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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 991 records · Page 55
All sourcesNASA NTRSDOE OSTI
DOE OSTI2015

Temperature-induced sign change of the magnetic interlayer coupling in Ni/Ni{sub 25}Mn{sub 75}/Ni trilayers on Cu{sub 3}Au(001)

We investigated the magnetic interlayer coupling between two ferromagnetic (FM) Ni layers through an antiferromagnetic (AFM) Ni{sub 25}Mn{sub 75} layer and the influence of this coupling on the exchange bias phenomenon. The interlayer coupling energy of an epitaxial trilayer of 14 atomic monolayers (ML) Ni/45 ML Ni{sub 25}Mn{sub 75}/16 ML Ni on Cu{sub 3}Au(001) was extracted from minor-loop magnetization measurements using in-situ magneto-optical Kerr effect. The interlayer coupling changes from ferromagnetic to antiferromagnetic when the temperature is increased above 300 K. This sign change is interpreted as the result of the competition between an antiparallel Ruderman-Kittel-Kasuya-Yosida (RKKY)-type interlayer coupling, which dominates at high temperature, and a stronger direct exchange coupling across the AFM layer, which is present only below the Néel temperature of the AFM layer.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2015

Resonance hybridization and near field properties of strongly coupled plasmonic ring dimer-rod nanosystem

Combined effects of polarization, split gap, and rod width on the resonance hybridization and near field properties of strongly coupled gold dimer-rod nanosystem are comparatively investigated in the light of the constituent nanostructures. By aligning polarization of the incident light parallel to the long axis of the nanorod, introducing small split gaps to the dimer walls, and varying width of the nanorod, we have simultaneously achieved resonance mode coupling, huge near field enhancement, and prolonged plasmon lifetime. As a result of strong coupling between the nanostructures and due to an intense confinement of near fields at the split and dimer-rod gaps, the extinction spectrum of the coupled nanosystem shows an increase in intensity and blueshift in wavelength. Consequently, the near field lifespan of the split-nanosystem is prolonged in contrast to the constituent nanostructures and unsplit-nanosystem. On the other hand, for polarization of the light perpendicular to the long axis of the nanorod, the effect of split gap on the optical responses of the coupled nanosystem is found to be insignificant compared to the parallel polarization. These findings and such geometries suggest that coupling an array of metallic split-ring dimer with long nanorod can resolve the huge radiative loss problem of plasmonic waveguide. In addition, the Fano-like resonances and immense near field enhancements at the split and dimer-rod gaps imply the potentials of the nanosystem for practical applications in localized surface plasmon resonance spectroscopy and sensing.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2015

Plasmon-enhanced electron-phonon coupling in Dirac surface states of the thin-film topological insulator Bi{sub 2}Se{sub 3}

Raman measurements of a Fano-type surface phonon mode associated with Dirac surface states (SS) in Bi{sub 2}Se{sub 3} topological insulator thin films allowed an unambiguous determination of the electron-phonon coupling strength in Dirac SS as a function of film thickness ranging from 2 to 40 nm. A non-monotonic enhancement of the electron-phonon coupling strength with maximum for the 8–10 nm thick films was observed. The non-monotonicity is suggested to originate from plasmon-phonon coupling which enhances electron-phonon coupling when free carrier density in Dirac SS increases with decreasing film thickness and becomes suppressed for thinnest films when anharmonic coupling between in-plane and out-of-plane phonon modes occurs. The observed about four-fold enhancement of electron-phonon coupling in Dirac SS of the 8–10 nm thick Bi{sub 2}Se{sub 3} films with respect to the bulk samples may provide new insights into the origin of superconductivity in this-type materials and their applications.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2016

Towards achieving strong coupling in three-dimensional-cavity with solid state spin resonance

We investigate the microwave magnetic field confinement in several microwave three-dimensional (3D)-cavities, using a 3D finite-element analysis to determine the best design and achieve a strong coupling between microwave resonant cavity photons and solid state spins. Specifically, we design cavities for achieving strong coupling of electromagnetic modes with an ensemble of nitrogen vacancy (NV) defects in diamond. We report here a novel and practical cavity design with a magnetic filling factor of up to 4 times (2 times higher collective coupling) than previously achieved using one-dimensional superconducting cavities with a small mode volume. In addition, we show that by using a double-split resonator cavity, it is possible to achieve up to 200 times better cooperative factor than the currently demonstrated with NV in diamond. These designs open up further opportunities for studying strong and ultra-strong coupling effects on spins in solids using alternative systems with a wider range of design parameters. The strong coupling of paramagnetic spin defects with a photonic cavity is used in quantum computer architecture, to interface electrons spins with photons, facilitating their read-out and processing of quantum information. To achieve this, the combination of collective coupling of spins and cavity mode is more feasible and offers a promising method. This is a relevant milestone to develop advanced quantum technology and to test fundamental physics principles.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2016

Study of the effect of loop inductance on the RF transmission line to cavity coupling coefficient

Coupling of RF power is an important aspect in the design and development of RF accelerating structures. RF power coupling employing coupler loops has the advantage of tunability of β, the transmission line to cavity coupling coefficient. Analytical expressions available in literature for determination of size of the coupler loop using Faraday’s law of induction show reasonably good agreement with experimentally measured values of β below critical coupling (β ≤ 1) but show large deviation with experimentally measured values and predictions by simulations for higher values of β. In actual accelerator application, many RF cavities need to be over-coupled with β > 1 for reasons of beam loading compensation, reduction of cavity filling time, etc. This paper discusses a modified analytical formulation by including the effect of loop inductance in the determination of loop size for any desired coupling coefficient. The analytical formulation shows good agreement with 3D simulations and with experimentally measured values. It has been successfully qualified by the design and development of power coupler loops for two 476 MHz pre-buncher RF cavities, which have successfully been conditioned at rated power levels using these coupler loops.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2020

A coupled cluster framework for electrons and phonons

Here, we describe a coupled cluster framework for coupled systems of electrons and harmonic phonons. Neutral and charged excitations are accessed via the equation-of-motion version of the theory. Benchmarks on the Hubbard–Holstein model allow us to assess the strengths and weaknesses of different coupled cluster approximations, which generally perform well for weak to moderate coupling. Finally, we report progress toward an implementation for ab initio calculations on solids and present some preliminary results on finite-size models of diamond with a linear electron–phonon coupling. We also report the implementation of electron–phonon coupling matrix elements from crystalline Gaussian type orbitals within the PySCF program package.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2021

Vibronic coupling in energy transfer dynamics and two-dimensional electronic–vibrational spectra

We introduce a heterodimer model in which multiple mechanisms of vibronic coupling and their impact on energy transfer can be explicitly studied. We consider vibronic coupling that arises through either Franck-Condon activity in which each site in the heterodimer has a local electron-phonon coupling or Herzberg-Teller activity in which the transition dipole moment coupling the sites has an explicit vibrational mode-dependence. We have computed two-dimensional electronic-vibrational (2DEV) spectra for this model while varying the magnitude of these two effects and find that 2DEV spectra contain static and dynamic signatures of both types of vibronic coupling. Franck-Condon activity emerges through a change in the observed excitonic structure, while Herzberg-Teller activity is evident in the appearance of significant side-band transitions that mimic the lower-energy excitonic structure. A comparison of quantum beating patterns obtained from analysis of the simulated 2DEV spectra shows that this technique can report on the mechanism of energy transfer, elucidating a means of experimentally determining the role of specific vibronic coupling mechanisms in such processes.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2023

Spin–phonon interactions and magnetoelectric coupling in Co 4 B 2 O 9 ( B = Nb, Ta)

In order to explore the consequences of spin–orbit coupling on spin–phonon interactions in a set of chemically similar mixed metal oxides, we measured the infrared vibrational properties of Co 4 B 2 O 9 (B = Nb, Ta) as a function of temperature and compared our findings with lattice dynamics calculations and several different models of spin–phonon coupling. Frequency vs temperature trends for the Co 2+ shearing mode near 150 cm –1 reveal significant shifts across the magnetic ordering temperature that are especially large in relative terms. Bringing these results together and accounting for noncollinearity, we obtain spin–phonon coupling constants of –3.4 and –4.3 cm –1 for Co 4 Nb 2 O 9 and the Ta analog, respectively. Analysis reveals that these coupling constants are derived from interlayer (rather than intralayer) exchange interactions and that the interlayer interactions contain competing antiferromagnetic and ferromagnetic contributions. At the same time, beyond-Heisenberg terms are minimized due to fortuitous symmetry considerations, different from most other 4d- and 5d-containing oxides. Comparison with other contemporary oxides shows that spin–phonon coupling in this family of materials is among the strongest ever reported, suggesting an origin for magnetoelectric coupling.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2011

COSMOLOGY OF CHAMELEONS WITH POWER-LAW COUPLINGS

In chameleon field theories, a scalar field can couple to matter with gravitational strength and still evade local gravity constraints due to a combination of self-interactions and the couplings to matter. Originally, these theories were proposed with a constant coupling to matter; however, the chameleon mechanism also extends to the case where the coupling becomes field dependent. We study the cosmology of chameleon models with power-law couplings and power-law potentials. It is found that these generalized chameleons, when viable, have a background expansion very close to {Lambda}CDM, but can in some special cases enhance the growth of the linear perturbations at low redshifts. For the models we consider, it is found that this region of the parameter space is ruled out by local gravity constraints. Imposing a coupling to dark matter only, the local constraints are avoided, and it is possible to have observable signatures on the linear matter perturbations.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2022

Nonlinear harmonics coupled by parallel wave propagations in a time-dependent plasma flow

In a time-dependent flow, nonlinear harmonics can be excited by coupling between linear waves and flow-induced harmonic waves. Examining the dispersion relations and selection rules for the coupling, we investigate nonlinearly coupled harmonics for waves propagating along the magnetic field line in a magnetized plasma, as well as waves in an unmagnetized plasma. The coupled harmonics in a plasma flow are described by analytic dispersion relations and selection rules. This nonlinear coupling is corroborated by the particle-in-cell simulation. Here, the coupled-harmonics model describes a mechanism for the excitation of nonlinear harmonics from linear waves in a time-dependent flow. The spectral analysis of the dispersion relation provides a useful way to evaluate the spatiotemporal behavior of a plasma flow.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2012

Reconstruction of a nonminimal coupling theory with scale-invariant power spectrum

A nonminimal coupling single scalar field theory, when transformed from Jordan frame to Einstein frame, can act like a minimal coupling one. Making use of this property, we investigate how a nonminimal coupling theory with scale-invariant power spectrum could be reconstructed from its minimal coupling counterpart, which can be applied in the early universe. Thanks to the coupling to gravity, the equation of state of our universe for a scale-invariant power spectrum can be relaxed, and the relation between the parameters in the action can be obtained. This approach also provides a means to address the Big-Bang puzzles and anisotropy problem in the nonminimal coupling model within Jordan frame. Due to the equivalence between the two frames, one may be able to find models that are free of the horizon, flatness, singularity as well as anisotropy problems.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2024

Controlling magnon-photon coupling in a planar geometry

Abstract The tunability of magnons enables their interaction with various other quantum excitations, including photons, paving the route for novel hybrid quantum systems. Here, we study magnon-photon coupling using a high-quality factor split-ring resonator and single-crystal yttrium iron garnet (YIG) sphere at room temperature. We investigate the dependence of the coupling strength on the size of the sphere and find that the coupling is stronger for spheres with a larger diameter as predicted by theory. Furthermore, we demonstrate strong magnon-photon coupling by varying the position of the YIG sphere within the resonator. Our experimental results reveal the expected correlation between the coupling strength and the rf magnetic field. These findings demonstrate the control of coherent magnon-photon coupling through the theoretically predicted square-root dependence on the spin density in the ferromagnetic medium and the magnetic dipolar interaction in a planar resonator.

36 MATERIALS SCIENCE↗
DOE OSTI2026

Coupling of Klein-Andreev resonant states in B⁢i 2 ⁢S⁢r 2 ⁢CaC⁢u 2 ⁢O 8+𝑥 -graphene-B⁢i 2⁢ S⁢r 2 ⁢CaC⁢u 2 ⁢O 8+𝑥 devices

Quantum devices require coherent coupling over macroscopic distances. Recently, resonances due to Klein tunneling and Andreev reflection states (KARS) have been observed in a naturally occurring p-n junction at the interface between B⁢i 2 ⁢S⁢r 2 ⁢CaC⁢u 2 ⁢O 8+𝑥 (BSCCO), a high−⁢𝑇 c superconductor (HTS), and graphene. The resonances appear as conductance oscillations with gating. Here, in this study, we show coupling between the KARS in BSCCO-graphene-BSCCO devices of varying separation (L). The coupling is evidenced by a power-law decay of resonance period as L increases from tens of nanometers to microns. These results demonstrate the long-distance coupling of KARS cavities in graphene-HTS junctions. The length dependence seen in experiments is supported by single-particle spectral functions which show KARS are coupled by transport modes in graphene. The strong coupling between KARS in BSCCO-graphene-BSCCO devices showcases the possibility of HTS-graphene junctions for quantum circuits and unconventional Josephson junctions.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2010

Qubit-oscillator system: An analytical treatment of the ultrastrong coupling regime

We examine a two-level system coupled to a quantum oscillator, typically representing experiments in cavity and circuit quantum electrodynamics. We show how such a system can be treated analytically in the ultrastrong coupling limit, where the ratio g/{Omega} between coupling strength and oscillator frequency approaches unity and goes beyond. In this regime the Jaynes-Cummings model is known to fail because counter-rotating terms have to be taken into account. By using Van Vleck perturbation theory to higher orders in the qubit tunneling matrix element {Delta} we are able to enlarge the regime of applicability of existing analytical treatments, including, in particular, also the finite-bias case. We present a detailed discussion on the energy spectrum of the system and on the dynamics of the qubit for an oscillator at low temperature. We consider the coupling strength g to all orders, and the validity of our approach is even enhanced in the ultrastrong coupling regime. Looking at the Fourier spectrum of the population difference, we find that many frequencies contribute to the dynamics. They are gathered into groups whose spacing depends on the qubit-oscillator detuning. Furthermore, the dynamics is not governed anymore by a vacuum Rabi splitting which scales linearly with g, but by a nontrivial dressing of the tunneling matrix element, which can be used to suppress specific frequencies through a variation of the coupling.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2011

Efficiency for preforming molecules from mixtures of light Fermi and heavy Bose atoms in optical lattices: The strong-coupling-expansion method

We discuss the application of a strong-coupling expansion (perturbation theory in the hopping) for studying light-Fermi-heavy-Bose (like {sup 40}K-{sup 87}Rb) mixtures in optical lattices. We use the strong-coupling method to evaluate the efficiency for preforming molecules, the entropy per particle, and the thermal fluctuations. We show that within the strong interaction regime (and at high temperature), the strong-coupling expansion is an economical way to study this problem. In some cases, it remains valid even down to low temperatures. Because the computational effort is minimal, the strong-coupling approach allows us to work with much larger system sizes, where boundary effects can be eliminated, which is particularly important at higher temperatures. Since the strong-coupling approach is so efficient and accurate, it allows one to rapidly scan through parameter space in order to optimize the preforming of molecules on a lattice (by choosing the lattice depth and interspecies attraction). Based on the strong-coupling calculations, we test the thermometry scheme based on the fluctuation-dissipation theorem and find the scheme gives accurate temperature estimation even at very low temperature. We believe this approach and the calculation results will be useful in the design of the next generation of experiments and will hopefully lead to the ability to form dipolar matter in the quantum degenerate regime.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2011

Quantum thermalization of two coupled two-level systems in eigenstate and bare-state representations

We study analytically the quantum thermalization of two coupled two-level systems (TLSs), which are connected with either two independent heat baths (IHBs) or a common heat bath (CHB). We understand the quantum thermalization in eigenstate and bare-state representations when the coupling between the two TLSs is stronger and weaker than the TLS-bath couplings, respectively. In the IHB case, we find that, when the two IHBs have the same temperatures, the two coupled TLSs in eigenstate representation can be thermalized with the same temperature as those of the IHBs. However, in the case of two IHBs at different temperatures, just when the energy detuning between the two TLSs satisfies a special condition, the two coupled TLSs in eigenstate representation can be thermalized with an immediate temperature between those of the two IHBs. In bare-state representation, we find a counterintuitive phenomenon that, under some conditions, the temperature of the TLS connected with the high-temperature bath is lower than that of the other TLS, which is connected with the low-temperature bath. In the CHB case, the coupled TLSs in eigenstate representation can be thermalized with the same temperature as that of the CHB in nonresonant cases. In bare-state representation, the TLS with a larger energy separation can be thermalized to a thermal equilibrium with a lower temperature. In the resonant case, we find a phenomenon of antithermalization. We also study the steady-state entanglement between the two TLSs in both the IHB and CHB cases.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2011

Continuous control of light group velocity from subluminal to superluminal propagation with a standing-wave coupling field in a Rb vapor cell

We present the continuous control of the light group velocity from subluminal to superluminal propagation with an on-resonant standing-wave coupling field in the 5S{sub 1/2}-5P{sub 1/2} transition of the {Lambda}-type system of {sup 87}Rb atoms. When a coupling field was changed from a traveling-wave to a standing-wave field by adjusting the power of a counterpropagating coupling field, the probe pulse propagation continuously transformed from subluminal propagation, due to electromagnetically induced transparency with the traveling-wave coupling field, to superluminal propagation, due to narrow enhanced absorption with the standing-wave coupling field. The group velocity of the probe pulse was measured to be approximately 0.004c to -0.002c as a function of the disparity between the powers of the copropagating and the counterpropagating coupling fields.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2011

Optimized coupling of cold atoms into a fiber using a blue-detuned hollow-beam funnel

We theoretically investigate the process of coupling cold atoms into the core of a hollow-core photonic-crystal optical fiber using a blue-detuned Laguerre-Gaussian beam. In contrast to the use of a red-detuned Gaussian beam to couple the atoms, the blue-detuned hollow beam can confine cold atoms to the darkest regions of the beam, thereby minimizing shifts in the internal states and making the guide highly robust to heating effects. This single optical beam is used as both a funnel and a guide to maximize the number of atoms into the fiber. In the proposed experiment, Rb atoms are loaded into a magneto-optical trap (MOT) above a vertically oriented optical fiber. We observe a gravito-optical trapping effect for atoms with high orbital momentum around the trap axis, which prevents atoms from coupling to the fiber: these atoms lack the kinetic energy to escape the potential and are thus trapped in the laser funnel indefinitely. We find that by reducing the dipolar force to the point at which the trapping effect just vanishes, it is possible to optimize the coupling of atoms into the fiber. Our simulations predict that by using a low-power (2.5 mW) and far-detuned (300 GHz) Laguerre-Gaussian beam with a 20-{mu}m-radius core hollow fiber, it is possible to couple 11% of the atoms from a MOT 9 mm away from the fiber. When the MOT is positioned farther away, coupling efficiencies over 50% can be achieved with larger core fibers.

74 ATOMIC AND MOLECULAR PHYSICS↗