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At least 973 records · Page 54

Gamma Spectrometry Examination of the AGR-3/4 Irradiation

The results from gamma spectrometry examination of the different components from the combined third and fourth U.S. Advanced Gas Reactor (AGR) TRISO-coated particle fuel irradiation tests (AGR-3/4) have been analyzed. This experiment was designed to provide information about in-pile fission product migration. In each of the 12 capsules, a single stack of four compacts with designed-to-fail (DTF) particles surrounded by inner and outer graphite and/or graphitic matrix rings and a graphite sink ring were irradiated in the Advanced Test Reactor (ATR) at Idaho National Laboratory (INL). Gamma spectrometry has been used to evaluate the gamma-emitting fission product inventory of compacts from the irradiation and evaluate the burnup of these compacts based on the activity of the radioactive cesium isotopes (i.e., Cs-134 and Cs-137) in the compacts. Burnup from gamma spectrometry compares well with predicted burnup from simulations. The inner and outer rings were also examined by gamma spectrometry to evaluate the total fission product inventory of the rings, and gamma emission computed tomography (GECT) was used to investigate the spatial distribution of gamma-emitting fission products within the rings. This report focuses on results obtained via the Precision Gamma Scanner (PGS) for the compacts and inner and outer rings. These non-destructive gamma measurements are currently being compared to recent destructive measurements of spatial fission product distributions in the rings and to predictions made via mathematical modeling. A separate report discusses the entire AGR-3/4 fission product mass balance for all irradiation capsule components including the inner and outer rings, graphite sink rings, capsule spacers, capsule foils, through tubes, and felts. This report is similar to the conference proceedings: Harp, J.M., Demkowicz, P.A., and Stempien, J.D., “Initial gamma spectrometry examination of the AGR-3/4 irradiation,” International Topical Meeting High Temperature Reactor Technology (HTR 2016), Las Vegas, NV, USA, November 2016, Paper HTR2016-18593, but it has been updated to reflect all the data that has been collected on AGR-3/4 using PGS. The Appendices contain extensive data from the collected gamma spectra.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

The SAS4A/SASSYS-1 Safety Analysis Code System

SAS4A/SASSYS-1 is a software simulation tool used to perform deterministic safety analysis of anticipated events as well as design basis and beyond design basis accidents for advanced nuclear reactors. This software can be used to assess the safety of a prescribed reactor design, but it cannot be used to configure a design to meet targeted performance objectives. Detailed, mechanistic models of steady-state and transient thermal,hydraulic, kinetic, and mechanical phenomena are employed to describe the response of the reactor core, the reactor primary and secondary coolant loops, the reactor control and protection systems and the balance-of-plant to accidents caused by changes in coolantflow, oss of heat rejection, or reactivity insertion. The consequences of single and double-fault accidents can be modeled, including fuel and coolant heating, fuel and cladding mechanical behavior, core reactivity feedbacks, coolant loop performance including natural circulation, and decay heat removal. Analyses are typically terminated upon demonstration of reactor and plant shutdown to permanently coolable conditions or upon violation of design basis margins. The objective of the analysis is to quantify accident consequences as measured by the transient behavior of system performance parameters, such as fuel and cladding temperatures, reactivity, and cladding strain. Originally developed for analysis of sodium cooled reactors with oxide fuel clad by stainless steel, the models In SAS4A/SASSYS-1 were subsequently extended and specialized to metallic fuel clad with advanced alloys and to several other coolant options including lead and LBE. METHOD OF SOLUTION: Each subassembly in the reactor core is represented with single or multiple-pin models. One channel represents one or more fuel pins and many channels are employed for a whole-core representation. Heat transfer in each pin is modeled with a two-dimensional (r/z) heat conduction equation. Single and two-phase coolant thermal-hydraulics are simulated with a unique, one-dimensional (axial) multiple-bubble liquid metal boiling model. The transient fuel and cladding mechanical oehavior models are integrated with fission product production,release, and transport models. UNIQUE FEATURES: The physical models in SAS4AJSASSYS-1 are highly detailed 1umerical representations of reactor accident conditions based on extensive laboratory and test reactor results. The models are specialized to liquid metal (sodium) cooled fast reactors with oxide or metallic fuel clad with stainless steel.

Source record↗

SAS4A/SASSYS-1 VERSION 5.2 SAFETY ANALYSIS CODE SYSTEM

SAS4A/SASSYS-1 is a software simulation tool used to perform deterministic safety analysis of anticipated events as well as design basis and beyond design basis accidents for advanced nuclear reactors. This software can be used to assess the safety of a prescribed reactor design, but it cannot be used to configure a design to meet targeted performance objectives. Detailed, mechanistic models of steady-state and transient thermal, hydraulic, kinetic, and mechanical phenomena are employed to describe the response of the reactor core, the reactor primary and secondary coolant loops, the reactor control and protection systems and the balance-of-plant to accidents caused by changes in coolant flow, oss of heat rejection, or reactivity insertion. The consequences of single and double-fault accidents can be modeled, including fuel and coolant heating, fuel and cladding mechanical behavior, core reactivity feedbacks, coolant loop performance including natural circulation, and decay heat removal. Analyses are typically terminated upon demonstration of reactor and plant shutdown to permanently coolable conditions or upon violation of design basis margins. The objective of the analysis is to quantify accident consequences as measured by the transient behavior of system performance parameters, such as fuel and cladding temperatures, reactivity, and cladding strain. Originally developed for analysis of sodium cooled reactors with oxide fuel clad by stainless steel, the models In SAS4A/SASSYS-1 were subsequently extended and specialized to metallic fuel clad with advanced alloys and to several other coolant options including lead and LBE. METHOD OF SOLUTION: Each subassembly in the reactor core is represented with single or multiple-pin models. One channel represents one or more fuel pins and many channels are employed for a whole-core representation. Heat transfer in each pin is modeled with a two-dimensional (r/z) heat conduction equation. Single and two-phase coolant thermal-hydraulics are simulated with a unique, one-dimensional (axial) multiple-bubble liquid metal boiling model. The transient fuel and cladding mechanical behavior models are integrated with fission product production,release, and transport models. UNIQUE FEATURES: The physical models in SAS4AJSASSYS-1 are highly detailed 1umerical representations of reactor accident conditions based on extensive laboratory and test reactor results. The models are specialized to liquid metal (sodium) cooled fast reactors with oxide or metallic fuel clad with stainless steel.«

Fanning, Thomas↗

Gamma Spectrometry Examination of the AGR-3/4 Irradiation

The results from gamma spectrometry examination of the different components from the combined third and fourth U.S. Advanced Gas Reactor (AGR) TRISO-coated particle fuel irradiation tests (AGR-3/4) have been analyzed. This experiment was designed to provide information about in-pile fission product migration. In each of the 12 capsules, a single stack of four compacts with designed-to-fail (DTF) particles surrounded by inner and outer graphite and/or graphitic matrix rings and a graphite sink ring were irradiated in the Advanced Test Reactor (ATR) at Idaho National Laboratory (INL). Gamma spectrometry has been used to evaluate the gamma-emitting fission product inventory of compacts from the irradiation and evaluate the burnup of these compacts based on the activity of the radioactive cesium isotopes (i.e., Cs-134 and Cs-137) in the compacts. Burnup from gamma spectrometry compares well with predicted burnup from simulations. The inner and outer rings were also examined by gamma spectrometry to evaluate the total fission product inventory of the rings, and gamma emission computed tomography (GECT) was used to investigate the spatial distribution of gamma-emitting fission products within the rings. This report focuses on results obtained via the Precision Gamma Scanner (PGS) for the compacts and inner and outer rings. These non-destructive gamma measurements are currently being compared to recent destructive measurements of spatial fission product distributions in the rings and to predictions made via mathematical modeling. A separate report discusses the entire AGR-3/4 fission product mass balance for all irradiation capsule components including the inner and outer rings, graphite sink rings, capsule spacers, capsule foils, through tubes, and felts. This report is similar to the conference proceedings: Harp, J.M., Demkowicz, P.A., and Stempien, J.D., “Initial gamma spectrometry examination of the AGR-3/4 irradiation,” International Topical Meeting High Temperature Reactor Technology (HTR 2016), Las Vegas, NV, USA, November 2016, Paper HTR2016-18593, but it has been updated to reflect all the data that has been collected on AGR-3/4 using PGS. The Appendices contain extensive data from the collected gamma spectra.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

UPDATES FROM THE INVOLUTE WORKING GROUP

The HFIR, RHF, and FRM II reactors represent a particular class of Research and Test Reactors that provide some of the most intense and continuous neutron fluxes for science, industry, and medical applications. These high-performance reactors have achieved compact cores by operating with Highly Enriched Uranium fuel (HEU, 235U/U ≥ 20 wt. %) and utilizing fuel plates curved as an involute. Due to the proliferation risks, the international community aims to reduce or eliminate, when possible, the use of HEU fuel in civilian facilities by converting them to a Low-Enriched Uranium fuel (LEU, 235U/U < 20 wt. %). Conversion of these reactors without significantly compromising their performance or safety is a challenging endeavor that can tremendously benefit from advanced computational tools and thus, eliminate unnecessary conservatism to ensure sufficient thermal margins. Therefore, models are being developed using modern Computational Fluid Dynamics (CFD) and Computational Structural Mechanics (CSM) software to evaluate the steady-state safety margins of various LEU designs instead of being reliant on the more traditional, conservative methods. To gain the confidence and acceptance of high-fidelity modeling by the nuclear regulators, Argonne National Laboratory (ANL) and the involute reactors have formed an informal scientific group, the Involute Working Group (IWG). The IWG facilitates inter-organizational collaboration on experimental benchmarking, code-to-code comparisons, and Verification and Validation (V&V). This paper describes some of the recent IWG efforts in validating software against the existing experimental data, as well as code-to-code comparisons of different software used by the IWG members.

Bergeron, Aurelien↗

Imminent: Irradiation Testing of (Th,Pu)O{sub 2} Fuel - 13560

Commercial-prototype thorium-plutonium oxide (Th-MOX) fuel pellets have been loaded into the material test reactor in Halden, Norway. The fuel is being operated at full power - with instrumentation - in simulated LWR / PHWR conditions and its behaviour is measured 'on-line' as it operates to high burn-up. This is a vital test on the commercialization pathway for this robust new thoria-based fuel. The performance data that is collected will support a fuel modeling effort to support its safety qualification. Several different samples of Th-MOX fuel will be tested, thereby collecting information on ceramic behaviours and their microstructure dependency. The fuel-cycle reasoning underpinning the test campaign is that commercial Th- MOX fuels are an achievable intermediate / near-term SNF management strategy that integrates well with a fast reactor future. (authors)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Postirradiation Examination of FUTURIX-FTA metallic alloy experiments

Two different metallic nuclear fuel alloys intended for transmutation applications in fast neutron spectrum nuclear reactors have been irradiated, and their performance has been evaluated after irradiation. These alloys contained elevated levels of plutonium and other minor actinides (Am, Np) compared to historically irradiated fast reactor fuel to ascertain the impact of these isotopes on fuel performance. The irradiation of these alloys was performed at the Phénix fast reactor in France to facilitate comparisons between true fast spectrum irradiations and pseudo-fast spectrum irradiations performed at the thermal neutron spectrum Idaho National Laboratory Advanced Test Reactor. The irradiation tests were designated FUTURIX-FTA DOE1 which contained a low-fertile alloy and FUTURIX-FTA DOE2 which contained a non-fertile alloy. The DOE1 fuel was irradiated to a measured burnup of 9.5 % fissions per initial heavy metal atom (FIMA), and the DOE2 fuel was irradiated to a measured burnup of 12.7 % fissions per initial heavy metal atom. This work reports baseline Postirradiation Examination (PIE) results for DOE1 and DOE2. Fuel swelling, fission product distribution, cladding strain, fission gas release, fuel microstructure, fuel cladding chemical interaction and minor actinide transmutation were all evaluated. Cladding strain was negligible and fission gas release was 52% for DOE1 and 69% for DOE2. The exams show the 2 pins behaved very similar to EBR-II metallic fuel experience. Minor actinides seem to not affect the performance of this candidate transmutation fuel. As a result, performance data from these irradiations can be used to inform the feasibility of minor actinide transmutation in future reactor systems.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Enhanced Micro-Pocket Fission Detector for High Temperature Reactors - FY17 FInal Project Report

A collaboration between the Idaho National Laboratory (INL), the Kansas State University (KSU), and the French Atomic Energy Agency, Commissariat à l'Énergie Atomique et aux Energies Alternatives, (CEA), has been initiated by the Nuclear Energy Enabling Technologies (NEET) Advanced Sensors and Instrumentation (ASI) program for developing and testing High Temperature Micro-Pocket Fission Detectors (HT MPFD), which are compact fission chambers capable of simultaneously measuring thermal neutron flux, fast neutron flux and temperature within a single package for temperatures up to 800 °C. The MPFD technology utilizes a small, multi-purpose, robust, in-core fission chambers and thermocouple. As discussed within this report, the small size, variable sensitivity, and increased accuracy of the MPFD technology represent a revolutionary improvement over current methods used to support irradiations in US Material Test Reactors (MTRs). Previous research conducted through NEET ASI1-3 has shown that the MPFD technology could be made robust and was successfully tested in a reactor core. This new project will further the MPFD technology for higher temperature regimes and other reactor applications by developing a HT MPFD suitable for temperatures up to 800 °C. This report summarizes the research progress for this three year project.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

AGR-2 Data Qualification Report for ATR Cycle 154B

This report provides the data qualification status of Advanced Gas Reactor-2 (AGR-2) fuel irradiation experimental data from Advanced Test Reactor (ATR) Cycle 154B as recorded in the Nuclear Data Management and Analysis System (NDMAS). This is the last cycle of AGR-2 irradiation, as the test train was pulled from the ATR core during the outage portion of ATR Cycle 155A. The AGR-2 data streams addressed in this report include thermocouple (TC) temperatures, sweep gas data (flow rates including new Fission Product Monitoring (FPM) downstream flows from Fission Product Monitoring System (FPMS) detectors, pressure, and moisture content), and FPMS data (release rates and release-to-birth rate ratios [R/Bs]) for each of the six capsules in the AGR-2 experiment. The final data qualification status for these data streams is determined by a Data Review Committee (DRC) comprised of AGR technical leads, Sitewide Quality Assurance (QA), and NDMAS analysts. The Data Review Committee reviewed the data acquisition process, considered whether the data met the requirements for data collection as specified in QA-approved Very High Temperature Reactor (VHTR) data collection plans, examined the results of NDMAS data testing and statistical analyses, and confirmed the qualification status of the data as given in this report.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Summary of Geometric Parameters and Their Effects on Performance of U-10Mo Fuel Plates

A monolithic plate-type fuel system has been under development to convert high-performance test reactors from highly enriched uranium to low-enrichment uranium fuels and is now moving into the qualification phase, a predecessor to the timely conversion of the target reactors. To qualify this fuel system, the plates must meet safety standards and perform well in a reactor. The plates must maintain mechanical integrity, exhibit geometric stability, and have stable and predictable in-reactor behavior. The requirement to maintain mechanical integrity under normal operating conditions is primarily demonstrated by successful testing. However, each high-performance reactor employs a distinct design, resulting in distinct plate geometries, with unique features, attributes, irregularities, and tolerances. Due to the abundance of such distinct geometric varieties, a single “generic” plate geometry capturing all extremes is not achievable. It is also impractical to test each of these proposed designs in a reactor. This limitation necessitates cautious evaluations since the thermomechanical response of a plate with a certain geometry may not be representative for a plate with a significantly different geometry. To address concerns related to in-reactor plate performance, large set of sensitivity studies were performed. These parametric studies aimed to better understand irradiation performance, while evaluating the sensitivity of results to various modeling inputs, including geometric, operational, and material parameters. This work studied selected geometric parameters based on provided fuel specifications and performed a series of parametric simulations. The resulting temperature, displacement, and stress strains were comparatively evaluated to determine the effects of various geometric parameters. This draft provides a “high-level summary” of our parametric sensitivity studies and summarizes the key findings.

42 ENGINEERING↗

AGC-2 Specimen Post Irradiation Data Package Report

This report documents results of the post-irradiation examination material property testing of the creep, control, and piggyback specimens from the irradiation creep capsule Advanced Graphite Creep (AGC)-2 are reported. This is the second of a series of six irradiation test trains planned as part of the AGC experiment to fully characterize the neutron irradiation effects and radiation creep behavior of current nuclear graphite grades. The AGC-2 capsule was irradiated in the Idaho National Laboratory Advanced Test Reactor at a nominal temperature of 600°C and to a peak dose of 5 dpa (displacements per atom). One half of the creep specimens were subjected to mechanical stresses (an applied stress of either 13.8, 17.2, or 20.7 MPa) to induce irradiation creep. All post-irradiation testing and measurement results are reported with the exception of the irradiation mechanical strength testing, which is the last destructive testing stage of the irradiation testing program. Material property tests were conducted on specimens from 15 nuclear graphite grades using a similar loading configuration as the first AGC capsule (AGC-1) to provide easy comparison between the two capsules. However, AGC-2 contained an increased number of specimens (i.e., 487 total specimens irradiated) and replaced specimens of the minor grade 2020 with the newer grade 2114. The data reported include specimen dimensions for both stressed and unstressed specimens to establish the irradiation creep rates, mass and volume data necessary to derive density, elastic constants (Young’s modulus, shear modulus, and Poisson’s ratio) from ultrasonic time of flight velocity measurements, Young’s modulus from the fundamental frequency of vibration, electrical resistivity, and thermal diffusivity and thermal expansion data from 100–500°C. No data outliers were determined after all measurements were completed. A brief statistical analysis was performed on the irradiated data and a limited comparison between pre- and post-irradiation properties is presented. A more complete evaluation of trends in the material property changes, as well as irradiation-induced creep due to irradiation, temperature, and applied load on specimens will be discussed in later AGC-2 post-irradiation examination analysis reports.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

AGC-2 Specimen Post Irradiation Data Package Report

This report documents results of the post-irradiation examination material property testing of the creep, control, and piggyback specimens from the irradiation creep capsule Advanced Graphite Creep (AGC)-2 are reported. This is the second of a series of six irradiation test trains planned as part of the AGC experiment to fully characterize the neutron irradiation effects and radiation creep behavior of current nuclear graphite grades. The AGC-2 capsule was irradiated in the Idaho National Laboratory Advanced Test Reactor at a nominal temperature of 600°C and to a peak dose of 5 dpa (displacements per atom). One-half of the creep specimens were subjected to mechanical stresses (an applied stress of either 13.8, 17.2, or 20.7 MPa) to induce irradiation creep. All post-irradiation testing and measurement results are reported with the exception of the irradiation mechanical strength testing, which is the last destructive testing stage of the irradiation testing program. Material property tests were conducted on specimens from 15 nuclear graphite grades using a similar loading configuration as the first AGC capsule (AGC-1) to provide easy comparison between the two capsules. However, AGC-2 contained an increased number of specimens (i.e., 487 total specimens irradiated) and replaced specimens of the minor grade 2020 with the newer grade 2114. The data reported include specimen dimensions for both stressed and unstressed specimens to establish the irradiation creep rates, mass and volume data necessary to derive density, elastic constants (Young’s modulus, shear modulus, and Poisson’s ratio) from ultrasonic time-of-flight velocity measurements, Young’s modulus from the fundamental frequency of vibration, electrical resistivity, and thermal diffusivity and thermal expansion data from 100–500°C. No data outliers were determined after all measurements were completed. A brief statistical analysis was performed on the irradiated data and a limited comparison between pre- and post-irradiation properties is presented. A more complete evaluation of trends in the material property changes, as well as irradiation-induced creep due to irradiation, temperature, and applied load on specimens will be discussed in later AGC-2 post-irradiation examination analysis reports.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Investigation of Treat M2 and M3 calibration experiments for benchmark analysis

The Transient Reactor Test Facility (TREAT) located at Idaho National Laboratory is a graphite moderated and reflected, air cooled core. This reactor was originally designed and operated to experimentally test fuel under extreme transient conditions. To this end, TREAT successfully performed many series of steady-state and transient tests until operations were discontinued in 1994. With the restart of the reactor planned for 2018, accurate models of previous reactor experiments are necessary to verify the ability to predict conditions for planned upcoming tests. In this work, the methodology for modeling the M2 and M3 calibration experiments (M2/M3CAL) will be described along with results from the variation of key parameters including the boron concentration. Additionally, this model will be used to demonstrate the correlation between reactor behavior and the implementation of 'nuclear graphite' thermal scattering law (TSL) data to capture the behavior of thermal neutrons in the TREAT core.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

AGR-1, AGR-2, AGR-3/4, and AGR-5/6/7 DimensionalChange Analysis

A series of fuel irradiation experiments have been planned in the Advanced Test Reactor (ATR) at Idaho National Laboratory (INL) to support the licensing and operation of the Advanced Reactor Technologies high temperature gas-cooled reactor. The advanced gas reactor (AGR) experiments are comprised of multiple independent capsules containing multiple cylindrical fuel compacts, placed inside of a graphite cylinder in ATR. The purpose of the AGR experiments is to provide data on fuel performance under irradiation, support fuel process development, qualify the fuel for normal operating conditions, provide irradiated fuel for accident testing, and support the development of fuel performance and fission product transport models. The advanced graphite creep (AGC) experiments provide irradiation creep data for design and licensing. To date, six irradiation campaigns have been completed: AGR-1 (December, 2006 – November, 2009); AGR-2 (June, 2010 – October, 2013); AGR-3/4 (December, 2011 – April, 2014); AGC-1 (September, 2009 – January, 2011); AGC-2 (April, 2011 – May, 2012); and AGC-3 (November, 2012 – April, 2014).

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Updated Results of Ultrasonic Transducer Irradiation Test

Ultrasonic technologies offer the potential for high accuracy and resolution in-pile measurement of a range of parameters, including geometry changes, temperature, crack initiation and growth, gas pressure and composition, and microstructural changes. Many Department of Energy-Office of Nuclear Energy (DOE-NE) programs are exploring the use of ultrasonic technologies to provide enhanced sensors for in-pile instrumentation during irradiation testing. For example, the ability of small diameter ultrasonic thermometers (UTs) to provide a temperature profile in candidate metallic and oxide fuel would provide much needed data for validating new fuel performance models. These efforts are limited by the lack of identified ultrasonic transducer materials capable of long term performance under irradiation test conditions. To address this need, the Pennsylvania State University (PSU) was awarded an Advanced Test Reactor National Scientific User Facility (ATR NSUF) project to evaluate the performance of promising magnetostrictive and piezoelectric transducers in the Massachusetts Institute of Technology Research Reactor (MITR) up to a fast fluence of at least 10{sup 21} n/cm{sup 2}. A multi-National Laboratory collaboration funded by the Nuclear Energy Enabling Technologies Advanced Sensors and Instrumentation (NEET-ASI) program also provided initial support for this effort. This irradiation, which started in February 2014, is an instrumented lead test and real-time transducer performance data are collected along with temperature and neutron and gamma flux data. The irradiation is ongoing and will continue to approximately mid-2015. To date, very encouraging results have been attained as several transducers continue to operate under irradiation. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Water-based Ria Testing in TREAT: Commissioning and Early Results

We have completed a series of reactivity-initiated accident commissioning tests with the static water capsule in the Transient Reactor Test Facility and completed some visual and non-destructive post-irradiation examinations on the fuel rods. The test campaign included a calibration test followed by five tests in the Static Environment Rodlet Transient Test Apparatus capsule. The conditions varied from room temperature and pressure up to 200°C and 2.5 MPa, with energy depositions varying between ~500–1100 J/gUO2. The series of tests allowed for a number of instrumentation qualifications and demonstrations, including cladding thermometry, rodlet plenum pressure, cladding elongation, and an electro-impedance boiling detector. This paper documents the design of the capsule and highlights some results from the commissioning tests and post-transient examination.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

USHPRR MP-1 Irradiation Test: Assessment of Edge Pitting and Bond Line Corrosion in Vendor Produced Fuel Plates

This report summarizes an effort to identify the source of anomalous localized edge pitting and bond line corrosive attack of experimental mini fuel plates manufactured at the commercial fuel vendor BWXT and tested in the Advanced Test Reactor (ATR) at Idaho National Laboratory (INL) as part of the Miniplate 1 (MP-1) irradiation test. The MP-1 test was conducted by the US High Performance Research Reactor Project (USHPRR) and overseen by the Fuel Qualification Pillar (FQ). The test involved evaluation of a mix of 62 “vendor” fuel plates fabricated at BWXT and 12 “laboratory” fuel plates fabricated at Idaho National Laboratory using commercial-scale and labscale fabrication processes respectively. The MP-1 test was the first in a series of tests to generate data to support qualification of a new plate-type low-enriched uranium (LEU) U-10Mo monolithic fuel system. The major objective of the MP-1 experiment was to test, for the first time, miniplates fabricated by a commercial fuel vendor over the range of irradiation conditions relevant to conversion of NRC regulated High Performance Research Reactors (HPRRs) from high-enriched uranium to LEU. The focus of the efforts described in this report are the vendor fuel plates to inform changes in the fabrication process prior to fabrication of the next miniplate experiment MP2.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

X-ray Analysis of Defects and Anomalies in AGR-5/6/7 TRISO Particles

Coated particle fuel batches J52O-16-93164, 93165, 93166, 93168, 93169, 93170, and 93172 were produced by Babcock and Wilcox Technologies (BWXT) for possible selection as fuel for the Advanced Gas Reactor Fuel Development and Qualification (AGR) Program’s AGR-5/6/7 irradiation test in the Idaho National Laboratory (INL) Advanced Test Reactor (ATR), or may be used for other tests. Each batch was coated in a 150-mm-diameter production-scale fluidized-bed chemical vapor deposition (CVD) furnace. Tristructural isotropic (TRISO) coatings were deposited on 425-μm-nominal-diameter spherical kernels from BWXT lot J52R-16-69317 containing a mixture of 15.4%-enriched uranium carbide and uranium oxide (UCO), with the exception of Batch 93164, which used similar kernels from BWXT lot J52L-16-69316. The TRISO-coatings consisted of a ~50% dense carbon buffer layer with 100-μmnominal thickness, a dense inner pyrolytic carbon (IPyC) layer with 40-μm-nominal thickness, a silicon carbide (SiC) layer with 35-μm-nominal thickness, and a dense outer pyrolytic carbon (OPyC) layer with 40-μm-nominal thickness. Each coated particle batch was sieved to upgrade the particles by removing over-sized and under-sized material, and the upgraded batch was designated by appending the letter A to the end of the batch number (e.g., 93164A). Secondary upgrading by sieving was performed on the upgraded batches to remove specific anomalies identified during analysis for Defective IPyC, and the upgraded batches were designated by appending the letter B to the end of the batch number (e.g., 93165B). Following this secondary upgrading, coated particle composite J52R-16-98005 was produced by BWXT as fuel for the AGR Program’s AGR-5/6/7 irradiation test in the INL ATR. This composite was comprised of coated particle fuel batches J52O-16-93165B, 93168B, 93169B, and 93170B.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗