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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 955 records · Page 53
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Spin-lattice model for cubic crystals

In this work, we present a methodology based on the Néel model to build a classical spin-lattice Hamiltonian for cubic crystals capable of describing magnetic properties induced by the spin-orbit coupling like magnetocrystalline anisotropy and anisotropic magnetostriction, as well as exchange magnetostriction. Taking advantage of the analytical solutions of the Néel model, we derive theoretical expressions for the parametrization of the exchange integrals and Néel dipole and quadrupole terms that link them to the magnetic properties of the material. This approach allows us to build accurate spin-lattice models with the desired magnetoelastic properties. We also explore a possible way to model the volume dependence of magnetic moment based on the Landau energy. This feature allows us to consider the effects of hydrostatic pressure on the saturation magnetization. We apply this method to develop a spin-lattice model for BCC Fe and FCC Ni, and we show that it accurately reproduces the experimental elastic tensor, magnetocrystalline anisotropy under pressure, anisotropic magnetostrictive coefficients, volume magnetostriction, and saturation magnetization under pressure at zero temperature. This work could constitute a step towards large-scale modeling of magnetoelastic phenomena.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2019

Intracellular Dynamics of Superparamagnetic Iron Oxide Nanoparticles for Magnetic Partical Imaging

Superparamagnetic iron oxide nanoparticles (SPIONs) are a foundational platform for a variety of biomedical applications. Of particular interest is Magnetic Particle Imaging (MPI), which is a growing area of research and development due to its advantages including high resolution and sensitivity with positive contrast. There has been signicant work in the area of in vivo optimization of SPIONs for MPI as well as their biodistribution in and clearance from the body. However, little is known about the dynamics of SPIONs following cellular internalization which may limit their usefulness in a variety of potential imaging and treatment applications. This work shows a clear 20% decrease in magnetic performance of SPIONs, as observed by Magnetic Particle Spectroscopy (MPS), after internalization and systematic consideration of applicable factors that aect SPION signal generation, including microstructure, environment, and interparticle interactions. There is no observed change to SPION microstructure after internalization, and the surrounding environment plays little to no role in magnetic response for the SPIONs studied here. Interparticle interactions described by dipole-dipole coupling of SPIONs held close to one another after internalization are shown to be the dominant cause of decreased magnetic performance in cells. These conclusions were drawn from transmission electron microscopy (TEM) image analysis at relevant length scales, experimentally prepared and characterized SPIONs in varied environmental conditions, and theoretical modeling with Monte Carlo simulations.

Teeman, Eric M.↗
DOE OSTI2014

An experimental verification of metamaterial coupled enhanced transmission for antenna applications

Inspired by the work of Bethe on electromagnetic transmission through subwavelength hole, there has been immense interest on the extraordinary transmission through subwavelength slot/slit on metal plates. The invention of metamaterials has boosted the extra ordinary transmission through subwavelength slots. We examine computationally and experimentally the concept of metamaterial cover using an array of split ring resonators (SRRs), for enhancing the transmission in a stacked dipole antenna working in the S band. The front to back ratio is considerably improved by enhancing the magnetic resonant strength in close proximity of the slit of the upper parasitic dipole. The effect of stacking height of the SRR monolayer on the resonant characteristics of the split ring resonators and its effect on antenna radiation characteristics has been studied.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2016

Prospects for quantum computing with an array of ultracold polar paramagnetic molecules

Arrays of trapped ultracold molecules represent a promising platform for implementing a universal quantum computer. DeMille [Phys. Rev. Lett. 88, 067901 (2002)] has detailed a prototype design based on Stark states of polar {sup 1}Σ molecules as qubits. Herein, we consider an array of polar {sup 2}Σ molecules which are, in addition, inherently paramagnetic and whose Hund’s case (b) free-rotor pair-eigenstates are Bell states. We show that by subjecting the array to combinations of concurrent homogeneous and inhomogeneous electric and magnetic fields, the entanglement of the array’s Stark and Zeeman states can be tuned and the qubit sites addressed. Two schemes for implementing an optically controlled CNOT gate are proposed and their feasibility discussed in the face of the broadening of spectral lines due to dipole-dipole coupling and the inhomogeneity of the electric and magnetic fields.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2013

SOLAR MAGNETIC ACTIVITY CYCLES, CORONAL POTENTIAL FIELD MODELS AND ERUPTION RATES

We study the evolution of the observed photospheric magnetic field and the modeled global coronal magnetic field during the past 3 1/2 solar activity cycles observed since the mid-1970s. We use synoptic magnetograms and extrapolated potential-field models based on longitudinal full-disk photospheric magnetograms from the National Solar Observatory's three magnetographs at Kitt Peak, the Synoptic Optical Long-term Investigations of the Sun vector spectro-magnetograph, the spectro-magnetograph and the 512-channel magnetograph instruments, and from Stanford University's Wilcox Solar Observatory. The associated multipole field components are used to study the dominant length scales and symmetries of the coronal field. Polar field changes are found to be well correlated with active fields over most of the period studied, except between 2003 and 2006 when the active fields did not produce significant polar field changes. Of the axisymmetric multipoles, only the dipole and octupole follow the poles whereas the higher orders follow the activity cycle. All non-axisymmetric multipole strengths are well correlated with the activity cycle. The tilt of the solar dipole is therefore almost entirely due to active-region fields. The axial dipole and octupole are the largest contributors to the global field except while the polar fields are reversing. This influence of the polar fields extends to modulating eruption rates. According to the Computer Aided CME Tracking, Solar Eruptive Event Detection System, and Nobeyama radioheliograph prominence eruption catalogs, the rate of solar eruptions is found to be systematically higher for active years between 2003 and 2012 than for those between 1997 and 2002. This behavior appears to be connected with the weakness of the late-cycle 23 polar fields as suggested by Luhmann. We see evidence that the process of cycle 24 field reversal is well advanced at both poles.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2016

SPATIAL DISTRIBUTION OF PAIR PRODUCTION OVER THE PULSAR POLAR CAP

Using an analytic, axisymmetric approach that includes general relativity, coupled to a condition for pair production deduced from simulations, we derive general results about the spatial distribution of pair-producing field lines over the pulsar polar cap. In particular, we show that pair production on magnetic field lines operates over only a fraction of the polar cap for an aligned rotator for general magnetic field configurations, assuming the magnetic field varies spatially on a scale that is larger than the size of the polar cap. We compare our result to force-free simulations of a pulsar with a dipole surface field and find excellent agreement. Our work has implications for first-principles simulations of pulsar magnetospheres and for explaining observations of pulsed radio and high-energy emission.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

Magnetic structure and magnetocalorics of GdPO 4

The magnetic ordering structure of GdPO 4 is determined at T = 60 mK by diffraction of hot neutrons with wavelength = 0.4696 Å. It corresponds to a non-collinear antiferromagnetic arrangement of the Gd moments with propagation vector k = (1/2, 0, 1/2). This arrangement is found to minimize the dipole-dipole interaction and the crystal field anisotropy energy, the magnetic superexchange being much smaller. The intensity of the magnetic reflections decreases with increasing temperature and vanishes at T ≈ 0.8 K, in agreement with the magnetic ordering temperature T N = 0.77 K, as reported in previous works based on heat capacity and magnetic susceptibility measurements. The magnetocaloric parameters have been determined from heat capacity data at constant applied fields up to 7 T, as well as from isothermal magnetization data. Lastly, the magnetocaloric effect, for a field change ΔB = 0 – 7T, reaches –ΔS T = 375.8mJ / cm 3 K –1 at T = 2.1 K, largely exceeding the maximum values reported to date for Gd-based magnetic refrigerants.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2014

Field Quality Study of a 1-m-Long Single-Aperture 11-T Nb$_3$Sn Dipole Model for LHC Upgrades

FNAL and CERN are carrying out a joint R&D program with the goal of building a 5.5-m-long twin-aperture 11-T Nb_3Sn dipole prototype that is suitable for installation in the LHC. An important part of the program is the development and test of a series of short single-aperture and twin-aperture dipole models with a nominal field of 11 T at the LHC operation current of 11.85 kA and 20% margin. This paper presents the results of magnetic measurements of a 1-m-long single-aperture Nb_3Sn dipole model fabricated and tested recently at FNAL, including geometrical field harmonics and effects of coil magnetization and iron yoke saturation.

43 PARTICLE ACCELERATORS↗
DOE OSTI2013

TWO NOVEL PARAMETERS TO EVALUATE THE GLOBAL COMPLEXITY OF THE SUN'S MAGNETIC FIELD AND TRACK THE SOLAR CYCLE

Since the unusually prolonged and weak solar minimum between solar cycles 23 and 24 (2008-2010), the sunspot number is smaller and the overall morphology of the Sun's magnetic field is more complicated (i.e., less of a dipole component and more of a tilted current sheet) compared with the same minimum and ascending phases of the previous cycle. Nearly 13 yr after the last solar maximum ({approx}2000), the monthly sunspot number is currently only at half the highest value of the past cycle's maximum, whereas the polar magnetic field of the Sun is reversing (north pole first). These circumstances make it timely to consider alternatives to the sunspot number for tracking the Sun's magnetic cycle and measuring its complexity. In this study, we introduce two novel parameters, the standard deviation (SD) of the latitude of the heliospheric current sheet (HCS) and the integrated slope (SL) of the HCS, to evaluate the complexity of the Sun's magnetic field and track the solar cycle. SD and SL are obtained from the magnetic synoptic maps calculated by a potential field source surface model. We find that SD and SL are sensitive to the complexity of the HCS: (1) they have low values when the HCS is flat at solar minimum, and high values when the HCS is highly tilted at solar maximum; (2) they respond to the topology of the HCS differently, as a higher SD value indicates that a larger part of the HCS extends to higher latitude, while a higher SL value implies that the HCS is wavier; (3) they are good indicators of magnetically anomalous cycles. Based on the comparison between SD and SL with the normalized sunspot number in the most recent four solar cycles, we find that in 2011 the solar magnetic field had attained a similar complexity as compared to the previous maxima. In addition, in the ascending phase of cycle 24, SD and SL in the northern hemisphere were on the average much greater than in the southern hemisphere, indicating a more tilted and wavier HCS in the north than the south, associated with the early reversal of the polar magnetic field in the north relative to the south.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2024

From Feast to Famine: A Systematic Study of Accretion onto Oblique Pulsars with 3D GRMHD Simulations

Disk-fed accretion onto neutron stars can power a wide range of astrophysical sources ranging from X-ray binaries, to accretion-powered millisecond pulsars, ultraluminous X-ray sources, and gamma-ray bursts. A crucial parameter controlling the gas–magnetosphere interaction is the strength of the stellar dipole. In addition, coherent X-ray pulsations in many neutron star systems indicate that the star's dipole moment is oblique relative to its rotation axis. Therefore, it is critical to systematically explore the 2D parameter space of the star's magnetic field strength and obliquity, which is what this work does, for the first time, in the framework of 3D general-relativistic magnetohydrodynamics. If the accretion disk carries its own vertical magnetic field, this introduces an additional factor: the relative polarity of the disk and stellar magnetic fields. We find that depending on the strength of the stellar dipole and the star–disk relative polarity, the neutron star's jet power can either increase or decrease with increasing obliquity. For weak dipole strength (equivalently, high accretion rate), the parallel polarity results in a positive correlation between jet power and obliquity, whereas the antiparallel orientation displays the opposite trend. For stronger dipoles, the relative-polarity effect disappears, and jet power always decreases with increasing obliquity. The influence of the relative polarity gradually disappears as obliquity increases. Highly oblique pulsars tend to have an increased magnetospheric radius, a lower mass accretion rate, and enter the propeller regime at lower magnetic moments than aligned stars.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2016

The effect of an offset polar cap dipolar magnetic field on the modeling of the vela pulsar's γ-ray light curves

We performed geometric pulsar light curve modeling using static, retarded vacuum, and offset polar cap (PC) dipole B-fields (the latter is characterized by a parameter ϵ), in conjunction with standard two-pole caustic (TPC) and outer gap (OG) emission geometries. The offset-PC dipole B-field mimics deviations from the static dipole (which corresponds to ϵ=0). In addition to constant-emissivity geometric models, we also considered a slot gap (SG) E-field associated with the offset-PC dipole B-field and found that its inclusion leads to qualitatively different light curves. Solving the particle transport equation shows that the particle energy only becomes large enough to yield significant curvature radiation at large altitudes above the stellar surface, given this relatively low E-field. Therefore, particles do not always attain the radiation-reaction limit. Our overall optimal light curve fit is for the retarded vacuum dipole field and OG model, at an inclination angle α=78{sub −1}{sup +1{sup {sup ∘}}} and observer angle ζ=69{sub −1}{sup +2{sup {sup ∘}}}. For this B-field, the TPC model is statistically disfavored compared to the OG model. For the static dipole field, neither model is significantly preferred. We found that smaller values of ϵ are favored for the offset-PC dipole field when assuming constant emissivity, and larger ϵ values favored for variable emissivity, but not significantly so. When multiplying the SG E-field by a factor of 100, we found improved light curve fits, with α and ζ being closer to best fits from independent studies, as well as curvature radiation reaction at lower altitudes.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

Status of the 11 T Nb$_{3}$Sn Dipole Project for the LHC

The planned upgrade of the LHC collimation system includes additional collimators in the LHC lattice. The longitudinal space for the collimators could be obtained by replacing some LHC main dipoles with shorter but stronger dipoles compatible with the LHC lattice and main systems. A joint development program with the goal of building a 5.5 m long two-in-one aperture Nb_3Sn dipole prototype suitable for installation in the LHC is being conducted by FNAL and CERN magnet groups. As part of the first phase of the program, 1 m long and 2 m long single aperture models are being built and tested, and the collared coils from these magnets will be assembled and tested in two-in-one configuration in both laboratories. In parallel with the short model magnet activities, the work has started on the production line in view of the scale-up to 5.5 m long prototype magnet. The development of the final cryo-assembly comprising two 5.5 m long 11 T dipole cold masses and the warm collimator in the middle, fully compatible with the LHC main systems and the existing machine interfaces, has also started at CERN. This paper summarizes the progress made at CERN and FNAL towards the construction of 5.5 m long 11 T Nb_3Sn dipole prototype and the present status of the activities related to the integration of the 11 T dipole and collimator in the LHC.

43 PARTICLE ACCELERATORS↗
DOE OSTI2017

Progress on the Development of the Nb 3 Sn 11T Dipole for the High Luminosity Upgrade of LHC

The high-luminosity large hadron collider (LHC) project at CERN entered into the production phase in October 2015 after the completion of the design study phase. In the meantime, the development of the 11 T dipole needed for the upgrade of the collimation system of the machine made significant progress with very good performance of the first two-in-one magnet model of 2-m length made at CERN. The 11 T dipole, which is more powerful than the current main dipoles of LHC, can be made shorter with an equivalent integrated field. This will allow creating space for the installation of additional collimators in specific locations of the dispersion suppressor regions. Following tests carried out during heavy ions runs of LHC in the end of 2015, and a more recent review of the project budget, the installation plan for the 11 T dipole was revised. Consequently, one 11 T dipole full assembly containing two 11 T dipoles of 5.5-m length will be installed on either side of interaction point 7. These two units shall be installed during the long shutdown 2 in years 2019-2020. After a brief reminder on the design features of the magnet, this paper describes the current status of the development activities, in particular the short model programme and the construction of the first full scale prototype at CERN. Finally, critical operations such as the reaction treatment and the coil impregnation are discussed, the quench performance tests results of the two-in-one model are reviewed and finally, the plan toward the production for the long shut down 2 is described.

43 PARTICLE ACCELERATORS↗
DOE OSTI2022

Systematic Errors Induced by Dipole Component Change in Quadrupole Beam-Based Alignment Measurements for Circular Accelerators

Beam-based alignment (BBA) for quadrupole magnets is now a well-established process for circular accelerators to steer beam orbit through the magnetic centers such that beam orbit is not disturbed when the gradients of quadrupoles are changed. At some facilities, the centers estimated from BBA techniques are also used as a proxy for steering beam through the centers of nearby nonlinear magnets to minimize degradation of nonlinear dynamics caused by off-centered orbit. The random errors associated with BBA are well known, but very little attention has been paid to the systematic error generated by a dipole component change, or equivalently a shift in the magnetic center, when the quadrupole strength is varied. The analytical formulas for this error and its amplification factor (potentially a few orders of magnitude) with respect to the magnetic center motion have been derived and confirmed with simulations. We address the significance of this error as well as the part that cannot be estimated from the beam-based measurement alone. Finally, the BBA measurements obtained at NSLS-II and their systematic errors on the order of hundreds of microns are discussed.

43 PARTICLE ACCELERATORS↗
DOE OSTI2017

Single‐Domain Ferromagnet of Noncentrosymmetric Uniaxial Magnetic Ions and Magnetoelectric Interaction

Abstract The feasibility of a single‐domain ferromagnet based on uniaxial magnetic ions was examined. For a noncentrosymmetric uniaxial magnetic ion of magnetic moment μ at a site of local electric dipole moment p , it is unknown to date whether μ prefers to be parallel or antiparallel to μ . The nature of this magnetoelectric interaction was probed in terms of analogical reasoning based on the Rashba effect and density functional theory (DFT) calculations. We show that μ and p prefer an antiparallel arrangement, predict that Fe‐doped CaZnOS is a single‐domain ferromagnet like a bar magnet, and find the probable cause for the ferromagnetism and weak magnetization hysteresis in Fe‐doped hexagonal ZnO and ZnS at very low dopant concentrations.

Koo, Hyun‐Joo↗
DOE OSTI2017

Single-Domain Ferromagnet of Noncentrosymmetric Uniaxial Magnetic Ions and Magnetoelectric Interaction

The feasibility of a single-domain ferromagnet based on uniaxial magnetic ions was examined. For a noncentrosymmetric uniaxial magnetic ion of magnetic moment μ at a site of local electric dipole moment p , it is unknown to date whether μ prefers to be parallel or antiparallel to μ . The nature of this magnetoelectric interaction was probed in terms of analogical reasoning based on the Rashba effect and density functional theory (DFT) calculations. Here, we show that μ and p prefer an antiparallel arrangement, predict that Fe-doped CaZnOS is a single-domain ferromagnet like a bar magnet, and find the probable cause for the ferromagnetism and weak magnetization hysteresis in Fe-doped hexagonal ZnO and ZnS at very low dopant concentrations.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2021

Emerged Metallicity in Molecular Ferromagnetic Wires

Supramolecular engineering bridges molecular assembly with macromolecular charge-transfer salts, promising the design to construct supramolecular architectures that integrate cooperative properties difficult or impossible to find in conventional lattices. Here, we report the crystal engineering design and kinetic growth of one-dimensional supramolecular wires composed of bis(ethylenedithio)tetrathiafulvalene (ET + ) cation and polymeric Cu[N(CN) 2 ] 2 – anion. A bulk ferromagnetic order is discovered for filling up the gap where strong ferromagnetism is missing in such ET molecule-based charge-transfer salts. Metallicity is induced by electric current from the semiconducting wire, which is attributed to strain effect by tuning its close molecular contact. This structural feature is evidenced through the combination of various mechanistic spectroscopic studies. Further, electric dipole is established from the close molecular contacts and is suggestive to stabilize ferromagnetic spin interaction through anions bridging spin sites. The breakthrough shown here provides a pathway to explore low-dimensional supramolecular materials exhibiting strong electron correlation, metallicity, and ferromagnetism.

77 NANOSCIENCE AND NANOTECHNOLOGY↗
DOE OSTI2024

Extraordinary phase transition revealed in a van der Waals antiferromagnet

While the surface-bulk correspondence has been ubiquitously shown in topological phases, the relationship between surface and bulk in Landau-like phases is much less explored. Theoretical investigations since 1970s for semi-infinite systems have predicted the possibility of the surface order emerging at a higher temperature than the bulk, clearly illustrating a counterintuitive situation and greatly enriching phase transitions. But experimental realizations of this prediction remain missing. Here, we demonstrate the higher-temperature surface and lower-temperature bulk phase transitions in CrSBr, a van der Waals (vdW) layered antiferromagnet. We leverage the surface sensitivity of electric dipole second harmonic generation (SHG) to resolve surface magnetism, the bulk nature of electric quadrupole SHG to probe bulk spin correlations, and their interference to capture the two magnetic domain states. Our density functional theory calculations show the suppression of ferromagnetic-antiferromagnetic competition at the surface is responsible for this enhanced surface magnetism. Our results not only show counterintuitive, richer phase transitions in vdW magnets, but also provide viable ways to enhance magnetism in their 2D form.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗