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NASA NTRS1982

Ground-based lidar measurements of ozone, water vapor and aerosols in the lower stratosphere and troposphere

Lidar measurements of ozone and water vapor concentrations were performed during several field experiments in 1980-1981 by means of the differential absorption laser technique. Profiles up to 26 km for ozone and up to 9 km for water vapor are presented. Also, a lidar survey of aerosol layers ranging from 12 to 23 km were performed following the Mt. St. Helens major eruption (May 1980). Experiments were conducted at the CNRS lidar facility of the Haute Provence Observatory which is located in southern France (44 deg N, 5 deg E). For ozone a vertical profile is recorded in three sequences, each requiring 15 min of acquisition time. The relative accuracy is better than 5 percent at the lower altitude and falls to 20 percent at 25 km. For water vapor the time sequences are 4 min or 8 min long and the accuracy is better than 10 percent in the lower troposphere.

Flamant, P. H.↗

NASA NTRS1982

Lidar measurements of tropospheric gases

Measurements of pollutants and water vapor in the troposphere using the differential absorption lidar (DIAL) technique are described. Measurements are made of sulfur dioxide in power plant plumes with a mobile DIAL system operated near 300 nm. Comparisons of sulfur dioxide concentrations determined with the DIAL system and in-stack monitors are found to be in agreement to within 18%. Vertical water vapor profiles with a ground-based lidar system are measured using the water vapor absorption line at 724.3 nm. Rawinsonde and DIAL water vapor profile data are shown to agree within 10% to an altitude of 2.5 km. Simulations are discussed for airborne DIAL measurements of sulfur dioxide, water vapor, and nitrogen dioxide.

Browell, E. V.↗

NASA NTRS1982

Radiative flux measurements in the troposphere

A new airborne radiometric system with a time resolution as high as 60 msec has been designed for measuring radiative fluxes in the atmosphere. To verify the instrument performance, the solar constant at the top of the atmosphere has been calculated using the radiative flux densities measured in the troposphere, and the result obtained has been found to agree with the standard value to within 4%. Total heating rates of 0.175 and 0.377 K/h have been determined for hazy and foggy atmospheres, respectively, and aerosol heating rates of 0.065 and 0.235 K/h have been deduced from the total heating rates.

Valero, F. P. J.↗

NASA NTRS1982

Direct measurements of ozone and nitrogen dioxide photolysis rates in the troposphere

The photolysis frequencies of ozone and nitrogen dioxide were measured under a variety of conditions commonly found in the troposphere. Ozone photolysis frequencies show a strong dependence on solar zenith angle, overhead ozone column, and temperature, but only a weak dependence on altitude (when only downward radiation is detected). Nitrogen dioxide photolysis frequencies also show strong dependence on solar zenith angle, but show little dependence on temperature, pressure, or altitude. Both j values are strongly affected by cloud cover, but aerosol loading has much less effect. The disagreement of measured j(O3) and j(NO2) with many modeled values, especially disagreement over altitude dependence, shows that atmospheric UV radioactive processes are complicated and poorly understood, although experimental conditions may not always be applicable to conditions modeled.

Dickerson, R. R.↗

NASA NTRS1982

Tropospheric CO measurement experiment from the second Space Shuttle flight

The MAPS experiment was designed to remotely measure the mixing ratio of carbon monoxide in the middle and upper troposphere using a gas filter radiometer as the sensing instrument. The asymmetrical worldwide distribution of CO is discussed as background, and the experimental scientific and technical objectives are briefly stated. The gas filter radiometer is described in detail, and the second Shuttle mission is summarized. Auxiliary and correlative data were obtained in order to evaluate the performance of the measurement system, to assess the effect of stratospheric ozone on the radiometer signals, and to determine the effect of the underlying surface. The experiment acquired about 32 hours of data between 38 deg N and 38 deg S, signal-to-noise ratios were as predicted and the instrument achieved satisfactory stability in spite of large temperature variations. Data reduction is in progress.

Reichle, H. G., Jr.↗

NASA NTRS1982

CO, O3, and aerosol measurements from NASA Global Tropospheric Experiment - Test flights 1981

A series of four instrument test flights was conducted during July 1981 in preparation for the NASA Global Tropospheric Experiment. The purpose of the flights was to demonstrate the feasibility and value of simultaneously measuring several specific atmospheric pollutants over a 25 deg latitudinal range. Carbon monoxide and methane grab samples were obtained simultaneously with nearly continuous in situ ozone and remote ozone and aerosol optical radar measurements. The sampling platform was a NASA Electra, a four engine turboprop aircraft. Attention is given to CO and CH4 sample collection and analysis, ozone measurement methods, the aerosol measurement method, an interpretation of the optical radar display, and a synergistic consideration of results.

Hinton, R. R.↗

NASA NTRS1982

PAN and the NOx budget of the troposphere

The present investigation has the objective to examine the interaction of NOx with the nonmethane hydrocarbons (NMHCs) photochemistry. Attention is given to the influence of temperature, transport, and hydrocarbon radical reactions on the profiles of peroxyacylnitrates (PANs) and NO2. A lumped NMHC chemical reaction scheme was used in a one-dimensional photochemical model of the global troposphere. Model calculations were performed with various temperature profiles and the corresponding solar zenith angles to examine seasonal variations in the profiles of PAN and NOx. A study of the effects of changing temperature and solar zenith angle on the profiles of PAN and NOx showed that the amount of NO2 tied up in PAN increased as temperature decreased.

Brewer, D. A.↗

NASA NTRS1982

The chlorine budget of the troposphere

It has been hypothesized that chlorine compounds in the stratosphere could photodissociate and release atomic chlorine which catalytically destroys ozone. For an accurate assessment of the possibility of stratospheric ozone depletion, it will be necessary to know the chlorine budget of the entire atmosphere, including the troposphere and the stratosphere. Most chlorine species in the atmosphere are emitted at the surface and diffuse upward. Measurements involving chlorine are reviewed and photochemical calculations are discussed. It is found that between 0.1-1.0 ppbv of inorganic chlorine is present at the surface and about 0.02 ppbv (parts per billion by volume) at the tropopause. Most of the inorganic chlorine is believed to be in the form of HCl, and thus natural in origin. For organic chlorine the corresponding numbers are 1.9 ppbv and 1.7 ppbv, respectively. At the surface approximately 32% of the organic chlorine is natural and 68% anthropogenic.

Augustsson, T. R.↗

NASA NTRS1982

Characterization of tropospheric desert aerosols at solar wavelengths by multispectral radiometry from Landsat

Characteristics of tropospheric desert aerosols are derived by comparing nadir spectral reflectivities computed from the radiative transfer models with reflectivities measured from Landsat. Over the ocean, reflectivities are compared, but over land the comparison is carried out by determining the ratios of the nadir reflectivity of the surface-atmosphere system over heavy aerosol concentration to the reflectivity of the underlying surface. This remote sensing technique is found to be a sensitive approach for measuring n sub 2, the imaginary part of the refractive index. The desert aerosols under study, in the Iran and Pakistan area, are essentially pure scatterers, inasmuch as an n sub 2 value of 0.001 + or - 0.001 was determined for each of the four Landsat spectral bands, that is, for a spectral interval from 0.5 to 1.1 microns.

Otterman, J.↗

NASA NTRS1982

Clouds and wet removal as causes of variability in the trace-gas composition of the marine troposphere

A modeling study of the effects of clouds and wet removal on the chemistry of the remote marine troposphere is described. Using a time-dependent model with parameterized vertical transport to calculate trace-gas concentrations, it is found that large variations in key species (e.g., HNO3, H2CO, and H2O2) result from simulations of sporadic rainfall, changes in cloud cover, and external inputs such as surface NO sources. Depending on the frequency and intensity of an event, the effects of these perturbations may persist for several days, thereby invalidating assumptions of photochemical equilibrium in the interpretation of measurements. Long-term integrations with fixed boundary conditions and regularly occurring cloud and rain episodes demonstrate a strong sensitivity of the mean concentration of longer-lived soluble gases to precipitation frequency but also confirm the validity of using properly chosen parameterizations of wet removal in steady state calculations.

Thompson, A. M.↗

NASA NTRS1982

Technology needs assessment of an atmospheric observation system for tropospheric research missions, part 1

The technology advancements needed to implement the atmospheric observation satellite systems for air quality research were identified. Tropospheric measurements are considered. The measurements and sensors are based on a model of knowledge objectives in atmospheric science. A set of potential missions and attendant spacecraft and sensors is postulated. The results show that the predominant technology needs will be in passive and active sensors for accurate and frequent global measurements of trace gas concentration profiles.

Alvarado, D. R.↗

NASA NTRS1983

The 1980 stratospheric-tropospheric exchange experiment

Data are presented from the Stratospheric-Tropospheric Water Vapor Exchange Experiment. Measurements were made during 11 flights of the NASA U-2 aircraft which provided data from horizontal traverser and samplings in and about the tops of extensive cirrus-anvil clouds produced by overshooting cumulus turrets. Aircraft measurements were made of water vapor, ozone, ambient and cloud top temperature, fluorocarbons, nitrous oxide, nitric acid, aerosols, and ice crystal populations. Balloonsondes were flown about twice daily providing data on ozone, wind fields, pressure and temperature to altitudes near 30 km. Satellite photography provided detailed cloud and cloud top temperature information. Descriptions of individual experiments and detailed compilations of all results are provided.

Margozzi, A. P.↗

NASA NTRS1983

Latitudinal variation of tropospheric ozone in a photochemical model

A zonally, vertically, and annually averaged numerical model of trace gases in the troposphere is used to examine the variation of ozone as a function of latitude. Processes included in the ozone budget are a source due to downward transport of ozone from the stratosphere, deposition at earth's surface, north-south diffusive transport, and photochemical reactions. Sensitivity of calculated ozone concentrations to the latitude variation and magnitude of the stratospheric source is presented. The model indicates a net photochemical source of ozone in the Northern Hemisphere and a net chemical sink in the tropical latitudes. Calculated variation of ozone concentration with latitude is in qualitative agreement with observations.

Hameed, S.↗

NASA NTRS1983

Troposphere-stratosphere (surface-55 km) monthly winter general circulation statistics for the Northern Hemisphere Four year averages

In response to theoretically predicted anthropogenic depletion of stratospheric ozone, there has been, in recent years, an increased effort in stratospheric modeling. For comparison between models and observations, it is not sufficient to only compare the morphology of model-generated parameters with observed parameter values. Model-generated statistics should also be compared with observation. It is one of the objectives of the present investigation to discuss a data set which can be used for this purpose for the Northern Hemisphere troposphere and stratosphere. However, the investigation is mainly concerned with a presentation of some of the general circulation statistics derived with the aid of the data set. Attention is given to winter monthly general circulation statistics which were derived from four years of daily 1200 GMT NOAA/NMC Northern Hemisphere analyses.

Geller, M. A.↗

NASA NTRS1983

The photochemistry of anthropogenic nonmethane hydrocarbons in the troposphere

A lumped, nonmethane hydrocarbon (NMHC) chemical mechanism is presently applied to a one-dimensional photochemical model of the troposphere. The profiles of OH, HO2, NO(x), and HNO3, showed only slight changes when NMHC chemistry was added. The integrated column of peroxyacetylnitrate (PAN), when NMHC chemistry was included, comprised 17 percent of the odd nitrogen budget. Advection is noted as an important possible mechanism for the removal of PAN at midlatitudes. The inclusion of such intermediate lifetime species as aldehydes and olefins has both provided additional sources of short-lived NMHC radicals, such as the peroxyacetyl radical that is the radical precursor of PAN, and offered a more detailed description of the concentrations of short-lived species and the overall NMHC chemistry.

Brewer, D. A.↗

NASA NTRS1983

Use of long-lived radon daughters as indicators of exchange between the free troposphere and the marine boundary layer

Fluxes and exchange coefficients are derived for the transport of Sr-90, Pb-210, Bi-210, and Po-210 between the free troposphere and the marine boundary layer and between the boundary layer and the sea surface. Radionuclide concentrations previously measured near Hawaii are used in the derivations. Values obtained for the free troposphere/boundary layer exchange coefficient (expressed as a piston velocity) were 185, 228 and 203 m/d for Pb-210, Bi-210, and Sr-90, respectively. The magnitude of the local sea-surface source of Po-210 is also determined.

Kritz, M. A.↗

NASA NTRS1983

Observations of the upper troposphere and lower stratosphere using the urbana coherent-scatter radar

The Urbana coherent-scatter radar was used to observe the upper troposphere and lower stratosphere, and 134 hours of data were collected. Horizontal wind measurements show good agreement with balloon-measured winds. Gravity waves were frequently observed, and were enhanced during convective activity. Updrafts and downdrafts were observed within thunderstorms. Power returns are related to hydrostatic stability, and changes in echo specularity are shown.

Goss, L. D.↗

NASA NTRS1983

Techniques for studying gravity waves and turbulence: Vertical wind speed power spectra from the troposphere and stratosphere obtained under light wind conditions

A joint France/U.S. experiment was conducted near the mouth of the Rhone river in southern France as part of the ALPEX program. This experiment used 3 vertically directed 50 MHz radars separated by 4 to 6 km. The main purpose of this experiment was to study the spatial characteristics of gravity waves. The good height resolution (750 meters) and time resolution (1 minute) and the continuous operation over many weeks have yielded high resolution vertical wind speed power spectra under a variety of synoptic conditions. Vertical spectra obtained during very quiet (low wind) conditions in the troposphere and lower stratosphere from a single site are presented.

Ecklund, W. L.↗