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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 991 records · Page 55
All sourcesNASA NTRSDOE OSTI
DOE OSTI2013

Agricultural approaches of remediation in the outside of the Fukushima Daiichi nuclear power plant

This paper outlines agricultural approaches of remediation activity done in contaminated areas around the Fukushima Daiichi Nuclear Power Plant. About the decontamination examination of contaminated areas, we have tried the land scale test of a rice field before and after planting by the use of currently recommended methods. Since farmers would carry out the land preparation by themselves, generation of secondary radioactive waste should be as low as possible through the decontamination works. For the radioactive nuclide migration control of rice by wet rice production, several types of decontamination methods such as zeolite addition and potassium fertilization in the soil have been examined. The results are summarized in the 4 following points. 1) Plowing and water discharge are effective for removing radioactive cesium from rice field. 2) Additional potassium fertilization is effective for reducing cesium radioactivity in the product. 3) No significant difference is observed with or without the zeolite addition. 4) Very low transfer factor of cesium from soil to brown rice has been obtained compared with literature values.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗
DOE OSTI2014

Effect of hydrocarbon adsorption on the wettability of rare earth oxide ceramics

Vapor condensation is routinely used as an effective means of transferring heat, with dropwise condensation exhibiting a 5 − 7x heat transfer improvement compared to filmwise condensation. However, state-of-the-art techniques to promote dropwise condensation rely on functional hydrophobic coatings, which are often not robust and therefore undesirable for industrial implementation. Natural surface contamination due to hydrocarbon adsorption, particularly on noble metals, has been explored as an alternative approach to realize stable dropwise condensing surfaces. While noble metals are prohibitively expensive, the recent discovery of robust rare earth oxide (REO) hydrophobicity has generated interest for dropwise condensation applications due to material costs approaching 1% of gold; however, the underlying mechanism of REO hydrophobicity remains under debate. In this work, we show through careful experiments and modeling that REO hydrophobicity occurs due to the same hydrocarbon adsorption mechanism seen previously on noble metals. To investigate adsorption dynamics, we studied holmia and ceria REOs, along with control samples of gold and silica, via X-Ray photoelectron spectroscopy (XPS) and dynamic time-resolved contact angle measurements. The contact angle and surface carbon percent started at ≈0 on in-situ argon-plasma-cleaned samples and increased asymptotically over time after exposure to laboratory air, with the rare earth oxides displaying hydrophobic (>90°) advancing contact angle behavior at long times (>4 days). The results indicate that REOs are in fact hydrophilic when clean and become hydrophobic due to hydrocarbon adsorption. Furthermore, this study provides insight into how REOs can be used to promote stable dropwise condensation, which is important for the development of enhanced phase change surfaces.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2015

The German product quality control of the compacted metallic nuclear waste - 15311

The treatment and safe disposal of spent nuclear fuel is a key challenge of nuclear energy utilization and has to be accomplished regardless the future nuclear of electricity production or phase-out policies. Until June 2005 approx. 6662 tons of spent fuel from German nuclear power plants was sent to the La Hague (France) and Sellafield (UK) plants for reprocessing. An equivalent amount of nuclear waste compounds has contractually to be returned to Germany, which is currently in progress. The returnable waste streams comprise mainly highly-active vitrified waste containing a major part of fission products and actinides, and intermediate-active super-compacted metallic waste containing reprocessed fuel element's structural materials and some technological waste from the reprocessing process itself. Shearing and dissolution of spent fuel leaves scraps of fuel metal cladding, the end-pieces and spacers which are contaminated, activated and irradiating from their life in a reactor core. In fact, this metallic intermediate level radioactive waste makes up a bit more than half of the total volume of the reprocessed waste. At La Hague the metallic waste is super-compacted. Several, typically eight, compacted discs are stacked in a stainless steel container, named CSD-C as for 'Colis Standard de Dechets Compactes'. 4104 containers of such CSD-Cs in 152 transport/storages casks have to be returned to Germany. Each one of them has to be checked and quality certified for its conformity with German national product specifications and acceptance criteria by independent national product quality control inspectors (PKS). The residue package documentation has to be complete and the characterization methods have to be comprehensive. Due to the heterogeneity of metallic waste the characterization and control of its properties is very complex. The nuclear characterization is performed by means of non-destructive measurements, where only a few key nuclides are measured directly. In fact, the proper calculation of the whole nuclear inventory relies on numerous supplementary simulations. The measurement and calculation methodology is scrutinized by PKS in detail and key points are benchmarked with our own simulations for the sake of an independent nuclear inventory declaration check. With respect to the vast amount of documentation and parameters, which have to be checked and verified, PKS had to optimize their checking procedures. For this purpose dedicated proof tools have been developed that shall be applied for selected indicative cross-checks of the relevant parameters. This contribution is dedicated to the procedure of quality control by PKS and examples of actually performed computational verifications of declared nuclear inventory. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
DOE OSTI2014

First scientific application of the membrane cryostat technology

We report on the design, fabrication, performance and commissioning of the first membrane cryostat to be used for scientific application. The Long Baseline Neutrino Experiment (LBNE) has designed and fabricated a membrane cryostat prototype in collaboration with IHI Corporation (IHI). Original goals of the prototype are: to demonstrate the membrane cryostat technology in terms of thermal performance, feasibility for liquid argon, and leak tightness; to demonstrate that we can remove all the impurities from the vessel and achieve the purity requirements in a membrane cryostat without evacuation and using only a controlled gaseous argon purge; to demonstrate that we can achieve and maintain the purity requirements of the liquid argon during filling, purification, and maintenance mode using mole sieve and copper filters from the Liquid Argon Purity Demonstrator (LAPD) R and D project. The purity requirements of a large liquid argon detector such as LBNE are contaminants below 200 parts per trillion oxygen equivalent. This paper gives the requirements, design, construction, and performance of the LBNE membrane cryostat prototype, with experience and results important to the development of the LBNE detector.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2013

Atomic layer deposition of TiN for the fabrication of nanomechanical resonators

Films of titanium nitride were grown by atomic layer deposition (ALD) over a range of temperatures from 120 Degree-Sign C to 300 Degree-Sign C, and their deposition rates were characterized by ellipsometry and reflectometry. The stress state of the films was evaluated by interferometry using a wafer bowing technique and varied from compressive (-18 MPa) to tensile (650 MPa). The crystal structure of the films was assessed by x-ray diffraction. The grain size varied with temperature in the range of 2-9 nm. The chemical composition of the films was ascertained by high-resolution x-ray photoelectron spectroscopy and showed the presence of O, Cl, and C contaminants. A mildly tensile (250 MPa) stressed film was employed for the fabrication (by electron beam lithography and reactive ion etching) of doubly clamped nanoresonator beams. The resonance frequency of resonators was assayed using an interferometric resonance testing apparatus. The devices exhibited sharp mechanical resonance peaks in the 17-25 MHz range. The uniformity and controllable deposition rate of ALD films make them ideal candidate materials for the fabrication of ultranarrow (<50 nm) nanobeam structures.

36 MATERIALS SCIENCE↗
DOE OSTI2017

2016 Groundwater Monitoring and Inspection Report Gnome-Coach, New Mexico, Site January 2017

The Gnome-Coach, New Mexico, Site was the location of an underground nuclear test in 1961 and a groundwater tracer test in 1963. Residual contamination remaining in the subsurface from these events requires long-term oversight. The Long-Term Surveillance and Maintenance Plan for the site describes the U.S. Department of Energy Office of Legacy Management’s (LM’s) plan for monitoring groundwater (radiochemical sampling and hydraulic head measurements), inspecting the site, maintaining the site’s institutional controls, evaluating and reporting data, and documenting the site’s records and data management processes. Groundwater monitoring and site inspection activities are conducted annually. This report summarizes the results of these activities conducted during the October 2015 through September 2016 reporting period. The site inspection and annual sampling were conducted on January 27, 2016. At the time of the site inspection, the signs installed near the emplacement shaft, near well USGS-1, and around the perimeter of the site were observed as being in good condition, as were the roads, wellheads, and Project Gnome monument. No new groundwater extraction wells or oil and gas wells were installed during this reporting period on the site or in the sections that surround the site. One new application was received by the New Mexico Oil Conservation Division to install a salt water disposal well approximately 0.8 miles northeast of the Project Gnome monument. The proposed well has a planned completion depth of 15,500 feet below ground surface, but as of November 2016 a drill date has not been established.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Next Generation Logistics Systems for Delivering Optimal Biomass Feedstocks to Biorefining Industries in the Southeastern U.S.

The diverse portfolio of biomass sources that is available in the Southeastern U.S., including a significant supply of pine “residue”, represents a valuable strategic position for the region. Through blends formulated based on critical properties, this project will take full advantage of the range in biomass properties afforded by the portfolio to produce a consistent, high-performance feedstock for the industry, while lowering cost. Key developments being targeted to enable this potential include whole-tree transport to a state-of-the-art merchandising depot that will further access biomass from ongoing, forest industry operations. The approach will more effectively utilize the tree and distribute cost, while minimizing in-woods contamination of the woody biomass component. To implement this vision, information on the chemical composition and changes that are induced during multiple preprocessing steps (size reduction, moisture removal, densification, etc.) is needed. New NIR sensor technology will be developed for online monitoring of important biomass properties. The data will be incorporated into a statistical process control platform to improve process efficiency and meet required specifications. Advanced process models are being developed to inform the techno-economic and life-cycle assessment of the program’s impact. The new system will ultimately reduce operational risks from supply chain disruptions, and allow operation of larger-scale biorefineries.

09 BIOMASS FUELS↗
DOE OSTI2019

Development of a Standard Test Method for Reducing the Uncertainties in Measuring the Capture Efficiency of Range Hoods

Cooking activities are a major source of indoor air pollutants. To control pollutants generated from cooking activities, a range hood is commonly used in residential kitchens. Several building codes require that a range hood be installed in new homes to control pollutants from cooking, and the required airflow rates for range hoods are specified by indoor air quality (IAQ) standards. However, air flow alone does not tell us how much of the cooking pollutants are exhausted by the range hood. A better metric to evaluate range hood IAQ performance is capture efficiency (CE)—the fraction of contaminants emitted during cooking that are exhausted directly to the outside via the range hood. This paper summarizes the development of a range hood CE test method for use in laboratory testing and equipment rating.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗
DOE OSTI2019

Environmentally significant shifts in trace element emissions from coal plants complying with the 1990 Clean Air Act Amendments

The Clean Air Act Amendments of 1990 (CAAAs) reduced criteria air pollution from coal-fired power plants (CFPPs) in the United States, but compliance strategies additionally altered the magnitude and phase of environmentally significant trace element emissions. This report quantitatively assesses changes in trace element emissions stemming from CAAAs compliance, attributes these changes to specific CAAAs compliance strategies, and discusses implications for future environmental regulatory design. We combine plant-level coal purchase and installed air pollution control device data with a trace element partitioning model to approximate changes in trace element mass entering and exiting CFPPs in the solid, liquid, and gas phase between 1993 and 2017. Though US coal combustion decreased by 2% during this period, the vast majority of trace element emissions reductions stem from the 18-64% reductions in the fleet-wide average concentrations of arsenic, bromine, chloride, lead, mercury, and selenium in the combusted coal. Combined with the installation of air pollution control technologies, these shifts concluded in nationwide reductions of gas phase trace element emissions by between 49 and 68% for the elements included in this study. In contrast, installation of flue gas desulfurization devices increased the mass of trace elements discharged in wastewater. This work reinforces the value of multi-phase emissions regulations in ensuring that contaminants are not shunted from regulated to unregulated phases.

29 ENERGY PLANNING, POLICY, AND ECONOMY↗
DOE OSTI2013

Oxidative DNA damage and repair in children exposed to low levels of arsenic in utero and during early childhood: Application of salivary and urinary biomarkers

The present study aimed to assess arsenic exposure and its effect on oxidative DNA damage and repair in young children exposed in utero and continued to live in arsenic-contaminated areas. To address the need for biological specimens that can be acquired with minimal discomfort to children, we used non-invasive urinary and salivary-based assays for assessing arsenic exposure and early biological effects that have potentially serious health implications. Levels of arsenic in nails showed the greatest magnitude of difference between exposed and control groups, followed by arsenic concentrations in saliva and urine. Arsenic levels in saliva showed significant positive correlations with other biomarkers of arsenic exposure, including arsenic accumulation in nails (r = 0.56, P < 0.001) and arsenic concentration in urine (r = 0.50, P < 0.05). Exposed children had a significant reduction in arsenic methylation capacity indicated by decreased primary methylation index and secondary methylation index in both urine and saliva samples. Levels of salivary 8-OHdG in exposed children were significantly higher (∼ 4-fold, P < 0.01), whereas levels of urinary 8-OHdG excretion and salivary hOGG1 expression were significantly lower in exposed children (∼ 3-fold, P < 0.05), suggesting a defect in hOGG1 that resulted in ineffective cleavage of 8-OHdG. Multiple regression analysis results showed that levels of inorganic arsenic (iAs) in saliva and urine had a significant positive association with salivary 8-OHdG and a significant negative association with salivary hOGG1 expression. - Highlights: • The effects of arsenic exposure in utero and through early childhood were studied. • Arsenic-exposed children had a reduction in arsenic methylation capacity. • Exposed children had more DNA damage, observed as elevated salivary 8-OHdG. • Lower salivary hOGG1 in exposed children indicated impairment of 8-OHdG repair. • Salivary and urinary 8-OHdG levels were discordant.

60 APPLIED LIFE SCIENCES↗
DOE OSTI2022

Promise of nonthermal plasmas in addressing emerging environmental and health problems: Present and future

Nonthermal atmospheric pressure plasmas transform input electrical energy efficiently into reactive species, charged particles, and photons. This “activated gas” is being investigated as solutions for a range of environmental and health problems facing society today. In this Perspective, we take a cursory look at a few of these societal problems and the reflected role that plasmas may play in charting the pathway to a solution buoyed by supporting research. Here, we survey the plasma-based opportunities in the removal of trace contaminants in water supporting methodologies such as water reuse, which addresses scarcity and pollution, the opportunity posed by plasmas-based chemical depolymerization for plastics recycling, and the application of plasmas for food security, which includes sterilization of foodstuffs and the improvement of crop yield. Finally, we also included a short review on how plasmas may help control disease spread. In each case, the scope of the problem is presented along with the potential plasma-based solution.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2017

Reliable SOFC Systems

The goal of this U.S. Department of Energy (DOE) sponsored project was to advance the reliability, robustness and endurance of low-cost SOFC technology suitable for ultimate deployment in ≥100 MWe Integrated Gasification Fuel Cell (IGFC) or Natural Gas Fuel Cell (NGFC) systems capable of ≥97% CO2 capture. The ultimate SOFC program goals are ≤ 0.2% per 1000 hours power degradation over a 5-plus year stack life, high-volume (≥ 250 MW/year) stack production cost of ≤$225/kWsystem net AC, and “power block” (exclusive of fuel supply, contaminant removal, and CO2 capture subsystems) capital cost of ≤ 900/kWsystem net AC (in year 2011). To progress towards the ultimate program goals, the specific objectives of this project were to achieve an SOFC stack power degradation rate of ≤1.5% per 1000 hours in a 100 kW (125 kW Peak) Modular Power Block (MPB) stand-alone power system under thermally self-sustained normal operating conditions and to verify the prospects for high volume SOFC stack production cost below the DOE target of ≤ 225/kW. This final technical report summarizes the progress made during the project period of 36 months. Significant progress was made in the areas of cell and stack technology development, Modular Power Block (MPB) development, sub-MW MPB system development, and MW-class SOFC System Development and Costing. The work focused on areas necessary for comprehensive development of an SOFC fuel cell system, including, active cell improvement, contaminant resistance, process engineering, and development of non-repeat module components. Additionally, several custom built balance-of-plant components were designed and fabricated to support the fuel cell system. SOFC cell and stack development focused on improving cell performance and durability. Enhancements were achieved in areas of electrode stability and impurity tolerance. Additionally, several quality control techniques and tools were developed to ensure predictable and repeatable fabrication of SOFC stacks. Module development continued previous development efforts to achieve footprint reduction and higher efficiency by incorporating balance-of-plant functional equipment into the fuel cell containment module. Several improvements were made to prior design. Control and instrumentation hardware was integrated within the module for serviceability and size reduction. The design efforts culminated in a complete SOFC power plant system. The designed plant was constructed and tested at FCE. Stack and system costs were updated, reflecting advances made in this program.

20 FOSSIL-FUELED POWER PLANTS↗
DOE OSTI2016

Bioaccumulation and elimination of mercury in juvenile seabass (Dicentrarchus labrax) in a warmer environment

Warming is an expected impact of climate change that will affect coastal areas in the future. These areas are also subjected to strong anthropogenic pressures leading to chemical contamination. Yet, the consequences of both factors for marine ecosystems, biota and consumers are still unknown. The present work aims to investigate, for the first time, the effect of temperature increase on bioaccumulation and elimination of mercury [(total mercury (THg) and methylmercury (MeHg)] in three tissues (muscle, liver, and brain) of a commercially important seafood species – European seabass (Dicentrarchus labrax). Fish were exposed to the ambient temperature currently used in seabass rearing (18 °C) and to the expected ocean warming (+4 °C, i.e. 22 °C), as well as dietary MeHg during 28 days, followed by a depuration period of 28 days fed with a control diet. In both temperature exposures, higher MeHg contents were observed in the brain, followed by the muscle and liver. Liver registered the highest elimination percentages (EF; up to 64% in the liver, 20% in the brain, and 3% in the muscle). Overall, the results clearly indicate that a warming environment promotes MeHg bioaccumulation in all tissues (e.g. highest levels in brain: 8.1 mg kg{sup −1} ww at 22 °C against 6.2 mg kg{sup −1} ww at 18 °C after 28 days of MeHg exposure) and hampers MeHg elimination (e.g. liver EF decreases after 28 days of depuration: from 64.2% at 18 °C to 50.3% at 22 °C). These findings suggest that seafood safety may be compromised in a warming context, particularly for seafood species with contaminant concentrations close to the current regulatory levels. Hence, results point out the need to strengthen research in this area and to revise and/or adapt the current recommendations regarding human exposure to chemical contaminants through seafood consumption, in order to integrate the expected effects of climate change. - Highlights: • Higher MeHg contents were found in the brain, followed by the muscle and liver. • A warmer environment enhances MeHg bioaccumulation and hampers MeHg elimination. • Ocean warming may compromise seafood safety. • Research combining climate change and pollution effects should be strengthened.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2014

Nature of Nano-Sized Plutonium Particles in Soils at the Hanford Site

The occurrence of plutonium dioxide (PuO2) either from direct deposition or from the precipitation of plutonium-bearing solutions in contaminated soils and sediments has been well described, particularly for the Hanford site in Washington State. However, past research has suggested that plutonium may exist in environmental samples at the Hanford site in chemical forms in addition to large size PuO2 particles and that these previously unidentified nano-sized particles maybe more reactive and thus more likely to influence the environmental mobility of Pu. Here we present evidence for the formation of nano-sized plutonium iron phosphate hydroxide structurally related to the rhabdophane group nanoparticles in 216-Z9 crib sediments from Hanford using transmission electron microscopy (TEM). The distribution and nature of these nanoparticles varied depending on the adjacent phases present. Fine electron probes were used to obtain electron diffraction and electron energy-loss spectra from specific phase regions of the 216-Z9 cribs specimens from fine-grained plutonium oxide and phosphate phases. Energy-loss spectra were used to evaluate the plutonium N4,5 (4d → 5f ) and iron L2,3 absorption edges. The iron plutonium phosphate formation may depend on the local micro-environment in the sediments, availability of phosphate, and hence the distribution of these minerals may control long-term migration of Pu in the soil. This study also points to the utility of using electron beam methods for determining the identity of actinide phases and their association with other sediment phases.

Cribs, Soil Contamination↗
DOE OSTI2014

A compact ultra-clean system for deploying radioactive sources inside the KamLAND detector

We describe a compact, ultra-clean device used to deploy radioactive sources along the vertical axis of the KamLAND liquid-scintillator neutrino detector for purposes of calibration. The device worked by paying out and reeling in precise lengths of a hanging, small-gauge wire rope (cable); an assortment of interchangeable radioactive sources could be attached to a weight at the end of the cable. All components exposed to the radiopure liquid scintillator were made of chemically compatible UHV-cleaned materials, primarily stainless steel, in order to avoid contaminating or degrading the scintillator. To prevent radon intrusion, the apparatus was enclosed in a hermetically sealed housing inside a glove box, and both volumes were regularly flushed with purified nitrogen gas. Finally, an infrared camera attached to the side of the housing permitted real-time visual monitoring of the cable’s motion, and the system was controlled via a graphical user interface.

42 ENGINEERING↗
DOE OSTI2018

Exploring cosmic origins with CORE: Survey requirements and mission design

Future observations of cosmic microwave background (CMB) polarisation have the potential to answer some of the most fundamental questions of modern physics and cosmology, including: what physical process gave birth to the Universe we see today? What are the dark matter and dark energy that seem to constitute 95% of the energy density of the Universe? Do we need extensions to the standard model of particle physics and fundamental interactions? Is the ΛCDM cosmological scenario correct, or are we missing an essential piece of the puzzle? In this paper, we list the requirements for a future CMB polarisation survey addressing these scientific objectives, and discuss the design drivers of the COREmfive space mission proposed to ESA in answer to the "M5" call for a medium-sized mission. The rationale and options, and the methodologies used to assess the mission's performance, are of interest to other future CMB mission design studies. COREmfive has 19 frequency channels, distributed over a broad frequency range, spanning the 60–600 GHz interval, to control astrophysical foreground emission. The angular resolution ranges from 2' to 18', and the aggregate CMB sensitivity is about 2 μK∙arcmin. The observations are made with a single integrated focal-plane instrument, consisting of an array of 2100 cryogenically-cooled, linearly-polarised detectors at the focus of a 1.2-m aperture cross-Dragone telescope. The mission is designed to minimise all sources of systematic effects, which must be controlled so that no more than 10 -4 of the intensity leaks into polarisation maps, and no more than about 1% of E-type polarisation leaks into B-type modes. COREmfive observes the sky from a large Lissajous orbit around the Sun-Earth L2 point on an orbit that offers stable observing conditions and avoids contamination from sidelobe pick-up of stray radiation originating from the Sun, Earth, and Moon. The entire sky is observed repeatedly during four years of continuous scanning, with a combination of three rotations of the spacecraft over different timescales. With about 50% of the sky covered every few days, this scan strategy provides the mitigation of systematic effects and the internal redundancy that are needed to convincingly extract the primordial B-mode signal on large angular scales, and check with adequate sensitivity the consistency of the observations in several independent data subsets. COREmfive is designed as a "near-ultimate" CMB polarisation mission which, for optimal complementarity with ground-based observations, will perform the observations that are known to be essential to CMB polarisation science and cannot be obtained by any other means than a dedicated space mission. It will provide well-characterised, highly-redundant multi-frequency observations of polarisation at all the scales where foreground emission and cosmic variance dominate the final uncertainty for obtaining precision CMB science, as well as 2' angular resolution maps of high-frequency foreground emission in the 300–600 GHz frequency range, essential for complementarity with future ground-based observations with large telescopes that can observe the CMB with the same beamsize.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

Fuel Flexibility: Landfill Gas Contaminant Mitigation for Power Generation

This research project focused on the mitigation of silica damage to engine-based renewable landfill gas energy systems. Characterization of the landfill gas siloxane contamination, combined with characterization of the silica deposits in engines, led to development of two new mitigation strategies. The first involved a novel method for removing the siloxanes and other heavy contaminants from the landfill gas prior to use by the engines. The second strategy sought to interrupt the formation of hard silica deposits in the engine itself, based on inspection of failed landfill gas engine parts. In addition to mitigation, the project had a third task to develop a robust sensor for siloxanes that could be used to control existing and/or future removal processes.

CHP↗