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NASA NTRS2007

Total Observed Organic Carbon (TOOC): A Synthesis of North American Observations

Measurements of organic carbon compounds in both the gas and particle phases made upwind, over and downwind of North America are synthesized to examine the total observed organic carbon (TOOC) in the atmosphere over this region. These include measurements made aboard the NOAA WP-3 and BAe-146 aircraft, the NOAA research vessel Ronald H. Brown, and at the Thompson Farm and Chebogue Point surface sites during the summer 2004 ICARTT campaign. Both winter and summer 2002 measurements during the Pittsburgh Air Quality Study are also included. Lastly, the spring 2002 observations at Trinidad Head, CA, surface measurements made in March 2006 in Mexico City and coincidentally aboard the C-130 aircraft during the MILAGRO campaign and later during the IMPEX campaign off the northwestern United States are incorporated. Concentrations of TOOC in these datasets span more than two orders of magnitude. The daytime mean TOOC ranges from 4.0 to 456 microg C/cubic m from the cleanest site (Trinidad Head) to the most polluted (Mexico City). Organic aerosol makes up 3-17% of this mean TOOC, with highest fractions reported over the northeastern United States, where organic aerosol can comprise up to 50% of TOOC. Carbon monoxide concentrations explain 46 to 86% of the variability in TOOC, with highest TOOC/CO slopes in regions with fresh anthropogenic influence, where we also expect the highest degree of mass closure for TOOC. Correlation with isoprene, formaldehyde, methyl vinyl ketone and methacrolein also indicates that biogenic activity contributes substantially to the variability of TOOC, yet these tracers of biogenic oxidation sources do not explain the variability in organic aerosol observed over North America. We highlight the critical need to develop measurement techniques to routinely detect total gas phase VOCs, and to deploy comprehensive suites of TOOC instruments in diverse environments to quantify the ambient evolution of organic carbon from source to sink.

Heald, C. L.↗

DOE OSTI2022

Impact of acute temperature and air pollution exposures on adult lung function: A panel study of asthmatics

Background Individuals with respiratory conditions, such as asthma, are particularly susceptible to adverse health effects associated with higher levels of ambient air pollution and temperature. This study evaluates whether hourly levels of fine particulate matter (PM 2.5 ) and dry bulb globe temperature (DBGT) are associated with the lung function of adult participants with asthma. Methods and findings Global positioning system (GPS) location, respiratory function (measured as forced expiratory volume at 1 second (FEV 1 )), and self-reports of asthma medication usage and symptoms were collected as part of the Exposure, Location, and Lung Function (ELF) study. Hourly ambient PM 2.5 and DBGT exposures were estimated by integrating air quality and temperature public records with time-activity patterns using GPS coordinates for each participant (n = 35). The relationships between acute PM 2.5 , DBGT, rescue bronchodilator use, and lung function collected in one week periods and over two seasons (summer/winter) were analyzed by multivariate regression, using different exposure time frames. In separate models, increasing levels in PM 2.5 , but not DBGT, were associated with rescue bronchodilator use. Conversely DBGT, but not PM 2.5 , had a significant association with FEV 1 . When DBGT and PM 2.5 exposures were placed in the same model, the strongest association between cumulative PM 2.5 exposures and the use of rescue bronchodilator was identified at the 0–24 hours (OR = 1.030; 95% CI = 1.012–1.049; p-value = 0.001) and 0–48 hours (OR = 1.030; 95% CI = 1.013–1.057; p-value = 0.001) prior to lung function measure. Conversely, DBGT exposure at 0 hours (β = 3.257; SE = 0.879; p-value>0.001) and 0–6 hours (β = 2.885; SE = 0.903; p-value = 0.001) hours before a reading were associated with FEV 1 . No significant interactions between DBGT and PM 2.5 were observed for rescue bronchodilator use or FEV 1 . Conclusions Short-term increases in PM 2.5 were associated with increased rescue bronchodilator use, while DBGT was associated with higher lung function (i.e. FEV 1 ). Further studies are needed to continue to elucidate the mechanisms of acute exposure to PM 2.5 and DBGT on lung function in asthmatics.

60 APPLIED LIFE SCIENCES↗

DOE OSTI2020

Atmospheric Temperature Inversions and He ι 5876 Core Profile Structure in White Dwarfs

Here we report distinctive core profiles in the strongest optical helium line, He ι λ5876, from high-resolution high-sensitivity observations of spectral type DB white dwarfs. By analyzing a sample of 40 stars from Keck/HIRES and VLT/UVES, we find the core appearance to be related to the degree of hydrogen and heavy element content in the atmosphere. New Ca K-line measurements or upper limits are reported for about half the sample stars. He ι λ5876 emission cores with a self-reversed central component are present for those stars with relatively low hydrogen abundance, as well as relatively low atmospheric heavy element pollution. This self-reversed structure disappears for stars with higher degrees of pollution and/or hydrogen abundance, giving way to a single absorption core. From our model atmospheres, we show that the self-reversed emission cores can be explained by temperature inversions in the upper atmosphere. We propose that the transition to a single absorption core is due to the additional opacity from hydrogen and heavy elements that inhibits the temperature inversions. Our current models do not exactly match the effective temperature range of the phenomenon or the amplitude of the self-reversed structure, which is possibly a result of missing physics such as 3D treatment, convective overshoot, and/or non-LTE effects. The He ι λ5876 line structure may prove to be a useful new diagnostic for calibrating temperature profiles in DB atmosphere models.

79 ASTRONOMY AND ASTROPHYSICS↗

NASA NTRS1975

Application of remote sensing to thermal pollution analysis

A comprehensive numerical model development program for near-field thermal plume discharge and far field general circulation in coastal regions is being carried on at the University of Miami Clean Energy Research Institute. The objective of the program is to develop a generalized, three-dimensional, predictive model for thermal pollution studies. Two regions of specific application of the model are the power plants sites at the Biscayne Bay and Hutchinson Island area along the Florida coastline. Remote sensing from aircraft as well as satellites are used in parallel with in situ measurements to provide information needed for the development and verification of the mathematical model. This paper describes the efforts that have been made to identify problems and limitations of the presently available satellite data and to develop methods for enhancing and enlarging thermal infrared displays for mesoscale sea surface temperature measurements.

Hiser, H. W.↗

NASA NTRSDate not supplied

1235 Preparing for TEMPO: A Review of Planned Metadata, Data Structure, and Distribution by NASA’s Atmospheric Science Data Center

The Atmospheric Science Data Center (ASDC) is in the Science Directorate located at the NASA Langley Research Center (LaRC), in Hampton, Virginia. The ASDC is one of NASA’s Distributed Active Archive Centers (DAAC) and supports over 60 projects and provides access to more than 1,000 archived collections. These datasets were created from satellite measurements, field experiments, and modeled data products. ASDC projects focus on the following Earth science disciplines: Radiation Budget, Clouds, Aerosols, and Tropospheric Composition. The ASDC is the official Distributed Active Archive Center (DAAC) of record for the upcoming Tropospheric Emissions: Monitoring of Pollution (TEMPO) instrument.. The instrument will share a ride on a commercial satellite as a hosted payload and will be launched to an orbit about 22,000 miles above Earth's equator. The investigation will, for the first time, use a space-based instrument to make accurate observations of tropospheric pollution concentrations of ozone, nitrogen dioxide, formaldehyde, and aerosols with high resolution and frequency over the U.S, Canada, and Mexico.

Ashlee Autore↗

NASA NTRSDate not supplied

1235 Preparing for TEMPO: A Review of Planned Metadata, Data Structure, and Distribution by NASA’s Atmospheric Science Data Center

Ashlee Autore↗

NASA NTRSDate not supplied

Satellite-Assisted Particulate Matter (SAPM) for the Models, In situ, and Remote sensing of Aerosols (MIRA) Working Group

Models, In situ, and Remote sensing of Aerosols (MIRA) is an international working group that aims to foster collaborations amongst these three major aerosol specialties. It consists of a collection of interdisciplinary and independently funded projects/topics with clearly-defined goals. Currently there are four MIRA topic areas, including Satellite-Assisted Particulate Matter (SAPM), which is focused specifically on fine particulate matter (PM2.5). The study of PM2.5 is important due to its significant contribution to air pollution and resultant, adverse human health effects. The goal of the SAPM topic group is to conduct and provide intercomparisons of various methods and techniques to obtain surface PM2.5 estimates assisted by satellite remote sensors, global aerosol models, and in situ aerosol measurements. Some benefits of space-based/model-assisted PM2.5 retrievals include providing PM2.5 approximations in regions with poor in situ ground station coverage and a means for assessing spatial/temporal PM2.5 variations on regional and/or global scales. Furthermore, benefits of spaceborne lidar/model-assisted PM2.5 retrievals include providing nighttime PM2.5 estimates and characterization of near-surface aerosol vertical structure. SAPM is seeking international datasets of mass scattering/absorption coefficient and aerosol hygroscopic properties for different aerosol species, as well as ground-based in situ PM2.5 measurements. In this poster presentation, we give an overview of SAPM, and show results from three recent/ongoing PM2.5 studies. These efforts involve deriving surface PM2.5 concentrations from two spaceborne lidars, the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) and Cloud-Aerosol Transport System (CATS), and investigating key variables that impact the estimation of PM2.5 from model simulated aerosol optical depth (AOD) using the Goddard Earth Observing System (GEOS) model.

Travis D. Toth↗

NASA NTRS2003

A Global Aerosol Model Forecast for the ACE-Asia Field Experiment

We present the results of aerosol forecast during the Aerosol Characterization Experiment (ACE-Asia) field experiment in spring 2001, using the Georgia Tech/Goddard Global Ozone Chemistry Aerosol Radiation and Transport (GOCART) model and the meteorological forecast fields from the Goddard Earth Observing System Data Assimilation System (GEOS DAS). The aerosol model forecast provides direct information on aerosol optical thickness and concentrations, enabling effective flight planning, while feedbacks from measurements constantly evaluate the model, making successful model improvements. We verify the model forecast skill by comparing model predicted total aerosol extinction, dust, sulfate, and SO2 concentrations with those quantities measured by the C-130 aircraft during the ACE-Asia intensive operation period. The GEOS DAS meteorological forecast system shows excellent skills in predicting winds, relative humidity, and temperature for the ACE-Asia experiment area as well as for each individual flight, with skill scores usually above 0.7. The model is also skillful in forecast of pollution aerosols, with most scores above 0.5. The model correctly predicted the dust outbreak events and their trans-Pacific transport, but it constantly missed the high dust concentrations observed in the boundary layer. We attribute this missing dust source to the desertification regions in the Inner Mongolia Province in China, which have developed in recent years but were not included in the model during forecasting. After incorporating the desertification sources, the model is able to reproduce the observed high dust concentrations at low altitudes over the Yellow Sea. Two key elements for a successful aerosol model forecast are correct source locations that determine where the emissions take place, and realistic forecast winds and convection that determine where the aerosols are transported. We demonstrate that our global model can not only account for the large-scale intercontinental transport, but also produce the small-scale spatial and temporal variations that are adequate for aircraft measurements planning.

Chin, Mian↗

NASA NTRS2020

Assessment of urban aerosol pollution over the Moscow megacity by the MAIAC aerosol product

We estimated the distribution of aerosol optical thickness (AOT) with a spatial resolution of 1 km over the Moscow megacity using the MAIAC aerosol product based on MODIS satellite data (Lyapustin et al., 2018) for the warm period of the year (May–September, 2001–2017). AERONET (Aerosol Robotic Network)-based validation of satellite estimates near the city centre at Moscow_MSU_MO and over the Moscow suburbs at Zvenigorod revealed that MAIAC AOT at 0.47 μm is in agreement with AERONET AOT though underestimated by 0.05–0.1 for AOT < 1 and overestimated for smoke conditions with AOT > 1. The MAIAC AOT biases were almost the same for the Moscow_MSU_MO and Zvenigorod AERONET sites, which indicated that the MAIAC algorithm effectively removed the effect of the bright urban surface in the city centre. For the ground-based measurements, the difference between annual median AOT at Moscow_MO_MSU and Zvenigorod (∆AOT) varied within -0:002 to +0:03, with statistically significant positive bias for most years, and an average ∆AOT was about 0.02. According to the MAIAC dataset, the ∆AOT varied within ±0:01 and was not statistically significant. The ∆AOT started decreasing recently due to intensive urban development of the territory around Zvenigorod and the decrease in pollutant emissions in Moscow, which is mainly caused by the environmental regulations. According to the MAIAC dataset, the most pronounced spatial AOT differences over the territory of Moscow were observed at the 5% quantile level, where they reached 0.05–0.06 over several locations and could be attributed to the stationary sources of aerosol pollution, for example, large areas of construction sites, aerosol pollution from roads and highways, or agriculture activities. The differences between the maximum and the mean AOT for different quantiles, except the 95% quantile, within the Moscow region, were about 0.02–0.04, which could be attributed to the local aerosol sources. The application of the MAIAC algorithm over the whole Moscow region has revealed a decreasing AOT trend over the centre of Moscow and an increasing trend over the “New” Moscow territory which experienced an intensive build-up and agricultural development.

urban aerosol pollution↗

NASA NTRS1971

Carbon monoxide pollution experiment. I - A solution to the carbon monoxide sink anomaly.

The observed lack of a high rate of growth in global CO concentration implies that there is some sink mechanism for destroying the CO as rapidly as it is being produced. A program is described which is intended to develop both the experiment concept and the remote sensor required to measure atmospheric CO with sufficient accuracy to locate the sink, whether it be at the earth's surface or in the upper atmosphere. The program calls for the development of a remote sensor which can look for surface sinks by mapping the vertical CO burden in the atmosphere on a daily basis, and which can look for an upper atmospheric sink by means of measurements of total CO in a horizontal path through the limb of the earth's atmosphere, using the sun as the source.

Grenda, R. N.↗

NASA NTRS1974

A study to identify and compare airborne systems for in-situ measurements of launch vehicle effluents

An in-situ system for monitoring the concentration of HCl, CO, CO2, and Al2O3 in the cloud of reaction products that form as a result of a launch of solid propellant launch vehicle is studied. A wide array of instrumentation and platforms are reviewed to yield the recommended system. An airborne system suited to monitoring pollution concentrations over urban areas for the purpose of calibrating remote sensors is then selected using a similar methodology to yield the optimal configuration.

Thomas, T. J.↗

NASA NTRS2019

A New Method to Retrieve the Diurnal Variability of Planetary Boundary Layer Height from Lidar Under Different Thermodynamic Stability Conditions

The planetary boundary layer height (PBLH) is an important parameter for understanding the accumulation of pollutants and the dynamics of the lower atmosphere. Lidar has been used for tracking the evolution of PBLH by using aerosol backscatter as a tracer, assuming aerosol is generally well-mixed in the PBL; however, the validity of this assumption actually varies with atmospheric stability. This is demonstrated here for stable boundary layers (SBL), neutral boundary layers (NBL), and convective boundary layers (CBL) using an 8-year dataset of micropulse lidar (MPL) and radiosonde (RS) measurements at the ARM Southern Great Plains, and MPL at the GSFC site. Due to weak thermal convection and complex aerosol stratification, traditional gradient and wavelet methods can have difficulty capturing the diurnal PBLH variations in the morning and forenoon, as well as under stable conditions generally. A new method is developed that combines lidar-measured aerosol backscatter with a stability dependent model of PBLH temporal variation (DTDS). The latter helps “recalibrate” the PBLH in the presence of a residual aerosol layer that does not change in harmony with PBL diurnal variation. The hybrid method offers significantly improved PBLH detection, with better correlation and smaller biases, under most thermodynamic conditions, especially for SBL and CBL. Relying on the physical process of PBL diurnal development, different schemes are developed for growing, maintenance, and decaying periods. Comprehensive evaluation of this new method shows much better tracking of diurnal PBLH variation and significantly smaller biases under various pollution levels.

Tianning Su↗

DOE OSTI2021

Optimal Design of Sustainable Ammonia-Based Food–Energy–Water Systems with Nitrogen Management

As the basis for virtually any form of nitrogen fertilizers, ammonia plays a vital role in agriculture; in addition, there has been an increased interest in its use as a carbon-free energy carrier. However, ammonia is also associated with two major environmental concerns: CO 2 emissions from the conventional production process and nitrogen pollution from the excessive use of ammonia-based fertilizers. To mitigate these environmental impacts, we develop an optimization framework for the design of a sustainable ammonia-based agricultural system that synergistically integrates the production of ammonia from renewable resources and effective measures for nitrogen management. The proposed model captures the effect of intermittency by incorporating both design and detailed operational decisions. Here, by applying a multiscale time representation that reduces the problem size and a tailored surrogate model that accurately approximates model nonlinearity, we are able to achieve optimal solutions within reasonable computation times. A computational case study is conducted using real-world data from a local farm in Morris, Minnesota, and the results indicate the trade-off between cost and nitrogen loss. Importantly, we show that practicing effective nitrogen management can significantly reduce the nitrogen loss with only a small increase in net present cost.

10 SYNTHETIC FUELS↗

DOE OSTI2025

Development of the Contamination Distribution Centered Toxics Mobility Vulnerability Index in the Beaumont–Port Arthur Region of Texas

This study advances the Toxics Mobility Inventory (TMI) and the Toxics Mobility Vulnerability Index (TMVI) to develop a new tool to assess the movement of hazardous substances and their implications for vulnerable communities. It emphasizes the need to include contamination distribution variables in such indices to address disproportionate impacts and more accurately reflect vulnerability. The study uses the TMI framework and TMVI methodology in the Beaumont–Port Arthur region of Texas, also integrating contamination distribution considerations into the analysis to develop a new framework and process. The new Contamination Distribution Centered Toxics Mobility Vulnerability Index (CDC-TMVI) consolidates climate change and topography variables into a broader built environment vulnerability category while introducing a contamination sources category. Using ArcGIS Pro and ToxPi tools, the study evaluates 27 geospatial variables across four categories: built environment vulnerability, social vulnerability, health outcomes, and contamination sources. The results indicate significant contributions from contamination and social vulnerability variables, highlighting areas with higher risks of flooding and air pollution. This article advocates for future research and policy efforts to enhance the integration of contamination sources and their spatial distributions into toxics mobility assessments to better protect vulnerable populations. Furthermore, the unique methodology and findings serve as a basis for developing targeted measures and strategic planning to improve environmental health.

contamination↗

NASA NTRS1977

Remotely sensed and laboratory spectral signatures of an ocean-dumped acid waste

An ocean-dumped acid waste plume was studied by using a rapid scanning spectrometer to remotely measure ocean radiance from a helicopter. The results of these studies are presented and compared with results from sea truth samples and laboratory experiments. An ocean spectral reflectance signature and a laboratory spectral transmission signature were established for the iron-acid waste pollutant. The spectrally and chemically significant component of the acid waste pollutant was determined to be ferric iron.

Lewis, B. W.↗

NASA NTRS1997

An Overview of the Tropospheric Aerosol Radiative Forcing Observational Experiment

Aerosol effects on atmospheric radiation are a leading source of uncertainty in predicting future climate. As a result, the International Global Atmospheric Chemistry Program has established a Focus on Atmospheric Aerosols (IGAC/FAA) and endorsed a series of aerosol field campaigns. TARFOX, the second in the IGAC/FAA series, was designed to reduce this uncertainty by measuring aerosol properties and effects in the US eastern seaboard, where one of the world's major plumes of industrial haze moves from the continent over the Atlantic Ocean. TARFOX's objectives are to: 1. Make simultaneous measurements of: (a) aerosol effects on radiation fields, and (b) the chemical, physical, and optical properties of the aerosols causing those effects. 2. Perform a variety of closure studies by using overdetermined data sets to test the mutual consistency of measurements and calculations of a wide range of aerosol properties and effects. 3. Use the results of the closure studies to assess and reduce uncertainties in estimates of aerosol radiative forcing, as well as to guide future field programs. An important subset of the closure studies is tests and improvements of algorithms used to derive aerosol properties and radiative effects from satellite measurements. The TARFOX Intensive Field Period (IFP) was conducted July 10-31, 1996. It included coordinated measurements from four satellites (GOES-8, NOAA-14, ERS-2, LANDSAT), four aircraft (ER-2, C-130, C-131, and a modified Cessna), land sites, and ships. A variety of aerosol conditions was sampled, ranging from relatively clean behind frontal passages to moderately polluted with aerosol optical depths exceeding 0.5 at mid-visible wavelengths. The latter conditions included separate incidents of enhancements caused primarily by anthropogenic sources and another incident of enhancement apparently influenced by recent fog processing. Spatial gradients of aerosol optical thickness were sampled to aid in isolating aerosol effects from other radiative effects and to more tightly constrain closure tests, including those of satellite retrievals. This talk gives an overview of TARFOX goals, rationale, methods, and initial key findings.

Russell, P. B.↗

NASA NTRS2002

Tropospheric Ozone during the TRACE-P Mission: Comparison between TOMS Satellite Retrievals and Aircraft Lidar Data, March 2001

Over the past several years, we have developed two new tropospheric ozone retrievals from the TOMS (Total Ozone Mapping Spectrometer) satellite instrument that are of sufficient resolution to follow pollution episodes. The modified-residual technique uses v. 7 TOMS total ozone and is applicable to tropical regimes in which the wave-one pattern in total ozone is observed. The TOMS-direct method ('TDOT' = TOMS Direct Ozone in the Troposphere) represents a new algorithm that uses TOMS radiances directly to extract tropospheric ozone in regions of constant stratospheric ozone. It is not geographically restricted, using meteorological regimes as the basis for classifying TOMS radiances and for selecting appropriate comparison data. TDOT is useful where tropospheric ozone displays high mixing ratios and variability characteristic of pollution. Some of these episodes were observed downwind of Asian biomass burning during the TRACE-P (Transport and Atmospheric Chemical Evolution-Pacific) field experiment in March 2001. This paper features comparisons among TDOT tropospheric ozone column depth, integrated uv-DIAL measurements made from NASA's DC-8, and ozonesonde data.

Frolov, A. D.↗

NASA NTRS2010

A Mesoscale Analysis of Column-Integrated Aerosol Properties in Northern India During the TIGERZ 2008 Pre-Monsoon Period and a Comparison to MODIS Retrievals

The Indo-Gangetic Plain (IGP) of the northern Indian subcontinent produces anthropogenic pollution from urban, industrial and rural combustion sources nearly continuously and is affected by convection-induced winds driving desert and alluvial dust into the atmosphere during the premonsoon period. Within the IGP, the NASA Aerosol Robotic Network (AERONET) project initiated the TIGERZ measurement campaign in May 2008 with an intensive operational period from May 1 to June 23, 2008. Mesoscale spatial variability of aerosol optical depth (AOD, tau) measurements at 500mn was assessed at sites around Kanpur, India, with averages ranging from 0.31 to 0.89 for spatial variability study (SVS) deployments. Sites located downwind from the city of Kanpur indicated slightly higher average aerosol optical depth (delta Tau(sub 500)=0.03-0.09). In addition, SVS AOD area-averages were compared to the long-tenn Kanpur AERONET site data: Four SVS area-averages were within +/- 1 cr of the climatological mean of the Kanpur site, while one SVS was within 2sigma below climatology. For a SVS case using AERONET inversions, the 440-870mn Angstrom exponent of approximately 0.38, the 440-870mn absorption Angstrom exponent (AAE) of 1.15-1.53, and the sphericity parameter near zero suggested the occurrence of large, strongly absorbing, non-spherical aerosols over Kanpur (e.g., mixed black carbon and dust) as well as stronger absorption downwind of Kanpur. Furthermore, the 3km and lOkm Terra and Aqua MODIS C005 aerosol retrieval algorithms at tau(sub 550) were compared to the TIGERZ data set. Although MODIS retrievals at higher quality levels were comparable to the MODIS retrieval uncertainty, the total number of MODIS matchups (N) were reduced with subsequent quality levels (N=25, QA>=0; N=9,QA>=l; N=6, QA>=2; N=1, QA=3) over Kanpur during the premonsoon primarily due to the semi-bright surface, complex aerosol mixture and cloud-contaminated pixels. The TIGERZ 2008 data set provided a unique opportunity to measure the spatial and temporal variations of aerosol loading in the IGP. The strong aerosol absorption derived from ground-based sun/sky radiometer measurements suggested the presence of a predominately black carbon and dust mixture during the pre-monsoon period. Consistent with the elevated heat-pump hypothesis, these absorbing aerosols found across Kanpur and the greater IGP region during the pre-monsoon period likely induced regional atmospheric warming, which lead to a more rapid advance of the southwest Asian monsoon and above normal precipitation over northern India in June 2008.

Giles, D. M.↗