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At least 973 records · Page 54

Temperature and conductivity in shock compressed bridgmanite MgSiO 3 up to 2 TPa

The melting behavior and transport properties of MgSiO 3 at multi-megabar pressures remain poorly constrained despite their importance for high-pressure silicate physics. Here we report the first direct measurements of temperature and optical reflectivity in shock-compressed bridgmanite (MgSiO 3 ) using laser-driven decaying shock compression combined with velocimetry and optical pyrometry. Temperature and reflectivity data spanning approximately 4000–60 000 K were used to constrain the MgSiO 3 melting curve and to infer its electrical conductivity. We find that the MgSiO 3 melting curve becomes shallower than that of iron above 400 GPa, yielding lower melting temperatures in planetary mantles than predicted by several previous theoretical estimates. Across the solid-liquid transition, the inferred electrical conductivity increases significantly, reaching ∼2000 Ω cm −1 . These results provide experimental benchmarks for theoretical models of silicate melting and transport under extreme pressure-temperature conditions.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Absolute dissociative electron attachment cross-section measurement of difluoromethane

Dissociative electron attachment (DEA) to difluoromethane (CH 2 F 2 ) has been studied in the electron energy range of 0 to 16 eV. Two resonant states around 2 and 11.4 eV leading to three different fragment anions (F - , CHF - , and F 2 - ) are observed. Ion-yield curves of the negative ions help us to locate the position of the resonant states. In the ion-yield curve of F - ions, one small hump near 9.8 eV followed by a peak around 15.2 eV is also observed. Absolute DEA cross sections of the F - ion is measured by using the well-known relative flow technique. Dissociation channels associated with each resonant states are identified by density-functional theory (DFT) calculations of the threshold energies. The theory matches quite well within the experimental uncertainty.

74 ATOMIC AND MOLECULAR PHYSICS↗

Phonon dispersion of Mo-stabilized γ -U measured using inelastic x-ray scattering

We have measured the room-temperature phonon spectrum of Mo-stabilized γ–U. The dispersion curves show unusual softening near the H point, q = [1/2,1/2,1/2], which may derive from the metastability of the γ–U phase or from strong electron-phonon coupling. Near the zone center, the dispersion curves agree well with theory, though significant differences are observed away from the zone center. The experimental phonon density of states is shifted to higher energy compared to theory and high-temperature neutron scattering. As a result, the elastic constants of γ-UMo are similar to those of body-centered cubic elemental metals.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Finite-element simulation of the liquid-liquid transition to metallic hydrogen

Hydrogen at high temperature and pressure undergoes a phase transition from a liquid molecular phase to a conductive atomic state, or liquid metallic hydrogen, sometimes referred to as the plasma phase transition (PPT). The PPT phase line was observed in a recent experiment studying laser-pulse heated hydrogen in a diamond anvil cell in the pressure range ~100–170 GPa for temperatures up to ~2000 K. Here, the experimental signatures of the transition are (i) a negative pressure-temperature slope, (ii) a plateau in the heating curve, assumed to be related to the latent heat of transformation, and (iii) an abrupt increase in the reflectance of the sample. We present a finite-element simulation that accurately takes into account the position and time dependence of the heat deposited by the laser pulse. We calculate the heating curves and the sample reflectance and transmittance. This simulation confirms that the observed plateaus are related to the phase transition; however, we find that large values of latent heat are needed and may indicate that dynamics at the transition are more complex than considered in current models. Finally, experiments are proposed that can distinguish between a change in optical properties due to a transition to a metallic state or due to closure of the band gap in molecular hydrogen.

08 HYDROGEN↗

Path integral Monte Carlo and density functional molecular dynamics simulations of warm dense MgSiO 3

In order to provide a comprehensive theoretical description of MgSiO 3 at extreme conditions, we combine results from path integral Monte Carlo and density functional molecular dynamics simulations and generate a consistent equation of state for this material. We consider a wide range of temperature and density conditions from 10 4 to 10 8 K and from 0.321 to 64.2 g/cm -3 (0.1- to 20-fold the ambient density). We study how the L and K shell electrons are ionized with increasing temperature and pressure. We derive the shock Hugoniot curve and compare with experimental results. Our Hugoniot curve is in good agreement with the experiments, and we predict a broad compression maximum that is dominated by the K shell ionization of all three nuclei while the peak compression ratio of 4.70 is obtained when the Si and Mg nuclei are ionized. To conclude, we analyze the heat capacity and structural properties of the liquid.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Shear banding, intermittency, jamming, and dynamic phases for skyrmions in inhomogeneous pinning arrays

In this work, we examine driven skyrmion dynamics in systems with inhomogeneous pinning where a strip of strong pinning coexists with a region containing no pinning. For driving parallel to the strip, we find that the initial skyrmion motion is confined to the unpinned region and the skyrmion Hall angle is zero. At larger drives, a transition occurs to a phase in which motion also appears within the pinned region, creating a shear band in the skyrmion velocity, while the skyrmion Hall angle is still zero. As the drive increases further, the flow becomes disordered and the skyrmion Hall angle increases with drive until saturating at the highest drives when the system transitions into a moving crystal phase. The different dynamic phases are associated with velocity and density gradients across the pinning boundaries. We map out the dynamic phases as a function of pinning strength, skyrmion density, and Magnus force strength, and correlate the phase boundaries with features in the velocity-force curves and changes in the local and global ordering of the skyrmion structure. For large Magnus forces, the shear banding instability is replaced by large-scale intermittent flow in the pinned region accompanied by simultaneous motion perpendicular to the direction of the drive, which appears as oscillations in the transport curves. We also examine the case of a drive applied perpendicular to the strip, where we find a jamming effect in which the skyrmion flow is blocked by skyrmion-skyrmion interactions until the drive is large enough to induce plastic flow.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Magnetic and superconducting anisotropy in Ni-doped RbEuFe 4 As 4 single crystals

We investigate the effect of Ni doping on the Fe site in single crystals of the magnetic superconductor RbEuFe 4 As 4 for doping concentrations of up to 4%. A clear suppression in the superconducting transition temperature is observed in specific-heat, resistivity, and magnetization measurements. Upon Ni doping, the resistivity curves shift up in a parallel fashion, indicating a strong increase of the residual resistivity due to scattering by charged dopant atoms while the shape of the curve and thus the electronic structure appear largely unchanged. The observed step Delta C/T c at the superconducting transition decreases strongly for increasing Ni doping in agreement with expectations based on a model of multiband superconductivity and strong interband pairing. The upper critical field slopes are reduced upon Ni doping for in-plane as well as out-of-plane fields, leading to a small reduction in the superconducting anisotropy. The specific-heat measurements of the magnetic transition reveal the same Berezinskii-Kosterlitz-Thouless behavior close to the transition temperature T m for all doping levels. The transition temperature is essentially unchanged upon doping. The in-plane to out-of-plane anisotropy of Eu magnetism observed at small magnetic fields is unaltered as compared to the undoped compound. In conclusion, all of these observations indicate a decoupling of the Eu magnetism from superconductivity and essentially no influence of Ni doping on the Eu magnetism in this compound.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Anisotropic magnetocaloric effect and critical behavior in CrCl 3

We report anisotropic magnetocaloric effect and magnetic critical behavior in the van der Waals crystal CrCl 3 . The maximum magnetic entropy change $-ΔS^{max}_M ~ 14.6 J kg -1 K -1 and the relative cooling power RCP ~ 340.3 J kg -1 near T c with a magnetic field change of 5 T are much larger when compared to CrI 3 or CrBr 3 . The rescaled ΔS M (T, H) curves collapse onto a universal curve, confirming the second-order ferromagnetic transition. Finally, further critical behavior analysis around T c presents a set of critical exponents β = 0.28 (1) with T c = 19.4 (2) K, γ = 0.89 (1) with T c = 18.95 (8) K, and δ = 4.6 (1) at T c = 19 K , which are close to those of the theoretical tricritical mean-field model.

2-dimensional systems↗

Anisotropic magnetocaloric effect and critical behavior in CrSbSe3

In this work, we report anisotropic magnetocaloric effect and critical behavior in a quasi-one-dimensional ferromagnetic CrSbSe 3 single crystal. The maximum magnetic entropy change - Δ S M max is 2.16 J kg - 1 K - 1 for the easy a axis (2.03 J kg - 1 K - 1 for the hard b axis) and the relative cooling power RCP is 163.1 J kg - 1 for the easy a axis (142.1 J kg - 1 for the hard b axis) near T c with a magnetic field change of 50 kOe. The magnetocrystalline anisotropy constant K u is estimated to be 148.5 kJ m - 3 at 10 K, decreasing to 39.4 kJ m - 3 at 70 K. The rescaled Δ S M ( T , H ) curves along all three axes collapse onto a universal curve, respectively, confirming the second-order ferromagnetic transition. Further critical behavior analysis around T c ~ 70 K gives that the critical exponents β = 0.26 ( 1 ) , γ = 1.32 ( 2 ) , and δ = 6.17 ( 9 ) for H ∥ a , while β = 0.28 ( 2 ) , γ = 1.02 ( 1 ) , and δ = 4.14 ( 16 ) for H ∥ b . The determined critical exponents suggest that the anisotropic magnetic coupling in CrSbSe 3 is strongly dependent on orientations of the applied magnetic field.

2-dimensional systems↗

High-pressure phase diagram of beryllium from ab initio free-energy calculations

In this report we use first-principles molecular dynamics simulations coupled with the thermodynamic integration method to study the hexagonal close-packed (hcp) to body-centered cubic (bcc) transition and melting of beryllium up to a pressure of 1600 GPa. We derive the melting line by equating solid and liquid Gibbs free energies and represent it by a Simon-Glatzel fit T m = 1564 K [1 + P/(15.6032 GPa)] 0.383 , which is in good agreement with previous two-phase simulations <6000 K. We also derive the hcp-bcc solid-solid phase boundary and show that the quasiharmonic approximation underestimates the stability of the hcp structure, predicting lower transition pressures between hcp and bcc phases. Our results are consistent with the stability regime predicted by the phonon quasiparticle method. We also predict that the hcp-bcc-liquid triple point is located at 164.7 GPa and 4314 K. In addition, we compute the shock Hugoniot curve and show that it is in good agreement with experiments, intersecting our derived melting curve at ~235 GPa and 4900 K. Finally, we make predictions for future ramp compression experiments. Starting with an isentropic compression of the liquid, we predict the path to intersect the melting line at low pressure and temperature, then to continue along the melting line over a large temperature interval of 7000 K as the sample remains in the mixed solid-liquid state before it enters the solid phase.

36 MATERIALS SCIENCE↗

Melting of magnesium oxide up to two terapascals using double-shock compression

Constraining the melting behavior of magnesium oxide, a major constituent of gaseous and rocky planets, is key to benchmarking their evolutionary models. Using a double-shock technique, we extended the MgO melt curve measurements to 2 TPa; this is twice the pressure achieved by previous melting experiments on any material. A temperature plateau is observed between 1218 and 1950 GPa in the second shock states, which is attributed to latent heat of melting. At 1950 GPa, the measured melting temperature is 17,600 K, 17% lower than recent theoretical predictions. Furthermore, the melting curve is steeper than that of MgSiO 3 , indicating that MgO is likely solid in the interior of Saturn-sized gas giants and extra-solar super-Earth planets.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Evidence for temperature chaos in spin glasses

We study the field cooled magnetization of a CuMn spin glass (SG) under temperature perturbations. The T-cycling curves are compared with the reference curve without temperature cycling. There is a crossover from the cumulative aging region to noncumulative aging region as the temperature change is increased. The cumulative aging range scales with the chaos length, ℓ c , becoming comparable to the correlation length, ξ, at the crossover boundary. The extracted chaos exponent, ζ=1.1, is in agreement with theoretical predictions. Furthermore, our results strongly suggest temperature chaos exists in real SG systems.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Slow spin dynamics and quantum tunneling of magnetization in the dipolar antiferromagnet DyScO 3

Here, we present a comprehensive study of static and dynamic magnetic properties in the Ising-like dipolar antiferromagnet (AFM) DyScO 3 by means of DC and AC magnetization measurements supported by classical Monte Carlo calculations. Our AC-susceptibility data show that the magnetic dynamics exhibit a clear crossover from an Arrhenius-like regime to quantum tunneling of magnetization (QTM) at T*=10K. Below T N =3.2K, DyScO 3 orders in an antiferromagnetic GxAy-type magnetic structure and the magnetization dynamics slow down to the minute timescale. The low-temperature magnetization curves exhibit complex hysteretic behavior, which depends strongly on the magnetic field sweep rate. We demonstrate that the low-field anomalies on the magnetization curve are related to the metamagnetic transition, while the hysteresis at higher fields is induced by a strong magnetocaloric effect. Our theoretical calculations, which take into account dipolar interaction between Dy 3+ moments, reproduce essential features of the magnetic behavior of DyScO 3 . We demonstrate that DyScO 3 represents a rare example of an inorganic compound, which exhibits QTM at a single-ion level and magnetic order due to classical dipolar interaction.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Pressure-induced metallization and loss of surface magnetism in FeSi

Single-crystalline FeSi samples with a conducting surface state were studied under high pressure and magnetic field by means of electrical resistance measurements to explore how the bulk semiconducting state and the surface state are tuned by the application of pressure. Here, we found that the energy gap associated with the semiconducting bulk phase begins to close abruptly at a critical pressure of ~10 GPa and the bulk material becomes metallic with no obvious sign of any emergent phases or non-Fermi liquid behavior in temperature dependent electrical resistance in the neighborhood of the critical pressure above 3 K. Moreover, the metallic phase appears to remain at near-ambient pressure upon release of the pressure. Interestingly, the hysteresis in the electrical resistance vs magnetic field curve associated with the magnetically ordered conducting surface state decreases with pressure and vanishes at the critical pressure, while the slope of the electrical resistance vs magnetic field curve, which has a negative value for pressure below the critical pressure, decreases in magnitude with pressure and changes sign at the critical pressure. Thus the conducting surface state and the corresponding two-dimensional magnetic order collapse at the critical pressure where the energy gap of the bulk material starts to close abruptly, revealing the connection between the conducting surface state and the semiconducting bulk state in FeSi.

36 MATERIALS SCIENCE↗

Primary $\gamma$-ray intensities and $\gamma$-strength functions from discrete two-step $\gamma$-ray cascades in radiative proton-capture experiments

Background: Reaction rates of radiative capture reactions can play a crucial role in the nucleosynthesis of heavy nuclei in explosive stellar environments. These reaction rates depend strongly on $\gamma$-ray decay widths in the reaction products, which are, for nonresonant capture reactions at high excitation energies, derived from the $\gamma$-ray strength function and the nuclear level density. Recently, the ratio method was applied to primary $\gamma$ rays observed from ($\textit{d, p}$) reactions and nuclear resonance fluorescence measurements to extract the dipole strength in atomic nuclei and to test the generalized Brink-Axel hypothesis. Purpose: The purpose of this work is to apply the ratio method to primary $\gamma$-ray intensities of the 63,65 Cu($\textit{p},\gamma$) reactions to extract $\gamma$-ray strength information on the nuclei 64,66 Zn. Here, the impact of spin distribution, total $\gamma$-ray decay widths, level densities, and width fluctuations on the application of the ratio method will be discussed. Additionally, by comparing the relative $\gamma$-ray strength at different excitation energies, conclusions on the validity of the generalized Brink-Axel hypothesis can be made. Method: The radiative proton capture reaction measurements have been performed at the HORUS $\gamma$-ray spectrometer of the University of Cologne at one excitation energy for each reaction. Primary $\gamma$-ray intensities have been determined by normalizing secondary $\gamma$-ray transitions in two-step cascades using their absolute branching ratio. The ratio method was applied to the measured primary $\gamma$-ray intensities as well as to previous measurements by Erlandsson et al. at different excitation energies. Results: The relative strength function curve for 64 Zn from our measurement shows no significant deviation from the previous measurement at a different excitation energy. The same is true for 66 Zn where both measurements were at almost the same excitation energy. Absolute $\gamma$-strength function values have been obtained by normalizing the relative curves to quasiparticle random phase approximation calculations because of the absence of experimental data in the respective energy region. Conclusion: The generalized Brink-Axel hypothesis, i.e., the independence of the strength function on the excitation energy, seems to hold in the studied energy region and nuclei. The method to obtain primary $\gamma$-ray intensities from two-step cascade spectra was shown to be a valuable and sensitive tool although its uncertainties are connected to the knowledge of the low-energy level scheme of the investigated nucleus. The scaling in the ratio method should be taken with care, because the relative strength is not a simple sum of $f_{E1}$ and $f_{M1}$ but a somewhat complex linear combination dependent on the excitation energy of the nucleus.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Apparent temperatures of neutron-poor and neutron-rich compound nuclei

The possibility of the dependence of the nuclear caloric curve on neutron excess sets a limit on the accuracy of our knowledge of the nuclear equation of state, and thus impacts predictive capabilities of nuclear reaction and nuclear astrophysics models. To date, theoretical models have not reached consensus on the magnitude or sign on the asymmetry dependence. To provide constraints, we have measured evaporated particles and heavy residues for complete and incomplete fusion-evaporation reactions in inverse kinematics. The temperatures extracted from the observed light charged particles tend to favor higher temperatures for the neutron-rich fused systems, though they are near the limits of the systematic uncertainty. The present measurement may be used as an upper limit to constrain the asymmetry dependence of the nuclear caloric curve.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Testing dark matter and modifications to gravity using local Milky Way observables

Galactic rotation curves are often considered the first robust evidence for the existence of dark matter. Yet, even in the presence of a dark matter halo, other galactic-scale observations, such as the Baryonic Tully-Fisher Relation and the Radial Acceleration Relation, remain challenging to explain. This has motivated long-distance, infrared modifications to gravity as an alternative to the dark matter hypothesis as well as various DM theories with similar phenomenology. In general, the standard lore has been that any model that reduces to the phenomenology of MOdified Newtonian Dynamics (MOND) on galactic scales explains essentially all galaxy-scale observables. We present a framework to test precisely this statement using local Milky Way observables, including the vertical acceleration field, the rotation curve, the baryonic surface density, and the stellar disk profile. We focus on models that predict scalar amplifications of gravity, i.e., models that increase the magnitude but do not change the direction of the gravitational acceleration. We find that models of this type are disfavored relative to a simple dark matter halo model because the Milky Way data necessitates a substantial amplification of the radial acceleration with little amplification of the vertical acceleration. We conclude that models which result in a MOND-like force struggle to simultaneously explain both the rotational velocity and vertical motion of nearby stars in the Milky Way.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Swampland cobordism conjecture and non-Abelian duality groups

We study the cobordism conjecture of McNamara and Vafa which asserts that the bordism group of quantum gravity is trivial. In the context of type IIB string theory compactified on a circle, this predicts the presence of D7-branes. On the other hand, the non-Abelian structure of the IIB duality group SL (2, Z) implies the existence of additional [p, q] 7-branes. We find that this additional information is instead captured by the space of closed paths on the moduli space of elliptic curves parameterizing distinct values of the type IIB axio-dilaton. This description allows to recover the full structure of non-Abelian braid statistics for 7-branes. Combining the cobordism conjecture with an earlier Swampland conjecture by Ooguri and Vafa, we argue that only certain congruence subgroups $\Gamma\subset$ SL(2, Z) specifying genus zero modular curves can appear in 8D F-theory vacua. This leads to a successful prediction for the allowed Mordell–Weil torsion groups for 8D F-theory vacua.

79 ASTRONOMY AND ASTROPHYSICS↗