A Fundamental and Feasibility Study of Ring- Vortex Gaseous-core Cavity Reactor Fifth Semiannual Report, 1 Feb. - 31 Jul. 1966
Feasibility study of ring-vortex gaseous-core cavity reactor
FLUID MECHANICS↗
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Recent research activities on high temperature pebble bed reactors at PSI - 18452
Recently, Paul Scherrer Institut (PSI) commenced a project on Feasibility and plausibility of innovative reactor concepts in an European electricity supply environment. The investigation in the project will be done on two reactor types: the pebble bed High-Temperature Gas-Cooled Reactor (HTGR) and Molten Salt Reactor (MSR) with the main focus being on the HTGR. Firstly, the project consists of an extensive literature study on the current status of the technology and research on the HTGR and MSR. Secondly, based on the findings from the literature survey, several topics of particular interest have been chosen for more thorough investigations. On the pebble bed HTGRs, the areas of investigation include risk assessment study, preliminary economic assessment, investigation of accident scenarios, and preliminary study on reduction of waste volumes. For both HTGR and MSR an analysis and optimization of the fuel cycle is foreseen. At the initial stage the equilibrium closed Th-U and U-Pu cycle performance will be evaluated and compared with 16 other reactor types. Later the knowledge from equilibrium study will be applied to optimize especially the MSR but also HTGR fuel cycle. At the end of the project, based on the literature survey and the results from the scoping studies, future research needs and areas of special interest will be identified for successive projects related to HTGR and MSR in PSI. (authors)
21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗
TEM Characterization of Nanostructured Grade 91 Neutron Irradiated to 6 DPA at 300 °C and 500 °C
Previously, samples of coarse grained (CG, grain diameter > 1 µm), ultra-fine grained (UFG, 1 µm> grain diameter> 100 nm), and nanocrystalline (NC, 100 nm> grain diameter) grade 91 steel were neutron irradiated in the Advanced Test Reactor (ATR) at Idaho National Laboratory (INL). Grade 91 is a ferritic/martensitic steel alloy with a nominal composition of Fe-9%Cr-1%Mo by weight, and it is being studied for applications in advanced nuclear reactor designs including as a fuel cladding material in gas cooled reactors. To assess the viability of this alloy for nuclear applications, the role of grain boundary size has not been sufficiently explored as a mechanism for developing radiation-tolerant materials. To achieve an UFG microstructure the material was processed using equal channel angular pressing (ECAP), and the NC microstructure was achieved through high pressure torsion (HPT). Such samples of various geometries for different types of characterization were irradiated to a dose of 6 displacements per atom (DPA) at separate temperature conditions of 300 °C and 500 °C. Thus, there were a total of 6 experimental conditions, three grain sizes (CG, UFG, and NC), each irradiated at two different temperature conditions (300 °C and 500 °C).
36 - MATERIALS SCIENCE↗
A study of fission product migration paths in irradiated TRISO particle SiC
Tristructural isotropic (TRISO) coated fuel particles used in high-temperature gas-cooled nuclear reactors (HTGRs) provide key advantages in terms of passive safety and reactor energy efficiencies. TRISO fuel consists of a number of special coating layers surrounding the fissile material in the kernel as shown in Fig. 1. The coating layers consist of a carbon buffer layer, inner pyrolytic carbon (PyC) layer, a silicon carbide (SiC) layer as well as an outer pyrolytic carbon layer. Together the layers act as a pressure vessel and barrier to the release of radioactive fission products into the reactor environment. The cubic 3C-SiC layer of thickness approximately 35 µm, acts as the primary barrier to the migration of metallic fission products out of the particle. The finding, more than three decades years ago, that silver can be released by intact TRISO particles has led to significant research to determine possible transport mechanisms of certain fission products in SiC. Out-of-reactor experiments did not reveal any significant lattice diffusion of silver in SiC1. Many earlier findings alternatively proposed a dominating role of fast diffusion paths such as grain boundaries and dislocations in enhancing fission product migration in SiC. Recently the role of the fission product palladium in enhancing the transport rate of silver in SiC2 was confirmed by transmission electron microscopy (TEM) of neutron-irradiated SiC from a TRISO coated particle from Compact 4-1-1, which was irradiated to an average burnup of 19.38% fissions per initial metal atom (FIMA); a time-averaged, volume-averaged temperature of 1072 °C; a time-averaged peak temperature of 1182 °C; and an average fast fluence of 4.13 x 1021 n/cm2 as part of the US Department of Energy's Advanced Gas Reactor (AGR)-1 experiment3. Although other studies found that Ag was found separately (without Pd) in TRISO coated particles irradiated at 11.4 %, 16.7 and 18.6% FIMA, Pd could have been present at lower than measureable concentrations4. In this study, SiC focussed ion beam (FIB) sections obtained from Compact 4-1-1 from the AGR-1 experiment were analysed in a double Cs-corrected JEOL ARM 200F using atomically resolved scanning transmission electron microscopy (STEM). By using atom resolved STEM in combination with electron energy loss spectroscopy (EELS) and large angle energy dispersive spectroscopy (EDS) a much better understanding of the migration routes and mechanisms of fission products in irradiated polycrystalline 3C-SiC was achieved.
11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
ART GCR Metals and High Temperature Design Methodology Overview
Overview presentation on high temperature metals and design methodology work for the ART Gas Cooled Reactor Program Review.
36 - MATERIALS SCIENCE↗
Assessment of multi-stage telescopic control rods in a pebble bed reactor. Part II: corrosion and wear performance
To support High-Temperature Gas-Cooled Reactor designs, the effects of corrosion and wear on a SS316L telescopic control rod prototype were investigated in helium at 775 °C with up to 5 ppm oxygen for durations up to 500 h. Three deployment conditions were tested to assess their impact on wear and oxide formation: severe cycles, daily cycles, and gravity-driven deployments. Here, a chromium-rich oxide layer developed on regions exposed to the helium flow, reaching up to 2 µm in the most affected areas. No carburization or decarburization was observed. Oxide breakthrough occurred mainly at grooves and contact points during severe cycling of the telescopic rod, while in the other tests it was limited to contact points. Friction forces increased due to oxide growth and thermal expansion, the latter being the dominant factor, but never enough to hinder rod deployment significantly. Coaxial misalignment of stages was identified as the main potential risk to reliable operation under normal conditions.
Control rod↗
ANL Design Team Analysis: Transportable Modular Reactor by Balance of Plant Elimination
HolosGen LLC is developing “Holos-Quad” a transportable gas-cooled reactor, with integral load following power conversion systems equipping subcritical power modules (SPMs), fully comprised within standard transport containers. The design eliminates the Balance of Plant (BoP) and greatly simplifies the design layout. A closed-loop full Brayton gas thermodynamic cycle converts the fuel cartridges thermal energy into electricity. This ARPA-E project utilizes advanced reactor modeling tools and manufacturing-testing of a scaled SPM equipped with a surrogate fuel cartridge to eliminate the most significant technology gaps to accelerate commercialization. The Argonne Design Team contributes to the research by demonstrating feasibility of various aspects of the Holos-Quad design by performing high-fidelity neutronic modeling, and investigating various reactivity control systems. This work consists of two main tasks: evaluation of HolosGen’s design features and alternative options study for reactivity control.
21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗
Gas-Liquid Two-Phase Flows Through Packed Bed Reactors in Microgravity
The simultaneous flow of gas and liquid through a fixed bed of particles occurs in many unit operations of interest to the designers of space-based as well as terrestrial equipment. Examples include separation columns, gas-liquid reactors, humidification, drying, extraction, and leaching. These operations are critical to a wide variety of industries such as petroleum, pharmaceutical, mining, biological, and chemical. NASA recognizes that similar operations will need to be performed in space and on planetary bodies such as Mars if we are to achieve our goals of human exploration and the development of space. The goal of this research is to understand how to apply our current understanding of two-phase fluid flow through fixed-bed reactors to zero- or partial-gravity environments. Previous experiments by NASA have shown that reactors designed to work on Earth do not necessarily function in a similar manner in space. Two experiments, the Water Processor Assembly and the Volatile Removal Assembly have encountered difficulties in predicting and controlling the distribution of the phases (a crucial element in the operation of this type of reactor) as well as the overall pressure drop.
Motil, Brian J.↗
Enhanced Gasification Reactor Design for Maximizing Gas-Particle Interaction
Explore the source record for details and available documents.
21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗
Effects of bypass flow and power change and deviation on performance of thermal mixing structure of HTR-PM - 18424
The temperature of bypass flow not flowing through the reactor core is obviously lower than that of the main coolant helium in a High Temperature Gas-cooled Reactor (HTGR). In addition, change and deviation of reactor power because of power regulation will introduce higher radial temperature difference of coolant helium from reactor to steam generator. In order to investigate the effects of bypass flow and power change and deviation on radial temperature difference of the helium flow entering the steam generator, model experiments and simulation calculations are proposed to evaluate the mixing performance of the thermal mixing structure at HTR-PM reactor core outlet. The experiments on Test Facility Hot Gas Mixing (TF-HGM) are carried out to observe the influences of bypass flow and reactor power deviation on mixing performance. In addition, some simulation calculations are conducted for the main mixing structure of the TF-HGM facility and the thermal mixing structure of HTR-PM. According to the results of experiments and simulation calculations, the maximum radial temperature difference at the outlet of the mixing structure fulfils the requirement by steam generator, less than 30 deg. C ({+-}15 deg. C), under all considered conditions. (authors)
21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗
Helium tribology of Inconel 617 subjected to laser peening for high temperature nuclear reactor applications
Inconel 617 is among the best candidates for utilization in high temperature gas cooled reactor tribo-components. However, the combined effects of sliding contact, along with intermittent idle times and very high temperature material degradation, deteriorates the alloy tribological performance, especially under a helium atmosphere. Laser peening is a surface treatment technique which can enhance the properties at the surface and subsurface by generating deep residual stresses and enhanced microstructure. In this work, we report the tribological behavior of regular laser peened as well as thermally-engineered laser peened Inconel 617 under helium and air atmospheres at 800 °C. In addition to friction and wear studies, the specimens are characterized by different analytical techniques to further understand the mechanisms involved in the peening process and sliding contact. Regardless of the peening process and post-process treatment types, it is observed that laser peening improves the tribological characteristics of Inconel 617. Interestingly, laser peening followed by helium thermal aging shows highly enhanced tribological behavior. This is attributed to the strengthening effect of the laser peening on the surface oxides providing an excellent and lasting protective and lubricating film under helium exposure.
42 ENGINEERING↗
HTGR Economic / Business Analysis and Trade Studies Market Analysis for HTGR Technologies and Applications
This report provides supplemental information to the assessment of target markets provided in Appendix A of the 2012 Next Generation Nuclear Plant (NGNP) Industry Alliance (NIA) business plan [NIA 2012] for deployment of High Temperature Gas-Cooled Reactors (HTGRs) in the 2025 – 2050 time frame. This report largely reiterates the [NIA 2012] assessment for potential deployment of 400 to 800 HTGR modules (100 to 200 HTGR plants with 4 reactor modules) in the 600-MWt class in North America by 2050 for electricity generation, co-generation of steam and electricity, oil sands operations, hydrogen production, and synthetic fuels production (e.g., coal to liquids). As the result of increased natural gas supply from hydraulic fracturing, the current and historically low prices of natural gas remain a significant barrier to deployment of HTGRs and other nuclear reactor concepts in the U.S. However, based on U.S. Department of Energy (DOE) Energy Information Agency (EIA) data, U.S. natural gas prices are expected to increase by the 2030 – 2040 timeframe when a significant number of HTGR modules could be deployed. An evaluation of more recent EIA 2013 data confirms the assumptions in [NIA 2012] of future natural gas prices in the range of approximately $7/MMBtu to $10/MMBtu during the 2030 – 2040 timeframe. Natural gas prices in this range will make HTGR energy prices competitive with natural gas, even in the absence of carbon-emissions penalties. Exhibit ES-1 presents the North American projections in each market segment including a characterization of the market penetration logic. Adjustments made to the 2012 data (and reflected in Exhibit ES-1) include normalization to the slightly larger 625MWt reactor module, segregation between steam cycle and more advanced (higher outlet temperature) modules, and characterization of U.S. synthetic fuel process applications as a separate market segment.
29 ENERGY PLANNING, POLICY, AND ECONOMY↗
Scaling and design analyses of a scaled-down, high-temperature test facility for experimental investigation of the initial stages of a VHTR air-ingress accident
Not Available
Arcilesi, Jr., David J. (ORCID:0000000245748149)↗
A Forward Feedback Control Scheme for a Solar Thermochemical Moving Bed Counter-Current Flow Reactor
Abstract Pelletized thermochemical energy storage media has a potential for long-duration energy storage. Production of solid-state energy storage media can be done within a cavity chemical reactor that captures concentrated solar radiation from a solar thermal field. The temperature stability of a solar reactor is directly influenced by the solar flux intercepted. This paper presents a low-order physical model to simulate the dynamic response of temperature inside a tubular plug-flow reactor prototype. Solid granular particles are fed to the reactor from the top whereas a counter-current flowing gas enters the reactor from the bottom. An in-house code was developed to model transient heat transfer of the reactor wall, gas, and moving particles. The model was preliminarily validated with packed beds for different temperature ranges and two gas flowrates. Dynamic response of the reactor temperature is simulated for different input power and gas/particle flowrates. The results show that the system response can be controlled efficiently by utilizing input power (solar flux) as a control parameter. A conventional proportional integral (PI) controller is designed to control the temperature inside the reactor and to maintain it during the solar flux intermittency. The controller parameters are tuned using the Ziegler–Nichols method to ensure optimal system response. The results show that the feedback control model is successful in tracking different reference reactor temperatures within a reasonable settling time of 30 min and eliminated overshoot. This study can be extended to include a hybrid reactor with a multi-input, multi-output variable system.
Energy & Fuels↗
Horizontal Split Table Conceptual Design for Advanced Reactor Validation
Oak Ridge National Laboratory and Lawrence Livermore National Laboratory are collaborating to develop a conceptual design for a horizontal split table for use in performing critical experiments. The goal of this design effort is to provide nuclear data testing and validation capabilities for advanced reactors such as pebble-bed high-temperature gas-cooled reactors, molten salt reactors, and heat pipe microreactor, but it could also be used for the current generation of reactors. The first concept being explored for the horizontal split table, a pebble-bed design based on the HTR-10 reactor, is described in this paper. A critical configuration corresponding to a footprint of about 4.5 m 2 was determined with SCALE/KENO-VI to fit the planned dimensions of the horizontal split table. The similarity of the pebble-bed design and the HTR-10 reactor application was assessed using SCALE/TSUNAMI, and a similarity coefficient $c_k$ of 0.9982 was obtained, proving that the concept will be useful for nuclear data validation and assimilation of pebble-bed type advanced reactors. In the proposed design, the materials with the highest $k_{eff}$ sensitivity are graphite and uranium, demonstrating that particular care must be given to carbon-related cross-section data. The effect of mechanical uncertainties between the fixed and moving tables was also assessed by calculating the reactivity change caused by vertical and horizontal gaps, as well as angular and torsion offsets between the two sides of the horizontal split table concept. The highest relative changes on the concept’s reactivity were caused by angular perturbations. The same analysis process is currently being used to create a molten salt advanced reactor type horizontal split table concept based on the Molten Salt Reactor Experiment (MSRE).
46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
Readiness Review of BWXT for Fabrication of AGR-5/6/7 TRISO Particles
INL readiness review assessment of BWXT readiness to commence fabrication of low-enriched TRISO coated fuel particles for the AGR-5/6/7 irradiation experiments. BWXT self-identified equipment issues preventing operation. INL identified two findings. The first was that disposition codes had not been assigned and documented on BWXT forms to ensure that off-specification materials could not be used in the fabrication of TRISO particles. The second was that chemical purity specifications were not reliably passed on to chemical suppliers, which resulted in the receipt of one acetylene cylinder with suspect impurity levels.
11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
AGR-3/4 Irradiation Test Train Disassembly and Component Metrology First Look Report
The AGR-3/4 experiment was designed to study fission product transport within graphitic matrix material and nuclear-grade graphite. To this end, this experiment consisted of 12 capsules, each fueled with 4 compacts containing UCO TRISO particles as driver fuel and 20 UCO designed-to-fail (DTF) fuel particles in each compact. The DTF fuel was fabricated with a thin pyrocarbon layer which was intended to fail during irradiation and provide a source of fission products. These fission products could then migrate through the compact and into the surrounding concentric rings of graphitic matrix material and/or nuclear graphite. Through post-irradiation examination (PIE) of the rings (including physical sampling and gamma scanning) fission product concentration profiles within the rings can be determined. These data can be used to elucidate fission product transport parameters (e.g. diffusion coefficients within the test materials) which will be used to inform and refine models of fission product transport. After irradiation in the Advanced Test Reactor (ATR) had been completed in April 2014, the AGR-3/4 experiment was shipped to the Hot Fuel Examination Facility (HFEF) at the Materials and Fuels Complex (MFC) for inspection, disassembly, and metrology. The AGR-3/4 test train was received at MFC in two separate shipments between February and April 2015. Visual examinations of the test train exterior did not indicate dimensional distortion, and only two small discolored areas were observed at the bottom of Capsules 8 and 9. No corresponding discoloration was found on the inside of these capsules, however. Prior to disassembly, the two test train sections were subject to analysis via the Precision Gamma Scanner (PGS), which did not indicate that any gross fuel relocation had occurred. A series of specialized tools (including clamps, cutters, and drills) had been designed and fabricated in order to carry out test train disassembly and recovery of capsule components (graphite rings and fuel compacts). This equipment performed well for separating each capsule in the test train and extracting the capsule components. Only a few problems were encountered. In one case, the outermost ring (the sink ring) was cracked during removal of the capsule through tubes. Although the sink ring will be analyzed in order to obtain a mass balance of fission products in the experiment, these cracks do not pose a major concern because the sink ring will not be analyzed in detail to obtain the spatial distribution of fission products. In Capsules 4 and 5, the compacts could not be removed from the inner rings. Strategies for removing the compacts are being evaluated. Sampling the inner rings with the compacts in-place is also an option. Dimensional measurements were made on the compacts, inner rings, outer rings, and sink rings. The diameters of all compacts decreased by 0.5 to 2.0 %. Generally, the extent of diametric shrinkage increased linearly with increasing neutron fluence. Most compact lengths also decreased. Compact lengths decreased with increasing fluence, reaching maximum shrinkage of about 0.9 % at a fast fluence of 4.0x10 25 n/m 2 E > 0.18 MeV. Above this fluence, the extent of length shrinkage appeared to decrease with fluence, and two compacts from Capsule 7 were found to have slightly increased in length (< 0.1 %) after a fluence of 5.2x10 25 n/m 2 .
21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗
AGR-3/4 Irradiation Test Train Disassembly and Component Metrology First Look Report
The AGR-3/4 experiment was designed to study fission product transport within graphitic matrix material and nuclear-grade graphite. To this end, this experiment consisted of 12 capsules, each fueled with 4 compacts containing UCO TRISO particles as driver fuel and 20 UCO designed-to-fail (DTF) fuel particles in each compact. The DTF fuel was fabricated with a thin pyrocarbon layer which was intended to fail during irradiation and provide a source of fission products. These fission products could then migrate through the compact and into the surrounding concentric rings of graphitic matrix material and/or nuclear graphite. Through post-irradiation examination (PIE) of the rings (including physical sampling and gamma scanning) fission product concentration profiles within the rings can be determined. These data can be used to elucidate fission product transport parameters (e.g. diffusion coefficients within the test materials) which will be used to inform and refine models of fission product transport. After irradiation in the Advanced Test Reactor (ATR) had been completed in April 2014, the AGR-3/4 experiment was shipped to the Hot Fuel Examination Facility (HFEF) at the Materials and Fuels Complex (MFC) for inspection, disassembly, and metrology. The AGR-3/4 test train was received at MFC in two separate shipments between February and April 2015. Visual examinations of the test train exterior did not indicate dimensional distortion, and only two small discolored areas were observed at the bottom of Capsules 8 and 9. No corresponding discoloration was found on the inside of these capsules, however. Prior to disassembly, the two test train sections were subject to analysis via the Precision Gamma Scanner (PGS), which did not indicate that any gross fuel relocation had occurred. A series of specialized tools (including clamps, cutters, and drills) had been designed and fabricated in order to carry out test train disassembly and recovery of capsule components (graphite rings and fuel compacts). This equipment performed well for separating each capsule in the test train and extracting the capsule components. Only a few problems were encountered. In one case, the outermost ring (the sink ring) was cracked during removal of the capsule through tubes. Although the sink ring will be analyzed in order to obtain a mass balance of fission products in the experiment, these cracks do not pose a major concern because the sink ring will not be analyzed in detail to obtain the spatial distribution of fission products. In Capsules 4 and 5, the compacts could not be removed from the inner rings. Strategies for removing the compacts are being evaluated. Sampling the inner rings with the compacts in-place is also an option. Dimensional measurements were made on the compacts, inner rings, outer rings, and sink rings. The diameters of all compacts decreased by 0.5 to 2.0 %. Generally, the extent of diametric shrinkage increased linearly with increasing neutron fluence. Most compact lengths also decreased. Compact lengths decreased with increasing fluence, reaching maximum shrinkage of about 0.9 % at a fast fluence of 4.0x1025 n/m2 E > 0.18 MeV. Above this fluence, the extent of length shrinkage appeared to decrease with fluence, and two compacts from Capsule 7 were found to have slightly increased in length (< 0.1 %) after a fluence of 5.2x1025 n/m2.
21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗