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All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

MOSAIC: An Effective FFT-based Numerical Method to Assess Aging Properties of Concrete

As the nuclear fleet in the United States ages and subsequent license renewal applications grow, the prediction of concrete durability at extended operation becomes more important. To address this issue, a Fast-Fourier Transform (FFT) method is utilized to simulate aging-related degradation of concrete within the Microstructure Oriented Scientific Analysis of Irradiated Concrete (MOSAIC) software. MOSAIC utilizes compositional phase maps to simulate damage from radiation-induced volumetric expansion (RIVE), applied force, creep, and thermal expansion. This compositional detail allows each mineral in the microstructure to be assigned specific material properties, allowing the simulation to be as accurate and representative as possible. The principal goal of MOSAIC is to simulate the effects of nonlinear aging mechanisms occurring in nuclear concrete on the macroscopic mechanical properties, using only the aggregate microstructure compositional information as a starting point. Here, several realistic example simulations are shown to demonstrate the utility and uniqueness of the MOSAIC software.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Revealing the Drag Instability in One-fluid Nonideal Magnetohydrodynamic Simulations of a 1D Isothermal C-shock

C-type shocks are believed to be ubiquitous in turbulent molecular clouds thanks to ambipolar diffusion. We investigate whether the drag instability in 1D isothermal C-shocks, inferred from the local linear theory of Gu & Chen, can appear in nonideal magnetohydrodynamic simulations. Two C-shock models (with narrow and broad steady-state shock widths) are considered to represent the typical environment of star-forming clouds. The ionization-recombination equilibrium is adopted for the one-fluid approach. In the 1D simulation, the inflow gas is continuously perturbed by a sinusoidal density fluctuation with a constant frequency. The perturbations clearly grow after entering the C-shock region until they start being damped at the transition to the post-shock region. We show that the profiles of a predominant Fourier mode extracted locally from the simulated growing perturbation match those of the growing mode derived from the linear analysis. Moreover, the local growth rate and wave frequency derived from the predominant mode generally agree with those from the linear theory. Therefore, we confirm the presence of the drag instability in simulated 1D isothermal C-shocks. We also explore the nonlinear behavior of the instability by imposing larger-amplitude perturbations to the simulation. We find that the drag instability is subject to wave steepening, leading to saturated perturbation growth. Issues concerning local analysis, nonlinear effects, one-fluid approach, and astrophysical applications are discussed.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS2019

An ALMA+ACA measurement of the shock in the Bullet Cluster

Context: The thermal Sunyaev-Zeldovich (SZ) effect presents a relatively new tool for characterizing galaxy cluster merger shocks, traditionally studied through X-ray observations. Widely regarded as the “textbook example” of a cluster merger bow shock, the western, most-prominent shock front in the Bullet Cluster (1E0657-56) represents the ideal test case for such an SZ study. Aims: We aim to characterize the shock properties using deep, high-resolution interferometric SZ effect observations in combination with priors from an independent X-ray analysis. Methods: Our analysis technique relies on the reconstruction of a parametric model for the SZ signal by directly and jointly fitting data from the Atacama Large Millimeter/submillimeter Array (ALMA) and Atacama Compact Array (ACA) in Fourier space. Results: The ALMA+ACA data are primarily sensitive to the electron pressure difference across the shock front. To estimate the shock Mach number M, this difference can be combined with the value for the upstream electron pressure derived from an independent Chandra X-ray analysis. In the case of instantaneous electron-ion temperature equilibration, we find M = 2.08 (+0.12,−0.12), in ≈ 2.4σ tension with the independent constraint from Chandra, M(X)= 2.74 ± 0.25. The assumption of purely adiabatic electron temperature change across the shock leads to M = 2.53 (+0.33,−0.25), in better agreement with the X-ray estimate M(X) = 2.57 ± 0.23 derived for the same heating scenario. Conclusion: We have demonstrated that interferometric observations of the thermal SZ effect provide constraints on the properties of the shock in the Bullet Cluster that are highly complementary to X-ray observations. The combination of X-ray and SZ data yields a powerful probe of the shock properties, capable of measuring M and addressing the question of electron-ion equilibration in cluster shocks. Our analysis is however limited by systematics related to the overall cluster geometry and the complexity of the post-shock gas distribution. To overcome these limitations, a simultaneous, joint-likelihood analysis of SZ and X-ray data is needed.

Luca Di Mascolo↗
NASA NTRS1974

Continuous Fourier transform system

Complex digital computer is not required, only summing amplifiers and attenuators are used for transformation of signal. Continuous transform system may be used for spectrum analysis, filtering, transfer function synthesis, and communications.

Munoz, R. M.↗
NASA NTRS2015

Mantle Water Contents Beneath the Rio Grande Rift (NM, USA): FTIR Analysis of Rio Puerco and Kilbourne Hole Peridotite Xenoliths

Peridotite xenoliths from the Rio Grande Rift (RGR) are being analyzed for H (sub 2) O contents by FTIR (Fourier Transform Infrared) as well as for major and trace element compositions. Nine samples are from the Rio Puerco Volcanic Field (RP) which overlaps the central RGR and southeastern Colorado Plateau; seventeen samples are from Kilbourne Hole (KH) in the southern RGR. Spinel Cr# (Cr/(Cr+Al)) (0.08-0.46) and olivine Mg# (Mg/(Mg plus Fe)) (0.883-0.911) of all RGR samples fall within the olivine-spinel mantle array from [1], an indicator that peridotites are residues of partial melting. Pyroxene H (sub 2) O in KH correlate with bulk rock and pyroxene Al (sub 2) O (sub 3).The KH clinopyroxene rare earth element (REE) variations fit models of 0-13 percent fractional melting of a primitive upper mantle. Most KH peridotites have bulk-rock light REE depleted patterns, but five are enriched in light REEs consistent with metasomatism. Variation in H (sub 2) O content is unrelated to REE enrichment. Metasomatism is seen in RP pyroxenite xenoliths [2] and will be examined in the peridotites studied here. Olivine H (sub 2) O contents are low (less than or equal to 15 parts per million), and decrease from core to rim within grains. This is likely due to H loss during xenolith transport by the host magma [3]. Diffusion models of H suggest that mantle H (sub 2) O contents are still preserved in cores of KH olivine, but not RP olivine. The average H (sub 2) O content of Colorado Plateau clinopyroxene (670 parts per million) [4] is approximately 300 parts per million higher than RGR clinopyroxene (350 parts per million). This upholds the hypothesis that hydration-induced lithospheric melting occurred during flat-slab subduction of the Farallon plate [5]. Numerical models indicate hydration via slab fluids is possible beneath the plateau, approximately 600 kilometers from the paleo-trench, but less likely approximately 850 kilometers away beneath the rift [6].

Schaffer, L. A.↗
NASA NTRS1993

On the stability analysis of approximate factorization methods for 3D Euler and Navier-Stokes equations

The convergence characteristics of various approximate factorizations for the 3D Euler and Navier-Stokes equations are examined using the von-Neumann stability analysis method. Three upwind-difference based factorizations and several central-difference based factorizations are considered for the Euler equations. In the upwind factorizations both the flux-vector splitting methods of Steger and Warming and van Leer are considered. Analysis of the Navier-Stokes equations is performed only on the Beam and Warming central-difference scheme. The range of CFL numbers over which each factorization is stable is presented for one-, two-, and three-dimensional flow. Also presented for each factorization is the CFL number at which the maximum eigenvalue is minimized, for all Fourier components, as well as for the high frequency range only. The latter is useful for predicting the effectiveness of multigrid procedures with these schemes as smoothers. Further, local mode analysis is performed to test the suitability of using a uniform flow field in the stability analysis. Some inconsistencies in the results from previous analyses are resolved.

Demuren, A. O.↗
DOE OSTI2023

Emulating the Deutsch-Josza algorithm with an inverse-designed terahertz gradient-index lens

An all-dielectric photonic metastructure is investigated for application as a quantum algorithm emulator (QAE) in the terahertz frequency regime; specifically, we show implementation of the Deustsh-Josza algorithm. The design for the QAE consists of a gradient-index (GRIN) lens as the Fourier transform subblock and patterned silicon as the oracle subblock. First, we detail optimization of the GRIN lens through numerical analysis. Then, we employed inverse design through a machine learning approach to further optimize the structural geometry. Through this optimization, we enhance the interaction of the incident light with the metamaterial via spectral improvements of the outgoing wave.

Blackwell, Ashley N.↗
NASA NTRS1980

Ground-state rotational constants of /C-13/H3D

Rotational constants for the vibrational ground state of (C-13)H3D, which has been detected in the atmospheres of Jupiter and Saturn, are reported. High-resolution spectra of monodeuteromethane were obtained in the region 1800 to 2500 kaysers by a vacuum Fourier interferometer, and the values of the rotational constants B0, D0J, D0JK, H0JJJ, H0JJK and H0JKK were calculated by an analysis of ground-state combination differences in the nu 2(A1) band. The calculated frequency and intensity of this transition are found to be in agreement with the observed values.

Chackerian, C., Jr.↗
NASA NTRS1981

Asymptotic form of the longitudinal correlation function for isotropic homogeneous turbulence

An asymptotic form is derived for the longitudinal correlation function for isotropic homogeneous turbulence in an incompressible fluid governed by the Navier-Stokes equation. The result is obtained from an analysis of the algebraic-differential structure of the two-point correlation tensor contained in the complex-valued Fourier transform of the probability measure over the turbulence ensemble, which reveals that the Hopf characteristic functional (the complex-valued Fourier transform of the probability measure) satisfies the Fourier interference inequality. Consequences of the expression obtained, in which the correlation function is a positive definite function of the inverse cube of the spatial coordinate as it approaches infinity, are shown to include the nonexistence of the Loitsianskii invariant, and the solution is shown to be consistent with empirical formulas.

Rosen, G.↗
NASA NTRS1987

Molecular line parameters for the atmospheric trace molecule spectroscopy experiment

During its first mission in 1985 onboard Spacelab 3, the ATMOS (atmospheric trace molecule spectroscopy) instrument, a high speed Fourier transform spectrometer, produced a large number of high resolution infrared solar absorption spectra recorded in the occultation mode. The analysis and interpretation of these data in terms of composition, chemistry, and dynamics of the earth's upper atmosphere required good knowledge of the molecular line parameters for those species giving rise to the absorptions in the atmospheric spectra. This paper describes the spectroscopic line parameter database compiled for the ATMOS experiment and referenced in other papers describing ATMOS results. With over 400,000 entries, the linelist catalogs parameters of 46 minor and trace species in the 1-10,000/cm region.

Brown, L. R.↗
NASA NTRS2007

Experimental Air-Broadened Line Parameters in the nu2 Band of CH3D

In this study we report the first experimental measurements of air-broadening and air-induced pressure-shift coefficients for approximately 378 transitions in the nu2 fundamental band of CH3D. These results were obtained from analysis of 17 room temperature laboratory absorption spectra recorded at 0.0056 cm(exp -1) resolution using the McMath-Pierce Fourier transform spectrometer located on Kitt Peak, Arizona. Three absorption cells with path lengths of 10.2, 25 and 150 cm were used to record the spectra. The total sample pressures ranged from 0.129x10(exp -2) to 52.855x10(exp -2) atm with CH3D volume mixing ratios of approximately 0.0109 in air. The spectra were analyzed using a multispectrum non-linear least-squares fitting technique. We report measurements for air pressure-broadening coefficients for transitions with quantum numbers as high as J" = 20 and K = 15, where K" = K' equivalent to K (for a parallel band). The measured air broadening coefficients range from 0.0205 to 0.0835 cm(exp -1) atm(exp -1) at 296 K. All the measured pressure-shift coefficients are negative and are found to vary from about -0.0005 to -0.0080 cm(exp -1) atm(exp -1) at the temperature of the spectra. We have examined the dependence of the measured broadening and shift parameters on the J" and K quantum numbers and also developed empirical expressions to describe the broadening coefficients in terms of m (m = -J", J" and J" + 1 in the (sup Q)P- (sup Q)Q-, and (sup Q)R-branch, respectively) and K. On average, the empirical expressions reproduce the measured broadening coefficients to within 4.4%.

Cross, Adriana Predoi↗
NASA NTRS2011

Effects of Hygrothermal Cycling on the Chemical, Thermal, and Mechanical Properties of 862/W Epoxy Resin

The hygrothermal aging characteristics of an epoxy resin were characterized over 1 year, which included 908 temperature and humidity cycles. The epoxy resin quickly showed evidence of aging through color change and increased brittleness. The influence of aging on the material s glass transition temperature (Tg) was evaluated by Differential Scanning Calorimetry (DSC) and Dynamic Mechanical Analysis (DMA). The Tg remained relatively constant throughout the year long cyclic aging profile. The chemical composition was monitored by Fourier Transform Infrared Spectroscopy (FTIR) where evidence of chemical aging and advancement of cure was noted. The tensile strength of the resin was tested as it aged. This property was severely affected by the aging process in the form of reduced ductility and embrittlement. Detailed chemical evaluation suggests many aging mechanisms are taking place during exposure to hygrothermal conditions. This paper details the influence of processes such as: advancement of cure, chemical degradation, and physical aging on the chemical and physical properties of the epoxy resin.

Miller, Sandi G.↗
NASA NTRS2015

Effects of Vehicle Weight and True Versus Indicated Airspeed on BVI Noise During Steady Descending Flight

Blade-vortex interaction noise measurements are analyzed for an AS350B helicopter operated at 7000 ft elevation above sea level. Blade-vortex interaction (BVI) noise from four, 6 degree descent conditions are investigated with descents flown at 80 knot true and indicated airspeed, as well as 4400 and 3915 pound take-off weights. BVI noise is extracted from the acquired acoustic signals by way of a previously developed time-frequency analysis technique. The BVI extraction technique is shown to provide a better localization of BVI noise, compared to the standard Fourier transform integration method. Using this technique, it was discovered that large changes in BVI noise amplitude occurred due to changes in vehicle gross weight. Changes in BVI noise amplitude were too large to be due solely to changes in the vortex strength caused by varying vehicle weight. Instead, it is suggested that vehicle weight modifies the tip-path-plane angle of attack, as well as induced inflow, resulting in large variations of BVI noise. It was also shown that defining flight conditions by true airspeed, rather than indicated airspeed, provides more consistent BVI noise signals.

Stephenson, James H.↗
NASA NTRS2018

Fire Induced Rock Spalls as Long-Term Traps for Ash

Severe fires accelerate rock weathering by spalling and exfoliation, creating abundant peels, flakes or spalls. In the following years, these spalls serve as physical traps which accommodate fine particles of dust, ash, organic matter, etc. We searched for traces of ash trapped under the spalls, after four major fires: 1989, 2005, 2010 and 2015 in Israel. Samples were collected beneath the spalls that formed on the rock outcrops, and in the immediate vicinity above and below them. Three laboratory analyses were performed: pH, EC and color. Five mineral/organic compounds were measured across the Mid-Infrared (MIR) spectral region at diffuse reflectance infrared Fourier transform mode: Hydroxylapatite (HAp), charcoal, organic carbon, montmorillonite and kaolinite. Several statistical analyses were performed: MANOVA, PCA and silhouette analysis on K-means clustering. The results show evidence of ash trapped under the spalls formed during the 2005 and 2010 fires, 6 to 11 years after the fires. Charcoal presence is evident, as well as increased amounts of HAp and organic carbon. In the exposed soil above or below the burned rock outcrop, these values are lower. Negligible amounts of ash were measured 27 years after the fire. In the 2015 burned outcrop, large amounts of charcoal were found above and below the outcrop, but not under the spalls. It seems that on the carbonate slopes of Israel and under Mediterranean climate, the time required for spalls to begin functioning as traps is longer than one rainy season, while ash traces are preserved in these traps for a period of two-three decades.

ash↗
NASA NTRS2018

Efficacy of FTIR Analysis in Determining CO2 Loading on Diglycolamine

In support of advanced air revitalization technologies to enable human spaceflight beyond low earth orbit, performance studies have been conducted using a liquid amine, Diglycolamine (DGA) between teams at NASA?s Johnson Spaceflight Center (JSC) and Ames Research Center (ARC). Liquid amines have been used in regenerable earth-based systems to remove CO2 from industrial systems as well as for closed-environment air revitalization because they can be regenerated at lower temperatures than solid sorbent systems. As an additional advantage to solid sorbent based systems, liquid sorbents can be cycled between an adsorbing contactor and degassing chamber, thereby reducing system complexity by operation in a continuous loop. In an effort to inform a regeneration system design for micro-gravity applications, ARC has performed a number of tests to characterize the degas mechanics of DGA. In order to accurately measure the amount of CO2 captured or released by the amine, methods such as gravimetric weighing and chemical decomposition are reasonable, however the initial design for a scaled down degas system required analysis on small sample sizes. In order to accomplish CO2 loading measurements with a sample size of approximately 500µL, Fourier-transform infrared spectroscopy (FTIR) was used. Calibration against acid decomposition showed relatively good correlation and test data showed reasonable adherence to expected trends, however more extensive testing should be conducted to fully validate the usage of FTIR to determine CO2 loading on DGA.

Diglycolamine↗
NASA NTRS1993

Effects of signal analysis parameters and noise removal on measured aircraft spectra

Special techniques must be applied when analyzing acoustic noise data from nonstationary sources such as aircraft flyover measurements. Since the Fourier transform is time dependent, the noise signal is divided into short time segments by introducing a window function so that the spectral characteristics remain reasonably stationary. Reducing the window width reduces the frequency resolution while increasing the window duration can lead to spectral smearing. A trade-off must be made between time resolution and frequency resolution. The effects of varying the window duration on narrow-band acoustic spectra and thus the frequency bin width are addressed in this study. The influence of window functions (rectangular, Hamming, etc.) are also investigated. Both a tonal noise source, XV-15 aircraft in the airplane mode, and a broadband noise source, a F-18 aircraft, are considered. When dealing with flight test data, not only is the signal nonstationary, often it is contaminated by both ambient background noise and internal noise generated by the data acquisition system and power generators. Since generator noise is highly tonal, this can be particularly troublesome when computing tone-corrected perceived noise level (PNLT). A scheme is presented in this paper to eliminate unwanted background and internal noise.

Kelly, Jeffrey J.↗