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At least 991 records · Page 55

CROCUS Dual Polarization Ceilometer Data at Northeastern Illinois University Rooftop

This dataset is from the Department of Energy Office of Science funded project, CROCUS Urban Integrated Field Laboratory (https://crocus-urban.org/). The dual-polarization ceilometer (Vaisala CL61) is an autonomous lidar system operating at 910 nm wavelength, providing valuable measurements for understanding atmospheric boundary layer evolution, air quality, and cloud-aerosol interactions. The CL61 measures the backscattered signal intensity alternating between parallel- and cross-polarization signals. The unique depolarization measurement capability improves discrimination between different particle types, such as liquid droplets, ice crystals, and aerosols. The depolarization is highly dependent on the scatterer shape and orientation (spherical vs non-spherical particles), with the linear depolarization ratio providing a measure of dominant backscatter signal component from atmospheric particles at various heights, essentially allowing discrimination between liquid and solid particles. With its efficient optical system, CL61’s improved signal-to-noise ratio compared to traditional ceilometers allows studying detailed vertical profiles of aerosols and clouds up to 15 km height.Datasets are stored in a netCDF data format, and we we encourage users to make use of the associated toolkits available from Unidata (https://www.unidata.ucar.edu/software/netcdf/), Project Pythia (https://foundations.projectpythia.org/core/data-formats/netcdf-cf.html), and our “Instrument Cookbooks” (https://crocus-urban.github.io/instrument-cookbooks) for more information on how to process the metadata-rich datasets.

54 ENVIRONMENTAL SCIENCES↗

Nuclei of two earth-grazing comets of fan-shaped appearance

The conceptual model of a collimated particle flow from isolated sources on the nucleus formulated for comets displaying a persisting sunward fanlike coma is successfully applied to two short-period comets, Pons-Winnecke (PW) and Schwassmann-Wachmann 3 (SW3), observed respectively in 1927 and 1930. For PW, the interpretation of fan-orientation pattern is compatible with the spin axis inertially fixed in May-June 1927, but for SW3 the interpretation requires rapid nucleus precession at a peak rate of about 1.4 deg/day. Both comets satisfy the basic conditions for displaying a fan in the time span covered by the fan observations. The emission sources are situated within 35 deg of the sunlit rotation pole of PW and within 19 deg of the pole of SW 3. A rotation period of 8.2 hr is suggested for PW if the rotation sense is prograde or 5.8 hr if it is retrograde. Water production rates and global loss and erosion rates for the comets are estimated.

Sekanina, Z.↗

Uncertainty quantification and optimization of precipitating hydrometeor parameters for winter precipitation in a cloud microphysics scheme

The precipitating hydrometeor parameters used in cloud microphysics schemes carry inherent uncertainties. The quantification of these uncertainties, together with parameter optimization, can significantly improve precipitation forecasts. This study investigates the effects of 13 parameters in the Weather Research and Forecasting (WRF) Double-Moment 6-class (WDM6) microphysics scheme, which define the hydrometeor characteristics such as fall velocity–diameter and mass–diameter relationships, as well as the shape parameter of the drop size distribution for precipitating particles such as rain, snow, and graupel on simulated winter precipitation. A comparison between the model's pre-defined parameters and observations from the International Collaborative Experiments for the PyeongChang 2018 Olympic and Paralympic winter games (ICE-POP 2018) field campaign reveals that the fall velocity–diameter relationship for rain, the mass–diameter relationships for snow and graupel, and the shape parameters for all precipitating particles in the WDM6 scheme deviate from the median values observed by the two-dimensional video disdrometer (2DVD). To quantify parameter sensitivities, a perturbed parameter ensemble (PPE) of 256 simulations was conducted within parameter ranges constrained by 2DVD observations for three winter precipitation cases. Bayesian optimization was then applied to identify parameter sets that minimized the root mean square error (RMSE) for each case, achieving reductions of up to 30.2 %. These results demonstrate that ensemble-based uncertainty quantification and parameter optimization can help identify key parameters and provide a pathway to improving precipitation simulation performance. In addition, measurement sites can be strategically selected based on regions that show high sensitivity to variations in hydrometeor characteristic parameters.

Bayesian optimization↗

Investigation of nanoparticulate silicon as printed layers using scanning electron microscopy, transmission electron microscopy, X-ray absorption spectroscopy and X-ray photoelectron spectroscopy

The presence of native oxide on the surface of silicon nanoparticles is known to inhibit charge transport on the surfaces. Scanning electron microscopy (SEM) studies reveal that the particles in the printed silicon network have a wide range of sizes and shapes. High-resolution transmission electron microscopy reveals that the particle surfaces have mainly the (111)- and (100)-oriented planes which stabilizes against further oxidation of the particles. X-ray absorption spectroscopy (XANES) and X-ray photoelectron spectroscopy (XPS) measurements at the O 1 s -edge have been utilized to study the oxidation and local atomic structure of printed layers of silicon nanoparticles which were milled for different times. XANES results reveal the presence of the +4 (SiO 2 ) oxidation state which tends towards the +2 (SiO) state for higher milling times. Si 2 p XPS results indicate that the surfaces of the silicon nanoparticles in the printed layers are only partially oxidized and that all three sub-oxide, +1 (Si 2 O), +2 (SiO) and +3 (Si 2 O 3 ), states are present. The analysis of the change in the sub-oxide peaks of the silicon nanoparticles shows the dominance of the +4 state only for lower milling times.

36 MATERIALS SCIENCE↗

Scattering Properties and Brightness Temperatures Associated with Solid Precipitation

In the past few years, early solid precipitation detection and retrieval algorithms have been developed and shown to be applicable for snowing clouds and blizzards. NOAA has an operational snow versus rain classifier based on AMSU-B observations. Solid precipitation retrieval algorithms reported in the literature over the past two years include those that rely on neural nets, statistics, or physical relationships. All of the algorithms require the use of millimeter-wave radiometer observations. The millimeter-wave frequencies are especially sensitive to the scattering and emission properties of frozen particles due to the ice particle refractive index. Passive radiometric channels respond to both the integrated particle mass throughout the volume and field of view, and to the amount, location, and size distribution of the frozen (and liquid) particles with the sensitivity varying for different frequencies and hydrometeor types. This investigation probes the sensitivity of scattering and absorption coefficients, and hence computed brightness temperatures, resulting from variations in solid precipitation cloud profiles. The first study compares the single scattering, absorption, and asymmetry parameters associated with snow particles in clouds. Several methodologies are used to convert the physical characteristics (e.g., shape, size distributions, ice-air-water ratios) of ice particles to electromagnetic properties (e.g., absorption, scattering, and asymmetry factors). These methodologies include: conversion to solid ice particles, homogeneous dielectric mixing, or discrete dipole approximation. Changes in the conversion methodology can produce computed brightness temperature differences greater than 50 Kelvin.

Skofronick-Jackson, Gail M.↗

Linearized T-Matrix and Mie Scattering Computations

We present a new linearization of T-Matrix and Mie computations for light scattering by non-spherical and spherical particles, respectively. In addition to the usual extinction and scattering cross-sections and the scattering matrix outputs, the linearized models will generate analytical derivatives of these optical properties with respect to the real and imaginary parts of the particle refractive index, and (for non-spherical scatterers) with respect to the ''shape'' parameter (the spheroid aspect ratio, cylinder diameter/height ratio, Chebyshev particle deformation factor). These derivatives are based on the essential linearity of Maxwell's theory. Analytical derivatives are also available for polydisperse particle size distribution parameters such as the mode radius. The T-matrix formulation is based on the NASA Goddard Institute for Space Studies FORTRAN 77 code developed in the 1990s. The linearized scattering codes presented here are in FORTRAN 90 and will be made publicly available.

Analytic linearization↗

Synthesis of nanograined zirconium diboride microsphere powder feedstock via emulsification of suspensions

Ceramic nanograined materials have desirable characteristics compared to their macroparticle counterparts but are rarely used in industrial applications due to issues with poor handleability and health hazards. Due to interparticle forces that become more dominant as the particle size decreases, it is difficult to use nanomaterials to fill dies, spread on surfaces, or flow through hoppers found in various manufacturing processes. In this work, we report a scalable gelcasting solution and unique emulsification process to create microspheres composed of nanoscale powders to enhance the flowability and handleability of nanomaterials. The gelcasting solution and emulsification process can be used with any nanoparticle composition that can be suspended in a liquid phase. This paper reports the effects of various parameters on zirconium diboride microsphere formation, such as surfactant content and mixing conditions. The microspheres maintain the nano-scale characteristics of the powder but improve its flowability by using cross-linked polyvinyl alcohol to combine irregularly shaped zirconium diboride nanoparticles with a particle diameter of 60 nm into larger spherical particles with a d 50 ~25 μm. This hierarchical feedstock engineering design combine the positive characteristics of materials across both length scales and improve the flowability of the feedstock from a Hausner Ratio of 1.56 to 1.19. The materials produced using this technique can be used in thermal plasma spray, die filling for hot pressing or spark plasma sintering, and binder jet printing applications.

36 MATERIALS SCIENCE↗

Bidirectional Reflectance of Flat, Optically Thick Particulate Layers: An Efficient Radiative Transfer Solution and Applications to Snow and Soil Surfaces

We describe a simple and highly efficient and accurate radiative transfer technique for computing bidirectional reflectance of a macroscopically flat scattering layer composed of nonabsorbing or weakly absorbing, arbitrarily shaped, randomly oriented and randomly distributed particles. The layer is assumed to be homogeneous and optically semi-infinite, and the bidirectional reflection function (BRF) is found by a simple iterative solution of the Ambartsumian's nonlinear integral equation. As an exact Solution of the radiative transfer equation, the reflection function thus obtained fully obeys the fundamental physical laws of energy conservation and reciprocity. Since this technique bypasses the computation of the internal radiation field, it is by far the fastest numerical approach available and can be used as an ideal input for Monte Carlo procedures calculating BRFs of scattering layers with macroscopically rough surfaces. Although the effects of packing density and coherent backscattering are currently neglected, they can also be incorporated. The FORTRAN implementation of the technique is available on the World Wide Web at http://ww,,v.giss.nasa.gov/-crmim/brf.html and can be applied to a wide range of remote sensing, engineering, and biophysical problems. We also examine the potential effect of ice crystal shape on the bidirectional reflectance of flat snow surfaces and the applicability of the Henyey-Greenstein phase function and the 6-Eddington approximation in calculations for soil surfaces.

Mishchenko, Michael I.↗

Development of Metallic Sensory Alloys

Existing nondestructive evaluation (NDE) technologies are inherently limited by the physical response of the structural material being inspected and are therefore not generally effective at the identification of small discontinuities, making the detection of incipient damage extremely difficult. One innovative solution to this problem is to enhance or complement the NDE signature of structural materials to dramatically improve the ability of existing NDE tools to detect damage. To address this need, a multifunctional metallic material has been developed that can be used in structural applications. The material is processed to contain second phase sensory particles that significantly improve the NDE response, enhancing the ability of conventional NDE techniques to detect incipient damage both during and after flight. Ferromagnetic shape-memory alloys (FSMAs) are an ideal material for these sensory particles as they undergo a uniform and repeatable change in both magnetic properties and crystallographic structure (martensitic transformation) when subjected to strain and/or temperature changes which can be detected using conventional NDE techniques. In this study, the use of a ferromagnetic shape memory alloy (FSMA) as the sensory particles was investigated.

Wallace Terryl A.↗

Full-wave simulations of ICRF heating regimes in toroidal plasma with non-Maxwellian distribution functions

At the power levels required for significant heating and current drive in magnetically-confined toroidal plasma, modification of the particle distribution function from a Maxwellian shape is likely (Stix 1975 Nucl. Fusion 15 737), with consequent changes in wave propagation and in the location and amount of absorption. In order to study these effects computationally, both the finite-Larmor-radius and the high-harmonic fast wave (HHFW), versions of the full-wave, hot-plasma toroidal simulation code TORIC (Brambilla 1999 Plasma Phys. Control. Fusion 41 1 and Brambilla 2002 Plasma Phys. Control. Fusion 44 2423), have been extended to allow the prescription of arbitrary velocity distributions of the form f(v(parallel to), v(perpendicular to) , psi, theta). For hydrogen (H) minority heating of a deuterium (D) plasma with anisotropic Maxwellian H distributions, the fractional H absorption varies significantly with changes in parallel temperature but is essentially independent of perpendicular temperature. On the other hand, for HHFW regime with anisotropic Maxwellian fast ion distribution, the fractional beam ion absorption varies mainly with changes in the perpendicular temperature. The evaluation of the wave-field and power absorption, through the full wave solver, with the ion distribution function provided by either a Monte-Carlo particle and Fokker-Planck codes is also examined for Alcator C-Mod and NSTX plasmas. Non-Maxwellian effects generally tend to increase the absorption with respect to the equivalent Maxwellian distribution.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Full-wave simulations of ICRF heating regimes in toroidal plasmas with non-Maxwellian distribution functions

At the power levels required for significant heating and current drive in magnetically-confined toroidal plasma, modification of the particle distribution function from a Maxwellian shape is likely [T. H. Stix, Nucl. Fusion, 15 737 (1975)], with consequent changes in wave propagation and in the location and amount of absorption. In order to study these effects computationally, both the finite-Larmor-radius and the high-harmonic fast wave (HHFW), versions of the full-wave, hot-plasma toroidal simulation code TORIC [M. Brambilla, Plasma Phys. Control. Fusion 41, 1 (1999) and M. Brambilla, Plasma Phys. Control. Fusion 44, 2423 (2002)], have been extended to allow the prescription of arbitrary velocity distributions of the form f(v||, v_perp, psi , theta). For hydrogen (H) minority heating of a deuterium (D) plasma with anisotropic Maxwellian H distributions, the fractional H absorption varies significantly with changes in parallel temperature but is essentially independent of perpendicular temperature. On the other hand, for HHFW regime with anisotropic Maxwellian fast ion distribution, the fractional beam ion absorption varies mainly with changes in the perpendicular temperature. The evaluation of the wave-field and power absorption, through the full wave solver, with the ion distribution function provided by either aMonte-Carlo particle and Fokker-Planck codes is also examined for Alcator C-Mod and NSTX plasmas. Non-Maxwellian effects generally tends to increase the absorption with respect to the equivalent Maxwellian distribution.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

e + e - angularity distributions at NNLL' accuracy

We present predictions for the e + e – event shape angularities at NNLL' resummed and O (α 2 s ) matched accuracy and compare them to LEP data at center-of-mass energies Q = 91.2 GeV and Q = 197 GeV. We perform the resummation within the framework of Soft-Collinear Effective Theory, and make use of recent results for the two-loop angularity soft function. We determine the remaining NNLL' and O (α 2 s ) ingredients from a fit to the EVENT2 generator, and implement a shape function with a renormalon-free gap parameter to model non-perturbative effects. Using values of the strong coupling α s (m Z ) and the universal non-perturbative shift parameter Ω 1 that are consistent with those obtained in previous fits to the thrust and C -parameter distributions, we find excellent agreement between our predictions and the LEP data for all angularities with a ϵ [–1, 0.5]. This provides a robust test of the predictions of QCD, factorization, and the universal scaling of the non-perturbative shift across different angularities. Promisingly, our results indicate that current degeneracies in the {α s (m Z ), Ω 1 } parameter space could be alleviated upon fitting these parameters to experimental data for the angularity distributions.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Coarse-grained methods for heterogeneous vesicles with phase-separated domains: Elastic mechanics of shape fluctuations, plate compression, and channel insertion

We develop coarse-grained particle approaches for studying the elastic mechanics of vesicles with heterogeneous membranes having phase-separated domains. We perform simulations both of passive shape fluctuations and of active systems where vesicles are subjected to compression between two plates or subjected to insertion into narrow channels. Analysis methods are developed for mapping particle configurations to continuum fields with spherical harmonics representations. Heterogeneous vesicles are found to exhibit rich behaviors where the heterogeneity can amplify surface two-point correlations, reduce resistance during compression, and augment vesicle transport times in channels. The developed methods provide general approaches for characterizing the mechanics of coarse-grained heterogeneous systems taking into account the roles of thermal fluctuations, geometry, and phase separation.

97 MATHEMATICS AND COMPUTING↗

Introduction to Particle Acceleration in the Cosmos

Accelerated charged particles have been used on Earth since 1930 to explore the very essence of matter, for industrial applications, and for medical treatments. Throughout the universe nature employs a dizzying array of acceleration processes to produce particles spanning twenty orders of magnitude in energy range, while shaping our cosmic environment. Here, we introduce and review the basic physical processes causing particle acceleration, in astrophysical plasmas from geospace to the outer reaches of the cosmos. These processes are chiefly divided into four categories: adiabatic and other forms of non-stochastic acceleration, magnetic energy storage and stochastic acceleration, shock acceleration, and plasma wave and turbulent acceleration. The purpose of this introduction is to set the stage and context for the individual papers comprising this monograph.

Gallagher, D. L.↗

Identifying Sample Provenance From SEM/EDS Automated Particle Analysis via Few-Shot Learning Coupled With Similarity Graph Clustering

Automated particle analysis (APA) provides a vast amount of compositional data via energy-dispersive X-ray spectroscopy along with size and shape data via scanning electron microscopy for individual particles in a sample. In many instances, APA data are leveraged to support identification of the source of a sample based on the detection of particles of a specific composition. Often, the particles that provide context make up a minuscule portion of the sample. Additionally, the interpretation of complex samples can be difficult due to the diversity of compositions both in the mixture and within a particle. In this work, we demonstrate a method to compute and cluster similarity graphs that describe inter-particle relationships within a sample using a multi-modal few-shot learning neural network. Here, as a proof-of-concept, we show that samples known to have been exposed to gunshot residue can be distinguished from samples occasionally mistaken for gunshot residue. Our workflow builds upon standard APA techniques and data processing methods to unveil additional information in a readily interpretable and quantitatively comparable format.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Determination of the complex refractive index and size distribution of atmospheric particulates from bistatic-monostatic lidar and solar radiometer measurements

A method is presented for inferring both the size distribution and the complex refractive index of atmospheric particulates from combined bistatic-monostatic lidar and solar radiometer observations. The basic input measurements are spectral optical depths at several visible and near-infrared wavelengths as obtained with a solar radiometer and backscatter and angular scatter coefficients as obtained from a biostatic-monostatic lidar. The spectral optical depth measurements obtained from the radiometer are mathematically inverted to infer a columnar particulate size distribution. Advantage is taken of the fact that the shape of the size distribution obtained by inverting the particulate optical depth is relatively insensitive to the particle refractive index assumed in the inversion. Bistatic-monostatic angular scatter and backscatter lidar data are then processed to extract an optimum value for the particle refractive index subject to the constraint that the shape of the particulate size distribution be the same as that inferred from the solar radiometer data. Specifically, the scattering parameters obtained from the bistatic-monostatic lidar data are compared with corresponding theoretical computations made for various assumed refractive index values. That value which yields best agreement, in a weighted least squares sense, is selected as the optimal refractive index estimate. The results of this procedure applied to a set of simulated measurements as well as to measurements collected on two separate days are presented and discussed.

Reagan, J. A.↗