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At least 937 records · Page 52

Recent Progress in Understanding the Sun's Magnetic Dynamo

100 years ago we thought that the Sun and stars shone as a result of slow gravitational contraction over a few tens of millions of years - putting astronomers at odds with geologists who claimed that the Earth was much, much older. That mystery was solved in the 1920s and 30s with the discovery of nuclear energy (proving that the geologists had it right all along). Other scientific mysteries concerning the Sun have come and gone but three major mysteries remain: 1) How does the Sun produce sunspots with an 11-year cycle? 2) What produces the huge explosions that result in solar flares, prominence eruptions, and coronal mass ejections? and 3) Why is the Sun's outer atmosphere, the corona, so darned hot? Recent progress in solar astronomy reveals a single key to understanding all three of these mysteries.The 11-year time scale for the sunspot cycle indicates the presence of a magnetic dynamo within the Sun. For decades this dynamo was though to operate within the Sun's convection zone - the outmost 30% of the Sun where convective currents transport heat and advect magnetic lines of force. The two leading theories for the dynamo had very different models for the dynamics of the convection zone. Actual measurements of the dynamics using the techniques of helioseismology showed that both of these models had to be wrong some 20 years ago. A thin layer of strongly sheared flow at the base of the convection zone (now called the tachocline) was then taken to be the seat of the dynamo. Over the last 10 years it has become apparent that a weak meridional circulation within the convection zone also plays a key role in the dynamo. This meridional circulation has plasma rising up from the tachocline in the equatorial regions, spreading out toward the poles at a top speed of about 10-20 m/s at the surface, sinking back down to the tachocline in the polar regions, and then flowing back toward the equator at a top speed of about 1-2 m/s in the tachocline itself. Recent dynamo models that include this meridional flow now appear to have some power for predicting the size of future sunspot cycles.

Hathaway, David. H.↗

UV/IR symmetries of the S -matrix and RG flow

The low energy S-matrix which describes non-relativistic scattering arising from finite-range forces has UV/IR symmetries that are hidden in the corresponding effective field theory (EFT) action. Furthermore, it is shown that the S-matrix symmetries are manifest as geometric symmetries of the RG flow of coupling constants in the EFT action in both three and two spatial dimensions. An example is given demonstrating that UV/IR symmetry breaking in the S-matrix implies strong constraints on the RG flow of the coefficients of the corresponding symmetry-breaking operators in the EFT.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Characterizing how size distribution and concentration affect echogenicity of ultrasound contrast agents

Here, we investigated the effects of UCA gas bubble size distribution and concentration on the generated ultrasound echogenicity signal. Gas bubble size characterization using Coulter Counter and cryogenic-SEM revealed the hollow structure and rare presence of microbubbles >10 µm in a commercial UCA product, Lumason™. Volume-weighed size and concentration were observed to be more sensitive to changes in UCA bubble stability than number-weighted size and concentration. Size distribution measurements showed that the force (e.g., shaking/agitation energy) used to redisperse the sample did not affect the size distribution, concentration, or echogenicity of the UCA sample. The ultrasound backscattering coefficient (BSC) of size fractionated and serial diluted microbubbles showed that the echogenicity signal correlates most with UCA bubble concentration, especially volume-weighted concentration. Findings from this study may be used to support demonstrating the equivalence of a generic UCA product to the reference listed drug.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Centrifugal Nuclear Thermal Rocket Challenges and Potential

The Centrifugal Nuclear Thermal Rocket (CNTR) is a liquid fueled fission propulsion concept designed to heat propellant to 5000 K prior to expansion through a nozzle. A specific impulse up to 1800 s may be achieved using hydrogen propellant, and a specific impulse up to 1000 s may be achieved using more storable propellants such as methane, ammonia, or propane. The high uranium density of the liquid metallic uranium or liquid uranium carbide fuel will help enable compact engines suitable for missions such as fast (<15 month) round trip human Mars missions or high delta-V missions in cislunar space. Long term applications of the CNTR could include the advanced exploration and utilization of the solar system through direct use of in-situ volatiles as propellant. Challenges associated with the CNTR are numerous. Centrifugal force is used to retain the liquid fuel in rotating fuel cylinders, and rotational velocities up to 5000 rpm may be required. Propellant flow must be directed such that all structures and moderators in the core are adequately cooled prior to the propellant entering the liquid fuel and being heated to 5000 K. The rotating fuel cylinder wall (RFCW) must have an inner surface designed to be compatible with liquid uranium metal or uranium carbide fuel up to at least 1500 K, and that inner surface may also need to be textured to help maintain acceptable wall temperatures. Propellant must flow radially inward through the RFCW while fuel is simultaneously contained. The RFCW should ideal-ly be made from a material with low neutron absorption to help minimize engine mass and facilitate the use of High Assay Low Enriched Uranium (HALEU) fuel in the system. The drive system for the rotating fuel cylinders must support all phases of operation. This paper will discuss computational and experimental research being conducted to address some of the challenges associated with the CNTR, and will also note potential mission benefits from the CNTR.

Michael G. Houts↗

Proposal for gravitational direct detection of dark matter

The only coupling dark matter is guaranteed to have with the standard model is through gravity. Here we propose a concept for direct dark matter detection using only this gravitational coupling. We suggest that an array of quantum-limited mechanical impulse sensors may be capable of detecting the correlated gravitational force created by a passing dark matter particle. We consider the effects of irreducible noise from couplings of the sensors to the environment and noise due to the quantum measurement process. We show that the signal from Planck-scale dark matter is in principle detectable using a large number of gram-scale sensors in a meter-scale array with sufficiently low quantum noise, and discuss some experimental challenges en route to achieving this target.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Global Sensitivity Analysis of Bulk Properties of an Atomic Nucleus

We perform a global sensitivity analysis of the binding energy and the charge radius of the nucleus 16 O to identify the most influential low-energy constants in the next-to-next-to-leading order chiral Hamiltonian with two- and three-nucleon forces. For this purpose, we develop a subspace-projected coupled-cluster method using eigenvector continuation [Frame D. et al., Phys. Rev. Lett. 121, 032501 (2018)]. With this method, we compute the binding energy and charge radius of 16 O at more than 106 different values of the 16 low-energy constants in one hour on a standard laptop computer. For relatively small subspace projections, the root-mean-square error is about 1% compared to full-space coupled-cluster results. We find that 58(1)% of the variance in energy can be apportioned to a single contact term in the 3 S 1 wave, whereas the radius depends sensitively on several low-energy constants and their higher-order correlations. The results identify the most important parameters for describing nuclear saturation and help prioritize efforts for uncertainty reduction of theoretical predictions. The achieved acceleration opens up an array of computational statistics analyses of the underlying description of the strong nuclear interaction in nuclei across the Segrè chart.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Multi-Physics System-level Simulations of a Generic Pebble Bed High-Temperature Gas Cooled Reactor with Coupled SAM/Griffin Model

A SAM model for a 200 MWth generic pebble bed high-temperature gas-cooled reactor (PBHTGR) is presented in this work. As an extension to the modeling effort from FY-22 (Ooi et al. (2022)), an improved core channel approach is used to model the pebble bed of the reactor. The improvement greatly simplifies the model and reduces the run time of the model. Furthermore, the SAM model is coupled to the Griffin reactor physics model from Stewart et al. (2021) using the MOOSE MultiApp system where neutronics calculations are performed by the Griffin model and thermal hydraulics calculations by the SAM model. Favorable predictions are produced by the SAM/Griffin coupled model for steady-state normal operating condition. A load-following transient is also simulated with the coupled model where the neutronics and thermal hydraulics responses of the core are predicted correctly by the model. A protected Pressurized Loss of Forced Cooling (PLOFC) accident is simulated with the SAM model, in which the reactor power is determined using the decay heat curve, and therefore the Griffin model is not needed and thus decoupled. A simplified RCCS (Reactor Cavity Cooling System) loop is added to the model to remove decay heat from the core during the transient. Qualitatively, the prediction by the SAM model matches the expected behavior of a PB-HTGR during a PLOFC accident.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Calculation of Spent Fuel Pool Time-to-Boil using Polaris/ORIGAMI [Slides]

The goal of this experiment was to calculate time-to-boil (TTB) for a Spent Fuel Pool (SFP). TTB is important for SFP management that represents the amount of time available to address loss of forced cooling. Researchers calculated and compared TTB for two cases using SCALE: SFP containing representative LEU fuel (≤ 5 wt %) and SFP containing representative LEU+ fuel (5 – 8 wt %). There were approximately 2300 fuel assemblies in the SFP for each case. Researchers concluded that the impact of LEU+ core on time-to-boil is very small. At such low cooling times, the impact of increased decay heat is not significant. Decay heat of SFP assemblies is small compared to discharge core decay heat.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Remote Handled Hot Cell Facility and Other Research Transuranic Waste (Debris)

This acceptable knowledge (AK) Summary Report has been prepared for the Central Characterization Program (CCP) for remote-handled (RH) transuranic (TRU) waste generated and managed by Sandia National Laboratories/New Mexico (SNL/NM) in Albuquerque, New Mexico. The waste described in this report was predominately generated in the SNL/NM Hot Cell Facility (HCF) during the removal and packaging of experimental material and decontamination operations in Building 6580 at Technical Area (TA)-V. The waste stream also includes a very small amount of waste (estimated at less than 1 gram of fuel similar to that used for research at the HCF) originating from classified research at TA-I. In addition, the waste also includes secondary waste termed by SNL/NM as process generated waste (PGW), created during repackaging operations for this waste at the Auxiliary Hot Cell Facility (AHCF). The waste has been stored at the Sandia Pulsed Reactor (SPR) Dense Pack Storage Facility within TA-V or the Manzano Bunkers located at Manzano Base within Kirtland Air Force Base. All of the waste is being repackaged at the AHCF. This report was prepared in accordance with CCP-TP-005, CCP Acceptable Knowledge Documentation (Reference 1), to implement the AK requirements of DOE/WIPP-02-3214, Remote-Handled TRU Waste Characterization Program Implementation Plan (WCPIP) (Reference 2); Waste Isolation Pilot Plant Hazardous Waste Facility Permit, Waste Analysis Plan (WIPP-WAP) (Reference 3); and DOE/WIPP-02-3122, Transuranic Waste Acceptance Criteria for the Waste Isolation Pilot Plant (WIPP-WAC) (Reference 4).

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Thermomechanical Processing of Uranium Alloys with 10 and 50 Weight Percent Zirconium

This work focuses on casting and thermomechanical processing for moderate sized (500-1000g) 10% by weight and 50% by weight uranium-zirconium alloys. Three castings of uranium – 10wt% zirconium and a fourth casting of uranium – 50wt% zirconium were completed using different castings processes. The first casting process relied on only induction mixing within the VIM system thereby eliminating the need for an arc-melting feedstock preparation step. The second casting process used the arc-melting process prior for feedstock to the same VIM system. In this study, the induction mixing process alone with a graphite crucible appears insufficient for the fabrication of UZr alloys. Graphite is suitable with the use of master alloy UZr feedstock produced by arc-melting. There was a moderate increase of approximately 100 ppm of carbon within the U10Zr alloys. However, there was a near 1000 ppm increase of carbon in the U50Zr alloy. This carbon content is considered too high for forming processes, and therefore, warrants the use of a ceramic crucible for UZr castings near 50wt% zirconium. Zirconia does not appear suitable for UZr castings near 50wt% zirconium. The use of Beryllia or Thoria may be a more suitable option. However, due to the significantly lower liquidus and lower zirconium content, Zirconia crucibles do appear viable for carbon reduction in the U10Zr system. Two thermomechanical processes are also studied in this work - hot extrusion of the U50Zr system and heat treatment in an argon atmosphere. This work demonstrated that extrusion of the U50Zr alloy near 680°C is a viable choice even with +1000 ppm carbon. Extrusion of the U50Zr system near 630°C was unsuccessful and does not appear viable unless significant force and tooling strength is available. There appears to be a moderate increase in extrudate hardness when compared to as-cast. Heat-treatment reduced the hardness of as-cast alloys in the U10Zr castings as well as resolve some variance in the microstructures. However, for the U50Zr billet that did not successfully extrude at 630°C, heat treatment at 900°C for 96 hours did not have a significant impact on hardness or microstructure.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Full-Scale Implementation of Propane Biosparge System for In-Situ Remediation of 1,4-Dioxane - 20174

1,4-Dioxane is a common co-contaminant with chlorinated solvents but is not readily remediated via similar treatment approaches (e.g., sorption, reductive dechlorination). However, 1,4-dioxane can be cometabolically biodegraded in the presence of alkane gases and oxygen. At Vandenberg Air Force Base in California, USA, historical use of chlorinated solvents resulted in 1,4-dioxane in groundwater across three vertical groundwater zones. Between April 2013 and December 2016, laboratory testing and various field demonstrations were conducted by us, and others. The results from these tests showed in-situ propane biosparging as a promising technology for reduction of both chlorinated solvent and 1,4-dioxane concentrations, with up to 99 percent reduction in groundwater concentrations. Stable isotope probing (SIP) was also used in 2015 to verify that biodegradation was a (destructive) mechanism occurring in the subsurface.). The success of the propane biosparge demonstrations, and confirmation of the biodegradation mechanism via SIP, has led to the full-scale implementation of a propane biosparge treatment system at Site 24 at Vandenberg Air Force Base. The treatment area is a relatively small footprint (e.g., less than 61 meters (200 feet) long), with 83 new wells installed simultaneously across the three groundwater zones. Ultimately 93 wells will be connected to an above-ground treatment system the includes an air compressor, a propane tank, controls to ensure safe operating conditions, and nutrient amendment elements. This full-scale system is currently known to be among the first of its kind. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Changes of deformed shell gaps at N ~ 100 in light rare-earth, neutron-rich nuclei

There have been compelling evidences indicating that deformed single-particle states in neutron- rich regions are different from those in the stable region. It was pointed out that for the light rare- earth (60Nd, 62Sm, and 64Gd), neutron-rich (N = 98-102) nuclei, the Woods-Saxon potential, the Nilsson modified oscillator potential with "universal" parameters, and the folded Yukawa potential all failed to describe the correct ordering of neutron single-particle states. The location and size of deformed shell gaps in this mass region are under current debate. We propose a modification for the "standard" Nilsson parameters of Bengtsson and Ragnarsson introduced in 1985. The proposed N-dependent spin-orbit interaction brings an effect of the tensor force for the deformed potential, which causes dynamic changes in deformed shell gaps with neutron number and deformation. By applying the modified Nilsson parameters to generate deformed bases for the Projected Shell Model, we demonstrate that the calculation can explain consistently the current experimental data, including the ground state configuration in odd-neutron nuclei, upbending of the yrast moment of inertia at higher spins and the energies of 2-quasineutron 6- and 4- isomers in even-even nuclei.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Compositing and Characterization of SE Quadrant Waste Exemplars

This report outlines the experimental investigation and characterization of transport properties in Hanford SE quadrant High-Level Waste (HLW). The goal of the study was to establish baseline behaviors of bulk composite rheology and settling characteristics to facilitate waste treatment process design for the Waste Treatment and Immobilization Plant (WTP) and avoid waste conditions and properties favorable to bubble cascade gas release events. The study focused on two major objectives: 1) identifying, obtaining, and preparing relevant Hanford tank waste samples for evaluation and 2) quantifying the “as-received” rheology and transport properties of the samples. Twenty-three centrifuged core segments originating from tanks AN-101, AN-106, and AW-105 were selected based on compositional relevance to SE quadrant PUREX cladding waste. These materials were composited into five waste composites enriched with target analytes: aluminum (Al), iron (Fe), phosphate (PO 4 ), uranium (U), and zirconium (Zr). Physical property and transport testing examined particle size distributions, bulk densities, settling behaviors, rheological properties, shear strengths, and just-suspended mixing speeds (NJS). Testing revealed two distinct composite classifications based on rheological characteristics: non-Newtonian composites (Fe and PO 4 ) and Newtonian composites (Al, U, and Zr). The Fe and PO 4 composites exhibited slow settling rates and reduced mobilization proclivity, attributable to strong particle-particle interactions and the formation of yield structures within non-Newtonian slurries. In contrast, the Al, U, and Zr composites displayed rapid settling and dense compaction behaviors, indicative of minimal structuring and interactions. Shear strengths for all composites were generally low relative to prior studies of SE quadrant waste, with only the U composite showing elevated strength approaching values reported in previous literature. Repeat shear strength measurements revealed contributions from dense granular material in the U composite and stronger cohesive properties in the Al composite. Settling data highlighted hindered settling behavior, with rates falling more than one order of magnitude below estimates based on Stokes’ law and rate decreasing as composite UDS content increased. NJS testing demonstrated different mobilization behaviors between cohesive and granular composites. The Fe composite required the highest mixing rate for resuspension, while the Al composite was the easiest to resuspend. Comparison of measured NJS against predictions made using the Zwietering correlation suggests non-Newtonian behavior alters resuspension mechanics, rendering non-Newtonian systems more stable against resuspension lift forces relative to their granular counterparts.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

IM3 Data Center Driven Grid Stress Dataset for the U.S. Western Interconnection

This dataset provides projected grid stress and reliability results (including all model inputs and outputs from an open-source grid operations modeling framework - GO), for the Integrated Multisector, Multiscale Modeling (IM3) project, under varying levels of data center demand growth between 2025 and 2035 in the U.S. Western Interconnection. The scenarios and sensitivity experiments are combinations of different data center demand growth rates and energy, weather, population and economic pathways. Data center demand growth projections were sourced from the Electric Power Research Institute (EPRI). The data center demand growth projection names are: Low (3.71% annual data center demand growth) Moderate (5% annual data center demand growth) High (10% annual data center demand growth) Higher (15% annual data center demand growth) Energy, weather, population and economic pathways are informed by two Shared Socioeconomic Pathways (SSP3 and SSP5) and two Representative Concentration Pathways (RCP4.5 and RCP8.5) following the hotter general circulation model (GCM) forcing group from a set of perturbed thermodynamics simulations. The resulting pathway names are: rcp45hotter_ssp3 rcp45hotter_ssp5 rcp85hotter_ssp3 rcp85hotter_ssp5 The main scenarios and sensitivity experiments are detailed below. Reference scenario: The projected grid stress and reliability results for the U.S. Western Interconnection from a previous study. This scenario does not consider data center demand growth explicitly. Data center scenario: Building on the reference scenario, this scenario considers various data center growth rates and how they impact the U.S. Western Interconnection. Data center loads are modeled as flat 8760-hr profiles. This scenario does not consider new generation and transmission capacities specifically designed to meet the new data center demands. The related folder is named "flat". Delayed generator retirements sensitivity experiment: Building on the data center scenario, this experiment explores the impact of different levels of natural gas and nuclear generator retirement delays. The resulting scenario names are: (1) postponing 100% nuclear retirements; (2) postponing 100% nuclear and 25% natural gas retirements; (3) postponing only 50% natural gas retirements; (4) postponing 100% nuclear and 50% natural gas retirements; (5) postponing 100% nuclear and 75% natural gas retirements; and (6) postponing 100% nuclear and 100% natural gas retirements. The related folder names are: no_gen_retire_0_gas, no_gen_retire_25_gas, no_gen_retire_50_gas, no_gen_retire_50_gas_only, no_gen_retire_75_gas, and no_gen_retire_100_gas. Demand response through curtailment sensitivity experiment: Building on the data center scenario, this experiment explores the impact of different participation and compensation levels of data center demand response. The resulting scenario names are: (1) 5% demand available for curtailment with 750 $/MWh compensation; (2) 5% demand available for curtailment with 500 $/MWh compensation; (3) 5% demand available for curtailment with 250 $/MWh compensation; (4) 15% demand available for curtailment with 750 $/MWh compensation; (5) 15% demand available for curtailment with 500 $/MWh compensation; and (6) 15% demand available for curtailment with 250 $/MWh compensation. The related folder names are: dr_cost_250_drup_0_drdown_5, dr_cost_250_drup_0_drdown_15, dr_cost_500_drup_0_drdown_5, dr_cost_500_drup_0_drdown_15, dr_cost_750_drup_0_drdown_5, and dr_cost_750_drup_0_drdown_15. Combination of delayed generator retirements and demand response through curtailment sensitivity experiment: The impact of combining postponing 100% nuclear and 25% natural gas retirements with 5% demand available for curtailment with 750 $/MWh compensation is simulated. The related folder is named "dr_cost_750_drup_0_drdown_5_nuc_100_gas_25". Please refer to the README file for a detailed description of the dataset including individual files and references.

Artificial Intelligence↗

Accurate ab initio Quartic Force Fields of Cyclic and Bent HC2N Isomers

Highly correlated ab initio quartic force field (QFFs) are used to calculate the equilibrium structures and predict the spectroscopic parameters of three HC2N isomers. Specifically, the ground state quasilinear triplet and the lowest cyclic and bent singlet isomers are included in the present study. Extensive treatment of correlation effects were included using the singles and doubles coupled-cluster method that includes a perturbational estimate of the effects of connected triple excitations, denoted CCSD(T). Dunning s correlation-consistent basis sets cc-pVXZ, X=3,4,5, were used, and a three-point formula for extrapolation to the one-particle basis set limit was used. Core-correlation and scalar relativistic corrections were also included to yield highly accurate QFFs. The QFFs were used together with second-order perturbation theory (with proper treatment of Fermi resonances) and variational methods to solve the nuclear Schr dinger equation. The quasilinear nature of the triplet isomer is problematic, and it is concluded that a QFF is not adequate to describe properly all of the fundamental vibrational frequencies and spectroscopic constants (though some constants not dependent on the bending motion are well reproduced by perturbation theory). On the other hand, this procedure (a QFF together with either perturbation theory or variational methods) leads to highly accurate fundamental vibrational frequencies and spectroscopic constants for the cyclic and bent singlet isomers of HC2N. All three isomers possess significant dipole moments, 3.05D, 3.06D, and 1.71D, for the quasilinear triplet, the cyclic singlet, and the bent singlet isomers, respectively. It is concluded that the spectroscopic constants determined for the cyclic and bent singlet isomers are the most accurate available, and it is hoped that these will be useful in the interpretation of high-resolution astronomical observations or laboratory experiments.

Inostroza, Natalia↗

High Elevation Radiation Array (HERA) detectors for airborne thunderstorm investigations

A high-energy atmospheric physics phenomenon, referred to as a terrestrial gamma ray flash (TGF), is associated with lightning and produces large bursts of energetic photon radiation. TGFs will be investigated using a suite of gamma-ray instruments designed and constructed to fly on ten United States Air Force (USAF) WC-130J Hurricane Hunter aircraft as part of an aircrew ionization study led by the Air Force Institute of Technology (AFIT) and the United States Air Force School of Aerospace Medicine (USAFSAM), in cooperation with the 53rd Weather Reconnaissance Squadron (WRS). Each instrument consists of one NaI and one plastic detector, a GPS timing device, and an instrument computer that performs data acquisition. High Elevation Radiation Array (HERA) detectors will be employed to maximize the chances of observing TGFs near their source and to gain a better understanding of their origin, mechanism, ubiquity, and to assess potential hazards posed to military and commercial aircrew and passengers. The HERA program, deployed on 10 separate Air Force aircraft over a multi-year campaign, will result in thousands of observational flight hours and be the largest concerted effort to date to observe TGFs in situ through aircraft observations. In this paper, we give an overview of the scientific goals of this campaign and how the HERA instruments have been designed to meet those goals. Here, we include a detailed description of the HERA instrument, along with mass model and signal processing simulations.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Final Design for Thermal/Epithermal eXperiments (TEX) with Chloride Absorbers to Provide Validation Benchmarks for Y-12 Electrorefining Facility

Uranium electrorefining operations at Y-12 require validation for chlorine absorption and reflection. Plutonium chloride solution operations at Los Alamos National Laboratory require chlorine absorption validation. The growing need for chlorine validation is evident to the wider criticality safety community, with multiple attendees at the recent TEX 2.0 meeting at Lawrence Livermore National Laboratory (May 2023) requesting validation for chlorine (Idaho National Laboratory (INL), Institute de radioprotection et de surete nucleaire (IRSN), Savannah River Nuclear Site (SRNS), LANL, and Y-12). Los Alamos National Laboratory has recently performed, and benchmarked, an experiment titled Chlorine Worth Study (CWS) for the internal operations at the lab, but due to the difficulties in precisely characterizing the material compositions of the chlorine absorbers it is advantageous to perform a complimentary study with a different chlorine-based absorber material. Furthermore, having a uranium-based vs plutonium-based experiment provides a separate and important validation basis for criticality safety and nuclear data evaluation. The original final design report for the study of chlorine absorption using the TEX-HEU experimental base was presented in 2022, but used the same chlorine-bearing materials that were found to be difficult to characterize in the LANL benchmark. A complete redesign of the experiment has been performed looking at alternative absorber materials in various forms to produce an experiment that is fully characterizable. This report presents five novel chlorine experiments using the TEX-HEU test bed which provides direct comparison to the Y-12 and INL/Terrapower application needs, utilizing sodium chloride (NaCl) absorber plates. The absorber plates will consist of granulated NaCl (≥99.5% pure), which will be fully encapsulated in aluminum tins, providing a simple but effective chlorine-based absorber material that can be completely characterized. Of the five configurations presented in this report, it is expected that two or three configurations will be down selected for the actual experiment, with the other configurations being alternates. Three of the configurations are in the standard configuration, where the absorber is placed directly on the HEU fuel plates, and two in the sandwich configuration, where the absorber is surrounded by polyethylene moderators to force additional neutron thermalization prior to reaching the absorber. There are two thicknesses of NaCl absorber plates: 3/16” and 1/4” active thicknesses (i.e. not including the encapsulation). Both variations of the absorbers have an active absorber radius of 6” and a total radius of 7.5” to match the diameter of the HEU plates, with the outer 1.5” being aluminum encapsulation. The high-density polyethylene (HDPE) moderators are of the thicknesses: 27/16”, 7/4”, 1/8”, 11/16”, and 3/4”. The final configurations have six (one sandwich and one standard configuration), eight (one sandwich and one standard configuration), and 18 total fuel layers (standard configuration). The standard and sandwich configurations were designed such that the differences in moderator thicknesses are 1” HDPE, which were already procured for the original CED-2. The proposed configurations were precisely tuned to closely match the sensitivity profiles and neutron spectra of the Y-12 upset cases and were also compared to the INL/Terrapower upset cases. The assessment of experimental uncertainties of the non-absorber components was predicted to be 0.00114 Δk eff . The assessment of uncertainties resulting from the absorbers was predicted to be 0.00029 Δk eff . This results in a total uncertainty of 0.00118 Δk eff . Many of the largest uncertainties, namely the moderator densities, may be reduced with precision dimensional inspection of the components. The 1” HDPE moderators as well as the HDPE reflectors from the original CED-2 were incorporated in the final designs presented here. Additional HDPE moderator plates must be fabricated to complete the configurations. NaCl absorber plates will by fabricated at LLNL. The total additional cost is expected to be $\$$54,250 for the remaining components. Precise inspection, including dimensional, mass, density, and impurity, is recommended for all components. LLNL estimates that these costs are around $\$$12,000. It is expected, based on previous TEX-HEU experiments, that three weeks of experimental facility time is needed to complete the experiments.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Implementation issues for a compact 6 degree of freedom force reflecting handcontroller with cueing of modes

Teleoperated control requires a master human interface device that can provide haptic input and output which reflect the responses of a slave robotic system. The effort reported in this paper addresses the design and prototyping of a six degree-of-freedom (DOF) Cartesian coordinate hand controller for this purpose. The device design recommended is an XYZ stage attached to a three-roll wrist which positions a flight-type handgrip. Six degrees of freedom are transduced and control brushless DC motor servo electronics similar in design to those used in computer controlled robotic manipulators. This general approach supports scaled force, velocity, and position feedback to aid an operator in achieving telepresence. The generality of the device and control system characteristics allow the use of inverse dynamics robotic control methodology to project slave robot system forces and inertias to the operator (in scaled form) and at the same time to reduce the apparent inertia of the robotic handcontroller itself. The current control design, which is not multiple fault tolerant, can be extended to make flight control or space use possible. The proposed handcontroller will have advantages in space-based applications where an operator must control several robot arms in a simultaneous and coordinated fashion. It will also have applications in intravehicular activities (within the Space Station) such as microgravity experiments in metallurgy and biological experiments that require isolation from the astronauts' environment. For ground applications, the handcontroller will be useful in underwater activities where the generality of the proposed handcontroller becomes an asset for operation of many different manipulator types. Also applications will emerge in the Military, Construction, and Maintenance/Manufacturing areas including ordnance handling, mine removal, NBC (Nuclear, Chemical, Biological) operations, control of vehicles, and operating strength and agility enhanced machines. Future avionics applications including advanced helicopter and aircraft control may also become important.

Jacobus, Heidi↗