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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 955 records · Page 53

Precision pulse shape simulation for proton detection at the Nab experiment

The Nab experiment at Oak Ridge National Laboratory, USA, aims to measure the beta-antineutrino angular correlation following neutron β decay to an anticipated precision of approximately 0.1%. The proton momentum is reconstructed through proton time-of-flight measurements, and potential systematic biases in the timing reconstruction due to detector effects must be controlled at the nanosecond level. In conclusion, we present a thorough and detailed semiconductor and quasiparticle transport simulation effort to provide precise pulse shapes, and report on relevant systematic effects and potential measurement schemes.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Decay of a microsecond seniority 3 isomeric state in Hf 155

Excited states in the neutron-deficient nuclide Hf 155 have been investigated in experiments performed at the Accelerator Laboratory of the University of Jyväskylä. The Hf 155 nuclei were produced in fusion-evaporation reactions induced by beams of 295 and 315 MeV Ni 58 ions bombarding an isotopically enriched Pd 102 target and separated using the recoil mass separator MARA. An isomeric state having a half-life of 510(30) ns was discovered and is interpreted as a seniority υ = 3 , ( π h 11 / 2 2 ⊗ ν f 7 / 2 ) 27 / 2 − configuration. The γ -ray transitions emitted in the deexcitation of the isomeric state to the ground state were identified and a level scheme was constructed, from which the excitation energy of the isomer was determined to be 2581.5(10) keV. A B ( E 2 ) value of 0.45(3) W.u. was deduced for the 105.4 keV transition depopulating the isomeric state. The deduced level scheme and B ( E 2 ) value are compared with systematics and shell-model calculations. Published by the American Physical Society 2024

Physics↗

X-ray free electron laser studies of electron and phonon dynamics of graphene adsorbed on copper

Here, we report optical pumping and x-ray absorption spectroscopy experiments at the Pohang Accelerator Laboratory free electron laser that probes the electron dynamics of a graphene monolayer adsorbed on copper in the femtosecond regime. By analyzing the results with ab initio theory we infer that the excitation of graphene is dominated by indirect excitation from hot electron-hole pairs created in the copper by the optical laser pulse. However, once the excitation is created in graphene, its decay follows a similar path as in many previous studies of graphene adsorbed on semiconductors, i.e., rapid excitation of strongly coupled optical phonons and eventual thermalization. It is likely that the lifetime of the hot electron-hole pairs in copper governs the lifetime of the electronic excitation of the graphene.

36 MATERIALS SCIENCE↗

Hydrogen density mapping in biomolecular crystals through dynamic nuclear polarization

Many fundamental biological processes, including those in photosynthetic reaction centers and enzyme active sites, involve charge and energy transfer, bond cleavage, protonation and hydrogen bonding. Because H atoms play such central roles in these reactions, accurately determining their positions is essential. Yet, conventional X-ray crystallography primarily resolves the heavy atoms in biological structures and provides limited insight into hydrogen, even at atomic resolution. Neutron macromolecular crystallography (NMC) overcomes this limitation by offering exceptional sensitivity to hydrogen and deuterium. Here, we present a theoretical framework for the development of dynamic nuclear polarization NMC (DNP-NMC) techniques, which exploit the alignment of neutron and proton nuclear spins to enhance and tune the hydrogen signal contribution. The DNP-NMC approach advances the resolution of H atoms within biomolecular crystals, whether bound to protein residues or present in solvent. The method establishes key relationships for the coherent structure factor of polarized neutron scattering from hydrogenous matter. It theoretically achieves full accuracy in phase reconstruction and offers a path to improve neutron structure determination, achieving accuracies exceeding ≳80% by incorporating titration states. Using a variant of the hybrid input/output phase-retrieval algorithm, it allows recovery of the hydrogen density with ≳90% phase accuracy. In conclusion, we further discuss sources of experimental uncertainty for the upcoming DNP-enabled, quasi-Laue IMAGINE-X experiment at Oak Ridge National Laboratory's High Flux Isotope Reactor.

dynamic nuclear polarization↗

Cyber Framework for Steering and Measurements Collection Over Instrument-Computing Ecosystems

We propose a framework to develop cyber solutions to support the remote steering of science instruments and measurements collection over instrument-computing ecosystems. It is based on provisioning separate data and control connections at the network level, and developing software modules consisting of Python wrappers for instrument commands and Pyro server-client codes that make them available across the ecosystem network. We demonstrate automated measurement transfers and remote steering operations in a microscopy use case for materials research over an ecosystem of Nion microscopes and computing platforms connected over site networks. The proposed framework is currently under further refinement and being adopted to science workflows with automated remote experiments steering for autonomous chemistry laboratories and smart energy grid simulations.

Al Najjar, Anees↗

Synergistic Flow-Induced Oscillation of Multiple Cylinders in Harvesting Marine Hydrokinetic Energy

Abstract Flow-induced oscillations/vibrations (FIO/V) of cylinders in tandem can be enhanced by proper in-flow spacing to increase hydrokinetic energy harnessing. In a farm of multiple cylinders in tandem, the effect of interference on harnessing efficiency arises. Three years of systematic experiments in the Marine Renewable Laboratory (MRELab) of the University of Michigan, on an isolated cylinder, and two and three cylinders in tandem have revealed that synergistic FIO can enhance oscillations of cylinders in close proximity. Two cylinders in tandem can harness 2.5–13.5 times the hydrokinetic power of one isolated cylinder. Three cylinders in tandem can harness 3.4–26.4 times the hydrokinetic power of one isolated cylinder. Negative impact on the harnessed energy by multiple cylinders, such as the shielding effect for the downstream cylinder/s, is possible. Specifically for the three-cylinder configuration, at a certain flow speed, the decrease in the power of the middle cylinder can be overcome by adjusting its stiffness and/or damping.

Engineering↗

Fermilab Phoebus

The Fermilab Phoebus code contains FNAL site-specific code to customize the Control Systems Studio Phoebus application. Phoebus is a tool used to create and present graphical displays based on current real-time and historic values of sensors, gauges, alarms, and many other devices in accelerators and physics experiments here and at other laboratories around the world.

Velarde, Mariana González [Fermi National Accelera↗

Expanded Validation of Uranium Systems with the KENO Monte Carlo Codes and SCALE 6.2.4

The development of accident-tolerant fuel and advanced reactors fueled with high-assay low-enriched uranium has created an increased focus on systems with uranium enrichments between 5 and 20 wt % 235 U. SCALE criticality safety validation reports generated at Oak Ridge National Laboratory contain very few benchmark experiments in this range. The work presented herein is an initial investigation of expanded validation of the entire range of enrichments for uranium-fueled systems, including consideration of over 300 newly developed KENO models. The vast majority of the new models are between 4.4 wt % and 37.5 wt % enrichment and include a variety of thermal, intermediate, and mixed neutron spectra. This work finds no strong evidence of an enrichment-dependent bias, but there are indications of a spectrum-dependent bias. There are, however, only a limited number of independent experiments included at this time to distinguish intermediate enrichment effects from intermediate spectrum effects. Further work in this area is ongoing for intermediate enrichment systems. In the long run, the addition of these models to the Verified, Archived Library and Inputs and Data is planned, as funding and staff availability allow.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Nuclear Physics Network Requirements Review Report

The Energy Sciences Network (ESnet) is the Office of Science’s high-performance network user facility, delivering highly reliable data transport capabilities optimized for the requirements of data-intensive science. In essence, ESnet is the circulatory system that enables the U.S. Department of Energy (DOE) science mission by connecting each and every DOE lab and its user facilities. ESnet is funded and stewarded by the Advanced Scientific Computing Research (ASCR) Program and managed and operated by the Scientific Networking Division at Lawrence Berkeley National Laboratory (LBNL). ESnet is widely regarded as a global leader in the research and education networking community. ESnet connects DOE national laboratories, user facilities, and major experiments so scientists can use remote instruments and computing resources as well as share data with collaborators, transfer large data sets, and access distributed data repositories. While ESnet provides network connectivity, it cannot be characterized as an internet service provider as it is specifically built to provide a range of network services that are tailored to meet the unique requirements of DOE’s data-intensive science.

97 MATHEMATICS AND COMPUTING↗

Evaluation of the 2018 Version of the Integrated Surveillance Program Database Pressure Equation

The Integrated Surveillance Program (ISP) Database Pressure Equation was developed to determine with reasonable certainty the total maximum pressure of hydrogen and other gases in packaged 3013 containers stored at Savannah River Site (SRS) in support of the destructive evaluation (DE) process. The pressure equation in the Department of Energy (DOE) 3013 Standard, “Standard for Stabilization, Packaging and Storage of Plutonium- Bearing Materials” (DOE-STD-3013-2004) used a bounding assumption that all the water is decomposed to form hydrogen. However, the results of Los Alamos National Laboratory (LANL) shelf-life experiments showed that hydrogen is consumed, and that the maximum pressures would not approach the design pressure of the 3013 container. Therefore, the ISP Database Pressure Equation was revised in 2008 to include terms for the generation of helium and hydrogen as a function of time, as well as the consumption of water and destruction of hydrogen based on shelf-life results. The 2008 ISP Database Pressure Equation provided a more reasonable estimate of the total maximum pressure in packaged 3013 containers than the pressure equation in versions of the 3013 Standard issued prior to 2018.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Evaluation of Engineered Barrier Systems FY20 Report

This report describes research and development (R&D) activities conducted during fiscal year 2020 (FY20) specifically related to the Engineered Barrier System (EBS) R&D Work Package in the Spent Fuel and Waste Science and Technology (SFWST) Campaign supported by the United States (U.S.) Department of Energy (DOE). The R&D activities focus on understanding EBS component evolution and interactions within the EBS, as well as interactions between the host media and the EBS. A primary goal is to advance the development of process models that can be implemented directly within the Generic Disposal System Analysis (GDSA) platform or that can contribute to the safety case in some manner such as building confidence, providing further insight into the processes being modeled, establishing better constraints on barrier performance, etc. The FY20 EBS activities involved not only modeling and analysis work, but experimental work as well. Despite delays to some planned activities due to COVID-19 precautions, progress was made during FY20 in multiple research areas and documented in this report as follows: (1) EBS Task Force: Task 9/FEBEX Modeling Final Report: Thermo-Hydrological Modeling with PFLOTRAN, (2) preliminary sensitivity analysis for the FEBEX in-situ heater test, (3) cement-carbonate rock interaction under saturated conditions: from laboratory to modeling, (4) hydrothermal experiments, (5) progress on investigating the high temperature behavior of the uranyl-carbonate complexes, (6) in-situ and electrochemical work for model validation, (7) investigation of the impact of high temperature on EBS bentonite with THMC modeling, (8) sorption and diffusion experiments on bentonite, (9) chemical controls on montmorillonite structure and swelling pressure, (10) microscopic origins of coupled transport processes in bentonite, (11) understanding the THMC evolution of bentonite in FEBEX-DP—coupled THMC modeling, (12) modeling in support of HotBENT, an experiment studying the effects of high temperatures on clay buffers/near-field, and (13) high temperature heating and hydration column test on bentonite.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Pyrolysis Modeling of PMMA decomposition studied by TGA

Data from four TGA experiments conducted at Sandia National Laboratories was used for determination of a pyrolysis model using a commercial thermokinetics program developed by Netzsch Instruments (Kinetics NEO, version 2.1). The data measured at 1 K/min and the average of three measurements at 50 K/min were used as input into Kinetics NEO. The model was developed using data in the range 373 to 773 K. An initial estimate of the energy of activation (E) and pre-exponential constant (A) were determined from the model-free Friedman approach.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Nuclear Software Validation for 7% Enriched UO 2 Fuel Lattices

This analysis performs validation for the Virtual Environment for Reaction Application’s (VERA’s) neutronics codes MPACT and Shift against measured data from the Seven Percent Critical Experiment (7uPCX) at Sandia National Laboratory. The benchmarking supports the future application of VERA for analysis of high-assay low-enriched uranium (HALEU) fuel in commercial pressurized water reactors (PWRs). VERA demonstrates very good agreement with measured data, and the deterministic code MPACT also agrees very well with higher-fidelity stochastic methods KENO-VI and Shift in both total neutron flux and fission rate distribution comparisons. Despite some significant differences between the 7uPCX and existing commercial PWRs that challenge the neutron cross section data and transport solver methods used by MPACT, all of the results are excellent. The agreement increases the confidence in the applicability and accuracy of VERA for reactor analysis of HALEU fuels in commercial reactors.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Proposed Subcritical Assembly for Nuclear Criticality Safety Training at the Oak Ridge National Laboratory

The design of a new subcritical assembly at Oak Ridge National Laboratory (ORNL) has been finalized. This design takes the feasibility study of the subcritical assembly performed in August 2020 to an implementable design. This subcritical assembly will support the Nuclear Criticality Safety Program (NCSP) training and education program. The addition of this subcritical assembly into the NCSP training and education will enhance the program by providing backup capacity for training if nuclear facility operations are disrupted at Sandia National Laboratories or the National Criticality Experiments Research Center; providing a new location that is more accessible to students in the Eastern portion of the United States; providing flexibility to support students from a diverse background (e.g., university students, foreign nationals). The proposed subcritical assembly uses legacy AGN-201M research reactor fuel plates that are available at the Y-12 National Security Complex. The final design of this subcritical assembly contains approximately 617 grams of 235 U as UO 2 powder distributed homogeneously in polyethylene. The fuel plates will have a graphite neutron reflector to obtain a core multiplication, M, from 10 to 20, corresponding to a $k_{eff}$ of 0.90 to 0.95, respectively. The subcritical assembly will be able to support at least four experiments for the training courses: (1) the addition of fissile material to the core (mass), (2) a core separation experiment (interaction), (3) the addition of moderators to the core (moderation), and (4) the addition of neutron absorbers to the core (poison/absorption). The subcritical assembly will be designed to be inherently safe—subcritical under all normal and abnormal conditions— and will provide the capability to conduct hands-on training to support NCSP and general nuclear criticality safety staff training and qualification goals.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

"My Life To This Point"

This is intended as a presentation/talk that the author will be giving at Southern University, located in Baton Rouge, LA. He will be talking to mostly Freshman about his experiences at Los Alamos National Laboratory, his current job at LANL, his path to getting his job, and some future goals.

99 GENERAL AND MISCELLANEOUS↗

Investigation of Methane Generation Rates from Simulated and Radioactive Waste at Evaporator Conditions

Savannah River National Laboratory researchers have performed 9 experiments with simulated waste and 13 experiments with radioactive waste to determine methane generation rates (MGR) applicable to Savannah River Site waste at temperatures greater than or equal to 100 °C. Data from these experiments was used to generate temperature-dependent expressions to conservatively account for methane generation at elevated temperatures. Measured MGRs and the derived expressions are reported in units of standard cubic feet per hour per gallon of solution, where standard conditions are 25 °C and 1 atm.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Nuclear Physics Network Requirements Review (Final Report)

The Energy Sciences Network (ESnet) is the high-performance network user facility for the US Department of Energy (DOE) Office of Science (SC) and delivers highly reliable data transport capabilities optimized for the requirements of data-intensive science. In essence, ESnet is the circulatory system that enables the DOE science mission by connecting all its laboratories and facilities in the US and abroad. ESnet is funded and stewarded by the Advanced Scientific Computing Research (ASCR) program and managed and operated by the Scientific Networking Division at Lawrence Berkeley National Laboratory (LBNL). ESnet is widely regarded as a global leader in the research and education networking community. ESnet interconnects DOE national laboratories, user facilities, and major experiments so that scientists can use remote instruments and computing resources as well as share data with collaborators, transfer large datasets, and access distributed data repositories. ESnet is specifically built to provide Between July 2023 and October 2023, ESnet and the Nuclear Physics program (NP) of the DOE SC organized an ESnet requirements review of NP-supported activities. Preparation for these events included identification of key stakeholders: program and facility management, research groups, and technology providers. Each stakeholder group was asked to prepare formal case study documents about its relationship to the NP program to build a complete understanding of the current, near-term, and long-term status, expectations, and processes that will support the science going forward.

97 MATHEMATICS AND COMPUTING↗