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At least 973 records · Page 54

Far infrared polarization of dust clouds

The recently observed 10-micron polarization of the Orion Nebula and the Galactic Center suggests that far infrared polarization may be found in these objects. Estimates are made of the degree of far infrared polarization that may exist in the Orion Nebula. The effects of radiation transfer are briefly considered and it is concluded that polarization observations over a range of wavelengths will be useful in deducing the optical depth structure of dust clouds.

Dennison, B.↗

C3H2 observations as a diagnostic probe for molecular clouds

Recently the three-membered ring molecule, cyclopropenylidene, C3H2, has been identified in the laboratory and detected in molecular clouds by Thaddeus, Vrtilek and Gottlieb (1985). This molecule is wide-spread throughout the Galaxy and has been detected in 25 separate sources including cold dust clouds, circumstellar envelopes, HII regions, and the spiral arms observed against the Cas supernova remnant. In order to evaluate the potential of C3H2 as a diagnostic probe for molecular clouds, and to attempt to identify the most useful transitions, statistical equilibrium calculations were carried out for the lowest 24 levels of the ortho species and the lowest 10 levels of the para species. Many of the sources observed by Matthews and Irvine (1985) show evidence of being optically thick in the 1(10)-1(01) line. Consequently, the effects of radiative trapping should be incorporated into the equilibrium calculations. This was done using the Large Velocity Gradient approximation for a spherical cloud of uniform density. Some results of the calculations for T(K)=10K are given. Figures are presented which show contours of the logarithm of the ratio of peak line brightness temperatures for ortho-para pairs of lines at similar frequencies. It appears that the widespread nature of C3H2, the relatively large strength of its spectral lines, and their sensitivity to density and molecular abundance combine to make this a useful molecule for probing physical conditions in molecular clouds. The 1(10)-1(01) and 2(20)-2(11) K-band lines may be especially useful in this regard because of the ease with which they are observed and their unusual density-dependent emission/absorption properties.

Avery, L. W.↗

The Emissions Model Intercomparison Project (Emissions-MIP): quantifying model sensitivity to emission characteristics

Abstract. Anthropogenic emissions of aerosols and precursor compounds are known to significantly affect the energy balance of the Earth–atmosphere system, alter the formation of clouds and precipitation, and have a substantial impact on human health and the environment. Global models are an essential tool for examining the impacts of these emissions. In this study, we examine the sensitivity of model results to the assumed height of SO2 injection, seasonality of SO2 and black carbon (BC) particulate emissions, and the assumed fraction of SO2 emissions that is injected into the atmosphere as particulate phase sulfate (SO4) in 11 climate and chemistry models, including both chemical transport models and the atmospheric component of Earth system models. We find large variation in atmospheric lifetime across models for SO2, SO4, and BC, with a particularly large relative variation for SO2, which indicates that fundamental aspects of atmospheric sulfur chemistry remain uncertain. Of the perturbations examined in this study, the assumed height of SO2 injection had the largest overall impacts, particularly on global mean net radiative flux (maximum difference of −0.35 W m−2), SO2 lifetime over Northern Hemisphere land (maximum difference of 0.8 d), surface SO2 concentration (up to 59 % decrease), and surface sulfate concentration (up to 23 % increase). Emitting SO2 at height consistently increased SO2 and SO4 column burdens and shortwave cooling, with varying magnitudes, but had inconsistent effects across models on the sign of the change in implied cloud forcing. The assumed SO4 emission fraction also had a significant impact on net radiative flux and surface sulfate concentration. Because these properties are not standardized across models this is a source of inter-model diversity typically neglected in model intercomparisons. These results imply a need to ensure that anthropogenic emission injection height and SO4 emission fraction are accurately and consistently represented in global models.

54 ENVIRONMENTAL SCIENCES↗

Observations of Carbon Isotopic Fractionation in Interstellar Formaldehyde

Primitive Solar System materials (e.g. chondrites. IDPs, the Stardust sample) show large variations in isotopic composition of the major volatiles (H, C, N, and O ) even within samples, witnessing to various degrees of processing in the protosolar nebula. For ex~ ample. the very pronounced D enhancements observed in IDPs [I] . are only generated in the cold. dense component of the interstellar medium (ISM), or protoplanetary disks, through ion-molecule reactions in the presence of interstellar dust. If this isotopic anomaly has an interstellar origin, this leaves open the possibility for preservation of other isotopic signatures throughout the form ation of the Solar System. The most common form of carbon in the ISM is CO molecules, and there are two potential sources of C-13 fractionation in this reservoir: low temperature chemistry and selective photodissociation. While gas-phase chemistry in cold interstellar clouds preferentially incorporates C-13 into CO [2], the effect of self-shielding in the presence of UV radiation instead leads to a relative enhancement of the more abundant isotopologue, 12CO. Solar System organic material exhibit rather small fluctuations in delta C-13 as compared to delta N-15 and delta D [3][1], the reason for which is still unclear. However, the fact that both C-13 depleted and enhanced material exists could indicate an interstellar origin where the two fractionation processes have both played a part. Formaldehyde (H2CO) is observed in the gas-phase in a wide range of interstellar environments, as well as in cometary comae. It is proposed as an important reactant in the formation of more complex organic molecules in the heated environments around young stars, and formaldehyde polymers have been suggested as the common origin of chondritic insoluable organic matter (IOM) and cometary refractory organic solids [4]. The relatively high gas-phase abundance of H2CO observed in molecular clouds (10(exp- 9) - 10(exp- 8) relative to H2) makes it feasible to observe its less common isotopologues. As a step in our investigation of C-13 fractionation patterns in the ISM, we here present comparisons between observations of the C-13 fraction in formaldehyde, and chemical fractionation models.

Wirstrom, E. S.↗

Measuring cloud properties from space - A review

A brief review of observations of clouds using satellites highlights open issues and directions for future studies. The key one is improved treatment of the effects of small-scale spatial inhomogeneity in remote sensing data analyses and in the treatment of radiation in climate models, though studies and observations of the spectral dependence of cloud-radiation interactions are also limited. Significant progress in understanding the role of clouds in climate, especially regarding cloud-radiation budget relationships, is expected in the next several years because of an unprecedent suite of global and regional observation and analysis programs.

Rossow, William B.↗

Some effects of 8-12 micron radiant energy transfer on the mass and heat budgets of cloud droplets

In standard treatments of the mass and energy budget of cloud droplets, radiant energy transfer is neglected on the grounds that the temperature difference between the droplet and its surroundings is small. This paper includes the effect of radiant heating and cooling of droplets by using the Eddington approximation for the solution of the radiative transfer equation. Although the calculation assumes that the cloud is isothermal and has a constant size spectrum with altitude, the heating or cooling of droplets by radiation changes the growth rate of the droplets very significantly. At the top of a cloud with a base at 2500 m and a top at 3000 m, a droplet will grow from 9.5 to 10.5 microns in about 4 min, assuming a supersaturation ratio of 1.0013. Such a growth rate is more than 20 times the growth rate for condensation alone, and may be expected to have a significant impact on estimates of precipitation formation as well as on droplet spectrum calculations.

Barkstrom, B. R.↗

Chapter 10 - Remote Sensing Measurements of Aerosol Properties

Satellite instruments have proven especially capable at monitoring the quantity of airborne particles in columns of atmosphere, globally. This chapter describes the principles of satellite measurements and retrieval algorithms, and surveys current instruments and their capabilities. We outline the issues associated with retrieval algorithms, such as surface characterization and aerosol proximity to clouds, and the challenges with interpretation of the results. The relationship between measured aerosol properties and climate-relevant aerosol properties simulated in models is outlined, as well as how measurements are used to evaluate models. Most space-based aerosol instruments are passive sensors that measure reflected sunlight at multiple wavelengths, some at multiple viewing angles. A few are active sensors that send out their own laser light and measure the returned signal. Except when clouds are present, the excess amount of light scattered back to space, beyond that expected from the surface and atmospheric gas, is attributed to aerosol. Satellite measurements are used in many ways in aerosol research. They often provide the only method for monitoring hazardous phenomena such as major wildfire and volcanic eruption plumes, especially in remote areas. Stable, long-term, near-global-scale satellite data records make it possible to identify regional and global aerosol trends. Aerosol radiative effects on climate can be quantified on a near-global scale and used to estimate the strength of aerosol–radiation and aerosol–cloud interactions as well as to evaluate climate model simulations of these interactions. Aerosol-type mapping from satellite imagery is helpful for source attribution, model validation, and to constrain particle light-absorption properties that are essential for radiative forcing calculations. The range of aerosol properties retrieved from satellite observations has grown considerably since the first global estimates of aerosol optical depth (τ a) over ocean were made in the late 1970s. Methods for retrieving particle size and light-absorption properties were explored in the 1990s using multispectral, multi-angle observations, and polarization in visible and near-infrared wavelengths. Sensitivity to particle light absorption, primarily from black or brown carbon content, improved with the inclusion of UV channels, and sensitivity to very thin aerosol layers in the upper troposphere and lower stratosphere was advanced with the use of limb-sounding instruments and active sensors. There are limitations to every measurement technique, including satellite aerosol remote sensing. For wide-swath, passive instruments, aerosol retrievals near clouds can present substantial challenges as far as 15 km away due to cloud-scattered light contaminating the signal. In nearly all cases, retrievals over bright snow and ice surfaces are precluded because surface reflectance uncertainties can overwhelm the aerosol signal. Similarly, meteorological cloud is identified and masked out where possible. Data from passive sensors also lack vertical resolution except those that view toward the limb or where multi-angle imagery is acquired over plumes from wildfires, erupting volcanoes, and wind-blown dust. Yet, passive sensors provide vastly more coverage than the active instruments that mitigate these issues. Particle microphysical information is qualitative from all remote sensing techniques, relying on proxies to infer particle composition, hygroscopicity, and the amount of light-absorbing material. Further, particles smaller than about 200 nm diameter cannot be distinguished from atmospheric gas molecules with remote sensing, which hinders studies of cloud condensation nuclei and their effects on clouds. Most satellite instruments dedicated to aerosol observations are in low-Earth, near-polar, sun-synchronous orbits, which means they cross the equator at the same local time each day. Most are set on cycles that repeat approximately every 16 days, which makes it difficult to monitor aerosol evolution locally. Geostationary satellites make it possible to observe changes occurring from minutes to hours over regions up to 8000 km in size, but lack coverage of high latitudes, and often provide more limited constraints on aerosol properties. Ground-truth data are vital for satellite aerosol-retrieval validation. The AErosol RObotic NETwork (AERONET) of sun photometers was created in 1993 and has become an established global network of over 350 instruments for validating satellite measurements. The network, as well as global networks of ground-based lidars, solar flux radiometers and other sun photometers, are widely used for evaluating global satellite retrievals and model simulations. NASA's Earth Observing System (EOS) program beginning in 1999 led to improvements in reliability, spatial resolution, and spectral resolution (and hence, to improved particle size discrimination and light absorption properties). Satellite payloads include advanced broad-swath and multi-angle imagers, along with the first space-based active sensor focused largely on long-term aerosol monitoring. Since about 2002, Europe's SENTINEL and operational meteorological satellite fleets are also providing sustained aerosol observations, with planned continuation until at least 2030. Satellite remote sensing instruments offer valuable data for evaluating aerosol representations in global climate models. They have been used to assess aerosol optical and physical properties, trends and distributions, and are applied increasingly as direct model constraints in data assimilation to create global aerosol reanalysis products. Aerosol optical depth is the most common quantity adopted for routine model evaluation, including multiwavelength data to loosely constrain particle-size distributions. These evaluations of multiple models have revealed general biases in their regional aerosol amounts and seasonal patterns of transport and removal. Although satellite measurements have near-global coverage, substantial errors can be introduced into the model observation comparison unless attention is paid to spatial and temporal collocation, cloud screening, subgrid-scale variability, and measurement uncertainties that vary with retrieval conditions.

aerosol properties↗

Geometrical Effects on the Electromagnetic Radiation from Lightning Return Strokes

The Los Alamos National Laboratory (LANL) Sferic Array has recorded electric-field-change waveforms simultaneously at several stations surrounding the ground-strike points of numerous return strokes in cloud-to-ground lightning flashes. Such data are available from the five-station sub-networks in both Florida and New Mexico. With these data it has been possible for the first time to compare the waveforms radiated in different directions by a given stroke. Such comparisons are of interest to assess both the effects of channel geometry on the fine structure of subsequent-stroke radiation fields and the role of branches in the more jagged appearance of first-stroke waveforms. This paper presents multiple-station, time-domain waveforms with a 200 Hz to 500 kHz pass-band from both first and subsequent return strokes at ranges generally between 100 and 200 km. The differences among waveforms of the same stroke received at stations in different directions from the lightning channel are often obvious. These differences are illustrated and interpreted in the context of channel tortuosity and branches.

Willett, John C.↗

Backscattered UV radiation - Effects of multiple scattering and the lower boundary of the atmosphere

A method is proposed for the calculation of a multiple-scattering correction to the single-scattering calculation of the radiance of the terrestrial atmosphere resulting from backscattered ultraviolet solar radiation in the spectral region used in the ozone profile inversion. This method uses jointly the usual analytical and Monte Carlo methods. Effects of the lower boundary of the atmosphere, cloud tops, and ground surface are investigated both qualitatively and quantitatively. The ratio of multiple to single scattering is determined, and its importance in ozone profile inversion of backscattered UV solar radiation from the terrestrial atmosphere is evaluated. The polarization of the atmospheric radiance is treated briefly.

Aruga, T.↗

On the virial theorem for turbulent molecular clouds

An Eulerian, rather than Lagrangian, form of the virial theorem is derived for a turbulent, magnetized cloud embedded in a steady, turbulent, low-density intercloud medium. The role of turbulent pressure in cloud confinement is clarified, and it is shown that, in the absence of a magnetic field, a cloud can be at a somewhat lower pressure than the intercloud medium. Simple forms for the magnetic term in the virial equation are obtained. Radiation pressure is considered; its effects are relatively small under average conditions in the interstellar medium. Under typical conditions, external pressure and magnetic fields are shown to have a relatively small effect on virial estimates of the mass of self-gravitating clouds.

Mckee, Christopher F.↗

Direct and remote sensing observations of the effects of ships on clouds

Under certain conditions ships can affect the structure of shallow overlying layer clouds. It has been suggested that this is due to particles emitted from the ships, which increase the concentration of cloud condensation nuclei in the air, which, in turn, increases the concentrations of cloud droplets and reduces the average size of the droplets. Two ship track signatures in stratus clouds were observed simultaneously from a satellite and from an aircraft. The airborne measurements showed that in the ship tracks the droplet sizes and concentrations, as well as the total concentrations of particles, were substantially different from those in adjacent clouds. Furthermore, in-situ solar radiation measurements showed a significant enhancement in the upwelling radiance within the ship tracks at visible wavelengths and a significant reduction in radiance at 2.2 micrometers. Remote sensing measurements from the NOAA-10 satellite showed the effects of these differences in cloud structure as an enhancement in cloud reflectivity at 0.63 and 3.7 micrometers. These observations support the contention that ship track signatures in clouds are produced primarily by particles generated by ships.

Radke, Lawrence F.↗

Dependence of tropical cyclone seeds and climate sensitivity on tropical cloud response

Projections of future tropical cyclone frequency are uncertain, ranging from a slight increase to a considerable decrease according to climate models. Estimation of how much the Earth’s surface temperature warms in response to greenhouse gas increase, quantified by effective climate sensitivity, is also uncertain. These two uncertainties have historically been studied independently as they concern different scales: One quantifies the extreme weather and the other the mean climate. Here, we show that these two uncertainties are not independent and are both influenced by the response of tropical clouds to warming. Across climate models, we show an anticorrelation between shortwave cloud radiative feedback and changes in the frequency of seed vortices, a prevalent type of tropical cyclone precursors. We further show an anticorrelation between effective climate sensitivity and tropical cyclone frequency changes, suggesting that global tropical cyclone frequency tends to decrease more substantially in models with larger temperature increase.

Science & Technology - Other Topics↗

Model Intercomparison of Indirect Aerosol Effects

Modeled differences in predicted effects are increasingly used to help quantify the uncertainty of these effects. Here, we examine modeled differences in the aerosol indirect effect in a series of experiments that help to quantify how and why model-predicted aerosol indirect forcing varies between models. The experiments start with an experiment in which aerosol concentrations, the parameterization of droplet concentrations and the autoconversion scheme are all specified and end with an experiment that examines the predicted aerosol indirect forcing when only aerosol sources are specified. Although there are large differences in the predicted liquid water path among the models, the predicted aerosol first indirect effect for the first experiment is rather similar, about -0.6 W/sq m to -0.7 W/sq m. Changes to the autoconversion scheme can lead to large changes in the liquid water path of the models and to the response of the liquid water path to changes in aerosols. Adding an autoconversion scheme that depends on the droplet concentration caused a larger (negative) change in net outgoing shortwave radiation compared to the 1st indirect effect, and the increase varied from only 22% to more than a factor of three. The change in net shortwave forcing in the models due to varying the autoconversion scheme depends on the liquid water content of the clouds as well as their predicted droplet concentrations, and both increases and decreases in the net shortwave forcing can occur when autoconversion schemes are changed. The parameterization of cloud fraction within models is not sensitive to the aerosol concentration, and, therefore, the response of the modeled cloud fraction within the present models appears to be smaller than that which would be associated with model "noise". The prediction of aerosol concentrations, given a fixed set of sources, leads to some of the largest differences in the predicted aerosol indirect radiative forcing among the models, with values of cloud forcing ranging from -0.3 W/sq m to -1.4W/sq m. Thus, this aspect of modeling requires significant improvement in order to improve the prediction of aerosol indirect effects.

Penner, J. E.↗

TPSAS-NF1676L-30044-DND

The Clouds and the Earth's Radiant Energy System (CERES) project now has over 17 years accurately observed top-of-the-atmosphere (TOA) flux record for climate monitoring and diagnostic studies. The CERES FluxByCldTyp dataset, which contains cloud properties and radiative fluxes for 42 cloud types sorted by cloud top pressure and cloud optical depth, is used to investigate the clouds and their associated TOA (top-of-the-atmosphere) fluxes changes over the tropical area during ENSO events during the observed period. Unlike past studies, this study shows the impact of ENSO on cloud properties like optical depth, cloud top effective pressure and temperature and TOA LW and SW fluxes for each sub cloud type. The study reveals the detailed contributions from different cloud types for radiative characteristics during different regimes of ENSOs. This is especially important for very small net TOA radiative balance due to the cancellation of the fluxes from different cloud types. The dataset serves as a more stringent validation of climate models for cloud properties and radiative fluxes.

Sun, Moguo↗

ENSO Tropical Cloud and TOA radiative signatures from the CERES observation

The Clouds and the Earth's Radiant Energy System (CERES) project now has over 15 years accurately observed top-of-the-atmosphere (TOA) flux record for climate monitoring and diagnostic studies. The CERES flux-by-cloud-type dataset, which contains cloud properties and radiative fluxes for 42 cloud types sorted by cloud top pressure and cloud optical depth, is used to investigate the clouds and their associated TOA (top-of-the-atmosphere) fluxes changes over the tropical area during ENSO events during the observed period. Unlike past studies, this study shows the impact of ENSO on cloud properties like optical depth, cloud top effective pressure and temperature and TOA LW and SW fluxes for each sub cloud type. The study reveals the detailed contributions from different cloud types for radiative characteristics during different phases of ENSO. This is especially important for very small net TOA radiative balance due to the cancellation of the fluxes from different cloud types. To further demonstrate the usefulness of this dataset, NCAR Community Atmosphere Model (CAM) is used to simulate the cloud and radiative changes during the period. The model cloud properties are converted to MODIS like cloud properties using modified MODIS simulator. The dataset serves as a more stringent validation of the model for cloud properties and radiative fluxes.

Moguo Sun↗

Reduction of Cloud Water in Ship Tracks: Observations and Large-Eddy Simulations

Ship tracks represent a natural laboratory to study the effects of aerosols on clouds. A number of observations and simulations have shown that increased droplet concentrations in ship tracks increase their total cross-sectional area, thereby enhancing cloud albedo and providing a negative radiative forcing at the surface and the top of the atmosphere. In some cases, cloud water has been found to be enhanced in ship tracks, which has been attributed to suppression of drizzle and implies an enhanced susceptibility of cloud albedo to droplet concentrations. However, more recently compiled observations indicate that cloud water is instead reduced in daytime ship tracks on average. Such a response is consistent with cloud-burning due to solar absorption by soot (the semi-direct radiative forcing of aerosols), recently suggested to be suppressing trade cumulus cloud coverage over the Indian Ocean. We will summarize observational evidence and present large-eddy simulations that consider these competing mechanisms in the effects of aerosols on cloud albedo.

Ackerman, A. S.↗

Midlatitude Cirrus Clouds Derived from Hurricane Nora: A Case Study with Implications for Ice Crystal Nucleation and Shape

Hurricane Nora traveled up the Bala Peninsula coast in the unusually warm El Nino waters of September 1997, until rapidly decaying as it approached Southern California on 24 September. The anvil cirrus blowoff from the final surge of tropical convection became embedded in subtropical flow that advected the cirrus across the western US, where it was studied from the Facility for Atmospheric Remote Sensing (FARS) in Salt Lake City, Utah. A day later, the cirrus shield remnants were redirected southward by midlatitude circulations into the Southern Great Plains, providing a case study opportunity for the research aircraft and ground-based remote sensors assembled at the Clouds and Radiation Testbed (CART) site in northern Oklahoma. Using these comprehensive resources and new remote sensing cloud retrieval algorithms, the microphysical and radiative cloud properties of this unusual cirrus event are uniquely characterized. Importantly, at both the FARS and CART sites the cirrus generated spectacular optical displays, which acted as a tracer for the hurricane cirrus, despite the limited lifetimes of individual ice crystals. Lidar polarization data indicate widespread regions of uniform ice plate orientations, and in situ particle masticator data show a preponderance of pristine, solid hexagonal plates and columns. It is suggested that these unusual aspects are the result of the mode of cirrus particle nucleation, presumably involving the lofting of sea-salt nuclei in thunderstorm updrafts into the upper troposphere. This created a reservoir of haze particles that continued to produce halide-saltcontaminated ice crystals during the extended period of cirrus cloud maintenance. The reference that marine microliters are embedded in the replicas of ice crystals collected over the CART site points to the longevity of marine effects. Various nucleation scenarios proposed for cirrus clouds based on this and other studies, and the implications for understanding cirrus radiative properties or a global scale, are discussed.

Sassen, Kenneth↗

Response to "The Iris Hypothesis: A Negative or Positive Cloud Feedback?"

Based on radiance measurements of Japan's Geostationary Meteorological Satellite, Lindzen et al. found that the high-level cloud cover averaged over the tropical western Pacific decreases with increasing sea surface temperature. They further found that the response of high-level clouds to the sea surface temperature had an effect of reducing the magnitude of climate change, which is referred as a negative climate feedback. Lin et al. reassessed the results found by Lindzen et al. by analyzing the radiation and clouds derived from the Tropical Rainfall Measuring Mission Clouds and the Earth's Radiant Energy System measurements. They found a weak positive feedback between high-level clouds and the surface temperature. We have found that the approach taken by Lin et al. to estimating the albedo and the outgoing longwave radiation is incorrect and that the inferred climate sensitivity is unreliable.

Chou, Ming-Dah↗