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At least 955 records · Page 53

Spectrum Unfolding with the MC-15

The Multiplicity Counter 15 tube detector or MC-15 is an optimized detector designed for use in the field. It is composed of 15 3 He tubes embedded in high density polyethylene (HDPE). Recent work has explored expanding the use of the MC-15 beyond multiplicity counting to neutron dosimetry applications. Knowledge of the neutron energy spectrum information is required to use a detector as a neutron dosimeter. The MC-15 tube layout is shown in Figure 1. The unique layout makes it possible to use the detector for neutron spectroscopy via spectrum unfolding. Spectrum unfolding requires (1) energy dependence of the detector response, (2) a detector response matrix that precisely quantifies the response to mono-energetic neutrons, (3) an initial guess spectrum, (4) an unfolding algorithm, and (5) measured data (counts in the case of the MC-15). An energy dependent detector response matrix (DRM) can be constructed by considering either each of the three rows of 3 He tubes as a distinct detector or each individual tube as a distinct detector. The HDPE separating the 3 He in the MC-15 provides the distinct energy dependent response for the rows and individual tubes. In this report we detail the development of detector response matrices for the MC-15 and the application of the Los Alamos Unfolding Code (LUC) to both simulated and measured data. Three MC-15 orientations were studied: (1) standard orientation with the MC-15 front facing the source, (2) standard orientation with Cd sheet, (3) 90° orientation with the side of the MC-15 facing the source.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

History of and Aftermath from the Withdrawal of the Intermediate-Range Nuclear Forces Treaty

On February 1, 2019, the United States and Russia withdrew from the three-decades old Intermediate-Range Nuclear Forces (INF) treaty. Events precipitating the withdrawal were allegations by both the United States and Russia of a variety of treaty violations. Until that point, the treaty had been a centerpiece of arms control and a key agreement of the global security architecture. The absence of such a pillar has the potential destabilize the status quo of arms control, creating significant uncertainty in global nuclear stability and security. In this paper, we present a historical review as overture to an analysis on the impacts of this development on force structure. This analysis examines the changes in U.S., Russian, and Chinese nuclear forces which may occur as a result of the treaty's demise. The article concludes with commentary on potential actions to preserve stability in a post-INF world.

45 MILITARY TECHNOLOGY, WEAPONRY, AND NATIONAL DEF↗

Enhancement of sub-thermal neutron flux through cold polyethylene

Total thermal neutron cross section measurements serve as the primary means of validation for thermal neutron scattering kernels, an important quantity for neutron transport calculations. In an effort to improve the quality of thermal neutron scattering kernels, researchers at Rensselaer Polytechnic Institute (RPI) designed and constructed a polyethylene based cold moderation system to enhance neutron flux below 10 meV when coupled with the Enhanced Thermal Target (ETT) at the RPI Gaerttner LINAC. The final design yielded an increase in sub-thermal neutron flux (below 10 meV) by a factor of 4.5 for a moderator temperature of 37.5 K relative to the ETT alone. A further increase to a factor of 6 is expected after a minor geometry modification and decrease in polyethylene temperature to 25 K. This novel capability will be used to conduct total thermal neutron cross section measurements from 0.0005–10 eV for different materials including moderator materials.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Hyperspectral x-ray imaging mapping capabilities for nuclear forensics

Nuclear forensics relies on the integration of complementary signatures to constrain the origins and history of materials. Outcomes benefit from the timeliness and precision of the disparate methods that form typical analysis chains. Sample forms are often either minute in quantity or contain signatures like morphology or composition heterogeneity encoded on a microscale, so many analysis techniques focus on resolving signatures on ever-smaller length scales. The new hyperspectral x-ray imaging (HXI) instrument developed at Los Alamos National Laboratory seeks to improve the information available from scanning electron microscopy (SEM) x-ray spectrum analysis through superior spectral energy resolution vs. typical energy dispersive spectroscopy (EDS) systems in common use in nuclear forensics and other microanalysis fields. Based on arrays of transition-edge sensor (TES) microcalorimeter detectors, this instrument achieves a typical energy resolution of 7 eV full-width at half-maximum (FWHM) at 2 keV, opening new possibilities in trace element detection/analysis and chemical state determination through spectral shape shifts. We present here some of the first applications of the HXI instrument to actinide samples and discuss potential maturation of this nascent technology for future analysis pipelines.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

A Qualitative Strategy for Fusion of Physics into Empirical Models for Process Anomaly Detection

To facilitate the automated online monitoring of power plants, a systematic and qualitative strategy for anomaly detection is presented. This strategy is essential to provide credible reasoning on why and when an empirical versus hybrid (i.e., physics-supported) approach should be used and to determine the ideal mix of these two approaches for a defined anomaly detection scope. Empirical methods are usually based on pattern, statistical, and causal inference. Hybrid methods include the use of physics models to train and test data methods, reduce data dimensionality, reduce data-model complexity, augment data, and reduce empirical uncertainty; hybrid methods also include the use of data to tune physics models. The presented strategy is driven by key decision points related to data relevance, simple modeling feasibility, data inference, physics-modeling value, data dimensionality, physics knowledge, method of validation, performance, data availability, and suitability for training and testing, cause-effect, entropy inference, and model fitting. The strategy is demonstrated through a pilot use case for the application of anomaly detection to capture a valve packing leak at the high-pressure coolant injection system of a nuclear power plant.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Quantitative Long-Term Monitoring of the Circulating Gases in the KATRIN Experiment Using Raman Spectroscopy

The Karlsruhe Tritium Neutrino (KATRIN) experiment aims at measuring the effective electron neutrino mass with a sensitivity of 0.2 eV/c2, i.e., improving on previous measurements by an order of magnitude. Neutrino mass data taking with KATRIN commenced in early 2019, and after only a few weeks of data recording, analysis of these data showed the success of KATRIN, improving on the known neutrino mass limit by a factor of about two. This success very much could be ascribed to the fact that most of the system components met, or even surpassed, the required specifications during long-term operation. Here, we report on the performance of the laser Raman (LARA) monitoring system which provides continuous high-precision information on the gas composition injected into the experiment’s windowless gaseous tritium source (WGTS), specifically on its isotopic purity of tritium—one of the key parameters required in the derivation of the electron neutrino mass. The concentrations cx for all six hydrogen isotopologues were monitored simultaneously, with a measurement precision for individual components of the order 10−3 or better throughout the complete KATRIN data taking campaigns to date. From these, the tritium purity, εT, is derived with precision of <10−3 and trueness of <3 × 10−3, being within and surpassing the actual requirements for KATRIN, respectively.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Development of a Nuclear Fuel Dissolution Monitor Based on Raman Spectroscopy

The processing of spent nuclear fuel and other nuclear materials is a critical component of nuclear material management with implications for global security. The first step of fuel processing is dissolution, with several charges of fuel sequentially added to a batch of solvent. The incomplete dissolution of a charge precludes the addition of the next charge. As the dissolution takes place in a heated, highly corrosive and radiological vessel, direct monitoring of the process is not possible. We discuss the use of Raman spectroscopy to indirectly monitor dissolution through an analysis of the gaseous emissions from the dissolver. Challenges associated with the implementation of Raman spectroscopy include the composition and physical characteristics of the offgas stream and the impact of operating conditions. Nonetheless, we observed that NO2 concentrations serve as a reliable indicator of process activity and correlate to the amount of fuel material that remains undissolved. These results demonstrate the promise of the method for monitoring nuclear material dissolution.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Double Image Polarimeter—Ultra Fast: Simultaneous Three-color (BVR) Polarimeter with Electron-multiplying Charge-coupled Devices

We describe a new instrument capable of high-precision (10{sup −5}) polarimetric observations simultaneously in three passbands (BVR). The instrument utilizes electron-multiplying charge-coupled device (EM CCD) cameras for high efficiency and fast image readout. The key features of the Double Image Polarimeter—Ultra Fast (DIPol-UF) are: (i) the optical design with high throughput and inherent stability; (ii) great versatility, which makes the instrument optimally suitable for observations of bright and faint targets; and (iii) a control system, which allows the use of the polarimeter remotely. Examples are given of the first results obtained from high signal-to-noise observations of bright nearby stars and of fainter sources such as X-ray binaries in their quiescent states.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

An Optical Overview of Blazars with LAMOST. II. Gamma-Ray Blazar Candidates and Updated Classifications

Blazars represent the dominant class of associated γ-ray sources detected by the Fermi Large Area Telescope (LAT). However, in the more recent release of the Fourth Fermi-LAT Point Source Catalog (4FGL), ∼25% of the sources associated with lower-energy counterparts show a multifrequency behavior similar to that of blazars, but lacks an optical spectroscopic confirmation of their nature and are therefore classified as Blazar Candidates of Uncertain Type (BCUs). A particularly challenging task in blazar studies is to classify these BCUs and, when possible to estimate their redshifts, in particular for BL Lac objects, characterized by almost featureless optical spectra with only weak emission lines. Continuing our study of blazars with Large Sky Area Multi-Object Fiber Spectroscopic Telescope (LAMOST) optical spectral data, we perform an extensive search for optical spectra available in the LAMOST Data Release 6 archive. Our aim is confirming the blazar nature of BCUs and to test if new data can allow us to get a redshift estimate for BL Lac objects that lack measurement, as well as to search for and discover changing-look blazars. We selected sources out of the 4FGL catalog, the list of targets from our follow-up spectroscopic campaign of unidentified and/or unassociated γ-ray sources, and the Roma-BZCAT multifrequency catalog of blazars, finding a total of 42 sources with available LAMOST DR6 spectra. We confirmed the blazar-like nature of four blazar candidates . For the remaining 37 sources we confirm their previous classification.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Analysis of Polarimetry Data with Angular Uncertainties

For a track based polarimeter, such as the Imaging X-ray Polarimetry Explorer (IXPE), the sensitivity to polarization depends on the modulation factor, which is a strong function of energy. In previous work, a likelihood method was developed that would account for this variation in order to estimate the minimum detectable polarization (MDP). That method essentially required that the position angles of individual events should be known precisely. In a separate work, however, it was shown that using a machine-learning method for measuring event tracks can generate track angle uncertainties, which can be used in the analysis. Here, the maximum likelihood method is used as a basis for revising the estimate of the MDP in a general way that can include uncertainties in event track position angles. The resultant MDP depends solely upon the distribution of track angle uncertainties present in the input data. Due to the physics of the IXPE detectors, it is possible to derive a simple relationship between these angular uncertainties and the energy-dependent modulation function as a step in the process.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

A Measurement of the Total Hadronic $\pi^-$ on Argon Cross Section in the Kinetic Energy Range from 0.2-1 Giga-Electron Volts in a Liquid Argon Time Projection Chamber

The liquid argon time projection chamber (LArTPC) technology offers fine-grained tracking along with excellent calorimetric and particle identification capabilities, making it a powerful tool for experimental neutrino physics. Thus, the LArTPC has become the technology of choice for studying neutrino oscillations over short ( 1000 km) baselines by experiments such as MicroBooNE, SBND, ICARUS, and DUNE. The LArIAT (Liquid Argon in a Test-beam) experiment exposes a LArTPC to a controlled beam of charged particles at the Fermilab Test Beam Facility to perform calibration studies and measurements of charged hadron-argon cross sections, with the goal of helping to reduce systematic uncertainties in LArTPC-based neutrino experiments. This work presents a measurement of the total hadronic π⁻-Ar cross section in the kinetic energy range from 0.2 GeV to 1 GeV, using data from the LArIAT experiment.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

“4H” X-ray camera

A 4H X-ray camera includes a high speed, high atomic number (Z), high spatial resolution sensor for sensing X-rays having energy over 30 keV and high speed readout electronics, and the high speed, high atomic number (Z), high spatial resolution sensor is coupled to the high speed readout electronics.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗