar burning environments is discussed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2018

Hauser-Feshbach fission fragment de-excitation with calculated macroscopic-microscopic mass yields

The Hauser-Feshbach statistical model is applied to the de-excitation of primary fission fragments using input mass yields calculated with macroscopic-microscopic models of the potential energy surface. We test the sensitivity of the prompt fission observables to the input mass yields for two important reactions, 235 U (n th , f) and 239 Pu (n th , f) , for which good experimental data exist. General traits of the mass yields, such as the location of the peaks and their widths, can impact both the prompt neutron and γ-ray multiplicities, as well as their spectra. Specifically, we use several mass yields to determine a linear correlation between the calculated prompt neutron multiplicity $\bar{v}$ and the average heavy-fragment mass $\langle$A h $\rangle$ of the input mass yields ∂$\bar{v}$/∂ $\langle$A h $\rangle$ = ± 0.1 (n / f )/u . The mass peak width influences the correlation between the total kinetic energy of the fission fragments and the total number of prompt neutrons emitted, $\bar{v}_T$ ( TKE ) . Finally, typical biases on prompt particle observables from using calculated mass yields instead of experimental ones are δ$\bar{v}$ = 4 % for the average prompt neutron multiplicity, δ$\overline{M}_γ$ = 1% for the average prompt γ-ray multiplicity, δ$\bar{ε}$ $LAB\atop{n}$ = 1 % for the average outgoing neutron energy, δ$\bar{ε}_γ$ = 1 % for the average γ-ray energy, and δ $\langle$TKE$\rangle$ = 0.4 % for the average total kinetic energy of the fission fragments.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2018

Experimental study of Ar 38 + α reaction cross sections relevant to the Ca 41 abundance in the solar system [Experimental study of Ar 38 + α induced cross sections relevant to the Ca 41 abundance in the solar system]

In massive stars, the 41 Ca(n,α) 38 Ar and 41 K(p,α) 38 Ar reactions have been identified as the key reactions governing the abundance of 41 Ca, which is considered as a potential chronometer for solar system formation. So far, due to experimental limitations, the 41 Ca(n,α) 38 Ar reaction rate is solely based on statistical model calculations. In the present study, we have measured the time-inverse 38 Ar(α,n) 41 Ca and 38 Ar(α,p) 41 K reactions using an active target detector. The reactions were studied in inverse kinematics using a 133-MeV 38 Ar beam and 4 He as the active-gas target. Both excitation functions were measured simultaneously in the energy range of 6.8 ≤ E c.m. ≤ 9.3 MeV. Furthermore by using detailed balance the 41 Ca(n,α) 38 Ar and 41 K(p,α) 38 Ar reaction rates were determined, which suggested a 20% increase in the 41 Ca yield from massive stars.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2019

Experimental constraints on the Zn 73 ( n , γ ) Zn 74 reaction rate

Background: The recent observation of a neutron-star merger finally confirmed one astrophysical location of the rapid neutron-capture process (r-process). Evidence of the production of A < 140 nuclei was seen, but there is still little detailed information about how those lighter elements are produced in such an environment. Many of the questions surrounding the A ≈ 80 nuclei are likely to be answered only when the nuclear physics involved in the production of r-process nuclei is well understood. Neutron-capture reactions are an important component of the r-process, and neutron-capture cross sections of r-process nuclei, which are very neutron rich, have large uncertainties. Purpose: Indirectly determine the neutron-capture cross section and reaction rate of 73 Zn(n,γ ) 74 Zn. Methods: The nuclear level density (NLD) and γ-ray strength function (γSF) of 74 Zn were determined following a total absorption spectroscopy (TAS) experiment focused on the β decay of 74 Cu into 74 Zn performed at the National Superconducting Cyclotron Laboratory. The NLD and γSF were used as inputs in a Hauser-Feshbach statistical model to calculate the neutron-capture cross section and reaction rate. Results: The NLD and γSF of 74 Zn were experimentally constrained for the first time using β-delayed γ rays measured with TAS and the β-Oslo method. The NLD and γSF were then used to constrain the neutron-capture cross section and reaction rate for the 73 Zn(n, γ ) 74 Zn reaction. In Conclusion, the uncertainty in the neutron-capture cross section and reaction rate of 73 Zn(n, γ ) 74 Zn calculated in TALYS was reduced to under a factor of 2 from a factor of 5 in the cross section and a factor of 11 in the reaction rate using the experimentally obtained NLD and γSF.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Strangeness-correlations on the pseudocritical line in ( 2 + 1 )-flavor QCD

We present some lattice QCD results on first ( χ 1 i ) and second ( χ 2 i ) cumulants of and correlations ( χ 11 i j ) among net baryon-number ( B ), strangeness ( S ) and electric charge ( Q ) along the pseudocritical line [ T p c ( μ B ) ] in the temperature ( T )–baryon chemical potential ( μ B ) phase diagram of ( 2 + 1 )-flavor QCD. We point out that violations of sum rules among second order cumulants, which hold in the isospin symmetric limit of vanishing electric charge chemical potential, are small along the T p c ( μ B ) for the entire range of μ B covered in the RHIC beam energy scan. For the strangeness neutral matter produced in heavy-ion collisions this leads to a close relation between χ 11 B S and χ 11 Q S . We compare lattice QCD results for χ 11 B S / χ 2 S along the T p c ( μ B ) line with preliminary experimental measurements of χ 11 B S / χ 2 S for collision energies 7.7 GeV ≤ s N N ≤ 62.4 GeV . While we find good agreements for s N N ≥ 39 GeV , differences are sizeable at smaller values of s N N . Moreover, we compare lattice QCD results for the ratio of the strangeness ( μ S ) to baryon ( μ B ) chemical potentials, which define a strangeness neutral system with fixed electric charge to baryon number density, with experimental results obtained by the STAR collaboration for μ S / μ B using strange baryon yields on the freeze-out line. Finally, we determine the baryon chemical potential at the freeze-out ( μ B f ) by comparing χ 1 B / χ 2 B along the T p c ( μ B ) with the experimentally measured net-proton cumulants χ 1 p / χ 2 p . We find that { μ B f , T p c ( μ B f ) } are consistent with the freeze-out parameters of the statistical-model fits to experimentally measured hadron yields for s N N ≥ 11.5 GeV . Published by the American Physical Society 2024

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2015

Self-replication with magnetic dipolar colloids

Colloidal self-replication represents an exciting research frontier in soft matter physics. Currently, all reported self-replication schemes involve coating colloidal particles with stimuli-responsive molecules to allow switchable interactions. In this paper, we introduce a scheme using ferromagnetic dipolar colloids and preprogrammed external magnetic fields to create an autonomous self-replication system. Interparticle dipole-dipole forces and periodically varying weak-strong magnetic fields cooperate to drive colloid monomers from the solute onto templates, bind them into replicas, and dissolve template complexes. We present three general design principles for autonomous linear replicators, derived from a focused study of a minimalist sphere-dimer magnetic system in which single binding sites allow formation of dimeric templates. We show via statistical models and computer simulations that our system exhibits nonlinear growth of templates and produces nearly exponential growth (low error rate) upon adding an optimized competing electrostatic potential. Lastly, we devise experimental strategies for constructing the required magnetic colloids based on documented laboratory techniques. We also present qualitative ideas about building more complex self-replicating structures utilizing magnetic colloids.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2018

Transition between inverse and direct energy cascades in multiscale optical turbulence

Transition between inverse and direct energy cascades in multiscale optical turbulence. Multiscale turbulence naturally develops and plays an important role in many fluid, gas, and plasma phenomena. Statistical models of multiscale turbulence usually employ Kolmogorov hypotheses of spectral locality of interactions (meaning that interactions primarily occur between pulsations of comparable scales) and scale-invariance of turbulent pulsations. However, optical turbulence described by the nonlinear Schrodinger equation exhibits breaking of both the Kolmogorov locality and scale-invariance. A weaker form of spectral locality that holds for multi-scale optical turbulence enables a derivation of simplified evolution equations that reduce the problem to a single scale modeling. We present the derivation of these equations for Kerr media with random inhomogeneities. Then, we find the analytical solution that exhibits a transition between inverse and direct energy cascades in optical turbulence.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2019

Breakdown of Fermi Degeneracy in the Simplest Liquid Metal

We are reporting the observation of the breakdown of electrons’ degeneracy and emergence of classical statistics in the simplest element: metallic deuterium. We have studied the optical reflectance, shock velocity and temperature of dynamically compressed liquid deuterium up to its Fermi temperature, TF. Above the insulator–metal transition, the optical reflectance shows the distinctive temperature-independent resistivity saturation, which is prescribed by the Mott-Ioffe-Regel minimum metallic limit, in agreement with previous experiments. At T > 0.4 T F , however, the reflectance of metallic deuterium starts to rise with a temperature-dependent slope, consistent with the breakdown of the Fermi surface. The experimentally inferred collisional time in this region exhibits the characteristic temperature dependence expected for a classical Landau-Spitzer plasma. Our observation of electron degeneracy lifting extends studies of degeneracy to new fermionic species, electron Fermi systems and offers an invaluable benchmark for quantum statistical models of Coulomb systems over a wide range of temperatures relevant to dense astrophysical objects and ignition physics.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2023

First Measurement of Antideuteron Number Fluctuations at Energies Available at the Large Hadron Collider

The first measurement of event-by-event antideuteron number fluctuations in high energy heavy-ion collisions is presented. The measurements are carried out at midrapidity (|η|<0.8) as a function of collision centrality in Pb-Pb collisions at $\sqrt{^sNN}$=5.02 TeV using the ALICE detector. A significant negative correlation between the produced antiprotons and antideuterons is observed in all collision centralities. The results are compared with a state-of-the-art coalescence calculation. While it describes the ratio of higher order cumulants of the antideuteron multiplicity distribution, it fails to describe quantitatively the magnitude of the correlation between antiproton and antideuteron production. On the other hand, thermal-statistical model calculations describe all the measured observables within uncertainties only for correlation volumes that are different with respect to those describing proton yields and a similar measurement of net-proton number fluctuations.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

ψ ( 2 S ) Suppression in Pb-Pb Collisions at the LHC

The production of the ψ ( 2 S ) charmonium state was measured with ALICE in Pb-Pb collisions at s NN = 5.02 TeV , in the dimuon decay channel. A significant signal was observed for the first time at LHC energies down to zero transverse momentum, at forward rapidity ( 2.5 < y < 4 ). The measurement of the ratio of the inclusive production cross sections of the ψ ( 2 S ) and J / ψ resonances is reported as a function of the centrality of the collisions and of transverse momentum, in the region p T < 12 GeV / c . The results are compared with the corresponding measurements in p p collisions, by forming the double ratio [ σ ψ ( 2 S ) / σ J / ψ ] Pb − Pb / [ σ ψ ( 2 S ) / σ J / ψ ] p p . It is found that in Pb-Pb collisions the ψ ( 2 S ) is suppressed by a factor of ∼ 2 with respect to the J / ψ . The ψ ( 2 S ) nuclear modification factor R AA was also obtained as a function of both centrality and p T . The results show that the ψ ( 2 S ) resonance yield is strongly suppressed in Pb-Pb collisions, by a factor of up to ∼ 3 with respect to p p . Comparisons of cross section ratios with previous Super Proton Synchrotron findings by the NA50 experiment and of R AA with higher- p T results at LHC energy are also reported. These results and the corresponding comparisons with calculations of transport and statistical models address questions on the presence and properties of charmonium states in the quark-gluon plasma formed in nuclear collisions at the LHC. © 2024 CERN, for the ALICE Collaboration 2024 CERN

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2022

Data-driven approach to parameterize SCAN + U for an accurate description of 3 d transition metal oxide thermochemistry

Semilocal density-functional theory (DFT) methods exhibit significant errors for the phase diagrams of transition-metal oxides that are caused by an incorrect description of molecular oxygen and the large self-interaction error in materials with strongly localized electronic orbitals. Empirical and semiempirical corrections based on the DFT + U method can reduce these errors, but the parameterization and validation of the correction terms remains an on-going challenge. Here we develop a systematic methodology to determine the parameters and to statistically assess the results by considering interlinked thermochemical data across a set of transition metal compounds. We consider three interconnected levels of correction terms: (1) a constant oxygen binding correction, (2) Hubbard-U correction, and (3) DFT/DFT + U compatibility correction. The parameterization is expressed as a unified optimization problem. We demonstrate this approach for 3d transition metal oxides, considering a target set of binary and ternary oxides. With a total of 37 measured formation enthalpies taken from the literature, the dataset is augmented by the reaction energies of 1710 unique reactions that were derived from the formation energies by systematic enumeration. To ensure a balanced dataset across the available data, the reactions were grouped by their similarity using clustering and suitably weighted. The parameterization is validated using leave-one-out cross validation (CV), a standard technique for the validation of statistical models. We apply the methodology to the strongly constrained and appropriately normed (SCAN) density functional. Based on the CV score, the error of binary (ternary) oxide formation energies is reduced by 40% (75%) to 0.10 (0.03) eV/atom. A simplified correction scheme that does not involve SCAN/SCAN + U compatibility terms still achieves an error reduction of 30% (25%). The method and tools demonstrated here can be applied to other classes of materials or to parameterize the corrections to optimize DFT + U performance for other target physical properties.

36 MATERIALS SCIENCE↗