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All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Quantitative Determination of Electronic Effects in Free Radicals through Open-Shell Hammett Substituent Constants

Hammett substituent constants (σ), which quantify the electronic effects of functional groups, are widely used for predicting the properties of organic compounds and investigating reaction mechanisms. While these values have been obtained for a wide range of closed-shell substituents, measurements of analogous values for open-shell substituents are rare due to challenges associated with their short lifetimes. Here, in this report, we developed a combined experimental and computational approach for quantifying the electronic properties of open-shell substituents based on changes in nitrile vibrational frequencies (ν(C≡N)). By coupling pulse radiolysis and time-resolved infrared spectroscopy (PR-TRIR), we measured ν(C≡N) IR bands of 30 para - and meta -substituted benzonitriles bearing C-, N-, and S-centered radicals. A linear scaling relationship was obtained between these experimental values and values obtained from DFT calculations. Using these computed values, two different Hammett constants, σ m , and σ p + , were determined for a series of C-, N-, O-, S-, Si-, and B-centered radicals. The differences between σm and σp+ values enable the separate evaluation of inductive and resonance effects in these open-shell substituents. The results suggest that there are three classes of radicals: one is electron withdrawing (σ m , σ p + > 0), one is electron donating (σm, σp+ < 0), and one is inductively withdrawing but resonance donating (σ m > 0, σ p + < 0). Our study represents a general approach to the analysis of the electronic properties of open-shell species and has potential applications in a wide range of molecular processes involving free radical intermediates.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS2019

Highly Accurate Quartic Force Field and Rovibrational Spectroscopic Constants for the Azirinyl Cation (c-C2NH2+) and Its Isomers

Azirinyl cation is an aromatic cyclic molecule that is isoelectronic with cyclopropenylidene, c-C3H2, and c-C3H3+. Cyclopropenylidene has been shown to be ubiquitous, existing in many different astrophysical environments. Given the similar chemistry between C and N, and the relative abundances between C and N in astrophysical environments, it is expected that there should be aromatic ringed molecules that incorporate N in the ring, but as yet, no such molecule has been identified. To address this issue, the present study uses high levels of electronic structure theory to compute a highly accurate quartic force field (QFF) for azirinyl cation and its two lowest lying isomers, the cyanomethyl and isocyanomethyl cations. The theoretical approach uses the singles and doubles coupled-cluster method that includes a perturbative correction for connected triple excitations, CCSD(T), together with extrapolation to the one-particle basis set limit and corrections for scalar relativity and core-correlation. The QFF is then used in a second order vibrational perturbation theory analysis (VPT2) to compute the fundamental vibrational frequencies and rovibrational spectroscopic constants for all three C2NH2+ isomers. The reliability of the VPT2 vibrational frequencies is tested by comparison to vibrational configuration interaction (VCI) calculations and excellent agreement is found between the two approaches. Fundamental vibrational frequencies and rovibrational spectroscopic constants for all singly substituted 13C, 15N, and D isotopologues are also reported. It is expected that the highly accurate spectroscopic data reported herein will be useful in the identification of these cations in high resolution experimental or astronomical observations.

Partha P Bera↗
DOE OSTI2024

A comprehensive numerical investigation on spray models for Direct-Injection Spark-Ignition engines

Gasoline direct-injection spark-ignition (DISI) engines generate a large portion of their unburned hydrocarbon (UHC) and soot emissions during the cold-start phase. A predictive computational fluid dynamics (CFD) modeling framework can be used to understand the physical processes that characterize fuel spray evolution and fuel-film formation at cold start conditions, which can help to reduce engine-out particulate emissions. This study systematically evaluated spray submodels and developed a set of simulation best practices for physical-numerical submodels with the goal of enabling accurate simulations of liquid spray behavior in a DISI engine. Three comprehensive experimental datasets containing free-spray projected liquid volume (PLV), liquid volume fraction (LVF), and near-field X-ray radiography data were used to validate the simulation results and evaluate the spray submodels. Systematic analysis delved into injected parcel distribution, droplet collision, spray breakup, and evaporation via a detailed assessment of the relevant spray submodels. Moreover, the effects of turbulence models and the initial turbulent flow properties on the liquid spray evolution were examined. Based on extensive calibration efforts, a set of simulation best practices for the free spray was developed and validated against the PLV/LVF data. Simulation results indicated that the uniform distribution for parcel initialization, coupled with appropriate droplet collision submodels, provides an improved spray morphology compared to the cluster distribution. The findings also underscored the importance of calibrating the Kelvin-Helmholtz Rayleigh-Taylor (KH-RT) breakup model constants and droplet heat transfer coefficient scaling factor to achieve favorable agreement regarding measured liquid penetration and spray widths. In conclusion, this study marks a substantial stride towards accurately predicting fuel film evolution and soot formation within DISI engine performance.

ECN Spray G↗
DOE OSTI2024

Melting point of iron at high pressure: An assessment of uncertainties and effect of electronic temperature

An accurate calculation of the melting point of iron at various pressures in the Earth's core is important for understanding the core structure, geodynamo, and the Earth's history. Previous studies have assessed the melt line of iron at these extreme conditions using various experimental measurement techniques as well as both ab initio and classic molecular dynamics simulations. However, experimental measurements have uncertainties up to several hundred Kelvin, and inconsistencies remain among simulation results. Here in this work, we propose an iterative framework that couples density functional theory (DFT) calculations and molecular dynamics simulations performed using an ensemble of interatomic potentials to assess the effect of electronic temperature on the melting point. We systematically validate the potentials by comparing lattice constants and phonon dispersion curves at 0 K and enthalpy differences between liquid and HCP, FCC, BCC phases of iron close to the melt line at 300 GPa with DFT. Our results show that HCP iron melts at 6144 K (at 300 GPa), BCC phase is thermodynamically unstable, and FCC is metastable at this temperature. The melting points of FCC and BCC phases at 300 GPa are 5858 and 5647 K, respectively.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
NASA NTRS1999

Room Temperature Thin Film Ba(x)Sr(1-x)TiO3 Ku-Band Coupled MicrostripPhase Shifters: Effects of Film Thickness, Doping, Annealing and Substrate Choice

We report on measurements taken on over twenty Ku-band coupled microstrip phase shifters (CMPS) using thin ferroelectric films of Ba(x)Sr(1-x)TiO3. This CMPS design is a recent innovation designed to take advantage of the high tunability and tolerate the high dielectric constant of ferroelectric films at Ku- and K-band frequencies. These devices are envisioned as a component in low-cost steerable beam phased area antennas, Comparisons are made between devices with differing film thickness, annealed vs unannealed, Mn-doped vs. undoped, and also substrates of LaAlO3 and MgO. A comparison between the CMPS structure and a CPW phase shifter was also made oil the same ferroelectric film.

VanKeuls, F. W.↗
NASA NTRS2016

Architecture for Mitigating Short-Term Warning Cosmic Threats: READI Project

Earth is being constantly bombarded by a large variety of celestial bodies and has been since its formation 4.5 billion years ago. Among those bodies, mainly asteroids and comets, there are those that have the potential to create large scale destruction upon impact. The only extinction-level impact recorded to date was 65 million years ago, during the era of dinosaurs. The probability of another extinction-level, or even city-killer, impact may be negligible, but the consequences can be severe for the biosphere and for our species. Therefore it is highly imperative for us to be prepared for such a devastating impact in the near future, especially since humanity is at the threshold of wielding technologies that allow us to do so. Majority of scientists, engineers, and policymakers have focused on long-term strategies and warning periods for Earth orbit crossing Near-Earth Objects (NEOs), and have suggested methods and policies to tackle such problems. However, less attention has been paid to short warning period NEO threats. Such NEOs test current technological and international cooperation capabilities in protecting ourselves, and can create unpredictable devastation ranging from local to global scale. The most recent example is the Chelyabinsk incident in Russia. This event has provided a wakeup call for space agencies and governments around the world towards establishing a Planetary Defense Program. The Roadmap for EArth Defense Initiative (READI) is a project by a team of international, intercultural, and interdisciplinary participants of the International Space University's Space Studies Program 2015 hosted by Ohio University, Athens, OH proposing a roadmap for space agencies, governments, and the general public to tackle NEOs with a short warning before impact. Taking READI as a baseline, this paper presents a technical description of methodologies proposed for detection and impact mitigation of a medium-sized comet (up to 800m across) with a short-warning period of two years on a collision course with Earth. The hypothetical comet is on a highly-inclined orbit having a high probability for Earth impact after its perihelion. For detection, we propose a space-based infrared detection system consisting of two satellites located at the Earth-Moon Lagrange points L1 and L2 coupled with space observatories, like the James Webb telescope and the Centennial telescope. These telescopes are supported by ground-based telescopes, like the Arecibo and Green Bank telescope, in the search for NEOs. Upon detection, the comet is tracked constantly using space- and ground-based telescopes. The deflection system is two-pronged, firstly involving the use of a high energy Directed Energy Laser Terminals (DELT) placed at Sun-Earth Lagrange points L4 and L5 so as to initiate and increase the ablation rate of the comet and deviate it from its collision trajectory, and secondly by the Hypervelocity Comet Intercept Vehicle (HCIV), a space-borne system combining a kinetic impactor with a thermonuclear device. The policy and international collaboration aspects to implement these methods are also outlined in the paper. The techniques mentioned could also be applied to mitigate medium-to-large sized asteroids (up to 2km across).

Laser Applications↗
NASA NTRS2016

Planetary Defense Architecture for Mitigating Short-Term Warning Cosmic Threats: READI Project

Earth is being constantly bombarded by a large variety of celestial bodies and has been since its formation 4.5 billion years ago. Among those bodies, mainly asteroids and comets, there are those that have the potential to create large scale destruction upon impact. The only extinction-level impact recorded to date was 65 million years ago, during the era of dinosaurs. The probability of another extinction-level, or even city-killer, impact may be negligible, but the consequences can be severe for the biosphere and for our species. Therefore it is highly imperative for us to be prepared for such a devastating impact in the near future, especially since humanity is at the threshold of wielding technologies that allow us to do so. Majority of scientists, engineers, and policymakers have focused on long-term strategies and warning periods for Earth orbit crossing Near-Earth Objects (NEOs), and have suggested methods and policies to tackle such problems. However, less attention has been paid to short warning period NEO threats. Such NEOs test current technological and international cooperation capabilities in protecting ourselves, and can create unpredictable devastation ranging from local to global scale. The most recent example is the Chelyabinsk incident in Russia. This event has provided a wakeup call for space agencies and governments around the world towards establishing a Planetary Defense Program. The Roadmap for EArth Defense Initiative (READI) is a project by a team of international, intercultural, and interdisciplinary participants of the International Space University's Space Studies Program 2015 hosted by Ohio University, Athens, OH proposing a roadmap for space agencies, governments, and the general public to tackle NEOs with a short warning before impact. Taking READI as a baseline, this paper presents a technical description of methodologies proposed for detection and impact mitigation of a medium-sized comet (up to 800m across) with a short-warning period of two years on a collision course with Earth. The hypothetical comet is on a highly-inclined orbit having a high probability for Earth impact after its perihelion. For detection, we propose a space-based infrared detection system consisting of two satellites located at the Earth-Moon Lagrange points L1 and L2 coupled with space observatories, like the James Webb telescope and the Centennial telescope. These telescopes are supported by ground-based telescopes, like the Arecibo and Green Bank telescope, in the search for NEOs. Upon detection, the comet is tracked constantly using space- and ground-based telescopes. The deflection system is two-pronged, firstly involving the use of a high energy Directed Energy Laser Terminals (DELT) placed at Sun-Earth Lagrange points L4 and L5 so as to initiate and increase the ablation rate of the comet and deviate it from its collision trajectory, and secondly by the Hypervelocity Comet Intercept Vehicle (HCIV), a space-borne system combining a kinetic impactor with a thermonuclear device. The policy and international collaboration aspects to implement these methods are also outlined in the paper. The techniques mentioned could also be applied to mitigate medium-to-large sized asteroids (up to 2km across).

Laser Applications↗
DOE OSTI2026

Self-oscillating synchronematic colloids

Self-oscillators that sustain periodic dynamics under constant input are ubiquitous in natural and engineered systems, where their interactions enable spatiotemporal coordination among many individual units. New forms of organization can emerge when these self-oscillating units are free to move and rotate, coupling their spatial arrangement and alignment with their oscillation frequencies and phases. Here, we report experiments and simulations on populations of Quincke colloids that behave as self-oscillating units with position, orientation, frequency, and phase. Depending on the initial distribution, these active oscillators spontaneously organize into distinct collective states characterized by temporal synchronization and directional alignment, which we term synchronematic order. In fluid-like clusters, this order is short-ranged and decays over a length scale set by the competition between hydrodynamic interactions and athermal noise. In crystalline clusters, these interactions drive flobal synchronization and circular alignment-synchronematic crystals-whose collective frequency increases with cluster size due to non-reciprocal interactions. Our results establish self-oscillating colloids as a model system for active oscillatory matter and reveal fundamental principles by which synchronization, alignment, and structure co-emerge, offering new pathways for designing adaptive, frequency-tunable materials.

colloids↗
DOE OSTI2024

Acoustoelastic characterization of plates using zero group velocity Lamb modes

Acoustoelasticity, a characteristic of material anharmonicity, gives rise to a link between wave propagation velocity and the stress state in materials. Ultrasonic techniques to monitor this coupling, particularly with high sensitivity and in a noncontact manner, can have widespread application both in the quantification of applied and residual stress and in the characterization of nonlinear material behavior through measurement of higher order elastic constants. Here, we use a laser ultrasonic technique to excite and detect zero group velocity (ZGV) Lamb wave resonances in aluminum plates under uniaxial loading. A laser line source is used to excite these resonances at different orientations with respect to the applied load, and the signals are detected using an interferometer. The effects of stress and source orientation on ZGV resonance frequencies are validated using the theory of acoustoelastic Lamb wave propagation. In addition, a model-based inversion technique is used to extract Murnaghan's third-order elastic constants from measurements of the stress dependence of the first two ZGV modes generated parallel and perpendicular to the applied load. Laser generation and detection of ZGV resonances is shown to be an effective and powerful approach for the noncontact and nondestructive acoustoelastic characterization of elastic waveguides.

36 MATERIALS SCIENCE↗
DOE OSTI2024

Formation of the oxyl’s potential energy surface by the spectral kinetics of a vibrational mode

One of the most reactive intermediates for oxidative reactions is the oxyl radical, an electron-deficient oxygen atom. The discovery of a new vibration upon photoexcitation of the oxygen evolution catalysis detected the oxyl radical at the SrTiO3 surface. The vibration was assigned to a motion of the sub-surface oxygen underneath the titanium oxyl (Ti–O●−) created upon hole transfer to (or electron extraction from) a hydroxylated surface site. Evidence for such an interfacial mode is derived from its spectral shape, which exhibited a Fano resonance—a coupling of a sharp normal mode to continuum excitations. Here, this Fano resonance is utilized to derive precise formation kinetics of the oxyl radical and its associated potential energy surface (PES). From the Fano lineshape, the formation kinetics are obtained from the anti-resonance (the kinetics of the coupling factor), the resonance (the kinetics of the coupled continuum excitations), and the frequency integrated spectrum (the kinetics of the normal mode’s cross-section). All three perspectives yield logistic function growth with a half-rise of 2.3 ± 0.3 ps and a time constant of 0.48 ± 0.09 ps. A non-equilibrium transient associated with photoexcitation is separated from the rise of the equilibrated PES. The logistic function characterizes the oxyl coverage at the very initial stages (t ∼ 0) to have an exponential growth rate that quickly decreases toward zero as a limiting coverage is reached. Such time-dependent reaction kinetics identify a dynamic activation barrier associated with the formation of a PES and quantify it for oxyl radical coverage.

Chemistry↗
DOE OSTI2022

Phonon-induced rotation of the electronic nematic director in superconducting Bi 2 Se 3

The doped topological insulator A x Bi 2 Se 3 , with A = {Cu,Sr,Nb}, becomes a nematic superconductor below T c ≈ 3–4 K. The associated electronic nematic director is described by an angle α and is experimentally manifested in the elliptical shape of the in-plane critical magnetic field H c2 . Because of the threefold rotational symmetry of the lattice, α is expected to align with one of three high-symmetry directions corresponding to the in-plane nearest-neighbor bonds, consistent with a Z 3 -Potts nematic transition. Here, we show that the nematic coupling to the acoustic phonons, which makes the nematic correlation length tend to diverge along certain directions only, can fundamentally alter this phenomenology in trigonal lattices. Compared to hexagonal lattices, the former possesses a sixth independent elastic constant c14 due to the fact that the in-plane shear strain doublet (ε xx – ε yy , – 2ε xy ) and the out-of-plane shear strain doublet (2ε yz , – 2ε zx ) transform as the same irreducible representation. We find that, when c 14 overcomes a threshold value, which is expected to be the case in doped Bi 2 Se 3 , the nematic director α unlocks from the high-symmetry directions due to the competition between the quadratic phonon-mediated interaction and the cubic nematic anharmonicity. This implies the breaking of the residual in-plane twofold rotational symmetry (C 2x ), resulting in a triclinic phase. Furthermore, we discuss the implications of these findings for the structure of nematic domains, for the shape of the in-plane H c2 in A x Bi 2 Se 3 , and for the presence of nodes inside the superconducting state.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2024

Laser pulse-length dependent ablation and shock generation in silicon at 5 × 10 14 W/ cm 2 intensities

The effect of laser pulse duration on energy coupling into a planar silicon target is investigated in experiments at the OMEGA-EP facility by varying the laser pulse length τ —spanning 3 orders of magnitude from 100 ps to 10 ns—while maintaining a constant peak laser intensity, I 0 = 5 × 10 14 W/ cm 2 . In theoretical models, the ablation pressure primarily scales for a given material with laser intensity and wavelength, which are all fixed variables here, allowing us to explore the specific role of laser pulse duration. Two-dimensional radiation-hydrodynamics simulations benchmarked with optical probing of the expanding plasma show that the pulse duration is critical for the ablation pressure to reach a steady state. Moreover, the pulse duration impacts shock decay and multiple wave effects, which strongly dictate the evolving shock profile that propagates within the laser-shocked target as ultimately measured by rear-surface diagnostics. The shock velocities inferred from the theoretical model, after considering shock decay, impedance matching, and shock Hugoniot, are found to be in good agreement with velocimetry measurements. However, discrepancies are observed with simulations for the shorter (0.1 ns) and longer (10 ns) pulse durations, which are respectively attributed to unaccounted contributions of kinetic absorption mechanisms and instabilities in simulations. Published by the American Physical Society 2024

Bailly-Grandvaux, M. (ORCID:0000000175294013)↗
DOE OSTI2025

Temperature and Strain Sensing Characteristics of a 128° YX-Cut LiNbO 3 Rayleigh-Mode SAW Sensor From Room to Cryogenic Temperatures

Accurate, passive, and wireless monitoring of cryogenic hardware is essential for high-energy physics, space propulsion, and biomedical instrumentation. Here, this study quantifies the coupled temperature-strain behavior of Rayleigh-mode surface acoustic-wave (SAW) delay-line sensors fabricated on 128° YX-cut LiNbO 3 . A nonlinear finite element (FE) model incorporating Varshni-based elastic constants, higher-order thermal expansion, and temperature-dependent piezo- and dielectric coefficients was developed and validated experimentally between 280K and 80K. Free-standing (first test condition) and bonded/wired (second test condition) devices exhibited indistinguishable thermal responses; the average temperature coefficient of delay (TCD) in the critical cryogenic range from 130K down to 80K differed by only 0.15 ppm/K (0.32%), confirming that bonding-induced stress is negligible. Over 280-80K the measured TCD was 61.77 ppm/K, while the FE model predicted an equivalent temperature coefficient of frequency (TCF) of −62.74 ppm/K with an overall coefficient of determination R2 = 0.998. In the critical cryogenic interval 130-80K the TCD fell to 47.66 ppm/K, indicating improved thermal stability at low temperature. Controlled loading (0-300 με) revealed a strain coefficient of delay (SCD) that rises from 0.53 ± 0.02 ppm/με at 300K to 1.05 ± 0.02 ppm/με at 80K. This modest sensitivity confirms that, for temperature sensing, strain is a second-order perturbation above 135K but must be compensated at deeper cryogenic levels. Overall, this work establishes a predictive multiphysics model together with repeatable wired measurements that confirm the suitability of SAW sensors for temperature and strain monitoring in extreme cryogenic environments, while also providing a baseline for future wireless implementations.

25 ENERGY STORAGE↗
NASA NTRS1994

Multiwavelength study of the magnetically active T Tauri star HD 283447

We observed the luminous T Tauri star HD 283447 = V773 Tauri simultaneously at X-ray, ultraviolet, optical photometric and spectroscopic, and radio wavelengths for several hours on UT 1992 September 11. ROSAT, IUE, Very Large Array (VLA) and an intercontinental Very Long Baseline Interferometry (VLBI) network, and three optical observatories participated in the campaign. The star is known for its unusually high and variable nonthermal radio continuum emission. High levels of soft X-ray and Mg II line emission are discovered, with luminosity L(sub x) = 5.5 x 10(exp 30) ergs/s (0.2 - 2 keV) and L(sub Mg II) = 1 x 10(exp 29) ergs/s, respectively. Optically, the spectrum exhibits rather weak characteristics of `classical' T Tauri stars. A faint, broad emission line component, probably due to a collimated wind or infall, is present. During the campaign, the radio luminosity decreased by a factor of 4, while optical/UV lines and X-ray emission remained strong but constant. The large gyrosynchrotron-emitting regions are therefore decoupled from the chromospheric and coronal emission. Five models for the magnetic geometry around the star are discussed; solar-type activity, dipole magnetosphere, star-disk magnetic coupling, disk magnetic fields, and close binary interaction. The data suggest that two magnetic geometries are simultaneously present: complex multipolar fields like those on the Sun, and a large-scale field possibly associated with the circumstellar disk.

Feigelson, Eric D.↗
NASA NTRS2003

Combustion Of Moving Droplets And Of Droplets Suspended Within A Convective Environment: Transient Numerical Results

The problem considered is that of a single-component liquid fuel (n-heptane) droplet undergoing evaporation and combustion in a hot, convective, low pressure, zero-gravity environment of infinite expanse. For a moving droplet, the relative velocity (U(sub infinity)) between the droplet and freestream is subject to change due to the influence of the drag force on the droplet. For a suspended droplet, the relative velocity is kept constant. The governing equations for the gas-phase and the liquid-phase consist of the unsteady, axisymmetric equations of mass, momentum, species (gas-phase only) and energy conservation. Interfacial conservation equations are employed to couple the two phases. Variable properties are used in the gas- and liquid-phase. Multicomponent diffusion in the gas-phase is accounted for by solving the Stefan-Maxwell equations for the species diffusion velocities. A one-step overall reaction is used to model the combustion. The governing equations are discretized using the finite volume and SIMPLEC methods. A colocated grid is adopted. Hyperbolic tangent stretching functions are used to concentrate grid points near the fore and aft lines of symmetry and at the droplet surface in both the gas- and liquid-phase. The discretization equations are solved using the ADI method with the TDMA used on each line of the two alternating directions. Iterations are performed within each time-step until convergence is achieved. The grid spacing, size of the computational domain and time-step were tested to ensure that all solutions are independent of these parameters. A detailed discussion of the numerical model is given.

Gogos, George↗
NASA NTRS2005

Changes in the Temperature of Saturn's Stratosphere from 2002 to 2004 and Direct Evidence of a Mesopause

The state of a planetary stratosphere is intricately linked to the radiation it receives from its host star. The stellar flux impinging on the the planetary stratosphere affects the temperature and chemistry occurring there. The revolution of the planet about its orbit coupled to the planets axial tilt can cause variations in the amount of flux captured by the planet at a given latitude over the period of a year even if the flux output of the star is constant. This variation of stellar flux at a given latitude during the orbit of a planet is what causes seasons. Saturn, with its axial tilt of 27 degrees, experiences seasonal forcing much like the Earth, albeit with far less solar flux and a year equal to 30 Earth years. In an attempt to measure the effect seasonal forcing has on the temperature structure of Saturn's stratosphere, we have started a long term observing program. By observing Saturn with a high-resolution mid-infrared spectrograph in the v(sub 4) band of methane, we can infer the stratospheric temperature between the pressure levels of 10 and 0.01 mbar. We present latitudinally resolved observations of Saturn's southern hemisphere from 2002 and 2004. We have analyzed the data using a line-by-line radiative transfer model and inferred stratospheric temperatures and winds. We compare the temperatures from the two observing runs and the predictions of a stratospheric seasonal climate model. The zonal winds in the southern hemisphere, between the 10 and 0.01 mbar pressure levels, will be shown and discussed.

Greathouse, Thomas K.↗
NASA NTRS2011

Correlating CFD Simulation with Wind Tunnel Test for the Full-Scale UH-60A Airloads Rotor

Data from the recent UH-60A Airloads Test in the National Full-Scale Aerodynamics Complex 40- by 80- Foot Wind Tunnel at NASA Ames Research Center are presented and compared to predictions computed by a loosely coupled Computational Fluid Dynamics (CFD)/Comprehensive analysis. Primary calculations model the rotor in free-air, but initial calculations are presented including a model of the tunnel test section. The conditions studied include a speed sweep at constant lift up to an advance ratio of 0.4 and a thrust sweep at constant speed into deep stall. Predictions show reasonable agreement with measurement for integrated performance indicators such as power and propulsive but occasionally deviate significantly. Detailed analysis of sectional airloads reveals good correlation in overall trends for normal force and pitching moment but pitching moment mean often differs. Chord force is frequently plagued by mean shifts and an overprediction of drag on the advancing side. Locations of significant aerodynamic phenomena are predicted accurately although the magnitude of individual events is often missed.

Romandr, Ethan↗
NASA NTRS2016

Highlights from 4STAR Sky-Scanning Retrievals of Aerosol Intensive Optical Properties from Multiple Field Campaigns with Detailed Comparisons of SSA Reported During SEAC4RS

The 4STAR (Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research) instrument combines airborne sun tracking capabilities of the Ames Airborne Tracking Sun Photometer (AATS-14) with AERONET (Aerosol Robotic Network)-like sky-scanning capability and adds state-of-the-art fiber-coupled grating spectrometry to yield hyperspectral measurements of direct solar irradiance and angularly resolved sky radiance. The combination of sun-tracking and sky-scanning capability enables retrievals of wavelength-dependent aerosol optical depth (AOD), mode-resolved aerosol size distribution (SD), asphericity, and complex refractive index, and thus also the scattering phase function, asymmetry parameter, single-scattering albedo (SSA), and absorption aerosol optical thickness (AAOT). From 2012 to 2014 4STAR participated in four major field campaigns: the U.S. Dept. of Energy's TCAP (Two-Column Aerosol Project) I & II campaigns, and NASA's SEAC4RS (Studies of Emissions, Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys) and ARISE (Arctic Radiation - IceBridge Sea & Ice Experiment) campaigns. Establishing a strong performance record, 4STAR operated successfully on all flights conducted during each of these campaigns. Sky radiance spectra from scans in either constant azimuth (principal plane) or constant zenith angle (almucantar) were interspersed with direct beam measurements during level legs. During SEAC4RS and ARISE, 4STAR airborne measurements were augmented with flight-level albedo from the collocated Shortwave Spectral Flux Radiometer (SSFR) providing improved specification of below-aircraft radiative conditions for the retrieval. Calibrated radiances and retrieved products will be presented with particular emphasis on detailed comparisons of ambient SSA retrievals and measurements during SEAC4RS from 4STAR, AERONET, HSRL2 (High Spectral Resolution Lidar), and from in situ measurements.

Radiance↗