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At least 991 records · Page 55

High quality AlSb for radiation detection

Provided is a method of making a radiation detector, including: growing a thin film on a substrate. The substrate is a silicon substrate. The thin film includes aluminum antimony alloy (AlSb). The growing is epitaxial growth via ultra-high vacuum molecular beam epitaxy (UHV-MBE).

Balakrishnan, Ganesh↗

Influence of dissolved salts and impurities on seawater on heat transfer and fluid flow through fuel channels and debris bed

This project aims to better understand this mechanism and its effect on heat transfer. Specifically, experimental research was conducted to investigate the long term coolability issues in scaled test setups. Advanced diagnostic and measurement techniques were investigated and incorporated into an annular test facility and a debris bed test facility. The diagnostic techniques investigated included: radioactively tagged salt solution, Frisch collar radiation detector array, neutron and x-ray imaging systems, and a Rayleigh backscatter-based fiber-optic temperature system. Models were checked against the in-situ experimental data and recommendations were made for modeling purposes.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Minimizing Backgrounds for the SuperCDMS SNOLAB Dark-Matter Experiment

Astronomical and cosmological observations indicate that large amounts of some slowly moving, unseen Dark Matter pervades the universe and outweighs normal matter by a factor of five. The Standard Model of Physics has no contender with the properties of this as-yet-undetected particle, so experimentalists build state-of-the-art radiation detectors to attempt to directly measure this Dark Matter. The Super Cryogenic Dark Matter Search (SuperCDMS) at Snolab is one such experiment, currently being constructed. This experiment uses ultra-cold, superconducting, high-purity silicon and germanium detectors to measure low-energy nuclear recoils from the elastic scattering of Dark Matter. I contributed to the calibration of the energy scale of low-energy nuclear recoils in CDMS II silicon detectors by computing an improved livetime correction for calibration data to verify the Monte Carlo rate normalization. Results indicate that the phonon collection efficiency of nuclear recoils relative to electron recoils is 95.2$^{+0.9}_{-0.7\%}$, and the ionization collection efficiency of low-energy nuclear recoils in silicon is lower than Lindhard prediction, consistent with other recent measurements. Backgrounds from the progeny decay of the abundant, naturally-occurring radioactive isotope radon-222 obstruct the sensitivity of essentially every dark-matter search. Radon concentrations in the Snolab cavern would contribute prohibitively large backgrounds if the volume surrounding the detectors were not purged with a low-flow low-radon gas. By measuring the radon diffusion and emanation, we identified acceptable gasket materials for sealing this radon purge, ensuring that the radon-induced backgrounds will be significantly lower than the other experimental backgrounds. A radon emanation system with a gas handling system and low-background radon detector was commissioned and used to measure the radon emanation of the proposed gaskets. A low-cost apparatus was constructed to measure the radon diffusion of gaskets with a commercial radon detector. The sensitivity of future generations of dark-matter detectors are expected to be dominated by long-lived low-energy beta- and alpha-emitting radon daughters such as 210 Pb on detector surfaces. I describe simulations indicating the detector could also be used to reduce background from material impurities plaguing rare-event searches, the commissioning of a prototype demonstration detector, and a gas handling system necessary to operate the detector. I demonstrated that the gas handling system reduces the otherwise dominant backgrounds by a factor of 62. This detector will therefore be able to detect 32 Si and 210 Pb 100 times better than currently available screeners.

Bowles, Michael A.↗

Evaluation of Oak Ridge National Laboratory Health Physics Research Reactor Operation Data for Critical Benchmark Creation [Abstract]

The Oak Ridge National Laboratory (ORNL) Health Physics Research Reactor (HPRR) was a research reactor designed and built at ORNL in 1961. The critical assembly was using a highly enriched uranium and molybdenum alloy as the fuel, and it could be operated in steady-state or burst modes. The reactor was used for about 25 years to produce a lot of publications related to dosimetry, radiobiology and radiation detectors testing before its decommissioning in 1987. In recent years, the idea of using legacy operation data from the to create a valuable critical accident alarm system shielding benchmark arose. Such a benchmark has been submitted to the International Criticality Safety Benchmark Experiment Project (ICSBEP) Technical Review Group for a potential inclusion in the 2022 version of the handbook. Another way to use the valuable data from the operation of the HPRR is to evaluate the feasibility of the creation of a subcritical or prompt supercritical benchmark for inclusion in the ICSBEP or the International Reactor Physics Experiments Evaluation Project (IRPhEP) handbooks. To initiate a burst, the HPRR had to be operated in a slightly subcritical state for a few minutes. Then, the insertion of the burst control rod would greatly increase the reactivity of the system and start the burst. No critical configuration of the HPRR critical assembly could be located. The only information available concerns stable subcritical and prompt supercritical states, found in a burst experiments’ logbook. In the recovered logbook pages, information about 8 different bursts is available. The information includes the rods positions before and during a burst, the recorded subcritical reactor period and reactivity, and the burst fission yield derived from the temperature elevation sulfur pellet irradiation analysis. By using the HPRR logbook information and the as-built drawings of the critical assembly, a highly detailed model of the HPRR was created with SCALE 6.2.4/KENO-VI. Eight KENO-VI models were created to replicate the sub-critical assembly configurations described in the eight bursts from the recovered logbook pages. KENO-VI calculates k eff and it can be linked to a reactivity value in cents by using the delayed neutron fraction B eff , also calculated by KENO-VI. KENO-VI can also be used to model the prompt super-critical configurations of the HPRR and to assess the similarity with the burst measurements by comparing the calculated k eff and the measured fission yields between each burst. Unfortunately, high uncertainty exist and the obtained discrepancies between experiments and calculation results are high, compromising the creation of a valuable critical benchmark from HPRR operation data. The reasons of the discrepancies and potential ways to solve them are explored.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Integration of Nuclear Material Accounting Data and Process Monitoring Data for Improvement on Detection Probability in Safeguarding Electrochemical Processing Facilities (Final Technical Report)

The KAERI advanced spent fuel conditioning process (ACP) process is a critical component of the US- South Korean nuclear cooperation and the following “123 Agreement.” Its development has received considerable attention in both countries. The ACP is an electrochemical processing (pyroprocessing) that recycles over 96% of the used nuclear fuel (UNF). It is also intrinsically proliferation-resistant in theory. In normal operation, the U/TRU product is very hot radiologically. In addition, the Cm provides a high level of spontaneous neutrons, making the product unsuitable for weapon use. However, as pointed in some study, “the need for safeguards to protect against the diversion and misuse of separated plutonium applies essentially equally to all grades of plutonium.” As pointed by many studies, the well-established traditional Nuclear Material Accounting (NMA) approach cannot be directly applied to electrochemical processing because of the lack of an input accountability tank, the non-continuous material flow, and the unsatisfactory level of confidence in sampling methods. Therefore, nuclear safeguards remain a grand challenge in the developing of commercial electrochemical separations facilities, especially around the heart of such facilities, the electrorefiner (ER) systems. In contrast to NMA data, process monitoring (PM) data is normally an indirect measurement of the SNM and is acquired much more frequently. In a broad sense, PM includes monitoring by various types of equipment, e.g. radiation detectors, cameras, voltage, current sensors. Because it is already being collected by the operator, the additional cost to safeguards is low. It has long been believed that PM data can supplement NMA data and help improve safeguards, although the benefits are hard to quantify. The U.S. DOE’s Material Protection, Accounting, and Control Technology (MPACT) campaign has made substantial investments into innovative PM sensor technology and predictive model development for real- or near real-time measurement and prediction of molten salt density and level, salt composition and actinide concentration especially Pu, the cell voltage, and the cell current to supplement traditional NMA. For aqueous-based reprocessing facilities, it is reported that PM, integrated with traditional NMA, have a high detection probability for specific diversions. For electrochemical reprocessing, preliminary studies have shown that PM data can support traditional NMA in various ways by providing a basis to estimate some of the in-processing nuclear material inventories. Despite early success, further studies on fusion of PM data and NMA data are still needed, which is the goal of this proposed work.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Compact and Handheld Radioisotope Imaging Systems for Bio-medicine*

Author: Andrew Weisenberger (Thomas Jefferson National Accelerator Facility) Thomas Jefferson National Accelerator Facility is a U.S. Department of Energy federally funded research and development center whose mission is to study quark gluon physics. The laboratory capitalizes on its unique technologies and expertise to explore ways of applying nuclear physics principles and technologies to societal needs. The Radiation Detector and Imaging Group, in collaboration with universities, industry and other government laboratories, has for several years been applying advances in nuclear physics detector technology to several applications, particularly in the development of compact and handheld nuclear imaging systems. I will provide a brief overview of Jefferson Lab and provide examples of how the group has leveraged nuclear physics to bring advances to nuclear medicine, medical research and plant biology. The group continues to develop medical devices based on both single photon emission computed tomography (SPECT) and positron emission tomography (PET), making use of technology originally developed for basic nuclear physics research. *Thomas Jefferson National Accelerator Facility is operated by Jefferson Science Associates, LLC under U.S. DOE Contract No. DE-AC05-06OR23177.

Weisenberger, Andrew↗

Microscale device and method for purification of radiopharmaceuticals

A microfluidic chip device for the purification of radiochemical compounds includes a chip having an injection channel and intersecting branch channels with a plurality of valves are located along the injection channel and branch channels and configured to retain a plug of solution containing the radiochemical compound. The chip further includes a serpentine channel segment (for separation) coupled to the output of the injection channel. A high voltage power source advances the plug of solution through the purification region and into the downstream fraction collection channel. The chip includes a downstream fraction collection channel coupled to the serpentine channel segment and having an optical and radiation detection regions. One or more branch fraction channels intersect with the fraction collection channel and include valves located therein so that the radiochemical compound that is detected using a radiation detector is directed into the desired branch fraction channel for subsequent use.

Van Dam, R. Michael↗

A New Control System Software for SANS BATAN Spectrometer in Serpong, Indonesia

The original main control system of the 36 meter small-angle neutron scattering (SANS) BATAN Spectrometer (SMARTer) has been replaced with the new ones due to the malfunction of the main computer. For that reason, a new control system software for handling all the control systems was also developed in order to put the spectrometer back in operation. The developed software is able to control the system such as rotation movement of six pinholes system, vertical movement of four neutron guide system with the total length of 16.5 m, two-directional movement of a neutron beam stopper, forward-backward movement of a 2D position sensitive detector (2D-PSD) along 16.7 m, etc. A Visual Basic language program running on Windows operating system was employed to develop the software and it can be operated by other remote computers in the local area network. All device positions and command menu are displayed graphically in the main monitor or window and each device control can be executed by clicking the control button. Those advantages are necessary required for developing a new user-friendly control system software. Finally, the new software has been tested for handling a complete SANS experiment and it works properly.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Characterizing the Thermal Column Beam in the University of Massachusetts Lowell Research Reactor

The University of Massachusetts Lowell operates a 1 MW, light water cooled and moderated Research Reactor (UMLRR) fueled by low-enriched uranium to generate neutron flux that is used at a variety of in-core and beam port facilities within the reactor to perform irradiation experiments for academic and industrial research. One of the irradiation sites is a graphite-moderated thermal column designed to deliver a collimated beam of thermal neutrons to a neutron radiography imaging system. A detailed characterization of the neutron beam is essential for the design and interpretation of experiments at the facility and for radiation safety. This work aimed to characterize the neutron flux and energy spectrum in the UMLRR thermal column beam by employing experimental and computational methods known as the foil activation and spectrum unfolding technique. A previously existing Monte Carlo N-Particle transport (MCNP) model of the UMLRR reactor core has been extended to the thermal column where the neutron flux and energy spectrum have been computed and experimentally validated. This work employed the foil activation and spectrum unfolding technique along with neutron transport computation to extend the knowledge of the neutron fluence and energy spectrum from the UMLRR core to the adjacent thermal column beam. Radiography systems are used for materials characterization, studying dynamic behavior of engineering systems, and for nuclear forensics applications. Foil activation is an experimental method where thin foils of highly pure materials are placed in the beam where interactions between the neutrons and the foil material activate radioisotopes in the foils whose activities can be measured after the irradiation. Downstream computation with MCNP and the spectrum unfolding code SAND can deconvolute the neutron fluence and energy spectrum that must have been necessary to induce the production rates of radioisotopes that were obtained through foil activation. The necessary ingredients for successful spectrum unfolding are the experimentally measured production rates and some a priori (initial guess) knowledge of the flux spectrum. The thermal column is equipped with a neutron radiography imaging system, so any experimenters who desire to use neutron radiography at UMass Lowell will benefit significantly from knowing the characteristics of the neutron beam. Comprehensive knowledge of these characteristics of the beam is essential to compare and benchmark results obtained for similar experiments at other facilities. The Integrated Nuclear Security and Safeguards Laboratory (INSSL) is pursuing the investigation of the performance of self-healing materials under stress-strain environments and the characterization of radiation detectors and special containers for storing and transporting nuclear material. This work contributes to the improvement of the current radiography system, expands the utility of the system for nuclear safeguards and security application and provides information that will enhance the general safety of the UMLRR experimental facilities. The main objective of this work has been achieved; an appropriate neutron flux spectrum for the UMLRR thermal column beam has been determined using the foil activation method followed by spectrum unfolding. There now exists an experimentally validated computational model of the neutron flux spectrum and the thermal column's neutron environment is characterized. We can conclude that the thermal column is well characterized; an appropriate neutron flux spectrum has been determined through an experimentally validated computational model. Future experimenters interested in the thermal column may now expand on the computational model or use the spectral information for their own purposes. The knowledge gained herein will be helpful for the INSSL's future work using neutron radiography to analyze the effectiveness of self-healing materials and special containers. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

AGC-4 As-Run Uncertainty Analysis

The concept of measuring neutron flux (or fluence rate) with activation foils has existed since the late 1940s and is a well-used methodology. Activation foils are selected for their unique isotopic cross sections that create reaction products with desirable properties: relatively simple radioactive decay scheme, measurable quantities of gamma-rays or betas, and half-lives appropriate for the irradiation and decay durations of the experiment. The activation materials, deemed flux wires, fluence wires, dosimeters, or flux foils, are fabricated to have a mass appropriate for the irradiation as well so the measurement using a radiation detector following the irradiation is sufficient but not overwhelming in terms of total activity. Activation measurement results are expressed in terms of reaction rate, which can then be used to “adjust” the neutron spectrum. The Advanced Graphite Creep (AGC)-4 experiment contained 26 flux wire packages, each containing an iron and a niobium wire inside a vanadium capsule. For all stackup positions, the value of fast to thermal neutrons is higher than expected, but the total neutron fluence is near the predicted value of ~2 x 1022 n/cm2. As compared to the predicted neutron spectrum, there are four takeaways in the results as compared to the predicted ATR irradiation: 1) Additional fast (fission) neutrons present, 2) Spectrum hardening due to temperature, 3) Spectrum hardening due to container attenuation, 4) Total neutron fluence is close to predicted values. Since the neutron energy spectrum is a key parameter when attributing neutron damage in materials, the adjusted energy-dependent spectrum and the total neutron fluence results from the dosimeters can be incorporated for future calculations.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Detection of gamma-neutron radiation by solid-state scintillation detectors. Detection of gamma-neutron radiation by novel solid-state scintillation detectors

It is known that solid-state scintillators can be used for detection of both gamma radiation and neutron flux. In the past, neutron detection efficiencies of such solid-state scintillators did not exceed 5-7%. At the same time it is known that the detection efficiency of the gamma-neutron radiation characteristic of nuclear fissionable materials is by an order of magnitude higher than the efficiency of detection of neutron fluxes alone. Thus, an important objective is the creation of detection systems that are both highly efficient in gamma-neutron detection and also capable of exhibiting high gamma suppression for use in the role of detection of neutron radiation. In this work, we present the results of our experimental and theoretical studies on the detection efficiency of fast neutrons from a {sup 239}Pu-Be source by the heavy oxide scintillators BGO, GSO, CWO and ZWO, as well as ZnSe(Te, O). The most probable mechanism of fast neutron interaction with nuclei of heavy oxide scintillators is the inelastic scattering (n, n'γ) reaction. In our work, fast neutron detection efficiencies were determined by the method of internal counting of gamma-quanta that emerge in the scintillator from (n, n''γ) reactions on scintillator nuclei with the resulting gamma energies of ∼20-300 keV. The measured efficiency of neutron detection for the scintillation crystals we considered was ∼40-50 %. The present work included a detailed analysis of detection efficiency as a function of detector and area of the working surface, as well as a search for new ways to create larger-sized detectors of lower cost. As a result of our studies, we have found an unusual dependence of fast neutron detection efficiency upon thickness of the oxide scintillators. An explanation for this anomaly may involve the competition of two factors that accompany inelastic scattering on the heavy atomic nuclei. The transformation of the energy spectrum of neutrons involved in the (n, n'γ) reactions towards lower energies and the isotropic character of scattering of the secondary neutrons may lead to the observed limitation of the length of effective interaction, since a fraction of the secondary neutrons that propagate in the forward direction are not subject to further inelastic scattering because of their substantially lower energy. At these reduced energies, it is the capture cross-section (n, γ) that becomes predominant, resulting in lower detection efficiency. Based on these results, several types of detectors have been envisioned for application in detection systems for nuclear materials. The testing results for one such detector are presented in this work. We have studied the possibility of creation of a composite detector with scintillator granules placed inside a transparent polymer material. Because of the low transparency of such a dispersed scintillator, better light collection conditions are ensured by incorporation of a light guide between the scintillator layers. This guide is made of highly transparent polymer material. The use of a high-transparency hydrogen-containing polymer material for light guides not only ensures optimum conditions of light collection in the detector, but also allows certain deceleration of neutron radiation, increasing its interaction efficiency with the composite scintillation panels; accordingly, the detector signal is increased by 5-8%. When fast neutrons interact with the scintillator material, the resulting inelastic scattering gamma-quanta emerge, having different energies and different delay times with respect to the moment of the neutron interaction with the nucleus of the scintillator material (delay times ranging from 1x10{sup -9} to 1.3x10{sup -6} s). These internally generated gamma-quanta interact with the scintillator, and the resulting scintillation light is recorded by the photo-receiver. Since neutron sources are also strong sources of low-energy gamma-radiation, the use of dispersed ZnSe(Te) scintillator material provides high gamma-radiation detection efficiency in that energy range. This new type of gamma-neutron detector is based on a 'sandwich' structure using a ZnSe composite film and light guide with a fast neutron detection efficiency of about 6%. Its high detection efficiency of low-energy gamma-radiation allows a substantial increase (by an order of magnitude) in the efficiency of detection of neutron sources and transuranic materials by means of simultaneous detection of accompanying gamma-radiation. The design and fabrication technology of this detector allows the creation of gamma-neutron detectors characterized by high sensitivity at relatively low costs (as compared with analogs using oxide scintillators) for portable inspection systems. The sandwich structure can be comprised of any number of plates, with no limitations on thickness or area.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Intelligent Pixel Detectors: Towards a Radiation Hard ASIC with On-Chip Machine Learning in 28 nm CMOS

Detectors at future high energy colliders will face enormous technical challenges. Disentangling the unprecedented numbers of particles expected in each event will require highly granular silicon pixel detectors with billions of readout channels. With event rates as high as 40 MHz, these detectors will generate petabytes of data per second. To enable discovery within strict bandwidth and latency constraints, future trackers must be capable of fast, power efficient, and radiation hard data-reduction at the source. We are developing a radiation hard readout integrated circuit (ROIC) in 28nm CMOS with on-chip machine learning (ML) for future intelligent pixel detectors. We will show track parameter predictions using a neural network within a single layer of silicon and hardware tests on the first tape-outs produced with TSMC. Preliminary results indicate that reading out featurized clusters from particles above a modest momentum threshold could enable using pixel information at 40 MHz.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Prediction of Leakage Current and Depletion Voltage in Silicon Detectors Under Extraterrestrial Radiation Conditions

Silicon detection is a mature technology for registering the passage of charged particles. At the same time it continues to evolve toward increasing radiation tolerance as well as precision and adaptability. For these reasons it is likely to remain a critical element of detection of systems associated with extraterrestrial exploration. Silicon sensor leakage current and depletion voltage depend on the integrated fluence received by the sensor and on its thermal history during and after the irradiation process. For minimal assumptions on shielding and hence on the particle energy spectrum, and using published data on Martian ground temperature, we predict the leakage current density and the depletion voltage, as a function of time, of silicon sensors in transit to and deployed continuously on the Mars surface for a duration of up to 28 Earth-years, for several sensor geometries and a worst-case temperature scenario.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

The Axion Dark-Matter eXperiment (ADMX): Recent Results

The axion is a hypothetical elementary particle whose existence would explain the baffling absence of CP violation in the strong interactions. It's properties in addition make it a good dark-matter candidate. Even though dark-matter axions would make up the overwhelming majority of mass in the universe, they are extraordinarily difficult to detect. We have developed a detector, ADMX, for dark-matter axions that is at heart an exquisitely sensitive detector of electromagnetic radiation. This talk will describe the progress we have made in this experimental search.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Dosimetric characterization of a synthetic single crystal diamond detector in clinical radiation therapy small photon beams

Purpose: To determine the potentialities of synthetic single crystal diamond Schottky diodes for accurate dose measurements in radiation therapy small photon beams. Methods: The dosimetric properties of a diamond-based detector were assessed by comparison with a reference microionization chamber. The diamond device was operated at zero bias voltage under irradiation with high-energy radiotherapic photon beams. The stability of the detector response and its dose and dose rate dependence were measured. Different square field sizes ranging from 1 Multiplication-Sign 1 cm{sup 2} to 10 Multiplication-Sign 10 cm{sup 2} were used during comparative dose distribution measurements by means of percentage depth dose curves (PDDs), lateral beam profiles, and output factors. The angular and temperature dependence of the diamond detector response were also studied. Results: The detector response shows a deviation from linearity of less than {+-}0.5% in the 0.01-7 Gy range and dose rate dependence below {+-}0.5% in the 1-6 Gy/min range. PDDs and output factors are in good agreement with those measured by the reference ionization chamber within 1%. No angular dependence is observed by rotating the detector along its axis, while {approx}3.5% maximum difference is measured by varying the radiation incidence angle in the polar direction. The temperature dependence was investigated as well and a {+-}0.2% variation of the detector response is found in the 18-40 Degree-Sign C range. Conclusions: The obtained results indicate the investigated synthetic diamond-based detector as a candidate for small field clinical radiation dosimetry in advanced radiation therapy techniques.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

High Elevation Radiation Array (HERA) detectors for airborne thunderstorm investigations

A high-energy atmospheric physics phenomenon, referred to as a terrestrial gamma ray flash (TGF), is associated with lightning and produces large bursts of energetic photon radiation. TGFs will be investigated using a suite of gamma-ray instruments designed and constructed to fly on ten United States Air Force (USAF) WC-130J Hurricane Hunter aircraft as part of an aircrew ionization study led by the Air Force Institute of Technology (AFIT) and the United States Air Force School of Aerospace Medicine (USAFSAM), in cooperation with the 53rd Weather Reconnaissance Squadron (WRS). Each instrument consists of one NaI and one plastic detector, a GPS timing device, and an instrument computer that performs data acquisition. High Elevation Radiation Array (HERA) detectors will be employed to maximize the chances of observing TGFs near their source and to gain a better understanding of their origin, mechanism, ubiquity, and to assess potential hazards posed to military and commercial aircrew and passengers. The HERA program, deployed on 10 separate Air Force aircraft over a multi-year campaign, will result in thousands of observational flight hours and be the largest concerted effort to date to observe TGFs in situ through aircraft observations. In this paper, we give an overview of the scientific goals of this campaign and how the HERA instruments have been designed to meet those goals. Here, we include a detailed description of the HERA instrument, along with mass model and signal processing simulations.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗