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NASA NTRS2021

Direct Measurements of Infrared Intensities of HCN and H2O + HCN Ices for Laboratory and Observational Astrochemistry

Hydrogen cyanide (HCN) is found in a wide variety of extraterrestrial environments within and beyond the solar system, and for that reason laboratory spectroscopists have studied this compound in many spectral regions, including the infrared (IR). However, one aspect that remains to be investigated is the intrinsic IR spectral intensities of solid HCN as opposed to relative band strengths, intrinsic intensities being needed to measure HCN abundances. Here we report measurements of IR absorption coefficients and band strengths, along with supporting refractive indices and densities, of both amorphous and crystalline HCN at two temperatures, one for interstellar work and one more relevant to the outer solar system. Spectra are presented at both temperatures, along with optical constants that can be used in numerical models. Despite widespread and longstanding interest in and investigations of solid HCN, this is the first time that the properties we are reporting have been measured in a single laboratory, avoiding the need for estimates or to combine results from various authors. We find that our measured band strength of ~1 × 1017 cm molecule1 for the CN vibration of HCN, in both amorphous HCN and in an H2O-rich ice, is substantially higher than an earlier estimate. Unless errors of 100% can be tolerated then our new value requires a rescaling of earlier work. Our results shed light on why HCN and other nitriles have been so difficult to identify in the solid state, in contrast to their many detections in the gas phase.

astrochemistry – methods: laboratory – solid state↗
NASA NTRS2021

Direct Measurements of Infrared Intensities of HCN and H2O + HCN Ices for Laboratory and Observational Astrochemistry

Hydrogen cyanide (HCN) is found in a wide variety of extraterrestrial environments within and beyond the solar system, and for that reason laboratory spectroscopists have studied this compound in many spectral regions, including the infrared (IR). However, one aspect that remains to be investigated is the intrinsic IR spectral intensities of solid HCN as opposed to relative band strengths, intrinsic intensities being needed to measure HCN abundances. Here we report measurements of IR absorption coefficients and band strengths, along with supporting refractive indices and densities, of both amorphous and crystalline HCN at two temperatures, one for interstellar work and one more relevant to the outer solar system. Spectra are presented at both temperatures, along with optical constants that can be used in numerical models. Despite widespread and longstanding interest in and investigations of solid HCN, this is the first time that the properties we are reporting have been measured in a single laboratory, avoiding the need for estimates or to combine results from various authors. We find that our measured band strength of ~1 × 1017 cm molecule1 for the CN vibration of HCN, in both amorphous HCN and in an H2O-rich ice, is substantially higher than an earlier estimate. Unless errors of 100% can be tolerated then our new value requires a rescaling of earlier work. Our results shed light on why HCN and other nitriles have been so difficult to identify in the solid state, in contrast to their many detections in the gas phase.

astrochemistry – methods: laboratory – solid state↗
NASA NTRS2018

The Photochemistry of Purine in Ice Analogs Relevant to Dense Interstellar Clouds

The aromatic nitrogen heterocyclic compound purine is the core structural framework of many important biomolecules, particularly nucleobases. Purine and purine derivatives have been observed in carbonaceous chondrites, and it has been hypothesized that the exogenous delivery of these compounds, along with many other biologically relevant compounds, may have played a role in the emergence of life. Numerous experiments in our laboratory have demonstrated that the nucleobases used by life to encode genetic material could have been produced abiotically under astrophysically relevant conditions. Specifically, the UV photoprocessing of pyrimidine and purine in simple ices of astrophysical interest has resulted in the production of all five biological nucleobases, namely, uracil (RNA), cytosine (RNA and DNA), thymine (DNA), adenine (RNA and DNA), and guanine (RNA and DNA). Additionally, follow-up work has examined the photochemistry of pyrimidine in more complex astrophysical ice mixtures to better understand the formation of these compounds under realistic conditions. In this work, we examine the photochemistry of purine in more complex ices of astrophysical interest and compare our results with those from simpler ice mixtures. We also examine the effects of competing parallel synthesis of organic compounds in the ices (unrelated to purine). Finally, we discuss the astrophysical and astrobiological implications of our findings.

Astrobiology↗
NASA NTRS2022

The Population of Galactic Centre Filaments – III. Candidate Radio and Stellar Sources

Recent MeerKAT radio continuum observations of the Galactic Centre at 20 cm show a large population of non-thermal radio filaments (NRFs) in the inner few hundred pc of the Galaxy. We have selected a sample of 57 radio sources, mainly compact objects, in the MeerKAT mosaic image that appear to be associated with NRFs. The selected sources are about four times the number of radio point sources associated with filaments than would be expected by random chance. Furthermore, an apparent correlation between bright IR stars and NRFs is inferred from their similar latitude distributions, suggesting that they both co-exist within the same region. To examine if compact radio sources are related to compact IR sources, we have used archival 2MASS, and Spitzer data to make spectral energy distribution of individual stellar sources coincident or close to radio sources. We provide a catalogue of radio and IR sources for future detailed observations to investigate a potential three-way physical association between NRFs, compact radio and IR stellar sources. This association is suggested by models in which NRFs are cometary tails produced by the interaction of a large-scale nuclear outflow with stellar wind bubbles in the Galactic Centre.

plasmas↗
NASA NTRS2022

Statistical Properties of the Population of the Galactic Center Filaments II: The Spacing between Filaments

We carry out a population study of magnetized radio filaments in the Galactic centre using MeerKAT data by focusing on the spacing between the filaments that are grouped. The morphology of a sample of 43 groupings containing 174 magnetized radio filaments are presented. Many grouped filaments show harp-like, fragmented cometary tail-like, or loop-like structures in contrast to many straight filaments running mainly perpendicular to the Galactic plane. There are many striking examples of a single filament splitting into two prongs at a junction, suggestive of a flow of plasma along the filaments. Spatial variations in spectral index, brightness, bending, and sharpening along the filaments indicate that they are evolving on a 105−6-yr time-scale. The mean spacings between parallel filaments in a given grouping peaks at ∼16 arcsec. We argue by modeling that the filaments in a grouping all lie on the same plane and that the groupings are isotropically oriented in 3D space. One candidate for the origin of filamentation is interaction with an obstacle, which could be a compact radio source, before a filament splits and bends into multiple filaments. In this picture, the obstacle or sets the length scale of the separation between the filaments. Another possibility is synchrotron cooling instability occurring in cometary tails formed as a result of the interaction of cosmic ray driven Galactic centre outflow with obstacles such as stellar winds. In this picture, the mean spacing and the mean width of the filaments are expected to be a fraction of a parsec, consistent with observed spacing.

plasmas↗
NASA NTRS2024

Soft X-ray Energy Spectra in the Wide-Field Galactic Disk Area Revealed with HaloSat

We analyzed data from HaloSat observations for five fields in the Galactic disk located far away from the Galactic center (135° < l < 254°) to understand the nature of soft X-ray energy emission in the Galactic disk. The fields have 14° diameter and were selected to contain no significant high-flux X-ray sources. All five HaloSat soft X-ray energy spectra (0.4–7 keV with energy resolution of < 100 eV below 1 keV) show a possibility of the presence of unresolved high-temperature plasma in the Galactic disk (UHTPGD) with a temperature of 0.8–1.0 keV and an emission measure of (8–11) × 10 −4 cm −6 pc in addition to the soft X-ray diffuse background components mainly studied at higher Galactic latitudes (solar wind charge exchange emission, Local Hot Bubble, Milky Way halo emission, and the cosmic X-ray background). This suggests that the UHTPGD is present across the whole Galactic disk. We also observed UHTPGD emission in a region with no bright sources in an XMM-Newton field contained within one of the HaloSat fields. The temperature and emission measure are consistent with those measured with HaloSat. Moreover, the stacked spectra of the X-ray pointlike sources and near-infrared-identified point sources such as stars in the XMM-Newton field also show a spectral feature similar to the UHTPGD emission. This suggests that the UHTPGD may partly originate from pointlike sources such as stars.

X-rays: diffuse background↗
NASA NTRS2023

The IAU Recommended Photometric System for Ultraviolet Astronomy

In the current era when access to space is becoming easier and at a lower cost thanks to the standardised cubesat technology, numerous missions are expected to be launched to observe, particularly, at ultraviolet wavelengths. Given the reduced dimensions of the telescope that a cubesat can carry, most of these missions will be focused on photometric surveys of a reduced sample of targets of interest, and therefore each mission will define their own photometric bands according to their scientific objectives and orbital constraints. However, in order to provide a coherent view of the ultraviolet sky, the data should be post-processed under a common framework. In 2017, the IAU working group on ultraviolet astronomy identified the need to define such a common framework for the upcoming ultraviolet missions, and coordinated the definition of a standard set of photometric bands that could serve for homogenizing the current and future data. This paper presents the procedure adopted by the working group for the definition of the standard photometric system, that was approved by the IAU during the General Assembly Business Sessions held in August, 2021. The photometric system consists of seven bands, denoted as UV1-UV7, all included in the range 115 - 400 nm. Some of these bands are based on existing filters, while others have been defined as theoretical bands with constant throughput. This system is to be regarded as a set of synthetic bands for post-processing the data of any mission, and an example of its application to the SPARCS cubesat is also included. The photometric bands are publicly available and can be downloaded from https://www.nuva.eu/uv-photometry/.

Ultraviolet: ISM↗