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DOE OSTI2024

Oak Ridge National Laboratory Neutron Spin Echo Beamline on NB-2

Neutron Spin Echo (NSE) spectroscopy uniquely measures the Q-dependence of slow relaxation dynamics, and having such a machine at HFIR will advance polarized neutron spectroscopy and promote the study of biophysical and energy materials using neutrons. The 2018 Instrument Advisory Board (IAB) advises Neutron Sciences Directorate, ORNL to upgrade the cold neutron delivery system at HFIR, addressing geometrical challenges in neutron transfer from the bright cold source. This is being optimized now: the entrance to the guide system is moving closer to the source, and more guides are being added. However, there are still significant challenges to making the cold flux at the sample world-class. With the proposed guide system, NB-2 can deliver more than 10 6 polarized neutrons per cm 2 /sec below 8Å, and probably 10Å with further optimization. With no potential for running user experiments with neutrons longer than 15Å, the utility of such a machine for biological studies is limited. However, there is a large demand for this class of spectrometer in materials science, chemical engineering, and nanotechnology. Workshops held over the past decade and the three-source vision have highlighted the community's need for a low-angle, high-energy resolution spectrometer at HFIR. A detailed design study of this spectrometer is needed, focusing on optimizing the neutron delivery system for SANS-type studies. This neutron spectrometer would complement studies already performed on both SNSNSE and BASIS by overlapping and extend the dynamic range accessible, while acknowledging the proposed machine, EXPANSE, at the Second Target Station. Two technologies currently exist for such a spectrometer: traditional DC solenoids like those on BL-15 at SNS and IN15 at the ILL, and RF-flipper-based machines similar to RESEDA at FRMII. Either instrument would satisfy the scientific justification. However, there are strong business and scientific cases to utilize the thermal flux, the resonant expertise developed at ORNL, and the potential to utilize an entangled beam of neutrons to probe quantum matter by adopting the neutron resonant spin-echo configuration.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DOE OSTI2026

AutoSAC-Automated Sample Activation Calculation on VULCAN

AutoSAC is an automated python program to conduct sample activation calculation immediately after neutron scattering experiment on VULCAN. AutoSAC takes account of sample dimensions, compositions, forms, sample environments, neutron beam configurations, neutron scattering history, and proton charged resolved beam power etc., and uses a simplified method to rapidly estimate the radioactivity at end of beam or after. It generates a draft report per sample and repository of radioactivity per measurement and provides feedback of current radioactivity and decay time back to a neutron proposal Slack channel to inform users immediately on sample handling. It also utilizes either the sample note field in EPICS or sample composition or thickness correction and takes slack prompt or command to conduct post-beam SAC by demand. The program can be shared to be used in other beamlines at spallation neutron source with modified instrument configurations including instrument specific characteristic beam fluxes.

An, Ke [Oak Ridge National Laboratory (ORNL), Oak ↗

NASA NTRS1979

Soft X-ray emission from the Lupus Loop and Sn 1006 supernova remnants

X-ray maps of the Lupus region have been obtained in a raster scan observation from SAS 3. These show the Lupus Loop to be a faint extended source of soft X-rays with a temperature about 2.5 million K. The most prominent feature of the region is the A.D. 1006 supernova remnant, which is unexpectedly bright at 0.2-1.0 keV. One speculative interpretation of the low-energy flux from SN 1006 is as blackbody radiation from a hot neutron star.

Winkler, P. F., Jr.↗

NASA NTRS1980

Flux distributions and colors of accretion disks

The disk model of Shakura and Sunyaev (1973) and Novikov and Thorne (1973) is used to calculate temperature distributions and integrated spectral fluxes for disks around a typical white dwarf and a typical neutron star, under the assumption that each element of the disk locally radiates as a blackbody. In addition, the disks' integrated UBV colors are calculated using the grid colors for real model atmospheres calculated by Buser and Kurucz (1978) and the observed colors given by Allen (1973). In all the calculations the effect of radiation from one part of the disk on all the other parts is included.

Pacharintanakul, P.↗

NASA NTRS1984

Magnetosphere, Rings, and Moons of Uranus

The observation of an ultraviolet aurora on Uranus implies the existence of a magnetosphere. It is suggested that the magnetospheres of Uranus and Saturn may be very similar. Charged particle sputtering of water ice surfaces on the Uranian moons may maintain an oxygen ion plasma torus similar to the heavy ion plasma torus at Saturn. Atmospheric cosmic ray albedo neutron decay may sustain an inner radiation belt with omnidirectional proton fluxes. If the 100 keV ion fluxes near 7 RU are similar to Saturnian ion fluxes at such energies, the Uranian aurora may be maintained by ion precipitation from the radiation belts at nearly the strong diffusion rate. This mechanism predicts comparable aurorae over both magnetic poles of Uranus, in contrast with the Faraday disc dynamo mechanism, which powers an aurora only over the sunlit pole of uranus. If, however, the 100 kev ion fluxes at Uranus are comparable to those at Saturn, any exposed methane ice surfaces on the moons and rings of Uranus would be quickly transformed by ion impacts to a black, carbonaceous polymer.

Cheng, A. F.↗

NASA NTRS1988

The Geminga X-ray counterpart and a blue optical identification

Based on optical photometry, the identification of the X-ray source 1E 0630+178 with a blue object inside the Einstein error circle is reported. The question of whether the X-rays could be thermal emission from the surface of a neutron star is addressed. The new optical data confirm that relative fluxes in the optical, X-ray, and gamma-ray bands closely match those of the Vela pulsar. The Vela pulsar is adopted as an 'observational model' for Geminga, whereby only the lack of radio emission from Geminga remains to be accounted for. Previous observational results and theoretical models for Geminga are reviewed in light of the new findings.

Halpern, J. P.↗

NASA NTRS1993

The return of the anomalous cosmic rays to 1 Au in 1992

New observations of low energy (approximately 1 to 200 MeV/nuc) cosmic rays measured by three newly launched experiments on Solar, Anomalous, and Magnetospheric Particle Explorer (SAMPEX) during 1992 and 1993 show the strong presence of anomalous cosmic ray (ACR) nitrogen and oxygen, well before the approaching solar minimum. When compared with ACR temporal variations over the past two solar cycles we find that the 1992-1993 fluxes are approximately 5 to 10 times their level at corresponding neutron monitor counting rates in 1969-1970 and 1985.

Mewaldt, R. A.↗

NASA NTRS1999

The Origin of the EUV Emission in Her X-1

Her X-1 exhibits a strong orbital modulation of its EUV (Extreme Ultraviolet Radiation) flux with a large decrease around time of eclipse of the neutron star, and a significant dip which appears at different orbital phases at different 35-day phases. We consider observations of Her X-1 in the EUVE by the Extreme Ultraviolet Explorer (EUVE), which includes data from 1995 near the end of the Short High state, and date from 1997 at the start of the Short High state. The observed EUV lightcurve has bright and faint phases. The bright phase can be explained as the low energy tail of the soft x-ray pulse. The faint phase emission has been modeled to understand its origin. We find: the x-ray heated surface of HZ Her is too cool to produce enough emission; the accretion disk does not explain the orbital modulation; however, reflection of x-rays off of HZ Her can produce the observed lightcurve with orbital eclipses. The dip can be explained by shadowing of the companion by the accretion disk. We discuss the constraints on the accretion disk geometry derived from the observed shadowing.

Leahy, D. A.↗

NASA NTRS1999

The Origin of the EUV Emission in Her X-1

Her X-1 exhibits a strong orbital modulation of its EUV flux with a large decrease around time of eclipse of the neutron star, and a significant dip which appears at different orbital phases at different 35-day phases. We consider observations of Her X-1 in the EUVE by the Extreme Ultraviolet Explorer (EUVE), which includes data from 1995 near the end of the Short High state, and date from 1997 at the start of the Short High state. The observed EUV lightcurve has bright and faint phases. The bright phase can be explained as the low energy tail of the soft x-ray pulse. The faint phase emission has been modeled to understand its origin. We find: the x-ray heated surface of HZ Her is too cool to produce enough emission; the accretion disk does not explain the orbital modulation; however, reflection of x-rays off of HZ Her can produce the observed lightcurve with orbital eclipses. The dip can be explained by shadowing of the companion by the accretion disk. We discuss the constraints on the accretion disk geometry derived from the observed shadowing.

Leahy, D. A.↗

NASA NTRS2011

Suzaku Captures a Possible Eclipse in IGR J16207-5129 and Identifies a Weak-Flaring State in IGR J17391-3021

We present the results from analyses of Suzaku observations of the supergiant X-ray binaries IGR Jl6207-5129 and IGR Jl7391-3021. For IGR Jl6207-5129, we provide the first broadband (0.5-60 keV) spectrum from which we confirm a large intrinsic column density (N(sub H) = 16 X 10(exp 22)/square cm), and constrain the cutoff energy for the first time (E(sub c) 19 keV). We observed a prolonged (> 30 ks) attenuation of the X-ray flux which we tentatively attribute to an eclipse of the probable neutron star by its massive companion. For IGR Jl739J-3021, we witnessed a transition from quiescence to a low-activity phase punctuated by weak flares whose peak luminosities in the 0.5-10 keV band are only a factor of 5 times that of the pre-flare emission. The weak flaring is accompanied by an increase in the absorbing column which suggests the accretion of obscuring clumps of wind. Placing this observation in the context of the recent Swift monitoring campaign, we now recognize that these low-activity epochs constitute the most common emission phase for this system, and perhaps in other supergiant fast X-ray transients (SFXTs) as well.

Bodaghee, Arash↗

DOE OSTI2023

Three-dimensional Dynamics of Strongly Twisted Magnetar Magnetospheres: Kinking Flux Tubes and Global Eruptions

Abstract The origins of the various outbursts of hard X-rays from magnetars (highly magnetized neutron stars) are still unknown. We identify instabilities in relativistic magnetospheres that can explain a range of X-ray flare luminosities. Crustal surface motions can twist the magnetar magnetosphere by shifting the frozen-in footpoints of magnetic field lines in current-carrying flux bundles. Axisymmetric (2D) magnetospheres exhibit strong eruptive dynamics, i.e., catastrophic lateral instabilities triggered by a critical footpoint displacement of ψ crit ≳ π . In contrast, our new three-dimensional (3D) twist models with finite surface extension capture important non-axisymmetric dynamics of twisted force-free flux bundles in dipolar magnetospheres. Besides the well-established global eruption resulting (as in 2D) from lateral instabilities, such 3D structures can develop helical, kink-like dynamics, and dissipate energy locally (confined eruptions). Up to 25% of the induced twist energy is dissipated and available to power X-ray flares in powerful global eruptions, with most of our models showing an energy release in the range of the most common X-ray outbursts, ≲10 43 erg. Such events occur when significant energy builds up while deeply buried in the dipole magnetosphere. Less energetic outbursts likely precede powerful flares, due to intermittent instabilities and confined eruptions of a continuously twisting flux tube. Upon reaching a critical state, global eruptions produce the necessary Poynting-flux-dominated outflows required by models prescribing the fast radio burst production in the magnetar wind—for example, via relativistic magnetic reconnection or shocks.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2025

Capsule Design and Preparation for YH x Specimen Irradiation in the High Flux Isotope Reactor

Advanced nuclear systems for terrestrial microreactors and space applications require moderator materials with high thermal stability, hydrogen retention, and efficient neutron moderation. Yttrium hydride (YH x ) is a promising candidate, but its irradiation performance and hydrogen stability remain insufficiently understood. To address this, Oak Ridge National Laboratory (ORNL) and Los Alamos National Laboratory, supported by the US Department of Energy’s Nuclear Science User Facilities program, have initiated an irradiation campaign in ORNL’s High Flux Isotope Reactor. The experiment employs six irradiation capsules containing YH x specimens (H/Y ≈ 1.9) designed for three target temperatures (300°C, 400°C, and 500°C) and two distinct neutron fast fluence levels. This report documents the irradiation test matrix, capsule design, specimen precharacterization, and experiment readiness for insertion. Planned postirradiation examinations will provide new insights into hydrogen retention and microstructural stability, advancing the understanding of YH x as a moderator for compact reactor applications.

36 MATERIALS SCIENCE↗

NASA NTRS1990

Gravitational radiation from the Galaxy

The spectral flux of gravitational radiation incident on earth from the Galactic W UMa binaries, unevolved binaries, cataclysmic binaries, neutron star binaries, black hole-neutron star binaries, and close white dwarf binary (CWDB) systems is calculated. The peak values for the strain amplitude hv produced by the binaries are: log hv = -17.0/sq rt Hz at log v = -4.40 Hz for W UMa's; log hv = -16.5/sq rt Hz at log v = -5.50 Hz for unevolved binaries; log hv = -18.2/sq rt Hz at log v = -5.15 Hz for neutron star binaries; log hv = -17.0/sq rt Hz at log v = -4.7 Hz for black hole-neutron star binaries; log hv = -18.0 /sq rt Hz at log v = -4.10 Hz for cataclysmic binaries, and log hv = -27.0/sq rt Hz at log v = -4.0 Hz for CWDBs. The gravitational flux at ultralow frequencies is emitted mainly by unevolved binaries. The integrated flux incident on earth is about 2.4 x 10 to the -9th ergs/sq cm/s.

Hils, D.↗

DOE OSTI2025

Capsule Design and Preparation for YH x Specimen Irradiation in the High Flux Isotope Reactor

36 MATERIALS SCIENCE↗

DOE OSTI2022

High-fidelity photoneutron detection via neutron activation analysis

To interdict illicit radioactive sources and prevent nuclear terror, governments have deployed portal monitor systems at ports of entry. Such portal monitors rely upon the detection of spontaneously-emitted radiation signatures, however, detection scenarios become more challenging for highly enriched uranium, which emits relatively few spontaneous radiation signatures. Photon active interrogation techniques can augment current cargo inspection scenarios and improve detection capabilities for illicit nuclear material. A high-energy photon interrogation source can induce photofission in nuclear material, producing strong radiation signatures for detection. Prompt fission signals are of specific interest because prompt neutrons are greater than 99% of the fission signal. When using detectors capable of spectroscopy, e.g., pulse shape discrimination-capable organic scintillators, the intense interrogating source often will cause pulse pile-up, degrading particle classification. In this work, we demonstrate photoneutron detection via neutron activation of aluminum and iron. The experiments rely upon nuclear reactions that can only be induced by neutrons, and are robust against pile-up, thereby providing high-confidence neutron rates. In this work, we apply neutron activation analysis for the detection of high-energy neutrons produced by high-energy photon irradiation; the depleted uranium sample was irradiated with a 9-MeV bremsstrahlung beam. We find that the irradiated depleted uranium produced an aluminum activation flux of 1.77 × 10 5 n cm –2 s –1 and an iron-56 activation flux of 1.05 × 10 5 n cm –2 s –1 . Furthermore, the ability to detect radioactivity induced by neutrons created in (, n) and photofission reactions demonstrates a new approach for photon active interrogation to identify nuclear materials.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DOE OSTI2020

D retention and depth profile behavior for single crystal tungsten with high temperature neutron irradiation

Single crystalline W (tungsten) samples irradiated at 633, 963 and 1073 K by neutrons to a damage level of 0.1 dpa were exposed to a high-flux D (deuterium) plasma at 673, 873 and 973 K, respectively, in TPE (Tritium Plasma Experiment) at INL (Idaho National Laboratory). Deuterium desorption was analyzed by TDS (Thermal Desorption Spectroscopy), and D depth profiles were determined by NRA (Nuclear Reaction Analysis) at SNL (Sandia National Laboratories). HIDT (Hydrogen Isotope Diffusion and Trapping) simulation code was applied to evaluate D behavior for neutron-damaged W at higher temperature. The D retention at depths up to 3 f.tm for the neutron-damaged sample at 673 K was two orders of magnitude larger than that for undamaged tungsten, and its D desorption spectrum had a single broad stage at around 900 K. As the neutron irradiation/plasma exposure temperature increased, D retention was largely reduced, and the desorption temperature was increased to higher temperatures above 1100 K. The D depth profiles by NRA also showed D migration toward bulk by higher temperature irradiation, compared to undamaged W. The HIDT simulation indicated that the major binding energy of D was changed from 1.43 eV to 2.07 eV at higher neutron irradiation and plasma exposure temperatures, suggesting that some vacancies and small vacancy clusters would aggregate to form larger voids, or depopulation of weak traps at high D plasma exposure temperatures. It can be said that more stable trapping sites played dominant roles in the D retention at higher neutron irradiation and plasma exposure temperature. The binding energy by HIDT simulation was almost consistent with the reported value by TMAP, but the consideration of not only total D retention measured by TDS but also D depth profile by NRA led to the more accurate D behavior in neutron-damaged W.

36 MATERIALS SCIENCE↗

DOE OSTI2021

Mechanical behavior of additively manufactured and wrought 316L stainless steels before and after neutron irradiation

Fabrication of nuclear reactor components using additive manufacturing (AM) methods is now a practical option since the AM technologies have advanced to allow for building of complex parts with high quality materials. To assess the mechanical performance of printed components in reactor-relevant conditions and to build a property database for the AM 316L stainless steel (SS), mechanical testing and characterization were performed before and after neutron irradiation. In this work, miniature tensile specimens were irradiated at the High Flux Isotope Reactor (HFIR) to 0.2 and 2 displacements per atom (dpa) at 300 and 600°C. The AM 316L SS was tested in the as-built, stress-relieved, and solution-annealed conditions, and the wrought (WT) 316L SS in solution-annealed condition as a reference alloy. The baseline test result showed that the AM 316L SS, regardless of the post-build heat treatment, had higher strength than the WT 316L SS, but similar ductility. Post-irradiation tensile testing was conducted at RT, 300°C, and 500°C for selected irradiation conditions. Neutron irradiation induced significant changes in the mechanical behavior of the AM stainless steels, including both hardening and softening. Although the as-built 316L steel after 300°C irradiation showed necking just after yielding, the overall property changes of the as-printed alloy became less significant after 600°C irradiation. Irradiation-induced ductilization was also observed after the higher temperature irradiation. In general, the strength change was smaller in the relatively stronger as-built and stress-relieved AM SSs than in the solution-annealed AM and WT SSs. These relatively lower strength 316L SSs overall retained higher ductility in the irradiation conditions tested, but the stronger 316L SSs demonstrated a similar level of ductility after the higher temperature (600°C) irradiation. It is a positive assessment for the AM 316L materials that no embrittlement was observed within the test and irradiation conditions of the experiment.

36 MATERIALS SCIENCE↗

DOE OSTI2022

Density Measurements of Various Molten Sodium, Magnesium, Potassium, and Uranium Chloride Salt Compositions Using Neutron Imaging

With an increased interest in the use of molten salts for energy generation, obtaining thermophysical properties of salt mixtures becomes critical for the understanding of salt performance and behavior. Density is one of the significant thermophysical properties of salt systems. This work presents the density measurement of molten chloride salt mixtures using neutron imaging. This work was performed at the Oak Ridge National Laboratory High-Flux Isotope Reactor. Here, resulting densities as a function of temperature for different molten chloride salts from this work were compared with calculated values using Redlich–Kister modeling. Agreement between the calculated and measured values was within 1–10%, with the exception of the ternary UCl 3 –NaCl–KCl salt that showed a 32% discrepancy between several literature reports; however, the results did align well with another neutron radiography article. Analysis of the radiographs suggests that microbubbles in the ternary mixture might have biased the density measurements.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗