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NASA NTRS2020

Black Carbon and Precipitation: an Energetics Perspective

Black carbon aerosols (BC) influence precipitation through a range of processes. The climate response to the presence of BC is however highly dependent on its vertical distribution. Here, we analyze the changes in the energy budget and precipitation impacts of adding a layer of BC at a range of altitudes in two independent global climate models. The models are run with atmosphere‐only and slab ocean model setup to analyze both fast and slow responses, respectively. Globally, precipitation changes are tightly coupled to the energy budget. We decompose the precipitation change into contributions from absorption of solar radiation, atmospheric longwave radiative cooling, and sensible heat flux at the surface. We find that for atmosphere‐only simulations, BC rapidly suppress precipitation, independent of altitude, mainly because of strong atmospheric absorption. This reduction is offset by increased atmospheric radiative longwave cooling and reduced sensible heat flux at the surface, but not of sufficient magnitude to prevent reduced precipitation. On longer timescales, when the surface temperature is allowed to respond, we find that the precipitation increase associated with surface warming can compensate for the initial reduction, particularly for BC in the lower atmosphere. Even though the underlying processes are strikingly similar in the two models, the resulting change in precipitation and temperature by BC differ quite substantially.

black carbon aerosols↗

NASA NTRS1996

A High Spectral Resolution Lidar Based on Absorption Filter

A High Spectral Resolution Lidar (HSRL) that uses an iodine absorption filter and a tunable, narrow bandwidth Nd:YAG laser is demonstrated. The iodine absorption filter provides better performance than the Fabry-Perot etalon that it replaces. This study presents an instrument design that can be used a the basis for a design of a simple and robust lidar for the measurement of the optical properties of the atmosphere. The HSRL provides calibrated measurements of the optical properties of the atmospheric aerosols. These observations include measurements of aerosol backscatter cross sections, optical depth, backscatter phase function depolarization, and multiple scattering. The errors in the HSRL data are discussed and the effects of different errors on the measured optical parameters are shown.

Piironen, Paivi↗

NASA NTRS1999

Remote Sensing of Volcanic Clouds: Sulfur Gases and Plume Top Topography

New absorption line parameters for H2S were published and submitted to the Gestion et Etude des Informations Spectroscopiques Atmospheriques (GEISA) and high resolution transmission molecular absorption (HITRAN) databases. These new absorption line parameters will make it possible to use observations from the future Tropospheric Emission Spectrometer (TES) instrument [Earth Observing System (EOS) Chemistry Mission (CHEM) platform] to make more accurate H2S measurements if it observes an H2S-rich volcanic cloud. H2S is the second most abundant volcanic sulfur gas, and like SO2, it also converts to H2SO4 aerosols and can have a climate impact. A paper on the Moderate-resolution Imaging-Spectroradiometer (MODIS) SO2 alert is being revised. New aspects in the revision include verification of the SO2 alert during the EOS mission; factors affecting SO2 detection at thermal infrared, ultraviolet, and microwave wavelengths; radiative transfer tests; more description of satellite instruments; and thermal surface alert installed for MODIS. Her research involves the use of remote sensing to generate maps of plume top altitude. This parameter is important for models of volcanic eruption, aircraft hazards, and climate impact. The topographic shape of the top surface of a volcanic plume can provide information necessary to understand the physics controlling the injection and dispersal of a volcanic plume in the atmosphere. Glaze et al. describe the application of a photoclinometric technique to volcanic plumes. The software algorithm has been improved to account for more general plume and illumination geometries and for easily extracting position information directly from Advanced Very High-Resolution Radiometer (AVHRR) level 1B data. Testing of the algorithm has focused on acquiring AVHRR data for a variety of volcanic plumes in an effort to identify problems with the software as well as model sensitivities. The plumes chosen were erupted from volcanoes at a variety of latitudes, at different times of day, and in different seasons. Another important issue that is being investigated is the importance of plume opacity. A diagram illustrates the method for deriving phi, the angle a wind-blown plume makes with the horizontal, in the direction perpendicular to the remote sensing scan. A figure shows a sample output of the algorithm, a wire mesh map of plume top topography. Additional information is contained in the original.

Crisp, Joy A.↗

NASA NTRS2012

A Miniaturized Laser Heterodyne Radiometer for a Global Ground-Based Column Carbon Monitoring Network

We present progress in the development of a passive, miniaturized Laser Heterodyne Radiometer (mini-LHR) that will measure key greenhouse gases (C02, CH4, CO) in the atmospheric column as well as their respective altitude profiles, and O2 for a measure of atmospheric pressure. Laser heterodyne radiometry is a spectroscopic method that borrows from radio receiver technology. In this technique, a weak incoming signal containing information of interest is mixed with a stronger signal (local oscillator) at a nearby frequency. In this case, the weak signal is sunlight that has undergone absorption by a trace gas of interest and the local oscillator is a distributive feedback (DFB) laser that is tuned to a wavelength near the absorption feature of the trace gas. Mixing the sunlight with the laser light, in a fast photoreceiver, results in a beat signal in the RF. The amplitude of the beat signal tracks the concentration of the trace gas in the atmospheric column. The mini-LHR operates in tandem with AERONET, a global network of more than 450 aerosol sensing instruments. This partnership simplifies the instrument design and provides an established global network into which the mini-LHR can rapidly expand. This network offers coverage in key arctic regions (not covered by OCO-2) where accelerated warming due to the release of CO2 and CH4 from thawing tundra and permafrost is a concern as well as an uninterrupted data record that will both bridge gaps in data sets and offer validation for key flight missions such as OCO-2, OCO-3, and ASCENDS. Currently, the only ground global network that routinely measures multiple greenhouse gases in the atmospheric column is TCCON (Total Column Carbon Observing Network) with 18 operational sites worldwide and two in the US. Cost and size of TCCON installations will limit the potential for expansion, We offer a low-cost $30Klunit) solution to supplement these measurements with the added benefit of an established aerosol optical depth measurement. Aerosols induce a radiative effect that is an important modulator of regional carbon cycles. Changes in the diffuse radiative flux fraction (DRF) due to aerosol loading have the potential to alter the terrestrial carbon exchange.

Wilson, Emily L.↗

NASA NTRS1997

Absorption and scattering properties of the Martian dust in the solar wavelengths

A new wavelength-dependent model of the single-scattering properties of the Martian dust is presented. The model encompasses the solar wavelengths (0.3 to 4.3 micrometers at 0.02 micrometer resolution) and does not assume a particular mineralogical composition of the particles. We use the particle size distribution, shape, and single-scattering properties at Viking Lander wavelengths presented by Pollack et al. [1995]. We expand the wavelength range of the aerosol model by assuming that the atmospheric dust complex index of refraction is the same as that of dust particles in the bright surface geologic units. The new wavelength-dependent model is compared to observations taken by the Viking Orbiter Infrared Thermal Mapper solar channel instrument during two dust storms. The model accurately matches afternoon observations and some morning observations. Some of the early morning observations are much brighter than the model results. The increased reflectance can be ascribed to the formation of a water ice shell around the dust particles, thus creating the water ice clouds which Colburn et al. [1989], among others, have predicted.

Atmosphere/analysis↗

NASA NTRS2000

BOREAS RSS-3 Atmospheric Measurements from a Helicopter-Mounted Sunphotometer

The BOREAS RSS-3 team collected and processed helicopter-based measurements of atmospheric conditions to estimates of aerosol optical thickness and atmospheric water vapor. The automatic sun-tracking photometer for helicopters was deployed during all three 1994 IFCs at numerous tower and auxiliary sites in both the NSA and the SSA. Six spectral channels (440, 540, 613, 670, 870, and 1030 nm) were chosen to span the visible and NIR wavelengths and to avoid gaseous absorption. One additional channel, 940 nm, was selected to measure the water column abundance above the helicopter platform. The data are stored in tabular ASCII files.

Hall, Forrest G.↗

NASA NTRS2009

Differential Absorption Lidar to Measure Sub-Hourly Variation of Tropospheric Ozone Profiles

A tropospheric ozone Differential Absorption Lidar (DIAL) system, developed jointly by the University of Alabama at Huntsville and NASA, is making regular observations of ozone vertical distributions between 1 and 8 km with two receivers under both daytime and nighttime conditions using lasers at 285 and 291 nm. This paper describes the lidar system and analysis technique with some measurement examples. An iterative aerosol correction procedure reduces the retrieval error arising from differential aerosol backscatter in the lower troposphere. Lidar observations with coincident ozonesonde flights demonstrate that the retrieval accuracy ranges from better than 10% below 4 km to better than 20% below 8 km with 750-m vertical resolution and 10-min temporal integration

Kuang, Shi↗

NASA NTRS2016

Giant Planets in Reflected Light: What Science Can We Expect?

Interpreting the reflection spectra of cool giant planets will be a challenge. Spectra of such worlds are expected to be primarily shaped by scattering from clouds and hazes and punctuated by absorption bands of methane, water, and ammonia. While the warmest giants may be cloudless, their atmospheres will almost certainly sport substantial photochemical hazes. Furthermore the masses of most direct imaging targets will be constrained by radial velocity observations, their radii, and thus atmospheric gravity, will be imperfectly known. The uncertainty in planet radius and gravity will compound with uncertain aerosol properties to make estimation of key absorber abundances difficult. To address such concerns our group is developing atmospheric retrieval tools to constrain quantities of interest, particular gas mixing ratios. We have applied our Markov Chain Monte Carlo methods to simulated data of the quality expected from the WFIRST CGI instrument and found that given sufficiently high SNR data we can confidentially identify and constrain the abundance of methane, cloud top pressures, gravity, and the star-planet-observer phase angle. In my presentation I will explain the expected characteristics of cool extrasolar giant planet reflection spectra, discuss these and other challenges in their interpretation, and summarize the science results we can expect from direct imaging observations.

methane↗

NASA NTRSDate not supplied

Coupling of Dust Mineralogy to Radiation in NASA GISS ModelE: Impact Upon Dust Optical Properties and Direct Radiative Effect

Estimates of dust direct radiative effect (DRE) are still largely uncertain mainly due to the poor constraining of regional variations of dust absorption, whose known connection with mineral composition is still largely neglected by most Earth System Models. The inaccurate knowledge of soil mineralogy and insufficient measurements of dust physical and optical properties still present the main challenges for a proper representation of the dust-radiation interaction in climate models. We recently upgraded the coupling of dust minerals to shortwave radiation in the NASA GISS ModelE. In particular, we extended the interaction to online-calculated minerals and implemented two different mixing configurations: i) external mixing of three main mineral components and ii) internal mixing of all minerals, allowing a dynamic fraction of iron oxides. We used a semi-empirical approach for the optical calculations, mostly based on aerosol chamber measurements from natural soils, aiming to reduce the influence of uncertain assumptions on the optical properties and mixing state of individual minerals. In this contribution, we present the results of our first calculations of dust optical properties and DREs based on different mixing configurations of interactive minerals. We show the changes to dust optical depth and single scattering albedo, with respect to the control case using homogeneous dust composition, and the consequent global and regional variations in dust DREs at the top of atmosphere and at surface. We also compare the model optical properties with AERONET data, filtered to identify dust scenes. We find that accounting for the diverse properties of dust minerals modifies the pattern of regional dust absorption and therefore its impact upon climate. We also show that the mineralogy effect is sensitive to the assumed mixing state of minerals.

dust direct radiative effect↗

NASA NTRS2010

Pulsed Airborne Lidar Measurements of Atmospheric CO2 Column Absorption and Line Shapes from 3-13 km Altitudes

We have developed a pulsed lidar technique for measuring the tropospheric CO2 concentrations as a candidate for NASA's planned ASCENDS space mission. Our technique uses two pulsed laser transmitters allowing simultaneous measurement of a CO2 absorption line in the 1570 nm band, O2 extinction in the Oxygen A-band and surface height and backscatter. The lidar measures the energy and time of flight of the laser echoes reflected from the atmosphere and surface. The lasers are rapidly and precisely stepped in wavelength across the CO2 line and an O2 line region during the measurement. The direct detection receiver uses a telescope and photon counting detectors, and measures the background light and energies of the laser echoes from the surface along with scattering from any aerosols in the path. The gas extinction and column densities for the CO2 and O2 gases are estimated from the ratio of the on- and off- line signals via the DIAL technique. Time gating is used to isolate the laser echo signals from the surface, and to reject laser photons scattered in the atmosphere. The time of flight of the laser pulses are also used to estimate the height of the scattering surface and to identify cases of mixed cloud and ground scattering. We have developed an airborne lidar to demonstrate the CO2 measurement from the NASA Glenn Lear-25 aircraft. The airborne lidar steps the pulsed laser's wavelength across the selected CO2 line with 20 steps per scan. The line scan rate is 450 Hz, the laser pulse widths are 1 usec, and laser pulse energy is 24 uJ. The time resolved laser backscatter is collected by a 20 cm telescope, detected by a photomultiplier and is recorded by a photon counting system. We made initial airborne measurements on flights during fall 2008. Laser backscatter and absorption measurements were made over a variety of land and water surfaces and through thin clouds. The atmospheric CO2 column measurements using the 1572.33 nm CO2 lines. Two flights were made above the US Department of Energy's (DOE) SGP ARM site at altitudes from 3-8 km. These flights were coordinated with DOE investigators who flew an in-situ CO2 sensor on a Cessna aircraft under the path. The increasing CO2 line absorptions with altitudes were evident and comparison with in-situ measurements showed agreements to 6 ppm. In spring 2009 we improved the aircraft's nadir window and during July and August we made 9 additional 2 hour long flights and measured the atmospheric CO2 absorption and line shapes using the 1572.33 nm CO2 line. Measurements were made at stepped altitudes from 3-13 km over a variety of surface types in Nebraska, Illinois, the SGP ARM site, and near and over the Chesapeake Bay in North Carolina and eastern Virginia. Strong laser signals and clear CO2 line shapes were observed at all altitudes, and some measurements were made through thin clouds. The flights over the ARM site were underflown with in-situ measurements made from the DOE Cessna. Analysis shows that the average signal levels follow predicted values, the altimetry measurements had an uncertainty of about 4 m, and that the average optical line depths follow the number density calculated from in-situ sensor readings. The Oklahoma and east coast flights were coordinated with a LaRC/ITT CO2 lidar on the LaRC UC-12 aircraft, a LaRC in-situ CO2 sensor, and the Oklahoma flights also included a JPL CO2 lidar on a Twin Otter aircraft. More details of the flights, measurements, analysis and scaling to space will be described in the presentation.

Abshire, James↗

DOE OSTI2023

Physicochemical characterization of free troposphere and marine boundary layer ice-nucleating particles collected by aircraft in the eastern North Atlantic

Abstract. Atmospheric ice nucleation impacts the hydrological cycle and climate by modifying the radiative properties of clouds. To improve our predictive understanding of ice formation, ambient ice-nucleating particles (INPs) need to be collected and characterized. Measurements of INPs at lower latitudes in a remote marine region are scarce. The Aerosol and Cloud Experiments in the Eastern North Atlantic (ACE-ENA) campaign, in the region of the Azores islands, provided the opportunity to collect particles in the marine boundary layer (MBL) and free troposphere (FT) by aircraft during the campaign's summer and winter intensive operation period. The particle population in samples collected was examined by scanning transmission X-ray microscopy with near-edge X-ray absorption fine structure spectroscopy. The identified INPs were analyzed by scanning electron microscopy with energy-dispersive X-ray analysis. We observed differences in the particle population characteristics in terms of particle diversity, mixing state, and organic volume fraction between seasons, mostly due to dry intrusion events during winter, as well as between the sampling locations of the MBL and FT. These differences are also reflected in the temperature and humidity conditions under which water uptake, immersion freezing (IMF), and deposition ice nucleation (DIN) proceed. Identified INPs reflect typical particle types within the particle population on the samples and include sea salt, sea salt with sulfates, and mineral dust, all associated with organic matter, as well as carbonaceous particles. IMF and DIN kinetics are analyzed with respect to heterogeneous ice nucleation rate coefficients, Jhet, and ice nucleation active site density, ns, as a function of the water criterion Δaw. DIN is also analyzed in terms of contact angles following classical nucleation theory. Derived MBL IMF kinetics agree with previous ACE-ENA ground-site INP measurements. FT particle samples show greater ice nucleation propensity compared to MBL particle samples. This study emphasizes that the types of INPs can vary seasonally and with altitude depending on sampling location, thereby showing different ice nucleation propensities, which is crucial information when representing mixed-phase cloud and cirrus cloud microphysics in models.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2021

Extreme Molecular Complexity Resulting in a Continuum of Carbonaceous Species in Biomass Burning Tar Balls from Wildfire Smoke

Biomass burning emits a wide range of carbonaceous particles into the atmosphere and has negative impacts on human health and the Earth’s radiative balance. Nonvolatile spherical organic aerosol particles, commonly known as tar balls, represent one of the most abundant particles in aged biomass burning smoke. However, the detailed molecular-level composition of ambient tar balls is largely unknown but critical to access their environmental impacts. Ambient aerosol samples collected during a wildfire event, which were ~90% tar balls by number fraction, were analyzed using ultrahigh resolution Orbitrap Elite mass spectrometry with four complementary ionization modes. Our results show the molecular composition of tar balls to be complex, composed of over 10,000 molecular formulas. Model estimated saturation mass concentrations and relative humidity dependent glass transition temperatures were consistent with low volatility and solid morphology as expected for tar balls. Room-temperature evaporation kinetics showed that these particles were composed of ~90% non-volatile species. The molecular complexity detected here signifies a continuum of carbonaceous species, ranging from C3 to C45 with continuous ranges of oxygenation and hydrogen saturation for each Cn. Approximately 24% of molecular formulas were estimated the be highly aromatic, which could indicate chemical compounds with negative health effects, and which may contribute to visible light absorption. The carbon continuum observed here has significant implications for the molecular characterization of atmospheric organic matter. The level of complexity detected here should not be ignored in future studies and we demonstrate that multiple analytical methods may be required to suitably interpret this complexity on a molecular level.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

NASA NTRS1983

Coherent infrared lidar mission and technology needs for measurements of transport and concentration of tropospheric trace species

The science justification and the feasibility of aircraft-based CO2 Doppler lidar measurements of transport between the free troposphere and the stratosphere (or planetary boundary layer) are discussed for a wide range of seasonal and geographic conditions. Ground-based coherent CO2 lidar aerosol scattering experiments using a stable ring resonator (about 50 mJ/pulse) CO2 laser with external injection locking are reported. Comparative studies of injection-locked CO2 laser unstable resonators and master oscillator power amplifiers are reported for future CO2 lidar missions with respect to requirements of pulse energy, duration/shape, frequency chirp, efficiency for heterodyne detection, and combined Doppler lidar and Differential Absorption Lidar missions.

Hess, R. V.↗

NASA NTRSDate not supplied

TPSAS-NF1676L-29194-DND

The Stratospheric Aerosol and Gas Experiment (SAGE) III instrument was deployed on the International Space Station (ISS) in early March 2017. SAGE III/ISS is the latest in the NASA lineage of solar occultation satellite instruments designed to monitor the vertical distribution of aerosol, ozone and other trace gases in the upper atmosphere. Originally built in the early 2000s, the SAGE III/ISS instrument required extensive testing and refurbishment prior to deliver to ISS, including the replacement of the neutral density filter that has been associated with some instrument response issues during the METEOR/3M mission. In particular, METEOR/3M measurements of the oxygen A-band absorption feature near 762 nm that were to be utilized to retrieve profiles of temperature and pressure were adversely affected by this instrument issue. Preliminary examination of the SAGE III/ISS oxygen A-band spectra indicate that the measurements are of higher fidelity than from the METEOR/3M instrument, which may permit successful retrieval of science quality temperature and pressure products. In this paper, we will provide an overview of the temperature and pressure retrieval algorithm, present preliminary analyses of the SAGE III/ISS oxygen A-band measurements, and an initial assessment of the quality of the temperature and pressure retrievals.

Michael Pitts↗

NASA NTRS1992

Observations of height-dependent pressure-perturbation structure of a strong mesoscale gravity wave

Airborne observations using a downward-looking, dual-frequency, near-infrared, differential absorption lidar system provide the first measurements of the height-dependent pressure-perturbation field associated with a strong mesoscale gravity wave. A pressure-perturbation amplitude of 3.5 mb was measured within the lowest 1.6 km of the atmosphere over a 52-km flight line. Corresponding vertical displacements of 250-500 m were inferred from lidar-observed displacement of aerosol layers. Accounting for probable wave orientation, a horizontal wavelength of about 40 km was estimated. Satellite observations reveal wave structure of a comparable scale in concurrent cirrus cloud fields over an extended area. Smaller-scale waves were also observed. Local meteorological soundings are analyzed to confirm the existence of a suitable wave duct. Potential wave-generation mechanisms are examined and discussed. The large pressure-perturbation wave is attributed to rapid amplification or possible wave breaking of a gravity wave as it propagated offshore and interacted with a very stable marine boundary layer capped by a strong shear layer.

Starr, David O'C.↗

NASA NTRS2013

Bounding the Role of Black Carbon in the Climate System: a Scientific Assessment

Black carbon aerosol plays a unique and important role in Earth's climate system. Black carbon is a type of carbonaceous material with a unique combination of physical properties. This assessment provides an evaluation of black-carbon climate forcing that is comprehensive in its inclusion of all known and relevant processes and that is quantitative in providing best estimates and uncertainties of the main forcing terms: direct solar absorption; influence on liquid, mixed phase, and ice clouds; and deposition on snow and ice. These effects are calculated with climate models, but when possible, they are evaluated with both microphysical measurements and field observations. Predominant sources are combustion related, namely, fossil fuels for transportation, solid fuels for industrial and residential uses, and open burning of biomass. Total global emissions of black carbon using bottom-up inventory methods are 7500 Gg/yr in the year 2000 with an uncertainty range of 2000 to 29000. However, global atmospheric absorption attributable to black carbon is too low in many models and should be increased by a factor of almost 3. After this scaling, the best estimate for the industrial-era (1750 to 2005) direct radiative forcing of atmospheric black carbon is +0.71 W/sq m with 90% uncertainty bounds of (+0.08, +1.27)W/sq m. Total direct forcing by all black carbon sources, without subtracting the preindustrial background, is estimated as +0.88 (+0.17, +1.48) W/sq m. Direct radiative forcing alone does not capture important rapid adjustment mechanisms. A framework is described and used for quantifying climate forcings, including rapid adjustments. The best estimate of industrial-era climate forcing of black carbon through all forcing mechanisms, including clouds and cryosphere forcing, is +1.1 W/sq m with 90% uncertainty bounds of +0.17 to +2.1 W/sq m. Thus, there is a very high probability that black carbon emissions, independent of co-emitted species, have a positive forcing and warm the climate. We estimate that black carbon, with a total climate forcing of +1.1 W/sq m, is the second most important human emission in terms of its climate forcing in the present-day atmosphere; only carbon dioxide is estimated to have a greater forcing. Sources that emit black carbon also emit other short-lived species that may either cool or warm climate. Climate forcings from co-emitted species are estimated and used in the framework described herein. When the principal effects of short-lived co-emissions, including cooling agents such as sulfur dioxide, are included in net forcing, energy-related sources (fossil fuel and biofuel) have an industrial-era climate forcing of +0.22 (0.50 to +1.08) W/sq m during the first year after emission. For a few of these sources, such as diesel engines and possibly residential biofuels, warming is strong enough that eliminating all short-lived emissions from these sources would reduce net climate forcing (i.e., produce cooling). When open burning emissions, which emit high levels of organic matter, are included in the total, the best estimate of net industrial-era climate forcing by all short-lived species from black-carbon-rich sources becomes slightly negative (0.06 W/sq m with 90% uncertainty bounds of 1.45 to +1.29 W/sq m). The uncertainties in net climate forcing from black-carbon-rich sources are substantial, largely due to lack of knowledge about cloud interactions with both black carbon and co-emitted organic carbon. In prioritizing potential black-carbon mitigation actions, non-science factors, such as technical feasibility, costs, policy design, and implementation feasibility play important roles. The major sources of black carbon are presently in different stages with regard to the feasibility for near-term mitigation. This assessment, by evaluating the large number and complexity of the associated physical and radiative processes in black-carbon climate forcing, sets a baseline from which to improve future climate forcing estimates.

black carbon↗

NASA NTRS1988

A simple formulation of the delta-four-stream approximation for radiative transfer parameterizations

A systematic development of the delta-four-stream approximation for calculations of radiative fluxes in planetary atmosphere is presented. It is shown that an analytic solution for this approximation can be derived explicitly, with minimum computational effort for flux calculations. Relative accuracy checks for reflection, transmission, and absorption for numerous asymmetry factors, single-scattering albedos, optical depths, and solar zenith angles have been performed with respect to the 'exact' results computed from the adding method for radiative transfer. Overall, results from the delta-four-stream approximation yield relative accuracies within about 5 percent. This approximation is well suited to radiative transfer parameterizations involving flux and heating calculations in aerosol and cloudy atmospheres.

Liou, Kuo-Nan↗

NASA NTRS2000

A Novel High Efficient Laser Transmitter Design for a Space-borne Ozone Differential Lidar (DIAL)

Development of a UV laser transmitter capable of operating from a space platform is a critical step in enabling global earth observations of aerosols and ozone at resolutions greater than current passive instrument capabilities. Tropospheric chemistry is well recognized as the next frontier for global atmospheric measurement. NASA Langley Research Center (LaRC) and the Canadian Space Agency (CSA) have jointly studied the requirements for a satellite based, global ozone monitoring instrument. The study, called Ozone Research using Advanced Cooperative Lidar Experiment (ORACLE) has defined the Differential Absorption Lidar (DIAL) instrument performance, weight and power, and configuration requirements for a space based measurement. In order to achieve the measurement resolution and acceptable signal-to-noise from lidar returns, 500mJ/pulse (5 Watts average power) is required at both 305-308nm and 315-320nm wavelengths. These are consecutive pulses, in a 10 Hz, double-pulsed format. The two wavelengths are used as the on- and off-lines for the ozone DIAL measurement. NASA Langley is currently developing technology for a UV laser transmitter capable of meeting the ORACLE requirements. Experimental efforts to date have shown that the UV generation scheme is viable, and that energies greater than l00mJ/pulse are possible. In this paper, we will briefly discuss the down select process for the proposed laser design, the study effort to date and the laser system design, including both primary and alternate approaches. We will describe UV laser technology that minimizes the total number of optical components (for enhanced reliability) as well as the number of UV coated optics required to transmit the light from the laser (for enhanced optical damage resistance). While the goal is to develop a laser that will produce 500 mJ of energy, we will describe an optional design that will produce output energies between 100 - 200 mJ/unit and techniques for combining multiple laser modules in order to transmit a minimum of 500mJ of UV energy in each pulse of the on- and off-line pulse pairs. This modular laser approach provides redundancy and significantly reduces development time, risk and cost when compared to the development of a single, 500mJ double-pulsed laser subsystem. Finally, we will summarize the laser development effort to date, including results that include the highest known UV energy ( 130 mJ at 320nm) ever produced by a solid-state laser operating in this wavelength region.

Edwards, W. C.↗