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All sourcesNASA NTRSDOE OSTI
DOE OSTI2026

Examining the Impacts of Microphysical-Dynamical Feedbacks on Convective Clouds in Different Aerosol Environments Using Enhanced Observational and Modeling Strategies

This project investigated how microphysical–dynamical feedbacks influence deep convective clouds across a range of aerosol conditions, storm lifecycles, and meteorological regimes, and how these sensitivities depend on the modeling framework used to represent convection and microphysics. Using the Aerosol, Cloud, Precipitation, and Climate (ACPC) Working Group model intercomparison simulations of isolated deep convection in the Houston region, we found a robust warm-phase aerosol response in most cloud-resolving models. Increased aerosol loading tended to suppress warm-rain production, increase cloud water, and reduce surface rainfall and near-surface evaporation. These impacts were typically strongest early in the convective lifecycle, with the largest aerosol-driven differences occurring during the first half of storm evolution. The ice-phase response, on the other hand, varied widely across modeling frameworks, and differed in sign, timing, and vertical structure. Ice microphysical pathways and parameterizations are therefore leading sources of uncertainty in aerosol–deep convection interactions. Theoretical analyses further suggested that aerosol-driven invigoration through cold-phase processes was much weaker than previously hypothesized for cold-based storms, and in warm-based storms could even reduce updraft strength. These results imply that any invigoration signal is more likely linked to warm-phase processes and peaks early in storm development.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1972

The Nimbus 4 infrared spectroscopy experiment. I - Calibrated thermal emission spectra.

Measurement of the infrared spectrum of the earth and atmosphere between 400 and 1600/cm. In an effort to obtain spectra with high absolute accuracy, it was necessary to incorporate many factors into the calibration, including small departures from unity in the emissivity of the on-board calibration source, imbalance between cold and warm calibration ports, and effects due to orbital variations in instrument temperature. The inclusion of such higher order corrections, along with careful data screening processes, has ensured a high quality data set that can be used in a variety of geophysical and meteorological investigations. Representative samples of data are presented that illustrate the behavior of the thermal emission spectra under a variety of conditions encountered in a typical orbit, including extremes in temperature, surface reststrahlung (or residual ray) effects, and various types of cloud conditions.

Hanel, R. A.↗
NASA NTRS1984

Remote sensing of air-sea interactions

A number of preliminary concepts for the measurement or inference of fluxes across the air-sea interface through remote sensing are proposed. All the methods are achievable from aircraft with state-of-the-art technology. Only one is now ready for space implementation. The focus is on cold outbreaks. Sensible (latent) heat flux is inferred from the difference between initial surface air temperature (vapor mixing ratio) and the downwind SST (and corresponding saturation mixing ratio). The downwind growth rate of the PBL as measured by lidar also provides estimates of surface heating and the cross-inversion entrainment velocity. The lidar also provides a measure of the depth of the inversion and its penetration by surface-forced convection; this permits estimates of the surface heat flux. Lidar and radiometric measurements of cloud top height and temperature provide means of deducing the temperature sounding downstream so that heating is computed with the aid of a known sounding upstream.

Atlas, D.↗
NASA NTRS1991

Detection of the greenhouse gas signal from space - A progress report

The spatial distribution of the expected changes in the atmospheric water vapor content and cloud cover, as predicted by the transient greenhouse gas (GHG) simulation of Hansen et al. (1988), are examined to determine whether the signals would be large enough and unique enough to be useful in a GHG detection study. The nature of the predicted GHG signal was first examined using the transient CO2 run from the GISS ocean/atmosphere general circulation model. Next, the remotely sensed irradiance characteristics data (as the measure of water vapor content) supplied by the HIRS/MSU sensors for the area of the equatorial cold tongue region (the region in which there are no measurement stations). It is shown that HIRS/MSU signals can provide data necessary for detecting GHS signals in atmospheric moisture for regions where ground observations are not possible.

Barnett, T. P.↗
NASA NTRS2002

Macroscopic Relationships among Latent Heating, Precipitation, Organized Convection and the Environment

Three-dimensional Cloud Resolving Model (CRM) simulations were conducted to examine the squall line observed on 26 January, 1999 from the Tropical Rainfall Measuring Mission Large Scale Biosphere Atmosphere Experiment in Amazonia (TRMM-LBA) field campaign. The computational domain was 600 kilometers x 180 kilometers x 20 kilometers with a horizontal resolution of 1 kilometer and a vertical resolution of 200 meters. The CRM was initialized from the Abracos Hill and Rebio soundings. Convection was initiated by a surface-based and NW-SE oriented cold pool over a region 60 kilometers in the y-direction and 30 kilometers wide in the x-direction. The cold pool temperature perturbation is a maximum of -6K at the surface, decreasing linearly to zero at 3 kilometers. The simulated convection is in the form of a NW-SE band that moves toward the southwest at a speed of 8 meters per second, and is generally comparable to radar observations.

Moncrieff, Mitchell W.↗
NASA NTRS2010

Detailed Structure of the Tropical Upper Troposphere and Lower Stratosphere as Revealed by Balloon Sonde Observations of Water Vapor, Ozone, Temperature, and Winds During the NASA TCSP and TC4 Campaigns

We report on balloon sonde measurements of water vapor and ozone using the cryogenic frost point hygrometer and electrochemical concentration cell ozonesondes made at Alajuela, Costa Rica (10.0 N, 84.2 W) during two NASA airborne campaigns: the Tropical Convective Systems and Processes (TCSP) mission in July 2005 and the Tropical Composition, Clouds, and Climate Coupling Experiment (TC4), July - August 2007. In both campaigns we found an upper troposphere that was frequently supersaturated but no evidence that deep convection had reached the tropopause. The balloon sondes were complemented by campaigns of 4 times daily high-resolution radiosondes from mid-June through mid-August in both years. The radiosonde data reveal vertically propagating equatorial waves that caused a large increase in the variability of temperature in the tropical tropopause layer (TTL). These waves episodically produced cold point tropopauses (CPTs) above 18 km, yet in neither campaign was saturation observed above approx 380 K or 17 km. The averages of the water vapor minima below this level were 5.2 ppmv in TCSP and 4.8 ppmv in TC4, and the individual profile minima all lay at or above approx 360 K. The average minima in this 360 C380 K layer provide a better estimate of the effective stratospheric entry value than the average mixing ratio at the CPT. We refer to this upper portion of the TTL as the tropopause saturation layer and consider it to be the locus of the final dehydration of nascent stratospheric air. As such, it is the local equivalent to the tape head of the water vapor tape recorder.

Selkirk, Henry B.↗
NASA NTRS2010

Layered Model for Radiation-Induced Chemical Evolution of Icy Surface Composition on Kuiper Belt and Oort Cloud Bodies

The diversity of albedos and surface colors on observed Kuiper Belt and Inner Oort Cloud objects remains to be explained in terms of competition between primordial intrinsic versus exogenic drivers of surface and near-surface evolution. Earlier models have attempted without success to attribute this diversity to the relations between surface radiolysis from cosmic ray irradiation and gardening by meteoritic impacts. A more flexible approach considers the different depth-dependent radiation profiles produced by low-energy plasma, suprathermal, and maximally penetrating charged particles of the heliospheric and local interstellar radiation environments. Generally red objects of the dynamically cold (low inclination, circular orbit) Classical Kuiper Belt might be accounted for from erosive effects of plasma ions and reddening effects of high energy cosmic ray ions, while suprathermal keV-MeV ions could alternatively produce more color neutral surfaces. The deepest layer of more pristine ice can be brought to the surface from meter to kilometer depths by larger impact events and potentially by cryovolcanic activity. The bright surfaces of some larger objects, e.g. Eris, suggest ongoing resurfacing activity. Interactions of surface irradiation, resultant chemical oxidation, and near-surface cryogenic fluid reservoirs have been proposed to account for Enceladus cryovolcanism and may have further applications to other icy irradiated bodies. The diversity of causative processes must be understood to account for observationally apparent diversities of the object surfaces.

Cooper, John F.↗
NASA NTRS2010

Layered Model for Radiation-Induced Chemical Evolution of Icy Surface Composition and Dynamics on Kuiper Belt and Oort Cloud Bodies

The diversity of albedos and surface colors on observed Kuiper Belt and Inner Oort Cloud objects remains to be explained in terms of competition between primordial intrinsic versus exogenic drivers of surface and near-surface evolution. Earlier models have attempted without success to attribute this diversity to the relations between surface radiolysis from cosmic ray irradiation and gardening by meteoritic impacts. A more flexible approach considers the different depth-dependent radiation profiles produced by low-energy plasma, suprathermal, and maximally penetrating charged particles of the heliospheric and local interstellar radiation environment. Generally red objects of the dynamically cold (low inclination, circular orbit) Classical Kuiper Belt might be accounted for from erosive effects of plasma ions and reddening effects of high energy cosmic ray ions, while suprathermal keV-MeV ions could alternatively produce more color neutral surfaces. The deepest layer of more pristine ice can be brought to the surface from meter to kilometer depths by larger impact events and potentially by cryovolcanic activity. The bright surfaces of some larger objects, e.g. Eris, suggest ongoing resurfacing activity. Cycles of atmospheric formation and surface freezeout can further account for temporal variation as observed on Pluto. The diversity of causative processes must therefore be understood to account for observationally apparent diversities of the object surfaces.

Cooper, John F.↗
DOE OSTI2020

Stellar population models based on the SDSS-IV MaStar library of stellar spectra – I. Intermediate-age/old models

ABSTRACT We use the first release of the SDSS/MaStar stellar library comprising ∼9000, high S/N spectra, to calculate integrated spectra of stellar population models. The models extend over the wavelength range 0.36–1.03 µm and share the same spectral resolution ($R\sim 1800$) and flux calibration as the SDSS-IV/MaNGA galaxy data. The parameter space covered by the stellar spectra collected thus far allows the calculation of models with ages and chemical composition in the range $\rm {\mathit{ t}\gt 200 \,Myr, -2 \lt = [Z/H] \lt = + 0.35}$, which will be extended as MaStar proceeds. Notably, the models include spectra for dwarf main-sequence stars close to the core H-burning limit, as well as spectra for cold, metal-rich giants. Both stellar types are crucial for modelling λ > 0.7 µm absorption spectra. Moreover, a better parameter coverage at low metallicity allows the calculation of models as young as 500 Myr and the full account of the blue horizontal branch phase of old populations. We present models adopting two independent sets of stellar parameters (Teff, log g, [Z/H]). In a novel approach, their reliability is tested ‘on the fly’ using the stellar population models themselves. We perform tests with Milky Way and Magellanic Clouds globular clusters, finding that the new models recover their ages and metallicities remarkably well, with systematics as low as a few per cent for homogeneous calibration sets. We also fit a MaNGA galaxy spectrum, finding residuals of the order of a few per cent comparable to the state-of-art models, but now over a wider wavelength range.

Maraston, C.↗
NASA NTRS1994

Physical Retrievals of Over-Ocean Rain Rate from Multichannel Microwave Imagery: Theoretical Characteristics of Normalized Polarization and Scattering Indices - Part 1

Microwave rain rate retrieval algorithms have most often been formulated in terms of the raw brightness temperatures observed by one or more channels of a satellite radiometer. Taken individually, single-channel brightness temperatures generally represent a near-arbitrary combination of positive contributions due to liquid water emission and negative contributions due to scattering by ice and/or visibility of the radiometrically cold ocean surface. Unfortunately, for a given rain rate, emission by liquid water below the freezing level and scattering by ice particles above the freezing level are rather loosely coupled in both a physical and statistical sense. Furthermore, microwave brightness temperatures may vary significantly (approx. 30-70 K) in response to geophysical parameters other than liquid water and precipitation. Because of these complications, physical algorithms which attempt to directly invert observed brightness temperatures have typically relied on the iterative adjustment of detailed micro-physical profiles or cloud models, guided by explicit forward microwave radiative transfer calculations. In support of an effort to develop a significantly simpler and more efficient inversion-type rain rate algorithm, the physical information content of two linear transformations of single-frequency, dual-polarization brightness temperatures is studied: the normalized polarization difference P of Petty and Katsaros (1990, 1992), which is intended as a measure of footprint-averaged rain cloud transmittance for a given frequency; and a scattering index S (similar to the polarization corrected temperature of Spencer et al.,1989) which is sensitive almost exclusively to ice. A reverse Monte Carlo radiative transfer model is used to elucidate the qualitative response of these physically distinct single-frequency indices to idealized 3-dimensional rain clouds and to demonstrate their advantages over raw brightness temperatures both as stand-alone indices of precipitation activity and as primary variables in physical, multichannel rain rate retrieval schemes. As a byproduct of the present analysis, it is shown that conventional plane-parallel analyses of the well-known foot-print-filling problem for emission-based algorithms may in some cases give seriously misleading results.

Petty, G. W.↗
NASA NTRS2021

Influence of the Saharan Air Layer on Hurricane Nadine (2012). Part I: Observations from the Hurricane and Severe Storm Sentinel (HS3) Investigation and Modeling Results

This study uses a model with aerosol–cloud–radiation coupling to examine the impact of Saharan dust and other aerosols on Hurricane Nadine (2012). To study aerosol direct (radiation) and indirect (cloud microphysics) effects from individual, as well as all aerosol species, eight different NU-WRF Model simulations were conducted. In several simulations, aerosols led to storm strengthening, followed by weakening relative to the control simulation. This variability of the aerosol impact may be related to whether aerosols are ingested into clouds within the outer rainbands or the eyewall. Upper-tropospheric aerosol concentrations indicate vertical transport of all aerosol types in the outer bands but only vertical transport of sea salt in the inner core. The results suggest that aerosols, particularly sea salt, may have contributed to a stronger initial intensification but that aerosol ingestion into the outer bands at later times may have weakened the storm in the longer term. In most aerosol experiments, aerosols led to a reduction in cloud and precipitation hydrometeors, the exception being the dust-only case that produced periods of enhanced hydrometeor growth. The Saharan air layer (SAL) also impacted Nadine by causing a region of strong easterlies impinging on the eastern side of the storm. At the leading edge of these easterlies, cool and dry air near the top of the SAL was being ingested into the outer-band convection. This midlevel low-equivalent-potential-temperature air gradually lowered toward the surface and eventually contributed to significant cold-pool activity in the eastern rainband and in the northeast quadrant of the storm. Such enhanced downdraft activity could have led to weakening of the storm, but it is not presently possible to quantify this impact.

Jainn J. Shi↗
DOE OSTI2022

Evaluating seasonal and regional distribution of snowfall in regional climate model simulations in the Arctic

In this study, we investigate how the regional climate model HIRHAM5 reproduces the spatial and temporal distribution of Arctic snowfall when compared to CloudSat satellite observations during the examined period of 2007–2010. For this purpose, both approaches, i.e., the assessments of the surface snowfall rate (observation-to-model) and the radar reflectivity factor profiles (model-to-observation), are carried out considering spatial and temporal sampling differences. The HIRHAM5 model, which is constrained in its synoptic representation by nudging to ERA-Interim, represents the snowfall in the Arctic region well in comparison to CloudSat products. The spatial distribution of the snowfall patterns is similar in both identifying the southeastern coast of Greenland and the North Atlantic corridor as regions gaining more than twice as much snowfall as the Arctic average, defined here for latitudes between 66 and 81°N. Excellent agreement (difference less than 1%) in the Arctic-averaged annual snowfall rate between HIRHAM5 and CloudSat is found, whereas ERA-Interim reanalysis shows an underestimation of 45% and significant deficits in the representation of the snowfall rate distribution. From the spatial analysis, it can be seen that the largest differences in the mean annual snowfall rates are an overestimation near the coastlines of Greenland and other regions with large orographic variations as well as an underestimation in the northern North Atlantic Ocean. To a large extent, the differences can be explained by clutter contamination, blind zone or higher resolution of CloudSat measurements, but clearly HIRHAM5 overestimates the orographic-driven precipitation. The underestimation of HIRHAM5 within the North Atlantic corridor south of Svalbard is likely connected to a poor description of the marine cold air outbreaks which could be identified by separating snowfall into different circulation weather type regimes. By simulating the radar reflectivity factor profiles from HIRHAM5 utilizing the Passive and Active Microwave TRAnsfer (PAMTRA) forward-modeling operator, the contribution of individual hydrometeor types can be assessed. Looking at a latitude band at 72–73°N, snow can be identified as the hydrometeor type dominating radar reflectivity factor values across all seasons. The largest differences between the observed and simulated reflectivity factor values are related to the contribution of cloud ice particles, which is underestimated in the model, most likely due to the small sizes of the particles. The model-to-observation approach offers a promising diagnostic when improving cloud schemes, as illustrated by comparison of different schemes available for HIRHAM5.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS2012

Global Estimates of PBL Depth from Space-Borne LIDAR

The planetary boundary layer (PBL) is responsible for communicating the exchange of energy, moisture, momentum, pollutants, and aerosols between the surface and the free atmosphere and is therefore crucial to many studies of the atmosphere. Unfortunately, there have historically been few observations of this important layer due to the complexity involved in its measurement. However, with the advent of more advanced satellites, global measurements of the PBL are now becoming possible. The PBL is often characterized by a high concentration of aerosols within the layer and low level clouds capping it and these are observable from space. The Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) satellite was launched in 2006 with the intention of observing aerosols and clouds and was the first space-based LIDAR optimized for this purpose. CALIPSO observations are therefore well suited to observing the depth of the PBL. Since it was launched, CALIPSO has been making nearly continuous measurements enabling a global picture of PBL depth. We plan to present a global PBL depth product and how it evolves throughout the year. The product is able to identify deeper PBL depths in the summer hemisphere over land and deeper depths along the northern hemisphere oceanic storm tracks in winter associated with cold air traveling over warm water. Large seasonal cycles are also evident in the subtropical desert locations among other features. In addition, comparisons will be made between several estimates of PBL depth based on turbulent intensity, meteorology profiles, and aerosol profiles from the GEOS5 model.

McGrath-Spangler, Erica lynn↗
DOE OSTI2024

Scale-Up Studies for the Dehydration of C 4+ Alcohols into Drop-In Diesel Fuel

Herein, we demonstrate the production of liter quantities of drop-in diesel-range ethers from biomass-derived alcohols. We report scale-up resultsfor the dehydration of a mixture of C 4+ alcohols using powder and pellet zeolite Ycatalyst in continuous flow and batch reactors. The activity of zeolite Y decreaseswith the introduction of an alumina binder. Large alcohols, as well as branchedand secondary alcohols, increase the coke content over the pellet Y catalyst. Thepellet formulation had lower carbon balances and selectivity to C 10+ ethers,suggesting that the pellet formulation increases alcohol absorption and cokeproduction. Crushing the pellet Y catalyst to smaller particle sizes does notrecover the activity of zeolite Y in its powder form. Cold flow experiments showthat particle agglomeration contributes to pressure buildup in the continuous flowreactor. C 10+ ether blends can be produced in batch reactors at high alcohol conversion regimes. One liter of a diesel #2 blend wasproduced by scaling up this reaction. The final blend consists of a substantial portion of C 10+ ethers (63.7 wt %), followed by heavyunknown products (27.4 wt %). Furthermore, the final alcohol and butyl ether concentration values were 7.3 and 1.5 wt %, respectively. Theblendstock reported in this paper can satisfy diesel #2 ASTM standards for density, cloud point, flashpoint, and cetane number.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS1991

Research aircraft observations of the mesoscale and microscale structure of a cold front over the eastern Pacific Ocean

The structure of an oceanic cold front is described on the basis of research aircraft observations taken during the Ocean Storms field experiment. Synoptic and mesoscale analyses compare the structure of an upper-level jet-front system observed slightly downstream from the wind speed maximum to its structure in the upstream entrance region. Stratospheric potential vorticity and ozone were found within the frontal zone down to about 800 mb. Microscale analyses of the front near the sea surface were carried out for a portion of the front having the signature of a 'rope' cloud in satellite imagery. A narrow (less than 1 km) zone of upward motion (about 4 m/s) and of horizontal shear (about 0.01/s) characterized the front near the surface. Significant alongfront variability was found, including lateral displacements in the frontal zone where there were weaker updrafts.

Bond, Nicholas A.↗
NASA NTRS1993

Gas-grain energy transfer in solar nebula shock waves: Implications for the origin of chondrules

Meteoritic chondrules provide evidence for the occurrence of rapid transient heating events in the protoplanetary nebula. Astronomical evidence suggests that gas dynamic shock waves are likely to be excited in protostellar accretion disks by processes such as protosolar mass ejections, nonaxisymmetric structures in an evolving disk, and impact on the nebula surface of infalling 'clumps' of circumstellar gas. Previous detailed calculations of gas-grain energy and momentum transfer have supported the possibility that such shock waves could have melted pre-existing chondrule-sized grains. The main requirement for grains to reach melting temperatures in shock waves with plausibly low Mach numbers is that grains existed in dust-rich zones (optical depth greater than 1) where radiative cooling of a given grain can be nearly balanced by radiation from surrounding grains. Localized dust-rich zones also provide a means of explaining the apparent small spatial scale of heating events. For example, the scale size of at least some optically thick dust-rich zones must have been relatively small (less than 10 kilometers) to be consistent with petrologic evidence for accretion of hot material onto cold chondrules. The implied number density of mm-sized grains for these zones would be greater than 30 m(exp -3). In this paper, we make several improvements of our earlier calculations to include radiation self-consistently in the shock jump conditions, and we include heating of grains due to radiation from the shocked gas. In addition, we estimate the importance of momentum feedback of dust concentrations onto the shocked gas which would tend to reduce the efficiency of gas dynamic heating of grains in the center of the dust cloud.

Hood, L. L.↗
DOE OSTI2021

Quantum Enhanced Cavity QED Interferometer with Partially Delocalized Atoms in Lattices

Herein, we propose a quantum enhanced interferometric protocol for gravimetry and force sensing using cold atoms in an optical lattice supported by a standing-wave cavity. By loading the atoms in partially delocalized Wannier-Stark states, it is possible to cancel the undesirable inhomogeneities arising from the mismatch between the lattice and cavity fields and to generate spin squeezed states via a uniform one-axis twisting model. The quantum enhanced sensitivity of the states is combined with the subsequent application of a compound pulse sequence that allows us to separate atoms by several lattice sites. This, together with the capability to load small atomic clouds in the lattice at micrometric distances from a surface, make our setup ideal for sensing short-range forces. We show that for arrays of 10 4 atoms, our protocol can reduce the required averaging time by a factor of 10 compared to unentangled lattice-based interferometers after accounting for primary sources of decoherence.

74 ATOMIC AND MOLECULAR PHYSICS↗
NASA NTRS2003

Molecular Carbon in the Galaxy: Laboratory and Observational Studies

In a collaboration with the Mats Larsson group from Stockholm, we carried out a new measurement of the rate of dissociative recombination of H(sup *, sub j), using a new pulsed supersonic beam source of rotationally cold H(sup *, sub j). This source was first designed and characterized in our lab by IR cavity ringdown spectroscopy, determining a rotationaYtranslationa1 temperature of 20-60K, depending on conditions. This new source was then taken to Stockholm for the recombination rate studies at the CRYRING storage ring. The recombination rate constant measured against temperature yields values consistent with the most recent calculations, whereas previous experimental measurements varied over a range of 10(exp 4) and were poor agreement with theory. This is a crucial achievement for understanding the ion chemistry of diffuse clouds. Moreover, this result in combination with recent observations implies a greatly enhanced (factor of 40) cosmic ray ionization rate in a diffuse cloud (zeta Persei) relative to previous studies. The implications of this are discussed in our recent Nature paper. An enhanced cosmic-ray flux towards zeta Persei inferred from a laboratory study of the H(sup *, sub j)-e(sup -) recombination rate.

Saykally, Richard James↗