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At least 973 records · Page 54

Direct astrophysical tests of chiral effective field theory at supranuclear densities

Recent observations of neutron stars with gravitational waves and X-ray timing provide unprecedented access to the equation of state (EoS) of cold dense matter at densities difficult to realize in terrestrial experiments. At the same time, predictions for the EoS equipped with reliable uncertainty estimates from chiral effective field theory ( x EFT) allow us to bound our theoretical ignorance. In this work, we analyze astrophysical data using a nonparametric representation of the neutron-star EoS conditioned on x EFT to directly constrain the underlying physical properties of the compact objects without introducing modeling systematics. We discuss how the data alone constrain the EoS at high densities when we condition on x EFT at low densities. Here, we also demonstrate how to exploit astrophysical data to directly test the predictions of x EFT for the EoS up to twice nuclear saturation density, in order to estimate the density at which these predictions might break down. We nd that the existence of massive pulsars, gravitational waves from GW170817, and NICER observations of PSR J0030+0451 favor x EFT predictions for the EoS up to nuclear saturation density over a more agnostic analysis by as much as a factor of 7 for the quantum Monte Carlo (QMC) calculations used in this work. While x EFT predictions using QMC are fully consistent with gravitational-wave data up to twice nuclear saturation density, NICER observations suggest that the EoS stiffens relative to these predictions at or slightly above nuclear saturation density. Additionally, for these QMC calculations, we marginalize over the uncertainty in the density at which x EFT begins to break down, constraining the radius of a 1.4M $\bigodot$ neutron star to R 1.4 = $11.40^{+1.38}_{–1.04}$ ($12.54^{+0.71}_{–0.63}$) km and the pressure at twice nuclear saturation density to p(2n sat ) = $14.2^{+18.1}_{–8.4}$ ($28.7^{+15.3}_{–15.0}$) MeV=fm 3 with massive pulsar and gravitational-wave (and NICER) data.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Consistent Nuclear Data Evaluations for Criticality Safety

Evaluations of nuclear data are based on statistical analysis of available experimental data and their uncertainties plus model calculations and their uncertainties. As the models are currently rather limited, the evaluations are heavily biassed toward experimental data, with the caveat that a thorough analysis is also required to understand possible discrepancies between data sets. Hence, as new experimental data become available, they are incorporated into the evaluation procedure. Recent measurements of the 233 U capture to fission cross section ratio at the Los Alamos Neutron Science Center have prompted a re-evaluation of the capture cross section in the resonance and fast regions up to 250 keV. We will discuss the challenges of including the new fast neutron experimental data in an evaluation that is consistent with the resonance region. We will also discuss our consistent evaluation procedure based on the Hauser-Feshbach statistical model for nuclear reactions and its application to the evaluations of 239 Pu and 139 La neutron-induced reactions.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Unraveling Emergent Quantum States in Magnetic Topological Insulators using High Pressure Neutron Scattering

This proposal aims to uncover novel quantum phenomena under high pressure and understand the pressure effects on the atomic electronic interactions in magnetic topological materials. This program supports a combined neutron scattering and materials discovery of novel magnetic materials that display the coexistence of magnetism plus other physical phenomena such as a non-trivial electronic band topology under high pressure. The goal of this project is to close a long-standing knowledge gap in quantum materials research by developing a high-pressure neutron scattering (HP-NS) toolbox to systematically determine the magnetic structures and electronic interactions present at high pressure.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Characterization of the inner edge of the neutron star crust

The poorly known crustal equation of state plays a critical role in many observational phenomena associated with a neutron star. Here using semiclassical Monte Carlo simulations, we explore the possible configurations of the inner edge of the neutron star crust for a variety of baryon densities and proton fractions. Applying the Kirkwood-Buff theory to these two-component systems, we observe how the isothermal compressibility reaches a maximum when isolated nonsymmetric (or quasispherical) clusters are formed in an extremely dilute neutron gas. To determine the neutron fraction, we suggest a geometrical model based on the behavior of the proton-neutron pair correlation function. Accordingly, the equation of state of the inner crust is calculated, illustrating that the nuclear energy in β equilibrium follows a power-law behavior with baryon density. As a possible astrophysical outcome of this study, our results could help refine the mass-radius relation. Finally, our results pave the way towards further investigations of the impact of the proton-neutron pair correlation function on transport properties within the neutron star crust.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Spin Susceptibility in Neutron Matter from Quantum Monte Carlo Calculations

The spin susceptibility in pure neutron matter is computed from auxiliary field diffusion Monte Carlo calculations over a wide range of densities. The calculations are performed for different spin asymmetries, while using twist-averaged boundary conditions to reduce finite-size effects. The employed nuclear interactions include both the phenomenological Argonne AV8′ + UIX potential and local interactions that are derived from chiral effective field theory up to next-to-next-to-leading order.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

High-resolution laser system for the S 3 -Low Energy Branch

Here, in this paper we present the first high-resolution laser spectroscopy results obtained at the GISELE laser laboratory of the GANIL-SPIRAL2 facility, in preparation for the first experiments with the S 3 -Low Energy Branch. Studies of neutron-deficient radioactive isotopes of erbium and tin represent the first physics cases to be studied at S 3 . The measured isotope-shift and hyperfine structure data are presented for stable isotopes of these elements. The erbium isotopes were studied using the 4f 12 6s 2 3 H 6 → 4f 12 ( 3 H)6s6p J = 5 atomic transition (415 nm) and the tin isotopes were studied by the 5s 2 5p 2 ( 3 P 0 ) → 5s 2 5p6s( 3 P 1 ) atomic transition (286.4 nm), and are used as a benchmark of the laser setup. Additionally, the tin isotopes were studied by the 5s 2 5p6s( 3 P 1 ) → 5s 2 5p6p( 3 P 2 ) atomic transition (811.6 nm), for which new isotope-shift data was obtained and the corresponding field-shift F 812 and mass-shift M 812 factors are presented.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

From ionic clusters dynamics to network constraints in ionic polymer solutions

Physical networks formed by ionizable polymers with ionic clusters as crosslinks are controlled by coupled dynamics that transcend from ionic clusters through chain motion to macroscopic response. Here, the coupled dynamics, across length scales, from the ionic clusters to the networks in toluene swollen polystyrene sulfonate networks, were directly correlated, as the electrostatic environment of the physical crosslinks was altered. The multiscale insight is attained by coupling neutron spin echo measurements with molecular dynamics simulations, carried out to times typical of relaxation of polymers in solutions. The experimental dynamic structure factor is in outstanding agreement with the one calculated from computer simulations, as the networks are perturbed by elevating the temperature and changing the electrostatic environment. In toluene, the long-lived clusters remain stable over hundreds of ns across a broad temperature range, while the polymer network remains dynamic. In conclusion, though the size of the clusters changes as the dielectric constant of the solvent is modified through the addition of ethanol, they remain stable but morph, enhancing the polymer chain dynamics.

36 MATERIALS SCIENCE↗

Domestic Safeguards Material Control and Accountancy Considerations for Molten Salt Reactors

Molten salt reactors (MSRs) are a class of nuclear reactor designs with features and operational characteristics that vary significantly more than the class of light water reactors (LWRs). MSR design concepts can be broadly categorized as solid-fueled reactors with molten salt as the coolant, liquid-fueled reactors with fuel dissolved in molten salt coolant and liquid-fueled reactors with fuel dissolved in molten salt that is contained in distinct fuel tubes with a nonfissile coolant. Proposed MSR concepts include features that are specific to each design. MSR concepts vary widely across these design features, including the physical, chemical, and isotopic composition of fresh and irradiated fuel. Operational neutron energy spectrums and breeding ratios also vary significantly across design concepts. Some concepts are burner reactors designed to transmute the spent nuclear fuel from LWRs or pressurized heavy water reactors (PHWRs), while others are breeder reactors designed to breed fissile 233 U from naturally occurring fertile 232 Th. Some MSR concepts are designed to be a part of a once-through fuel cycle, while others involve chemical separation. Those that include plans to recycle the fuel differ by whether the chemical processing would be done onsite, as a process connected to the fuel salt itself, or offsite at a reprocessing facility similar to how LWR or PHWR spent fuel is reprocessed in some countries. Each overall design concept contains various aspects of each of these features to produce a unique facility

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Looking back at 50 years of cutting-edge capabilities: LANSCE ‘underpins Los Alamos as a world-class scientific institution’

What started with an idea and a memo has since grown into a one-of-a-kind, world-renowned facility that contributes to the nation’s advancement of science and technology. First known as LAMPF (Los Alamos Meson Physics Facility) until the 1990s when it became LANSCE (Los Alamos Neutron Science Center), the facility is celebrating the 50th anniversary of its first full-capacity proton beam on June 9, 1972. Since then, LANSCE has contributed to a range of national security goals, such as supporting the Lab’s stockpile stewardship program, helping to advance the science of medical radioisotopes, improving the understanding of hydrodynamics, and more. “LANSCE has served the nation through its near-unique capabilities,” said Alan Carr, Senior Historian at the National Security Research Center, which houses the facility’s evolution through decades of documents, photos and other materials. “Since 1972, LANSCE has been the Lab’s major experimental science facility and underpins Los Alamos as a world-class scientific institution. This was true 50 years ago and is still true today.” In commemoration of this anniversary, we’re taking a look back at LANSCE’s historic five decades, including its first director, earliest milestones and important contributions to national security.

43 PARTICLE ACCELERATORS↗

Subcriticality Measurements for a Changing Concentration Uranyl Nitrate Solution Tank by Californium Source-Driven Noise Analysis

Subcritical californium source-driven noise analysis (CSDNA) measurements were performed at the Oak Ridge Critical Experiments Facility in 1983 using a stainless-steel tank with an inside diameter of 76.2 cm and a height of 91.4 cm but only filled with a uranyl (93.16 wt.% 235 U) nitrate solution to a height of 76.2 cm for all measurements. The free acid content of the uranyl nitrate solution was less than 0.01 N to minimize hazards in handling. The total available highly enriched uranium for these measurements was 5,296 g. The concentration of the solution was varied from the highest density of 14.71 grams of uranium per liter (g U/L) initially in 16 steps, lowering the concentration to 0.3492 g U/L, and finally using a tank filled with only water. The tank had a Plexiglas lid to minimize evaporation. The Cf source was contained in a re-entrant Lexan tube which could be in the solution parallel to the axis of the cylindrical tank. The detectors were 3 He proportional counters in the solution in shrink-fit tubing to isolate the counters from the fissile solution and adjacent to the outside of the tank. In some cases, the detectors were scintillators adjacent to the outside of the tank. In other cases, the source was external to the tank. Some data presented in this report are from notes and are not in the logbook. The prompt neutron decay constant was obtained from fitting the date from the CSDNA measurements. The purpose of this report is to document the experimental information for the measurements performed so that later, researchers could perform the required uncertainty and calculational analyses and documentation to use these data for an International Nuclear Criticality Safety Benchmark Program (ICSBEP) or a Nuclear Energy Agency benchmark. The prompt neutron decay measurements could be the basis of as International Reactor Physic Benchmark Program. The data from these measurements are available from the Records Management Services Department of Oak Ridge National Laboratory, and the logbook is also available from the ICSBEP at Idaho National Laboratory. Preparation of the present report is part of a larger cooperative effort between Idaho National Laboratory (INL) and Oak Ridge National Laboratory (ORNL) to document more than 15 undocumented critical and subcritical experiments enumerated in ORNL/TM-2019/18 and performed by ORNL at ORCEF and other USDOE critical experiments facilities using more than 500 operational days of critical facility time.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

AXTAR: Mission Design Concept

The Advanced X-ray Timing Array (AXTAR) is a mission concept for X-ray timing of compact objects that combines very large collecting area, broadband spectral coverage, high time resolution, highly flexible scheduling, and an ability to respond promptly to time-critical targets of opportunity. It is optimized for sub-millisecond timing of bright Galactic X-ray sources in order to study phenomena at the natural time scales of neutron star surfaces and black hole event horizons, thus probing the physics of ultra-dense matter, strongly curved spacetimes, and intense magnetic fields. AXTAR s main instrument, the Large Area Timing Array (LATA) is a collimated instrument with 2 50 keV coverage and over 3 square meters effective area. The LATA is made up of an array of super-modules that house 2-mm thick silicon pixel detectors. AXTAR will provide a significant improvement in effective area (a factor of 7 at 4 keV and a factor of 36 at 30 keV) over the RXTE PCA. AXTAR will also carry a sensitive Sky Monitor (SM) that acts as a trigger for pointed observations of X-ray transients in addition to providing high duty cycle monitoring of the X-ray sky. We review the science goals and technical concept for AXTAR and present results from a preliminary mission design study

Ray, Paul S.↗

Evaluation of Irradiation Creep Effects in HT9 Cladding for FAST Experiments

The push for advanced reactor fuels for improved reactor safety and efficiency had led to a renewed interest in metallic fuel for nuclear reactor applications. Experimental investigation is necessary to ensure a robust understanding of the thermomechanical properties of new metallic fuel designs. Unfortunately, with the current experimental facilities, thoroughly investigating the responses of metallic fuel burnup would take a prohibitively long time. To alleviate this, the Fission Accelerated Steady State Test (FAST) was developed to accelerate the irradiation testing while simultaneously decreasing the sensitivity to fabrication tolerances by reducing the fuel diameter and scaling the experiment. This method successfully scales the radiation effects on the fuel, but the HT9 cladding is not exposed to prototypic radiation conditions. This raises questions on whether the FAST experiment results are truly indicative of the HT9 cladding performance due to radiation induced creep effects not being appropriately accounted for. Using BISON fuel performance code, the simulated FAST cladding strain is compared to simulated EBR-II cladding strain. This is done through a sensitivity study of input parameters and scaling of neutron fluence on the cladding. This allows a parametric comparison of physical phenomena on the effective difference between cladding strains between FAST and equivalent burnup EBR-II fuel pins. The results show that the irradiation induced deformation (creep or swelling) is insignificant compared to the thermal-mechanical deformation. Therefore, the difference between the FAST experiment cladding and the EBR-II experiment cladding is negligible and comparison of fuel system performance between the two experiments is appropriate.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Development for Integrated System-Level Analysis Capabilities in SAM for Molten Salt Reactors

In recent years, there has been renewed interest in Molten Salt Reactors (MSRs) for their potential advantages compared to reactors that rely on solid fuel. In response to such interest, many methods and codes have been developed to capture the unique features of MSRs. Among them, the System Analysis Module (SAM) is a modern system analysis tool that provides fast-running, modest-fidelity, whole-plant transient analysis capabilities, essential for fast-turnaround design scoping and engineering analyses of advanced reactor concepts. For liquid-fuel MSRs, the complex physics and chemistry involved in MSR operation—such as reactor kinetics, fluid flow, heat transfer, and salt composition dynamics—pose significant challenges for system-level modeling. Specific modeling capabilities are needed for system-level transient simulation. This paper presents recent advancements in SAM capability enhancements for system-level modeling of MSRs, focusing on improved simulation fidelity, computational efficiency, and multi-physics integration. Key enhancements include the development of species transport, Delayed Neutron Precursor (DNP) drift, modified Point Kinetics Equations (PKE), decay heat modeling, key fission product behavior, salt corrosion, and thermal-hydraulic coupling, as well as code robustness and performance enhancements for MSR applications. The code enhancement allows for better predictive accuracy in safety analysis, transient behavior, and operational optimization, thus supporting the design and licensing of next-generation MSRs. Results from case studies are presented to demonstrate the benefits of these enhancements in accurately capturing key reactor transient behaviors.

Hu, Rui (ORCID:0000000237712920)↗

Properties of first-order hadron-quark phase transition from inverting neutron star observables

By inverting the observational data of several neutron star observables in the three-dimensional parameter space of the constant speed of sound (CSS) model while fixing all hadronic equation-of-state parameters at their currently known most probable values, we constrain the three parameters of the CSS model and their correlations. Using two lower radius limits of $R$ $2.01$ = $11.41$ km and $R$ $2.01$ = $12.2$ km for PSR J0740+6620 obtained from two independent analyses using different approaches by the Neutron Star Interior Composition Explorer (NICER) Collaboration, the speed of sound squared $c$ $^2_{QM}$ in quark matter is found to have a lower limit of 0.35 or 0.43 in units of $c$ $2$ , above its conformal limit of $c$ $^2_{QM}$ < $1/3$. Furthermore, an approximately linear correlation between the first-order hadron-quark transition density $ρ$ $t$ and its strength $Δε$ is found. Moreover, the presence of twin stars is deemed improbable by the present work.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Three-dimensional structure of hybrid magnetic skyrmions determined by neutron scattering

Magnetic skyrmions are topologically protected chiral spin textures which present opportunities for next-generation magnetic data storage and logic information technologies. The topology of these structures originates in the geometric configuration of the magnetic spins, more generally described as the structure. While the skyrmion structure is most often depicted using a two-dimensional projection of the three-dimensional (3D) structure, recent works have emphasized the role of all three dimensions in determining the topology and their response to external stimuli. Here, grazing-incidence small-angle neutron scattering and polarized neutron reflectometry are used to determine the 3D structure of hybrid skyrmions. The structure of the hybrid skyrmions, which includes a combination of Néel-like and Bloch-like components along their length, is expected to significantly contribute to their notable stability, which includes ambient conditions. To interpret the neutron scattering data, micromagnetic simulations of the hybrid skyrmions were performed, and the corresponding diffraction patterns were determined using a Born approximation transformation. The converged magnetic profile reveals the magnetic structure along with the skyrmion depth profile, including the thickness of the Bloch and Néel segments and the diameter of the core.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Non-Equilibrium Effects in Quantum Magnets

While most often the state of a material will tend toward an equilibrium determined by its environment, there are many cases of scientific and technological interest where materials are manipulated to be or are found in non-equilibrium configurations. For example, data can be stored in hard drives by deliberately altering the magnetic orientation in a material to store information in non-equilibrium pattern. In this project, the main goals were studies of non-equilibrium properties of quantum magnets using neutron scattering as the primary experimental method. Neutron scattering allows characterization of magnetic correlation lengths sensitive to the presence of defects. It can also be used to distinguish equilibrium from non-equilibrium states via energy transfer rates. Typical bulk state magnetization relaxation times are too short to perform many neutron scattering measurements of interest. To enable the study of non-equilibrium conditions, materials with longer magnetic relaxation times were targeted. CoNb 2 O 6 was used in two experiments related to non-equilibrium physics. In the first, evidence for defects created via the Kibble-Zurek mechanism (KZM) was sought by quenching across a magnetic field-dependent phase transition. Somewhat unexpectedly, clear evidence for KZM-induced defects was absent. Additional measurements of CoNb 2 O 6 were made to better characterize its crystal field and other properties to provide a better theoretical understanding to enable more effective non-equilibrium physics measurements. In another project, LiHo 0.45 Y 0.55 F 4 was used to compare a quantum annealing protocol to a thermal annealing one since magnetic fields can be used to control the thermal fluctuations in LiHo 0.45 Y 0.55 F 4 . In addition, a new pulsed magnet power supply and new techniques were developed suitable for neutron scattering experimental environments to enable faster magnetic field changes for producing non-equilibrium conditions. The power supply developed for this project has wider technological applications in addition to faster magnetic field ramps.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

β - p and β - α decay of the 11 Be neutron halo ground state

Beta-delayed proton emission from the neutron halo ground state of 11 Be raised much attention due to the unusually high decay rate. It was argued that this may be due to the existence of a resonance just above the proton decay threshold. In this letter, we use the lenses of real-energy continuum shell model to describe several observables including the Gamow–Teller rates for the β - -delayed α and proton decays, and argue that, within our model, the large β - p branching ratio cannot be reconciled with other data.

11Be↗