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At least 991 records · Page 55

2018 Long-Term Hydrologic Monitoring Program Report for Rio Blanco, Colorado, Site

This report presents the monitoring data collected by the U.S. Department of Energy (DOE) Office of Legacy Management (LM) at the Rio Blanco, Colorado, Site (Figure 1). The Rio Blanco site was the location of an underground nuclear test during which three nuclear devices were detonated nearly simultaneously in a single borehole in 1973. The test resulted in residual radionuclide contamination at the detonation depths of 5840, 6230, and 6690 feet (ft) (DOE 2015). Monitoring includes the collection of samples from groundwater wells and surface water locations near the site to assess for any potential impacts that may be attributed to the Rio Blanco nuclear test. This report summarizes the laboratory analytical results obtained from the sampling event conducted in 2018. This annual report and previous reports are available on the LM public website at https://www.lm.doe.gov/rio_blanco/Sites.aspx. Data collected during this and previous monitoring events are available on the Geospatial Environmental Mapping System (GEMS) website at https://gems.lm.doe.gov/#site=RBL.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Engineered Barrier System Research Activities at LBNL (FY2020 Progress Report)

The design of a radioactive waste repository typically involves a multi-barrier system, including the natural barrier system (NBS), i.e., the host rock and its surrounding subsurface environment, and an engineered barrier system (EBS). The EBS is to be constructed from the man-made, engineered materials placed within a repository. The repository includes the waste form, waste canisters, buffer materials, backfill, and seals. The most common buffer material for EBS is compacted bentonite, which features low permeability and high retardation of radionuclides. Extensive studies concerning the behavior of bentonite backfill in crystalline and argillite/shale geologic environments for nuclear waste disposal have been conducted by means of laboratory experiments, numerical modeling, and large-scale in situ tests in Underground Research Laboratories (URLs) in Switzerland, France, Belgium, and Japan. This report includes the results of LBNL’s research activities conducted according to the objectives and scope of the work packages “SF-20LB01030802 Engineered Barrier System R&D - LBNL” and “SF-20LB01030806 Engineered Barrier System International Collaborations - LBNL” of the Spent Fuel and Waste Science and Technology (SFWST) (formerly called Used Fuel Disposal) Campaign of the Department of Energy’s (DOE) Office of Nuclear Energy. LBNL research studies included laboratory scale tests and modeling of the evolution of the EBS bentonite and associated coupled processes, and impacts of high temperature on parameters and processes relevant to the performance of crystalline and argillite repositories, including the evaluation of the technical basis for applying the maximum allowable temperature. The results of these studies are being addressing the technical elements necessary to evaluate the EBS design concepts. Emphasis is on the study of thermal, mechanical, and chemical processes that influence the performance of EBS, and the development of modeling capability for reliable assessment of these processes, and ultimately supporting the development of the GDSA model with detailed coupled THMC process models.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Applying Waveform Correlation to Mining Blasts Using a Global Sparse Network

Agencies that monitor for underground nuclear tests are interested in techniques that automatically characterize mining blasts to reduce the human analyst effort required to produce high-quality event bulletins. Waveform correlation is effective in finding similar waveforms from repeating seismic events, including mining blasts. We report the results of an experiment that uses waveform templates recorded by multiple International Monitoring System stations of the Preparatory Commission for the Comprehensive Nuclear-Test-Ban Treaty Organization for up to 10 years prior to the time period of interest to detect and identify mining blasts that occur during single weeks of study. We discuss approaches for template selection, threshold setting, and event detection that are specialized for mining blasts and a sparse, global network. We apply the approaches to two different weeks of study for each of two geographic regions, Wyoming and Scandinavia, to evaluate the potential for establishing a set of standards for waveform correlation processing of mining blasts that can be effective for operational monitoring systems with a sparse network. We compare candidate events detected with our processing methods to the Reviewed Event Bulletin of the International Data Centre to develop an intuition about potential reduction in analyst workload.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

Charge response and energy calibration of ProtoDUNE-

ProtoDUNE-SP is a test bed liquid argon time projection chamber (LArTPC) for the far detector of the Deep Underground Neutrino Experiment (DUNE). This LArTPC was calibrated using cosmic-ray cathode-crossing muons, electric field maps, and purity-monitor data to correct for nonuniformities in the detector response and cosmic-ray stopping muons to perform the absolute energy scale calibration for further physics analysis.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

2020 LANL Contributions to the BATS Test in WIPP

The DOE Office of Nuclear Energy (DOE-NE) repository research and development program seeks to provide a sound technical basis for multiple viable disposal options, increase confidence in the robustness of generic disposal concepts, and develop science and engineering tools needed to support disposal concept implementation. Sandia, Los Alamos, and Lawrence Berkeley National labs are conducting research into salt, which includes the Brine Availability Test in Salt (BATS) field test at the Waste Isolation Pilot Plant (WIPP), a DOE Office of Environmental Management facility. BATS is leveraging the existing infrastructure associated with the WIPP to advance science informing generic disposal concepts. BATS is an ongoing heated borehole experiment being conducted in the WIPP underground. The goal of this experiment is to reduce the uncertainty associated with spent nuclear fuel disposition in geologic salt formations. The BATS experiments is designed to accomplish this by increasing our understanding of brine migration in salt, assessing damaged zones from mining and drilling, simulating a post-closure environment, confirming salt properties, and providing data for model validation. Phased testing for generic salt repository R&D was proposed in 2015. Subsequently, borehole thermal testing was developed as a first step in this process. This document summarizes the work conducted on the BATS experiment during fiscal year 2020 with an emphasis on the contributions by Los Alamos National Lab.

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FIU Project1: Chemical Process Alternatives for Radioactive Waste [Slides]

"The U.S. DOE Hanford Site has the largest number of high-level waste (HLW) storage tanks and the largest volume of HLW in the United States. The safe storage, retrieval, treatment, and disposal of approximately 53 million gallons of highly toxic, high-level radioactive waste stored in Hanford’s 177 underground tanks are a national priority. Retrieval and treatment of waste from these tanks pose a considerable challenge. Florida International University has been conducting research on several promising alternative processes and technologies that can be applied to address several technology gaps in the current waste retrieval and conditioning plans. Specifically, FIU has been involved in: the evaluation of non-metallic materials in the waste transfer system, evaluation of alternative HLW instrumentation for in-tank applications and the development of technologies to assist in the inspection of tank bottoms at Hanford."

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Continuous Laboratory-Scale Melter Runs for System Evaluation

The Waste Treatment and Immobilization Plant (WTP) will process and stabilize waste that is stored in underground tanks on the Hanford Site. Currently, the first phase of the planned WTP startup and operation, called Direct Feed Low-Activity Waste (DFLAW), involves directly feeding only the liquid portion of the waste to electric melters in the WTP Low-Activity Waste (LAW) Vitrification Facility without full pretreatment. A second portion of the tank waste, called high-level waste (HLW), is set to contain most of the radioactivity inventory.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Imagery Applications for Advanced Event Analytics (WBS 24.3.1.3.3-IDC FY202 Final Project Report)

Accurate event locations and replicability of location analyses are essential for assessing the nature of an event, its context, ambient site conditions, and proximity to relevant facilities and infrastructure. Additionally, accurate event locations provide valuable information that reduce uncertainties, improve confidence in event analyses, and inform in-field verification activities. However, event location/relocation and replicability are difficult due to a number of factors, including spatially-sparse network coverage in some areas of the globe and variability in seismic data processing. This team proposed that the incorporation of high-fidelity imagery as a data backbone to the analytical assessment of a suspected underground explosion and/or an advanced seismic event bulletin produced by the International Data Centre (IDC) of the Preparatory Commission for the Comprehensive Nuclear-Test-Ban Treaty Organization (CTBTO PrepCom) could reduce uncertainties and improve confidence in analyses. Specifically, temporally-separated images can reduce uncertainty by identifying areas where change has occurred (e.g., building construction or demolition, road or facilities improvements). The primary goal of this project was to develop an automated geospatial processing script for imagery change detection to better reflect needs of the technical community (including the IDC) and to make the use of such a tool accessible in a variety of settings across platforms. Technical experts at Los Alamos National Laboratory successfully built GAIA: the Geospatial Automated Imagery Analysis tool, to fill this need. GAIA combines five tool components to produce orthorectified time separated imagery and imagery change detection maps. Our toolkit (1) reduces error by providing a standardized workflow for image analyses and (2) significantly reduces processing time from between 7 and 24+ hours to approximately 5 minutes. Technical experts at Sandia National Laboratories supported GAIA via beta-testing and by introducing a web-based system approach for increased applicability. To test the function, performance, broad application, and ease-of-use of GAIA, we applied it to four separate test cases. The results of this preliminary investigation show promise in reducing uncertainty in seismic event locations: if satellite imagery can show regions where operations that produce seismic activity likely occurred, then pursuing imagery to locate epicenters of seismic nuclear events could reduce the time needed to find the true epicenter location.

58 GEOSCIENCES↗

Inverting infrasound data for the seismoacoustic source time functions and surface spall at the Source Physics Experiments Phase II: Dry Alluvium Geology

This report presents the infrasound data recorded as part of the Source Physics Experiment - Phase 2, Dry Alluvium Geology. This experiment, also known colloquially as DAG, consisted of four underground chemical explosions at the Nevada National Security Site. We focus our analysis on only the fourth explosion (DAG-4) as we determined that this was the only event that produced clear source-generated infrasound energy as recorded by the DAG sensors. We analyze the data using two inversion methods. The first method is designed to estimate the point-source seismoacoustic source time functions, and the second inversion method is designed to estimate the first-order characteristics (e.g. horizontal dimensions and maximum amplitude) of the actual spall surface. For both analysis methods, we are able to fit the data reasonably well, with various assumptions of the source model. The estimated seismoacoustic source appears to be a combination of a buried, isotropic explosion with a maximum amplitude of ~2 x 10 9 Nm and a vertically oriented force, applied to the Earth's surface with a maximum amplitude of 4 x 10 7 N. We use the vertically oriented force to simulate surface spall. The estimated spall surface has an approximate radius of ~40 m with a maximum acceleration magnitude in the range of 0.8 to 1.5 m/s/s. These estimates are approximately similar to the measured surface acceleration at the site.

58 GEOSCIENCES↗

Radionuclide Screening Analysis and Transport Parameters for Pahute Mesa Detonations, Nevada National Security Site

A “screening analysis” is implemented at Pahute Mesa (PM), Nevada National Security Site (NNSS), to determine subsets of the 43 radionuclides listed in the radionuclide inventory of Finnegan et al. (2016) that are of relevance or potential relevance to the hydrologic source term (HST) for assessment of radionuclide transport in groundwater. Consideration is added to how levels of contamination are defined and whether any other radionuclides not in the inventory are relevant to the HST. A model is developed to estimate a range of possible source concentrations in groundwater that account for uncertainty in partitioning into melt glass and sorption into surrounding rock of the exchange zone for the 82 PM underground nuclear tests detonated in vertical shafts. The model also accounts for the varied hydrogeochemical settings. Transport parameters needed for the screening model calculations are developed from databases for hydrogeologic units, chemistry, mineralogy, fracture spacing, fracture aperture, fracture openness, matrix porosity, bulk density, saturation, and alteration. Of key importance is consideration of diagenetic zonation of the mineralogy related to hydrothermal alteration. The screening analysis compares model results with available groundwater radiochemistry data. Consistency between screening model results and available data helps validate the model for application to all 43 radionuclides, most of which have no measurements or only non-detect measurements of concentration in groundwater. The screening analysis determines that ten radionuclides – tritium, Sr-90, I-129, Cs-137, U-232, U-233, U-234, U-238, and the total of Pu-239 and Pu-240 are relevant to the HST. Determination of relevance is primarily based on data and/or model results indicating source concentration exceeding a maximum contaminant level (MCL) out to 100 years since the time of detonation. U-238 is relevant to assessment of contamination relative to MCLs for uranium and gross alpha particle activity. Five other radionuclides – C-14, Cl-36, Tc-99, Np-237, and Pu-238 – are determined potentially relevant to the HST based on a 0.1 MCL threshold. The screening analysis recommends additional attention to the natural daughter radionuclides of the uranium series (U-238) and thorium series (Th-232) decay chains, particularly Ra-226 and Ra-228, that were not included the inventory.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

Updating Hadron Production Models to Better Predict Neutrino Flux for DUNE

The Deep Underground Neutrino Experiment (DUNE) is an ongoing project at Fermilab with international collaboration and over 190 institutions involved. DUNE has three primary science goals, one of which is searching for the origin of the imbalance of matter and antimatter in the universe. Accomplishing this goal will require the study of neutrinos and the phenomenon of neutrino oscillation.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Imagery Applications for Advanced Event Analytics (WBS 24.3.1.3.3-IDC FY2020 Final Project Report)

Accurate event locations and replicability of location analyses are essential for assessing the nature of an event, its context, ambient site conditions, and proximity to relevant facilities and infrastructure. Additionally, accurate event locations provide valuable information that reduce uncertainties, improve confidence in event analyses, and inform in-field verification activities. However, event location/relocation and replicability are difficult due to a number of factors, including spatially-sparse network coverage in some areas of the globe and variability in seismic data processing. This team proposed that the incorporation of high-fidelity imagery as a data backbone to the analytical assessment of a suspected underground explosion and/or an advanced seismic event bulletin produced by the International Data Centre (IDC) of the Preparatory Commission for the Comprehensive Nuclear-Test-Ban Treaty Organization (CTBTO PrepCom) could reduce uncertainties and improve confidence in analyses. Specifically, temporally-separated images can reduce uncertainty by identifying areas where change has occurred (e.g., building construction or demolition, road or facilities improvements). The primary goal of this project was to develop an automated geospatial processing script for imagery change detection to better reflect needs of the technical community (including the IDC) and to make the use of such a tool accessible in a variety of settings across platforms. Technical experts at Los Alamos National Laboratory successfully built GAIA: the Geospatial Automated Imagery Analysis tool, to fill this need. GAIA combines five tool components to produce orthorectified time-separated imagery and imagery change detection maps. Our toolkit (1) reduces error by providing a standardized workflow for image analyses and (2) significantly reduces processing time from between 7 and 24+ hours to approximately 5 minutes. Technical experts at Sandia National Laboratories supported GAIA via beta-testing and by introducing a web-based system approach for increased applicability. To test the function, performance, broad application, and ease-of-use of GAIA, we applied it to four separate test cases. The results of this preliminary investigation show promise in reducing uncertainty in seismic event locations: if satellite imagery can show regions where operations that produce seismic activity likely occurred, then pursuing imagery to locate epicenters of seismic nuclear events could reduce the time needed to find the true epicenter location.

58 GEOSCIENCES↗

UNESE Data Analysis - Disko Elm Gas Transport Characteristics (NA-22 Quarterly Report)

Two research papers describing gas transport studies in subsurface containment environments appropriate for underground nuclear explosions were revised and accepted for publication in the peer-reviewed journals, Nature – Scientific Reports and Journal of Geophysical Research. The Nature – Scientific Reports paper is a primary deliverable and describes the gas-transport experiment performed in P Tunnel (NNSS) and 1) subsequent analysis of field data as part of the UNESE program. The Journal of Geophysical Research paper describes an experiment, supported mainly by DARPA and led by researchers at Weston Geophysical and New Mexico Tech., with 2) analyses supported by this project to evaluate the ability of SF6 gas tracer to track xenon gas migration under conditions related to a previous UNESE experiment. Two new tasks consider 3) evaluation of detonation heating and multiphase flow on arrival of xenon at the surface and 4) the impact of surface or Langmuir adsorption of gases being transported through pores and along fractures.

58 GEOSCIENCES↗

Exploratory Efforts to Constrain Geologic Material Properties from Remote Sensing Data: Joint Study (FY2020 Final Report)

Identification and characterization of underground events from surface or remote data requires a thorough understanding of the rock material properties. However, material properties usually come from borehole data, which is expensive and not always available. A potential alternative is to use topographic characteristics to approximate the strength, but this has never been done before quantitatively. Here we present the results from the first steps towards this goal. We have found that there are strong correlations between compressive and tensile strengths and slopes, but these correlations vary depending on data analysis details. Rugosity may be better correlated to strength than slope values. More comprehensive analyses are needed to fully understand the best method of predicting strength from topography for this area. We also found that misalignment of multiple GIS datasets can have a large influence on the ability to make interpretations. Lastly, these results will require further study in a variety of climatic conditions before being applicable to other sites.

58 GEOSCIENCES↗

Summary Report for the NEPA Impact Analysis. Revision 1

The Waste Isolation Pilot Plant (WIPP), located in southeastern New Mexico, has been developed by the U.S. Department of Energy (DOE) for the geologic (deep underground) disposal of defense-related transuranic (TRU) waste. Containment of TRU waste at the WIPP facility is derived from standards set forth in Title 40 of the Code of Federal Regulations (CFR), Part 191. The DOE assesses compliance with the containment standards according to the Certification Criteria in Title 40 CFR Part 194 by means of Performance Assessment (PA) calculations performed by Sandia National Laboratories (SNL). WIPP PA calculations estimate the probability of radionuclide releases from the repository to the accessible environment for a regulatory period of 10,000 years after facility closure. The DOE Carlsbad Field Office (CBFO) has initiated a National Environmental Policy Act (NEPA) action for a proposal to excavate and use additional transuranic (TRU) waste disposal panels at the WIPP facility. This report documents an analysis undertaken as part of an effort to evaluate the potential environmental consequences of the proposed action. Although not explicitly required for a NEPA analysis, evaluations of a dose indicator to hypothetical members of the public after final facility closure are presented in this report. The analysis is carried out in two stages: first, Performance Assessment (PA) calculations quantify the potential releases to the accessible environment over a 10,000-year post-closure period. Second, dose was evaluated for three hypothetical exposure pathways using the conservative radionuclide concentrations assumed to be released to the accessible environment.

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Site 200 - Building 225 Construction Project: Steel Pipe Abandonment Work Plan (October 2020)

In December 2019, a capped, 4-inch diameter pipe located inside a square concrete collar was discovered on the north side of a driveway leading into a construction project located at the northeast corner of First Street and Avenue and petroleum like odors were reported to Lawrence Livermore National Laboratory's (LLNL) Environment, Safety and Health (ES&H) staff. The pipe was also found to contain liquid, which was sampled. Analysis of the liquid showed the presence of refined petroleum hydrocarbons - primarily benzene, toluene, ethylbenzene and total xylenes, and lead. Based on various historical documents and maps, the pipe is assumed to be associated with one, or more of four 25,000-gallon, single-wall, concrete-construction, underground storage tanks (USTs) installed by the U.S. Department of Navy in approximately 1943. The USTs were reported to have been closed - abandoned in place and filled with sand in 1950.

54 ENVIRONMENTAL SCIENCES↗