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NASA NTRS1990

Spallation processes and nuclear interaction products of cosmic rays

Most cosmic-ray nuclei heavier than helium have suffered nuclear collisions in the interstellar gas, with transformation of nuclear composition. The isotopic and elemental composition at the sources has to be inferred from the observed composition near the Earth. The source composition permits tests of current ideas on sites of origin, nucleosynthesis in stars, evolution of stars, the mixing and composition of the interstellar medium and injection processes prior to acceleration. The effects of nuclear spallation, production of radioactive nuclides and the time dependence of their decay provide valuable information on the acceleration and propagation of cosmic rays, their nuclear transformations, and their confinement time in the Galaxy. The formation of spallation products that only decay by electron capture and are relatively long-lived permits an investigation of the nature and density fluctuations (like clouds) of the interstellar medium. Since nuclear collisions yield positrons, antiprotons, gamma rays and neutrinos, we shall discuss these topics briefly.

Non-NASA Center↗

NASA NTRS1980

On krypton isotopic abundances in the sun and in the solar wind

The Kr isotopic systematics in the meteorite Pesyanoe which is known to contain solar-type gases, are reported. Discrepancies in the isotopic data of fractions released at stepwise increasing temperatures cannot be reconciled with spallation Kr components, although spallation effects are significant. Fractionation mechanisms on the parent body and in the solar wind source region are considered and the implications for solar abundances discussed.

Marti, K.↗

NASA NTRS2001

Correlation of Upper-Atmospheric 7-Be with Solar Energetic Particle Events

A surprisingly large concentration of radioactive 7-Be was observed in the upper atmosphere at altitudes above 320 km on the LDEF satellite that was recovered in January 1990. We report on follow-up experiments on Russian spacecraft at altitudes of 167 to 370 km during the period of 1996 to 1999, specifically designed to measure 7-Be concentrations in low earth orbit. Our data show a significant correlation between the 7-Be concentration and the solar energetic proton fluence at Earth, but not with the overall solar activity. During periods of low solar proton fluence, the concentration is correlated with the galactic cosmic ray fluence. This indicates that spallation of atmospheric N by both solar energetic particles and cosmic rays is the primary source of 7-Be in the ionosphere.

Phillips, G. W.↗

DOE OSTI2022

Decay Dose Shielding Analysis with Hybrid Unstructured Mesh/Constructive Solid Geometry Monte Carlo Calculation and ADVANTG Acceleration

The Oak Ridge National Laboratory (ORNL) Second Target Station (STS) neutron production facility is an accelerator driven pulsed neutron source that is currently being actively developed at ORNL. The neutrons are produced by proton-induced spallation reactions. A proton beam of 700 kW power is delivered to a spallation target in short, less than 1 µs long pulses, with 15 Hz repetition rate. The spallation target of ORNL STS is a rotating water-cooled tungsten target with tantalum cladding housed in a stainless-steel shroud. It is divided into 21 segments. These segments become highly activated due to spallation reactions or nuclei transmutation by the emitted neutrons. The radioactive nuclides continue to decay after ceasing operation. The decay dose rates generated from the target segments once they are removed from their operational location within the core vessel must be accurately quantified to determine the shielding configurations of remote handling tools and transport casks and to aid in planning maintenance events. To determine the shielding configurations needed for an activated target segment after ceasing operation, both the hybrid unstructured mesh (UM)/constructive solid geometry (CSG) approach that was previously utilized for STS analyses [1] and the ADVANTG code [2] were used. Even though the ADVANTG code does not include UM capability, the utilization of its advanced variance reduction technique was crucial to accelerate the extremely difficult final photon transport calculation in this analysis. This paper also describes the procedures taken to mitigate the convergence issues that occur when ADVANTG uses a source definition that does not match the source of the final Monte Carlo (MC) calculation. These convergence issues often occur because of inconsistencies between source and transport biasing parameters.

Ibrahim, Ahmad↗

NASA NTRS1993

The elemental and isotopic composition of Galactic cosmic-ray nuclei from scandium through nickel

Measurements of the relative elemental and isotopic abundances of iron-group Galactic cosmic rays at energies of about 325 MeV per nucleon have been made. The source abundance ratio of Ni-60/Ni-58 is 1.07 +/- 0.39, which is a factor of 2.8 +/- 1.0 larger than the solar system value. Our measurements imply the presence of Co-59 at the source, which can be reconciled with the predictions of conventional nucleosynthesis models if there exists a time delay of more than about 100,000 yr between nucleosynthesis and acceleration. Most of the Mn-54 produced by spallation during cosmic-ray propagation in the Galaxy is found to have decayed to Fe-54, indicating a confinement time of greater than 2 Myr. The source ratio of Fe-54/Fe-56 corrected for the Mn-54 decay is 0.046+/- 0.020, which is consistent with the solar system value of 0.063.

Leske, Richard A.↗

DOE OSTI2018

A review of the thermal expansion of magnetite

Thermal expansion data from various sources were placed on an equivalent basis and fitted true (α T ) and mean (α M ) coefficients of thermal expansion were generated. Recent models of oxide spallation in boiler tubes cite and use Central Electricity Generating Board (CEGB) data for αM, but details of how the CEGB data was generated were not known. Here, the CEGB data were found to be derived from an earlier source but given (unconventionally) in terms of small temperature step α M increments.

36 MATERIALS SCIENCE↗

DOE OSTI2017

The production rate of cosmogenic deuterium at the Moon's surface

The hydrogen (D/H) isotope ratio is a key tracer for the source of planetary water. However, secondary processes such as solar wind implantation and cosmic ray induced spallation reactions have modified the primordial D/H signature of ‘water’ in all rocks and soils recovered on the Moon. We re-evaluate the production rate of cosmogenic deuterium (D) at the Moon's surface through ion microprobe analyses of hydrogen isotopes in olivines from eight Apollo 12 and 15 mare basalts. Furthermore, these in situ measurements are complemented by CO2 laser extraction-static mass spectrometry analyses of cosmogenic noble gas nuclides ( 3 He, 21 Ne, 38 Ar). Cosmic ray exposure (CRE) ages of the mare basalts, derived from their cosmogenic 21Ne content, range from 60 to 422 Ma. These CRE ages are 35% higher, on average, than the published values for the same samples. The amount of D detected in the olivines increases linearly with increasing CRE ages, consistent with a production rate of (2.17±0.11)×10 -12 mol(g rock) -1 Ma -1 . This value is more than twice as high as previous estimates for the production of D by galactic cosmic rays, indicating that for water-poor lunar samples, i.e., samples with water concentrations ≤50 ppm, corrected D/H ratios have been severely overestimated.

58 GEOSCIENCES↗

DOE OSTI2015

Technical Design Report, Second Target Station

The Second Target Station (STS) is a proposed upgrade for SNS. It includes a doubling of the accelerator power and an additional instrument hall. The new instrument hall will receive a 467 kW 10 Hz beam. The parameters and preliminary design aspects of the STS are presented for the accelerator, target systems, instrument hall, instruments and civil construction aspects.

43 PARTICLE ACCELERATORS↗

NASA NTRS1979

Predictions of induced background radiations at gamma/X-ray experiment envelopes in NASA spacecraft

This work seeks to predict secondary radiation levels induced in spacecraft structures by space protons. The radiations analyzed are secondary neutrons from spallation and evaporation reactions and gamma and beta rays from the decay of induced radioactivity, as sources of interfering background to spaceborne measurements of galactic and planetary gamma rays below 10 MeV. The spacecraft considered are the Multi-Mission Spacecraft (MMS) and the Space Shuttle, modeled as spherical shells. The proton environment is that of the South Atlantic Anomaly, as well as cosmic ray protons. The induced radioactivity is analyzed in terms of its interference with various gamma-ray lines of astrophysical interest, as well as its contribution to several spectral regions of the gamma-ray continuum. The buildup of the line and continuum radioactivity background is predicted for a period of nearly 9 months in orbit (approximately 4100 orbits). In addition, background contributions from cosmic ray electron bremsstrahlung and earth gamma-ray albedo are estimated.

Fischbein, W. L.↗

DOE OSTI2012

Conceptual configurations of an accelerator-driven subcritical system utilizing minor actinides

This paper purposes an Accelerator-Driven Subcritical (ADS) system which utilizes the Minor Actinides (MAs) from the US spent nuclear fuel inventory. A mobile fuel concept with micro-particles suspended in the liquid metal is adopted in the purposed system to avoid difficulties of developing and testing new MAs solid fuel forms. Three ADS configurations were developed and analyzed using the Monte Carlo fuel burnup methodology. The analyses demonstrated the capabilities of the proposed system to utilize the MAs and to dispose of the US spent nuclear fuels. (authors)

43 PARTICLE ACCELERATORS↗

DOE OSTI2012

EVIDENCE FOR MULTIPLE SOURCES OF {sup 10}Be IN THE EARLY SOLAR SYSTEM

Beryllium-10 is a short-lived radionuclide (t{sub 1/2} = 1.4 Myr) uniquely synthesized by spallation reactions and inferred to have been present when the solar system's oldest solids (calcium-aluminum-rich inclusions, CAIs) formed. Yet, the astrophysical site of {sup 10}Be nucleosynthesis is uncertain. We report Li-Be-B isotope measurements of CAIs from CV chondrites, including CAIs that formed with the canonical {sup 26}Al/{sup 27}Al ratio of {approx}5 Multiplication-Sign 10{sup -5} (canonical CAIs) and CAIs with Fractionation and Unidentified Nuclear isotope effects (FUN-CAIs) characterized by {sup 26}Al/{sup 27}Al ratios much lower than the canonical value. Our measurements demonstrate the presence of four distinct fossil {sup 10}Be/{sup 9}Be isochrons, lower in the FUN-CAIs than in the canonical CAIs, and variable within these classes. Given that FUN-CAI precursors escaped evaporation-recondensation prior to evaporative melting, we suggest that the {sup 10}Be/{sup 9}Be ratio recorded by FUN-CAIs represents a baseline level present in presolar material inherited from the protosolar molecular cloud, generated via enhanced trapping of galactic cosmic rays. The higher and possibly variable apparent {sup 10}Be/{sup 9}Be ratios of canonical CAIs reflect additional spallogenesis, either in the gaseous CAI-forming reservoir, or in the inclusions themselves: this indicates at least two nucleosynthetic sources of {sup 10}Be in the early solar system. The most promising locale for {sup 10}Be synthesis is close to the proto-Sun during its early mass-accreting stages, as these are thought to coincide with periods of intense particle irradiation occurring on timescales significantly shorter than the formation interval of canonical CAIs.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2016

Apparent Explosion Moments from Rg Waves Recorded on SPE

Seismic moments for the first four chemical tests making up phase I of the Source Physics Experiments (SPE) are estimated from 6-Hz Rg waves recorded along a single radial line of geophones under the assumption that the tests are pure explosions. These apparent explosion moments are compared with moments determined from the reduced displacement potential method applied to free-field data. Light detection and ranging (lidar) observations, strong ground motions on the free surface in the vicinity of ground zero, and moment tensor inversion results are evidence that the fourth test SPE-4P is a pure explosion, and the moments show good agreement, 8×10 10 N·m for free-field data versus 9×10 10 N·m for Rg waves. In stark contrast, apparent moments for the first three tests are smaller than near-field moments by factors of 3–4. Relative amplitudes for the three tests determined from Rg interferometry using SPE-4P as an empirical Green’s function indicate that radiation patterns are cylindrically symmetric within a factor of 1.25 (25%). This fact assures that the apparent moments are reliable even though they were measured on just one azimuth. Spallation occurred on the first three tests, and ground-based lidar detected permanent deformations. As such, the source medium suffered late-time damage. In conclusion, destructive interference between Rg waves radiated by explosion and damage sources will reduce amplitudes and explain why apparent moments are smaller than near-field moments based on compressional energy emitted directly from the source.

47 OTHER INSTRUMENTATION↗

NASA NTRS1986

Galactic cosmic ray composition

An assessment is given of the galactic cosmic ray source (GCRS) elemental composition and its correlation with first ionization potential. The isotopic composition of heavy nuclei; spallation cross sections; energy spectra of primary nuclei; electrons; positrons; local galactic reference abundances; comparison of solar energetic particles and solar coronal compositions; the hydrogen; lead; nitrogen; helium; and germanium deficiency problems; and the excess of elements are among the topics covered.

Meyer, J. P.↗

DOE OSTI2019

Explosion Source Models and the Scattering Origin of Regional Phases from SPE Phase 1 Coda Spectral Ratios: Monitoring Implications –Discrimination and Yield Estimation

The Source Physics Experiment (SPE) explosions provide comprehensive ground truth information, and near-source recordings that are rarely available in typical monitoring scenarios. Here, we analyze these data together with local and regional distance recordings to isolate source and propagation effects, and to potentially improve monitoring at distance. We examine source spectral ratios, which can be measured to high precision by taking advantage of many SPE and independently operated stations, as well as the redundancy available from coda waves. Classical source models (Mueller and Murphy, 1971, MM71; Denny and Johnson, 1991, DJ91) predict the source ratios poorly; however, a hybrid model (MM71 with DJ91 cavity radii) performs better. We observe a distinct spectral modulation at 6-9 Hz that is not predicted by classical models, most likely caused by short period surface waves (Rg) interfering with those produced by spallation of near surface layers. The same modulation is observed for compressional (P) and shear (S) waves at distance, indicating that local and regional phases originate as near-source Rg that is scattered into body waves. The scattering process must be accounted for quantitatively to best use remotely recorded signals to monitor treaty compliance, discriminate event types, and estimate explosion yields over broad regions.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2014

Twin boundary spacing effects on shock response and spall behaviors of hierarchically nanotwinned fcc metals

Atomistic deformation mechanisms of hierarchically nano-twinned (NT) Ag under shock conditions have been investigated using a series of large-scale molecular dynamics simulations. For the same grain size d and the same spacing of primary twins λ{sub 1}, the average flow stress behind the shock front in hierarchically NT Ag first increases with decreasing spacing of secondary twins λ{sub 2}, achieving a maximum at a critical λ{sub 2}, and then drops as λ{sub 2} decreases further. Above the critical λ{sub 2}, the deformation mechanisms are dominated by three type strengthening mechanisms: (a) partial dislocations emitted from grain boundaries (GBs) travel across other boundaries; (b) partial dislocations emitted from twin boundaries (TBs) travel across other TBs; (c) formation of tertiary twins. Below the critical λ{sub 2}, the deformation mechanism are dominated by two softening mechanisms: (a) detwinning of secondary twins; (b) formation of new grains by cross slip of partial dislocations. Moreover, the twin-free nanocrystalline (NC) Ag is found to have lower average flow stress behind the shock front than those of all hierarchically NT Ag samples except the one with the smallest λ{sub 2} of 0.71 nm. No apparent correlation between the spall strength and λ{sub 2} is observed in hierarchically NT Ag, since voids always nucleate at both GBs and boundaries of the primary twins. However, twin-free NC Ag is found to have higher spall strength than hierarchically NT Ag. Voids can only nucleate from GBs for twin-free NC Ag, therefore, twin-free NC Ag has less nucleation sources along the shock direction when compared to hierarchically NT Ag, which requiring higher tensile stress to create spallation. These findings should contribute to the understandings of deformation mechanisms of hierarchically NT fcc metals under extreme deformation conditions.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

NASA NTRS1985

Abundances of secondary elements among the ultra heavy cosmic rays: Results from HEAO-3

Observations of the abundances of elements of charge 62 or = Z or = 73 in the cosmic radiation from the HEAO-3 Heavy Nuclei Experiment (HNE) are discussed. These elements, having solar, and presumably source, abundances much less than the heavier Pt and Pb groups, are expected to be largely products of spallation. Thus they are indicators of the conditions prevailing during the propagation of cosmic rays. The abundances have changed from those reported previously due to a different data selection. This resulted in better charge resolution and in a higher mean energy for the particles. All the particles included in this paper were required to have had a cutoff rigidity R sub c 5 GV. This allowed the charge determination to be based solely on the Cerenkov measurement.

Klarmann, J.↗

NASA NTRS1985

Abundances of secondary elements among the ultra heavy cosmic rays: Results from HEAO-3

Observations of the abundances of elements of charge 62 or Z or = 73 in the cosmic radiation from the HEAO-3 Heavy Nuclei Experiment (HNE) are discussed. These elements, having solar, and presumably source, abundances much less than the heavier Pt and Pb groups, are expected to be largely products of spallation. Thus they are indicators of the conditions prevailing during the propagation of cosmic rays. The abundances have changed from those reported previously due to a different data selection. This results in better charge resolution and in a higher mean energy for the particles. All the particles included were required to have had a cutoff rigidity R sub c 5 GV. This allowed the charge determination to be based solely on the Cherenkov measurement.

Klarmann, J.↗

NASA NTRS1992

Ionizing radiation exposure of LDEF (pre-recovery estimates)

The long duration exposure facility (LDEF), launched into a 258 nautical mile orbit with an inclination of 28.5 degrees, remained in space for nearly 6 yr. The 21,500 lb NASA satellite was one of the largest payloads ever deployed by the Space Shuttle. LDEF completed 32,422 orbits and carried 57 major experiments representing more than 200 investigators from 33 private companies, 21 universities and nine countries. The experiments covered a wide range of disciplines including basic science, electronics, optics, materials, structures and power and propulsion. A number of the experiments were specifically designed to measure the radiation environment. These experiments are of specific interest, since the LDEF orbit is essentially the same as that of the Space Station Freedom. Consequently, the radiation measurements on LDEF will play a significant role in the design of radiation shielding of the space station. The contributions of the various authors presented here attempt to predict the major aspects of the radiation exposure received by the various LDEF experiments and therefore should be helpful to investigators who are in the process of analyzing experiments which may have been affected by exposure to ionizing radiation. The paper discusses the various types and sources of ionizing radiation including cosmic rays, trapped particles (both protons and electrons) and secondary particles (including neutrons, spallation products and high-LET recoils), as well as doses and LET spectra as a function of shielding. Projections of the induced radioactivity of LDEF are also discussed.

Flight Experiment↗