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NASA NTRSDate not supplied

Parallel Plate Capacitor Aluminum KIDs for Future Far-Infrared Space-Based Observatories

Future space-based far-infrared astrophysical observatories will require exquisitely sensitive detectors consistent with the low optical backgrounds. The PRobe far-Infrared Mission for Astrophysics (PRIMA) will deploy arrays of thousands of superconducting kinetic inductance detectors (KIDs) sensitive to radiation between 25 and 265 μm. Here, we present laboratory characterization of prototype, 25 – 80 μm wavelength, low-volume, aluminum KIDs designed for the low-background environment expected with PRIMA. A compact parallel plate capacitor is used to minimize the detector footprint and suppress TLS noise. A novel resonant absorber is designed to enhance response in the band of interest. We present noise and optical efficiency measurements of these detectors taken with a low background cryostat and a cryogenic blackbody. A microlens-hybridized KID array is found to be photon noise limited down to about 50 aW with a limiting detector NEP of about 6.5×10 −19 W/Hz 1/2 . A fit to an NEP model shows that our optical system is well characterized and understood down to 50 aW. We discuss future plans for low-volume aluminum KID array development as well as the testbeds used for these measurements.

Far-Infrared↗

NASA NTRS1990

Energetics and dynamics of resonant and nonresonant scattering in strong magnetic fields

The energetics and the dynamics resulting from electron-photon resonant and nonresonant scattering in a plasma with magnetic field about 10 to the 12th G are studied in detail. Precise analytic results are obtained in the optically thin limit, and numerical results are presented for the optically thick case. For the latter, it is found that when the equilibrium temperature T(C) is determined by the cooling/heating balance due solely to cyclotron resonant scattering, the ratio of T(C) to the superstrong field B remains fairly constant for N(e) up to about 6 x 10 to the 21st electrons/sq cm. This line-dominated region comes to an end when the extra heating from the hard continuum photons becomes competitive with the line processes and drives T(C) well above the pure line value. For parameters characteristic of GB 880205, the thickness of the line-dominated region is determined to be between 10 to the 21st and 10 to the 22nd electrons/sq cm.

Lamb, Don Q.↗

NASA NTRS2021

Crucial Factors for Lyα Transmission in the Reionizing Intergalactic Medium: Infall Motion, H II Bubble Size, and Self-shielded Systems

Using the CoDa II simulation, we study the Lyα transmissivity of the intergalactic medium (IGM) during reionization. At z>6, a typical galaxy without an active galactic nucleus fails to form a proximity zone around itself due to the overdensity of the surrounding IGM. The gravitational infall motion in the IGM makes the resonance absorption extend to the red side of Lyα, suppressing the transmission up to roughly the circular velocity of the galaxy. In some sight lines, an optically thin blob generated by a supernova in a neighboring galaxy results in a peak feature, which can be mistaken for a blue peak. Redward of the resonance absorption, the damping-wing opacity correlates with the global IGM neutral fraction and the UV magnitude of the source galaxy. Brighter galaxies tend to suffer lower opacity because they tend to reside in larger H II regions, and the surrounding IGM transmits redder photons, which are less susceptible to attenuation, owing to stronger infall velocity. The H II regions are highly nonspherical, causing both sight-line-to-sight-line and galaxy-to-galaxy variation in opacity. Also, self-shielded systems within H II regions strongly attenuate the emission for certain sight lines. All these factors add to the transmissivity variation, requiring a large sample size to constrain the average transmission. The variation is largest for fainter galaxies at higher redshift. The 68% range of the transmissivity is similar to or greater than the median for galaxies with M(sub UV) ≽ -21 at z ≽ 7, implying that more than a hundred galaxies would be needed to measure the transmission to 10% accuracy.

Reionization↗

NASA NTRS2018

Remote Detection Sodium Cell Magnetometry Using Amplitude Modulated Light

We have investigated the performance of a remote-detection sodium cell magnetometer using synchronous optical pumping with amplitude modulated light. The magnetometer is used to measure ambient geomagnetic field with high-sensitivity using backscattered resonance fluorescence.

Line shapes and shifts and Spectroscopy↗

NASA NTRS1995

Slightly anharmonic systems in quantum optics

We consider an arbitrary atomic system (n-level atom or many such atoms) interacting with a strong resonant quantum field. The approximate evolution operator for a quantum field case can be produced from the atomic evolution operator in an external classical field by a 'quantization prescription', passing the operator arguments to Wigner D-functions. Many important phenomena arising from the quantum nature of the field can be described by such a way.

Klimov, Andrey B.↗

DOE OSTI2023

Fabrication Development for SPT-SLIM, a Superconducting Spectrometer for Line Intensity Mapping

Line Intensity Mapping (LIM) is a new observational technique that uses low-resolution observations of line emission to efficiently trace the large-scale structure of the Universe out to high redshift. Common mm/sub-mm emission lines are accessible from ground-based observatories, and the requirements on the detectors for LIM at mm-wavelengths are well matched to the capabilities of large-format arrays of superconducting sensors. We describe the development of an R = lambda/Delta lambda = 300 on-chip superconducting filter-bank spectrometer covering the 120-180 GHz band for future mm-LIM experiments, focusing on SPT-SLIM, a pathfinder LIM instrument for the South Pole Telescope. Radiation is coupled from the telescope optical system to the spectrometer chip via an array of feedhorn-coupled orthomode transducers. Superconducting microstrip transmission lines then carry the signal to an array of channelizing half-wavelength resonators, and the output of each spectral channel is sensed by a lumped element kinetic inductance detector (leKID). Key areas of development include incorporating new low-loss dielectrics to improve both the achievable spectral resolution and optical efficiency and development of a robust fabrication process to create a galvanic connection between ultra-pure superconducting thin-films to realize multi-material (hybrid) leKIDs. We provide an overview of the spectrometer design, fabrication process, and prototype devices.

microstrip resonators↗

DOE OSTI2020

Detecting Phase-Resolved Magnetization Dynamics by Magneto-Optic Effects at 1550 nm Wavelength

We demonstrate the detection of phase-resolved magnetization dynamics with combinatorial magneto-optic Kerr and Faraday effects. The method uses a continuous-wave laser that is amplitude-modulated at the spin dynamic frequencies, and thus allows for coherent tracking of the spin dynamics, akin a “lock-in” type measurement. In particular, our method, using a single 1550-nmwavelength, probes simultaneously the ferromagnetic resonance of Y 3 Fe 5 O 12 (YIG) and Permalloy (Py = Ni 80 Fe 20 ) in a YIG-Pyhetero structure. The fiber-based magneto-optic components also have the advantage of being made into a compact, tabletop or even portable system with yet robust measurement performances. We believe that our method will be found useful in studying hybrid quantum magnonic systems and/or investigating phase-resolved spin dynamics in nanomagnet structures involving both ferromagnetic insulators and metals.

42 ENGINEERING↗

NASA NTRS1999

A Comparison of Ultraviolet, Optical, and X-Ray Imagery of Selected Fields in the Cygnus Loop

During the Astro-1 and Astro-2 Space Shuttle missions in 1090 and 199.5, far ultraviolet (FUV) images of five 40' diameter fields around the rim of the Cygnus Loop supernova remnant were observed with the Ultraviolet Imaging Telescope (UIT). These fields sampled a broad range of conditions including both radiative and nonradiative shocks in various geometries and physical scales. In these shocks, the UIT B5 band samples predominantly C IV Lambda-1550 and the hydrogen two-photon recombination continuum. Smaller contributions are made by emission lines of He II Lambda-1640 and O III] Lambda-1665. We present these new FUV images and compare them with optical H-alpha and [O III], and ROSAT HRI X-ray images. Comparing the UIT images with those from the other bands provides new insights into the spatial variations and locations of these different types of emission. By comparing against shock model calculations and published FUV spectroscopy at select locations, we surmise that resonance scattering in the strong FUV permitted lines is widespread in the Cygnus Loop. especially in the bright optical filaments typically selected for observation in most previous studies.

Danforth, Charles W.↗

DOE OSTI2020

Quantum dot polarisation converter in an optomechanical cavity

We propose a scheme of a quantum photon polarisation converter, which is based on controlled electron – photon – phonon transitions in a hybrid semiconductor nanostructure. This structure consists of a GaAs/InAs quantum dot (QD) that has a parallelepiped shape and contains a single electron, and an optomechanical microcavity (MC) based on a photonic crystal (PC) that supports two orthogonally polarised photonic modes and one mechanical (phonon) mode. Within the framework of the microscopic theory, the QD and MC performance characteristics are found. Populations of states of the system as functions of time and its parameters are calculated. The principal possibility of photon polarisation conversion using transitions in a five-level resonance scheme for coherent (single-photon) and steady-state (subphoton) regimes is shown. The MC optical and mechanical spectra are simulated, and the PC structure parameters are selected to ensure the efficient operation of the converter. (paper)

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2020

Ultrathin, polarization-independent, achromatic metalens for focusing visible light

An optical device includes a titanium dioxide substrate layer on a quartz base of a substrate. The substrate is configured to focus light in visible wavelength spectrum of 400 nm to 700 nm. The substrate comprises a first zone and a second zone. In some embodiments, the first zone and the second zone are concentric circles. A plurality of resonators are disposed on the substrate, the plurality of resonators comprising a first plurality corresponding to the first zone and a second plurality corresponding to the second zone. Each resonator is comprised of a dielectric material with a defined thickness “t” in the range of 30 nm to 300 nm. Each resonator has a radius “r” in the range of 30 nm to 300 nm and a gap “g” between adjacent resonators in the range of 5 nm to 200 nm. The first plurality of resonators in the first zone have a first radius within a first radius range that is different from a second radius range of the second plurality of resonators in the second zone. The plurality of resonators form a metasurface that defines at least in part an ultra-thin achromatic lens of the optical device.

47 OTHER INSTRUMENTATION↗

NASA NTRS1994

Magnetospheric imaging of high latitude ion outflows

High latitude ion outflows mostly consist of upward streaming O(+) and He(+) emanating from the ionosphere. At heights above 1000 km, these flows consist of cold and hot components which resonantly scatter solar extreme ultraviolet (EUV) light, however, the ion populations respond differently to Doppler shifting resulting from the large relative velocities between the ions and the Sun. The possibility of optical detection of the Doppler effect on the scattering rate will be discussed for the O(+) (83.4 nm) ions. We have contrasted the EUV solar resonance images of these outflows by simulations of the 30.4 nm He(+) and 83.4 nm O(+) emissions for both quiet and disturbed geomagnetic conditions. Input data for the 1000 km level has been obtained from the EICS instrument aboard the Dynamics Explorer (DE) satellite. Our results show emission rates of 50 and 56 milli-Rayleighs at 30.4 nm for quiet and disturbed conditions and 65 and 75 milli-Rayleighs at 83.4 nm for quiet and disturbed conditions, respectively, obtained for a polar orbiting satellite and viewing radially outward. We also find that an imager at an equatorial distance of 9 R(sub E) or more is in a favorable position for detecting ion outflows, particularly when the plasmapause is depressed in latitude. However, an occultation disk is necessary to obscure the bright plasmaspheric emissions.

Garrido, D. E.↗

NASA NTRS1971

Tests and comparisons of gravity models.

Optical observations of the GEOS satellites were used to obtain orbital solutions with different sets of geopotential coefficients. The solutions were compared before and after modification to high order terms (necessary because of resonance) and were then analyzed by comparing subsequent observations with predicted trajectories. The most important source of error in orbit determination and prediction for the GEOS satellites is the effect of resonance found in most published sets of geopotential coefficients. Modifications to the sets yield greatly improved orbits in most cases. The results of these comparisons suggest that with the best optical tracking systems and gravity models, satellite position error due to gravity model uncertainty can reach 50-100 m during a heavily observed 5-6 day orbital arc. If resonant coefficients are estimated, the uncertainty is reduced considerably.

Marsh, J. G.↗

DOE OSTI2023

Phonon-induced collective modes in spin-orbit coupled polar metals

We study the interplay between collective electronic and lattice modes in polar metals in an applied magnetic field aligned with the polar axis. Static spin-orbit coupling leads to the appearance of a particle-hole spin-flip continuum that is gapped at low energies in a finite field. We find that a weak spin-orbit assisted coupling between electrons and polar phonons induces the emergence of electronic collective modes. The strength of the applied magnetic field tunes the number of modes and their energies, which can lie both above and below the particle-hole continuum. For a range of field values, we identify Fano-type interference between the electronic continuum and phonons. Here, we show that signatures of these collective modes can be observed in optical spectroscopy experiments, and we provide the corresponding theoretical predictions.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2021

Nonlinear Optics Measurements in IOTA

Nonlinear integrable optics is a recently proposed accelerator lattice design approach which allows to generate an amplitude dependent tune shift which is needed in high brightness accelerators to mitigate fast coherent instabilities. Whereas usually octupoles are used to achieve this task, this concept allows doing so without exciting any resonances, in turn preventing any particle loss. The concept is based around a special magnet design, together with specific constraints on the optics of the accelerator. To study such a system, the Integrable Optics Test Accelerator (IOTA) was recently constructed and commissioned at Fermilab. For the assessment of the performance of this concept, good knowledge of the optics and the (non-)linear dynamics without the special magnet is of key importance. As such, measurements were conducted in the IOTA ring, using the captured turn-by-turn data by the beam position monitors after excitation to infer quantities such as amplitude detuning and resonance driving terms. In this note, first results of these measurements are presented.

43 PARTICLE ACCELERATORS↗

DOE OSTI2022

Magnetic and Optical Properties of Au–Co Solid Solution and Phase-Separated Thin Films and Nanoparticles

The chemical composition and morphology of Au x Co 1–x thin films and nanoparticles are controlled via a combination of cosputtering, pulsed laser-induced dewetting (PLiD), and annealing, leading to tunable magnetic and optical properties. Regardless of chemical composition, the as-deposited thin films and as-PLiD nanoparticles are found to possess a face-centered cubic (FCC) Au x Co 1–x solid-solution crystal structure. Annealing results in large phase-separated grains of Au and Co in both the thin films and nanostructures for all chemical compositions. The magnetic and optical properties are characterized via vibrating sample magnetometry (VSM), ellipsometry, optical transmission spectroscopy, and electron energy loss spectroscopy (EELS). Despite the exceptionally high magnetic anisotropy inherent to Co, the presence of sufficient Au (72 atom %) in the Au x Co 1–x solid solution results in superparamagnetic thin films. Among the as-PLiD nanoparticle samples, an increased Co composition leads to a departure from traditional ferromagnetism in favor of wasp-waisted hysteresis caused by magnetic vortices. Phase separation resulting from annealing leads to ferromagnetism for all compositions in both the thin films and nanoparticles. The optical properties of Au x Co 1–x nanostructures are also largely influenced by the chemical morphology, where the Au x Co 1–x intermixed solid solution has significantly damped plasmonic performance relative to pure Au and comparable to pure Co. Phase separation greatly enhances the quality factor, optical absorption, and electron energy loss spectroscopy (EELS) signatures. The enhancement of the localized surface plasmon resonances (LSPRs) scales with the reduction in Co composition, despite EELS evidence that excitation of the Co portions of a nanoparticle can provide a similar, and in some instances enhanced, LSPR resonance compared to Au. This behavior, however, is seemingly limited to the LSPR dipole mode, while higher-order modes are greatly damped by a Co aloof position. As a result, this observed magneto-plasmonic functionality and tunability could be applicable in biomedicine, namely, cancer therapeutics.

annealing (metallurgy)↗

DOE OSTI2020

FeS colloids – formation and mobilization pathways in natural waters

For this study, we have used synchrotron-based X-ray absorption spectroscopy (structure of Fe–S clusters), transmission electron microscopy (solid-phase crystallinity), Fourier-transform ion-cyclotron-resonance mass spectrometry (identity and composition of natural organic carbon compounds), inductively coupled plasma optical emission spectrometry (total aqueous Fe), and the revised ferrozine method (aqueous Fe( II ) and Fe( III ) concentrations) to determine the stability and nature of colloids generated by sulfidation of ferrihydrite nanoparticles in the absence and presence of organic compounds. We observed that reductive dissolution of ferrihydrite by aqueous sulfide generates nm-scale FeS clusters. Their subsequent aggregation, which promotes settling of FeS aggregates into the solid fraction, was directly correlated with sulfide/Fe ratio. At sulfide/Fe ratios ≤0.5, FeS clusters and larger colloids remained in suspension for at least 14 days (and up to several months). At sulfide/Fe ratios >0.5, sulfidation reaction rates were rapid and FeS cluster aggregation was accelerated. Moreover, the presence of organic compounds increased the time of suspension of FeS colloids, whereas increased ionic strength inhibited the generation of FeS colloids. We present a general conceptual model to predict when and where FeS colloids can form and enhance or inhibit the mobility of contaminants and nutrients associated with them. Our study indicates that in lowsalinity fresh groundwater systems poor in sulfate (i.e. low sulfidation; lakes, floodplains, peatlands etc.), the ferrihydrite sulfidation reaction generates aqueous FeS clusters and larger colloids that remain suspended over long time periods, thus mobilizing a substantial fraction of the total aqueous Fe and S.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2020

Photonic integration for UV to IR applications

Photonic integration opens the potential to reduce size, power, and cost of applications normally relegated to table- and rack-sized systems. Today, a wide range of precision, high-end, ultra-sensitive, communication and computation, and measurement and scientific applications, including atomic clocks, quantum communications, processing, and high resolution spectroscopy, are ready to make the leap from the lab to the chip. However, many of these applications operate at wavelengths not accessible to the silicon on insulator-based silicon photonics integration platform due to absorption, power handling, unwanted nonlinearities, and other factors. Next generation photonic integration will require ultra-wideband photonic circuit platforms that scale from the ultraviolet to the infrared and that offer a rich set of linear and nonlinear circuit functions as well as low loss and high power handling capabilities. This article provides an assessment of the field in ultra-wideband photonic waveguides to bring power efficient, ultra-high performance systems to the chip-scale and enable compact transformative precision measurement, signal processing, computation, and communication techniques.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2020

Photoacoustic methane gas analyser based on a 3.3-μm optical parametric oscillator

We demonstrate a bench-scale prototype of a photoacoustic (PA) methane gas analyser that takes advantage of an optical parametric oscillator (OPO) based on a fan-out MgO : PPLN structure and resonant differential PA detector. The OPO emits in a repetitively pulsed mode (∼1750 Hz) at an idler wavelength of ∼3.3 μm with an average power of ∼40 – 50 mW. Using the prototype laser PA gas analyser, we experimentally demonstrate the feasibility of measuring the background methane concentration in air (∼2 – 3 ppm of CH{sub 4}). The threshold sensitivity of the PA gas analyser (1σ) is determined to be ∼ 49 ppb of CH{sub 4}. (paper)

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗