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NASA NTRS2020

AWARE: The Atmospheric Radiation Measurement (ARM) West Antarctic Radiation Experiment

The US Department of Energy Atmospheric Radiation Measurement (ARM) West Antarctic Radiation Experiment (AWARE) performed comprehensive meteorological and aerosol measurements, and ground-based atmospheric remote sensing at two Antarctic stations using the most advanced instrumentation available. A suite of cloud research radars, lidars, spectral and broadband radiometers, aerosol chemical and microphysical sampling equipment, and meteorological instrumentation was deployed at McMurdo Station on Ross Island from December 2015 through December 2016. A smaller suite of radiometers and meteorological equipment including radiosondes, optimized for surface energy budget measurement, was deployed on the West Antarctic Ice Sheet between 4 December 2015 and 17 January 2016. AWARE provided Antarctic atmospheric data comparable to several well-instrumented high Arctic sites that have operated for many years and that reveal numerous contrasts with the Arctic in aerosol and cloud microphysical properties. These include persistent differences in liquid cloud occurrence, cloud height and cloud thickness. Antarctic aerosol properties are also quite different from the Arctic in both seasonal cycle and composition, due to the continent’s isolation from lower latitudes by Southern Ocean storm tracks. Antarctic aerosol number and mass concentrations are not only non-negligible but perhaps play a more important role than previously recognized because of the higher sensitivities of clouds at the very low concentrations caused by the large-scale dynamical isolation. Antarctic aerosol chemical composition, particularly organic components, has implications for local cloud microphysics. The AWARE data set, fully available online in the ARM Program data archive, offers numerous case studies for unique and rigorous evaluation of mixed-phase cloud parameterization in climate models.

Atmospheric Radiation Measurement (ARM)↗

DOE OSTI2024

Partition between supercooled liquid droplets and ice crystals in mixed-phase clouds based on airborne in situ observations

Abstract. The onset of ice nucleation in mixed-phase clouds determines the lifetime and microphysical properties of ice clouds. In this work, we develop a novel method that differentiates between various phases of mixed-phase clouds, such as clouds dominated by pure liquid or pure ice segments, compared with those having ice crystals surrounded by supercooled liquid water droplets or vice versa. Using this method, we examine the relationship between the macrophysical and microphysical properties of Southern Ocean mixed-phase clouds at −40 to 0 °C (e.g. stratiform and cumuliform clouds) based on the in situ aircraft-based observations during the US National Science Foundation Southern Ocean Clouds, Radiation, Aerosol Transport Experimental Study (SOCRATES) flight campaign. The results show that the exchange between supercooled liquid water and ice crystals from a macrophysical perspective, represented by the increasing spatial ratio of regions containing ice crystals relative to the total in-cloud region (defined as ice spatial ratio), is positively correlated with the phase exchange from a microphysical perspective, represented by the increasing ice water content (IWC), decreasing liquid water content (LWC), increasing ice mass fraction, and increasing ice particle number fraction (IPNF). The mass exchange between liquid and ice becomes more significant during phase 3 when pure ice cloud regions (ICRs) start to appear. Occurrence frequencies of cloud thermodynamic phases show a significant phase change from liquid to ice at a similar temperature (i.e. −17.5 °C) among three types of definitions of mixed-phase clouds based on ice spatial ratio, ice mass fraction, or IPNF. Aerosol indirect effects are quantified for different phases using number concentrations of aerosols greater than 100 or 500 nm (N>100 and N>500, respectively). N>500 shows stronger positive correlations with ice spatial ratios compared with N>100. This result indicates that larger aerosols potentially contain ice-nucleating particles (INPs), which facilitate the formation of ice crystals in mixed-phase clouds. The impact of N>500 is also more significant in phase 2 when ice crystals just start to appear in the mixed phase compared with phase 3 when pure ICRs have formed, possibly due to the competing aerosol indirect effects on primary and secondary ice production in phase 3. The thermodynamic and dynamic conditions are quantified for each phase. The results show stronger in-cloud turbulence and higher updraughts in phases 2 and 3 when liquid and ice coexist compared with pure liquid or ice (phases 1 and 4, respectively). The highest updraughts and turbulence are seen in phase 3 when supercooled liquid droplets are surrounded by ice crystals. These results indicate both updraughts and turbulence support the maintenance of supercooled liquid water amongst ice crystals. Overall, these results illustrate the varying effects of aerosols, thermodynamics, and dynamics through various stages of mixed-phase cloud evolution based on this new method that categorizes cloud phases.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2026

Evaluating the Collision‐Coalescence Process in Idealized Cloud Convection Using Large‐Eddy Simulations With Lagrangian Microphysics

Drizzle initiation through the collision and coalescence of cloud droplets plays a crucial role in warm cloud precipitation. Recent theoretical studies suggest that the influence of collisional growth on the droplet size distribution can be quantified by a non-dimensional drizzle number (Dz). Here, large-eddy simulations with Lagrangian microphysics are employed to evaluate the theory by simulating a tall convection-cloud chamber under various conditions. Results show that the smaller the Dz, the larger the impact of collisions on the right tail of the droplet size distribution, consistent with the theory. The simulations confirm that the collision rate can be estimated from the droplet size distribution interacting only with cloud droplets of the same size at the mode radius. This suggests that the idealized theory can be a useful tool to design a cloud chamber for drizzle investigation, as well as to represent drizzle formation in models of real atmospheric clouds.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2015

Holistic Interactions of Shallow Clouds, Aerosols, and Land-Ecosystems (HI-SCALE) Science Plan

Cumulus convection is an important component in the atmospheric radiation budget and hydrologic cycle over the Southern Great Plains and over many regions of the world, particularly during the summertime growing season when intense turbulence induced by surface radiation couples the land surface to clouds. Current convective cloud parameterizations contain uncertainties resulting in part from insufficient coincident data that couples cloud macrophysical and microphysical properties to inhomogeneities in boundary layer and aerosol properties. The Holistic Interactions of Shallow Clouds, Aerosols, and Land-Ecosystems (HI-SCALE) campaign is designed to provide a detailed set of measurements that are needed to obtain a more complete understanding of the life cycle of shallow clouds by coupling cloud macrophysical and microphysical properties to land surface properties, ecosystems, and aerosols. HI-SCALE consists of 2, 4-week intensive observational periods, one in the spring and the other in the late summer, to take advantage of different stages and distribution of “greenness” for various types of vegetation in the vicinity of the Atmospheric Radiation and Measurement (ARM) Climate Research Facility’s Southern Great Plains (SGP) site as well as aerosol properties that vary during the growing season. Most of the proposed instrumentation will be deployed on the ARM Aerial Facility (AAF) Gulfstream 1 (G-1) aircraft, including those that measure atmospheric turbulence, cloud water content and drop size distributions, aerosol precursor gases, aerosol chemical composition and size distributions, and cloud condensation nuclei concentrations. Routine ARM aerosol measurements made at the surface will be supplemented with aerosol microphysical properties measurements. The G-1 aircraft will complete transects over the SGP Central Facility at multiple altitudes within the boundary layer, within clouds, and above clouds.

Fast, JD↗

NASA NTRS1998

Monte Carlo Calculations of Polarized Microwave Radiation Emerging from Cloud Structures

The last decade has seen tremendous growth in cloud dynamical and microphysical models that are able to simulate storms and storm systems with very high spatial resolution, typically of the order of a few kilometers. The fairly realistic distributions of cloud and hydrometeor properties that these models generate has in turn led to a renewed interest in the three-dimensional microwave radiative transfer modeling needed to understand the effect of cloud and rainfall inhomogeneities upon microwave observations. Monte Carlo methods, and particularly backwards Monte Carlo methods have shown themselves to be very desirable due to the quick convergence of the solutions. Unfortunately, backwards Monte Carlo methods are not well suited to treat polarized radiation. This study reviews the existing Monte Carlo methods and presents a new polarized Monte Carlo radiative transfer code. The code is based on a forward scheme but uses aliasing techniques to keep the computational requirements equivalent to the backwards solution. Radiative transfer computations have been performed using a microphysical-dynamical cloud model and the results are presented together with the algorithm description.

Kummerow, Christian↗

DOE OSTI2017

Holistic Interactions of Shallow Clouds, Aerosols, and Land-Ecosystems (HI-SCALE) Field Campaign Report

Cumulus convection is an important component in the atmospheric radiation budget and hydrologic cycle over the southern Great Plains and over many regions of the world, particularly during the summertime growing season when intense turbulence induced by surface radiation couples the land surface to clouds. Current convective cloud parameterizations contain uncertainties resulting in part from insufficient coincident data that couples cloud macrophysical and microphysical properties to inhomogeneities in land surface, boundary layer, and aerosol properties. The Holistic Interactions of Shallow Clouds, Aerosols, and Land-Ecosystems (HI-SCALE) campaign was designed to provide a detailed set of measurements that are needed to obtain a more complete understanding of the lifecycle of shallow clouds by coupling cloud macrophysical and microphysical properties to land surface properties, ecosystems, and aerosols. Some of the land-atmosphere-cloud interactions that can be studied using HI-SCALE data are shown in Figure 1. HI-SCALE consisted of two 4-week intensive operation periods (IOPs), one in the spring (April 24-May 21) and the other in the late summer (August 28-September 24) of 2016, to take advantage of different stages of the plant lifecycle, the distribution of “greenness” for various types of vegetation in the vicinity of the U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) Climate Research Facility Southern Great Plains (SGP) site, and aerosol properties that vary during the growing season. As expected, satellite measurements indicated that the Normalized Difference Vegetation Index (NDVI) was much “greener” in the vicinity of the SGP site during the spring IOP than the late summer IOP as a result of winter wheat maturing in the spring and being harvested in the early summer. As shown in Figure 2, temperatures were cooler than average and soil moisture was high during the spring IOP, while temperatures were warmer than average and soil moisture was low during the late summer IOP. These factors likely influence the occurrence and lifecycle of shallow clouds. Most of the instrumentation was deployed on the ARM Aerial Facility (AAF) Gulfstream 1 (G-1) aircraft, including those that measure atmospheric turbulence, cloud water content and drop size distributions, aerosol precursor gases, aerosol chemical composition and size distributions, and cloud condensation nuclei (CCN) concentrations. The specific instrumentation is listed in Table 1. The team of scientists participating in the G-1 flights were from Pacific Northwest National Laboratory (PNNL), Brookhaven National Laboratory (BNL), and the University of Washington. Routine ARM aerosol measurements made at the surface were supplemented with aerosol microphysical properties measurements, with support from the DOE Environmental Molecular Sciences Laboratory (EMSL) User Facility and the Atmospheric System Radiation (ASR) program. This included deploying a scanning mobility particle sizer (SMPS) to measure aerosol size distribution, a proton transfer reaction-mass spectrometer (PTR-MS) to measure volatile organic compounds, an aerosol mass spectrometer (AMS) to measure bulk aerosol composition, and the single-particle laser ablation time-of-flight mass spectrometer (SPLAT II) to measure single-particle aerosol composition at the SGP site Guest Instrumentation Facility. In this way, characterization of aerosol properties at the surface and on the G-1 were consistent. In addition, the HI-SCALE: Nanoparticle Composition and Precursors add-on campaign was conducted during the second IOP in which several state-of-the-science chemical ionization mass spectrometers were deployed to measure nanoparticle composition and precursors. Scientists participating in the surface measurements were from PNNL, BNL, University California–Irvine, Augsberg College, Colorado University, Aerodyne Inc., and Aerosol Dynamics Inc.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2023

Insights of warm-cloud biases in Community Atmospheric Model 5 and 6 from the single-column modeling framework and Aerosol and Cloud Experiments in the Eastern North Atlantic (ACE-ENA) observations

There has been a growing concern that most climate models predict precipitation that is too frequent, likely due to lack of reliable subgrid variability and vertical variations in microphysical processes in low-level warm clouds. In this study, the warm-cloud physics parameterizations in the singe-column configurations of NCAR Community Atmospheric Model version 6 and 5 (SCAM6 and SCAM5, respectively) are evaluated using ground-based and airborne observations from the Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) Aerosol and Cloud Experiments in the Eastern North Atlantic (ACE-ENA) field campaign near the Azores islands during 2017–2018. The 8-month single-column model (SCM) simulations show that both SCAM6 and SCAM5 can generally reproduce marine boundary layer cloud structure, major macrophysical properties, and their transition. The improvement in warm-cloud properties from the Community Atmospheric Model 5 and 6 (CAM5 to CAM6) physics can be found through comparison with the observations. Meanwhile, both physical schemes underestimate cloud liquid water content, cloud droplet size, and rain liquid water content but overestimate surface rainfall. Modeled cloud condensation nuclei (CCN) concentrations are comparable with aircraft-observed ones in the summer but are overestimated by a factor of 2 in winter, largely due to the biases in the long-range transport of anthropogenic aerosols like sulfate. We also test the newly recalibrated autoconversion and accretion parameterizations that account for vertical variations in droplet size. Compared to the observations, more significant improvement is found in SCAM5 than in SCAM6. This result is likely explained by the introduction of subgrid variations in cloud properties in CAM6 cloud microphysics, which further suppresses the scheme's sensitivity to individual warm-rain microphysical parameters. The predicted cloud susceptibilities to CCN perturbations in CAM6 are within a reasonable range, indicating significant progress since CAM5 which produces an aerosol indirect effect that is too strong. The present study emphasizes the importance of understanding biases in cloud physics parameterizations by combining SCM with in situ observations.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2016

Final DOE-ASR Report for the Project “Advancing our Understanding and the Remote Sensing of Ice Clouds”

This project has evolved during its execution, and what follows are the key project findings. This project has arguably provided the first global view of how cirrus cloud (defined as having cloud base temperature T < 235 K) nucleation physics (evaluated through satellite retrievals of ice particle number concentration Ni, effective diameter De and ice water content IWC) evolves with the seasons for a given temperature, latitude zone and surface type (e.g. ocean vs. land), based on a new satellite remote sensing method developed for this project. The retrieval method is unique in that it is very sensitive to the small ice crystals that govern the number concentration Ni, allowing Ni to be retrieved. The method currently samples single-layer cirrus clouds having visible optical depth ranging from about 0.3 to 3.0, using co-located observations from the Infrared Imaging Radiometer (IIR) and from the CALIOP (Cloud and Aerosol Lidar with Orthogonal Polarization) lidar aboard the CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation) polar orbiting satellite, employing IIR channels at 10.6 μm and 12.05 μm. Retrievals of Ni are primarily used to estimate the cirrus cloud formation mechanism; that is, either homo- or heterogeneous ice nucleation (henceforth hom and het). This is possible since, in general, hom produces more than an order of magnitude more ice crystals than does het. Thus the retrievals provide insight on how these mechanisms change with the seasons for a given latitude zone or region, based on the years 2008 and 2013. Using a conservative criterion for hom cirrus, on average, the sampled cirrus clouds formed through hom occur about 43% of the time in the Arctic and 50% of the time in the Antarctic, and during winter at mid-latitudes in the Northern Hemisphere, hom cirrus occur 37% of the time. Elsewhere (and during other seasons in the Northern Hemisphere mid-latitudes), this hom cirrus fraction is lower, and it is lowest in the tropics. Thus, the microphysical properties of cirrus clouds in the Polar Regions are much different than they are in the tropics; something unknown prior to this study. Moreover, the frequency of cirrus cloud occurrence in the Polar Regions varies strongly with season, peaking during winter in the Arctic and during spring in the Antarctic. Considering these seasonal changes in microphysics and inferred cloud coverage, this leads us to speculate that the buildup of Arctic cirrus during winter may significantly contribute to tropospheric heating in that region, possibly affecting winter jet-stream dynamics and mid-latitude weather patterns through the thermal-wind balance relationship. This cirrus cloud research provides essential guidance for realistically representing cirrus clouds in climate models; guidance previously unavailable. For example, mid-latitude hom cirrus were widespread during winter over or nearby mountainous terrain, evidently due to mountain-induced waves that produce strong updrafts at cirrus cloud levels. The treatment of turbulent mountain stress and gravity waves will likely need to be improved in climate models in order to adequately represent cirrus clouds outside the tropics. Another goal of this project was to develop a ground-based 94-GHz radar retrieval for winter snowstorms, based on (1) an improved analytical framework describing the interaction of radiation from radar with snowfall and (2) the development of a steady-state snow growth model that predicts the height-evolution of the ice particle size distribution through ice particle growth by vapor diffusion, aggregation and riming (i.e. the growth of snow through collisions with supercooled cloud droplets). Although activities (1) and (2) were completed, there was insufficient time to test and finalize the radar retrieval scheme. However, activity (2) provided a new method for relating ice particle mass “m” and projected area “A” to the ice particle maximum dimension “D”. The ice cloud microphysical processes (which determine ice cloud radiative properties) in climate models are parameterized in terms of these m-D and A-D relationships. By improving these relationships, the ice cloud radiative properties in Community Atmosphere Model version 5, or CAM5 (an atmosphere global climate model, or GCM) were improved. Student funding from the University of Nevada, Reno, was combined with funds from this project to conduct some basic research on the mechanism of the North American monsoon, or NAM. Federal research on the NAM has dwindled since 2006, but atmospheric soundings taken during research vessel cruises in the Gulf of California (GC) during the North American Monsoon Experiment (NAME) were used to reveal a likely mechanism that explains the relationship between an intrusion of tropical warm water into the GC during late spring-early summer and the onset of relatively heavy NAM rainfall in northwest Mexico and the southwestern United States. These soundings, combined with reanalysis data, satellite sea surface temperatures and satellite measurements of outgoing longwave radiation were used to develop and provide evidence for a planetary-scale NAM mechanism. As far as we know, no other physical explanation has been offered for the spring-summer evolution of the NAM system.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1990

The polar stratospheric cloud event of January 24, 1989. I - Microphysics

Rapid adiabatic cooling induced by synoptic forcing led to polar stratospheric cloud (PSC) formation on January 24, 1989, at altitudes sampled by the ER-2 aircraft. Particle characteristics measured by the Forward Scattering Spectrometer Probe (FSSP) on the ER-2 were compared to those calculated using a theoretical PSC microphysics model. Although calculations were sensitive to local changes in cooling rate, generally favorable agreement was found, that in particle surface area being especially important since this parameter dictates heterogeneous chemical rates. The overall model performance suggests that the current approach for simulating Type 1 (nitric acid trihydrate) PSC formation under rapid cooling conditions is well founded and can be used to study the effects of heterogeneous chemistry on stratospheric composition.

Poole, L. R.↗

DOE OSTI2022

Shallow Cumulus Properties as Captured by Adiabatic Fraction in High-Resolution LES Simulations

Abstract Shallow convective clouds are important players in Earth’s energy budget and hydrological cycle, and are abundant in the tropical and subtropical belts. They greatly contribute to the uncertainty in climate predictions due to their unresolved, complex processes that include coupling between the dynamics and microphysics. Analysis of cloud structure can be simplified by considering cloud motions as a combination of moist adiabatic motions like adiabatic updrafts and turbulent motions leading to deviation from adiabaticity. In this work, we study the sizes and occurrence of adiabatic regions in shallow cumulus clouds during their growth and mature stages, and use the adiabatic fraction (AF) as a continuous metric to describe cloud processes and properties from the core to the edge. To do so, we simulate isolated trade wind cumulus clouds of different sizes using the System of Atmospheric Modeling (SAM) model in high resolution (10 m) with the Hebrew University spectral bin microphysics (SBM). The fine features in the clouds’ dynamics and microphysics, including small near-adiabatic volumes and a thin transition zone at the edge of the cloud (∼20–40 m in width), are captured. The AF is shown to be an efficient measure for analyzing cloud properties and key processes determining the droplet-size distribution formation and shape during the cloud evolution. Physical processes governing the properties of droplet size distributions at different cloud regions (e.g., core, edge) are analyzed in relation to AF. Significance Statement 1) This study investigates the evolution of cumulus clouds (Cu) using a 10-m-resolution LES model with spectral bin microphysics. 2) The study improves the understanding of the mutual effects of adiabatic updrafts and lateral entrainment and mixing. 3) The study demonstrates the existence of an adiabatic core in nonprecipitating Cu. 4) Shapes of the droplet size distributions are closely related to the adiabatic fraction values. 5) Utilization of high resolution reveals the existence of physically significant small features in the cloud structure, such as a narrow cloud interface zone and small adiabatic volumes.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS2003

Global Multispectral Cloud Retrievals from MODIS

The Moderate Resolution Imaging Spectroradiometer (MODIS) was developed by NASA and launched onboard the Terra spacecraft on December 18,1999 and Aqua spacecraft on May 4,2002. It achieved its final orbit and began Earth observations on February 24, 2000 for Terra and June 24, 2002 for Aqua. A comprehensive set of remote sensing algorithms for cloud masking and the retrieval of cloud physical and optical properties has been developed by members of the MODIS atmosphere science team. The archived products from these algorithms have applications in climate change studies, climate modeling, numerical weather prediction, as well as fundamental atmospheric research. In addition to an extensive cloud mask, products include cloud-top properties (temperature, pressure, effective emissivity), cloud thermodynamic phase, cloud optical and microphysical parameters (optical thickness, effective particle radius, water path), as well as derived statistics. We will describe the various cloud properties being analyzed on a global basis from both Terra and Aqua, and will show characteristics of cloud optical and microphysical properties as a function of latitude for land and ocean separately, and contrast the statistical properties of similar cloud types in various parts of the world.

King, Michael D.↗

NASA NTRS2003

Global Multispectral Cloud Retrievals from MODIS

King, Michael D.↗

DOE OSTI2016

A long-term study of aerosol–cloud interactions and their radiative effect at the Southern Great Plains using ground-based measurements

Empirical estimates of the microphysical response of cloud droplet size distribution to aerosol perturbations are commonly used to constrain aerosol–cloud interactions in climate models. Instead of empirical microphysical estimates, here macroscopic variables are analyzed to address the influence of aerosol particles and meteorological descriptors on instantaneous cloud albedo and the radiative effect of shallow liquid water clouds. Long-term ground-based measurements from the Atmospheric Radiation Measurement (ARM) program over the Southern Great Plains are used. A broad statistical analysis was performed on 14 years of coincident measurements of low clouds, aerosol, and meteorological properties. Here two cases representing conflicting results regarding the relationship between the aerosol and the cloud radiative effect were selected and studied in greater detail. Microphysical estimates are shown to be very uncertain and to depend strongly on the methodology, retrieval technique and averaging scale. For this continental site, the results indicate that the influence of the aerosol on the shallow cloud radiative effect and albedo is weak and that macroscopic cloud properties and dynamics play a much larger role in determining the instantaneous cloud radiative effect compared to microphysical effects. On a daily basis, aerosol shows no correlation with cloud radiative properties (correlation = -0.01 ± 0.03), whereas the liquid water path shows a clear signal (correlation = 0.56 ± 0.02).

54 ENVIRONMENTAL SCIENCES↗

NASA NTRSDate not supplied

Survey of microphysical properties of marine boundary-layer clouds in the Western North Atlantic

Oceanic low level clouds strongly affect the atmospheric radiation budget. Uncertainties in their microphysical properties and cover currently limit the accuracy of climate predictions. Further, studies quantifying the relative importance of aerosol and dynamics on cloud properties in specific meteorological regimes are poorly constrained by observations in the Western North Atlantic boundary layer. Low level clouds were measured during the Aerosol Cloud meTereology Interactions oVer the western ATlantic Experiment (ACTIVATE) campaign in winter and summer 2020. The two NASA LaRC research aircraft HU-25 Falcon and UC-12 B-200 King Air conducted 35 simultaneous flights to investigate aerosol-cloud interactions of maritime clouds and their impact on radiation. Number concentration, liquid water content, ice water content, and particle size distribution in the size range of 3 µm to 1460 µm in diameter were measured with the fast forward scattering cloud probe (FCDP) and 2-dimensional optical array imaging probe (2D-S) onboard the Falcon. Here, we present an overview of late winter (February-March) and late summer (August-September) oceanic cloud properties in the region 65°W to 80°W and 30°N to 40°N. We compare cloud properties in these two seasons and investigate their dependence on meteorological parameters and aerosol abundance. In a case study, we present cloud observations in a cold air outbreak event on 1 March 2020 with a specific focus on mixed-phase clouds.

microphysical properties↗

DOE OSTI2014

Statistical characteristics of cloud variability. Part 2: Implication for parameterizations of microphysical and radiative transfer processes in climate models

The effects of subgrid cloud variability on grid-average microphysical rates and radiative fluxes are examined by use of long-term retrieval products at the Tropical West Pacific, Southern Great Plains, and North Slope of Alaska sites of the Department of Energy's Atmospheric Radiation Measurement program. Four commonly used distribution functions, the truncated Gaussian, Gamma, lognormal, and Weibull distributions, are constrained to have the same mean and standard deviation as observed cloud liquid water content. The probability density functions are then used to upscale relevant physical processes to obtain grid-average process rates. It is found that the truncated Gaussian representation results in up to 30% mean bias in autoconversion rate, whereas the mean bias for the lognormal representation is about 10%. The Gamma and Weibull distribution function performs the best for the grid-average autoconversion rate with the mean relative bias less than 5%. For radiative fluxes, the lognormal and truncated Gaussian representations perform better than the Gamma and Weibull representations. The results show that the optimal choice of subgrid cloud distribution function depends on the nonlinearity of the process of interest, and thus, there is no single distribution function that works best for all parameterizations. Examination of the scale (window size) dependence of the mean bias indicates that the bias in grid-average process rates monotonically increases with increasing window sizes, suggesting the increasing importance of subgrid variability with increasing grid sizes.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2016

Regime dependence of cloud condensate variability observed at the Atmospheric Radiation Measurement Sites

Microphysical processes and cloud–radiation interaction occur on spatial scales of variability smaller than those represented explicitly in global weather forecasting and climate models. It is therefore necessary to parametrize the unresolved heterogeneity of humidity and cloud condensate in order to predict process rates accurately. Ground‐based observations from the Atmospheric Radiation Measurement sites located in various climatic regions of the world provide a source of high‐temporal‐resolution observations of cloud condensate. A number of different retrieval products for cloud condensate are assessed for the different geographical regions, years and seasons. The retrieval reliability varies with cloud type, but for cloud categories largely unaffected by precipitation a comparison across sites and longer time periods is possible. These observations confirm previously documented variability behaviour as a function of cloud fraction, but also reveal a systematic regime dependence that is not captured by existing parametrizations. Condensate variability measured as a fractional standard deviation (FSD) in warm boundary‐layer clouds is greater in the Tropics than in mid and high latitudes for scenes with comparable cloud type and fraction, with the observed FSD varying from 1.2 in the Tropics to 0.4 in the Arctic. A parametrization of the FSD of cloud liquid condensate based on the grid‐box mean total water amount and cloud fraction is formulated and shown to capture the observed range of FSD values better across different geographical sites and different seasons. The regime dependence of FSD for cirrus cloud is less pronounced than that for liquid clouds and is found largely to agree with FSD values previously derived from satellite observations.

Ahlgrimm, Maike↗

NASA NTRS2019

Laboratory Investigations of Cloud Particle Formation and Sublimation on Titan, Mars, and Earth

Microphysical modeling of cloud formation and growth relies on fundamental measurements of the properties of condensable gases which form cloud particles. NASA's Ames Chemistry Laboratory has the capability to measure vapor pressures and heterogeneous nucleation conditions for a variety of gases found in the atmospheres of solar system bodies. Highlights from work for Earth, Mars, and Titan demonstrate the range of conditions and atmospheres studied to date.

Iraci, Laura T.↗

DOE OSTI2018

Polar Liquid Cloud Base Detection Algorithms for High Spectral Resolution or Micropulse Lidar Data

Liquid layers in clouds affect their microphysical processes, as well as the atmospheric energy budget. However, explicit liquid cloud base height (LCBH) detection algorithms using ground-based instruments (e.g., lidars) are currently absent in the literature. Most studies use either fixed lidar parameter thresholds or cloud base height data products that do not distinguish between ice and liquid, all of which might introduce inconsistencies and errors in the resolved LCBHs. In this paper, two LCBH detection algorithms are presented; the first algorithm uses the high spectral resolution lidar (HSRL) data, and yields satisfactory results. The second algorithm incorporates micropulse lidar (MPL) data for the LCBH detection. A 1-year long comparison of data gathered at Barrow, Alaska, and McMurdo Station, Antarctica, which includes other cloud base detection methodologies (ceilometer, MPL value-added product cloud base height, LCBHs detected using a fixed MPL depolarization threshold) emphasize the merits of the MPL algorithm.

Silber, Israel↗