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NASA NTRS1994

Coagulation algorithms with size binning

The Smoluchowski equation describes the time evolution of an aerosol particle size distribution due to aggregation or coagulation. Any algorithm for computerized solution of this equation requires a scheme for describing the continuum of aerosol particle sizes as a discrete set. One standard form of the Smoluchowski equation accomplishes this by restricting the particle sizes to integer multiples of a basic unit particle size (the monomer size). This can be inefficient when particle concentrations over a large range of particle sizes must be calculated. Two algorithms employing a geometric size binning convention are examined: the first assumes that the aerosol particle concentration as a function of size can be considered constant within each size bin; the second approximates the concentration as a linear function of particle size within each size bin. The output of each algorithm is compared to an analytical solution in a special case of the Smoluchowski equation for which an exact solution is known . The range of parameters more appropriate for each algorithm is examined.

Statton, David M.↗

NASA NTRS1994

Constraints placed on the chondrule-forming process by merrihueite in the Mezoe-Madaras chondrite

A few unusual chondrules in the Mezoe-Madaras L3 chondrite contain the peralkaline mineral merrihueite, (K, Na)2(Fe, Mg)5Si12O30, formed by reaction of free silica in the chondrules with K, Na, Fe-rich nebular gas. Vapor fractionation was required to create chondrules poor in Al and rich in Si, and the fractionated condensate produced had to aggregate into protochondrules very promptly (on the order of hours or less) to prevent it from mixing with dust of more generalized composition in the nebula. The traditional paradigm for chondrule formation, involving a series of unrelated events (chemical fractionation of precursor dust; clumping of the dust; melting of the dust-clumps), is inadequate for making these chondrules. A rapid process, all stages of which are related, is required. We propose that this occurred during the cooling and contraction of the volume of hot gas created by a small transient high-energy event in the nebula, of unspecified nature. Microdroplets of silicate melt created by condensation from the cooling, contracting gas had velocity vectors directed toward the center of the volume. Coalescence occurred in the crowded central zone where the microdroplets converged. The Mezoe-Madaras merriihueite-bearing chondrules may have been formed by an atypically low-energy nebular event, which achieved the needed chemical fractionations by only partially vaporizing precursor dust. More commonplace chondrule types may have been created by the same basic process, but involving higher-energy events in which precursor dust was completely vaporized and recondensed.

Wood, John A.↗

NASA NTRS1994

Regional rainfall climatologies derived from Special Sensor Microwave Imager (SSM/I) data

Climatologies of convective precipitation were derived from passive microwave observations from the Special Sensor Microwave Imager using a scattering-based algorithm of Adler et al. Data were aggregated over periods of 3-5 months using data from 4 to 5 years. Data were also stratified by satellite overpass times (primarily 06 00 and 18 00 local time). Four regions (Mexico, Amazonia, western Africa, and the western equatorial Pacific Ocean (TOGA COARE area) were chosen for their meteorological interest and relative paucity of conventional observations. The strong diurnal variation over Mexico and the southern United States was the most striking aspect of the climatologies. Pronounced morning maxima occured offshore, often in concativities in the coastline, the result of the increased convergence caused by the coastline shape. The major feature of the evening rain field was a linear-shaped maximum along the western slope of the Sierra Madre Occidental. Topography exerted a strong control on the rainfall in other areas, particularly near the Nicaragua/Honduras border and in Guatemala, where maxima in excess of 700 mm/month were located adjacent to local maxima in terrain. The correlation between the estimates and monthly gage data over the southern United States was low (0.45), due mainly to poor temporal sampling in any month and an inadequate sampling of the diurnal cycle. Over the Amazon Basin the differences in morning versus evening rainfall were complex, with an alternating series of morning/evening maxima aligned southwest to northeast from the Andes to the northeast Brazilian coast. A real extent of rainfall in Amazonia was slightly higher in the evening, but a maximum in morning precipitation was found on the Amazon River just east of Manaus. Precipitation over the water in the intertropical convergence zone (ITCZ) north of Brazil was more pronounced in the morning, and a pronounced land-/sea-breeze circulation was found along the northeast coast of Brazil. Inter-comparison of four years revealed 1992 to be the driest over Amazonia, with about a 23% decrease in mean rate compared to the 4-year mean estimated rain rate.

Negri, Andrew J.↗

NASA NTRS1994

Physics of interplanetary dust capture via impact into organic polymer foams

The physics of hypervelocity impacts into foams is of interest because of the possible application to interplanetary dust particle (IDP) capture by spacecraft. We present a model for the phenomena occurring in such impacts into low-density organic polymer foams. Particles smaller than foam cells behave as if the foam is a series of solid slabs and are fragmented and, at higher velocities, thermally altered. Particles much larger than the foam cells behave as if the foam were a continuum, allowing the use of a continuum mechanics model to describe the effects of drag and ablation. Fragmentation is expected to be a major process, especially for aggregates of small grains. Calculations based on these arguments accurately predict experimental data and, for hypothetical IDPs, indicate that recovery of organic materials will be low for encounter velocities greater than 5 km/s. For an organic particle 100 micrometers in diameter, approx. 35% of the original mass would be collected in an impact at 5 km/s, dropping to approx. 10% at 10 km/s and approx. 0% at 15 km/s. For the same velocities the recovery ratios for troilite (FeS) are approx. 95%, 65%, and 50%, and for olivine (Mg2SiO4) they are approx. 98%, 80%, and 65%, demonstrating that inorganic materials are much more easily collected. The density of the collector material has only a second-order effect, changing the recovered mass by less than 10% of the original mass.

Anderson, William W.↗

NASA NTRS1994

Exobiology experiments for Earth-orbital platforms

Low-gravity (microgravity) studies relevant to prebiotic evolution and the history of the biogenic elements (C, H, N, O, P, S) are particularly suited to orbital platforms. Relevant to these topics are phenomena such as gas-particle interactions (e.g., formation of organic aerosols via photolytic reactions) including nucleation, condensation, evaporation, adsorption, and catalytic reactions on surfaces; and, small-particle or grain interactions (e.g., growth of interstellar dust particles and planetesimals) including processes such as aggregation (or coagulation), scavenging, and collisions. Both gas-particle and grain (i.e., dust, crystals, organic aerosols, etc.) interactions studies can benefit from microgravity and are pertinent to studies in the areas of chemical evolution in the solar nebula, the interstellar medium, and planetary atmospheres; growth of planetesimals; and prebiotic evolution. In general, the microgravity environment allows for long duration and controlled simulations of processes occurring in exobiologically significant systems such as Titan's atmosphere, interstellar dust clouds, and the solar nebula in which gas-particle or particle-particle interactions play a significant role.

Huntington, J. L.↗

NASA NTRS1994

A double-moment multiple-phase four-class bulk ice scheme, Part 1: Description

A detailed ice-phase bulk microphysical scheme has been developed for simulating the hydrometeor distributions of convective and stratiform precipitation in different large-scale environmental conditions. The proposed scheme involves 90 distinct microphysical processes, which predict the mixing ratios and the number concentrations of small ice crystals, snow, graupel, and frozen drops/hail, as well as the mixing ratios of liquid water on wet precipitation ice (snow, graupel, frozen drops). The number of adjustable coefficients has been significantly reduced in comparison with other bulk schemes. Additional improvements have been made to the parameterization in the following areas: (1) representing small ice crystals with nonzero terminal fall velocities and dispersive size distributions, (2) accurate and computationally efficient calculations of precipitation collection processes, (3) reformulating the collection equation to prevent unrealistically large accretion rates, (4) more realistic conversion by riming between different classes of precipitation ice, (5) preventing unrealistically large rates of raindrop freezing and freezing of liquid water on ice, (6) detailed treatment of various rime-splintering ice multiplication mechanisms, (7) a simple representation of the Hobbs-Rangno ice enhancement process, (8) aggregation of small ice crystals and snow, and (9) allowing explicit competition between cloud water condensation and ice deposition rates rather than using saturation adjustment techniques. For the purposes of conserving the higher moments of the particle distributions, preserving the spectral widths (or slopes) of the particle spectra is shown to be more important than strict conservation of particle number concentration when parameterizing changes in ice-particle number concentrations due to melting, vapor transfer processes (sublimation of dry ice, evaporation from wet ice), and conversion between different hydrometeor species. The microphysical scheme is incorporated into a nonhydrostatic cloud model in Part 2 of this study. The model performed well in simulating the radar and microphysical structures of a midlatitude-continental squall lines and a tropical-maritime squall system with minimal tuning of the parameterization, even though the vertical profiles of radar reflectivity differed substantially between these storms.

Ferrier, Brad Shoenberg↗

NASA NTRS1995

Exobiology research on Space Station Freedom

The Gas-Grain Simulation Facility (GGSF) is a multidisciplinary experiment laboratory being developed by NASA at Ames Research Center for delivery to Space Station Freedom in 1998. This facility will employ the low-gravity environment of the Space Station to enable aerosol experiments of much longer duration than is possible in any ground-based laboratory. Studies of fractal aggregates that are impossible to sustain on Earth will also be enabled. Three research areas within exobiology that will benefit from the GGSF are described here. An analysis of the needs of this research and of other suggested experiments has produced a list of science requirements which the facility design must accommodate. A GGSF design concept developed in the first stage of flight hardware development to meet these requirements is also described.

Huntington, J. L.↗

NASA NTRS1994

ASCA measurements of the grain-scattered X-ray halos of eclipsing massive X-ray binaries: Vela X-1 and Centaurus X-3

We have measured the decaying dust-scattered X-ray halo of Cen X-3 during its binary eclipse with the ASCA solid-state imaging spectrometer (SIS). The surface brightness profile (SBP) of the image in the low-energy band (0.5-3 keV) lies substantially above the point-spread function (PSF) of the X-ray telescope, while the SBP in the high-energy band (5-10 keV) exhibits no significant deviation. By contrast, the SBPs of Vela X-1 during its eclipse are consistent with the PSF in both the low- and high-energy bands -- strong evidence that a dust halo is indeed present in Cen X-3. Accordingly, we modeled the SBP of Cen X-3 taken from six consecutive time segments under the principal assumptions that the dust is distributed uniformly along a segment of the line of sight, the grains have a power-law size distribution, and the low-energy source flux was the same function of orbital phase before as during our observation. The best-fit set of parameters included a grain density value of 1.3 g/cu cm, substanially less than the density of 'astronomical silicate.' This result supports the idea that interstellar grains are 'fluffy' aggregates of smaller solid particles. We attribute the failure to detect a halo of Vela X-1 during its eclipse phase to extended strong circumsource absorption that probably occurred before the eclipse and allowed the halo to decay away before the observation began.

Woo, Jonathan W.↗

NASA NTRS1994

A model composition for Mars derived from the oxygen isotopic ratios of martian/SNC meteorites

Oxygen is the most abundant element in most meteorites, yet the ratios of its isotopes are seldom used to constrain the compositional history of achondrites. The two major achondrite groups have O isotope signatures that differ from any plausible chondritic precursors and lie between the ordinary and carbonaceous chondrite domains. If the assumption is made that the present global sampling of chondritic meteorites reflects the variability of O reservoirs at the time of planetessimal/planet aggregation in the early nebula, then the O in these groups must reflect mixing between known chondritic reservoirs. This approach, in combination with constraints based on Fe-Mn-Mg systematics, has been used previously to model the composition of the basaltic achondrite parent body (BAP) and provides a model precursor composition that is generally consistent with previous eucrite parent body (EPB) estimates. The same approach is applied to Mars exploiting the assumption that the SNC and related meteorites sample the martian lithosphere. Model planet and planetesimal compositions can be derived by mixing of known chondritic components using O isotope ratios as the fundamental compositional constraint. The major- and minor-element composition for Mars derived here and that derived previously for the basaltic achondrite parent body are, in many respects, compatible with model compositions generated using completely independent constraints. The role of volatile elements and alkalis in particular remains a major difficulty in applying such models.

Delaney, J. S.↗

NASA NTRS1994

CM chondrites exhibit the complete petrologic range from type 2 to 1

Recognition and characterization of the different CM lithologies as components in all meteorites could reveal details of the nature and chronology of alteration and brecciation events on hydrous asteroids. The CM chondrites are of particular interest, as they are the most common carbonaceous chondrites and are found as clasts within other types of meteorites, which suggests that the CM parent asteroids are (or were) widespread in the sections of the asteroid belt providing samples to Earth. Some CM2s, including EET 90047, ALH 83100, and Y 82042, are more 'extensively' altered, and are distinguished by a high proportion of Mg-rich phyllosilicates and Ca-Mg carbonates, frequently in rounded aggregates, and near absence of olivine or pyroxene. 'Completely' altered CMs, called CM1s, essentially lack olivine or pyroxene; these include EET 83334, ALH 88045, and the CM1 clasts in Kaidun. Cold Bokkeveld and EET 84034, both highly brecciated CMs, consist of both extensively and completely altered lithologies. We describe how these lithologies further cosntrain physicochemical conditions on hydrous asteroids. We conclude that CM chondrites exhibit the petrologic range 2 through 1, and that progressive alteration on the parent hydrous asteroid(s) was accompanied by significant increases in temperature (to a peak of approximately 450 C), fO2, water-rock ratio, and (locally) degree of chemical leaching, all well beyond the conditions recorded by CM2s.

Zolensky, M. E.↗

NASA NTRS1993

Optical effects of space weathering: The role of the finest fraction

The optical properties of lunar soils are different than those of rocks which they are derived. As a consequence of lunar space weathering, soils are darker and exhibit a distinctive red-sloped continuum and weaker mineral absorption bands. The accumulation of dark glass-welded aggregates (agglutinates) has been thought to account for these optical effects of space weathering on lunar soils. Spectroscopic analyses of agglutinate separates and size fractions for a suite of lunar soils presented here indicate that the agglutinate paradigm is insufficient to fully account for lunar optical alteration. It is the finest fraction of lunar soils (less than 25 microns which constitute approximately 25% wt.) that dominates the optical properties of the bulk soil. Unlike size fractions of most silicates for which the finest fraction is the brightest, the lunar soil size fractions all have comparable albedos in the short-wavelength visible. In the near infrared, however, it is the finest fraction that exhibits the steep red continuum and weak absorption bands. The properties of the finest fraction cannot be duplicated by preparing a fine fraction by grinding larger agglutinate-rich soil particles. These results suggest space weathering on airless bodies is dominated by surface correlated processes (perhaps associated with the developement of fine-grained Fe(dot) on or near the surface of grains), and the accumulation of the large agglutinates is not necessarily required to account for lunar optical alteration.

Pieters, C. M.↗

NASA NTRS1994

Rarefied solids

One important limit to creating low density materials is the objects' own weight. As a solid or colloidal matrix becomes more rarefied, gravity acts destructively to compress its suporting skeleton. We describe experimental results and propose a model which matches the low gravity behavior of rarefied or fractal solids. On parabolic airplane flights, we sought to demonstrate a key component of producing higher surface area fractals. Flight paths were selected to give a range of gravity levels: 0.01 g/g(sub 0) (low), 0.16 g(sub 0) (Lunar), 0.33 g/g(sub 0) (Martian), 1 g/g(sub 0) (Earth) and 1.8 g/g(sub 0) (high) (where g(sub 0) = 980 cm/sq s). Results using the model material of hydrophobic silica indicated that stable agglomeration of such tenuous objects can increase markedly in reduced gravity. Optical characterization revealed that fractal dimension changed directly with varying gravity. As measured by fractal dimension, effective surface area and roughness increased by 40% in low gravity. This finding supports the conclusion that relieving internal weight stresses on delicate aggregates can enhance their overall size (by two orders of magnitude) and internal surface area. We conclude that gravitational restructuring limits the overall size and void content of low-density solids. These sparse colloidal regimes may present new and technologically attractive physics, ranging from improved insulators, liquid-like tension in a 'solid' matrix, and characteristically low conductivities for sound and (8 to 14 micrometers wavelength) infrared radiation.

Noever, D. A.↗

NASA NTRS1993

Carbonaceous chondrite clasts in the howardites Bholghati and EET87513

Twenty-two carbonaceous chondrite clasts from the two howardites Bholghati and EET87513 were analyzed. Clast N from EET87513 is a fragment classified as CM2 material on the basis of texture, bulk composition, mineralogy, and bulk O isotopic composition. Carbonaceous chondrite clasts from Bholghati, for which less data are available because of their small size, can be divided into two petrologic types: C1 and C2. C1 clasts are composed of opaque matrix with rare coarse-grained silicates as individual mineral fragments; textures resemble CI meteorites and some dark inclusions from CR meteorites. Opaque matrix is predominantly composed of flaky saponite; unlike typical CI and CR meteorites, serpentine is absent in the samples we analyzed. C2 clasts contain chondrules, aggregates, and individual fragments of coarse-grained silicates in an opaque matrix principally composed of saponite and anhydrous ferromagnesian silicates with flaky textures similar to phyllosilicates. These anhydrous ferromagnesian silicates are interpreted as the product of heating of pre-existing serpentine. The carbonaceous chondrite clasts we have studied from these two howardites are, with one notable exception (clast N from EET87513), mineralogically distinct from typical carbonaceous chondrites. However, these clasts have very close affinities to carbonaceous chondrites and have also experienced thermal metamorphism and aqueous alteration, but to different degrees.

Buchanan, P. C.↗

NASA NTRS1994

Cluster growth modeling of plateau erosion

The pattern of erosion of a plateau along an escarpment may be modeled usng cluster growth techniques, recently popularized in models of drainage network evolution. If erosion on the scarp takes place in discrete events at rates subject to local substrate strength, the whole range of behavior is described by a combination of three cluster growth mechanisms: invasion percolation, Eden growth and diffusion-limited aggregation (DLA). These model the relative importance of preexisting substrate strength, background weathering, and seepage weathering and erosion respectively. The rate of seepage processes is determined by the efflux of groundwater at the plateau margin, which in turn is determined by the pressure field in the plateau aquifer. If this process acted alone, it would produce erosion patterns in the form of Laplacian fractals, with groundwater recharge from a distant source, or Poissionian fractals, with groundwater recharge uniform over the plateau. DLA is used to mimic the Laplacian or Poissonian potential field and the corresponding seepage growth process. The scaling structure of clusters grown by pure DLA, invasion percolation, or Eden growth is well known; this study presents a model which combines all three growth mechanisms for the first time. Mixed growth processes create clusters with different scaling properties and morphologies over distinct length scale ranges, and this is demonstrable in natural examples of plateau erosion.

Stark, Colin P.↗

NASA NTRS1995

Cosmic dust synthesis by accretion and coagulation

The morphology of grains grown by accretion and coagulation is revaled by a new laboratory method of synthesizing cosmic dust analogs. Submicron carbon particles, grown by accretion of carbon atoms from a gas, have a spherical shape with a cauliflower-like surface and an internal micro-structure of radial columns. This shape is probably common for grains grown by accretion at a temperature well below the melting point. Coagulated grains, consisting of spheres that collided to form irregular strings, were also synthesized. Another shape we produced had a bumpy non- spherical morphology, like an interplanetary particle collected in the terrestrial stratosphere. Besides these isolated grains, large spongy aggregates of nanometer-size particles were also found for various experimental conditions. Grains were synthesized using ions to sputter a solid target, producing an atomic vapor at a low temperature. The ions were provided by a plasma, which also provided electrostatic levitation of the grains during their growth. The temporal development of grain growth was studied by extinguishing the plasma after various intervals.

Praburam, G.↗

NASA NTRS1994

Dynamic modeling of orographically induced precipitation

Local orography governs the triggering of cloud formation and the enhancement of processes such as condensation and hydrometeor nucleation and growth in mountainous regions. Intense, lengthy precipitation events are typical upwind of the topographic divide, with sharply decreasing magnitude and duration on the lee side. Differences in mean annual precipitation of several hundred percent between windward slopes of orographic barriers and adjacent valleys or lee side slopes are not unusual. Because much of the streamflow in areas such as the western United States is derived from mountainous areas that are remote and often poorly instrumented, modeling of orographic precipitation has important implications for water resources management. Models of orographically induced precipitation differ by their treatment of atmospheric dynamics and by the extent to which they rely on bulk parameterization of cloud and precipitation physics. Adiabatic ascent and a direct proportionality between efficiency and orographically magnified updrafts are the most frequent assumptions in orographic precipitation modeling. Space-time discretization (i.e., resolution) is a major issue because of the high spatial variability of orographic precipitation. For a specific storm, relative errors as large as 50 to 100% are common in the forecast/hindcast of precipitation intensity and can be even larger in the case of catastrophic storms. When monthly or seasonal timescales are used to evaluate model performance, the magnitude of such errors decreases dramatically, reaching values as low as 10 to 15%. Current research is focusing on the development of data assimilation techniques to incorporate radar and satellite observations, and on the development of aggregation and disaggregation methodologies to address the implications of modeling a multiscale problem at restricted spatial and temporal resolutions.

Barros, Ana Paula↗

NASA NTRS1993

Conservative force model performance for TOPEX/Poseidon precision orbit determination

The TOPEX/Poseidon spacecraft was launched on August 10, 1992 to study the Earth's oceans. To achieve maximum benefit from the altimetric data collected, mission requirements dictate that TOPEX/Poseidon's orbit must be computed at an unprecedented level of accuracy. In order to satisfy these requirements, a model which accounts for the satellite's complex geometry, attitude, and surface properties has been developed. This `box-wing' representation treats the spacecraft as the combination of flat plates arranged in the shape of a box and a connecetd solar array. The nonconservative forces acting on each of the eight surfaces are computed independently, yielding vector accelerations which are summed to compute the total aggregate effect on the satellite center-of-mass. Parameters associated with each flat plate were derived from a finite element analysis of the spacecraft. Certain parameters can be inferred from tracking data and have been adjusted to obtain a better representation of the satellite acceleration history. Changes in the nominal mission profile and the presence of an `anomalistic' force have complicated this tuning process. Model performance, parameter sensitivities, and the `anomalistic' force will be discussed.

Marshall, J. Andrew↗

NASA NTRS1994

Catastrophic disruption experiments: Recent results

This paper presents a review of the progress in the field of catastrophic disruption experiments over the past 4 years, since the publication of the review paper by Fujiwara et al. (1989). We describe the development of new techniques to produce shattering impacts relevant to the study of the collisional evolution of the asteroids, and summarize the results from numerous experiments which have been performed to date, using a variety of materials for both the impactor and the targets. Some of these, such as ice-on-ice, loose aggregates and pressurized targets, are quite new and have provided novel and exciting results. Some of the gaps existing previously in the data on fragment ejection-angle distributions, as well as translational and rotational velocity fields (including fine fragments) have been filled, and these new results will be surveyed.

Martelli, G.↗