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All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

CELAVI (Circular Economy Lifecycle Assessment and VIsualization) [SWR-20-87]

A circular economy emphasizes the efficient use of all resources (e.g., materials, land, water). Despite anticipated overall benefits to society, the transition to a circular economy is likely to create regional differences in impacts. Current tools are unable to fully evaluate these potential externalities, which will be important for informing research prioritization and regional decision making. The Circular Economy Lifecycle Assessment and VIsualization (CELAVI) framework allows stakeholders to quantify and visualize potential regional and sectoral transfers of impacts that could result from transitioning to a circular economy, with particular focus on energy materials. The framework uses system dynamics to model material flows for multiple circular economy pathways and decisions are based on learning-by-doing and are implemented via cost and strategic value of different circular economy pathways. It uses network theory to track the spatial and sectoral flow of functional units across a graph and discrete event simulation to to step through time and evaluate lifecycle assessment data at each time step. The framework is designed to be flexible and scalable to accommodate multiple energy materials and multiple energy technologies. The primary goal of CELAVI is to help answer questions about how material flows and environmental and economic impacts of energy systems might change if the circularity of energy systems increases.

Eberle, Annika↗
DOE OSTI2022

CELAVI (Circular Economy Lifecycle Assessment and VIsualization) v.1.3.1 9/30/2022 [SWR-20-87]

A circular economy emphasizes the efficient use of all resources (e.g., materials, land, water). Despite anticipated overall benefits to society, the transition to a circular economy is likely to create regional differences in impacts. Current tools are unable to fully evaluate these potential externalities, which will be important for informing research prioritization and regional decision making. The Circular Economy Lifecycle Assessment and VIsualization (CELAVI) framework allows stakeholders to quantify and visualize potential regional and sectoral transfers of impacts that could result from transitioning to a circular economy, with particular focus on energy materials. The framework uses system dynamics to model material flows for multiple circular economy pathways and decisions are based on learning-by-doing and are implemented via cost and strategic value of different circular economy pathways. It uses network theory to track the spatial and sectoral flow of functional units across a graph and discrete event simulation to to step through time and evaluate lifecycle assessment data at each time step. The framework is designed to be flexible and scalable to accommodate multiple energy materials and multiple energy technologies. The primary goal of CELAVI is to help answer questions about how material flows and environmental and economic impacts of energy systems might change if the circularity of energy systems increases.

Eberle, Annika↗
DOE OSTI2022

Organic Macromolecular materials for Efficient Transport Properties in Light-Energy Conversion Applications. Final Report

We are grateful for the Department of Energy for support of this research related to the improvement of power conversion efficiency of organic photovoltaic architectures over the years. As we noted at the beginning and now, the fundamental photophysical pathways that connect the absorption of light to the production of charge carriers remain elusive in spite of continuing experimental and theoretical efforts. Our investigations were directed toward gaining information about the mechanism of this ultrafast, long-range charge separation in photovoltaic systems with non-fullerene acceptors. This problem is still of high importance for the organic photovoltaics because solving this problem will allow us to minimize the contribution of the geminate recombination and trapping the charges in bound charge transfer states. Extremely low charge separation driving energy specific to non-fullerene acceptor systems reduces the energy loss in organic photovoltaic cells making them competitive with inorganic and perovskite photovoltaic systems. A major accomplishment of this study was to detail the long-range ballistic charge separation in donor-non-fullerene acceptor photovoltaic systems. We have successfully probed the spatial structure of ultrafast long-range (~40nm) ballistic charge separation in donor-non-fullerene acceptor photovoltaic system. We performed a systematic investigation of the delocalized states in their connection to the efficient long-range charge separation using the pulse pair interferometric near-field microscopy method. This method possesses unique capability of detecting coherent effects with spatial resolution of few tens of nanometers. These measurements allowed us the determination of delocalized excitations locally in a thin film photovoltaic system and to be connected to the long-range charge separation and the power conversion efficiency. We also investigated long-lived coupled triplet pairs in a singlet fission process for the possibility of concerted extraction of two electrons from triplet entangled states. New experimental and theoretical approaches of the concerted double electron extraction were carried out. The impact of this work is the development of important structure-property relationships to the design criteria of more efficient organic photovoltaic cells in accordance with the BES mission.

14 SOLAR ENERGY↗
NASA NTRS1977

A model for microwave intensity propagation in an inhomogeneous medium

A combined analytic and phenomenological approach, utilizing Maxwell's equations in the Born approximation with radiative transfer theory, is used to describe the propagation of microwave intensity in a scattering medium characterized by three-dimensional random fluctuations in refractive index, as well as nonrandom variations in permittivity, temperature, and loss. This approach yields microwave intensities as a function of polarization, direction, and position. Numerical techniques are presented to solve the transport equations, which include cases of spatially varying coefficients, and highly peaked phase functions. Some computed results illustrating the behavior of microwave intensity in various media are presented. Included are the angular and frequency spectra of thermal emission from semi-infinite media, and the diffuse transmission and reflection response of a scattering layer. The effects of scatterer geometry and scale sizes; correlation function; and gradients in temperature, loss, and scattering parameters are also demonstrated. This model should be particularly useful in interpreting active and passive remote sensing data.

Fisher, A. D.↗
NASA NTRS1979

Influence of convection on free growth of dendrite crystals from solution

The free growth of dendrites in a uniformly supercooled solution was examined using cine photography with a Schlieren optical system. Crystals were grown in the bulk of the solution from a centrally located capillary tube, nucleated at the interface with a liquid nitrogen cooled wire. Crystals propagated along the tube, the slower growing orientations eliminated, and emerged at the tip, usually growing parallel to the tube direction. For both sodium sulfate decahydrate from its solution and ice from sodium chloride solution, growth rate and fineness of dendrites increased with supercooling. In sodium sulfate, upward convection of the less dense depleted solution occurs; downward convection was observed for the rejected, more concentrated sodium chloride solution. In both cases, there was a spatial and temporal delay in the release of the convective plume from the moving dendrite tip. The role of this convection on the growth characteristics and the production of secondary crystals is examined. A proposed low-g experiment to examine differences in growth rate, crystal texture, and secondary nucleation in a reduced convective regime where molecular diffusion is the dominant transfer process is discussed.

Hallett, J.↗
NASA NTRS1984

Analytical estimates of turbulent MHD transport coefficients

Turbulent transfer rates from small-scale MHD excitations to large-scale Fourier modes are calculated algebraically, using the method of Biskamp and Welter. Three cases are considered: two-dimensional Navier-Stokes flows, two-dimensional incompressible MHD, and the weakly three-dimensional Strauss equations. In all cases, an initially large spectral gap between the small-scale and large-scale excitations is assumed, and attention focusses on the initial values of the back-transfer rates. The sign of the transfer is determined by the sign of an analytically calculable eddy viscosity and/or anomalous resistivity. We are able to confirm the results of Biskamp and Welter for the case of two-dimensional MHD, but find some differences for the case of the Strauss equations. It is argued that the Strauss equations may not exhibit an inverse cascade phenomenon for the spatially periodic case unless their initial spectra are such that the behavior is essentially that of two-dimensional MHD.

Montgomery, D.↗
NASA NTRS1994

Direct and indirect methods for correcting the aerosol effect on remote sensing

Aspects of aerosol studies and remote sensing are reviewed. Aerosol scatters solar radiation before it reaches the surface and scatters and absorbs it again after it is reflected from the surface and before it reaches the satellite sensor. The effect is spectrally and spatially dependent. Therefore atmospheric aerosol (dust, smoke and air pollution particles) has a significant effect on remote sensing. Correction for the aerosol effect was never achieved on an operational basis though several case studies were demonstrated. Correction can be done in a direct way by deriving the aerosol loading from the image itself and correcting for it using the appropriate radiative transfer model or by an indirect way, by defining remote sensing functions that are less dependent on the aerosol loading. To some degree this was already achieved in global remote sensing of vegetation where a composite of several days of NDVI (Normalized Difference Vegetation Index) measurements, choosing the maximal value, was used instead of a single cloud screened value. The Atmospheric Resistant Vegetation Index (ARVI) introduced recently for the NASA Earth Observing System EOS-MODIS is the most appropriate example of indirect correction, where the index is defined in such a way that the atmospheric effect in the blue spectral channel cancels to a large degree the atmospheric in the red channel in computations of a vegetation index. Atmospheric corrections can also use aerosol climatology and ground based instrumentation.

Kaufman, Yoram J.↗
NASA NTRS2001

Cloud Structure and Cloud-Radiation Interaction: From Smallest Observable Scales (Less than 10 m) to GCM Grid Scales (More than 100 km)

In this presentation we review the fractal nature of internal cloud structure from cm- to km-scales as captured by in-situ probes during long horizontal penetrations by aircraft. We uncover the non-Poissonian spatial distribution of cloud droplets at submeter scales and confirm scale-invariant behavior for large scales. Based on these structural characteristics, we generate simple fractal cloud models that reproduce statistical scaling properties of real clouds. These stochastic models represent a link between nonlinear science, in general, and cloud-radiation interaction, in particular. Next we run three-dimensional radiative transfer computations on these synthetic fractal clouds and compare the structure of the resulting radiation fields with the known structure of the cloud model and with satellite images of real clouds. The different behaviors observed for small and large-scale variabilities will be discussed in detail. We find that while the large-scale fluctuations of the resulting radiation fields resemble those in the original scale-invariant cloud structure, the radiation at small scales is much smoother than its cloud liquid water counterpart. This violates scale-invariance and produces a scale-break at 0.2-0.5 km that is clearly observed in high-resolution satellite data such as from Landsat. Finally, we show how radiative transfer Green function theory in the photon diffusion limit explains (and predicts) the above phenomena of "radiative smoothing."

Marshak, Alexander↗
NASA NTRSDate not supplied

Tools for Performing SBG hyperspectral Observing System Simulation Experiment

One of NASA’s Decadal Survey mission, Surface Biology and Geology (SBG), will include a hyperspectral remote sensing imager, which has a very high spatial resolution and a wide spectral coverage (from UV to Near IR). Unprecedented large data volumes will be generated by the SBG hyperspectral instrument. Before the launch of the new satellite, an Observing System Simulation Experiment (OSSE) can be used to study different designs of the new satellite system. One of the key components in an OSSE study is a radiative transfer model (RTM) or forward model. In this presentation, we will describe a Principal Component-based Radiative Transfer Model (PCRTM) which is capable of simulating atmospheric (TOA) radiance or reflectance spectra from far IR to visible and UV spectral regions (50 wavenumber to 30000 wavenumber) quickly and accurately. Multiple scattering from multiple layers of clouds/aerosols are included in the model. The PCRTM has a very good accuracy relative to reference line-by-line radiative transfer models (LBLRTM), and it saves 3-4 orders of magnitude computational time relative to LBLRTM or MODTRAN. The PCRTM model has been successfully used to analyze large volumes of data from hyperspectral sensors such as AIRS, CrIS, and IASI. It has also been used to perform OSSE studies for the Climate Absolute Radiance and Refractivity Observatory (CLARREO) mission. Another useful tool for the OSSE is surface Bidirectional Reflectance Distribution Function (BRDF) database. It is very crucial for the SBG OSSE to include realistic BRDF spectra. Currently, most of the surface reflectance spectra such as those in the ECOSIS and ECOSTRESS are measured at specific observation geometries. We have developed a hyperspectral bidirectional reflectance (HSBR) model which combines Ross-Li BRDF model with the existing reflectance spectral libraries using a principal component analysis. This HSBR model can provide realistic BRDF spectra under various observation conditions. It can also be used to generate realistic BRDF spectra using measurements from multi-band imagers or spectrometers such as MODIS or VIIRS.

Xu Liu↗
DOE OSTI2026

Collisionless Larmor coupling and blob formation in a laser-plasma expanding into a magnetized ambient plasma

Collisionless Larmor coupling is a fundamental process in space and astrophysical plasmas that enables momentum transfer between an expanding plasma and a magnetized ambient medium. Here, in this paper, we report on the laboratory experimental study of Larmor coupling leading to the formation of a plasma blob associated with a laser-driven, super-Alfvénic plasma flow on the Large Plasma Device at the University of California, Los Angeles. The high-repetition rate enables systematic spatial and temporal scans of the plasma evolution using Doppler spectroscopy, as well as measurements of the magnetic field, electrostatic field, and self-emission of both debris and ambient ions using filtered imaging. We observe the self-focusing of the laser-produced plasma and the formation of a secondary diamagnetic cavity associated with a blob composed of background ions. Doppler spectroscopy reveals the transverse velocity distribution of the background ions, providing direct evidence of ion energization via Larmor coupling. The systematic spatial and temporal scans enabled by the high-repetition-rate experiment allow for a detailed characterization of the ion dynamics. These experimental observations are supported by numerical simulations that provide more insight into the kinetic-scale physics associated with blob formation as well as the role of the ambient plasma density.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2026

Redefining precision interferometry and spectroscopy with high-performance optical interference coatings

High-performance optical interference coatings have transformed precision interferometry and spectroscopy by enabling unparalleled control over light–matter interactions. This review explores recent innovations in ion-beam sputtered amorphous dielectric, as well as substrate-transferred crystalline coatings, and their impact on systems at the forefront of precision metrology. These state-of-the-art coating techniques generate multilayers with ultralow optical losses, yielding mirrors with exceptional reflectivity. Refinements in their noise performance push the ultimate limits of sensitivity, resolution, and stability in demanding laser-based metrology applications. These technologies underpin the most advanced timekeeping and spatial measurement tools, enabling high-finesse reference cavities for the world’s most precise optical atomic clocks and low-noise reflective test masses for km-baseline gravitational-wave detectors. Emerging hybrid designs combining these techniques expand access to the mid-infrared spectral region, enabling the first ultralow-optical-loss coatings in the 3000–5000 nm wavelength range for enhanced spectroscopy and trace-gas detection. We highlight how these technologies redefine coating performance metrics and set new benchmarks in quantum science, fundamental physics, and precision optical sensing.

Cole, Garrett D. [University of Arizona, Tucson, A↗
DOE OSTI2023

LBNF/DUNE Cryostats and Cryogenics Infrastructure for the DUNE Far Detector (Design Report)

DUNE is an international experiment dedicated to addressing some of the questions at the forefront of particle physics and astrophysics, including the mystifying preponderance of matter over antimatter in the early universe. The dual-site experiment will employ an intense neutrino beam focused on both a near detector and a cryogenic far detector. The DUNE far detector implements liquid argon time-projection chamber (LArTPC) technology, and combines many tens-of-kilotons of fiducial mass with sub-centimeter spatial resolution to collect neutrino events and image them with high precision. Given its size, this detector will be implemented as a set of up to four modules, each of which will require its own cryostat that will contain approximately 17.5 metric kilotons of ultra-pure liquid argon (LAr). The cryogenics infrastructure to support the detector modules includes systems to receive, transfer, store, purify, and maintain the LAr. This design report describes the cryostats and the cryogenics infrastructure required for the first two detector modules; this infrastructure is designed to support expansion to up to four far detector modules.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2024

Improving Cost and Efficiency of the Scalable Solid Oxide Fuel Cells Power System

The objective of this project was to design and develop a 20kW range small-scale solid oxide fuel cells (SOFC) power system for applications such as data centers and commercial buildings. The original plan included a 5,000 hours demonstration and a Techno-Economic Analysis (TEA) which were dropped as part of project termination. The original project plan was to use a stack with a cross-flow cell design which had previously been tested for 500 hours at a community college in Malta, NY. However, it was decided to move to the advanced R-SOFC co-flow cell developed under Department of Energy Award DE-FE0031971. The advanced cell design has the advantage of a larger active area for the same manufacturing footprint which results in fewer required cells for the same stack power, hence a higher volumetric power density (kW/L) and lower cost per kW than the original cross-flow cell design. A full SOFC system Simulink model was developed and calibrated with testing data from a fuel cell stack and BOP (balance of plant) components. The simulation results from the calibrated model showed an acceptable match with the experimental data. A structural analysis conducted for various load scenarios indicated no high stress areas for all spatial directions. Major electrical system components were acquired, built and successfully tested. System sensors were verified and validated against controls. Safety checks, a diagnostic check, PID tuning, and control software commissioning tasks were also conducted. The power electronics prototype was delivered and trial testing completed. Balance of Plant component testing and simulation work was conducted to characterize Reformer-Heat Exchanger heat transfer and backpressure and reformer catalyst methane conversion and product selectivity. Simulations were conducted to design the Anode and Cathode fluid passages and size the air-air and fuel-fuel heat exchangers. A Burner operation map was created from test data and the Anode Gas Recirculation blower was tested to evaluate its durability. The SOFC system used a horizontal style design where components sit directly on a casting with a direct connection to the skid. This design has efficient packaging and a small footprint with approximate dimensions of 750 mm x 700 mm x 1700 mm. An SOFC system was built and successfully tested at the Malta, NY facility The system for over 500 hours under load of which over 300 hours was at full load of 20 kW.

30 DIRECT ENERGY CONVERSION↗
DOE OSTI2022

ENSO Impact on Winter Precipitation in the Southeast United States through a Synoptic Climate Approach

The ENSO impact on winter precipitation in the Southeast United States was analyzed from the perspective of daily weather types (WTs). We calculated the dynamic contribution associated with the change in frequency of the WTs and the thermodynamic contribution due to changes in the spatial patterns of the environmental fields of the WTs. Six WTs were obtained using a k-means clustering analysis of 850 hPa winds in reanalysis data from November to February of 1948–2022. All the WTs can only persist for a few days. The most frequent winter weather type is WT1 (shallow trough in Eastern U.S.), which can persist or likely transfer to WT4 (Mississippi River Valley ridge). WT1 becomes less frequent in El Niño years, while the frequency of WT4 does not change much. WTs 2–6 correspond to a loop of eastward propagating waves with troughs and ridges in the mid-latitude westerlies. Three WTs with a deep trough in the Southeast U.S., which are WT2 (east coast trough), WT3 (off east coast trough) and WT6 (plains trough), become more frequent in El Niño years. The more frequent deep troughs (WTs 2, 3 and 6) and less frequent shallow trough (WT1) result in above-normal precipitation in the coastal Southeast U.S. in the winter of El Niño years. WT5 (off coast Carolina High), with maximum precipitation extending from Mississippi Valley to the Great Lakes, becomes less frequent in El Niño years, which corresponds to the below-normal precipitation from the Great Lakes to Upper Mississippi and Ohio River Valley in El Niño years, and vice versa in La Niña years. The relative contribution of the thermodynamic and dynamic contribution is location dependent. On the east coast, the two contributions are similar in magnitude.

Qian, Jian-Hua↗
NASA NTRS1988

Modified radiative transfer theory for a two-layer anisotropic random medium

The modified radiative transfer (MRT) equations which describe propagation and scattering of the electromagnetic field intensity in a layered anisotropic random medium are derived from the Bethe-Salpeter equation with the ladder approximation and the Dyson equation with the nonlinear approximation. The extinction matrices and scattering phase matrices for both mean and incoherent field intensities are obtained. Backscattering enhancement is observed due to the spatial coherent effect between upward and downward propagating waves. It also occurs for the half-space case, because of coupling between ordinary and extraordinary waves. The depolarization effect is predicted in the first-order renormalization approximation to the MRT equation.

Lee, J. K.↗
NASA NTRS1996

Three-Dimensional Electromagnetic Monte Carlo Particle-in-Cell Simulations of Critical Ionization Velocity Experiments in Space

Although the existence of the critical ionization velocity (CIV) is known from laboratory experiments, no agreement has been reached as to whether CIV exists in the natural space environment. In this paper we move towards more realistic models of CIV and present the first fully three-dimensional, electromagnetic particle-in-cell Monte-Carlo collision (PIC-MCC) simulations of typical space-based CIV experiments. In our model, the released neutral gas is taken to be a spherical cloud traveling across a magnetized ambient plasma. Simulations are performed for neutral clouds with various sizes and densities. The effects of the cloud parameters on ionization yield, wave energy growth, electron heating, momentum coupling, and the three-dimensional structure of the newly ionized plasma are discussed. The simulations suggest that the quantitative characteristics of momentum transfers among the ion beam, neutral cloud, and plasma waves is the key indicator of whether CIV can occur in space. The missing factors in space-based CIV experiments may be the conditions necessary for a continuous enhancement of the beam ion momentum. For a typical shaped charge release experiment, favorable CIV conditions may exist only in a very narrow, intermediate spatial region some distance from the release point due to the effects of the cloud density and size. When CIV does occur, the newly ionized plasma from the cloud forms a very complex structure due to the combined forces from the geomagnetic field, the motion induced emf, and the polarization. Hence the detection of CIV also critically depends on the sensor location.

Wang, J.↗
NASA NTRS2011

An Algorithm for the Retrieval of 30-m Snow-Free Albedo from Landsat Surface Reflectance and MODIS BRDF

We present a new methodology to generate 30-m resolution land surface albedo using Landsat surface reflectance and anisotropy information from concurrent MODIS 500-m observations. Albedo information at fine spatial resolution is particularly useful for quantifying climate impacts associated with land use change and ecosystem disturbance. The derived white-sky and black-sky spectral albedos maybe used to estimate actual spectral albedos by taking into account the proportion of direct and diffuse solar radiation arriving at the ground. A further spectral-to-broadband conversion based on extensive radiative transfer simulations is applied to produce the broadband albedos at visible, near infrared, and shortwave regimes. The accuracy of this approach has been evaluated using 270 Landsat scenes covering six field stations supported by the SURFace RADiation Budget Network (SURFRAD) and Atmospheric Radiation Measurement Southern Great Plains (ARM/SGP) network. Comparison with field measurements shows that Landsat 30-m snow-free shortwave albedos from all seasons generally achieve an absolute accuracy of +/-0.02 - 0.05 for these validation sites during available clear days in 2003-2005,with a root mean square error less than 0.03 and a bias less than 0.02. This level of accuracy has been regarded as sufficient for driving global and regional climate models. The Landsat-based retrievals have also been compared to the operational 16-day MODIS albedo produced every 8-days from MODIS on Terra and Aqua (MCD43A). The Landsat albedo provides more detailed landscape texture, and achieves better agreement (correlation and dynamic range) with in-situ data at the validation stations, particularly when the stations include a heterogeneous mix of surface covers.

Shuai, Yanmin↗
DOE OSTI2023

RadVolViz: An Information Display-Inspired Transfer Function Editor for Multivariate Volume Visualization

In volume visualization transfer functions are widely used for mapping voxel properties to color and opacity. Typically, volume density data are scalars which require simple 1D transfer functions to achieve this mapping. If the volume densities are vectors of three channels, one can straightforwardly map each channel to either red, green or blue, which requires a trivial extension of the 1D transfer function editor. Here, we devise a new method that applies to volume data with more than three channels. These types of data often arise in scientific scanning applications, where the data are separated into spectral bands or chemical elements. Our method expands on prior work in which a multivariate information display, RadViz, was fused with a radial color map, in order to visualize multi-band 2D images. In this work, we extend this joint interface to blended volume rendering. The information display allows users to recognize the presence and value distribution of the multivariate voxels and the joint volume rendering display visualizes their spatial distribution. We design a set of operators and lenses that allow users to interactively control the mapping of the multivariate voxels to opacity and color. This enables users to isolate or emphasize volumetric structures with desired multivariate properties. Furthermore, it turns out that our method also enables more insightful displays even for RGB data. We demonstrate our method with three datasets obtained from spectral electron microscopy, high energy X-ray scanning, and atmospheric science.

36 MATERIALS SCIENCE↗