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At least 973 records · Page 54

PACE Microphysical Aerosol Properties from Polarimetry (PACE-MAPP)

We present the Plankton, Aerosols, Clouds and Ecosystems Microphysical Aerosol Properties from Polarimetry (PACE-MAPP) polarimetric remote sensing algorithm developed for the newly launched NASA PACE satellite observing system. The objective of PACE-MAPP is to retrieve detailed fine-mode (marine, pollution and smoke) and coarse-mode (sea-salt and dust) aerosol properties over the ocean for a range of light to heavy aerosol loadings using PACE’s polarimetric-imaging capabilities at multiple angles and wavelengths from the ultraviolet (UV) to the near-infrared (NIR). An additional objective for PACE-MAPP is to discriminate aerosols from thin clouds. The PACE-MAPP polarimetric remote sensing retrieval algorithm uses coupled atmosphere-ocean vector radiative transfer, optimal estimation, artificial intelligence and powerful inherent optical property look-up-tables for the Earth’s aerosol, cloud, and hydrosol particles. PACE-MAPP is the only retrieval algorithm designed to invert aerosol/ocean products using both polarimeters onboard PACE. We present results using PACE-MAPP to retrieve aerosol and ocean remote sensing products from measurements by the Hyper-Angular Rainbow Polarimeter #2 (HARP2) and Spectro-polarimeter for Planetary Exploration one (SPEXone) polarimeter instruments onboard PACE.

Snorre Stamnes↗

Performance of black silicon photodiodes for VUV detection in noble liquids

Black silicon (b-Si) photodiodes are an emerging technology that employs silicon nanostructures to enhance the efficiency of photon detection. Recently, we demonstrated nearly 100% quantum efficiency at <200 nm vacuum ultraviolet (VUV) wavelengths at ambient and in noble liquids, making such devices particularly useful for direct detection of scintillation light in noble liquid detectors. This is important in nuclear science experiments like DarkSide, LUX, XENON, and nEXO, where detection of weak VUV scintillation photons in noble liquids are used to identify rare physics radiation events. Here, we measured the response of b-Si photodiode to the scintillation light generated by alpha particles, all immersed in a LAr and LXe test cell. We established a guideline for future development of b-Si photodetectors with internal gain to reach single-photon sensitivity.

47 OTHER INSTRUMENTATION↗

A recent time of minimum for and atmospheric-eclipse in the ultraviolet spectrum of the Wolf-Rayet eclipsing binary V444 Cygni

The 1200-1900 angstrom region and fine error sensor observations in the optical for V444 Cyg were continuously observed. More than half of a primary minimum and almost a complete secondary minimum were observed. It is found that the time of minimum for the secondary eclipse is consistent with that for primary eclipse, and the ultraviolet times of minimum are consistent with the optical ones. The spectrum shows a considerable amount of phase dependence. The general shaps and depths of the light curves for the FES signal and the 1565-1900 angstrom continuum are similar to those for the blue continuum. The FES, however, detected an atmospheric eclipse in line absorption at about the phase the NIV absorption was strongest. It is suggested that there is a source of continuum absorption shortward of 1460 angstrom which exists throughout a large part of the extended atmosphere and which, by implication, must redden considerably the ultraviolet continuua of WN stars. A fairly high degree of ionization for the inner part of the WN star a atmosphere is implied.

Eaton, J. E.↗

A polarimeter for the high resolution ultraviolet spectrometer/polarimeter

The design requirements of the polarimeter were established by the scientific optical objectives of the experiment to be launched aboard the Solar Max Mission which will study active solar regions. The polarization of the light is accomplished by a rotating magnesium fluoride quarter wave plate. The quarter wave plates are rotated in 22 1/2 degree steps about an axis coincidental with the light beam. As the light beam passes through the wave plate, the transformation that occurs can be expressed by mathematical equations. By having the wave plates calibrated, the data obtained from solar flares can be analyzed and meaningful information provided to the investigators. The polarimeter has two wave plates with different optical characteristics to provide both redundancy and versatility. A four mirror polarizer was added behind one wave plate to provide additional polarization. The mechanical design, testing, and operation of the polarimeter for the high resolution ultraviolet spectrometer/polarimeter are described.

Calvert, J. A.↗

Impact of wildfires on regional ozone and PM 2.5 : Considering the light absorption of Brown carbon

The influence of wildfire brown carbon (BrC) in moderating the formation of O 3 and fine particulate matter (PM 2.5 ) due to its absorption of ultraviolet (UV) radiation is, for the first time, investigated using a modified community multiscale air quality (CMAQ) model. The wavelength-dependent imaginary refractive index of the organic carbon from wildfires, which are needed by the CMAQ model for its inline photolysis rate calculation, are generated experimentally from wood burning aerosols from a combustion chamber. On high emission days of the Bastrop County Complex fire in Texas in early September 2011, BrC UV absorption reduces the daytime average NO 2 photolysis rate by up to 38% in the core region of the wildfire plume compared to the base scenario that does not consider BrC absorption. Consequently, O 3 production in the smoke plume is suppressed compared to the base scenario due to reduced HO x radical concentrations. Further, in the core region, the predicted O 3 increase due to wildfire reaches as high as 47–123 ppb without considering BrC absorption, the predicted increase of O 3 is 5–15% lower when BrC absorption is considered. Similarly, considering the BrC UV absorption leads to approximately 1% (or ~2–3 µgm -3 ) lower estimation of the wildfire emissions’ impact on total PM 2.5 . This change is small because secondary aerosols, which are the components affected by BrC absorption, only account for a small fraction of the total PM 2.5 in wildfire impacted regions in this study. In addition, our study shows that assumptions about aerosol mixing state (core-shell vs. homogeneous) in the inline photolysis rate calculation would not significantly affect out assessment of the impact of wildfire BrC light absorption on O 3 and PM 2.5 .

54 ENVIRONMENTAL SCIENCES↗

Probing coherent electronic superpositions of singly and doubly excited states of krypton with extreme-ultraviolet four-wave-mixing spectroscopy

Radiative nonlinear four-wave mixing can monitor the evolution of electronic wave packets, providing access to lifetimes and quantifying the light-induced couplings between excited states. In this article, we report the observation of quantum beats in an autoionizing electronic wave packet in krypton, probed using this technique. Analysis of the signal reveals that these beats originate from the contribution of previously unassigned, doubly excited states interacting with singly excited ones. We introduce a minimal theoretical model, based on multichannel quantum-defect theory, which quantitatively reproduces both the wave-packet dynamics and the static spectrum. This work combines a versatile, noncommensurate XUV-IR-based experimental scheme with a tractable model, establishing a powerful approach for the metrology and control of complex, correlated electronic states.

74 ATOMIC AND MOLECULAR PHYSICS↗

Ultraviolet photometry from the orbiting astronomical observatory. XVI - The stellar Lyman-alpha absorption line

The stellar Lyman-alpha line at 1216 A was observed in 29 lightly reddened stars of spectral type B2.5 to B9 by a far-UV spectrophotometer on OAO-2. The equivalent widths obtained range from 15 A at type B2.5 to 65 A at type B8; in the late-B stars, the L-alpha line removes 2 to 3% of the total stellar flux. In this sampling, the strength of the L-alpha line correlates well with measures of the Balmer discontinuity and Balmer line strengths; luminosity classification does not seem to affect the line strength. The observed line widths also agree with the predictions of Mihala's grid of non-LTE model atmospheres. In some cases, the L-alpha line influences the interstellar column densities reported in the interstellar OAO-2 L-alpha survey. Hence, these data toward lightly reddened B2 and B1.5 stars should be regarded as upper limits only.

Savage, B. D.↗

Determination of the light ion abundances in the strong-helium star HR 3089

Using line blanketed model stellar atmospheres and a spectrum synthesis approach, a differential abundance study of the ultraviolet spectrum of HR 3089 relative to the normal star lambda Sco was performed. Both stars were found to have the same abundances of carbon and silicon, but the helium and nitrogen are significantly enhanced in HR 3089. The atmospheric parameters and the distribution of abundances found for HR 3089 agree well with the results of Osmer and Peterson on sharp-lined helium-rich stars. The rotational velocity of 160 km/sec found for HR 3089 places a constraint on the role of diffusion in producing the abundance anomalies. Examination of the resonance lines of C II, N II, Si III and Si IV shows no evidence for mass loss in either star.

Lester, J. B.↗

The Link Between UV Extinction and Infrared Cirrus

Low resolution spectra from the International Ultraviolet Explorer satellite were used to derive ultraviolet extinction curves for stars in four clusters away from the galactic plane. The extinction in three of the clusters is very similar to the general interstellar curve defined by Seaton. Stars in the fourth region, near the Rho Ophiuci dark cloud, have extinction curves that are characterized by a small "linear" term component. The star BD +36 deg 781 is unique amongst the 20 stars observed in that it shows evidence for extinction by diamond grains near 1700 angstroms. We used data from the final release of the IRAS Sky Survey Atlas (ISSA) to determine the 60 micron to 100 micron intensity ratio for the infrared cirrus. The ISSA data, which have been corrected for zodiacal light, gave intensity ratios that are more robust and self-consistent than for other data sets that we used. When the infrared and ultraviolet data are combined, we see a general trend for low values of the ultraviolet "linear term" (al) to correlate with high values of 60 micron/100 micron ratio. This implies that, in regions where the average dust temperature is hotter (high 60 micron/100 micron ratio), there is a relative absence of the small silicate grains that are responsible for the ultraviolet linear term. However, the new data do not bear out our earlier contention that the 60 micron and 100 micron emissions are poorly correlated spatially in regions where the 60 micron/100 micron ratio is low. Only NGC 1647 shows this result. It may be that the different dust types are particularly poorly mixed in this area.

Hackwell, John A.↗

Energy density driven ultrafast electronic excitations in a cuprate superconductor

Controlling nonequilibrium dynamics in quantum materials requires ultrafast probes with spectral selectivity. We report femtosecond reflectivity measurements on the cuprate superconductor Bi 2⁢ Sr 2⁢ CaCu 2 ⁢O 8+𝛿 using free-electron laser extreme-ultraviolet (23.5–177 eV) and near-infrared (1.5 eV) pump pulses. EUV pulses access deep electronic states, while NIR light excites valence-band transitions. Despite these distinct channels, both schemes produce nearly identical dynamics: above 𝑇 𝑐 , excitations relax through fast (100–300 fs) and slower (1–5 ps) channels; below 𝑇 𝑐 , a delayed component signals quasiparticle recombination and condensate recovery. We find that when electronic excitations are involved, the ultrafast response is governed mainly by absorbed energy rather than by the microscopic nature of the excitation. In contrast, bosonic driving in the THz or midinfrared produces qualitatively different dynamics. By demonstrating that EUV excitation of a correlated superconductor yields macroscopic dynamics converging with those from optical pumping, this work defines a new experimental paradigm: FEL pulses at core-level energies provide a powerful means to probe and control nonequilibrium electronic states in quantum materials on their intrinsic femtosecond timescales. This establishes FEL-based EUV pumping as a new capability for ultrafast materials science, opening routes toward soft x-ray and attosecond studies of correlated dynamics.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Transformation of Radiation-Induced Molecular Point Defects and Color Centers in LiF Crystals under Influence of Light

The influences of UV light and integral light pulses from lamps on γ-irradiated LiF crystals with impurities of hydroxyl and magnesium ions have been investigated. The optical absorption and luminescence of color centers in different bleaching stages are studied depending on the crystal exposure time under UV light or on the number of light pulses. IR spectra of molecular hydrogen-bonded complexes and hydroxyl ions in different bleaching stages are presented. The transformation of strong hydrogen-bonded complexes under illumination into complexes with weak hydrogen bond (and vice versa) is studied. It is shown how molecular hydrogen-bonded complexes involving hydroxyl affect the transformation of color centers during the crystal bleaching.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Single-shot imaging with randomized structured illumination at a free electron laser

Stroboscopic nanoscale imaging with free electron laser light is revolutionizing our understanding of fast dynamics in heterogeneous systems. The short wavelength of X-ray and extreme ultraviolet radiation makes it possible to achieve nanoscale resolution, while resonance with atomic transitions gives access to electronic and magnetic degrees of freedom. Here, we report on our implementation of a recently developed imaging method, randomized probe imaging, at a free electron laser. The advantage of randomized probe imaging over existing methods is its compatibility with extended and strongly scattering samples. Our implementation delivers robust single-shot reconstructions at up to a full-pitch resolution of 400 nm over a field of view with a 40 µm diameter. We also demonstrate single-shot imaging of magnetic domain structures using circular dichroism at resonance, paving the way to future time-resolved studies of magnetic dynamics, shock physics, and the dynamics of collective electronic phases.

47 OTHER INSTRUMENTATION↗

Materials screening chamber for testing materials resistance to atomic oxygen

A unique test chamber for exposing material to a known flux of oxygen atoms is described. The capabilities and operating parameters of the apparatus include production of an oxygen atom flux in excess of 5 x 10 to the 16th atoms/sq cm-sec, controlled heating of the sample specimen, RF circuitry to contain the plasma within a small volume, and long exposure times. Flux measurement capabilities include a calorimetric probe and a light titration system. Accuracy and limitations of these techniques are discussed. An extension to the main chamber to allow simultaneous ultraviolet and atomic oxygen exposure is discussed. The oxygen atoms produced are at thermal energies. Sample specimens are maintained at any selected temperature between ambient and 200 C, to within + or - 2 C. A representative example of measurements made using the chamber is presented.

Pippin, H. G.↗

Color/magnitude calibration for National Aeronautics and Space Administration (NASA) standard Fixed-Head Star Trackers (FHST)

This paper characterizes and analyzes the spectral response of Ball Aerospace fixed-head star trackers, (FHST's) currently in use on some three-axis stabilized spacecraft. The FHST output is a function of the frequency and intensity of the incident light and the position of the star image in the field of view. The FHST's on board the Extreme Ultraviolet Explorer (EUVE) have had occasional problems identifying stars with a high B-V value. These problems are characterized by inaccurate intensity counts observed by the tracker. The inaccuracies are due to errors in the observed star magnitude values. These errors are unique to each individual FHST. For this reason, data were also collected and analyzed from the Upper Atmosphere Research Satellite (UARS). As a consequence of this work, the Goddard Space Flight Center (GSFC) Flight Dynamics Division (FDD) hopes to improve the attitude accuracy on these missions and to adopt better star selection procedures for catalogs.

Landis, J.↗

Multiwavelength Observations of a Dramatic High-Energy Flare in the Blazar 3C 279

The blazar 3C 279, one of the brightest identified extragalactic objects in the gamma-ray sky, underwent a large (factor of approximately 10 in amplitude) flare in gamma-rays toward the end of a 3 week pointing by Compton Gamma Ray Observatory (CGRO), in 1996 January-February. The flare peak represents the highest gamma-ray intensity ever recorded for this object. During the high state, extremely rapid gamma-ray variability was seen, including an increase of a factor of 2.6 in approximately 8 hr, which strengthens the case for relativistic beaming. Coordinated multifrequency observations were carried out with Rossi X-Ray Timing Explorer (RXTE), Advanced Satellite for Cosmology and Astrophysics (ASCA; or, Astro-D), Roentgen Satellite (ROSAT), and International Ultraviolet Explorer (IUE) and from many ground-based observatories, covering most accessible wavelengths. The well-sampled, simultaneous RXTE light curve shows an outburst of lower amplitude (factor of approximately = 3) well correlated with the gamma-ray flare without any lag larger than the temporal resolution of approximately 1 day. The optical-UV light curves, which are not well sampled during the high-energy flare, exhibit more modest variations (factor of approximately 2) and a lower degree of correlation. The flux at millimetric wavelengths was near a historical maximum during the gamma-ray flare peak, and there is a suggestion of a correlated decay. We present simultaneous spectral energy distributions of 3C 279 prior to and near to the flare peak. The gamma-rays vary by more than the square of the observed IR-optical flux change, which poses some problems for specific blazar emission models. The synchrotron self-Compton (SSC) model would require that the largest synchrotron variability occurred in the mostly unobserved submillimeter/far-infrared region. Alternatively, a large variation in the external photon field could occur over a time-scale of a few days. This occurs naturally in the "mirror" model wherein the flaring region in the jet photoionizes nearby broad emission line clouds, which, in turn, provide soft external photons that are Comptonized to gamma-ray energies.

Wehrle, A. E.↗

Multiwavelength Observations of a Dramatic High-Energy Flare in the Blazar 3C 279

The blazar 3C 279, one of the brightest identified extragalactic objects in the gamma-ray sky, underwent a large (factor of approx. 10 in amplitude) flare in gamma-rays toward the end of a 3 week pointing by Compton Gamma Ray Observatory (CGRO), in 1996 January-February. The flare peak represents the highest gamma-ray intensity ever recorded for this object. During the high state, extremely rapid gamma-ray variability was seen, including an increase of a factor of 2.6 in approx. 8 hrs., which strengthens the case for relativistic beaming. Coordinated multifrequency observations were carried out with Rossi X-Ray Timing Explorer (RXTE), Advanced Satellite for Cosmology and Astrophysics (ASCA; or, Astro-D), Roentgen Satellite (ROSAT), and International Ultraviolet Explorer (IUE) and from many ground-based observatories, covering most accessible wavelengths. The well-sampled, simultaneous RXTE light curve shows an outburst of lower amplitude (factor of approx. or equal to 3) well correlated with the gamma-ray flare without any lag larger than the temporal resolution of approx. 1 day. The optical-UV light curves, which are not well sampled during the high-energy flare, exhibit more modest variations (factor of approx. 2) and a lower degree of correlation. The flux at millimetric wavelengths was near a historical maximum during the gamma-ray flare peak, and there is a suggestion of a correlated decay. We present simultaneous spectral energy distributions of 3C 279 prior to and near to the flare peak. The gamma-rays vary by more than the square of the observed IR-optical flux change, which poses some problems for specific blazar emission models. The synchrotron self-Compton (SSC) model would require that the largest synchrotron variability occurred in the mostly unobserved submillimeter/far-infrared region. Alternatively, a large variation in the external photon field could occur over a time scale of a few days. This occurs naturally in the "mirror" model wherein the flaring region in the jet photoionizes nearby broad emission line clouds, which, in turn, provide soft external photons that are Comptonized to gamma-ray energies.

Wehrle, A. E.↗

Corongraphic Observations and Analyses of The Ultraviolet Solar Corona

The activities supported under NASA Grant NAG5-613 included the following: 1) reduction and scientific analysis of data from three sounding rocket flights of the Rocket Ultraviolet Coronagraph Spectrometer, 2) development of ultraviolet spectroscopic diagnostic techniques to provide a detailed empirical description of the extended solar corona, 3) extensive upgrade of the rocket instrument to become the Ultraviolet Coronal Spectrometer (UVCS) for Spartan 201,4) instrument scientific calibration and characterization, 5) observation planning and mission support for a series of five Spartan 201 missions (fully successful except for STS 87 where the Spartan spacecraft was not successfully deployed and the instruments were not activated), and 6) reduction and scientific analysis of the UVCS/Spartan 201 observational data. The Ultraviolet Coronal Spectrometer for Spartan 201 was one unit of a joint payload and the other unit was a White Light Coronagraph (WLC) provided by the High Altitude Observatory and the Goddard Space Flight Center. The two instruments were used in concert to determine plasma parameters describing structures in the extended solar corona. They provided data that could be used individually or jointly in scientific analyses. The WLC provided electron column densities in high spatial resolution and high time resolution. UVCS/Spartan provided hydrogen velocity distributions, and line of sight hydrogen velocities. The hydrogen intensities from UVCS together with the electron densities from WLC were used to determine hydrogen outflow velocities. The UVCS also provided O VI intensities which were used to develop diagnostics for velocity distributions and outflow velocities of minor ions.

Kohl, John L.↗

Time-Resolved Ultraviolet Spectroscopy of the M-Dwarf GJ 876 Exoplanetary System

Extrasolar planets orbiting M-stars may represent our best chance to discover habitable worlds in the coming decade. The ultraviolet spectrum incident upon both Earth-like and Jovian planets is critically important for proper modeling of their atmospheric heating and chemistry. In order to provide more realistic inputs for atmospheric models of planets orbiting low-mass stars, we present new near- and far-ultraviolet (NUV and FUV) spectroscopy of the M-dwarf exoplanet host GJ 876 (U4V). Using the COS and STIS spectrographs aboard the Hubble Space Telescope, we have measured the 1150 - 3140 Ang. spectrum of GJ 876. We have reconstructed the stellar H I Ly-alpha emission line profile, and find that the integrated Ly-apha flux is roughly equal to the rest of the integrated flux (1150 - 1210 Ang + 1220 - 3140 Ang) in the entire ultraviolet bandpass (F(Ly-alpha)/F(FUV+NUV) approximately equals 0.7). This ratio is approximately 2500 x greater than the solar value. We describe the ultraviolet line spectrum and report surprisingly strong fluorescent emission from hot H2 (T(H2) > 2000 K). We show the light-curve of a chromospheric + transition region flare observed in several far-UV emission lines, with flare/ quiescent flux ratios :2: 10. The strong FUV radiation field of an M-star (and specifically Ly-alpha) is important for determining the abundance of O2 - and the formation of biomarkers - in the lower atmospheres of Earth-like planets in the habitable zones of low-mass stars.

France, Kevin↗