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At least 973 records · Page 54

Estimation of cirrus cloud particle fallspeeds from vertically pointing Doppler radar

The First ISCCP (International Satellite Cloud Climatology Project) Regional Experiment 2 (FIRE 2) was conducted in Coffeyville, Kansas in late 1991 to study the microphysical and radiative properties of cirrus clouds. A variety of active and passive remote sensors were employed, including an 8-mm-wavelength cloud-sensing Doppler radar developed at the Wave Propagation Laboratory (WPL). The radar, having excellent sensitivity to cloud particles (-30 dBZ at 10 km), good spatial resolution (37 m), and velocity precision (.05 ms -1), is an excellent tool for observing cirrus clouds. Having this radar directed toward the zenith for long periods of time during FIRE 2 permitted the reflectivity-weighted particle fallspeed to be related to reflectivity which allowed a separation of ice particle fallspeeds from vertical air motions. Additionally, such relationships proved useful in other multi-sensor techniques for determining vertical profiles of ice particle characteristic size and ice water content in cirrus clouds. The analysis method and the results of applying it to cirrus cloud reflectivity and velocity data collected during FIRE 2 are discussed.

Orr, Brad W.↗

Orbiting Rainbows: Optical Manipulation of Aerosols and the Beginnings of Future Space Construction

Our objective is to investigate the conditions to manipulate and maintain the shape of an orbiting cloud of dust-like matter so that it can function as an ultra-lightweight surface with useful and adaptable electromagnetic characteristics, for instance, in the optical, RF, or microwave bands. Inspired by the light scattering and focusing properties of distributed optical assemblies in Nature, such as rainbows and aerosols, and by recent laboratory successes in optical trapping and manipulation, we propose a unique combination of space optics and autonomous robotic system technology, to enable a new vision of space system architecture with applications to ultra-lightweight space optics and, ultimately, in-situ space system fabrication. Typically, the cost of an optical system is driven by the size and mass of the primary aperture. The ideal system is a cloud of spatially disordered dust-like objects that can be optically manipulated: it is highly reconfigurable, fault-tolerant, and allows very large aperture sizes at low cost. See Figure 1 for a scenario of application of this concept. The solution that we propose is to construct an optical system in space in which the nonlinear optical properties of a cloud of micron-sized particles are shaped into a specific surface by light pressure, allowing it to form a very large and lightweight aperture of an optical system, hence reducing overall mass and cost. Other potential advantages offered by the cloud properties as optical system involve possible combination of properties (combined transmit/receive), variable focal length, combined refractive and reflective lens designs, and hyper-spectral imaging. A cloud of highly reflective particles of micron-size acting coherently in a specific electromagnetic band, just like an aerosol in suspension in the atmosphere, would reflect the Sun's light much like a rainbow. The only difference with an atmospheric or industrial aerosol is the absence of the supporting fluid medium. This new concept is based on recent understandings in the physics of optical manipulation of small particles in the laboratory and the engineering of distributed ensembles of spacecraft clouds to shape an orbiting cloud of micron-sized objects. In the same way that optical tweezers have revolutionized micro- and nano-manipulation of objects, our breakthrough concept will enable new large scale NASA mission applications and develop new technology in the areas of Astrophysical Imaging Systems and Remote Sensing because the cloud can operate as an adaptive optical imaging sensor. While achieving the feasibility of constructing one single aperture out of the cloud is the main topic of this work, it is clear that multiple orbiting aerosol lenses could also combine their power to synthesize a much larger aperture in space to enable challenging goals such as exoplanet detection. Furthermore, this effort could establish feasibility of key issues related to material properties, remote manipulation, and autonomy characteristics of cloud in orbit. There are several types of endeavors (science missions) that could be enabled by this type of approach, i.e. it can enable new astrophysical imaging systems, exoplanet search, large apertures allow for unprecedented high resolution to discern continents and important features of other planets, hyperspectral imaging, adaptive systems, spectroscopy imaging through limb, and stable optical systems from Lagrange-points. Future micro-miniaturization might hold promise of a further extension of our dust aperture concept to other more exciting smart dust concepts with other associated capabilities.

Space Construction↗

A Hierarchical Modeling Study of the Interactions Among Turbulence, Cloud Microphysics, and Radiative Transfer in the Evolution of Cirrus Clouds

This project used a hierarchy of cloud resolving models to address the following science issues of relevance to CRYSTAL-FACE: What ice crystal nucleation mechanisms are active in the different types of cirrus clouds in the Florida area and how do these different nucleation processes influence the evolution of the cloud system and the upper tropospheric humidity? How does the feedback between supersaturation and nucleation impact the evolution of the cloud? What is the relative importance of the large-scale vertical motion and the turbulent motions in the evolution of the crystal size spectra? How does the size spectra impact the life-cycle of the cloud, stratospheric dehydration, and cloud radiative forcing? What is the nature of the turbulence and waves in the upper troposphere generated by precipitating deep convective cloud systems? How do cirrus microphysical and optical properties vary with the small-scale dynamics? How do turbulence and waves in the upper troposphere influence the cross-tropopause mixing and stratospheric and upper tropospheric humidity? The models used in this study were: 2-D hydrostatic model with explicit microphysics that can account for 30 size bins for both the droplet and crystal size spectra. Notably, a new ice crystal nucleation scheme has been incorporated into the model. Parcel model with explicit microphysics, for developing and evaluating microphysical parameterizations. Single column model for testing bulk microphysics parameterizations

Curry, Judith↗

Quantifying Uncertainty in Ice Particle Velocity–Dimension Relationships Using MC3E Observations

Abstract Ice particle terminal fall velocity ( V t ) is fundamental for determining microphysical processes, yet remains extremely challenging to measure. Current theoretical best estimates of V t are functions of Reynolds number. The Reynolds number is related to the Best number, which is a function of ice particle mass, area ratio ( A r ), and maximum dimension ( D max ). These estimates are not conducive for use in most models since model parameterizations often take the form , where ( α , β ) depend on habit and D max . A previously developed framework is used to determine surfaces of equally plausible ( α , β ) coefficients whereby ice particle size/shape distributions are combined with V t best estimates to determine mass- ( V M ) or reflectivity-weighted ( V Z ) velocities that closely match parameterized V M ,SD or V Z ,SD calculated using the ( α , β ) coefficients using two approaches. The first uses surfaces of equally plausible ( a , b ) coefficients describing mass ( M )–dimension relationships (i.e., ) to calculate mass- or reflectivity-weighted velocity from size/shape distributions that are then used to determine ( α , β ) coefficients. The second investigates how uncertainties in A r , D max , and size distribution N ( D ) affect V M or V Z . For seven of nine flight legs flown on 20 and 23 May 2011 during the Mesoscale Continental Convective Clouds Experiment (MC3E), uncertainty from natural parameter variability—namely, the variability in ice particle parameters in similar meteorological conditions—exceeds uncertainties arising from different A r assumptions or D max estimates. The combined uncertainty between A r , D max , and N ( D ) produced smaller variability in ( α , β ) compared to varying M ( D ), demonstrating M ( D ) must be accurately quantified for model fall velocities. Primary sources of uncertainty vary considerably depending on environmental conditions. Significance Statement Ice particle fall velocity is fundamental for numerous processes within clouds, and hence is a critical property that must be accurately represented in weather and climate models. Using aircraft observations of ice particle shapes and sizes obtained in clouds behind midlatitude thunderstorms, this work develops a new framework for estimating ice particle fall velocities and their uncertainty, including quantifying the importance of different uncertainty sources from cloud microphysics measurements. Natural parameter variability contributes the most uncertainty in ice particle fall velocity estimates, although other sources can also be important contributors to uncertainty in certain conditions. Additional work examining ice particle data is needed to further understand how dependent uncertainty in certain ice particle properties are to local environmental conditions.

Meteorology & Atmospheric Sciences↗

Survey of microphysical properties of marine boundary-layer clouds in the Western North Atlantic

Oceanic low level clouds strongly affect the atmospheric radiation budget. Uncertainties in their microphysical properties and cover currently limit the accuracy of climate predictions. Further, studies quantifying the relative importance of aerosol and dynamics on cloud properties in specific meteorological regimes are poorly constrained by observations in the Western North Atlantic boundary layer. Low level clouds were measured during the Aerosol Cloud meTereology Interactions oVer the western ATlantic Experiment (ACTIVATE) campaign in winter and summer 2020. The two NASA LaRC research aircraft HU-25 Falcon and UC-12 B-200 King Air conducted 35 simultaneous flights to investigate aerosol-cloud interactions of maritime clouds and their impact on radiation. Number concentration, liquid water content, ice water content, and particle size distribution in the size range of 3 µm to 1460 µm in diameter were measured with the fast forward scattering cloud probe (FCDP) and 2-dimensional optical array imaging probe (2D-S) onboard the Falcon. Here, we present an overview of late winter (February-March) and late summer (August-September) oceanic cloud properties in the region 65°W to 80°W and 30°N to 40°N. We compare cloud properties in these two seasons and investigate their dependence on meteorological parameters and aerosol abundance. In a case study, we present cloud observations in a cold air outbreak event on 1 March 2020 with a specific focus on mixed-phase clouds.

microphysical properties↗

Parameterization of Cloud Optical Properties for a Mixture of Ice Particles for use in Atmospheric Models

Based on the single-scattering optical properties that are pre-computed using an improve geometric optics method, the bulk mass absorption coefficient, single-scattering albedo, and asymmetry factor of ice particles have been parameterized as a function of the mean effective particle size of a mixture of ice habits. The parameterization has been applied to compute fluxes for sample clouds with various particle size distributions and assumed mixtures of particle habits. Compared to the parameterization for a single habit of hexagonal column, the solar heating of clouds computed with the parameterization for a mixture of habits is smaller due to a smaller cosingle-scattering albedo. Whereas the net downward fluxes at the TOA and surface are larger due to a larger asymmetry factor. The maximum difference in the cloud heating rate is approx. 0.2 C per day, which occurs in clouds with an optical thickness greater than 3 and the solar zenith angle less than 45 degrees. Flux difference is less than 10 W per square meters for the optical thickness ranging from 0.6 to 10 and the entire range of the solar zenith angle. The maximum flux difference is approximately 3%, which occurs around an optical thickness of 1 and at high solar zenith angles.

Chou, Ming-Dah↗

Possible NASA Contributions to HEAT

A four-year experiment (HEAT) has been proposed (one summer in the field, 2005) to determine the sources and causes for the enhanced cloud-to-ground lightning over Houston, Texas, in association with simultaneous experiments by the Environmental Protection Agency (EPA) and the Texas Natural Resource Conservation Commission (TNRCC). Houston is the third most populous city in the United States and the region contains 50% of the petroleum refining capacity of the United States. Recent studies covering the period 1989-2000 document a 50% increase of cloud-to-ground lightning in the Houston area as compared to background values, which is second in flash density only to the Tampa Bay, Florida area. It is suggested that the elevated flash densities could result from several factors, including, 1) the convergence due to the urban heat island effect and complex sea breeze, and 2) the increasing levels of air pollution from anthropogenic sources producing numerous small droplets and thereby suppressing mean droplet size. The latter effect would enable more cloud water to reach the mixed phase region where it is involved in the formation of precipitation and the separation of electric charge, leading to an enhancement of lightning. The primary goals of HEAT are to examine the effects of (1) pollution, (2) the urban heat island, and (3) the complex coastline, on storms and lightning characteristics in the Houston area. The project is a multi- agency effort and will employ numerous observing capabilities and expertise. Dr. Shepherd has been asked to serve as a possible co- investigator to contribute expertise in areas related to urban impacts on precipitation variability. Dr. Shepherd is also a key NASA representative in the interagency effort. This presentation will provide an overview of recent NASA research focused on urban rainfall in Houston and offer potential NASA capabilities that could contribute to HEAT.

Shepherd, J. M.↗

Compositional Grading in an Impact-produced Spherule Bed, Barberton Greenstone Belt, South Africa: A Key to Condensation History of Rock Vapor Clouds

The chemical and physical processes by which spherules form during the condensation of impact-produced rock vapor clouds are poorly understood. Although efforts have been made to model the processes of spherule formation, there is presently a paucity of field data to constrain the resulting theoretical models. The present study examines the vertical compositional variability in a single early Archean spherule bed in the Barberton Greenstone Belt (BGB), South Africa, in order to better identify the process by which impact vapor clouds condense and spherules form and accumulate. The BGB spherule beds are suitable for this type of study because of their great thickness, often exceeding 25cm of pure spherules, due to the massive sizes of the impactors. Two main problems complicate analysis of vertical compositional variability of graded spherule beds: (1) differential settling of particles in both the vapor and water column due to density and size differences and (2) turbulence within the vapor cloud. The present study compares sections of spherule bed S3 from four different depositional environments in the Barberton Greenstone Belt: (1) The Sheba Mine section (SAF-381) was deposited under fairly low energy conditions in deep water, providing a nice fallout sequence, and also has abundant Ni-rich spinels; (2) Jay's Chert section (SAF-380) was deposited in subaerial to shallow-water conditions with extensive post-depositional reworking by currents. The spherules also have preserved spinels; (3) the Loop Road section (loc. SAF-295; samp. KSA-7) was moderately reworked and has only rare preservation of spinels; and (4) the shallow-water Barite Syncline section (loc. SAF-206; samp KSA-1) has few to no spinels preserved and is not reworked. Although all of the spherule beds have been altered by silica diagenesis and K-metasomatism, most of the compositional differences between these sections appear to reflect their diagenetic histories, possibly related to their differing depositional environments. Sulfate diagenesis in the Barite Syncline and Loop road sections may account for the loss of spinels.

Krull, A. E.↗

Airborne measurements of Space Shuttle exhaust constituents

Airborne measurements of hydrogen chloride (HCl) and particulates made during penetrations into and flights under Space Shuttle exhaust clouds from launches STS-1, -2, and -5 are presented to permit comparison with dispersion model predictions for Space Shuttle exhaust clouds, and with previous measurements made in Titan III exhaust clouds. Analytical techniques employed for the Shuttle measurements were developed and refined during earlier Titan III exhaust cloud measurements and include the measurements of particulate concentrations, size distributions, and the partitioning of HCl between the gaseous and aerosol phases. The results are useful in understanding the dynamics of ground cloud development, atmospheric dispersion, and potential environmental effects of Shuttle effluents.

Cofer, W. R., III↗

Multiple scattering lidar returns from stratus clouds

Multiple scattering lidar returns from stratus clouds were measured using a multi-field-of-view (MFOV) lidar operating at 1.054 microns. The detector consists of four concentric silicon photodiodes which define half-angle fields of view (FOV) of 3.8, 12.5, 25 and 38.5 mrad. The central FOV receives the conventional lidar signal, while the outer FOV's receive only multiply scattered contributions. The ratios of the signals in the outer FOV's to the signal in the central FOV is an indication of the lateral spreading of the scattered component of the laser pulse as it propagates through the cloud. MFOV lidar returns from stratus clouds measured between October 1991 and March 1992 can be divided into two distinct types, those with large multiple scattering ratios and those with small ratios. An example of each type of return is shown. Both measurements were made at an elevation angle of 45 degrees. Clouds with small multiple scattering signals probably have a high concentration of much larger particles on the order of hundreds of micrometers in size. This is a typical size range for suspended ice crystals or precipitations. Stratus clouds often have a high concentration of ice crystals even when there is no precipitation. Large ice crystals would give smaller signals in the outer FOV's because much of the scattered intensity is contained in a narrow diffraction peak with an angular width on the order of milliradians. The result is that for a given extinction, many more orders of scattering are required for the laser pulse to spread out. So far we have not been able to do simulations of MFOV lidar returns from ice crystal clouds because of uncertainties about the phase function of the crystals, particularly the magnitude of the backscatter peak at 180 degrees. On two occasions, MFOV lidar returns measured just prior to snowfall, showed a striking vertical profile. An example is shown. From 900 to 1300m, the multiply scattered signals are negligible compared to the return in the central FOV. Abruptly, at 1300m strong signals begin in the outer FOVs. These results could be explained by the presence of a cloud layer composed of water droplets at a range of 1300m (or 900m above ground) with snow precipitations forming at the bottom of the cloud. By measuring the polarization ratio of lidar signals, Pal and Carswell have observed snow precipitating from a cloud layer composed of water droplets. Based on these results, we believe that analysis of multiple scattering lidar returns can yield important information on the phase of cloud particles.

Hutt, D. L.↗

ARM shortwave spectrometers to study the clear-cloud transition zone and mixing processes

The proposed research is a collaborative effort between NASA/Goddard Space Flight Center and the Hebrew University of Jerusalem. While the NASA team focused on analyzing ground-based hyper-spectral radiance observations to understand cloud edge properties and their connection to mixing processes, the Hebrew University team tackled the problem through cloud modeling activities. By approximating the shortwave spectra in the cloud-clear transition zone as a linear combination of purely clear and purely cloudy spectra we can characterize the variations of cloud optical thickness and cloud droplet effective radius in the transition zone. When applying this method to the measurements of a ground-based shortwave spectroradiometer at the ARM’s SGP site, representing continental conditions, and MAGIC field campaign between Log Angeles, California and Honolulu, Hawaii, representing maritime scenarios, we found that cloud optical depth consistently decreases in both cases, but droplet size decreases much more substantially for the continental regime, suggesting different mixing processes for the continental and maritime conditions. The investigation and measurements of radiation clouds were coupled with a unique cloud modeling. A novel spectral bin microphysics was developed and implemented to the System of Atmospheric Modeling (SAM). In order to resolve cloud transition zones with high spatial gradients of microphysical variables a unique high resolution (10 m) was used in simulations. The model calculates droplet size distributions in each grid point. The model output was transferred to the NASA/GSFC team for utilization in radiative calculations and testing of both radiative algorithm and model representation.

54 ENVIRONMENTAL SCIENCES↗

Counterflow Virtual Impactor (CVI) Inlet Aboard Aircraft (INLETCVI-AIR) Instrument Handbook

The counterflow virtual impactor (CVI) inlet separates out and samples cloud elements via inertial impaction. Warm, dry, particle-free carrier gas of known composition is pumped to the tip of the inlet in the direction opposite of the flow of air. The flow lines of the incoming free stream air are split. Larger droplets and ice crystals suspended in the sample air have enough inertia to penetrate the counterflow and enter the sample flow, while smaller, unactivated particles follow the streamlines of the air flowing around the inlet’s tip (Noone et al. 1988). The instrument is capable of sampling cloud elements as a function of cut size by changing the velocity of counterflow at the probe tip. The CVI cut size is usually defined as a diameter of a smallest particle for which penetration rate is 50%. For the U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) user facilityGulfstream-159 aircraft’s CVI inlet, that value is usually around 13 microns. The dry heated air, normally used as the carrier gas, also serves to evaporate water from the hydrometeor, leaving the residuals to be sampled by in-cabin aerosol instrumentation. The number concentration of the droplet residue in the CVI sample line is usually increased with respect to corresponding cloud element number concentration. The CVI performance as a concentrator is usually described via CVI enhancement factor, which is a conversion factor between ambient volumetric concentration (not adjusted to standard temperature and pressure) and volumetric concentration in the CVI sample line.

54 ENVIRONMENTAL SCIENCES↗

Introduction to MODIS Cloud Products

The Earth's radiative energy balance and hydrological cycle are fundamentally coupled with the distribution and properties of clouds. Therefore, the ability to remotely infer cloud properties and their variation in space and time is crucial for establishing climatologies as a reference for validation of present-day climate models and in assessing future climate change. Remote cloud observations also provide data sets useful for testing and improving cloud model physics, and for assimilation into numerical weather prediction models. The MODerate Resolution Imaging Spectroradiometer (MODIS) imagers on the Terra and Aqua Earth Observing System (EOS) platforms provide the capability for globally retrieving these properties using passive solar reflectance and infrared techniques. In addition to providing measurements similar to those offered on a suite of historical operational weather platforms such as the Advanced Very High Resolution Radiometer (AVHRR), the High-resolution Infrared Radiation Sounder (HIRS), and the Geostationary Operational Environmental Satellite (GOES), MODIS provides additional spectral and/or spatial resolution in key atmospheric bands, along with on-board calibration, to expand the capability for global cloud property retrievals. The core MODIS operational cloud products include cloud top pressure, thermodynamic phase, optical thickness, particle size, and water path, and are derived globally at spatial resolutions of either 1- or 5-km (referred to as Level-2 or pixel-level products). In addition, the MODIS atmosphere team (collectively providing cloud, aerosol, and clear sky products) produces a combined gridded product (referred to as Level-3) aggregated to a 1 equal-angle grid, available for daily, eight-day, and monthly time periods. The wealth of information available from these products provides critical information for climate studies as well as the continuation and improved understanding of existing satellite-based cloud climatologies derived from heritage instruments. This chapter provides an overview of the MODIS Level-2 and -3 operational cloud products.

Baum, Bryan A.↗

Microphysical Properties of Tropical Tropopause Layer Cirrus

Pervasive cirrus clouds in the tropical tropopause layer (TTL) play an important role in determining the composition of stratospheric air through dehydration of tropospheric air entering the stratosphere. This dehydration affects Earth's energy budget and climate, yet uncertainties remain regarding the microphysical processes that govern TTL cirrus. TTL cirrus were sampled with the NASA Global Hawk UAV for over 30 hr in the Western Pacific in 2014 during the Airborne Tropical TRopopause EXperiment. In situ measurements by a Fast Cloud Droplet Probe and Hawkeye probe (combination Fast Cloud Droplet Probe, Two‐Dimensional Stereo optical array probe, and Cloud Particle Imager) provided particle concentrations and sizing between 1‐ and 1,280‐μm diameter and high resolution images for habit identification. We present the variability in ice concentrations, size distributions, and habits as functions of temperature, altitude, and time since convective influence. Observed ice particles were predominantly small and quasi‐spheroidal in shape, with the percentage of quasi‐spheroids increasing with decreasing temperature. In comparison to the large fraction of the population consisting of quasi‐spheroids, faceted habits (columns, plates, rosettes, and budding rosettes) constituted a smaller percentage of the overall population and exhibited the opposite correlation with temperature. The trend of higher percentages of faceted crystals occurring at warmer temperatures may be due to diffusional growth or aggregation as particles descend through cloud, and/or the more rapid diffusional growth rate at warmer temperatures. Sampling was typically well away from deep convection, however, and very few aggregates were observed, so the trend of higher percentages of faceted habits is likely attributable to diffusional growth.

Woods, Sarah↗

The radiation budget of a Cirrus layer deduced from simultaneous aircraft observations and model calculations

Several aircraft were employed during the FIRE Cirrus IFO in order to make nearly simultaneous observations of cloud properties and fluxes. A segment of the flight data collected on 28 October 1988 during which the NASA Ames ER-2 overflew the NCAR King Air was analyzed. The ER-2 flew at high altitude making observations of visible and infrared radiances and infrared flux and cloud height and thickness. During this segment, the King Air flew just above the cloud base making observations of ice crystal size and shape, local meteorological variables, and infrared fluxes. While the two aircraft did not collect data exactly coincident in space and time, they did make observations within a few minutes of each other. For this case study, the infrared radiation balance of the cirrus layer is of primary concern. Observations of the upwelling 10 micron radiance, made from the ER-2, can be used to deduce the 10 micron optical depth of the layer. The upwelling broadband infrared flux is also measured from the ER-2. At the same time, the upwelling and downwelling infrared flux at the cloud base is obtained from the King Air measurements. Information on cloud microphysics is also available from the King Air. Using this data in conjunction with atmospheric temperature and humidity profiles from local radiosondes, the necessary inputs for an infrared radiative transfer model can be developed. Infrared radiative transfer calculations are performed with a multispectral two-stream model. The model fluxes at the cloud base and at 19 km are then compared with the aircraft observations to determine whether the model is performing well. Cloud layer heating rates can then be computed from the radiation exchange.

Ackerman, Thomas P.↗

Analysis of thermal radiation of a gas-particulate-cloud in a pressurized oxy-coal combustor

Pressurized oxy-combustion (POC) aims to reduce carbon emissions from coal-fired power plants. In the POC process, pulverized coal is burned at elevated pressure in an O2-CO2 environment. The elevated pressure and high CO2 and H2O concentrations strongly impact thermal radiation, thereby significantly distinguishing POC system from conventional atmospheric-pressure air-fired and oxy-fuel combustion. Consequently, a thorough understanding of thermal radiation in POC is required to promote the development of novel combustors. The present computational work analyzes thermal radiation of the gaseous and particle phases in the pilot-scale POC combustor in Washington University in St. Louis. Particularly, the radiation characteristics of the gaseous and particulate cloud were estimated by employing the statistical narrow band model and the large-particle model. It is found that thermal radiation of a particulate cloud dominates in the combustor under the conditions of a furnace temperature of 1500 K and no substantial particle loss. Another important result is that the gas-and-particulate cloud can be approximately treated as a graybody under the same conditions. To be more specific, the results of spectral radiation intensity of a gas comprised of 40% (vol) H2O and 60% CO2 show that when the pressure is increased to 15 bar, and the radiation pathlength to 100 cm, the spectral radiation profile of the gas phase approaches that of a blackbody at the respective temperature. In addition, the emissivity of the particulate cloud has been evaluated as a function of the particle concentration and diameter by means of the large particle model. It is shown that the emissivity grows with the particle concentration but decreases with the particle size for the same mass of a particulate cloud. The emissivity of a particulate cloud in oxy- combustion exceeds that in air-fired combustion. This work could be used to validate the assumption of the gray gas model adopted in numerical simulations.

Li, Lei↗

4-8 micron spectrophotometry of OH 0739-14

Spectrophotometry of the dust-embedded late-type star OH 0739-14 shows an absorption feature at 6.0 microns characteristic of H2O ice at temperatures significantly lower than 150 K, confirming the identification of H2O ice in the circumstellar shell in this source. The differences in the infrared spectra of HO 0739-14 and embedded molecular cloud sources are attributed to the different cloud lifetimes and temperature regimes in which the molecules are formed. A lower limit to the mass loss rate of 0.0001 solar mass per year is derived, based on the column density of ice and the size and the expansion velocity of the circumstellar cloud.

Soifer, B. T.↗