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DOE OSTI2021

Magnetoelastic standing waves induced in UO 2 by microsecond magnetic field pulses

Significance UO 2 is of particular interest due to its use as a nuclear fuel, its unusually poor thermal conductivity, and its uniquely strong magnetoelastic properties characterized by a linear coupling between strain and magnetization. We clearly observe mechanical standing waves and elastic resonances in a single crystal, induced by microsecond magnetic field pulses. The phase and amplitude of the mechanical resonances are modulated by the piezomagnetic switching behavior, offering a sensitive probe for otherwise hard to detect magnetic dynamics in UO 2 . We highlight the importance of magnetic domains in the attenuation of the mechanical resonances and the robustness of the antiferromagnetic state in UO 2 against externally applied magnetic fields to 150 T.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

DOE OSTI2022

237 Np Mössbauer Isomer Shifts: A Lesson About the Balance of Static and Dynamic Electron Correlation in Heavy Element Complexes

A large set of neptunium compounds with different oxidation states (III to VII) was assembled to study the Mössbauer isomer shift by wave function calculations and better understand covalency in f-elements complexes. The contact density approach was used to calculate the isomer shift using complete active space self-consistent field (CASSCF) multiconfiguration wave functions, as well as matrix product states [from Density Matrix Renormalization Group (DMRG) algorithms] for large active spaces. Dynamic correlation effects for the isomer shifts were treated via CASPT2 energy derivatives with respect to the nuclear radius. The CASSCF calculations appear to produce different orbital overlocalization errors for low and high Np oxidation states. For compounds with low Np oxidation numbers, the errors can be attributed to the overlocalization of the 5f orbitals. For the compounds with high Np oxidation numbers, the main errors arise from an overlocalization of ligand orbitals and concomitant to weak donation bonding. Attempts to mitigate the overlocalization errors with large active spaces using DMRG were only partially successful, showing that explicit treatment of dynamic correlation is necessary for accurate predictions of Mössbauer isomer shifts. The CASPT2 calculations perform very satisfactorily. For a subset of Np compounds, both static and dynamic correlation effects were substantial. Furthermore, a rational active space selection based on orbital entanglement diagrams proved beneficial for determining the optimal reference wave function.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2024

Chiral catalysis of nuclear fusion in molecules

At low energies, nuclear fusion is strongly affected by electron screening of the Coulomb repulsion among the fusing nuclei. It may thus be possible to catalyze nuclear fusion in molecules (i.e., to fuse specific nuclei in situ) through quantum control of electron wave functions in intense laser fields. The circularly polarized (chiral) laser field can effectively squeeze the electron wave functions, greatly enhancing the screening in the spatial region relevant for the fusion process. Here, we estimate the corresponding fusion probabilities, and find that the proposed chiral catalysis of nuclear fusion in molecules may be observable, potentially with important practical applications.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

NASA NTRS1984

Physical aspects of computing the flow of a viscous fluid

One of the main themes in fluid dynamics at present and in the future is going to be computational fluid dynamics with the primary focus on the determination of drag, flow separation, vortex flows, and unsteady flows. A computation of the flow of a viscous fluid requires an understanding and consideration of the physical aspects of the flow. This is done by identifying the flow regimes and the scales of fluid motion, and the sources of vorticity. Discussions of flow regimes deal with conditions of incompressibility, transitional and turbulent flows, Navier-Stokes and non-Navier-Stokes regimes, shock waves, and strain fields. Discussions of the scales of fluid motion consider transitional and turbulent flows, thin- and slender-shear layers, triple- and four-deck regions, viscous-inviscid interactions, shock waves, strain rates, and temporal scales. In addition, the significance and generation of vorticity are discussed. These physical aspects mainly guide computations of the flow of a viscous fluid.

Mehta, U. B.↗

NASA NTRS1985

Test particle modeling of wave-induced energetic electron precipitation

A test particle computer model of the precipitation of radiation belt electrons is extended to compute the dynamic energy spectrum of transient electron fluxes induced by short-duration VLF wave packets traveling along the geomagnetic field lines. The model is adapted to estimate the count rate and associated spectrum of precipitated electrons that would be observed by satellite-based particle detectors with given geometric factor and orientation with respect to the magnetic field. A constant-frequency wave pulse and a lightning-induced whistler wave packet are used as examples of the stimulating wave signals. The effects of asymmetry of particle mirror heights in the two hemispheres and the atmospheric backscatter of loss cone particles on the computed precipitated fluxes are discussed.

Chang, H. C.↗

NASA NTRS1991

Comparison of magnetosonic wave and water group ion energy densities at Comet Giacobini-Zinner

Measurements of the Comet Giacobini-Zinner (GZ) are presented to determine to what extent wave-particle scattering redistributed the initial pick-up energy of the ion population. Also examined is the difference between the ion thermal energy and the energy in the magnetic fields of the waves. In spite of uncertainty of about a factor of 2 noted in the pick-up and mass-loaded regions, it is shown that less than approximately 50 percent of the pick-up energy is converted into wave magnetic energy in the inbound pick-up region.

Staines, K.↗

NASA NTRS1993

Coupling between plate vibration and acoustic radiation

A detailed numerical investigation of the coupling between the vibration of a flexible plate and the acoustic radiation is performed. The nonlinear Euler equations are used to describe the acoustic fluid while the nonlinear plate equation is used to describe the plate vibration. Linear, nonlinear, and quasi-periodic or chaotic vibrations and the resultant acoustic radiation are analyzed. We find that for the linear plate response, acoustic coupling is negligible. However, for the nonlinear and chaotic responses, acoustic coupling has a significant effect on the vibration level as the loading increases. The radiated pressure from a plate undergoing nonlinear or chaotic vibrations is found to propagate nonlinearly into the far field. However, the nonlinearity due to wave propagation is much weaker than that due to the plate vibrations. As the acoustic wave propagates into the far field, the relative difference in level between the fundamental and its harmonics and subharmonics decreases with distance.

Frendi, Abdelkader↗

NASA NTRS1986

Intercomparison and calibration of wind and wave measurements at various frequencies

Radars are increasingly being used for determinations of the small-scale wave and turbulence fields of the atmosphere. It is important to understand as fully as possible the likely sources of error or bias in radar velocity determinations. This is especially true for the determination of wave and turbulence parameters which often rely on the measurement of first or second order deviations from the prevailing wind and therefore require better precision and time resolution than is usually required for measurements of the mean winds alone. The intercomparison of velocity measurements made with different techniques (e.g., radar and balloon) can be expected to help determine not only the relative effectiveness of the different methods, but also the degree of reliability.

Vincent, R. A.↗

NASA NTRS1989

Chromospheric-coronal coupling during solar flares: Current systems and particle acceleration

Two-dimensional (three velocity) electrostatic particle simulations are used to investigate the particle heating and acceleration associated with the impulsive phase of a solar flare. A crossfield current in the high corona (which is presumably driven by reconnection processes) is used to initiate the flare. Due to the differential motion of the electrons and ions, currents, and associated quasi-static electric fields are generated with the primary current and balancing return current being on adjacent field lines. These currents extend from the corona down into the chromosphere. Electrons can be accelerated to energies exceeding 100 keV on short time scales via the quasi-static fields and wave-particle interactions. The spectra of these electrons has a broken power-law distribution which hardens in time. The spatially separate primary and return currents are closed by the cross-field acceleration of the ambient ions into the primary current regions. These ions are then accelerated upwards into the corona by the same quasi-static electric field accelerating the electrons downwards. This acceleration can account for the broadened stationary and weak blue shifted component seen in soft x ray line emissions and enhancements in heavy ion abundances seen in the solar wind in associations with solar flares.

Winglee, Robert M.↗

NASA NTRS2001

Electromagnetic Ion Cyclotron Waves in the High Altitude Cusp: Polar Observations

High-resolution magnetic field data from the Polar Magnetic Field Experiment (MFE) show that narrow band waves at frequencies approximately 0.2 to 3 Hz are a permanent feature in the vicinity of the polar cusp. The waves have been found in the magnetosphere adjacent to the cusp (both poleward and equatorward of the cusp) and in the cusp itself. The occurrence of waves is coincident with depression of magnetic field strength associated with enhanced plasma density, indicating the entry of magnetosheath plasma into the cusp region. The wave frequencies are generally scaled by the local proton cyclotron frequency, and vary between 0.2 and 1.7 times local proton cyclotron frequency. This suggests that the waves are generated in the cusp region by the precipitating magnetosheath plasma. The properties of the waves are highly variable. The waves exhibit both lefthanded and right-handed polarization in the spacecraft frame. The propagation angles vary from nearly parallel to nearly perpendicular to the magnetic field. We find no correlation among wave frequency, propagation angle and polarization. Combined magnetic field and electric field data for the waves indicate that the energy flux of the waves is guided by the background magnetic field and points downward toward the ionosphere.

Le, Guan↗

NASA NTRS1999

FAST Observations of Acceleration Processes in the Cusp--Evidence for Parallel Electric Fields

The existence of precipitating keV ions in the Earth's cusp originating at the magnetosheath provide unique means to test our understanding of particle acceleration and parallel electric fields in the lower altitude acceleration region. On numerous occasions, the FAST (The Fast Auroral Snapshot) spacecraft has encountered the Earth's cusp regions near its apogee of 4175 km which are characterized by their signatures of dispersed keV ion injections. The FAST instruments also reveal a complex microphysics inherent to many, but not all, of the cusp regions encountered by the spacecraft, that include upgoing ion beams and conics, inverted-V electrons, upgoing electron beams, and spikey DC-coupled electric fields and plasma waves. Detailed inspection of the FAST data often show clear modulation of the precipitating magnetosheath ions that indicate that they are affected by local electric potentials. For example, the magnetosheath ion precipitation is sometimes abruptly shut off precisely in regions where downgoing localized inverted-V electrons are observed. Such observations support the existence of a localized process, such as parallel electric fields, above the spacecraft which accelerate the electrons downward and consequently impede the precipitating ion precipitation. Other acceleration events in the cusp are sometimes organized with an apparent cellular structure that suggests Alfven waves or other large-scale phenomena are controlling the localized potentials. We examine several cusp encounters by the FAST satellite where the modulation of energetic session on acceleration particle populations reveals evidence of localized acceleration, most likely by parallel electric fields.

Pfaff, R. F.. Jr.↗

NASA NTRS1973

Angular magnetic field beam improves efficiency in klystrons and traveling wave tubes

Special lens shaping allows variation of focusing strength with radius. Lens can be either converging or diverging depending on charge of particles and direction of angular magnetic field. There is potential use for lens in particle analyzers, electron beam welding systems, microwave tube refocusing systems, and possible display type devices.

Neugebauer, W.↗

NASA NTRS1971

Five-minute oscillations in the solar magnetic field.

Evidence for the existence of 5 min oscillations in the photospheric and low chromospheric magnetic fields is presented, their properties discussed, and a possible production mechanism suggested. It is pointed out that, because the solar magnetic field is frozen into the oscillating plasma, there are several ways in which the oscillations in the plasma (which are observed as velocity oscillations) could be transferred to the magnetic field. It is shown schematically how vertical waves could cause oscillations in a horizontal magnetic field, and how horizontal waves could cause oscillations in a vertical magnetic field.

Tanenbaum, A. S.↗

NASA NTRS1990

A laboratory study of the electromagnetic bias of rough surface scattering by water waves

The design, development, and use of a focused-beam radar to measure the electromagnetic bias introduced by the scattering of radar waves by a roughened water surface are discussed. The bias measurements were made over wide ranges of environmental conditions in a wavetank laboratory. Wave-elevation data were provided by standard laboratory capacitance probes. Backscattered radar power measurements coincident in time and space with the elevation data were produced by the radar. The two data sets are histogrammed to produce probability density functions for elevation and radar reflectivity, from which the electromagnetic bias is computed. The experimental results demonstrate that the electromagnetic bias is quite variable over the wide range of environmental conditions that can be produced in the laboratory. The data suggest that the bias is dependent upon the local wind field and on the amplitude and frequency of any background wave field that is present.

Parsons, Chester L.↗

NASA NTRS1978

Radiative shock dynamics. II - Hydrogen continua

The interaction between radiation and a shock wave propagating through a stellar atmosphere is investigated. Departures from local thermodynamic equilibrium (LTE) are permitted in the first two levels of a 10-level hydrogen atom; levels 3-10 are in LTE. A piston moving at constant velocity into the bottom of the atmosphere drives a shock wave. This shock produces precursor radiation that diffuses through the gas well ahead of the shock and causes a mild luminosity flash in the emergent Balmer and free-free radiation when it reaches the surface. The precursor wave deposits a large amount of radiative energy in the outer layers of the atmosphere, initiating a radiation-induced pressure wave. The process of energy transfer from the radiation field to the compression wave is similar to the Eddington valve mechanism which drives stellar pulsations. Material is accelerated outward by the radiation-induced wave; eventually it free-falls inward, hits the quasistationary atmosphere, and forms an accretion shock. The piston driven shock is weakened by radiative energy losses. When it reaches the surface, the shock is invisible in the continuum radiation.

Klein, R. I.↗

NASA NTRS1984

ISEE-3 wave measurements in the distant geomagnetic tail and boundary layer

The ISEE-3 excursion into the distant tail region reveals a complex structure with several wave, particle and field characteristics that differ significantly from those measured closer to earth. The most striking results are found within the distant boundary layer where intense electrostatic turbulence levels are detected in association with bidirectional electron distributions. The wave amplitudes appear to increase with increasing downstream distance and the polarizations are those expected for ion acoustic oscillations. Near the boundary of the distant plasmas sheet the turbulence spectra are essentially identical to those measured much closer to earth on IMP-8. It is also found that in the distant tail the continuum radiation spectrum has a low frequency cutoff that is much higher than the minimum value for the local plasma frequency.

Scarf, F. L.↗

NASA NTRS1986

Electron acceleration via kinetic Alfven waves

Obliquely propagating shear Alfven waves are effected by kinetic effects. The polarization and dispersion of these waves are discussed and it is shown that electrons can be effectively accelerated along field lines by these waves. Several nonlinear effects such as solitary waves, nonlinear damping due to current-driven instabilities, and anomalous resistivity are also discussed. Recent observations of electric and magnetic field perturbations on auroral field lines which seem to be related to these waves are described. However, the evidence for the existence of these kinetic Alfven waves is not firm.

Goertz, C. K.↗

NASA NTRS1994

Whistler mode waves in the Jovian magnetosheath

During the Ulysses flyby of Jupiter in February 1992, the spacecraft traversed the Jovian magnetosheath for a few hours during the inbound pass and for aa few days during the outbound pass. Burstlike electomagnetic waves at frequencies of approximately 0.1-0.4 of the local electron cyclotron frequency have been observed by the Unified Radio and Plasma Wave (URAP) experiement. The waves were more often observed in the regions which were probably the outer or the middle magnetosheath, especially near the bow shock, and rarely seen in the magnetosphere/magnetosheath boundary layer. The propagation angles of the waves are estimated by comparing the measurements of the wave electric and magnetic fields in the spacecraft spin plane with the corresponding values calculated using the cold plasma dispersion relation under local field and plasma conditions. It is found that the waves propagate obliquely with wave angles between approximately 30 deg and 50 deg. These waves are likely to be the whistler mode waves which are excited by suprathermal electrons with a few hundred eV and a slight anisotropy (T(sub perp)/T(sub parallel) approximately 1.1-1.5). They are probably similar in nature to the lion roars observed in the Earth's magnetosheath. Signature of coupling between the mirror and the whistler mode have also been observed. The plasma conditions which favor the excitation of the whistler mode instability during the wave events exists as observed by the plasma experiement of Ulysses.

Lin, Naiguo↗